首页 > 最新文献

International Journal of Multiphase Flow最新文献

英文 中文
Microfluidic study of effect of dispersed phase viscosity and continuous phase viscosity on emulsification in a cross-junction chip 交叉接合芯片中分散相粘度和连续相粘度对乳化影响的微流体研究
IF 3.8 2区 工程技术 Q1 Engineering Pub Date : 2024-06-02 DOI: 10.1016/j.ijmultiphaseflow.2024.104885
Huiyu Wang , Bei Wei , Jian Hou , Yongsheng Liu , Yang Zhang , Tong Peng

Immiscible flow of oil phase and displacing phase with surfactant can cause emulsification during the oil development. However, it is still unclear how the viscosity of each phase influences the emulsification at the micro level. In this study, we investigated the flow regimes and emulsification of two immiscible fluids in a cross-junction device by using an oil-surfactant system and an oil-surfactant/polymer system. Based on the experimental data, we analyzed the flow regimes and draw flow regime maps of the two systems. Moreover, we established the new scaling laws that include the capillary number, the flow rate ratio, and the viscosity ratio of two phases to predict the droplet diameter or slug length. The findings indicated that there are four flow regimes in the oil-surfactant system, including threading, squeezing, dripping, and jetting regimes. Besides, a new type of flow regime, irregular dripping regime, appears in the oil-surfactant/polymer system. According to the regime maps, the area of dripping regime decreases with the increase of the viscosity of dispersed phase or continuous phase. For both systems, the regression equations with the viscosity ratio have better fitting effect than those without the viscosity ratio. Meanwhile, compared with the effect of viscosity ratio of two phases, the flow rate ratio of two phases has higher influence on droplet diameter and slug length. The experiments present detailed emulsification processes at pore scale and provide new insights for the prediction of emulsion droplets and slugs.

油相和带有表面活性剂的置换相的不相容流动会在石油开发过程中造成乳化。然而,目前还不清楚各相的粘度如何在微观层面上影响乳化作用。在本研究中,我们使用油-表面活性剂体系和油-表面活性剂/聚合物体系研究了两种不相溶流体在交叉接合装置中的流动状态和乳化作用。根据实验数据,我们分析了两种体系的流态并绘制了流态图。此外,我们还建立了包括毛细管数、流速比和两相粘度比的新比例定律,以预测液滴直径或液滴长度。研究结果表明,油-表面活性剂体系存在四种流态,包括螺纹流态、挤压流态、滴流态和喷射流态。此外,在油-表面活性剂-聚合物体系中还出现了一种新型流态--不规则滴流态。根据流态图,滴落流态的面积随着分散相或连续相粘度的增加而减小。对于这两种体系,有粘度比的回归方程比无粘度比的回归方程具有更好的拟合效果。同时,与两相粘度比的影响相比,两相流速比对液滴直径和液滴长度的影响更大。实验展示了孔隙尺度下的详细乳化过程,为预测乳液液滴和液滴长度提供了新的见解。
{"title":"Microfluidic study of effect of dispersed phase viscosity and continuous phase viscosity on emulsification in a cross-junction chip","authors":"Huiyu Wang ,&nbsp;Bei Wei ,&nbsp;Jian Hou ,&nbsp;Yongsheng Liu ,&nbsp;Yang Zhang ,&nbsp;Tong Peng","doi":"10.1016/j.ijmultiphaseflow.2024.104885","DOIUrl":"10.1016/j.ijmultiphaseflow.2024.104885","url":null,"abstract":"<div><p>Immiscible flow of oil phase and displacing phase with surfactant can cause emulsification during the oil development. However, it is still unclear how the viscosity of each phase influences the emulsification at the micro level. In this study, we investigated the flow regimes and emulsification of two immiscible fluids in a cross-junction device by using an oil-surfactant system and an oil-surfactant/polymer system. Based on the experimental data, we analyzed the flow regimes and draw flow regime maps of the two systems. Moreover, we established the new scaling laws that include the capillary number, the flow rate ratio, and the viscosity ratio of two phases to predict the droplet diameter or slug length. The findings indicated that there are four flow regimes in the oil-surfactant system, including threading, squeezing, dripping, and jetting regimes. Besides, a new type of flow regime, irregular dripping regime, appears in the oil-surfactant/polymer system. According to the regime maps, the area of dripping regime decreases with the increase of the viscosity of dispersed phase or continuous phase. For both systems, the regression equations with the viscosity ratio have better fitting effect than those without the viscosity ratio. Meanwhile, compared with the effect of viscosity ratio of two phases, the flow rate ratio of two phases has higher influence on droplet diameter and slug length. The experiments present detailed emulsification processes at pore scale and provide new insights for the prediction of emulsion droplets and slugs.</p></div>","PeriodicalId":339,"journal":{"name":"International Journal of Multiphase Flow","volume":null,"pages":null},"PeriodicalIF":3.8,"publicationDate":"2024-06-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141274540","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Deterministic drag modelling for spherical particles in Stokes regime using data-driven approaches 利用数据驱动方法为斯托克斯体系中的球形颗粒建立确定性阻力模型
IF 3.8 2区 工程技术 Q1 Engineering Pub Date : 2024-06-01 DOI: 10.1016/j.ijmultiphaseflow.2024.104880
Hani Elmestikawy , Julia Reuter , Fabien Evrard , Sanaz Mostaghim , Berend van Wachem

In this paper, we develop a deterministic drag model for stationary spherical particles in a Stokes flow using a cascade of data-driven approaches. The model accounts for the variation in drag experienced by each particle within fixed random arrangements. The developed model is a symbolic expression that offers explainability, ease of implementation, and computational efficiency. Firstly, we generate particle-resolved direct numerical simulation data of the flow past periodic random arrangements of stationary spherical particles with volume fractions between 0.05 and 0.4 using the method of regularized Stokeslets. Secondly, we train graph neural networks (GNs) on the generated data to learn the pairwise influence of neighbouring particles on a reference particle. The GNs are converted to symbolic expressions using genetic programming (GP), unveiling repeated subexpressions. Finally, these subexpressions constitute the foundation of the proposed algebraic model, further refined via non-linear regression. The proposed model can qualitatively mimic the pairwise influences as predicted by the GN and can capture the drag variations with accuracy from 74% and up to 84.7% when compared to the particle-resolved simulations. Due to the interpretability of the proposed model, we are able to explore how neighbour positions alter the drag of a particle in an assembly. The proposed model is a promising tool for studying the dynamics of particle assemblies in Stokes flow.

