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Analysis for the ARIANE BM1 and BM3 samples: nuclide inventory and decay heat 阿丽亚娜BM1和BM3样品的分析:核素库存和衰变热
IF 0.5 Q3 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2021-01-01 DOI: 10.1051/epjn/2021017
D. Rochman, A. Vasiliev, H. Ferroukhi, M. Hursin
The Mixed Oxide samples (MOX) ARIANE Post Irradiation Examination samples BM1 and BM3 have been analyzed in this work, based on various two- and three-dimensional models. Calculated and measured nuclide inventories are compared based on CASMO5, SIMULATE and SNF simulations, and calculated values for the decay heat of the assembly containing the samples are also provided. For uncertainty propagation, the covariance information from three different nuclear data libraries are used. Uncertainties from manufacturing tolerances and operating conditions are also considered. The results from these two samples are compared with the ones from two UO2 samples, namely GU1 and GU3, also from the ARIANE program, applying the same calculation scheme and uncertainty assumptions. It is shown that a two-dimensional assembly model provides better agreement with the measurements than a two-dimensional single pin model, and that the full core three-dimensional model provides similar results compared to the assembly model, although no 148Nd normalization is applied for the full core model. For the MOX assembly decay heat, as expected, heavy actinides have a higher contribution compared to the cases with the UO2 samples; additionally, decay heat uncertainties are moderately smaller in the case of the MOX assembly.
本文基于各种二维和三维模型,对混合氧化物样品(MOX) ARIANE辐照后检测样品BM1和BM3进行了分析。基于CASMO5、simulation和SNF模拟,比较了核素库存的计算值和实测值,并给出了包含样品的组件的衰变热的计算值。对于不确定性传播,使用了来自三个不同核数据库的协方差信息。还考虑了制造公差和操作条件的不确定性。采用相同的计算方案和不确定性假设,将这两个样本的结果与同样来自ARIANE项目的两个UO2样本GU1和GU3的结果进行了比较。结果表明,二维装配模型比二维单针模型更符合测量结果,全岩心三维模型与装配模型的结果相似,尽管全岩心模型没有应用148Nd归一化。对于MOX组装衰变热,与UO2样品相比,重锕系元素的贡献更高;此外,在MOX组件的情况下,衰变热不确定性相对较小。
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引用次数: 5
Nuclear data assimilation, scientific basis and current status 核资料同化、科学依据及现状
IF 0.5 Q3 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2021-01-01 DOI: 10.1051/EPJN/2021008
E. Ivanov, Cyrille De Saint-Jean, V. Sobes
The use of Data Assimilation methodologies, known also as a data adjustment, liaises the results of theoretical and experimental studies improving an accuracy of simulation models and giving a confidence to designers and regulation bodies. From the mathematical point of view, it approaches an optimized fit to experimental data revealing unknown causes by known consequences that would be crucial for data calibration and validation. Data assimilation adds value in a ND evaluation process, adjusting nuclear data to particular application providing so-called optimized design-oriented library, calibrating nuclear data involving IEs since all theories and differential experiments provide the only relative values, and providing an evidence-based background for validation of Nuclear data libraries substantiating the UQ process. Similarly, it valorizes experimental data and the experiments, as such involving them in a scientific turnover extracting essential information inherently contained in legacy and newly set up experiments, and prioritizing dedicated basic experimental programs. Given that a number of popular algorithms, including deterministic like Generalized Linear Least Square methodology and stochastic ones like Backward and Hierarchic or Total Monte-Carlo, Hierarchic Monte-Carlo, etc., being different in terms of particular numerical formalism are, though, commonly grounded on the Bayesian theoretical basis. They demonstrated sufficient maturity, providing optimized design-oriented data libraries or evidence-based backgrounds for a science-driven validation of general-purpose libraries in a wide range of practical applications.
