首页 > 最新文献

SPIE NanoScience + Engineering最新文献

英文 中文
Active control of light beam in transformation optics (Presentation Recording) 变换光学中光束的主动控制(演示记录)
Pub Date : 2015-10-05 DOI: 10.1117/12.2186132
Hui Liu
The control of electromagnetic radiation in transformation optical metamaterials brings the development of vast variety of optical devices. Of a particular importance is the possibility to control the propagation of light with light. In this work, we use a structured planar cavity to enhance the thermo-optic effect in a transformation optical waveguide. In the process, a control laser produces apparent inhomogeneous refractive index change inside the waveguides. The trajectory of a second probe laser beam is then continuously tuned in the experiment. The experimental results agree well with the developed theory. The reported method can provide a new approach toward development of transformation optical devices where active all-optical control of the impinging light can be achieved.
光超材料变换过程中电磁辐射的控制带来了各种光学器件的发展。特别重要的是用光来控制光的传播的可能性。在这项工作中,我们使用结构平面腔来增强变换光波导中的热光效应。在此过程中,控制激光器在波导内部产生明显的不均匀折射率变化。然后在实验中对第二个探测激光束的轨迹进行连续调谐。实验结果与所建立的理论相吻合。该方法为实现对入射光的主动全光控制的变换光学器件的研制提供了一条新的途径。
{"title":"Active control of light beam in transformation optics (Presentation Recording)","authors":"Hui Liu","doi":"10.1117/12.2186132","DOIUrl":"https://doi.org/10.1117/12.2186132","url":null,"abstract":"The control of electromagnetic radiation in transformation optical metamaterials brings the development of vast variety of optical devices. Of a particular importance is the possibility to control the propagation of light with light. In this work, we use a structured planar cavity to enhance the thermo-optic effect in a transformation optical waveguide. In the process, a control laser produces apparent inhomogeneous refractive index change inside the waveguides. The trajectory of a second probe laser beam is then continuously tuned in the experiment. The experimental results agree well with the developed theory. The reported method can provide a new approach toward development of transformation optical devices where active all-optical control of the impinging light can be achieved.","PeriodicalId":432358,"journal":{"name":"SPIE NanoScience + Engineering","volume":"12 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2015-10-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"121745340","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Nonlinearities in hyperbolic plasmonic metamaterials (Presentation Recording) 双曲等离子体超材料的非线性(演讲记录)
Pub Date : 2015-10-05 DOI: 10.1117/12.2190133
A. B. Barbosa Neira, Silvia Peruh, Giuseppe Marini, M. Nasir, A. Krasavin, N. Olivier, W. Dickson, G. Wurtz, A. Zayats
We will present experimental studies and numerical modeling of nonlinear optical processes in plasmonic metamaterials based on assemblies of metallic nanorods and other complex geometries. Second- and third-order nonlinear optical response originating from a plasmonic component of the metamaterial will be discussed. Such plasmonic metamaterials can be used for engineering enhanced nonlinear optical properties with the required spectral and temporal response. We will also discuss a novel concept of an on-chip ultrafast all-optical modulator based on a hyperbolic metamaterial integrated in a silicon waveguide.
我们将介绍基于金属纳米棒和其他复杂几何结构的等离子体超材料非线性光学过程的实验研究和数值模拟。将讨论由超材料的等离子体成分引起的二阶和三阶非线性光学响应。这种等离子体超材料可以用于工程上增强非线性光学特性,并具有所需的光谱和时间响应。我们还将讨论基于集成在硅波导中的双曲超材料的片上超快全光调制器的新概念。
{"title":"Nonlinearities in hyperbolic plasmonic metamaterials (Presentation Recording)","authors":"A. B. Barbosa Neira, Silvia Peruh, Giuseppe Marini, M. Nasir, A. Krasavin, N. Olivier, W. Dickson, G. Wurtz, A. Zayats","doi":"10.1117/12.2190133","DOIUrl":"https://doi.org/10.1117/12.2190133","url":null,"abstract":"We will present experimental studies and numerical modeling of nonlinear optical processes in plasmonic metamaterials based on assemblies of metallic nanorods and other complex geometries. Second- and third-order nonlinear optical response originating from a plasmonic component of the metamaterial will be discussed. Such plasmonic metamaterials can be used for engineering enhanced nonlinear optical properties with the required spectral and temporal response. We will also discuss a novel concept of an on-chip ultrafast all-optical modulator based on a hyperbolic metamaterial integrated in a silicon waveguide.","PeriodicalId":432358,"journal":{"name":"SPIE NanoScience + Engineering","volume":"44 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2015-10-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"122088514","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Effect of photonic density of states on spin-flip induced fluorescence contrast in diamond nitrogen-vacancy center ensembles (Presentation Recording) 态光子密度对金刚石氮-空位中心系综自旋翻转诱导荧光对比的影响(演讲记录)
Pub Date : 2015-10-05 DOI: 10.1117/12.2187485
M. Shalaginov, S. Bogdanov, Jing Liu, A. Lagutchev, A. Kildishev, D. Peroulis, J. Irudayaraj, A. Boltasseva, V. Shalaev
Diamond based nitrogen-vacancy (NV) centers are promising solid state defects for applications in quantum information technologies. On the one hand, there is a growing interest in enhancing their single-photon emission by coupling them to plasmonic structures. On the other hand, the dependence of emission intensity on the electron spin state enables room temperature quantum information readout. We study the fluorescence contrast resulting from the spin resonance in the conditions of an increased photonic density of states. Fluorescence observations from NV center ensembles in diamond nanocrystals coupled to structures supporting plasmonic modes experimentally confirm the analytical results.