在本文中,我们利用一系列数据驱动方法,为斯托克斯流中的静止球形粒子建立了一个确定性阻力模型。该模型考虑了每个粒子在固定随机排列中的阻力变化。所开发的模型是一种符号表达式,具有可解释性、易于实施和计算效率高等特点。首先,我们使用正则化斯托克斯小方法,生成了经过体积分数在 0.05 和 0.4 之间的周期性随机排列的静止球形粒子的粒子分辨流的直接数值模拟数据。其次,我们在生成的数据上训练图神经网络(GN),以学习相邻粒子对参考粒子的成对影响。使用遗传编程(GP)将图神经网络转换为符号表达式,从而揭示重复的子表达式。最后,这些子表达式构成了拟议代数模型的基础,并通过非线性回归进一步完善。所提出的模型可以定性地模仿 GN 预测的成对影响,并能捕捉阻力变化,与粒子解析模拟相比,准确率从 74% 到 84.7%。由于所提模型的可解释性,我们能够探索相邻位置如何改变装配中粒子的阻力。提出的模型是研究斯托克斯流中粒子集合体动力学的一个很有前途的工具。
{"title":"Deterministic drag modelling for spherical particles in Stokes regime using data-driven approaches","authors":"Hani Elmestikawy ,&nbsp;Julia Reuter ,&nbsp;Fabien Evrard ,&nbsp;Sanaz Mostaghim ,&nbsp;Berend van Wachem","doi":"10.1016/j.ijmultiphaseflow.2024.104880","DOIUrl":"10.1016/j.ijmultiphaseflow.2024.104880","url":null,"abstract":"<div><p>In this paper, we develop a deterministic drag model for stationary spherical particles in a Stokes flow using a cascade of data-driven approaches. The model accounts for the variation in drag experienced by each particle within fixed random arrangements. The developed model is a symbolic expression that offers explainability, ease of implementation, and computational efficiency. Firstly, we generate particle-resolved direct numerical simulation data of the flow past periodic random arrangements of stationary spherical particles with volume fractions between 0.05 and 0.4 using the method of regularized Stokeslets. Secondly, we train graph neural networks (GNs) on the generated data to learn the pairwise influence of neighbouring particles on a reference particle. The GNs are converted to symbolic expressions using genetic programming (GP), unveiling repeated subexpressions. Finally, these subexpressions constitute the foundation of the proposed algebraic model, further refined via non-linear regression. The proposed model can qualitatively mimic the pairwise influences as predicted by the GN and can capture the drag variations with accuracy from 74% and up to 84.7% when compared to the particle-resolved simulations. Due to the interpretability of the proposed model, we are able to explore how neighbour positions alter the drag of a particle in an assembly. The proposed model is a promising tool for studying the dynamics of particle assemblies in Stokes flow.</p></div>","PeriodicalId":339,"journal":{"name":"International Journal of Multiphase Flow","volume":null,"pages":null},"PeriodicalIF":3.8,"publicationDate":"2024-06-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S0301932224001575/pdfft?md5=5d2959f5764662cb99846a6919d91383&pid=1-s2.0-S0301932224001575-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141275278","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Eulerian–Lagrangian multiscale numerical analysis of multimodal partial shedding dynamics 多模态部分脱落动力学的欧拉-拉格朗日多尺度数值分析
IF 3.8 2区 工程技术 Q1 Engineering Pub Date : 2024-06-01 DOI: 10.1016/j.ijmultiphaseflow.2024.104876
Beichen Tian , Biao Huang , Linmin Li , Yue Wu

The objective of this paper is to investigate the multimodal partial shedding dynamics from a multiscale perspective of cloud cavitating flows under two distinct cavity shedding mechanisms, namely the re-entrant jet mechanism and the shock wave propagation mechanism. A two-way Eulerian–Lagrangian coupling algorithm is applied to capture the multiscale vapor topologies from microbubble to large-scale cavities. The large-scale cavity evolution is solved through large eddy simulations (LES) with the volume of fraction (VOF) method in Eulerian frame. The sub-grid microbubbles are tracked in Lagrangian frame based on the discrete bubble model (DBM) method. The predictions agree well with experimental observation of the periodical cavity evolution and microbubble dynamics under both the re-entrant jet mechanism and shock wave mechanism around a NACA66 hydrofoil. The numerical simulation provides detailed analysis of the cavitating turbulent flow on the microbubble behavior with emphasis on the spatial-temporal distribution characteristics of microbubbles. The results show that the number and mean size of microbubbles in the cavitation region increase gradually with the growth of attached sheet cavity, development of re-entrant jet and collapse of largescale cavity for both cavitation patterns. Meanwhile, microbubbles are mainly distributed on the largescale interfaces where have high value of vorticity and turbulent kinetic energy under the effect of re-entrant jet and vortex structures. And the probability density functions (PDFs) of microbubble exhibit gamma distributions with a dominant peak at approximately 50 μm for both shedding mechanisms. However, the shock wave formation and propagation process only occurs in the final stage of cavitating flow under shock wave mechanism causing the condensation of vapor and the decrease of the number and mean size of microbubbles. Moreover, the microbubbles are uniformly distributed along the streamwise and vertical directions behind shock wave front.

