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Exploring the bubble-electrolyte interplay in membrane electrolyzers: PIV measurement of electrolyte flow regimes 探索膜电解槽中气泡-电解质的相互作用:电解质流动状态的PIV测量
IF 3.8 2区 工程技术 Q1 MECHANICS Pub Date : 2025-11-17 DOI: 10.1016/j.ijmultiphaseflow.2025.105550
Jonas Görtz, Andreas Jupke
Gas-evolving electrochemical processes, such as water-splitting, are heavily affected by the presence of gas bubbles. Detached electrogenerated bubbles alter electrolyte conductivity, and attached bubbles reduce the active electrode surface area. However, due to the complex interaction between gas bubbles and electrolyte flow, estimating gas phase fractions and flow patterns within membrane-separated parallel plate electrolyzers is challenging. Utilizing a partially transparent electrolyzer equipped with a 5k high-speed camera, this work applies particle image velocimetry (PIV) to capture time-averaged detailed flow fields across different current densities, superficial electrolyte velocities, heights, and electrode-membrane gaps. The findings reveal distinct flow regimes transforming from quasi-steady segregated flows under no net flow conditions into pseudo-turbulent flows with increased forced convection. Moreover, variations in current density, superficial electrolyte velocity, and electrode-membrane gap are shown to critically define the upward flow regime’s width and turbulence levels. Out of all studied parameters, we found the superficial electrolyte velocity to be the predominant factor for the width of the bubble curtain. The presented findings support understanding bubble-electrolyte interactions, flow patterns, and gas phase distribution in parallel-plate electrolyzers.
气体演化的电化学过程,如水分解,受到气泡存在的严重影响。分离的电生成气泡改变了电解质的导电性,附着的气泡减少了活性电极的表面积。然而,由于气泡和电解质流动之间复杂的相互作用,估计膜分离平行板电解槽内的气相分数和流动模式是具有挑战性的。利用配备5k高速摄像机的部分透明电解槽,本研究应用粒子图像测速技术(PIV)捕获不同电流密度、表面电解质速度、高度和电极膜间隙的时间平均详细流场。研究结果揭示了不同的流动形式,从无净流条件下的准稳定分离流动转变为强制对流增加的伪湍流流动。此外,电流密度、表面电解质速度和电极-膜间隙的变化对向上流动的宽度和湍流水平有重要影响。在所有研究的参数中,我们发现表面电解质速度是影响气泡幕宽度的主要因素。所提出的发现支持理解气泡-电解质的相互作用,流动模式,并在平行板电解槽气相分布。
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引用次数: 0
Numerical study of particle rolling entrainment in wall turbulence on rough bed 粗糙床壁面湍流中颗粒滚动夹带的数值研究
IF 3.8 2区 工程技术 Q1 MECHANICS Pub Date : 2025-11-17 DOI: 10.1016/j.ijmultiphaseflow.2025.105548
Yicong Zhu, Yan Zhang, Ping Wang
The transport of sediment particles in turbulent flow is widespread in nature. The entrainment of bed particle represents the first step in forming and developing multiphase flow. According to the observed fact that the duration of fluid force acting on the particles is equally significant as its magnitude, event-based entrainment criterions have been developed to analyze the dynamical interactions between the particles and turbulence. However, these models, mainly based on wind tunnel or water channel experiments, only focus on the fluid forces and particle motions in two-dimensional plane (streamwise and vertical). Recent studies highlight the importance of spanwise fluid action, which depends on particle bed arrangement. In this work, the semi-resolved particle Lagrangian tracking method and direct numerical simulation of wall turbulence four-way coupled with particles are employed to simulate the rolling entrainment of individual particles for different bed arrangement and various Shields numbers. The simulation results illustrate that on specific bed arrangement, the spanwise fluid effect cannot be neglected and will lead to none-streamwise rolling entrainment. The fluid structures surrounding the particles during the entrainment process were analyzed, revealing that at lower Shields numbers, sweep events are the primary driving force for particle entrainment. Furthermore, for particles initiating motion in the spanwise direction, the conditional surrounding spanwise velocity field is asymmetrical and the spanwise structures are according the direction of motion. After simplifying the complex three-dimensional force/torque analysis by a projection method, a three-dimensional impulse criterion for particle entrainment was developed and validated by the numerical simulation results.
