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A quasi-two level analytic model for end pumped alkali metal vapor laser 端抽运碱金属蒸汽激光器的准二能级解析模型
Pub Date : 2008-05-12 DOI: 10.1117/12.782875
G. Hager, J. McIver, D. Hostutler, G. Pitz, G. Perram
In this paper we describe a quasi-two level analytic model for end pumped Alkali metal vapor lasers. The model is developed by considering the steady state rate equations for the number densities of the, 2S1/2, 2P3/2, and 2P1/2, energy states for the three level laser system. The approximation is then made that the relaxation between the two upper levels, 2P3/2 and 2P1/2, caused by collisions with additive ethane is much faster, in fact infinitely fast, by comparison with any other process in the system including stimulated emission. With this assumption the ratio of the number densities for the upper two levels, 2P3/2 and 2P1/2, is given by its statistical equilibrium value and the mathematical description becomes that of a quasi-two level system from which an analytic solution can be extracted. The analytic model description gives expressions for the threshold pump power and the slope efficiency including intra-cavity losses. Applications of the model and comparisons with the steady state three level model developed by Beach et al. will be presented.
本文描述了端泵浦碱金属蒸汽激光器的准二能级解析模型。考虑了三能级激光系统2S1/2、2P3/2和2P1/2能级的稳态速率方程,建立了该模型。与系统中任何其他过程(包括受激辐射)相比,由附加乙烷碰撞引起的两个上能级(2P3/2和2P1/2)之间的弛豫要快得多,实际上是无限快。在此假设下,上两层2P3/2和2P1/2的数密度之比由其统计平衡值给出,其数学描述成为准两层系统的数学描述,并可从中提取解析解。解析模型给出了泵浦阈值功率和含腔内损耗的斜率效率的表达式。将介绍该模型的应用以及与Beach等人开发的稳态三能级模型的比较。
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引用次数: 12
Conical nozzles for pulsed laser propulsion 脉冲激光推进用锥形喷嘴
Pub Date : 2008-05-12 DOI: 10.1117/12.782430
J. Sinko, N. Dhote, J. Lassiter, D. Gregory
A CO2 laser of 300 ns pulse length, operating at 10.6 μm wavelength and from 1-4 J pulse energy was used to ablate carbon-doped Delrin® (polyoxymethylene, or POM) targets in a set of conical aluminum minithrusters at standard temperature and pressure. Nozzles with lengths ranging from 0.5 - 5 cm were used (corresponding to expansion ratios of about 4 to 16), as well as a bare sample with no nozzle. A piezoelectric force sensor was used to record the imparted impulse for fluences in the range of 1-100 J/cm2 for each thruster. The effect of increasing the expansion ratio on the impulse generation for single pulse laser propulsion experiments will be described. The study will also clarify the effect of confining air from an ambient atmosphere in augmenting impulse generation.
在标准温度和压力下,利用脉冲长度为300 ns、波长为10.6 μm、脉冲能量为1 ~ 4j的CO2激光,烧蚀了锥形铝微型推力器中掺杂碳的Delrin®(polyoxymethylene, POM)靶材。使用长度为0.5 - 5cm的喷嘴(对应于膨胀比约为4至16),以及没有喷嘴的裸样品。利用压电力传感器记录每个推力器在1-100 J/cm2范围内的影响所传递的脉冲。讨论了增大膨胀比对单脉冲激光推进实验脉冲产生的影响。该研究还将阐明从环境大气中限制空气对增加脉冲产生的影响。
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引用次数: 14
Investigations of the ultrafast laser induced melt dynamics by means of transient quantitative phase microscopy (TQPm) 用瞬态定量相显微镜(TQPm)研究超快激光诱导熔体动力学
Pub Date : 2008-05-12 DOI: 10.1117/12.782618
I. Mingareev, A. Horn
Modifications of bulk aluminum irradiated well above ablation threshold (F < 300 J.cm-2) have been investigated in situ by means of shadowgraphy and transient quantitative phase microscopy (TQPm) using ultrafast laser radiation (tp=80 fs, λ=800 nm). This novel pump-probe technique enables quantitative time-resolved measurements of object's properties, e.g. dimensions of melt droplets and layer thickness or transient refractive index changes. A series of time-resolved phase images of vaporized material and/or melt, which are induced by n=1..8 pulses on an aluminum target, are obtained using TQPm. Dynamics and characteristics of melting, dependence of the ablated material volume on process parameters and thereby induced structural modifications have been studied. An increase of material ejection rate is observed at delay time of approximately τ=300 ns and τ>800 ns after the incident pulse. Transient refractive index modifications have been investigated in technical glass (Schott D263) by means of TQPm. By using high-repetition rate ultra-short pulsed laser radiation (tp=400 fs, λ=1045 nm, frep=1 MHz) focused by a microscope objective (w0 ≈ 4 μm) heat accumulation and thereby glass melting as well as welding is enabled. Transient optical phase variation has been measured up to τ=2.1 μs after the incident pulse and can be attributed to the generation of free charge carriers and compression forces inside glass.