本文旨在从多尺度角度研究云空化流在两种不同空穴脱落机制(即再入射机制和冲击波传播机制)下的多模态部分脱落动力学。应用双向欧拉-拉格朗日耦合算法捕捉了从微气泡到大尺度空腔的多尺度水汽拓扑结构。大尺度空腔的演化是通过欧拉框架下的大涡度模拟(LES)和体积分数法(VOF)求解的。在拉格朗日框架下,基于离散气泡模型(DBM)方法对子网格微气泡进行了跟踪。预测结果与围绕 NACA66 水翼的再入射流机制和冲击波机制下的周期性空腔演化和微气泡动力学的实验观测结果非常吻合。数值模拟详细分析了空化湍流对微泡行为的影响,重点研究了微泡的时空分布特征。结果表明,在两种空化模式下,空化区域内的微泡数量和平均尺寸随着附着片空腔的增长、再入射流的发展和大尺度空腔的崩溃而逐渐增大。同时,在再入射流和涡旋结构的作用下,微气泡主要分布在涡度和湍动能值较高的大尺度界面上。在两种脱落机制下,微气泡的概率密度函数(PDF)均呈伽马分布,在约 50 μm 处有一个主峰。然而,冲击波的形成和传播过程只发生在冲击波机制下空化流的最后阶段,导致蒸汽凝结,微气泡的数量和平均尺寸减小。此外,微气泡沿冲击波前沿的流向和垂直方向均匀分布。
{"title":"Eulerian–Lagrangian multiscale numerical analysis of multimodal partial shedding dynamics","authors":"Beichen Tian ,&nbsp;Biao Huang ,&nbsp;Linmin Li ,&nbsp;Yue Wu","doi":"10.1016/j.ijmultiphaseflow.2024.104876","DOIUrl":"10.1016/j.ijmultiphaseflow.2024.104876","url":null,"abstract":"<div><p>The objective of this paper is to investigate the multimodal partial shedding dynamics from a multiscale perspective of cloud cavitating flows under two distinct cavity shedding mechanisms, namely the re-entrant jet mechanism and the shock wave propagation mechanism. A two-way Eulerian–Lagrangian coupling algorithm is applied to capture the multiscale vapor topologies from microbubble to large-scale cavities. The large-scale cavity evolution is solved through large eddy simulations (LES) with the volume of fraction (VOF) method in Eulerian frame. The sub-grid microbubbles are tracked in Lagrangian frame based on the discrete bubble model (DBM) method. The predictions agree well with experimental observation of the periodical cavity evolution and microbubble dynamics under both the re-entrant jet mechanism and shock wave mechanism around a NACA66 hydrofoil. The numerical simulation provides detailed analysis of the cavitating turbulent flow on the microbubble behavior with emphasis on the spatial-temporal distribution characteristics of microbubbles. The results show that the number and mean size of microbubbles in the cavitation region increase gradually with the growth of attached sheet cavity, development of re-entrant jet and collapse of largescale cavity for both cavitation patterns. Meanwhile, microbubbles are mainly distributed on the largescale interfaces where have high value of vorticity and turbulent kinetic energy under the effect of re-entrant jet and vortex structures. And the probability density functions (PDFs) of microbubble exhibit gamma distributions with a dominant peak at approximately 50 μm for both shedding mechanisms. However, the shock wave formation and propagation process only occurs in the final stage of cavitating flow under shock wave mechanism causing the condensation of vapor and the decrease of the number and mean size of microbubbles. Moreover, the microbubbles are uniformly distributed along the streamwise and vertical directions behind shock wave front.</p></div>","PeriodicalId":339,"journal":{"name":"International Journal of Multiphase Flow","volume":null,"pages":null},"PeriodicalIF":3.8,"publicationDate":"2024-06-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141235062","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Mechanism investigation and model assessment of methane flow condensation in minichannels based on numerical simulation 基于数值模拟的微型渠道甲烷流凝结机理研究与模型评估
IF 3.8 2区 工程技术 Q1 Engineering Pub Date : 2024-06-01 DOI: 10.1016/j.ijmultiphaseflow.2024.104887
Yuwei Sun , Haocheng Wang , Feng Nie , Maoqiong Gong

Cryogenic refrigerants represented by methane differ significantly in thermophysical properties from working fluids at ambient temperature. Thus, examining their small-scale heat transfer and flow characteristics is essential for designing compact condensers within the cryogenic field. The numerical simulation of methane condensation in minichannels is conducted, and the process of phase-change mass and energy transfer is investigated by programming. Detailed condensation flow field information is obtained, and surface tension and gravity influences are elucidated. Synergy analysis indicates that the synergy near the tube wall still needs to be improved. Heat transfer performance is proved to be dependent on the relative significance of turbulence intensity and condensate film thickness. The tube inclination exerts a more noticeable influence on the condensation heat transfer for large diameters, which is supported by the dominance of gravity in the condensation heat transfer mechanism at larger diameters. At higher vapor quality and mass flux, the heat transfer enhancement governed by surface tension is more significant. The condensate at the bottom is mainly formed by the accumulation of condensate sliding off the tube top driven by gravity as the diameter increases, reducing the heat transfer region. The mass flux augments the frictional pressure drop more noticeably at high vapor quality. The prediction performance of empirical correlations is evaluated, and all the selected correlations underestimate the frictional pressure drop of methane. Moreover, the figure of merit analysis demonstrates that the pressure drop produced by diameter reduction is more substantial than heat transfer enhancement, suggesting the requirement to assess the pressure drop loss in practical applications.