数据同化方法的使用,也称为数据调整,将理论和实验研究的结果联系起来,提高了模拟模型的准确性,并给设计者和监管机构带来了信心。从数学的角度来看,它接近于实验数据的优化拟合,通过已知的结果揭示未知的原因,这对数据校准和验证至关重要。数据同化在ND评估过程中增加了价值,根据特定应用调整核数据,提供所谓的优化设计导向库,校准涉及IEs的核数据,因为所有理论和差异实验都提供了唯一的相对值,并为证实UQ过程的核数据库的验证提供了循证背景。同样,它对实验数据和实验进行评估,从而使它们参与科学周转,提取遗留和新建立的实验中固有的基本信息,并优先考虑专门的基础实验计划。鉴于许多流行的算法,包括确定性的,如广义线性最小二乘方法和随机的,如向后和层次或总蒙特卡罗,层次蒙特卡罗等,在特定的数值形式方面不同,但是,通常以贝叶斯理论为基础。它们展示了足够的成熟度,为在广泛的实际应用中科学驱动的通用库验证提供了优化的面向设计的数据库或基于证据的背景。
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引用次数: 1
Pu multi-recycling scenarios towards a PWR fleet for a stabilization of spent fuel inventories in France 为稳定法国的乏燃料库存,向压水堆机群提供了多种回收方案
IF 0.5 Q3 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2021-01-01 DOI: 10.1051/epjn/2021022
F. Courtin, Camille Laguerre, Philippe Miranda, C. Chabert, G. Martin
Nuclear scenario studies are performed to explore the impact of possible evolutions of nuclear fleets. The nuclear fuel cycle simulation tool COSI, developed by CEA, is used to model these dynamic scenarios and to evaluate them with respect to uranium and plutonium management, fuel reprocessing and waste production. In recent years, scenarios have focused on transitions from the current nuclear French fleet to a deployment of SFR. However, the French Multi-annual Energy Planning has recently postponed the deployment of this technology to the second half of the 21st century. Alternative solutions of plutonium management in PWR are investigated to stabilize total inventories of spent nuclear fuels. The MIX concept is based on homogeneous fuel assemblies where fuel rods are composed of plutonium blended with enriched uranium. In this study, a transition from the current French fleet to an EPR™ fleet is simulated. Two power capacities of the future EPR™ fleet are considered. A progressive deployment of fuel multi-recycling in the EPR™ fleet is implemented to enable stabilization of all spent fuels and plutonium inventories. Natural uranium consumption is also minimized thanks to ERU fuel batches in EPR™. Results are compared with plutonium and uranium mono-recycling in a PWR fleet.
进行核情景研究以探索核舰队可能演变的影响。由CEA开发的核燃料循环模拟工具COSI用于模拟这些动态情景,并在铀和钚管理、燃料后处理和废物产生方面对它们进行评价。近年来,方案的重点是从目前的法国核舰队过渡到部署SFR。然而,法国的多年度能源规划最近将这项技术的部署推迟到21世纪下半叶。研究了压水堆钚管理的备选方案,以稳定乏燃料总库存。MIX概念基于均质燃料组件,其中燃料棒由混合了浓缩铀的钚组成。在这项研究中,模拟了从目前的法国舰队到EPR™舰队的过渡。考虑了未来EPR™机队的两种功率容量。在EPR™机群中逐步部署燃料多重回收,以稳定所有乏燃料和钚库存。由于EPR™中的ERU燃料批次,天然铀的消耗也最小化。结果与压水堆中钚和铀的单一回收进行了比较。
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引用次数: 2
Effects of the initial granular structure of clay sealing materials on their swelling properties: experiments and DEM simulations 粘土密封材料初始颗粒结构对其膨胀性能的影响:实验和DEM模拟
IF 0.5 Q3 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2020-11-01 DOI: 10.1051/epjn/2019059
B. Dardé, A. Tang, J. Roux, P. Dangla, Jean-Michel Pereira, J. Talandier, M. Vu
Pellet-based expansive clay materials are considered as a sealing material for closing the galleries in radioactive waste disposal concepts. In repository conditions, the granular mixture progressively homogenises upon hydration by the host rock pore water. The present study focuses on the material behaviour before homogenisation. A grain-scale experimental characterisation is first performed in the laboratory. A model describing the hydromechanical behaviour of a pellet is proposed based on the experimental results. Then, suction-controlled swelling pressure tests are performed in the laboratory. Using Discrete Element Method (DEM) and the model proposed for a single pellet, the tests are successfully simulated. It is highlighted that (i) the swelling pressure evolves in two phases in the investigated suction range, controlled by the granular structure of the mixture; (ii) wall effects at the laboratory scale affects the material response; (iii) measurement variability associated to the sensor diameter is non-negligible; (iv) DEM is a valuable tool able to provide insight into the material behaviour.