利用超快激光(tp=80 fs, λ=800 nm),利用阴影成像和瞬态定量相显微镜(TQPm)原位研究了远高于烧蚀阈值(F < 300 J.cm-2)的大块铝的修饰。这种新颖的泵浦探针技术能够定量测量物体的特性,例如熔体液滴的尺寸和层厚度或瞬态折射率变化。由n=1引起的汽化材料和/或熔体的一系列时间分辨相图像。用TQPm在铝靶上获得了8个脉冲。研究了熔炼的动力学和特性、烧蚀材料体积与工艺参数的关系以及由此引起的结构改变。在入射脉冲后约τ=300 ns和τ> 800ns的延迟时间内观察到物质喷射速率的增加。利用TQPm技术研究了Schott D263玻璃的瞬态折射率变化。利用高重复频率的超短脉冲激光辐射(tp=400 fs, λ=1045 nm, frep=1 MHz)通过显微镜物镜(w0≈4 μm)聚焦,实现了玻璃的热积累,从而实现了玻璃的熔化和焊接。在入射脉冲后测量到τ=2.1 μs的瞬态光学相位变化,这可归因于玻璃内部产生的自由载流子和压缩力。
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引用次数: 0
Influence of nitrogen oxides NO and NO2 additives on singlet oxygen production in pulsed electron-beam sustained discharge 氮氧化物NO和NO2添加剂对脉冲电子束持续放电中单线态产氧的影响
Pub Date : 2008-05-12 DOI: 10.1117/12.782481
A. Ionin, Y. Klimachev, A. Kozlov, A. Kotkov, I. Kochetov, A. Napartovich, O. Rulev, L. Seleznev, D. Sinitsyn, N. P. Vagin, N. Yuryshev
Influence of nitrogen oxides NO and NO2 on specific input energy (SIE) and time behavior of singlet delta oxygen (SDO) luminescence excited by pulsed e-beam sustained discharge in oxygen was experimentally and theoretically studied. NO and NO2 addition into oxygen results in small increase and decrease of SIE, respectively, the latter being connected with large energy of electron affinity to NO2. The addition of 0.1-0.3% nitrogen oxides was experimentally and theoretically demonstrated to result in notable enhancement of SDO lifetime, which is related to a decrease of atomic oxygen concentration in afterglow. There was experimentally demonstrated that for getting high SDO concentration at gas pressure 30-60 Torr for the time interval less than ~0.5 s one needs to add not less than 0.2% nitrogen oxides into oxygen. Temperature dependence of relaxation constant for SDO quenching by unexcited oxygen was estimated by using experimental data on time behavior of SDO luminescence.
实验和理论研究了氮氧化物NO和NO2对脉冲电子束持续放电激发单重态δ氧(SDO)发光比输入能(SIE)和时间行为的影响。向氧中添加NO和NO2分别导致SIE的小幅增加和降低,后者与对NO2的大电子亲和能有关。实验和理论证明,添加0.1-0.3%的氮氧化物可显著提高SDO的寿命,这与余辉中原子氧浓度的降低有关。实验证明,要在30-60 Torr的气压下,在小于~0.5 s的时间间隔内获得较高的SDO浓度,需要向氧气中加入不少于0.2%的氮氧化物。利用SDO发光时间行为的实验数据,估计了SDO被非激发氧猝灭时弛豫常数的温度依赖性。
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引用次数: 0
Mode-locked electron-beam sustained discharge CO laser 锁模电子束持续放电一氧化碳激光器
Pub Date : 2008-05-08 DOI: 10.1117/12.782491
A. Ionin, Y. Klimachev, A. Kotkov, A. Kozlov, L. Seleznev, D. Sinitsyn
Actively mode-locked electron-beam-sustained-discharge CO-laser producing ~10 ns (FWHM) pulses repetition rate 10 MHz for both single-line and multiline mode of operation was experimentally studied. The total laser pulse duration was ~0.5 ms for both mode-locked and free running laser conditions. The specific output energy in multiline CO-laser mode of operation was up to 20 J l-1 Amagat-1 and the laser efficiency up to 3.5%. The active mode-locking was achieved for single-line CO-laser mode of operation in the spectral range 5.2-5.3 micron. The radiation can be used for laser ablation, for pumping an optical parametric amplifier in optical stochastic cooling of relativistic heavy ions, and for studying vibrational and rotational relaxation of NO molecules.