以甲烷为代表的低温制冷剂的热物理性质与环境温度下的工作流体有很大不同。因此,研究它们的小尺度传热和流动特性对于设计低温领域的紧凑型冷凝器至关重要。本文对甲烷在微型通道中的冷凝进行了数值模拟,并通过编程研究了相变传质和传能过程。获得了详细的冷凝流场信息,并阐明了表面张力和重力的影响。协同作用分析表明,管壁附近的协同作用仍需改进。事实证明,传热性能取决于湍流强度和冷凝液膜厚度的相对重要性。管子的倾斜度对大直径冷凝传热的影响更为明显,这与重力在大直径冷凝传热机制中的主导地位有关。在蒸汽质量和质量通量较高的情况下,表面张力对传热的促进作用更为显著。随着直径的增大,底部的冷凝水主要是由从管顶滑落的冷凝水在重力作用下累积形成的,从而缩小了传热区域。在蒸汽质量较高时,质量通量会更明显地增加摩擦压降。对经验相关性的预测性能进行了评估,所有选定的相关性都低估了甲烷的摩擦压降。此外,优点分析表明,直径减小产生的压降比传热增强产生的压降更大,这表明在实际应用中需要评估压降损失。
{"title":"Mechanism investigation and model assessment of methane flow condensation in minichannels based on numerical simulation","authors":"Yuwei Sun ,&nbsp;Haocheng Wang ,&nbsp;Feng Nie ,&nbsp;Maoqiong Gong","doi":"10.1016/j.ijmultiphaseflow.2024.104887","DOIUrl":"10.1016/j.ijmultiphaseflow.2024.104887","url":null,"abstract":"<div><p>Cryogenic refrigerants represented by methane differ significantly in thermophysical properties from working fluids at ambient temperature. Thus, examining their small-scale heat transfer and flow characteristics is essential for designing compact condensers within the cryogenic field. The numerical simulation of methane condensation in minichannels is conducted, and the process of phase-change mass and energy transfer is investigated by programming. Detailed condensation flow field information is obtained, and surface tension and gravity influences are elucidated. Synergy analysis indicates that the synergy near the tube wall still needs to be improved. Heat transfer performance is proved to be dependent on the relative significance of turbulence intensity and condensate film thickness. The tube inclination exerts a more noticeable influence on the condensation heat transfer for large diameters, which is supported by the dominance of gravity in the condensation heat transfer mechanism at larger diameters. At higher vapor quality and mass flux, the heat transfer enhancement governed by surface tension is more significant. The condensate at the bottom is mainly formed by the accumulation of condensate sliding off the tube top driven by gravity as the diameter increases, reducing the heat transfer region. The mass flux augments the frictional pressure drop more noticeably at high vapor quality. The prediction performance of empirical correlations is evaluated, and all the selected correlations underestimate the frictional pressure drop of methane. Moreover, the figure of merit analysis demonstrates that the pressure drop produced by diameter reduction is more substantial than heat transfer enhancement, suggesting the requirement to assess the pressure drop loss in practical applications.</p></div>","PeriodicalId":339,"journal":{"name":"International Journal of Multiphase Flow","volume":null,"pages":null},"PeriodicalIF":3.8,"publicationDate":"2024-06-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141279490","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Growth of solitary slugs in long pipes 长管道中独居蛞蝓的生长
IF 3.8 2区 工程技术 Q1 Engineering Pub Date : 2024-05-31 DOI: 10.1016/j.ijmultiphaseflow.2024.104883
Roel Belt , Ivar Eskerud Smith , Gunnar Staff , Chris Lawrence

We show that a pipe transporting gas and liquid can be operated at conditions where both stratified flow and slug flow are stable. In this bi-stable flow regime, it is possible to observe stratified flow or regular hydrodynamic slug flow, depending on the inlet conditions. However, it is also possible to get one single slug at a time in the pipe. The distinctive characteristic of such “solitary” slugs is that they grow continuously as they travel along the pipe and therefore, in long pipelines, they can reach lengths up to thousands of pipe diameters and flood the downstream process installations. We first show how the length of solitary slugs can be predicted using slug tracking simulations. Based on those transient simulation results, we provide an explanation for the slug growth and we propose a simple quasi-steady-state model allowing us to predict the slug length in good agreement with the transient simulations. Finally, we explain how we can determine the boundaries of the bi-stable flow regime in which solitary slugs occur.

我们的研究表明,输送气体和液体的管道可以在分层流和蛞蝓流均稳定的条件下运行。在这种双稳定流状态下,可以观察到分层流或规则的水动力蛞蝓流,具体取决于入口条件。不过,也有可能在管道中一次只出现一个蛞蝓。这种 "单个 "蛞蝓的显著特点是,它们在沿着管道移动的过程中不断增长,因此,在长管道中,它们的长度可达数千个管径,并淹没下游工艺装置。我们首先展示了如何通过蛞蝓跟踪模拟来预测孤蛞蝓的长度。在这些瞬态模拟结果的基础上,我们解释了蛞蝓生长的原因,并提出了一个简单的准稳态模型,使我们能够预测蛞蝓长度,并与瞬态模拟结果保持良好一致。最后,我们解释了如何确定发生孤流的双稳态流体的边界。
{"title":"Growth of solitary slugs in long pipes","authors":"Roel Belt ,&nbsp;Ivar Eskerud Smith ,&nbsp;Gunnar Staff ,&nbsp;Chris Lawrence","doi":"10.1016/j.ijmultiphaseflow.2024.104883","DOIUrl":"https://doi.org/10.1016/j.ijmultiphaseflow.2024.104883","url":null,"abstract":"<div><p>We show that a pipe transporting gas and liquid can be operated at conditions where both stratified flow and slug flow are stable. In this bi-stable flow regime, it is possible to observe stratified flow or regular hydrodynamic slug flow, depending on the inlet conditions. However, it is also possible to get one single slug at a time in the pipe. The distinctive characteristic of such “solitary” slugs is that they grow continuously as they travel along the pipe and therefore, in long pipelines, they can reach lengths up to thousands of pipe diameters and flood the downstream process installations. We first show how the length of solitary slugs can be predicted using slug tracking simulations. Based on those transient simulation results, we provide an explanation for the slug growth and we propose a simple quasi-steady-state model allowing us to predict the slug length in good agreement with the transient simulations. Finally, we explain how we can determine the boundaries of the bi-stable flow regime in which solitary slugs occur.</p></div>","PeriodicalId":339,"journal":{"name":"International Journal of Multiphase Flow","volume":null,"pages":null},"PeriodicalIF":3.8,"publicationDate":"2024-05-31","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141291334","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Research on the cavitation flow interference and impact loads of successively launched underwater projectiles 连续发射水下射弹的空化流干扰和冲击载荷研究
IF 3.8 2区 工程技术 Q1 Engineering Pub Date : 2024-05-29 DOI: 10.1016/j.ijmultiphaseflow.2024.104878
Shan Gao , Yao Shi , Shuai Zhang , Guang Pan