湍流中泥沙颗粒的输运在自然界中是普遍存在的。床层颗粒的夹带是多相流形成和发展的第一步。根据观察到的作用在粒子上的流体力的持续时间与其大小同等重要的事实,建立了基于事件的夹带准则来分析粒子与湍流之间的动力学相互作用。然而,这些模型主要基于风洞或水道实验,只关注二维平面(流向和垂直)的流体力和粒子运动。最近的研究强调了横向流体作用的重要性,这取决于颗粒床的排列。本文采用半分辨粒子拉格朗日跟踪法和粒子耦合壁面湍流四向直接数值模拟,模拟了不同床层布置和不同屏蔽数下单个粒子的滚动夹带。模拟结果表明,在特定的床层布置下,展向流体效应不可忽视,将导致非流向滚动夹带。分析了颗粒在夹带过程中周围的流体结构,揭示了在较低的屏蔽数下,扫描事件是颗粒夹带的主要驱动力。此外,对于沿展向运动的粒子,条件环绕的展向速度场是不对称的,展向结构是符合运动方向的。采用投影法简化了复杂的三维力/力矩分析,建立了粒子夹带的三维冲量判据,并通过数值模拟结果进行了验证。
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引用次数: 0
The effect of liquid properties on stratified-to-annular transition in a horizontal pipe 液体性质对水平管层向环空过渡的影响
IF 3.8 2区 工程技术 Q1 MECHANICS Pub Date : 2025-11-17 DOI: 10.1016/j.ijmultiphaseflow.2025.105552
Semyon A. Zdornikov, Sergey V. Isaenkov, Andrey V. Cherdantsev
Under low liquid loading, gas-liquid flow in a horizontal pipe has two main flow patterns: stratified and annular flows, which have significantly different integral characteristics such as pressure drop and heat transfer rate. Here we investigate transition between these flow patterns in a horizontal 20 mm pipe using working liquids with different viscosity and surface tension. Backlit visualization with background images is employed to distinguish the flow patterns and measure the height of liquid lifting. Brightness-Based Laser-Induced Fluorescence technique is used to measure film thickness and investigate spatiotemporal evolution of waves on film surface. Several unexpected observations were made. For large gas speeds, both reduced surface tension and increased viscosity facilitate upward climbing of thin liquid film and transition to annular flow. Circumferential spreading of disturbance waves is not directly related to the climbing of thin liquid film, and often shows opposite tendencies regarding the change in liquid properties. Transition to annular flow may occur in absence of disturbance waves, which confirms secondary role of large waves in liquid lifting. The liquid with low surface tension behaves as if it was more viscous, which might be related to intensive entrapment of gas bubbles by the liquid film.
