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Pollutant removal efficiency of bare and planted rain gardens with diverse planting mixtures 采用不同种植混合物的裸露雨水花园和种植雨水花园的污染物去除效率
Pub Date : 2024-06-08 DOI: 10.2166/wst.2024.192
Sandeep Kumar, Krishna Kumar Singh
This study examines the influence of planting mixture variations on the quality of the percolated water of the rain garden with and without plants. Six planting mixtures in experimental rain gardens have been used. It has been noted that pollutant removal efficiency of RG can exhibit variations based on specific parameters. Notably, RG6, utilizing a planting mix of 75% topsoil and 25% compost, demonstrated the highest performance. These results draw attention to the critical role of the specific planting mixtures in influencing the performance of vital parameters related to pollutant removal. The observation shows that RG5 exhibits exceptional removal efficiency in pH, Total Suspended Solids (TSS), Biological Oxygen Demand (BOD), and Chemical Oxygen Demand (COD), and RG6 performs best in electrical conductivity (EC), Total Dissolved Solids (TDS), Total Nitrogen (TN), and Total Phosphorus (TP) removal. In particular, when analyzing pollutant removal on a surface with Madagascar periwinkle plants, RG6 emerges as the most effective, achieving an impressive efficiency of approximately 49%. For the bare surface, pollutant removal efficiency is 40%. The study outcome will be useful in deciding the composition of the planting mixture, which will keep the rain garden to improve quality and quantitatively hydrological performance, lowering urban flooding magnitude.
本研究探讨了种植混合物的变化对有植物和无植物雨水花园渗水水质的影响。在实验雨水花园中使用了六种种植混合物。人们注意到,RG 的污染物去除效率会因特定参数而变化。值得注意的是,采用 75% 表土和 25% 堆肥混合种植的 RG6 表现出最高的性能。这些结果提醒人们注意特定种植混合物在影响污染物去除相关重要参数性能方面的关键作用。观察结果表明,RG5 在 pH 值、总悬浮固体 (TSS)、生物需氧量 (BOD) 和化学需氧量 (COD) 方面表现出卓越的去除效率,而 RG6 在电导率 (EC)、总溶解固体 (TDS)、总氮 (TN) 和总磷 (TP) 的去除方面表现最佳。特别是在分析长春花表面的污染物去除率时,RG6 的去除率最高,达到了令人印象深刻的 49% 左右。而裸露表面的污染物去除率为 40%。研究结果将有助于决定种植混合物的组成,从而使雨水花园在质量和数量上提高水文性能,降低城市洪水的规模。
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引用次数: 0
Model-based assessment of in-sewer heat recovery potentials considering wastewater treatment-specific temperature limits 基于模型的污水热回收潜力评估,考虑到废水处理的特定温度限制
Pub Date : 2024-06-08 DOI: 10.2166/wst.2024.190
Dirk Muschalla, W. Sprung, Stefan Reinstaller, Markus Pichler, F. Kretschmer
Due to the ongoing climate and energy crisis, wastewater is becoming increasingly important as a source of renewable energy. In urban areas, heat recovery from the sewer is considered a promising approach, as the locations of supply and demand are close to each other. In this context, it is crucial that negative impacts on temperature-sensitive processes in the downstream wastewater treatment plant are strictly avoided. To support the necessary planning and authorization, this paper presents a model-based approach to assess the thermal energy level of the wastewater at any given location in the sewer, taking into account the influent temperature constraints of the wastewater treatment plant. The entire modelling is based on the open-source software SWMM 5, which was extended by a temperature model. The concept showed its practicability and informative value during a full-scale field application in the sewer systems of the Austrian city of Graz. All modelling is based on freely available software, which makes the approach easy transferable to other cities with comparable infrastructural boundary conditions.