在放射性废物处理概念中,颗粒基膨胀粘土材料被认为是封闭通道的密封材料。在储存库条件下,颗粒混合物在宿主岩石孔隙水的水合作用下逐渐均质。本研究的重点是均质化前的材料行为。首先在实验室中进行颗粒尺度的实验表征。基于实验结果,提出了一个描述球团流体力学行为的模型。然后,在实验室中进行抽吸控制膨胀压力测试。利用离散单元法(DEM)和针对单个颗粒提出的模型,成功地模拟了试验。强调指出:(i)在所研究的吸力范围内,膨胀压力分为两个阶段,由混合物的颗粒结构控制;(ii)实验室规模的壁效应影响材料响应;(iii)与传感器直径相关联的测量可变性是不可忽略的;(iv)DEM是一种有价值的工具,能够深入了解材料行为。
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引用次数: 8
Metrology applications to D&D issues: issues at stake for INSIDER European project 计量应用于D&D问题:内部欧洲项目的利害关系问题
IF 0.5 Q3 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2020-11-01 DOI: 10.1051/epjn/2019052
D. Roudil, M. Crozet, S. Picart, B. Russell, M. Herranz, S. Boden, P. Peerani, L. Aldave de Las Heras
Nuclear metrology is an essential aspect to consider for further improvements of the initial characterization of sites under decommissioning. The H2020 Euratom project INSIDER in June 2017 aims at improving the management of contaminated materials arising from decommissioning and dismantling (D&D) operations by proposing an integrated methodology for radiological characterization. This methodology is based on advanced statistical processing and modelling, coupled with adapted or innovative measurement methods. A metrological approach supports the qualification of this integrated methodology with a concrete application to real projects representative of the use cases identified in the project. Assessment of the outcomes will be used for providing recommendations and guidance resulting in pre-standardization texts.
核计量学是进一步改进退役场址初始特征的一个重要方面。2017年6月,欧洲原子能机构H2020项目“内幕”旨在通过提出放射性表征的综合方法,改善退役和拆除(D&D)操作中产生的污染材料的管理。这种方法是基于先进的统计处理和建模,加上适应或创新的测量方法。计量方法支持这种集成方法的资格,并将其具体应用于代表项目中确定的用例的实际项目。对结果的评估将用于提供建议和指导,从而形成标准化前的文本。
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引用次数: 1
A minimal predictive model for better formulations of solvent phases with low viscosity 低粘度溶剂相更好配方的最小预测模型
IF 0.5 Q3 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2020-11-01 DOI: 10.1051/epjn/2019055
Maximilian Pleines, M. Hahn, J. Duhamet, T. Zemb
The viscosity increase of the organic phase when liquid–liquid extraction processes are intensified causes difficulties for hydrometallurgical processes on industrial scale. In this work, we have analyzed this problem for the example of N,N-dialkylamides in the presence of uranyl nitrate experimentally. Furthermore, we present a minimal model at nanoscale that allows rationalizing the experimental phenomena by connecting the molecular, mesoscopic and macroscopic scale and that allows predicting qualitative trends in viscosity. This model opens broad possibilities in optimizing constraints and is a further step towards knowledge-based formulation of extracting microemulsions formed by microstructures with low connectivity, even at high load with heavy metals.
