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Investigating the apparent anomalous cooling of soot during laser-induced incandescence experiments 研究在激光诱导白炽实验中烟灰的明显异常冷却
IF 2 3区 物理与天体物理 Q3 OPTICS Pub Date : 2025-12-18 DOI: 10.1007/s00340-025-08550-8
Stephen Robinson-Enebeli, Christof Schulz, Kyle J. Daun

While time-resolved laser-induced incandescence (TiRe-LII) has become a standard laser-based diagnostic for soot, there remain unexplained observations in some datasets. One such effect is the so-called “anomalous cooling”, in which the pyrometric temperature decays faster than can be explained by conventional heat transfer models immediately following the peak temperature. This work investigates this phenomenon through experiments on soot entrained in different bath gases and irradiated in the low-fluence regime, where particle sublimation is minimal. The anomalous cooling phenomenon is caused by the contribution of particles in the probe volume that have been heated beyond the sublimation threshold to the overall incandescence signal, due to nonuniform laser fluence. Particles in these “hot spot” regions feature a faster cooling rate due to sublimation, contributing to the effect of apparent anomalous cooling. Particle-size polydispersity also plays a notable but minor role. The effect depends on the bath-gas composition, which is attributed to differences in species-specific heat transfer.

虽然时间分辨激光诱导白炽灯(TiRe-LII)已成为基于激光诊断烟灰的标准方法,但在一些数据集中仍存在无法解释的观察结果。其中一种效应就是所谓的“反常冷却”,即高温衰减速度比传统传热模型所能解释的要快。本研究通过对不同浴气中夹带的煤烟进行实验,并在颗粒升华最小的低通量状态下辐照,研究了这一现象。异常冷却现象是由探针体积中被加热到超过升华阈值的粒子对整个白炽信号的贡献引起的,这是由于不均匀的激光影响。这些“热点”区域的粒子由于升华而具有更快的冷却速度,从而导致明显的异常冷却效果。粒径多分散性也起着显著但次要的作用。这种影响取决于浴气成分,这是由于物种特有的传热差异造成的。
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引用次数: 0
Seven-light-screen precision target and high-accuracy calibration of its invisible spatial structure parameters 七光屏精密靶及其不可见空间结构参数的高精度标定
IF 2 3区 物理与天体物理 Q3 OPTICS Pub Date : 2025-12-12 DOI: 10.1007/s00340-025-08612-x
Fen Gao, Yuzhun He, Pengwei Shi

Seven-light-screen precision target is an new exterior ballistic parameter testing device that enables non-contact measurement of multiple parameters with a single shot, including impact coordinates, flight velocity vector, pitch and azimuth angles of the flight direction, and velocity attenuation rate for obliquely incident flying targets. Precise calibration of structural parameters for invisible light-screen array of seven-light-screen precision target is crucial for ensuring its accuracy and constitutes an essential step in its development. In this paper, we proposes a high-accuracy calibration method. It uses a light-blocking probe to simulate the entry of a projectile into the invisible light screen for the extraction of the actual light screen center. Dual theodolites are employed in conjunction with the readings of a grating ruler during screen crossing to quickly and accurately locate the coordinate points within the screen. Multiple extracted screen coordinate points are then fitted to reconstruct the actual light screen plane, achieving accurate spatial position calibration of multiple invisible screens. This paper introduces the structure and measurement principle of seven-light-screen target, describes the calibration system's composition and working principle, and derives the specific calibration algorithm formulas. The constructed system was applied to calibrate an actual seven-screen target. Live-fire experiments were conducted based on this calibrated target, and the measured impact coordinates were compared against results from cardboard target measurements. The research results show that the structural parameters obtained by the proposed calibration method are accurate. After calibration, the coordinate measurement accuracy of the seven-light-screen precision target within a 1 m × 1 m target sensor area is better than 1.5 mm. This calibration method is universal for the calibration of light-screen arrays with similar principles and provides an effective solution for calibrating structure parameters of multi-light-screen precision targets.