由于持续的气候和能源危机,废水作为一种可再生能源正变得越来越重要。在城市地区,从下水道回收热量被认为是一种很有前景的方法,因为供需双方的位置很近。在这种情况下,必须严格避免对下游污水处理厂中对温度敏感的工艺产生负面影响。为了支持必要的规划和授权,本文提出了一种基于模型的方法,用于评估下水道中任何给定位置的废水热能水平,同时考虑到废水处理厂的进水温度限制。整个建模基于开源软件 SWMM 5,并通过温度模型进行了扩展。在奥地利格拉茨市下水道系统的全面实地应用中,这一概念显示了其实用性和信息价值。所有建模都是基于免费提供的软件,这使得该方法可以很容易地移植到具有类似基础设施边界条件的其他城市。
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引用次数: 0
Metrics to quantify the degree of co-location of urban water infrastructure 量化城市水基础设施共用地点程度的指标
Pub Date : 2024-06-08 DOI: 10.2166/wst.2024.191
Shamsuddin Daulat, B. Roghani, J. Langeveld, M. Rokstad, Franz Tscheikner-Gratla
Co-located infrastructure networks such as roads, water, and sewer in theory offer the possibility for integrated multi-infrastructure interventions. However, how closely these networks are aligned in space and time determines the practical extent to which such coordinated interventions can be realized. This study quantifies the spatial alignment of the aforementioned infrastructure networks and demonstrates its application for integrated interventions and potential cost savings. It proposes two metrics, namely (1) shared surface area and (2) shared trench volume, to quantify the spatial relationship (i.e., degree of co-location) of infrastructures. Furthermore, the study demonstrates how the degree of co-location can be used as a proxy for cost-saving potential of integrated interventions compared to silo-based, single-infrastructure, interventions. Through six case studies conducted in Norwegian municipalities, the research reveals that implementing integrated interventions across road, water, and sewer networks can result in potential average cost savings of 24% in urban areas and 11% in rural areas. Utility-specific savings under different cost-sharing scenarios were also analyzed. To identify the yearly potential of integrated multi-infrastructure interventions, future work should add the temporal alignment of rehabilitation of infrastructures (i.e., time of intervention needed for the infrastructures).
从理论上讲,道路、供水和下水道等共用基础设施网络为多基础设施综合干预提供了可能。然而,这些网络在空间和时间上的紧密配合程度决定了此类协调干预措施的实际实现程度。本研究对上述基础设施网络的空间排列进行了量化,并展示了其在综合干预和潜在成本节约方面的应用。研究提出了两个指标,即(1)共享表面积和(2)共享沟槽体积,用于量化基础设施的空间关系(即共用位置的程度)。此外,该研究还展示了如何利用共建程度来衡量综合干预措施与基于筒仓的单一基础设施干预措施相比的成本节约潜力。通过在挪威城市开展的六项案例研究,该研究揭示了在道路、供水和下水道网络之间实施综合干预措施,可为城市地区节省 24% 的潜在平均成本,为农村地区节省 11% 的潜在平均成本。此外,还分析了不同成本分摊方案下的具体节支情况。为确定多基础设施综合干预的年度潜力,未来的工作应增加基础设施修复的时间调整(即基础设施所需的干预时间)。
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引用次数: 0
Synergistic effect and microbial community structure of waste-activated sludge and kitchen waste solids residue mesophilic anaerobic co-digestion 垃圾活性污泥和厨余固体残渣中温厌氧协同消化的协同效应和微生物群落结构
Pub Date : 2024-06-07 DOI: 10.2166/wst.2024.186
Tongzhan Xue, Xiangyu Yan, Weihua Li, Jiajia Xu, Xinlei Yang
Anaerobic co-digestion was conducted on the solid residues after three-phase separation of kitchen waste (KWS) and waste-activated sludge (WAS), the synergistic effects and process performance were studied during co-digestion at different ratios of KWS to WAS. KWS and WAS mix ratios of 0:1, 1:4, 1:3, 1:2, 1:1, 2:1, 3:1, 4:1 and 1:0 (based on TS). The results showed that a ratio of KWS to WAS of 1:1 got a very high methane recovery with a methane yield of 310.45 ± 30.05 mL/g VSadded. The highest concentration of free ammonia among all reaction systems was only 70.23 ± 5.53 mg/L, which was not enough to produce ammonia inhibition in the anaerobic co-digestion system. However, when the KWS content exceeded 50%, methane inhibition and prolongation of the lag phase were observed due to the accumulation of volatile fatty acids (VFAs), and during the lag phase. Microbial community analysis showed that various bacterial groups involved in acid production and hydrolysis were mainly dominated by phylum Firmicutes, Chloroflexi, Proteobacteria and Bacteroidetes. Hydrogenotrophic methanogen was found to dominate all archaeal communities in the digesters. Co-digestion of KWS with WAS significantly increased the relative abundance of Methanobacterium compared with anaerobic digestion of SS alone.