The cavitation flow can have a great impact on the projectile's water-exit attitude and stability. At present, the research on cavitation flow is mainly focused on the single projectile, while less research has been conducted on the cavitation flow of projectiles successively launched underwater. In this paper, a verification of the flow simulation method and validation of the cavitation model is presented. The multiphase flow associated with cavitation flows, interference characteristics of the cavitation vortex structure, and load characteristics of the projectiles successively launched underwater are studied. The results show that owing to the flow interference, the attitude of the projectile is deflected to the outside. A large-scale cavity shedding phenomenon of the inside cavity occurs under the incoming flow. A large number of small-scale vortex rings appear above the water surface in the projectile that successively exited the water. As the cavitation number of the projectiles launched successively decreases, the turbulent vortex structure is gradually enriched. In addition, both the inside and the outside are subject to extremely high peak collapse loads. Remarkably, the peak pulsating pressure generated by the collapse of the cavity is strongly correlated with the state of the cavity when the head of the projectile touches the water surface.

空化流对弹丸的出水姿态和稳定性有很大影响。目前,对空化流的研究主要集中在单发弹丸上,对水下连续发射弹丸的空化流研究较少。本文对流动模拟方法进行了验证,并对空化模型进行了验证。研究了与空化流相关的多相流、空化涡结构的干涉特性以及水下连续发射弹丸的载荷特性。结果表明,由于流动干扰,弹丸的姿态向外偏转。在射入流的作用下,内腔出现了大规模的空腔脱落现象。先后出水的弹丸在水面上方出现大量小尺度涡环。随着发射弹丸的空化数逐渐减少,湍流涡旋结构逐渐丰富。此外,内部和外部都承受着极高的峰值坍塌载荷。值得注意的是,空腔塌陷产生的峰值脉动压力与弹丸头部接触水面时的空腔状态密切相关。
{"title":"Research on the cavitation flow interference and impact loads of successively launched underwater projectiles","authors":"Shan Gao ,&nbsp;Yao Shi ,&nbsp;Shuai Zhang ,&nbsp;Guang Pan","doi":"10.1016/j.ijmultiphaseflow.2024.104878","DOIUrl":"https://doi.org/10.1016/j.ijmultiphaseflow.2024.104878","url":null,"abstract":"<div><p>The cavitation flow can have a great impact on the projectile's water-exit attitude and stability. At present, the research on cavitation flow is mainly focused on the single projectile, while less research has been conducted on the cavitation flow of projectiles successively launched underwater. In this paper, a verification of the flow simulation method and validation of the cavitation model is presented. The multiphase flow associated with cavitation flows, interference characteristics of the cavitation vortex structure, and load characteristics of the projectiles successively launched underwater are studied. The results show that owing to the flow interference, the attitude of the projectile is deflected to the outside. A large-scale cavity shedding phenomenon of the inside cavity occurs under the incoming flow. A large number of small-scale vortex rings appear above the water surface in the projectile that successively exited the water. As the cavitation number of the projectiles launched successively decreases, the turbulent vortex structure is gradually enriched. In addition, both the inside and the outside are subject to extremely high peak collapse loads. Remarkably, the peak pulsating pressure generated by the collapse of the cavity is strongly correlated with the state of the cavity when the head of the projectile touches the water surface.</p></div>","PeriodicalId":339,"journal":{"name":"International Journal of Multiphase Flow","volume":null,"pages":null},"PeriodicalIF":3.8,"publicationDate":"2024-05-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141249401","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Dynamic response of the elastic boundary near a single cavitation bubble 单个空化气泡附近弹性边界的动态响应
IF 3.8 2区 工程技术 Q1 Engineering Pub Date : 2024-05-28 DOI: 10.1016/j.ijmultiphaseflow.2024.104884
Qingmiao Ding , Xiaoman Li , Yanyu Cui , Shugang Yang , Longfei Li

We studied the physical mechanism behind the bubble-elastic boundary interaction. In the present paper, three high-speed cameras were used to simultaneously test. Through digital image correlation technology, experimental data were obtained and analyzed, such as elastic boundary deformation. The results revealed that, due to the convex-concave deformation of the elastic boundary, the maximum collapse velocity occurred on both sides of the bubble wall. The deformation of the elastic boundary first increased and then decreased as the initial bubble-boundary distance decreased. We found that the convex deformation of the elastic boundary was exceptional, and nearby was gully, which greatly disturbed the flow field and thus affected the bubble collapse evolution. The boundary deformation velocity was in the shape of a ring, that is, the deformation was transmitted around the boundary in the form of a wave, diffusing energy. Overall, elastic boundary absorbed energy through its own convex-concave deformation, and this energy was transferred to the elastic boundary to alleviate the damage of cavitation bubbles.