随着液液萃取过程的加剧,有机相的粘度增加,给工业规模的湿法冶金工艺带来了困难。本文以硝酸铀酰存在下的N,N-二基酰胺为例,对这一问题进行了实验分析。此外,我们提出了一个纳米尺度的最小模型,通过连接分子、介观和宏观尺度,使实验现象合理化,并允许预测粘度的定性趋势。该模型为优化约束开辟了广阔的可能性,并且是朝着基于知识的配方提取由低连通性微结构形成的微乳液的进一步一步,即使在重金属高负荷下也是如此。
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引用次数: 5
Hydraulic and statistical study of metastable phenomena in PWR rod bundles 压水堆棒束亚稳现象的水力学和统计研究
IF 0.5 Q3 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2020-11-01 DOI: 10.1051/epjn/2019057
F. Muller
The analysis of fuel rod bundle flows constitutes a key element of Pressurized-Water Reactors (PWR) safety studies. The present work aims at improving our understanding of nefarious reorganisation phenomena observed by numerous studies in the flow large-scale structures. 3D simulations allowed identifying two distinct reorganisations consisting in a sign change for either a transverse velocity in rod-to-rod gaps or for a subchannel vortex. A Taylor “frozen turbulence” hypothesis was adopted to model the evolution of large-scale 3D structures as transported-2D. A statistical method was applied to the 2D field to determine its thermodynamically stable states through an optimization problem. Similarities were obtained between the PWR coherent structures and the stable states in a simplified 2D geometry. Further, 2D simulations allowed identifying two possible flow bifurcations, each related to one of the reorganisations observed in 3D simulations, laying the foundations for a physical explanation of this phenomenon.
燃料棒束流动分析是压水堆安全性研究的一个重要内容。目前的工作旨在提高我们对流动大尺度结构中大量研究观察到的恶性重组现象的理解。3D模拟可以识别出两种不同的重组,包括在杆到杆间隙的横向速度或子通道涡旋的符号变化。采用Taylor“冻结湍流”假说,将大尺度三维结构的演化建模为传输-二维。将统计方法应用于二维场,通过优化问题确定其热力学稳定状态。在简化的二维几何结构中,得到了压水堆相干结构与稳定状态的相似性。此外,2D模拟可以识别出两种可能的流动分支,每种分支都与3D模拟中观察到的一种重组有关,为这种现象的物理解释奠定了基础。
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引用次数: 0
INSIDER UC2: the BR3 biological shield preliminary results and future work 内幕UC2:BR3生物屏蔽初步结果和未来工作
IF 0.5 Q3 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2020-11-01 DOI: 10.1051/epjn/2019054
W. Broeckx, B. Rogiers, N. Mangelschots, R. Vandyck, Greet Verstrepen, S. Boden
Aiming at economical optimization, the characterisation of the biological shield of the Belgian Reactor 3 is one of the three use cases intended to validate the integrated characterization methodology developed within the INSIDER project. Pre-existing data were used to define the sampling design strategy. The additional sampling and analysis program consisted of total gamma measurements at the inner surface of the biological shield (secondary data) and gamma spectrometry measurements on drill core samples (primary data). The newly acquired data is supplemented with the historical available data. The full data set currently consists of a total of 283 secondary and 379 primary data points. Preliminary calculations already provide a clear-cut representation of the three different end-stage classes: unconditional clearance, conditional clearance and radioactive waste. On the short term, the current model will be further refined and completed with proper risk evaluation. On the longer term, we envisage a global uncertainty calculation and sensitivity analysis of the entire process.
