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Bioventing in Shallow Tundra Overlying Permafrost 冻土上浅层冻土带的生物通风
Pub Date : 1998-09-01 DOI: 10.1080/10588339891334474
D. White, R. Irvine
The purpose of this research was to investigate the feasibility of suction bioventing for treatment of contaminated tundra soil. Two laboratory-scale venting reactors were prepared with tundra from Arctic Alaska and operated, one for 32 d and the other for 52 d. For each rectangular reactor, suction was applied to a central well screened at mid-depth, while opposite ends of the reactor were screened to serve as air intake zones. The volume of liquid and gas recovered from the suction well was quantified daily. Numbers for heterotrophic organisms, pH, and dissolved organic carbon were quantified in the recovered liquid. The suction pump held a full vacuum (i.e., 101 kPa vac) for the duration of both experiments, indicating continuous obstruction of pneumatic and hydraulic conductivity. In both reactors, the soil in the proximity of the suction well separated from the bulk of the soil, precluding hydraulic communication. Furthermore, the soil nearest the well screen compacted, forming a barrier to appreciab...
本研究的目的是探讨吸式生物通气处理冻土带污染土壤的可行性。用阿拉斯加北极地区的冻土带制备了两个实验室规模的通风反应器,一个运行32 d,另一个运行52 d。对于每个矩形反应器,将吸力施加于中间深度屏蔽的中央井,而反应器的两端被屏蔽作为进气区。每天定量从抽吸井中回收的液体和气体的体积。对回收液中异养生物、pH和溶解有机碳的数量进行了量化。在两个实验期间,吸入泵保持全真空(即101 kPa vac),表明气动和水力传导持续受阻。在两个反应器中,靠近吸力井的土壤与大部分土壤分离,阻止了水力通信。此外,离筛管最近的土壤被压实,形成了一个屏障,阻挡了采油。
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引用次数: 1
Potential of Phytoremediation for Treatment of PAHs in Soil at MGP Sites 植物修复处理MGP站点土壤中多环芳烃的潜力
Pub Date : 1998-07-01 DOI: 10.1080/10588339891334401
S. Pradhan, J. Conrad, J. Paterek, V. Srivastava
Phytoremediation is a natural, aesthetically pleasing, low-cost technology that employs plant-influenced microbial, chemical, and physical processes to remediate contaminated soils and waters. The Institute of Gas Technology (IGT) conducted a laboratory study to determine the potential of phytoremediation to remediate soils contaminated with polynuclear aromatic hydrocarbons (PAHs). The soils used for the study were collected from a former manufactured gas plant (MGP) site in Newark, NJ. Phytoremediation was assessed both as a primary remediation technology and as a final polishing step for soil treatment. The following three plant species were used for the 6-month laboratory study: alfalfa (Medicago sativa), switch grass (Panicum virgatum), and little bluestem grass (Schizachyrium scoparium). Using both alfalfa and switch grass for primary treatment of PAH-contaminated soil, a 57% reduction in total PAH concentration was observed after 6-months of treatment. Final polishing of that soil using alfalfa fur...
植物修复是一种自然的、美观的、低成本的技术,它利用植物影响的微生物、化学和物理过程来修复受污染的土壤和水。气体技术研究所(IGT)进行了一项实验室研究,以确定植物修复修复被多核芳烃(PAHs)污染的土壤的潜力。用于研究的土壤是从新泽西州纽瓦克的一个前人造气厂(MGP)收集的。植物修复被评价为主要的修复技术和土壤处理的最后抛光步骤。在为期6个月的实验室研究中,采用了苜蓿(Medicago sativa)、柳枝草(Panicum virgatum)和小蓝茎草(Schizachyrium scoparium) 3种植物。采用苜蓿和曲枝草对多环芳烃污染土壤进行初步处理,处理6个月后,多环芳烃总浓度降低了57%。最后用紫花苜蓿打磨土壤……
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引用次数: 180
Phytoremediation of Organic Contaminants: A Review of Phytoremediation Research at the University of Washington 有机污染物的植物修复:华盛顿大学植物修复研究综述
Pub Date : 1998-07-01 DOI: 10.1080/10588339891334366
L. Newman, S. Doty, Katrina L. Gery, P. Heilman, I. Muiznieks, T. Q. Shang, Sarah T. Siemieniec, S. Strand, Xiaoping Wang, Angela M Wilson, M. Gordon
As overwhelmingly positive results have become available regarding the ability of plants to degrade compounds such as trichloroethylene, phytoremediation studies are expanding. Studies to determine the potential for phytoremediation of fully chlorinated compounds, such as carbon tetrachloride and tetrachloroethylene, brominated compounds, such as ethylene dibromide and dibromochloropropane, and nonhalogenated compounds, such as methyl-t-butyl ether (MTBE), are underway. When using phytoremediation, it is important to select not only a plant that is capable of degrading the pollutant in question, but also one that will grow well in that specific environment. In ecologically sensitive areas, such as the Hawaiian Islands, only plants native to the area can be used. One way to supplement the arsenal of plants available for remedial actions is to utilize genetic engineering tools to insert into plants those genes that will enable the plant to metabolize a particular pollutant. Hybrid technologies, such as usin...