金刚石基氮空位(NV)中心是量子信息技术中有应用前景的固体缺陷。一方面,人们对通过将它们与等离子体结构耦合来增强它们的单光子发射越来越感兴趣。另一方面,发射强度对电子自旋态的依赖使室温量子信息读出成为可能。我们研究了在增加光子态密度的条件下自旋共振产生的荧光对比。在支持等离子体模式的结构耦合的金刚石纳米晶体中NV中心系综的荧光观测实验证实了分析结果。
{"title":"Effect of photonic density of states on spin-flip induced fluorescence contrast in diamond nitrogen-vacancy center ensembles (Presentation Recording)","authors":"M. Shalaginov, S. Bogdanov, Jing Liu, A. Lagutchev, A. Kildishev, D. Peroulis, J. Irudayaraj, A. Boltasseva, V. Shalaev","doi":"10.1117/12.2187485","DOIUrl":"https://doi.org/10.1117/12.2187485","url":null,"abstract":"Diamond based nitrogen-vacancy (NV) centers are promising solid state defects for applications in quantum information technologies. On the one hand, there is a growing interest in enhancing their single-photon emission by coupling them to plasmonic structures. On the other hand, the dependence of emission intensity on the electron spin state enables room temperature quantum information readout. We study the fluorescence contrast resulting from the spin resonance in the conditions of an increased photonic density of states. Fluorescence observations from NV center ensembles in diamond nanocrystals coupled to structures supporting plasmonic modes experimentally confirm the analytical results.","PeriodicalId":432358,"journal":{"name":"SPIE NanoScience + Engineering","volume":"243 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2015-10-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"124672680","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Semiconductor nanoplatelets: a new colloidal system for low-threshold high-gain stimulated emission (Presentation Recording) 半导体纳米薄片:一种新的低阈值高增益受激发射胶体系统(演讲录音)
Pub Date : 2015-10-05 DOI: 10.1117/12.2186667
M. Pelton, C. She, Igor Fedin, Dmitriy S. Dolzhnikov, S. Ithurria, Erfan Baghani, S. O’Leary, A. Demortière, R. Schaller, D. Talapin
Quantum wells (QWs) are thin semiconductor layers than confine electrons and holes in one dimension. They are widely used for optoelectronic devices, particularly semiconductor lasers, but have so far been produced using expensive epitaxial crystal-growth techniques. This has motivated research into the use of colloidal semiconductor nanocrystals, which can be synthesized chemically at low cost, and can be processed in the solution phase. However, initial demonstrations of optical gain from colloidal nanocrystals involved high thresholds. Recently, colloidal synthesis methods have been developed for the production of thin, atomically flat semiconductor nanocrystals, known as nanoplatelets (NPLs). We investigated relaxation of high-energy carriers in colloidal CdSe NPLs, and found that the relaxation is characteristic of a QW system. Carrier cooling and relaxation on time scales from picoseconds to hundreds of picoseconds are dominated by Auger-type exciton-exciton interactions. The picosecond-scale cooling of hot carriers is much faster than the exciton recombination rate, as required for use of these NPLs as optical gain and lasing materials. We therefore investigated amplified spontaneous emission using close-packed films of NPLs. We observed thresholds that were more than 4 times lower than the best reported value for colloidal nanocrystals. Moreover, gain in these films is 4 times higher than gain reported for other colloidal nanocrystals, and saturates at pump fluences more than two orders of magnitude above the ASE threshold. We attribute this exceptional performance to large optical cross-sections, relatively slow Auger recombination rates, and narrow ensemble emission linewidths.