七光屏精密靶是一种新型的外弹道参数测试装置,可实现对斜入射飞行目标的冲击坐标、飞行速度矢量、飞行方向俯仰角和方位角、速度衰减率等多项参数的单次非接触测量。七光屏精密靶标不可见光屏阵列结构参数的精确标定是保证其精度的关键,是其研制的重要环节。本文提出了一种高精度的标定方法。它采用阻光探头模拟抛射物进入不可见光屏,以提取实际光屏中心。双经纬仪与光栅尺的读数一起使用,在屏幕穿越期间快速准确地定位屏幕内的坐标点。然后对提取的多个屏幕坐标点进行拟合,重建实际光屏平面,实现多个不可见屏幕的精确空间位置标定。介绍了七光屏靶的结构和测量原理,阐述了标定系统的组成和工作原理,推导了具体的标定算法公式。所构建的系统被用于标定一个实际的七屏靶。在此基础上进行了实弹射击实验,并将测量的冲击坐标与纸板靶测量结果进行了比较。研究结果表明,该方法得到的结构参数是准确的。标定后,7光屏精密目标在1m × 1m目标传感器区域内的坐标测量精度优于1.5 mm。该标定方法对原理相似的光幕阵列标定具有通用性,为多光幕精密目标的结构参数标定提供了有效的解决方案。
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引用次数: 0
Negative index metamaterial controlled propagation of surface plasmons 负折射率超材料控制表面等离子体的传播
IF 2 3区 物理与天体物理 Q3 OPTICS Pub Date : 2025-12-11 DOI: 10.1007/s00340-025-08613-w
Tatjana Gric

Understanding the plasmonic behavior of materials with large-scale inhomogeneity (like negative index metamaterial) is crucial because these materials cannot be modeled as simple scatterers. This is due to the emergence of plasmonic materials other than those based on noble metals and the advancement of sophisticated materials processing techniques. Propagation of surface plasmons can be achieved using a metamaterial and dielectric interface. Control of the surface plasmons opens the wide avenues for a broad range of applications. Similarly, the shape of individual surface nanostructures or the phase control of individual elements in an array of such structures can be used to regulate the propagation of surface plasmons at the interface between metal films and dielectric materials. Here, we show how to regulate surface plasmon propagation at the negative index metamaterial-dielectric interface. The negative index metamaterial enables the surface modes, while the adjacent dielectric is what tunes their properties.

理解具有大规模非均匀性的材料(如负折射率超材料)的等离子体行为是至关重要的,因为这些材料不能被建模为简单的散射体。这是由于等离子体材料的出现,而不是基于贵金属的材料,以及复杂材料加工技术的进步。表面等离子体的传播可以通过使用超材料和介电界面来实现。表面等离子体的控制为广泛的应用开辟了广阔的途径。同样,单个表面纳米结构的形状或此类结构阵列中单个元素的相位控制可用于调节金属薄膜和介电材料之间界面的表面等离子体的传播。在这里,我们展示了如何调节表面等离子体在负折射率超材料-介电界面的传播。负折射率的超材料实现了表面模式,而相邻的介电介质则调节了它们的特性。
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引用次数: 0
Electromechanically tunable third-harmonic generation at THz frequencies using nonlinear graphene metasurface 利用非线性石墨烯超表面在太赫兹频率下产生机电可调谐的三次谐波
IF 2 3区 物理与天体物理 Q3 OPTICS Pub Date : 2025-12-08 DOI: 10.1007/s00340-025-08610-z
Mitali Sahu, Partha Roy Chaudhuri

Unusual characteristics of graphene as a tunable and nonlinear 2D material embedded in a novel voltage-controlled electromechanical design of the metasurface is implemented to achieve effective tunable third harmonic generation (THG) in the terahertz (THz) regime. This approach offers certain advantages over conventional methods based on tuning the Fermi energy of graphene via electrical or chemical doping, such as a broader tuning range and post-fabrication reconfigurability. We introduce mechanical tunability through a suspended graphene sheet placed over an oxide grating on a gold substrate. Applying a low voltage in the range of (1{-}5:text{V}) between the graphene and gold layers induces mechanical bending of the graphene, resulting in a tunable shift in the resonance frequency. Simulations exhibit a continuous fundamental frequency (FF) shift of (2.9:text{T}text{H}text{z}) with only a (:5:text{V}) potential, enabling a dynamic control of the THG output without modifying the metasurface structure. This compact and efficient platform holds promise for tunable THz sources in spectroscopy and imaging applications.