我们研究了气泡-弹性边界相互作用背后的物理机制。本文使用三台高速摄像机同时进行测试。通过数字图像相关技术,获得并分析了弹性边界变形等实验数据。结果表明,由于弹性边界的凸凹变形,最大塌陷速度出现在气泡壁的两侧。随着初始气泡边界距离的减小,弹性边界的变形先增大后减小。我们发现,弹性边界的凸形变很特殊,附近有沟壑,这极大地扰乱了流场,从而影响了气泡的塌陷演化。边界形变速度呈环状,即形变以波的形式在边界周围传播,扩散能量。总的来说,弹性边界通过自身的凸凹变形吸收能量,并将能量传递给弹性边界,从而减轻了空化气泡的破坏。
{"title":"Dynamic response of the elastic boundary near a single cavitation bubble","authors":"Qingmiao Ding ,&nbsp;Xiaoman Li ,&nbsp;Yanyu Cui ,&nbsp;Shugang Yang ,&nbsp;Longfei Li","doi":"10.1016/j.ijmultiphaseflow.2024.104884","DOIUrl":"10.1016/j.ijmultiphaseflow.2024.104884","url":null,"abstract":"<div><p>We studied the physical mechanism behind the bubble-elastic boundary interaction. In the present paper, three high-speed cameras were used to simultaneously test. Through digital image correlation technology, experimental data were obtained and analyzed, such as elastic boundary deformation. The results revealed that, due to the convex-concave deformation of the elastic boundary, the maximum collapse velocity occurred on both sides of the bubble wall. The deformation of the elastic boundary first increased and then decreased as the initial bubble-boundary distance decreased. We found that the convex deformation of the elastic boundary was exceptional, and nearby was gully, which greatly disturbed the flow field and thus affected the bubble collapse evolution. The boundary deformation velocity was in the shape of a ring, that is, the deformation was transmitted around the boundary in the form of a wave, diffusing energy. Overall, elastic boundary absorbed energy through its own convex-concave deformation, and this energy was transferred to the elastic boundary to alleviate the damage of cavitation bubbles.</p></div>","PeriodicalId":339,"journal":{"name":"International Journal of Multiphase Flow","volume":null,"pages":null},"PeriodicalIF":3.8,"publicationDate":"2024-05-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141191671","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Physics-aware recurrent convolutional neural networks for modeling multiphase compressible flows 用于多相可压缩流建模的物理感知递归卷积神经网络
IF 3.8 2区 工程技术 Q1 Engineering Pub Date : 2024-05-28 DOI: 10.1016/j.ijmultiphaseflow.2024.104877
Xinlun Cheng , Phong C.H. Nguyen , Pradeep K. Seshadri , Mayank Verma , Zoë J. Gray , Jack T. Beerman , H.S. Udaykumar , Stephen S. Baek

Multiphase compressible flow systems can exhibit unsteady and fast-transient dynamics, marked by sharp gradients and discontinuities, and material boundaries that interact with the evolving flow. The transient nature of the dynamics presents challenges to employing artificial intelligence (AI) and data-driven models for predicting flow behaviors. In this study, we explore the potential of physics-aware recurrent convolutional neural networks (PARC) to model the spatiotemporal dynamics of multiphase flows in the presence of shocks and reaction fronts. PARC is a neural network model that incorporates the generic form of the diffusion–advection–reaction equation in its network architecture, which mimics the process of solving the governing equations of fluid flows. In contrast to physics-informed machine learning approaches such as physics-informed neural networks (PINNs) where models are trained to directly minimize the residual of governing equations, PARC takes a dynamical systems viewpoint and does not seek to minimize potentially nonconvex and nonlinear loss terms. To assess the ability of PARC to accurately learn and simulate the physics of multiphase flows, we train and test PARC on various flow simulation problems, including the Burgers’ equation, fluid flow behind a cylindrical cross-section, and unsteady shock interactions with a particle at varying Mach numbers. We analyze PARC’s performance and examine sources of error in its prediction, in terms of differentiation and integration schemes and different weighting strategies for the model update. Based on our observations, we discuss PARC’s capabilities and limitations in multiphase flow applications and propose future research directions.

多相可压缩流动系统会表现出不稳定和快速瞬态动态,其特征是急剧的梯度和不连续性,以及与不断变化的流动相互作用的材料边界。动力学的瞬态特性给采用人工智能(AI)和数据驱动模型预测流动行为带来了挑战。在本研究中,我们探索了物理感知递归卷积神经网络(PARC)的潜力,以模拟存在冲击和反应锋的多相流的时空动态。PARC 是一种神经网络模型,在其网络结构中纳入了扩散-平流-反应方程的一般形式,模拟了流体流动的管理方程求解过程。与物理信息神经网络(PINNs)等物理信息机器学习方法相比,PARC 从动态系统的角度出发,不寻求最小化潜在的非凸和非线性损失项。为了评估 PARC 准确学习和模拟多相流物理过程的能力,我们在各种流动模拟问题上对 PARC 进行了训练和测试,其中包括布尔格斯方程、圆柱截面后的流体流动以及在不同马赫数下粒子与非定常冲击的相互作用。我们分析了 PARC 的性能,并从微分和积分方案以及模型更新的不同加权策略方面研究了其预测误差的来源。根据观察结果,我们讨论了 PARC 在多相流应用中的能力和局限性,并提出了未来的研究方向。
{"title":"Physics-aware recurrent convolutional neural networks for modeling multiphase compressible flows","authors":"Xinlun Cheng ,&nbsp;Phong C.H. Nguyen ,&nbsp;Pradeep K. Seshadri ,&nbsp;Mayank Verma ,&nbsp;Zoë J. Gray ,&nbsp;Jack T. Beerman ,&nbsp;H.S. Udaykumar ,&nbsp;Stephen S. Baek","doi":"10.1016/j.ijmultiphaseflow.2024.104877","DOIUrl":"10.1016/j.ijmultiphaseflow.2024.104877","url":null,"abstract":"<div><p>Multiphase compressible flow systems can exhibit unsteady and fast-transient dynamics, marked by sharp gradients and discontinuities, and material boundaries that interact with the evolving flow. The transient nature of the dynamics presents challenges to employing artificial intelligence (AI) and data-driven models for predicting flow behaviors. In this study, we explore the potential of physics-aware recurrent convolutional neural networks (PARC) to model the spatiotemporal dynamics of multiphase flows in the presence of shocks and reaction fronts. PARC is a neural network model that incorporates the generic form of the diffusion–advection–reaction equation in its network architecture, which mimics the process of solving the governing equations of fluid flows. In contrast to physics-informed machine learning approaches such as physics-informed neural networks (PINNs) where models are trained to directly minimize the residual of governing equations, PARC takes a dynamical systems viewpoint and does not seek to minimize potentially nonconvex and nonlinear loss terms. To assess the ability of PARC to accurately learn and simulate the physics of multiphase flows, we train and test PARC on various flow simulation problems, including the Burgers’ equation, fluid flow behind a cylindrical cross-section, and unsteady shock interactions with a particle at varying Mach numbers. We analyze PARC’s performance and examine sources of error in its prediction, in terms of differentiation and integration schemes and different weighting strategies for the model update. Based on our observations, we discuss PARC’s capabilities and limitations in multiphase flow applications and propose future research directions.</p></div>","PeriodicalId":339,"journal":{"name":"International Journal of Multiphase Flow","volume":null,"pages":null},"PeriodicalIF":3.8,"publicationDate":"2024-05-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S030193222400154X/pdfft?md5=ff92eaff42909502185eb211e52010ca&pid=1-s2.0-S030193222400154X-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141191820","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Physical correctness of numerical modeling electrohydrodynamic processes in two-phase immiscible liquids basing on the phase-field and arbitrary Lagrangian–Eulerian methods 基于相场和任意拉格朗日-欧勒方法的两相不相溶液体电流体动力过程数值建模的物理正确性
IF 3.8 2区 工程技术 Q1 Engineering Pub Date : 2024-05-27 DOI: 10.1016/j.ijmultiphaseflow.2024.104881
Vladimir Chirkov, Grigorii Utiugov, Petr Kostin, Andrey Samusenko