对厨余(KWS)和废物活性污泥(WAS)三相分离后的固体残留物进行了厌氧协同消化,研究了在不同比例的 KWS 和 WAS 协同消化过程中的协同效应和工艺性能。KWS 和 WAS 的混合比例分别为 0:1、1:4、1:3、1:2、1:1、2:1、3:1、4:1 和 1:0(基于 TS)。结果表明,KWS 与 WAS 的比例为 1:1,甲烷回收率非常高,甲烷产量为 310.45 ± 30.05 mL/g VSadded。在所有反应系统中,游离氨的最高浓度仅为 70.23 ± 5.53 mg/L,不足以在厌氧协同消化系统中产生氨抑制。然而,当 KWS 含量超过 50%时,由于挥发性脂肪酸(VFAs)的积累,在滞后期会出现甲烷抑制和滞后期延长的现象。微生物群落分析表明,参与产酸和水解的各种细菌群主要以坚固菌门、绿僵菌门、变形菌门和类杆菌门为主。在消化器中的所有古细菌群落中,都发现养氢甲烷菌占主导地位。与单独厌氧消化 SS 相比,协同消化 KWS 和 WAS 能显著提高甲烷菌的相对丰度。
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引用次数: 0
Implementing a completely autotrophic nitrogen removal over nitrite process using a novel umbrella basalt fiber carrier 利用新型伞状玄武岩纤维载体实现完全自养的亚硝酸盐脱氮过程
Pub Date : 2024-06-07 DOI: 10.2166/wst.2024.188
Shan-Wei Li, Wei Xu, Yu-Jie Xie, Liang Fu, Qi Gao, Xiao-Chun Wang, Yan Li, Zhiqiang Wu
The completely autotrophic nitrogen removal over nitrite (CANON) process is significantly hindered by prolonged start-up periods and unstable nitrogen removal efficiency. In this study, a novel umbrella basalt fiber (BF) carrier with good biological affinity and adsorption performance was used to initiate the CANON process. The CANON process was initiated on day 64 in a sequencing batch reactor equipped with umbrella BF carriers. During this period, the influent NH4+-N concentration gradually increased from 100 to 200 mg·L−1, and the dissolved oxygen was controlled below 0.8 mg L−1. Consequently, an average ammonia nitrogen removal efficiency (ARE) and total nitrogen removal efficiency (TNRE) of ∼90 and 80% were achieved, respectively. After 130 days, ARE and TNRE remained stable at 92 and 81.1%, respectively. This indicates a reliable method for achieving rapid start-up and stable operation of the CANON process. Moreover, Candidatus Kuenenia and Candidatus Brocadia were identified as dominant anammox genera on the carrier. Nitrosomonas was the predominant genus among ammonia-oxidizing bacteria. Spatial differences were observed in the microbial population of umbrella BF carriers. This arrangement facilitated autotrophic nitrogen removal in a single reactor. This study indicates that the novel umbrella BF carrier is a highly suitable biocarrier for the CANON process.