量子阱是一种将电子和空穴限制在一维空间内的薄半导体层。它们广泛用于光电子器件,特别是半导体激光器,但迄今为止都是使用昂贵的外延晶体生长技术生产的。这激发了对胶体半导体纳米晶体使用的研究,这种纳米晶体可以用低成本的化学方法合成,并且可以在溶液中加工。然而,胶体纳米晶体的光学增益的初始演示涉及高阈值。最近,胶体合成方法已被开发用于生产薄的,原子平面的半导体纳米晶体,称为纳米片(NPLs)。我们研究了胶体CdSe NPLs中高能载流子的弛豫,发现弛豫是量子阱系统的特征。在皮秒到数百皮秒的时间尺度上,载流子的冷却和弛豫主要是由俄歇型激子-激子相互作用控制的。热载流子的皮秒级冷却比激子复合速率快得多,这是使用这些NPLs作为光学增益和激光材料所需要的。因此,我们利用不良贷款的致密薄膜研究了放大的自发辐射。我们观察到的阈值比胶体纳米晶体的最佳报道值低4倍以上。此外,这些薄膜的增益比其他胶体纳米晶体的增益高4倍,并且在泵浦影响下比ASE阈值高两个数量级以上。我们将这种特殊的性能归因于大的光学截面,相对较慢的俄歇复合率和较窄的系综发射线宽。
{"title":"Semiconductor nanoplatelets: a new colloidal system for low-threshold high-gain stimulated emission (Presentation Recording)","authors":"M. Pelton, C. She, Igor Fedin, Dmitriy S. Dolzhnikov, S. Ithurria, Erfan Baghani, S. O’Leary, A. Demortière, R. Schaller, D. Talapin","doi":"10.1117/12.2186667","DOIUrl":"https://doi.org/10.1117/12.2186667","url":null,"abstract":"Quantum wells (QWs) are thin semiconductor layers than confine electrons and holes in one dimension. They are widely used for optoelectronic devices, particularly semiconductor lasers, but have so far been produced using expensive epitaxial crystal-growth techniques. This has motivated research into the use of colloidal semiconductor nanocrystals, which can be synthesized chemically at low cost, and can be processed in the solution phase. However, initial demonstrations of optical gain from colloidal nanocrystals involved high thresholds. Recently, colloidal synthesis methods have been developed for the production of thin, atomically flat semiconductor nanocrystals, known as nanoplatelets (NPLs). We investigated relaxation of high-energy carriers in colloidal CdSe NPLs, and found that the relaxation is characteristic of a QW system. Carrier cooling and relaxation on time scales from picoseconds to hundreds of picoseconds are dominated by Auger-type exciton-exciton interactions. The picosecond-scale cooling of hot carriers is much faster than the exciton recombination rate, as required for use of these NPLs as optical gain and lasing materials. We therefore investigated amplified spontaneous emission using close-packed films of NPLs. We observed thresholds that were more than 4 times lower than the best reported value for colloidal nanocrystals. Moreover, gain in these films is 4 times higher than gain reported for other colloidal nanocrystals, and saturates at pump fluences more than two orders of magnitude above the ASE threshold. We attribute this exceptional performance to large optical cross-sections, relatively slow Auger recombination rates, and narrow ensemble emission linewidths.","PeriodicalId":432358,"journal":{"name":"SPIE NanoScience + Engineering","volume":"9545 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2015-10-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"129971028","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Effect of substrate surface free energy on the optoelectronic and morphological properties of organolead halide perovskite solar cell materials (Presentation Recording) 衬底表面自由能对有机卤化铅钙钛矿太阳能电池材料光电性能和形态性能的影响(演讲记录)
Pub Date : 2015-10-05 DOI: 10.1117/12.2188843
R. C. Shallcross, James G. Stanfill, N. Armstrong
Here, we show how the surface free energy of the electron-collecting oxide contact has a very pronounced effect on the nucleation free energy of solution-processed organolead halide perovskite thin films, which influences the crystal size/orientation, band-edge energies, conductivity and, ultimately, the performance of solar cell devices. While a great deal of the research community’s attention has been focused on the perovskite deposition methodology (e.g., starting precursors, annealing conditions, etc.), we demonstrate how the surface free energy of the oxide contact itself can be modified to control morphology and optoelectronic properties of the resulting hybrid perovskite thin films. The surface free energy of high-quality oxide contacts deposited by chemical vapor deposition (CVD) and atomic layer deposition (ALD) is modified by functionalization with a variety of self-assembled monolayers. We explore a number of deposition methodologies (e.g., a variety of single step and sequential step approaches) and their effect on the morphological and electronic properties of the resulting perovskite thin films deposited on these modified oxide contacts. Standard atomic force microscopy (AFM) and its conductive analog (cAFM) show how the oxide surface free energy ultimately affects the nanoscale morphology and charge transport characteristics of these semiconductor films. Photoelectron spectroscopy is used to elucidate the chemical composition (e.g., X-ray photoelectron spectroscopy - XPS), band edge energies (e.g., ultraviolet photoelectron spectroscopy - UPS), and the presence of gap states above the valence band (high sensitivity UPS measurements near the Fermi energy) of the hybrid perovskite materials as a function of the oxide surface free energy.