低液载条件下,水平管内气液流动主要有分层流和环空流两种流型,两种流型在压降和换热率等整体特征上存在显著差异。在这里,我们使用不同粘度和表面张力的工作液体研究了水平20毫米管道中这些流动模式之间的转换。采用带背景图像的背光可视化技术识别流体流动模式,测量流体提升高度。利用基于亮度的激光诱导荧光技术测量薄膜厚度,研究薄膜表面波的时空演变。得出了一些意想不到的观察结果。当气体流速较大时,表面张力的降低和粘度的增加都有利于薄液膜向上爬升并过渡到环空流动。扰动波的周向传播与液体薄膜的爬升没有直接关系,而往往与液体性质的变化呈相反的趋势。在没有扰动波的情况下,可能会发生向环空流动的过渡,这证实了大波在液体举升中的次要作用。低表面张力的液体表现出更强的粘性,这可能与液体膜对气泡的密集捕获有关。
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引用次数: 0
Eliminating gas accumulation in horizontal diverging channels under two-phase flow using upstream solid cross-flow steps 采用上游固体横流台阶消除两相流条件下水平分流通道内的天然气聚集
IF 3.8 2区 工程技术 Q1 MECHANICS Pub Date : 2025-11-17 DOI: 10.1016/j.ijmultiphaseflow.2025.105547
Michael Mansour , Mena Shenouda , Nicola Zanini , Dominique Thévenin
Gas accumulation in gas–liquid two-phase flows creates major challenges in centrifugal pumps and diverging channels, as trapped gas in low-pressure separation zones promotes flow separation, reduces pressure recovery, and increases the risk of system failure. To address this, the present study proposes a novel and simple passive control strategy using upstream cross-flow solid steps of varying heights (2, 5, and 8 mm) in a horizontal diverging channel. Controlled experiments combining Laser Doppler Anemometry (LDA), high-speed imaging, and pressure measurements were performed to evaluate the effect of step height on flow separation, bubble behavior, and pressure recovery. Results show that steps of 5 mm and 8 mm could successfully eliminate gas accumulation and significantly improve pressure recovery compared to the baseline without steps, while the 2 mm step had only a marginal effect. These improvements are attributed to enhanced bubble breakup, increased vertical dispersion, and elevated turbulence, while reducing flow separation. The findings not only provide benchmark data for validating two-phase flow models but also offer practical design guidelines for improving gas handling in centrifugal pumps and related industrial systems.
气液两相流中的气体聚集给离心泵和分流通道带来了重大挑战,因为低压分离区中的气体会促进流动分离,降低压力恢复,并增加系统故障的风险。为了解决这个问题,本研究提出了一种新颖而简单的被动控制策略,在水平分流通道中使用不同高度(2、5和8毫米)的上游横流固体台阶。结合激光多普勒风速测量(LDA)、高速成像和压力测量进行控制实验,以评估台阶高度对流动分离、气泡行为和压力恢复的影响。结果表明,与不加台阶的基线相比,5 mm和8 mm台阶可以成功消除天然气聚集,并显著提高压力采收率,而2 mm台阶仅具有边际效果。这些改进归功于增强的气泡破裂、增加的垂直分散和增强的湍流,同时减少了流动分离。这些发现不仅为验证两相流模型提供了基准数据,而且为改善离心泵和相关工业系统的气体处理提供了实用的设计指南。
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引用次数: 0
Experimental study of single bubble rising behavior in an air–water system under parallel wall confinement 平行壁面约束下空气-水系统单泡上升行为的实验研究
IF 3.8 2区 工程技术 Q1 MECHANICS Pub Date : 2025-11-17 DOI: 10.1016/j.ijmultiphaseflow.2025.105549
Liu Liu, Shiming Zhang, Gangliang Liu, Yu Qiu, Dongling Wu, Hongjie Yan
The effect of parallel-wall confinement on single bubble rising dynamics was systematically investigated using the shadowgraph technique. Experiments were performed in rectangular channels under varying degrees of lateral confinement to examine the evolution of bubble aspect ratio, terminal velocity, and drag force. Results reveal that confinement increases the average bubble aspect ratio, which exhibits a strong dependence on the Weber number (We), indicating that bubble deformation is primarily governed by the interplay between inertial and surface tension forces. Terminal velocity decreases significantly with increasing confinement, and for bubbles of equal volume, velocity drops monotonically as the wall spacing (GAP) narrows. Correspondingly, the total drag force increases under stronger confinement. The instantaneous drag shows a clear dependence on both the Reynolds number (Re) and the Eötvös number (Eo), while the time-averaged drag correlates primarily with Eo. Based on the experimental dataset, a predictive model for bubble aspect ratio as a function of We is proposed, which outperforms existing models in terms of generality across a wide range of confinement levels. Furthermore, by introducing a wall-effect correction factor that accounts for Eo and the confinement ratio (s), the proposed terminal velocity model achieves a mean relative error of 6.70%, significantly enhancing its predictive accuracy. Finally, a unified drag force model applicable to both confined and unconfined regimes is developed, offering improved scalability and robustness for engineering applications.