由于关于植物降解三氯乙烯等化合物的能力已经取得了压倒性的积极结果,植物修复研究正在扩大。目前正在进行研究,以确定植物修复全氯化化合物(如四氯化碳和四氯乙烯)、溴化化合物(如二溴乙烯和二溴氯丙烷)和非卤化化合物(如甲基-t-丁基醚)的潜力。在使用植物修复时,重要的是不仅要选择能够降解污染物的植物,而且要选择能够在特定环境中生长良好的植物。在生态敏感地区,比如夏威夷群岛,只能使用当地的原生植物。补充可用于补救行动的植物库的一种方法是利用基因工程工具将那些使植物能够代谢特定污染物的基因插入植物中。混合技术,例如使用…
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引用次数: 92
Natural Attenuation of Trichloroethylene in Rhizosphere Soils at the Savannah River Site 萨凡纳河遗址根际土壤中三氯乙烯的自然衰减
Pub Date : 1998-07-01 DOI: 10.1080/10588339891334429
R. Brigmon, N. C. Bell, D. Freedman, C. Berry
Extensive trichloroethylene (TCE) groundwater contamination has resulted from discharges to a former seepage basin in the A/M Area at the Department of Energy's Savannah River Site. The direction of groundwater flow has been determined and a seep line where the contaminated groundwater is estimated to emerge as surface water has been identified in a region of the Southern Sector of the A/M Area. This study was undertaken to estimate the potential of four rhizosphere soils along the seep line to naturally attenuate TCE. Microcosms were setup to evaluate both biotic and abiotic attenuation of TCE. Results demonstrated that sorption to soil was the dominant mechanism during the first week of incubation, with as much as 90% of the TCE removed from the aqueous phase. Linear partitioning coefficients (Kd) ranged from 0.83 to 7.4 mL/g, while organic carbon partition coefficients (Koc) ranged from 72 to 180 mL/gC. Diffu-sional losses from the microcosms appeared to be a dominant fate mechanism during the remainde...
大量三氯乙烯(TCE)地下水污染是由于排放到能源部萨凡纳河遗址a /M地区的前渗流盆地造成的。已经确定了地下水的流向,并在a /M区南段的一个地区确定了一条渗水线,估计受污染的地下水将以地表水的形式出现。本研究旨在评估沿渗漏线的四种根际土壤自然衰减TCE的潜力。建立了微环境来评估TCE的生物和非生物衰减。结果表明,在培养的第一周,对土壤的吸附是主要机制,高达90%的TCE从水相中去除。线性分配系数(Kd)为0.83 ~ 7.4 mL/g,有机碳分配系数(Koc)为72 ~ 180 mL/gC。从微观世界的扩散损失似乎是一个主要的命运机制在剩余的…
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引用次数: 45
PHYTOREMEDIATION: CURRENT VIEWS ON AN EMERGING GREEN TECHNOLOGY 植物修复:对一项新兴绿色技术的看法
Pub Date : 1998-07-01 DOI: 10.1080/10588339891334438
P. Flathman, G. Lanza
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引用次数: 256
Selenium Accumulation by Brassica Napus Grown in Se-Laden Soil From Different Depths of Kesterson Reservoir 凯斯特森水库不同深度富硒土壤中甘蓝型油菜的硒积累
Pub Date : 1998-07-01 DOI: 10.1080/10588339891334393
G. Bañuelos, H. Ajwa, Lin Wu, S. Zambrzuski
Selenium (Se) may be present in soils and sediments in high concentrations and yet not be mobile or available for plant uptake. Phytoremediation of Se by canola (Brassica napus) was evaluated in sediment from Kesterson Reservoir at three different depths (0 to 30, 30 to 60, 60 to 90 cm) under greenhouse and field conditions. In the greenhouse study, total soil Se concentrations at preplant ranged from 10 to 112 mg kg−1. Shoot Se concentrations of canola were 182, 53, and 19 mg kg−1 DM in the 0 to 30, 30 to 60, and 60 to 90 cm depths, respectively. Percentages of Se accumulated by canola relative to total Se loss in the soil at postharvest were as high as 24%. In the field study, total soil Se concentrations were as high as 26 mg kg−1 soil. Field-grown canola accumulated approximately 50 mg kg−1 DM, which accounted for less than 10% of total Se lost in the soil at postharvest. Phytoremediation of Se-laden soils under field conditions was about 50% of that observed under controlled greenhouse conditions. Th...