在这里,我们展示了收集电子的氧化物接触的表面自由能如何对溶液处理的有机卤化铅钙钛矿薄膜的成核自由能产生非常显著的影响,从而影响晶体尺寸/取向、带边能量、电导率,并最终影响太阳能电池器件的性能。虽然研究界的大量注意力都集中在钙钛矿沉积方法上(例如,起始前驱体,退火条件等),但我们展示了如何修改氧化物接触本身的表面自由能来控制所得到的杂化钙钛矿薄膜的形貌和光电性能。采用化学气相沉积(CVD)和原子层沉积(ALD)制备的高质量氧化触点的表面自由能被各种自组装的单层功能化修饰。我们探索了多种沉积方法(例如,各种单步和顺序步骤方法)以及它们对沉积在这些修饰氧化物触点上的钙钛矿薄膜的形态和电子特性的影响。标准原子力显微镜(AFM)及其导电模拟物(cAFM)显示了氧化物表面自由能最终如何影响这些半导体薄膜的纳米级形貌和电荷输运特性。光电子能谱用于阐明混合钙钛矿材料的化学成分(例如,x射线光电子能谱- XPS),能带边缘能量(例如,紫外光电子能谱- UPS),以及价带以上的间隙态(接近费米能的高灵敏度UPS测量)作为氧化物表面自由能的函数。
{"title":"Effect of substrate surface free energy on the optoelectronic and morphological properties of organolead halide perovskite solar cell materials (Presentation Recording)","authors":"R. C. Shallcross, James G. Stanfill, N. Armstrong","doi":"10.1117/12.2188843","DOIUrl":"https://doi.org/10.1117/12.2188843","url":null,"abstract":"Here, we show how the surface free energy of the electron-collecting oxide contact has a very pronounced effect on the nucleation free energy of solution-processed organolead halide perovskite thin films, which influences the crystal size/orientation, band-edge energies, conductivity and, ultimately, the performance of solar cell devices. While a great deal of the research community’s attention has been focused on the perovskite deposition methodology (e.g., starting precursors, annealing conditions, etc.), we demonstrate how the surface free energy of the oxide contact itself can be modified to control morphology and optoelectronic properties of the resulting hybrid perovskite thin films. The surface free energy of high-quality oxide contacts deposited by chemical vapor deposition (CVD) and atomic layer deposition (ALD) is modified by functionalization with a variety of self-assembled monolayers. We explore a number of deposition methodologies (e.g., a variety of single step and sequential step approaches) and their effect on the morphological and electronic properties of the resulting perovskite thin films deposited on these modified oxide contacts. Standard atomic force microscopy (AFM) and its conductive analog (cAFM) show how the oxide surface free energy ultimately affects the nanoscale morphology and charge transport characteristics of these semiconductor films. Photoelectron spectroscopy is used to elucidate the chemical composition (e.g., X-ray photoelectron spectroscopy - XPS), band edge energies (e.g., ultraviolet photoelectron spectroscopy - UPS), and the presence of gap states above the valence band (high sensitivity UPS measurements near the Fermi energy) of the hybrid perovskite materials as a function of the oxide surface free energy.","PeriodicalId":432358,"journal":{"name":"SPIE NanoScience + Engineering","volume":"15 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2015-10-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"130003496","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
Two layer metamaterials for selective frequency transmission in the terahertz region (Presentation Recording) 用于太赫兹区域选择性频率传输的两层超材料(演示记录)
Pub Date : 2015-10-05 DOI: 10.1117/12.2188966
M. Landau
We have fabricated a metamaterial tunable filter for dynamic frequency selection in the terahertz region. The metamaterial consists of a sandwich of two meta-surfaces grown on high resistivity silicon wafers. The first meta-surface consists of a two-dimensional array of gold double split ring resonators and the second meta-surface consisits of an array of gold cut rods. Both meta-surfaces are fabricated for a response in the terahertz region. Our terahertz pulses are produced using the standard Austin switch technique. The terahertz pulse is focused onto the two meta-surfaces which are sandwiched together to produce a transmission window. Together, with the right orientation, translation, and parallelism of the two meta-surfaces, we achieve filtering of terahertz pulses. Since the unit cells for the inclusions are on the order of 100 microns, control of the translation, orientation, and parallelism of the two meta-surfaces with respect to each other and with respect to the orientation and direction of the impinging terahertz field is a challenge. We describe our technique for doing this and present data on our frequency filtering in the terahertz.