完全自养的亚硝酸盐脱氮(CANON)工艺因启动期长和脱氮效率不稳定而受到严重阻碍。本研究采用了一种具有良好生物亲和性和吸附性能的新型伞状玄武岩纤维(BF)载体来启动 CANON 工艺。在一个配备了伞状玄武岩纤维载体的序批式反应器中,CANON 工艺于第 64 天启动。在此期间,进水 NH4+-N 浓度从 100 mg-L-1 逐渐增加到 200 mg-L-1,溶解氧控制在 0.8 mg L-1 以下。因此,平均氨氮去除率(ARE)和总氮去除率(TNRE)分别达到了 90% 和 80%。130 天后,氨氮去除率和总氮去除率分别稳定在 92% 和 81.1%。这表明有一种可靠的方法可以实现 CANON 工艺的快速启动和稳定运行。此外,Kuenenia 菌和 Brocadia 菌被确定为载体上的优势厌氧菌属。亚硝基单胞菌是氨氧化细菌中的优势菌属。在伞状 BF 载体的微生物群中观察到了空间差异。这种排列方式有利于在单个反应器中进行自养脱氮。这项研究表明,新型伞状生物燃料载体是一种非常适合 CANON 工艺的生物载体。
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引用次数: 0
Full-length 16S rRNA gene sequencing reveals the operating mode and chlorination-aggravated SWRO biofouling at a nuclear power plant 全长 16S rRNA 基因测序揭示了核电站的运行模式和氯化加重的 SWRO 生物污垢
Pub Date : 2024-06-07 DOI: 10.2166/wst.2024.185
Kaijia Ren, H. Ming, Siyu Liu, Xianlong Lang, Yuan Jin, Jingfeng Fan
Reverse osmosis (RO) membrane fouling and biological contamination problems faced by seawater desalination systems are microbiologically related. We used full-length 16S rRNA gene sequencing to assess the bacterial community structure and chlorine-resistant bacteria (CRB) associated with biofilm growth in different treatment processes under the winter mode of a chlorinated seawater desalination system in China. At the outset of the winter mode, certain CRB, such as Acinetobacter, Pseudomonas, and Bacillus held sway over the bacterial community structure, playing a pivotal role in biofouling. At the mode's end, Deinococcus and Paracoccus predominated, with Pseudomonas and Roseovarius following suit, while certain CRB genera still maintained their dominance. RO and chlorination are pivotal factors in shaping the bacterial community structure and diversity, and increases in total heterotrophic bacterial counts and community diversity in safety filters may adversely affect the effectiveness of subsequent RO systems. Besides, the bacterial diversity and culturable biomass in the water produced by the RO system remain high, and some conditionally pathogenic CRBs pose a certain microbial risk as a source of drinking water. Targeted removal of these CRBs will be an important area of research for advancing control over membrane clogging and ensuring water quality safety in the future.
海水淡化系统面临的反渗透(RO)膜污垢和生物污染问题与微生物有关。我们利用全长 16S rRNA 基因测序技术评估了中国含氯海水淡化系统冬季模式下不同处理工艺中的细菌群落结构和与生物膜生长相关的耐氯菌(CRB)。在冬季模式开始时,某些耐氯细菌(如醋酸杆菌、假单胞菌和芽孢杆菌)控制着细菌群落结构,在生物污损中发挥着关键作用。在冬季模式结束时,Deinococcus 和 Paracoccus 占主导地位,假单胞菌和 Roseovarius 紧随其后,而某些 CRB 菌属仍保持着优势地位。反渗透和氯化是形成细菌群落结构和多样性的关键因素,安全过滤器中异养细菌总数和群落多样性的增加可能会对后续反渗透系统的效果产生不利影响。此外,反渗透系统产水中的细菌多样性和可培养生物量仍然很高,一些条件致病性 CRB 作为饮用水源会带来一定的微生物风险。有针对性地去除这些 CRB 将是未来推进膜堵塞控制和确保水质安全的一个重要研究领域。
{"title":"Full-length 16S rRNA gene sequencing reveals the operating mode and chlorination-aggravated SWRO biofouling at a nuclear power plant","authors":"Kaijia Ren, H. Ming, Siyu Liu, Xianlong Lang, Yuan Jin, Jingfeng Fan","doi":"10.2166/wst.2024.185","DOIUrl":"https://doi.org/10.2166/wst.2024.185","url":null,"abstract":"\u0000 \u0000 Reverse osmosis (RO) membrane fouling and biological contamination problems faced by seawater desalination systems are microbiologically related. We used full-length 16S rRNA gene sequencing to assess the bacterial community structure and chlorine-resistant bacteria (CRB) associated with biofilm growth in different treatment processes under the winter mode of a chlorinated seawater desalination system in China. At the outset of the winter mode, certain CRB, such as Acinetobacter, Pseudomonas, and Bacillus held sway over the bacterial community structure, playing a pivotal role in biofouling. At the mode's end, Deinococcus and Paracoccus predominated, with Pseudomonas and Roseovarius following suit, while certain CRB genera still maintained their dominance. RO and chlorination are pivotal factors in shaping the bacterial community structure and diversity, and increases in total heterotrophic bacterial counts and community diversity in safety filters may adversely affect the effectiveness of subsequent RO systems. Besides, the bacterial diversity and culturable