硒(Se)可能以高浓度存在于土壤和沉积物中,但不能移动或供植物吸收。在温室和田间条件下,研究了油菜对Kesterson水库沉积物中不同深度(0 ~ 30cm、30 ~ 60cm、60 ~ 90cm)硒的修复作用。在温室研究中,植前土壤全硒浓度为10 ~ 112 mg kg−1。在0 ~ 30cm、30 ~ 60cm和60 ~ 90cm深度,油菜茎部硒浓度分别为182、53和19 mg kg−1 DM。采后油菜积累硒量占土壤总硒损失的比例高达24%。在田间研究中,土壤总硒浓度高达26 mg kg - 1。田间种植的油菜积累了约50 mg kg - 1 DM,占采后土壤总硒损失的不到10%。大田条件下植物对含硒土壤的修复效果约为温室控制条件下的50%。Th……
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引用次数: 33
Phytoremediation of Mercury- and Methylmercury-Polluted Soils Using Genetically Engineered Plants 利用基因工程植物修复汞和甲基汞污染土壤
Pub Date : 1998-07-01 DOI: 10.1080/10588339891334384
Andrew C. P. Heaton, C. L. Rugh, Nian-jie Wang, R. Meagher
Inorganic mercury in contaminated soils and sediments is relatively immobile, though biological and chemical processes can transform it to more toxic and bioavailable methylmercury. Methylmercury is neurotoxic to vertebrates and is biomagnified in animal tissues as it is passed from prey to predator. Traditional remediation strategies for mercury contaminated soils are expensive and site-destructive. As an alternative we propose the use of transgenic aquatic, salt marsh, and upland plants to remove available inorganic mercury and methylmercury from contaminated soils and sediments. Plants engineered with a modified bacterial mercuric reductase gene, merA, are capable of converting Hg(II) taken up by roots to the much less toxic Hg(0), which is volatilized from the plant. Plants engineered to express the bacterial organo-mercurial lyase gene, merB, are capable of converting methylmercury taken up by plant roots into sulfhydryl-bound Hg(II). Plants expressing both genes are capable of converting ionic mercu...
受污染土壤和沉积物中的无机汞是相对不流动的,尽管生物和化学过程可以将其转化为毒性更强、生物可利用性更高的甲基汞。甲基汞对脊椎动物具有神经毒性,当它从猎物传递到捕食者时,在动物组织中会被生物放大。传统的汞污染土壤修复策略既昂贵又具有破坏性。作为一种替代方案,我们建议使用转基因水生、盐沼和旱地植物来去除污染土壤和沉积物中的无机汞和甲基汞。经过改良的细菌汞还原酶基因merA改造的植物能够将根吸收的汞(II)转化为毒性小得多的汞(0),后者从植物中挥发出来。表达细菌有机汞裂解酶基因merB的植物能够将植物根部吸收的甲基汞转化为巯基结合的汞(II)。表达这两种基因的植物能够转化离子汞。
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引用次数: 191
Phytoremediation of No. 2 fuel oil-contaminated soil. 2号燃料油污染土壤的植物修复
Pub Date : 1998-07-01 DOI: 10.1080/10588339891334410
E. Carman, Tom L. Crossman, E. Gatliff
Phytoremediation has been implemented at an industrial site in Wisconsin to promote in situ remediation of No. 2 fuel oil-contaminated soil. The goal of the project is to utilize microbial-enhancing processes within the rhizosphere of trees to stimulate biodegradation of diesel range organics (DROs) within four contaminated hot spots at the site. Between 40 and 90% reductions in the concentrations of the DROs were observed over the course of a 24-week bench-scale bioventing study performed in 1994. In addition to a reduction in the concentration of DROs, the chromatograms for those analyses exhibited a relative decrease in the proportion of the more water soluble and available shorter chained or lower molecular weight DROs compared to their higher molecular weight counterparts in the fuel. In addition to a decrease in concentration, this observed change in the pattern of the chromatograms over time is consistent with biodegradation of DROs. An agronomic assessment performed in 1995 indicated that conditio...