The paper examines two numerical approaches to the simulation of electrical deformation and coalescence processes in water-in-oil emulsions: the phase-field method and the arbitrary Lagrangian–Eulerian approach. The former employs a diffuse interface, while the latter utilizes a sharp interface. The study analyzes the correctness of the computer simulation results and identifies less obvious limits of the applicability of these numerical techniques. The paper is based on a step-by-step comparison of data from two independent numerical models and quantitative verification using original experimental data, including data on unsteady-state droplet deformation and the threshold between coalescence and non-coalescence. The main findings are as follows. Both methods, the modified phase-field approach and the arbitrary Lagrangian–Eulerian one, are fundamentally capable of providing physically and quantitatively correct results for modeling electrohydrodynamic processes in two-phase immiscible liquids. On the one hand, the phase-field method demands thorough tuning and has limited applicability for simulating long-term processes. On the other hand, the arbitrary Lagrangian–Eulerian approach offers greater precision and requires fewer computational resources compared to the phase-field method, although it demands a manual adjustment of geometry when the system's topology changes. It is noteworthy that the phase-field method, without careful tuning, fails to yield quantitatively accurate results; errors, such as discrepancies in the time convergence of droplets under the influence of an electric field, can reach magnitudes of tens of percentages.

本文研究了模拟油包水型乳液电变形和凝聚过程的两种数值方法:相场法和任意拉格朗日-欧勒法。前者采用扩散界面,后者采用尖锐界面。研究分析了计算机模拟结果的正确性,并确定了这些数值技术在适用性方面不太明显的限制。本文基于对两个独立数值模型数据的逐步比较,并利用原始实验数据(包括非稳态液滴变形数据以及凝聚与非凝聚之间的阈值)进行定量验证。主要发现如下。修正相场法和任意拉格朗日-欧拉法这两种方法都能从根本上为两相不相溶液体的电流体力学过程建模提供物理和定量上正确的结果。一方面,相场方法需要全面调整,对模拟长期过程的适用性有限。另一方面,任意拉格朗日-欧勒方法与相场方法相比,精度更高,所需计算资源更少,但当系统拓扑结构发生变化时,需要手动调整几何形状。值得注意的是,相场法如果不经过仔细调整,就无法得到定量精确的结果;误差,例如液滴在电场影响下的时间收敛差异,可以达到数十个百分点。
{"title":"Physical correctness of numerical modeling electrohydrodynamic processes in two-phase immiscible liquids basing on the phase-field and arbitrary Lagrangian–Eulerian methods","authors":"Vladimir Chirkov,&nbsp;Grigorii Utiugov,&nbsp;Petr Kostin,&nbsp;Andrey Samusenko","doi":"10.1016/j.ijmultiphaseflow.2024.104881","DOIUrl":"10.1016/j.ijmultiphaseflow.2024.104881","url":null,"abstract":"<div><p>The paper examines two numerical approaches to the simulation of electrical deformation and coalescence processes in water-in-oil emulsions: the phase-field method and the arbitrary Lagrangian–Eulerian approach. The former employs a diffuse interface, while the latter utilizes a sharp interface. The study analyzes the correctness of the computer simulation results and identifies less obvious limits of the applicability of these numerical techniques. The paper is based on a step-by-step comparison of data from two independent numerical models and quantitative verification using original experimental data, including data on unsteady-state droplet deformation and the threshold between coalescence and non-coalescence. The main findings are as follows. Both methods, the modified phase-field approach and the arbitrary Lagrangian–Eulerian one, are fundamentally capable of providing physically and quantitatively correct results for modeling electrohydrodynamic processes in two-phase immiscible liquids. On the one hand, the phase-field method demands thorough tuning and has limited applicability for simulating long-term processes. On the other hand, the arbitrary Lagrangian–Eulerian approach offers greater precision and requires fewer computational resources compared to the phase-field method, although it demands a manual adjustment of geometry when the system's topology changes. It is noteworthy that the phase-field method, without careful tuning, fails to yield quantitatively accurate results; errors, such as discrepancies in the time convergence of droplets under the influence of an electric field, can reach magnitudes of tens of percentages.</p></div>","PeriodicalId":339,"journal":{"name":"International Journal of Multiphase Flow","volume":null,"pages":null},"PeriodicalIF":3.8,"publicationDate":"2024-05-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141191840","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Investigation of the minimum filling amount of ionic liquid in the multi-stage ionic liquid compressor 多级离子液体压缩机中离子液体最小填充量的研究
IF 3.8 2区 工程技术 Q1 Engineering Pub Date : 2024-05-25 DOI: 10.1016/j.ijmultiphaseflow.2024.104879
Lingzi Wang , Yiling Liao , He Lv , Yi Guo , Jianmei Feng , Xueyuan Peng