利用影图技术系统地研究了平行壁约束对单泡上升动力学的影响。在不同程度的侧向约束下,在矩形通道中进行了实验,研究了气泡展弦比、终端速度和阻力的演变。结果表明,约束增大了气泡的平均长径比,其与韦伯数(We)有很强的依赖性,表明气泡变形主要由惯性和表面张力之间的相互作用决定。终端速度随约束的增加而显著降低,对于等体积气泡,终端速度随壁面间距(GAP)的减小而单调下降。相应地,在更强的约束条件下,总阻力增大。瞬时阻力明显依赖于雷诺数Re和Eötvös数Eo,而时间平均阻力主要与Eo相关。基于实验数据集,提出了气泡长径比作为We函数的预测模型,该模型在大范围约束水平的通用性方面优于现有模型。此外,通过引入考虑Eo和约束比s的壁效应校正因子,所提出的终端速度模型的平均相对误差为6.70%,显著提高了模型的预测精度。最后,建立了一个适用于受限和非受限工况的统一阻力模型,为工程应用提供了更好的可扩展性和鲁棒性。
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引用次数: 0
Shadowgraphy measurements of bubble jet coupled with surface oscillations 气泡射流与表面振荡耦合的阴影测量
IF 3.8 2区 工程技术 Q1 MECHANICS Pub Date : 2025-11-15 DOI: 10.1016/j.ijmultiphaseflow.2025.105543
Marc Vacher , Tullio Traverso , Christophe Josserand , Stéphane Perrard , Sophie Ramananarivo
We present an image processing method to track and characterize the motion of air–liquid interfaces occurring in aerated liquid baths. In a rectangular tank filled with water, an immersed sparger injects air vertically at a constant flow rate and creates well-defined sloshing oscillations of the free surface. The phenomenon is referred to as self-induced sloshing.
We retrieve the positions of both the surface and the jet position using a tailored image processing method based on shadowgraphy. Using Complex Orthogonal Decomposition (COD), we reveal the main spatial and temporal dynamics of the oscillations.
我们提出了一种图像处理方法来跟踪和表征发生在加气液浴中的气液界面的运动。在一个装满水的矩形水箱中,浸入式喷淋器以恒定的流速垂直注入空气,并在自由表面产生明确的晃动振荡。这种现象被称为自激晃动。我们使用基于阴影术的定制图像处理方法来检索表面和射流位置的位置。利用复正交分解(COD)揭示了振荡的主要时空动力学。
{"title":"Shadowgraphy measurements of bubble jet coupled with surface oscillations","authors":"Marc Vacher ,&nbsp;Tullio Traverso ,&nbsp;Christophe Josserand ,&nbsp;Stéphane Perrard ,&nbsp;Sophie Ramananarivo","doi":"10.1016/j.ijmultiphaseflow.2025.105543","DOIUrl":"10.1016/j.ijmultiphaseflow.2025.105543","url":null,"abstract":"<div><div>We present an image processing method to track and characterize the motion of air–liquid interfaces occurring in aerated liquid baths. In a rectangular tank filled with water, an immersed sparger injects air vertically at a constant flow rate and creates well-defined sloshing oscillations of the free surface. The phenomenon is referred to as self-induced sloshing.</div><div>We retrieve the positions of both the surface and the jet position using a tailored image processing method based on shadowgraphy. Using Complex Orthogonal Decomposition (COD), we reveal the main spatial and temporal dynamics of the oscillations.</div></div>","PeriodicalId":339,"journal":{"name":"International Journal of Multiphase Flow","volume":"195 ","pages":"Article 105543"},"PeriodicalIF":3.8,"publicationDate":"2025-11-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145569374","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
High throughput measurement of bubble coalescence times using digital millifluidics 使用数字微流体的高通量气泡聚结时间测量
IF 3.8 2区 工程技术 Q1 MECHANICS Pub Date : 2025-11-15 DOI: 10.1016/j.ijmultiphaseflow.2025.105544
Ange Combrouze , Alexandra Klimenko , Nicolas Passade-Boupat , Pascal Panizza , François Lequeux , Laurence Talini , Emilie Verneuil
Foams may form in oil mixtures, such as lubricants, as a result of air entrainment. The long lifetimes of those foams significantly impair the thermal properties of lubricants and increase power losses by engines (Zhan et al., 2022). In order to improve the efficiency of lubricants, we offer here to gain insights in the stability of bubbles in binary mixtures of miscible oils as a function of bubble size and liquid composition. To do so, using a micro-millifluidic set-up, we control the formation of bubbles in oil mixtures and study variations in their coalescence time. The set-up allows to easily vary the curvature of the bubbles over one decade, perform statistics over a large number of coalescence events and measure coalescence times that span more than three orders of magnitude.