植物修复已在威斯康星州的一个工业场地实施,以促进2号燃料油污染土壤的原位修复。该项目的目标是利用树木根际内的微生物增强过程来刺激现场四个污染热点内柴油范围有机物(DROs)的生物降解。在1994年进行的一项为期24周的试验性生物排放研究中,观察到DROs浓度降低了40%至90%。除了DROs的浓度降低之外,这些分析的色谱图显示,与燃料中分子量较高的DROs相比,水溶性更强、可用的短链或低分子量DROs的比例相对减少。除了浓度下降外,观察到的色谱模式随时间的变化与DROs的生物降解一致。1995年进行的一项农艺评估表明……
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引用次数: 40
Phytotreatment of TNT-Contaminated Groundwater tnt污染地下水的植物处理
Pub Date : 1998-07-01 DOI: 10.1080/10588339891334375
R. Rivera, V. Medina, S. Larson, S. McCutcheon
Phytoremediation is a viable technique for treating nitroaromatic compounds, particularly munitions. Continuous flow phyto-reactor studies were conducted at the following three influent concentrations of 2,4,6-trinitrotoluene (TNT): 1, 5, and 10 ppm. A control was also prepared with an influent TNT concentration of 5 ppm. Flow rates were systematically reduced to increase hydraulic retention times (HRT) which ranged from 12 to 76 days. Initially, the control reactor removed TNT as efficiently as the plant reactors. With time, however, the efficiency of the control became less than that of the plant reactors, suggesting that adsorption was initially the mechanism for removal. Up to 100% of the TNT was removed. Aminodinitrotoluene (ADNT) effluent concentration was higher for higher TNT influent concentrations. Increasing the retention time reduced ADNT concentration in the effluent. Supplementary batch studies confirmed that ADNT and diaminonitrotoluene (DANT) were phytodegraded. Preliminary batch studies w...
植物修复是处理硝基芳香族化合物特别是军需品的一种可行技术。连续流动植物反应器研究在以下三种输入浓度的2、4、6-三硝基甲苯(TNT)下进行:1、5和10 ppm。还制备了输入TNT浓度为5ppm的对照物。系统地降低流量以增加水力滞留时间(HRT),其范围从12天到76天不等。最初,控制反应堆与核电站反应堆一样有效地去除了TNT。然而,随着时间的推移,控制的效率变得低于工厂反应器的效率,这表明吸附最初是去除的机制。高达100%的TNT被清除。TNT浓度越高,氨二硝基甲苯(ADNT)出水浓度越高。延长停留时间可降低出水中ADNT的浓度。补充批量研究证实ADNT和二氨基硝基甲苯(DANT)被植物降解。初步批量研究…
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引用次数: 43
Numerical Simulations and Long-Column Tests of LNAPL Displacement and Trapping by a Fluctuating Water Table 波动水位对LNAPL位移和捕获的数值模拟和长柱试验
Pub Date : 1998-05-01 DOI: 10.1080/10588339891334294
D. Steffy, C. Johnston, D. Barry
Long-column laboratory tests were performed to validate improvements to the MOFAT program for simulating LNAPL displacement and entrapment in response to a fluctuating water table. The long-column tests consisted of a fluctuating water table and its subsequent displacement and entrapment of an LNAPL. The modifications of MOFAT include a linear LNAPL trapping estimate and a new scaling technique for the inhibition portion of the fluctuation (water table rise). Improved prediction of the LNAPL trapping was obtained by assuming the amount of LNAPL that is trapped by a rising water table is proportional to the antecedent water content of the porous medium. The pressure- saturation relationship for the air- water drainage system was scaled to estimate the LNAPL- water and air-LNAPL drainage relationships. Scaled inhibition pressure- saturation relationships are improved by incorporating a correction for contact angle hysteresis and surface roughness. The incorporation of these changes into MOFAT led to noticable improvements in the numerical simulation of the experimental data.
进行了长柱实验室测试,以验证MOFAT程序的改进,以模拟LNAPL位移和夹持,以响应波动的地下水位。长柱试验包括波动的地下水位及其随后的位移和LNAPL的夹持。MOFAT的改进包括线性LNAPL捕获估计和对波动抑制部分(地下水位上升)的新标度技术。通过假设地下水位上升所捕获的LNAPL量与孔隙介质先前的含水量成正比,可以改进对LNAPL捕获的预测。对空气-水排水系统的压力-饱和度关系进行了缩放,以估计LNAPL-水和空气-LNAPL排水关系。通过结合对接触角滞后和表面粗糙度的校正,改进了阻垢压力-饱和度关系。将这些变化纳入MOFAT后,实验数据的数值模拟得到了显著改善。
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引用次数: 34
期刊
Journal of Soil Contamination
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