我们制作了一个用于太赫兹区域动态频率选择的超材料可调谐滤波器。这种超材料由生长在高电阻硅晶片上的两个超表面组成。第一元表面由金双裂环谐振器的二维阵列组成,第二元表面由金切割棒阵列组成。这两种元表面都是为太赫兹区域的响应而制造的。我们的太赫兹脉冲是用标准的奥斯汀开关技术产生的。太赫兹脉冲聚焦在两个被夹在一起的元表面上,形成一个传输窗口。结合两个元表面的正确方向、平移和平行度,我们实现了太赫兹脉冲的滤波。由于内含物的单元格在100微米量级,因此控制两个元表面相对于彼此以及相对于撞击太赫兹场的方向和方向的平移、方向和平行度是一个挑战。我们描述了我们的技术,并介绍了我们在太赫兹频率滤波的数据。
{"title":"Two layer metamaterials for selective frequency transmission in the terahertz region (Presentation Recording)","authors":"M. Landau","doi":"10.1117/12.2188966","DOIUrl":"https://doi.org/10.1117/12.2188966","url":null,"abstract":"We have fabricated a metamaterial tunable filter for dynamic frequency selection in the terahertz region. The metamaterial consists of a sandwich of two meta-surfaces grown on high resistivity silicon wafers. The first meta-surface consists of a two-dimensional array of gold double split ring resonators and the second meta-surface consisits of an array of gold cut rods. Both meta-surfaces are fabricated for a response in the terahertz region. Our terahertz pulses are produced using the standard Austin switch technique. The terahertz pulse is focused onto the two meta-surfaces which are sandwiched together to produce a transmission window. Together, with the right orientation, translation, and parallelism of the two meta-surfaces, we achieve filtering of terahertz pulses. Since the unit cells for the inclusions are on the order of 100 microns, control of the translation, orientation, and parallelism of the two meta-surfaces with respect to each other and with respect to the orientation and direction of the impinging terahertz field is a challenge. We describe our technique for doing this and present data on our frequency filtering in the terahertz.","PeriodicalId":432358,"journal":{"name":"SPIE NanoScience + Engineering","volume":"3 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2015-10-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"134169734","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Second-harmonic generation in an atomic phase-matched nonlinear 2D crystal (Presentation Recording) 原子相位匹配非线性二维晶体的二次谐波产生(呈现记录)
Pub Date : 2015-10-05 DOI: 10.1117/12.2187575
Mervin Zhao, Ziliang Ye, Yu Ye, Hanyu Zhu, Yuan Wang, Y. Iwasa, Xiang Zhang
The second harmonic generation (SHG) produced from two-dimensional atomic crystals have been utilized recently in studying the grain boundaries and electronic structure of such ultra-thin materials. However, the SHG in many of these crystals, such as transition metal dichalcogenides (TMDCs), only occur in odd numbered layers with limited intensity due to their noncentrosymmetric nature. Here, we probe the SHG from the bulk noncentrosymmetric molybdenum disulfide (MoS2). Whereas the commonly studied 2H crystal phase’s anti-parallel nonlinear dipoles in adjacent layers give an oscillatory SH response, the parallel nonlinear dipoles of each atomic layer in the 3R phase constructively interfere to amplify the nonlinear light. Due to this interference, we observed the atomically phase-matched condition yielding a quadratic dependence between the intensity and layer number. Additionally, we probed the layer evolution of the A and B excitonic transitions in 3R-MoS2 using SHG spectroscopy and found distinct electronic structure differences arising from the crystal geometry. These findings demonstrate the dramatic effect of the symmetry and layer stacking of these atomic crystals.