biomass in the water produced by the RO system remain high, and some conditionally pathogenic CRBs pose a certain microbial risk as a source of drinking water. Targeted removal of these CRBs will be an important area of research for advancing control over membrane clogging and ensuring water quality safety in the future.","PeriodicalId":298320,"journal":{"name":"Water Science & Technology","volume":" 6","pages":""},"PeriodicalIF":0.0,"publicationDate":"2024-06-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141375453","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Purification of acidic wastewater containing Cd(II) using a red mud–loess mixture: Column test, breakthrough curve, and speciation of Cd 利用赤泥无水混合物净化含 Cd(II) 的酸性废水:色谱柱测试、突破曲线和镉的标示
Pub Date : 2024-06-07 DOI: 10.2166/wst.2024.187
Yisi Lu, Xiaofeng Liu, Hao Zhang, Jiashi Li
In this study, the safety of a red mud–loess mixture (RM–L) for the remediation of groundwater polluted by acid mine drainage (AMD) containing Cd(II) in mining areas was systematically analyzed and clarified. The effects of the initial concentration, flow rate, and packing height on the breakthrough performance and longevity of RM–L as a permeable reactive barrier (PRB) packing material were explored by column tests. The results show that the breakthrough time, saturation time, and adsorption capacity of Cd(II) in RM–L increased with decreasing initial concentration and flow rate, as well as increasing packing height. Moreover, RM–L had a long-term effective acid buffering capacity for acidic wastewater containing Cd(II). An increase in the packing height led to a longer longevity of the PRB than the theoretical value. In addition, the speciation of Cd on RM–L was dominated by carbonate form and iron–manganese oxide form. The surface of the RM–L particles evolved from a dense lamellar structure to small globular clusters after purifying the acidic wastewater containing Cd(II), due to the corrosion of H+ and the reoccupation and coverage by increasingly enriched adsorbates and precipitates of heavy metal ions.
本研究系统分析并阐明了赤泥-无水混合物(RM-L)在修复矿区含镉(II)酸性矿井排水(AMD)污染的地下水方面的安全性。通过柱试验探讨了初始浓度、流速和填料高度对 RM-L 作为渗透反应屏障(PRB)填料的突破性能和寿命的影响。结果表明,RM-L 对镉(II)的突破时间、饱和时间和吸附容量随初始浓度和流速的降低以及填料高度的增加而增加。此外,RM-L 对含 Cd(II)的酸性废水具有长期有效的酸缓冲能力。填料高度的增加使 PRB 的寿命比理论值更长。此外,RM-L 上的镉主要以碳酸盐形式和铁锰氧化物形式存在。在净化含镉(II)的酸性废水后,RM-L 颗粒的表面从致密的片状结构演变为小球状团块,这是由于 H+ 的腐蚀以及重金属离子的吸附物和沉淀物的富集和覆盖。
{"title":"Purification of acidic wastewater containing Cd(II) using a red mud–loess mixture: Column test, breakthrough curve, and speciation of Cd","authors":"Yisi Lu, Xiaofeng Liu, Hao Zhang, Jiashi Li","doi":"10.2166/wst.2024.187","DOIUrl":"https://doi.org/10.2166/wst.2024.187","url":null,"abstract":"\u0000 \u0000 In this study, the safety of a red mud–loess mixture (RM–L) for the remediation of groundwater polluted by acid mine drainage (AMD) containing Cd(II) in mining areas was systematically analyzed and clarified. The effects of the initial concentration, flow rate, and packing height on the breakthrough performance and longevity of RM–L as a permeable reactive barrier (PRB) packing material were explored by column tests. The results show that the breakthrough time, saturation time, and adsorption capacity of Cd(II) in RM–L increased with decreasing initial concentration and flow rate, as well as increasing packing height. Moreover, RM–L had a long-term effective acid buffering capacity for acidic wastewater containing Cd(II). An increase in the packing height led to a longer longevity of the PRB than the theoretical value. In addition, the speciation of Cd on RM–L was dominated by carbonate form and iron–manganese oxide form. The surface of the RM–L particles evolved from a dense lamellar structure to small globular clusters after purifying the acidic wastewater containing Cd(II), due to the corrosion of H+ and the reoccupation and coverage by increasingly enriched adsorbates and precipitates of heavy metal ions.","PeriodicalId":298320,"journal":{"name":"Water Science & Technology","volume":" 20","pages":""},"PeriodicalIF":0.0,"publicationDate":"2024-06-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141373092","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Performance analysis of snail shell biomaterials in solar stills for clean water production: nature-inspired innovation for sustainability 清洁水生产太阳能蒸馏器中蜗牛壳生物材料的性能分析:自然启发下的可持续创新