为了实现经济优化,比利时3号反应堆生物屏蔽的表征是旨在验证INSIDER项目中开发的综合表征方法的三个用例之一。使用预先存在的数据来定义抽样设计策略。额外的采样和分析程序包括生物屏蔽内表面的总伽马测量值(二次数据)和岩芯样本的伽马光谱测量值(一次数据)。新获取的数据由历史可用数据进行补充。完整的数据集目前共由283个辅助数据点和379个主数据点组成。初步计算已经明确表示了三种不同的终末期类别:无条件清除、有条件清除和放射性废物。在短期内,目前的模型将进一步完善,并进行适当的风险评估。从长远来看,我们设想对整个过程进行全局不确定性计算和敏感性分析。
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引用次数: 2
JRC in Euratom Research and Training Programme − 2014–2020 联合研究中心在欧洲原子能机构研究和培训计划- 2014-2020
IF 0.5 Q3 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2020-09-01 DOI: 10.1051/epjn/2019036
S. Abousahl, A. Bucalossi, Victor Esteban Gran, Manuel Martin Ramos
The Euratom Research and Training Programme 2014–2018 and its extension 2019–2020 (the Euratom Programme) is implemented through direct actions in fission − i.e. research performed by the Commission's Joint Research Centre (JRC), and through indirect actions in fission– i.e. via competitive calls for proposals, and in fusion − i.e. through a comprehensive named-beneficiary co-fund action managed by the Commission's Directorate-General for Research & Innovation (RTD). The general objective of the Programme is “to pursue nuclear research and training activities with an emphasis on the continuous improvement of nuclear safety, security and radiation protection, in particular to potentially contribute to the long-term decarbonisation of the energy system in a safe, efficient and secure way.” The Programme is an integral part of Horizon 2020, the EU Framework Programme for Research and Innovation. The direct actions implemented by the JRC constitute an important part of the Euratom Programme and pursue specific objectives covering: nuclear safety, radioactive waste management, decommissioning, emergency preparedness; nuclear security, safeguards and non-proliferation; standardisation; knowledge management; education and training; and support to the policy of the Union on these fields. The JRC multi-annual work programme for nuclear activities fully reflects the aforementioned objectives. It is structured in about 20 projects, and allocates 48% of its resources to nuclear safety, waste management, decommissioning and emergency preparedness, 33% to nuclear security, safeguards and non-proliferation, 12% to reference standards, nuclear science and non-energy applications and 7% to education, training and knowledge management. To ensure that direct actions are in line with and complement the research and training needs of Member States, JRC is continuously interacting with the main research and scientific institutions in the EU, and actively participating in several technological platforms and associations. JRC also participates as part of the consortia in indirect actions, which allows JRC scientist to engage in top level scientific research, and yields maintaining and further developing JRC's scientific excellence. At the same time, the members of the consortia can have access to unique research infrastructure. The participation of JRC in indirect actions can be improved by exploiting synergies inside the Euratom Programme, and also with the future Horizon Europe Framework Programme. In preparation of the next Euratom Programme 2021–2025, two pilot projects on knowledge management and on open access to JRC research infrastructure will explore and test this improved involvement of JRC in indirect actions. The paper highlights some of the achievements of recent JRC direct actions with a focus on the interaction with EU MS research organisations, as well as some of the most important elements of the Commission Proposal for the next (2021–2025) Euratom Prog