二维原子晶体产生的二次谐波(SHG)最近被用于研究这类超薄材料的晶界和电子结构。然而,在许多这些晶体中,如过渡金属二硫族化物(TMDCs),由于它们的非中心对称性质,SHG只出现在奇数层中,强度有限。在这里,我们探测了非中心对称二硫化钼(MoS2)的SHG。通常研究的2H相相邻层的反平行非线性偶极子会产生振荡的SH响应,而3R相各原子层的平行非线性偶极子会产生相振干涉,放大非线性光。由于这种干扰,我们观察到原子相位匹配条件在强度和层数之间产生二次依赖关系。此外,我们利用SHG光谱探测了3R-MoS2中A和B激子跃迁的层演化,发现晶体几何形状引起了明显的电子结构差异。这些发现证明了这些原子晶体的对称性和层堆叠的巨大影响。
{"title":"Second-harmonic generation in an atomic phase-matched nonlinear 2D crystal (Presentation Recording)","authors":"Mervin Zhao, Ziliang Ye, Yu Ye, Hanyu Zhu, Yuan Wang, Y. Iwasa, Xiang Zhang","doi":"10.1117/12.2187575","DOIUrl":"https://doi.org/10.1117/12.2187575","url":null,"abstract":"The second harmonic generation (SHG) produced from two-dimensional atomic crystals have been utilized recently in studying the grain boundaries and electronic structure of such ultra-thin materials. However, the SHG in many of these crystals, such as transition metal dichalcogenides (TMDCs), only occur in odd numbered layers with limited intensity due to their noncentrosymmetric nature. Here, we probe the SHG from the bulk noncentrosymmetric molybdenum disulfide (MoS2). Whereas the commonly studied 2H crystal phase’s anti-parallel nonlinear dipoles in adjacent layers give an oscillatory SH response, the parallel nonlinear dipoles of each atomic layer in the 3R phase constructively interfere to amplify the nonlinear light. Due to this interference, we observed the atomically phase-matched condition yielding a quadratic dependence between the intensity and layer number. Additionally, we probed the layer evolution of the A and B excitonic transitions in 3R-MoS2 using SHG spectroscopy and found distinct electronic structure differences arising from the crystal geometry. These findings demonstrate the dramatic effect of the symmetry and layer stacking of these atomic crystals.","PeriodicalId":432358,"journal":{"name":"SPIE NanoScience + Engineering","volume":"44 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2015-10-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"133523687","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Metasurface-enabled quantum vacuum effects over macroscopic distances (Presentation Recording) 宏观距离上的超表面量子真空效应(演示记录)
Pub Date : 2015-10-05 DOI: 10.1117/12.2187434
P. Jha, X. Ni, Chihhui Wu, Y. Wang, Xiang Zhang
Quantum vacuum engineering is an active field of research. Here we use recent advances in the field of metasurface (2D-array of sub-wavelength scale nano-antennas) to construct an anisotropic quantum vacuum (AQV) in the vicinity of a quantum emitter located at some macroscopic distance from the metasurface. Such AQV can induce quantum interference among several atomic transitions, even when the transition dipole moment corresponding to the decay channels are orthogonal. Recently, there have been few theoretical proposal to use metamaterials to engineer the back-action. All these approaches, which works in the near field (few tens of nanometers from the surface), suffers from trapping an atom at these distance, surface interactions like quenching, Casimir force etc. Hence it’s pivotal to construct the back-action over macroscopic distance. We harness the polarization dependent response of a metasurface to engineer the back-action of the spontaneous emission from the atom to itself. We show strong anisotropy in the decay rate of a quantum emitter which is a manifestation of AQV. Engineering light-matter interaction over macroscopic distances opens new possibilities for long-range interaction between quantum emitters for quantum information processing, spin-optics/spintronics etc.
量子真空工程是一个活跃的研究领域。本文利用超表面(亚波长尺度纳米天线的二维阵列)领域的最新进展,在距离超表面一定宏观距离的量子发射极附近构建了各向异性量子真空(AQV)。这种AQV可以诱导几个原子跃迁之间的量子干涉,即使与衰变通道对应的跃迁偶极矩是正交的。近年来,很少有利用超材料来设计反作用力的理论建议。所有这些在近场(距离表面几十纳米)工作的方法,都受到在这些距离捕获原子、表面相互作用(如淬火、卡西米尔力等)的困扰。因此,构造宏观距离上的反作用是关键。我们利用超表面的偏振相关响应来设计原子对自身自发发射的反向作用。我们发现量子发射极的衰减速率具有很强的各向异性,这是AQV的一种表现。在宏观距离上设计光物质相互作用为量子发射体之间的远程相互作用开辟了新的可能性,用于量子信息处理、自旋光学/自旋电子学等。