石墨烯作为一种可调谐的非线性二维材料,嵌入在一种新型压控机电设计的超表面中,实现了在太赫兹(THz)区域内有效的可调谐三次谐波产生(THG)。与通过电或化学掺杂调整石墨烯的费米能的传统方法相比,这种方法具有一定的优势,例如更宽的调谐范围和制造后的可重构性。我们通过放置在金衬底上的氧化光栅上的悬浮石墨烯片引入机械可调性。在石墨烯和金层之间施加(1{-}5:text{V})范围内的低电压会引起石墨烯的机械弯曲,从而导致共振频率的可调偏移。模拟结果显示,基频(FF)的连续位移为(2.9:text{T}text{H}text{z}),电势仅为(:5:text{V}),从而可以在不改变超表面结构的情况下动态控制THG输出。这种紧凑而高效的平台有望在光谱学和成像应用中实现可调谐太赫兹源。
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引用次数: 0
Direct laser writing of in-volume diffractive optical elements with high speed and high resolution 高速、高分辨率的体内衍射光学元件直接激光写入
IF 2 3区 物理与天体物理 Q3 OPTICS Pub Date : 2025-12-05 DOI: 10.1007/s00340-025-08581-1
C. Ingenhag, S. Stein, A. Schüller-Ruhl, R. Fleischhaker

We demonstrate fast, high-resolution fabrication of in-volume diffractive optical elements (DOEs) by combining galvanometric scanning with a microscope objective ((text {NA}=0.4)) and a 1 ps laser source. Carefully chosen parameters exploit nonlinear absorption in fused silica to create highly localized refractive-index modifications. Estimating the scaling laws of energy deposition, single-pulse writing becomes feasible, yielding a ( Delta n approx 0.5 times 10^{{ - 2}} ) and modification dimensions below the nominal focal spot. Using a layer-stacking scheme in z, we assemble multi-level phase masks: examples include a 4-level, 250 × 250 px DOE (2 µm pixels) and a 10-level, 416 × 416 px DOE (1.2 µm pixels). Phase-contrast microscopy confirms the written phase structure and comparison with theoretical phase data shows strong correspondence. Optical characterization at 532 nm reproduces target intensity distributions with high fidelity (overlap (>80)% against the computed discretized mask in a selected region; >66% vs. the original target). Yet, production times remain short (8–9 min for the high-resolution DOE, 60 s for the 4-level device), demonstrating that we improve trade-off between quality and speed to a level good enough for practical applications.

我们展示了快速,高分辨率制造的体积内衍射光学元件(do),结合振镜扫描与显微镜物镜((text {NA}=0.4))和1 ps激光源。精心选择的参数利用非线性吸收在熔融二氧化硅,以创建高度局部化的折射率修改。估计能量沉积的标度规律,单脉冲写入成为可能,产生( Delta n approx 0.5 times 10^{{ - 2}} )和修正尺寸低于标称焦斑。使用z中的层堆叠方案,我们组装了多级相位掩模:示例包括4级,250 × 250像素的DOE(2µm像素)和10级,416 × 416像素的DOE(1.2µm像素)。相衬显微镜证实了书面相结构,并与理论相数据进行了比较,显示出很强的一致性。532 nm的光学表征再现了高保真度(重叠)的目标强度分布 (>80)% against the computed discretized mask in a selected region; >66% vs. the original target). Yet, production times remain short (8–9 min for the high-resolution DOE, 60 s for the 4-level device), demonstrating that we improve trade-off between quality and speed to a level good enough for practical applications.
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引用次数: 0
Modification of resonance-induced enhancement of high-order harmonics in the laser plasmas containing atoms and ions 含原子和离子的激光等离子体中共振诱导高次谐波增强的修正
IF 2 3区 物理与天体物理 Q3 OPTICS Pub Date : 2025-12-05 DOI: 10.1007/s00340-025-08608-7
Rashid A. Ganeev

The difference in harmonic intensity distribution during frequency up-conversion of 800 nm, 65 fs pulses in a few laser-induced plasmas (Li, Ge, Yb, and As) at variable concentrations of ions is demonstrated. At small fluencies of heating pulses that create laser-induced plasmas, the prevailing presence of neutrals leads to a gradual decrease in harmonic yield. The stronger laser ablation caused the appearance of the singly and doubly charged ions, which led to the enhancement of the single harmonic or small group of harmonics in the vicinity of the ionic transitions possessing large oscillator strengths. These resonance-enhanced harmonics become significantly larger than the neighboring harmonics. The peculiarities of this process are analyzed at different fluencies of the ablating pulses.