Pub Date : 2024-06-07 DOI: 10.2166/wst.2024.189
R. Dhivagar, Subbarama Kousik Suraparaju, Farruh Atamurotov, Kalimuthu Gopi Kannan, Serikzhan Opakhai, Adil A. M. Omara
In this current investigation, the experimental performance of a solar still basin was significantly enhanced by incorporating snail shell biomaterials. The outcomes of the snail shell-augmented solar still basin (SSSS) are compared with those of a conventional solar still (CSS). The utilization of snail shells proved to facilitate the reduction of saline water and enhance its temperature, thereby improving the productivity of the SSSS. Cumulatively, the SSSS productivity was improved by 4.3% over CSS. Furthermore, the SSSS outperformed in energy and exergy efficiency of CSS by 4.5 and 3.5%, respectively. Economically, the cost per liter of distillate (CPL) for the CSS was 3.4% higher than SSSS. Moreover, the SSSS showed a shorter estimated payback period (PBP) of 141 days which was 6 days less than CSS. Considering the environmental impact, the observed CO2 emissions from the SSSS were approximately 14.6% higher than CSS over its 10-year lifespan. Notably, the SSSS exhibited a substantial increase in the estimated carbon credit earned (CCE) compared to the CSS. Ultimately, the research underscores the efficacy of incorporating snail shells into solar still basins as a commendable approach to organic waste management, offering economic benefits without compromising environmental considerations.
在本次研究中,通过加入蜗牛壳生物材料,太阳能蒸馏池的实验性能得到了显著提高。蜗牛壳增强型太阳能蒸馏器(SSSS)的结果与传统太阳能蒸馏器(CSS)的结果进行了比较。事实证明,利用蜗牛壳有助于减少盐水并提高其温度,从而提高太阳能蒸发器的生产率。与 CSS 相比,SSSS 的生产率累计提高了 4.3%。此外,该系统的能源效率和放能效率分别比 CSS 系统高出 4.5% 和 3.5%。在经济上,CSS 的每升馏分油成本 (CPL) 比 SSSS 高 3.4%。此外,SSSS 的估计投资回收期较短,为 141 天,比 CSS 少 6 天。考虑到对环境的影响,在 10 年使用期内,观察到的 SSSS 二氧化碳排放量比 CSS 高出约 14.6%。值得注意的是,与 CSS 相比,SSSS 估算的碳信用额(CCE)大幅增加。最终,这项研究强调了将蜗牛壳纳入太阳能蒸馏池的功效,认为这是一种值得称赞的有机废物管理方法,既能带来经济效益,又不影响环境因素。
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引用次数: 0
Comparative life cycle assessment of excreta management systems through composting and biomethanization: case of a low-income tropical country 通过堆肥和生物甲烷化对粪便管理系统进行生命周期比较评估:一个低收入热带国家的案例
Pub Date : 2024-06-06 DOI: 10.2166/wst.2024.184
Davidson Jean-Baptiste, Frédéric Monette
Low-income tropical regions, such as Haiti, grapple with environmental issues stemming from inadequate sanitation infrastructure for fecal sludge management. This study scrutinizes on-site sanitation systems in these regions, evaluating their environmental impacts and pinpointing improvement opportunities. The focus is specifically on systems integrating excreta valorization through composting and/or anaerobic digestion. Each system encompasses toilet access, evacuation, and sludge treatment. A comparative life cycle assessment was undertaken, with the functional unit managing one ton of excreta in Haiti over a year. Six scenarios representing autonomous sanitation systems were devised by combining three toilet types (container-based toilets (CBTs), ventilated improved pit (VIP) latrines, and flush toilets (WC)) with two sludge treatment processes (composting and biomethanization). Biodigester-based systems exhibited 1.05 times higher sanitary impacts and 1.03 times higher ecosystem impacts than those with composters. Among toilet types, CBTs had the lowest impacts, followed by VIP latrines, with WCs having the highest impacts. On average, WC scenarios were 3.85 times more impactful than VIP latrines and 4.04 times more impactful than those with CBTs regarding human health impact. Critical variables identified include the use of toilet paper, wood shavings, greenhouse gas emissions, and construction materials.