{"title":"Metasurface-enabled quantum vacuum effects over macroscopic distances (Presentation Recording)","authors":"P. Jha, X. Ni, Chihhui Wu, Y. Wang, Xiang Zhang","doi":"10.1117/12.2187434","DOIUrl":"https://doi.org/10.1117/12.2187434","url":null,"abstract":"Quantum vacuum engineering is an active field of research. Here we use recent advances in the field of metasurface (2D-array of sub-wavelength scale nano-antennas) to construct an anisotropic quantum vacuum (AQV) in the vicinity of a quantum emitter located at some macroscopic distance from the metasurface. Such AQV can induce quantum interference among several atomic transitions, even when the transition dipole moment corresponding to the decay channels are orthogonal. Recently, there have been few theoretical proposal to use metamaterials to engineer the back-action. All these approaches, which works in the near field (few tens of nanometers from the surface), suffers from trapping an atom at these distance, surface interactions like quenching, Casimir force etc. Hence it’s pivotal to construct the back-action over macroscopic distance. We harness the polarization dependent response of a metasurface to engineer the back-action of the spontaneous emission from the atom to itself. We show strong anisotropy in the decay rate of a quantum emitter which is a manifestation of AQV. Engineering light-matter interaction over macroscopic distances opens new possibilities for long-range interaction between quantum emitters for quantum information processing, spin-optics/spintronics etc.","PeriodicalId":432358,"journal":{"name":"SPIE NanoScience + Engineering","volume":"58 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2015-10-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"132794882","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
PT-symmetric scatterers (Presentation Recording) pt对称散射体(演示记录)
Pub Date : 2015-10-05 DOI: 10.1117/12.2189863
M. Miri, Nicholas S. Nye, M. Khajavikhan, D. Christodoulides
Parity-time (PT) symmetric complex structures can exhibit peculiar properties which are otherwise unattainable in traditional Hermitian systems. This is achieved by judiciously involving balanced regions of gain and loss. Here we investigate the scattering properties of PT-symmetric diffraction gratings. The presence of the imaginary potential can modify the light transport properties in their far field. This is an outcome of a local power flow taking place between the gain and loss regions in the near field. We show that for a certain gain/loss contrast, all the negative diffraction orders can be eliminated while the positive diffraction orders can be amplified.
奇偶时(PT)对称复杂结构可以表现出在传统厄米系统中无法达到的特殊性质。这是通过明智地涉及得失平衡区域来实现的。本文研究了pt对称衍射光栅的散射特性。虚势的存在可以改变光在远场的输运特性。这是在近场增益和损耗区域之间发生的局部功率流的结果。结果表明,在一定的增益/损耗对比下,所有负衍射阶可以消除,而正衍射阶可以放大。
{"title":"PT-symmetric scatterers (Presentation Recording)","authors":"M. Miri, Nicholas S. Nye, M. Khajavikhan, D. Christodoulides","doi":"10.1117/12.2189863","DOIUrl":"https://doi.org/10.1117/12.2189863","url":null,"abstract":"Parity-time (PT) symmetric complex structures can exhibit peculiar properties which are otherwise unattainable in traditional Hermitian systems. This is achieved by judiciously involving balanced regions of gain and loss. Here we investigate the scattering properties of PT-symmetric diffraction gratings. The presence of the imaginary potential can modify the light transport properties in their far field. This is an outcome of a local power flow taking place between the gain and loss regions in the near field. We show that for a certain gain/loss contrast, all the negative diffraction orders can be eliminated while the positive diffraction orders can be amplified.","PeriodicalId":432358,"journal":{"name":"SPIE NanoScience + Engineering","volume":"14 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2015-10-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"133040538","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Hydrodynamics of micro-objects near curved surfaces (Presentation Recording) 曲面附近微物体的流体力学(演示记录)
Pub Date : 2015-10-05 DOI: 10.1117/12.2190312
Shu Zhang, D. Carberry, T. Nieminen, H. Rubinsztein-Dunlop
Boundary walls have a strong influence on the drag force on optically trapped object near surface. Faxen’s correction has shown how a flat surface modifies the hydrodynamic drag. However, to date, the effect of curved walls at microscopic scale on both translational and rotational movement of micro-objects has not been studied. Here we describe our experiments which aim to study the drag force on optically trapped particles moving near walls with different curvatures. The curved walls were made using 3D laser nano-printing (Nanoscribe), and optical tweezers were used to trap micro-objects near the walls. The translational and rotational motion of the optically trapped particle is related to the drag coefficients. By monitoring the change in the motion of particle, we determined the increase in drag force for particles translating or rotating at different distances from surfaces with different curvatures. These results are essential for calibrating the drag force on particles, and thus enable accurate rheology at the micron-scale. This opens the potential for microrheology under different conditions, such as within microdevices, biological cells and studies of biological processes