泡沫可能在油混合物中形成,如润滑油,由于空气夹带。这些泡沫的长寿命显著损害了润滑油的热性能,增加了发动机的功率损失(Zhan et al., 2022)。为了提高润滑油的效率,我们在这里提供了关于气泡大小和液体成分在混相油二元混合物中的稳定性的信息。为此,我们使用微微流体装置控制油混合物中气泡的形成,并研究其聚结时间的变化。该装置可以很容易地在十年内改变气泡的曲率,对大量的聚结事件进行统计,并测量超过三个数量级的聚结时间。
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引用次数: 0
Sound propagation through inhomogeneous and polydisperse bubble clouds: A decoupling approach 声音在非均匀和多分散气泡云中的传播:一种解耦方法
IF 3.8 2区 工程技术 Q1 MECHANICS Pub Date : 2025-11-14 DOI: 10.1016/j.ijmultiphaseflow.2025.105545
Ying Cai , Yunqiao Liu , Benlong Wang , Shu Takagi
Our study explores the effects of bubble–bubble interactions on plane sound wave propagation through spatially inhomogeneous and polydisperse bubbly liquids by extending the idea of bubble screen model (Pham et al., 2021). We introduce a decoupling approach to obtain the acoustic response of a bubble cloud, considering multiple interactions among bubbles. This approach consists of two key steps: firstly, the transformation of the randomly distributed bubble cloud into an organized system, and secondly, the decomposition of the interaction problem within the restructured system. Two distinct interaction mechanisms are identified, namely the intra-layer interactions and inter-layer interactions, corresponding to synchronous and asynchronous collective oscillations respectively. Based on the decoupling approach, we develop a modified effective medium model (MEMM) that demonstrates the different roles played by these interaction mechanisms and enables efficient predictions of acoustic propagation through bubble clouds with random spatial and size distributions. Using two-way coupled Eulerian–Lagrangian simulations, we validate the accuracy of this interaction decoupling for ordered bubble arrays, covering both linear and nonlinear regimes of bubble oscillations. Through discussions on spatial disorder and polydispersity, the applicability of this model is extended to more generalized bubble clouds with nonuniform distributions.
我们的研究通过扩展气泡屏模型的思想,探讨了气泡-气泡相互作用对平面声波在空间非均匀和多分散的气泡液体中传播的影响(Pham et al., 2021)。我们引入了一种解耦方法来获得气泡云的声学响应,考虑了气泡之间的多重相互作用。该方法包括两个关键步骤:首先,将随机分布的气泡云转化为有组织的系统,其次,分解重构系统内的交互问题。确定了两种不同的相互作用机制,即层内相互作用和层间相互作用,分别对应于同步和异步集体振荡。基于解耦方法,我们开发了一个改进的有效介质模型(MEMM),该模型展示了这些相互作用机制所起的不同作用,并能够有效预测具有随机空间和尺寸分布的气泡云中的声波传播。使用双向耦合欧拉-拉格朗日模拟,我们验证了这种相互耦耦对有序气泡阵列的准确性,涵盖了气泡振荡的线性和非线性区域。通过对空间无序性和多分散性的讨论,将该模型的适用性扩展到更广义的非均匀分布气泡云。
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引用次数: 0
Film thickness measurement of film flow discharged from a rectangular nozzle with high aspect ratio 高宽高比矩形喷嘴出膜流的膜厚测量
IF 3.8 2区 工程技术 Q1 MECHANICS Pub Date : 2025-11-14 DOI: 10.1016/j.ijmultiphaseflow.2025.105540
Masaya Saito, Ryuma Kojima, Shigeo Hosokawa
Film thickness distributions of the liquid films discharged from a rectangular nozzle with a high aspect ratio was successfully measured by using the adsorption of light due to the presence of fluorescence dye molecules solved in the liquid film. The measured results indicated that surface tension affects the liquid film thickness, especially in the edge region of the film flow, and that the acceleration of the film flow is higher than the gravitational acceleration.