2014年至2018年欧洲原子能共同体研究与培训计划及其2019年至2020年的延期(欧洲原子能联盟计划)是通过裂变方面的直接行动(即委员会联合研究中心(JRC)进行的研究)和裂变方面的间接行动(即竞争性征求建议书)实施的,以及融合——即通过由委员会研究与创新总局(RTD)管理的全面指定受益人共同基金行动。该计划的总体目标是“开展核研究和培训活动,重点是持续改进核安全、安保和辐射防护,特别是以安全、高效和有保障的方式为能源系统的长期脱碳做出潜在贡献。”,欧盟研究与创新框架计划。联合研究委员会实施的直接行动是欧洲原子能共同体方案的重要组成部分,旨在实现以下具体目标:核安全、放射性废物管理、退役、应急准备;核安全、保障监督和不扩散;标准化;知识管理;教育和培训;以及支持欧盟在这些领域的政策。联合研究中心核活动多年期工作方案充分体现了上述目标。它由大约20个项目组成,将48%的资源分配给核安全、废物管理、退役和应急准备,33%分配给核安保、保障监督和不扩散,12%分配给参考标准、核科学和非能源应用,7%分配给教育、培训和知识管理。为了确保直接行动符合并补充成员国的研究和培训需求,JRC不断与欧盟的主要研究和科学机构互动,并积极参与几个技术平台和协会。JRC还作为财团的一部分参与间接行动,这使JRC科学家能够从事顶级科学研究,并有助于保持和进一步发展JRC的科学卓越性。同时,财团成员可以使用独特的研究基础设施。可以通过利用欧洲原子能共同体方案内部的协同作用以及与未来地平线欧洲框架方案的协同作用,改善联合研究中心对间接行动的参与。在准备下一个欧洲原子能共同体2021-2025年计划时,两个关于知识管理和开放获取联合研究中心研究基础设施的试点项目将探索和测试联合研究中心在间接行动中的这种改进参与。该文件强调了联合研究委员会最近直接行动的一些成就,重点是与欧盟MS研究组织的互动,以及委员会下一个(2021-2025年)欧洲原子能共同体计划提案的一些最重要内容,重点是联合研究委员会在参与间接行动方面的新定位。
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引用次数: 2
A nuclear owner/operator perspective on ways and means for joint programming on predisposal activities 核所有人/运营者对联合拟订处置前活动方案的方法和手段的看法
IF 0.5 Q3 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2020-09-01 DOI: 10.1051/epjn/2019039
M. Pieraccini, Sylvain Granger
Nuclear decommissioning is a worldwide competitive market. It is also the main source of radioactive waste from the nuclear energy field. In order to reduce the waste volume it is necessary to sort the actual radioactive waste to be disposed of and to separate them from other materials that could be recycled. Since 2015, Electricité de France (EDF) has gathered the waste management and dismantling (WM&D) projects, the related competences and human resources in the WM&D field, in a dedicated directorate (DP2D) and a company group called Cyclife (including waste treatment facilities). Taking into account the experience gained by carrying out its own WM&D projects as well as contributing to international cooperation, EDF considers that integrating collaborative research and development (R&D) on pre-disposal and waste management could be carried out following four main objectives: (1) alignment of the application of regulatory frameworks through appropriate definition of criteria and rules for radioactive waste to enable sensible worldwide comparison of technics; (2) improvement of technical and organisational aspects of nuclear reactors decommissioning using a demonstrator facility to be in operation, at first for graphite reactors, by 2022; (3) development of new techniques to decontaminate/homogenize metallic materials through a dedicated recycling route. These technics will be implemented in a new treatment facility foreseen to be available by 2030; and (4) increased training of decommissioning operators with the help of new technologies. All these improvements are aiming, beyond technical and experimental aspects, at reducing environmental impacts of nuclear activities as well as preserving the radioactive disposal volumes, as they are considered by EDF as rare resources.
核退役是一个全球性的竞争市场。它也是核能领域放射性废物的主要来源。为了减少废物量,有必要对要处理的实际放射性废物进行分类,并将它们与其他可回收的材料分开。自2015年以来,法国电力公司(EDF)将废物管理和拆除(WM&D)项目、WM&D领域的相关能力和人力资源聚集在一个专门的理事会(DP2D)和一个名为Cyclife的公司集团(包括废物处理设施)中。考虑到开展自身的核废料处理项目所获得的经验以及对国际合作的贡献,法国电力公司认为,可以将预先处置和废物管理方面的合作研究与开发(R&D)结合起来,实现以下四个主要目标:(1)通过适当定义放射性废物的标准和规则,协调监管框架的应用,以便在全球范围内合理地比较技术;(2)利用一个示范设施在2022年前开始运行,首先用于石墨反应堆,改进核反应堆退役的技术和组织方面;(3)发展新技术,通过专门的回收路线净化/均匀化金属材料。这些技术将在一个新的处理设施中实施,预计到2030年可用;(4)利用新技术加强对退役操作人员的培训。除技术和实验方面外,所有这些改进的目的是减少核活动对环境的影响,并保持放射性处理量,因为法国电力公司认为它们是稀有资源。
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引用次数: 1
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EPJ Nuclear Sciences & Technologies
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