实验研究了单线和多线工作模式下主动锁模电子束持续放电co激光器产生~10 ns (FWHM)脉冲重复率10 MHz。在锁模和自由运行条件下,激光总脉冲持续时间为~0.5 ms。在多线CO-laser工作模式下,比输出能量高达20 J -1 Amagat-1,激光效率高达3.5%。在光谱范围为5.2 ~ 5.3微米的单线co激光器工作模式下实现了主动锁模。该辐射可用于激光烧蚀,泵浦光学参量放大器用于相对论重离子的光学随机冷却,以及研究NO分子的振动和旋转弛豫。
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引用次数: 1
Collisional quenching and radiation trapping kinetics for Rb(5p) in the presence of ethane 乙烷存在下Rb(5p)的碰撞猝灭和辐射俘获动力学
Pub Date : 2008-05-08 DOI: 10.1117/12.801721
D. Hostutler, G. Hager, M. Heaven
Optically pumped alkali vapor lasers have been constructed using excitation of the D2 line (2P3/2-2S1/2) followed by lasing on the D1 line (2P1/2-2S1/2). Collisional relaxation is used to transfer population from 2P3/2 to the 2P1/2 level. The collision partner used for this step must have a large cross section for inducing transfer between the 2PJ levels, combined with a very small cross section for electronic quenching of the form M(2PJ)+Q→M(2S1/2)+Q (where M is an alkali metal and Q is the energy transfer agent). Ethane has proved to be an effective energy transfer agent for optically pumped Rb and Cs lasers. However, modeling of data for the Rb/C2H6 laser with the literature value for the quenching rate constant was unsuccessful. We have reexamined the quenching of Rb(2PJ) by C2H6 using time-resolved fluorescence techniques. Radiation trapping was significant under the conditions of our measurements, and an analysis of the interplay between the kinetics of trapping and quenching was carried out. It was found that quenching of Rb(2PJ) by C2H6 was very inefficient. The upper bound established for the quenching cross section was two orders of magnitude lower than that indicated by the previous determination.
利用D2线(2P3/2-2S1/2)的激发和D1线(2P1/2-2S1/2)的激光,构建了光抽运碱蒸汽激光器。碰撞松弛用于将种群从2P3/2转移到2P1/2水平。用于此步骤的碰撞伙伴必须具有较大的横截面,以诱导2PJ能级之间的转移,并结合非常小的横截面,以形成M(2PJ)+Q→M(2S1/2)+Q(其中M是碱金属,Q是能量转移剂)。乙烷已被证明是光泵浦Rb和Cs激光器的有效能量转移剂。然而,用文献中的淬火速率常数对Rb/C2H6激光器的数据进行建模是不成功的。我们用时间分辨荧光技术重新研究了C2H6对Rb(2PJ)的猝灭作用。在我们的测量条件下,辐射捕获是显著的,并对捕获动力学和猝灭之间的相互作用进行了分析。发现C2H6对Rb(2PJ)的猝灭效率很低。淬火截面的上界比先前的测定结果低两个数量级。
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引用次数: 8
Critical fluence effects in laser propulsion 激光推进中的临界通量效应
Pub Date : 2008-05-08 DOI: 10.1117/12.782469
J. Sinko, D. Gregory
The fluence dependence of the laser ablation of selected polymers was studied within the range from 1-150 J/cm2. A TEA CO2 laser operating at 10.6 μm with 300 ns main pulse length and up to 20 J pulse energy was used to ablate prepared polymer samples with single pulses of laser energy. Measurements of parameters such as the ablated mass per spot area (Δma), momentum coupling coefficient (Cm), specific impulse (Isp), and internal efficiency (ηi) will be plotted as functions of fluence. Critical threshold effects observed throughout the experiments will be described in detail.