利用溶解在液膜中的荧光染料分子对光的吸附,成功地测量了高纵横比矩形喷嘴排出液膜的膜厚分布。测量结果表明,表面张力影响液膜厚度,特别是在膜流边缘区域,膜流加速度大于重力加速度。
{"title":"Film thickness measurement of film flow discharged from a rectangular nozzle with high aspect ratio","authors":"Masaya Saito,&nbsp;Ryuma Kojima,&nbsp;Shigeo Hosokawa","doi":"10.1016/j.ijmultiphaseflow.2025.105540","DOIUrl":"10.1016/j.ijmultiphaseflow.2025.105540","url":null,"abstract":"<div><div>Film thickness distributions of the liquid films discharged from a rectangular nozzle with a high aspect ratio was successfully measured by using the adsorption of light due to the presence of fluorescence dye molecules solved in the liquid film. The measured results indicated that surface tension affects the liquid film thickness, especially in the edge region of the film flow, and that the acceleration of the film flow is higher than the gravitational acceleration.</div></div>","PeriodicalId":339,"journal":{"name":"International Journal of Multiphase Flow","volume":"195 ","pages":"Article 105540"},"PeriodicalIF":3.8,"publicationDate":"2025-11-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145569375","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Large-Eddy-Simulation framework for two-phase flows with heat transfer: Application to a two-dimensional jet in cross-flow 大涡流——含传热的两相流的模拟框架:在横流中二维射流中的应用
IF 3.8 2区 工程技术 Q1 MECHANICS Pub Date : 2025-11-13 DOI: 10.1016/j.ijmultiphaseflow.2025.105542
Damien Fouquet, Julien Carmona, Vincent Moureau
This study proposes a Large-Eddy-Simulation framework for two-phase flows with heat transfer that is applied to a two-dimensional Liquid Jet in Cross-flow, a complex configuration with high deformation of the interface, where the framework behaves correctly and is in-line with the expected flow physics.
本研究提出了一个大涡模拟框架,用于两相流动的传热,该框架应用于二维液体射流的交叉流,这是一个具有高界面变形的复杂配置,其中框架表现正确,符合预期的流动物理。
{"title":"Large-Eddy-Simulation framework for two-phase flows with heat transfer: Application to a two-dimensional jet in cross-flow","authors":"Damien Fouquet,&nbsp;Julien Carmona,&nbsp;Vincent Moureau","doi":"10.1016/j.ijmultiphaseflow.2025.105542","DOIUrl":"10.1016/j.ijmultiphaseflow.2025.105542","url":null,"abstract":"<div><div>This study proposes a Large-Eddy-Simulation framework for two-phase flows with heat transfer that is applied to a two-dimensional Liquid Jet in Cross-flow, a complex configuration with high deformation of the interface, where the framework behaves correctly and is in-line with the expected flow physics.</div></div>","PeriodicalId":339,"journal":{"name":"International Journal of Multiphase Flow","volume":"195 ","pages":"Article 105542"},"PeriodicalIF":3.8,"publicationDate":"2025-11-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145517910","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
期刊
International Journal of Multiphase Flow
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