在不同浓度离子下,800 nm, 65 fs脉冲在几种激光诱导等离子体(Li, Ge, Yb和As)中频率上转换时谐波强度分布的差异。在产生激光诱导等离子体的小通量加热脉冲中,中性点的普遍存在导致谐波产量逐渐下降。较强的激光烧蚀引起了单电荷和双电荷离子的出现,导致具有较大振荡强度的离子跃迁附近的单谐波或小群谐波增强。这些共振增强的谐波明显大于相邻的谐波。在不同的烧蚀脉冲频率下,分析了烧蚀过程的特点。
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引用次数: 0
Numerical and experimental investigation of surface figure error in high-repetition-rate XFEL mirrors 高重复率XFEL反射镜表面图形误差的数值与实验研究
IF 2 3区 物理与天体物理 Q3 OPTICS Pub Date : 2025-11-29 DOI: 10.1007/s00340-025-08607-8
Zhen Wang, Weizhen Lei, Xiaohao Dong, Yajun Tong

This study systematically quantifies the surface figure error (SFE) of the first reflection mirror (M1) in SHINE’s FEL-I beamline via numerical calculations and experiments, analyzing contributions of thermal SFE (from X-ray heat loads) and non-thermal SFE (mechanical-related: clamping force, mirror self-gravity, In-Ga liquid gravity; manufacturing-induced). Results demonstrate that thermal SFE dominates at (ge )50 kHz (over 96% of total SFE); at (le )10 kHz, non-thermal SFE accounts for up to 38% (manufacturing-induced SFE leads in effective footprint zone, In-Ga liquid gravity impacts mechanical-related SFE more than other factors). This work clarifies thermal/non-thermal SFE dynamics across repetition rates, providing a basis for M1 optimization and high-repetition-rate XFEL mirror design.

本研究通过数值计算和实验系统地量化了SHINE的feli光束线中第一反射镜(M1)的表面图形误差(SFE),分析了热SFE(来自x射线热载荷)和非热SFE(机械相关:夹紧力、反射镜自重力、in - ga液体重力、制造诱导)的贡献。结果表明,在(ge ) 50 kHz(大于96 kHz)时,热SFE占主导地位% of total SFE); at (le )10 kHz, non-thermal SFE accounts for up to 38% (manufacturing-induced SFE leads in effective footprint zone, In-Ga liquid gravity impacts mechanical-related SFE more than other factors). This work clarifies thermal/non-thermal SFE dynamics across repetition rates, providing a basis for M1 optimization and high-repetition-rate XFEL mirror design.
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引用次数: 0
Second harmonic generation of circularly polarized Hermite-cosh Gaussian laser beam in magnetized plasma 圆极化厄米-柯希高斯激光束在磁化等离子体中的二次谐波产生
IF 2 3区 物理与天体物理 Q3 OPTICS Pub Date : 2025-11-29 DOI: 10.1007/s00340-025-08605-w
Danish Nazir, Vishal Thakur

This work examines the second harmonic generation of a Hermite-cosh-Gaussian (HChG) laser beam with circular polarisation in a magnetised plasma. In order to explain relativistic electron motion and the distinctive transverse structure of the Hermite-cosh-Gaussian beam, it is assumed that the nonlinear current density is the cause of second harmonic generation. By using the paraxial approximation, analytical formulas for the second harmonic field amplitude are derived, reflecting dependencies on plasma density and beam characteristics (mode indices, intensity, and beam width). The wiggler magnetic field enhances the phase-matching conditions to permit resonant SHG by giving the second-harmonic photons some more velocity. Furthermore, the wiggler field will contribute to the maintenance of the cyclotron frequency, which confines the plasma electrons and increases SHG efficiency. While the HChG profile delivers mode-selective gain in SHG efficiency, circular polarisation improves azimuthal symmetry in the nonlinear current. The findings demonstrate how structured beams may be used to generate high-harmonics in laser-plasma interactions in a customised manner.