边界壁面对近表面光捕获物体的阻力有较大的影响。Faxen的修正显示了平坦的表面是如何改变流体动力阻力的。然而,迄今为止,微观尺度上的弯曲壁对微观物体的平移和旋转运动的影响尚未得到研究。本文描述了我们的实验,目的是研究在不同曲率的壁面附近运动的光捕获粒子的阻力。利用三维激光纳米打印技术(Nanoscribe)制作出弯曲的壁面,并用光学镊子捕获壁面附近的微物体。光捕获粒子的平移和旋转运动与阻力系数有关。通过监测质点运动的变化,我们确定了质点在不同曲率表面上平移或旋转不同距离时阻力的增加。这些结果对于校准颗粒上的阻力至关重要,从而实现微米尺度上的精确流变。这为不同条件下的微流变学开辟了潜力,例如在微设备、生物细胞和生物过程的研究中
{"title":"Hydrodynamics of micro-objects near curved surfaces (Presentation Recording)","authors":"Shu Zhang, D. Carberry, T. Nieminen, H. Rubinsztein-Dunlop","doi":"10.1117/12.2190312","DOIUrl":"https://doi.org/10.1117/12.2190312","url":null,"abstract":"Boundary walls have a strong influence on the drag force on optically trapped object near surface. Faxen’s correction has shown how a flat surface modifies the hydrodynamic drag. However, to date, the effect of curved walls at microscopic scale on both translational and rotational movement of micro-objects has not been studied. Here we describe our experiments which aim to study the drag force on optically trapped particles moving near walls with different curvatures. The curved walls were made using 3D laser nano-printing (Nanoscribe), and optical tweezers were used to trap micro-objects near the walls. The translational and rotational motion of the optically trapped particle is related to the drag coefficients. By monitoring the change in the motion of particle, we determined the increase in drag force for particles translating or rotating at different distances from surfaces with different curvatures. These results are essential for calibrating the drag force on particles, and thus enable accurate rheology at the micron-scale. This opens the potential for microrheology under different conditions, such as within microdevices, biological cells and studies of biological processes","PeriodicalId":432358,"journal":{"name":"SPIE NanoScience + Engineering","volume":"50 1","pages":"0"},"PeriodicalIF":0.0,"publicationDate":"2015-10-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"116718314","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
期刊
SPIE NanoScience + Engineering
全部 Acc. Chem. Res. ACS Applied Bio Materials ACS Appl. Electron. Mater. ACS Appl. Energy Mater. ACS Appl. Mater. Interfaces ACS Appl. Nano Mater. ACS Appl. Polym. Mater. ACS BIOMATER-SCI ENG ACS Catal. ACS Cent. Sci. ACS Chem. Biol. ACS Chemical Health & Safety ACS Chem. Neurosci. ACS Comb. Sci. ACS Earth Space Chem. ACS Energy Lett. ACS Infect. Dis. ACS Macro Lett. ACS Mater. Lett. ACS Med. Chem. Lett. ACS Nano ACS Omega ACS Photonics ACS Sens. ACS Sustainable Chem. Eng. ACS Synth. Biol. Anal. Chem. BIOCHEMISTRY-US Bioconjugate Chem. BIOMACROMOLECULES Chem. Res. Toxicol. Chem. Rev. Chem. Mater. CRYST GROWTH DES ENERG FUEL Environ. Sci. Technol. Environ. Sci. Technol. Lett. Eur. J. Inorg. Chem. IND ENG CHEM RES Inorg. Chem. J. Agric. Food. Chem. J. Chem. Eng. Data J. Chem. Educ. J. Chem. Inf. Model. J. Chem. Theory Comput. J. Med. Chem. J. Nat. Prod. J PROTEOME RES J. Am. Chem. Soc. LANGMUIR MACROMOLECULES Mol. Pharmaceutics Nano Lett. Org. Lett. ORG PROCESS RES DEV ORGANOMETALLICS J. Org. Chem. J. Phys. Chem. J. Phys. Chem. A J. Phys. Chem. B J. Phys. Chem. C J. Phys. Chem. Lett. Analyst Anal. Methods Biomater. Sci. Catal. Sci. Technol. Chem. Commun. Chem. Soc. Rev. CHEM EDUC RES PRACT CRYSTENGCOMM Dalton Trans. Energy Environ. Sci. ENVIRON SCI-NANO ENVIRON SCI-PROC IMP ENVIRON SCI-WAT RES Faraday Discuss. Food Funct. Green Chem. Inorg. Chem. Front. Integr. Biol. J. Anal. At. Spectrom. J. Mater. Chem. A J. Mater. Chem. B J. Mater. Chem. C Lab Chip Mater. Chem. Front. Mater. Horiz. MEDCHEMCOMM Metallomics Mol. Biosyst. Mol. Syst. Des. Eng. Nanoscale Nanoscale Horiz. Nat. Prod. Rep. New J. Chem. Org. Biomol. Chem. Org. Chem. Front. PHOTOCH PHOTOBIO SCI PCCP Polym. Chem.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1