Ionic liquid compressors are the ideal solution for hydrogen refueling stations, and multi-stage compression is an inevitable choice for achieving high-pressure refueling, such as 90 MPa level. However, the initial filling amount of the ionic liquid in the compression chamber is lacking basis as the characteristics of gas-liquid two-phase flow during the reciprocating movement of the liquid piston are not understood. This study numerically investigates the variation characteristics of the gas-liquid interface in the compression chambers under different structural and operating parameters of a five-stage ionic liquid compressor. Based on the fluctuation feature of the phase interface, the minimum liquid piston heights in each stage that ensure effective sealing for the compression chamber with different stroke-to-diameter ratios (r) are determined. Finally, the mathematical relationship for calculating the minimum ionic liquid filling amount related to structural parameter r and suction pressure is established, which provides guidance for the design of the ionic liquid compressor.

离子液体压缩机是加氢站的理想解决方案,多级压缩是实现高压加氢(如 90 兆帕)的必然选择。然而,由于不了解液体活塞往复运动过程中气液两相流动的特点,压缩腔中离子液体的初始充注量缺乏依据。本研究对五级离子液体压缩机在不同结构和运行参数下压缩腔气液界面的变化特征进行了数值研究。根据相界面的波动特征,确定了在不同冲程与直径比(r)的压缩腔中,每级确保有效密封的最小液体活塞高度。最后,建立了计算最小离子液体填充量与结构参数 r 和吸气压力的数学关系,为离子液体压缩机的设计提供了指导。
{"title":"Investigation of the minimum filling amount of ionic liquid in the multi-stage ionic liquid compressor","authors":"Lingzi Wang ,&nbsp;Yiling Liao ,&nbsp;He Lv ,&nbsp;Yi Guo ,&nbsp;Jianmei Feng ,&nbsp;Xueyuan Peng","doi":"10.1016/j.ijmultiphaseflow.2024.104879","DOIUrl":"https://doi.org/10.1016/j.ijmultiphaseflow.2024.104879","url":null,"abstract":"<div><p>Ionic liquid compressors are the ideal solution for hydrogen refueling stations, and multi-stage compression is an inevitable choice for achieving high-pressure refueling, such as 90 MPa level. However, the initial filling amount of the ionic liquid in the compression chamber is lacking basis as the characteristics of gas-liquid two-phase flow during the reciprocating movement of the liquid piston are not understood. This study numerically investigates the variation characteristics of the gas-liquid interface in the compression chambers under different structural and operating parameters of a five-stage ionic liquid compressor. Based on the fluctuation feature of the phase interface, the minimum liquid piston heights in each stage that ensure effective sealing for the compression chamber with different stroke-to-diameter ratios (<em>r</em>) are determined. Finally, the mathematical relationship for calculating the minimum ionic liquid filling amount related to structural parameter <em>r</em> and suction pressure is established, which provides guidance for the design of the ionic liquid compressor.</p></div>","PeriodicalId":339,"journal":{"name":"International Journal of Multiphase Flow","volume":null,"pages":null},"PeriodicalIF":3.8,"publicationDate":"2024-05-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141163635","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
期刊
International Journal of Multiphase Flow
全部 Acc. Chem. Res. ACS Applied Bio Materials ACS Appl. Electron. Mater. ACS Appl. Energy Mater. ACS Appl. Mater. Interfaces ACS Appl. Nano Mater. ACS Appl. Polym. Mater. ACS BIOMATER-SCI ENG ACS Catal. ACS Cent. Sci. ACS Chem. Biol. ACS Chemical Health & Safety ACS Chem. Neurosci. ACS Comb. Sci. ACS Earth Space Chem. ACS Energy Lett. ACS Infect. Dis. ACS Macro Lett. ACS Mater. Lett. ACS Med. Chem. Lett. ACS Nano ACS Omega ACS Photonics ACS Sens. ACS Sustainable Chem. Eng. ACS Synth. Biol. Anal. Chem. BIOCHEMISTRY-US Bioconjugate Chem. BIOMACROMOLECULES Chem. Res. Toxicol. Chem. Rev. Chem. Mater. CRYST GROWTH DES ENERG FUEL Environ. Sci. Technol. Environ. Sci. Technol. Lett. Eur. J. Inorg. Chem. IND ENG CHEM RES Inorg. Chem. J. Agric. Food. Chem. J. Chem. Eng. Data J. Chem. Educ. J. Chem. Inf. Model. J. Chem. Theory Comput. J. Med. Chem. J. Nat. Prod. J PROTEOME RES J. Am. Chem. Soc. LANGMUIR MACROMOLECULES Mol. Pharmaceutics Nano Lett. Org. Lett. ORG PROCESS RES DEV ORGANOMETALLICS J. Org. Chem. J. Phys. Chem. J. Phys. Chem. A J. Phys. Chem. B J. Phys. Chem. C J. Phys. Chem. Lett. Analyst Anal. Methods Biomater. Sci. Catal. Sci. Technol. Chem. Commun. Chem. Soc. Rev. CHEM EDUC RES PRACT CRYSTENGCOMM Dalton Trans. Energy Environ. Sci. ENVIRON SCI-NANO ENVIRON SCI-PROC IMP ENVIRON SCI-WAT RES Faraday Discuss. Food Funct. Green Chem. Inorg. Chem. Front. Integr. Biol. J. Anal. At. Spectrom. J. Mater. Chem. A J. Mater. Chem. B J. Mater. Chem. C Lab Chip Mater. Chem. Front. Mater. Horiz. MEDCHEMCOMM Metallomics Mol. Biosyst. Mol. Syst. Des. Eng. Nanoscale Nanoscale Horiz. Nat. Prod. Rep. New J. Chem. Org. Biomol. Chem. Org. Chem. Front. PHOTOCH PHOTOBIO SCI PCCP Polym. Chem.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1