海地等低收入热带地区因用于粪便污泥管理的卫生基础设施不足而面临环境问题。本研究仔细研究了这些地区的现场卫生系统,评估了它们对环境的影响,并指出了改进的机会。重点特别放在通过堆肥和/或厌氧消化实现排泄物价值化的系统上。每个系统都包括厕所接入、排空和污泥处理。以海地一年管理一吨排泄物为功能单元,进行了生命周期比较评估。通过将三种厕所类型(集装箱式厕所(CBT)、通风改良坑式厕所(VIP)和抽水马桶(WC))与两种污泥处理工艺(堆肥和生物甲烷化)相结合,设计了代表自主卫生系统的六种方案。与使用堆肥器的厕所相比,使用生物发酵器的厕所对卫生的影响高出 1.05 倍,对生态系统的影响高出 1.03 倍。在厕所类型中,CBT 的影响最小,其次是 VIP 厕所,而 WC 的影响最大。平均而言,在对人类健康的影响方面,WC 方案的影响是 VIP 厕所的 3.85 倍,是 CBT 方案的 4.04 倍。确定的关键变量包括卫生纸的使用、木屑、温室气体排放和建筑材料。
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引用次数: 0
Combination of co-pyrolyzed biomass–sludge biochar and ultrasound for persulfate activation in antibiotic degradation: efficiency, synergistic effect, and reaction mechanism 热解生物质-污泥生物炭与超声波结合用于抗生素降解中的过硫酸盐活化:效率、协同效应和反应机制
Pub Date : 2024-06-06 DOI: 10.2166/wst.2024.183
Wan Jiang, Yiming Liu, Shenpeng Wang, Haifeng Yang, Xiulei Fan
A carbon material Cu-corn straw-sludge biochar (Cu-CSBC) was prepared by hydrothermally modifying sewage sludge and corn stover. The composite coupled to ultrasound can effectively catalyze the activation of PS for organic pollutants degradation, and the removal rate of 20 mg/L TC reached 89.15% in 5 min in the presence of 0.5 g/L Cu-CSBC and 3 mM PS. The synergistic effect between the factors in the system, the reaction mechanism, and the efficient removal of TC in the aqueous environment were explored in a Cu-CSBC/US/PS system established for that purpose. Quenching experiments and electron paramagnetic resonance analysis both demonstrated the Cu-CSBC/US/PS system generated •OH, SO4–•, 1O2, and O2- •, which involved in the reaction. The Cu, carboxyl, and hydroxyl groups on the Cu-CSBC surface promoted the generation of radicals and non-radicals for the degradation process, which was dominated by both radical and non-radical pathways. The degradation pathway is proposed by measuring the intermediate products with LC-MS. Finally, the stability of the Cu-CSBC/US/PS system was tested under various reaction conditions. This study not only prepared a novel biochar composite material for the active degradation of organic pollutants by PS but also provided an effective method for the resource utilization of solid waste and sludge treatment.
通过对污水污泥和玉米秸秆进行水热改性,制备了一种碳材料铜-玉米秸秆-污泥生物炭(Cu-CSBC)。在 0.5 g/L Cu-CSBC 和 3 mM PS 的条件下,5 min 内对 20 mg/L TC 的去除率达到 89.15%。在为此而建立的 Cu-CSBC/US/PS 系统中,探讨了系统中各因素之间的协同效应、反应机理以及水环境中 TC 的高效去除。淬火实验和电子顺磁共振分析均表明,Cu-CSBC/US/PS 系统在反应中产生了-OH、SO4-、1O2 和 O2- -。Cu-CSBC 表面的铜、羧基和羟基促进了降解过程中自由基和非自由基的生成,其中以自由基和非自由基途径为主。通过使用 LC-MS 测量中间产物,提出了降解途径。最后,测试了 Cu-CSBC/US/PS 系统在各种反应条件下的稳定性。该研究不仅制备了一种新型生物炭复合材料,可用于 PS 活性降解有机污染物,还为固体废弃物的资源化利用和污泥处理提供了一种有效的方法。
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引用次数: 0
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