在1 ~ 150 J/cm2范围内研究了所选聚合物激光烧蚀的影响关系。利用工作波长为10.6 μm、主脉冲长度为300 ns、脉冲能量为20 J的TEA CO2激光器,对制备的聚合物样品进行单脉冲激光烧蚀。测量参数,如每点面积的烧蚀质量(Δma)、动量耦合系数(Cm)、比脉冲(Isp)和内部效率(ηi)将绘制为影响的函数。在整个实验中观察到的临界阈值效应将被详细描述。
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引用次数: 12
Femtosecond x-ray diffuse scattering measurements of semiconductor ablation dynamics 半导体烧蚀动力学的飞秒x射线漫射测量
Pub Date : 2008-05-08 DOI: 10.1117/12.784094
A. Lindenberg, S. Engemann, K. Gaffney, K. Sokolowski-Tinten, J. Larsson, D. Reis, P. Lorazo, J. Hastings
Femtosecond time-resolved small and wide-angle x-ray diffuse scattering techniques are applied to investigate the ultrafast nucleation processes that occur during the ablation process in semiconducting materials. Following intense optical excitation, a transient liquid state of high compressibility characterized by large-amplitude density fluctuations is observed and the build-up of these fluctuations is measured in real-time. Small-angle scattering measurements reveal the first steps in the nucleation of nanoscale voids below the surface of the semiconductor and support MD simulations of the ablation process.
应用飞秒时间分辨小广角x射线漫射散射技术研究了半导体材料烧蚀过程中的超快成核过程。在强烈的光激发后,观察到具有大振幅密度波动特征的高压缩性瞬态,并实时测量这些波动的积累。小角度散射测量揭示了半导体表面下纳米级空洞成核的第一步,并支持烧蚀过程的MD模拟。
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引用次数: 1
Nanopulsed laser modification of Ge/Si heterostructures 纳米脉冲激光修饰Ge/Si异质结构
Pub Date : 2008-05-08 DOI: 10.1117/12.782596
G. Ivlev, E. Gatskevich
Laser-induced phase transitions in a-Ge/Si heterostructures (amorphous Ge films on crystalline Si substrate) have been studied by optical diagnostics and numerical simulation methods. The samples were irradiated by (i) a ruby laser with pulse duration 80 ns (FWHM) and wavelength 694 nm and (ii) an ArF excimer laser (10 ns and 193 nm). Time resolved reflectivity measurements showed the discrepancy in dynamics of reflectivity of probing beam for different regimes of laser irradiation. This discrepancy can be explained by differing kinetics of solid-liquid phase transitions in Ge films: (i) intermediate crystallization or (ii) simultaneous solidification of molten Ge layer from the surface and from the substrate.
采用光学诊断和数值模拟方法研究了激光诱导的a-Ge/Si异质结构(晶体Si衬底上的非晶Ge薄膜)的相变。分别用脉冲长80 ns (FWHM)、波长694 nm的红宝石激光器和10 ns、波长193 nm的ArF准分子激光器照射样品。时间分辨反射率测量表明,在不同的激光照射条件下,探测光束的反射率动态变化存在差异。这种差异可以用锗膜固液相变动力学的不同来解释:(i)中间结晶或(ii)熔化的锗层从表面和衬底同时凝固。
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引用次数: 0
On the mechanism of resonant infrared polymer ablation: the case of polystyrene 共振红外聚合物烧蚀机理研究:以聚苯乙烯为例
Pub Date : 2008-05-08 DOI: 10.1117/12.786387
S. Johnson, D. M. Bubb, K. Schriver, R. Haglund
We investigate the fundamental mechanisms of resonant-infrared laser ablation of polymers using polystyrene as a model material. Time-resolved plume shadowgraphy coupled with laser-induced temperature-rise calculations indicate that spinodal decomposition of a superheated surface layer is the primary mechanism for the initial stages of material removal. The majority of the ablated material is then released by way of recoil-induced ejection of liquid which proceeds for some tens of microseconds following a ~μs laser pulse excitation. The recoil-induced ejection of liquid material as the dominant ablation mechanism helps to explain previous observations of laser deposition of intact polymeric material.
以聚苯乙烯为模型材料,研究了共振红外激光烧蚀聚合物的基本机理。时间分辨羽流阴影成像与激光诱导的温升计算相结合表明,过热表层的旋量分解是物质去除初始阶段的主要机制。在~μs的激光脉冲激发下,大部分烧蚀材料以液体反冲喷射的方式释放出来,这一过程持续数十微秒。液体材料的反冲喷射是主要的烧蚀机制,有助于解释先前观察到的完整聚合物材料的激光沉积。
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引用次数: 2
期刊
High-Power Laser Ablation
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