本文研究了在磁化等离子体中具有圆偏振的厄米-cosh-高斯(HChG)激光束的二次谐波产生。为了解释相对论性电子运动和厄米-科什-高斯光束独特的横向结构,假设非线性电流密度是二次谐波产生的原因。通过使用近轴近似,导出了二次谐波场振幅的解析公式,反映了等离子体密度和光束特性(模式指数、强度和光束宽度)的依赖关系。摆动磁场通过给二次谐波光子更多的速度来增强相位匹配条件,从而允许共振SHG。此外,摆动场将有助于维持回旋加速器的频率,从而限制等离子体电子,提高SHG效率。虽然HChG剖面提供了SHG效率的模式选择增益,但圆极化改善了非线性电流的方位角对称性。这一发现展示了如何使用结构光束以定制的方式在激光等离子体相互作用中产生高谐波。
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引用次数: 0
Topological exciton dynamics in strain-engineered lead halide perovskite quantum dots 应变工程卤化铅钙钛矿量子点的拓扑激子动力学
IF 2 3区 物理与天体物理 Q3 OPTICS Pub Date : 2025-11-28 DOI: 10.1007/s00340-025-08600-1
Moses Udoisoh, Kabir Kehinde Adedeji, Salihu Ahmad, oluwatife Daniel Olaleye

The manipulation of quantum states via mechanical strain offers a pathway to engineer topological excitons in soft semiconductors. Here, we present a theoretical framework that shows that helical strain transforms lead halide perovskite quantum dots (QDs) into a platform for topological excitonics. Using a first-principles-informed framework combining strain-modulated Lamé eigenstates and non-perturbative Coulomb interactions, we identify a strain-driven topological transition at critical ellipticity (k = 0.59 pm 0.02), (corresponding to ≈ 2% torsional strain) marked by inversion of the exciton Chern number ((C = 0 to 1)) and π-Berry phase accumulation. Quantitative calculations yield an exciton binding-energy enhancement up to 45 meV and photoluminescence (PL) redshifts of ≈ 72 meV, in agreement with experimental data. The computed deformation potential (− 0.8 eV/% strain), group-velocity scaling (v ∝ k1.7), and Chern-number inversion confirm a strain-driven topological crossover supported by Berry-phase accumulation. Comparison with reported PL and diffusion measurements validates the predictive accuracy of the Lamé-Coulomb formalism, which bridges continuum elasticity with quantum confinement. These findings proposes perovskite QDs as experimentally accessible hosts of strain-tunable topological excitons, enabling reconfigurable quantum-photonic and optoelectronic devices based on mechanically programmable excitonic states.

通过机械应变对量子态的操纵为设计软半导体中的拓扑激子提供了一条途径。在这里,我们提出了一个理论框架,表明螺旋应变将卤化铅钙钛矿量子点(QDs)转变为拓扑激子学的平台。利用结合应变调制lam本征态和非摄动库仑相互作用的第一原理框架,我们确定了临界椭圆度(k = 0.59 pm 0.02)处应变驱动的拓扑跃迁,(对应于≈2)% torsional strain) marked by inversion of the exciton Chern number ((C = 0 to 1)) and π-Berry phase accumulation. Quantitative calculations yield an exciton binding-energy enhancement up to 45 meV and photoluminescence (PL) redshifts of ≈ 72 meV, in agreement with experimental data. The computed deformation potential (− 0.8 eV/% strain), group-velocity scaling (v ∝ k1.7), and Chern-number inversion confirm a strain-driven topological crossover supported by Berry-phase accumulation. Comparison with reported PL and diffusion measurements validates the predictive accuracy of the Lamé-Coulomb formalism, which bridges continuum elasticity with quantum confinement. These findings proposes perovskite QDs as experimentally accessible hosts of strain-tunable topological excitons, enabling reconfigurable quantum-photonic and optoelectronic devices based on mechanically programmable excitonic states.
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引用次数: 0
Exploring the laser-induced fluorescence of dissolved oxygen as a method for its contactless detection 探索溶解氧激光诱导荧光的非接触检测方法
IF 2 3区 物理与天体物理 Q3 OPTICS Pub Date : 2025-11-26 DOI: 10.1007/s00340-025-08602-z
Anatoliy A. Kosterev

The laser-induced fluorescence of oxygen in organic solvents was investigated as a potential contactless method for quantifying its concentration. The fluorescence was excited directly by a diode laser radiation in the 1270 nm oxygen absorption band. Neither a sensitizer nor singlet oxygen traps were added to the solvent. An uncooled photodiode was used as a detector. A simple kinetic model was used for assessing the oxygen concentration from the signal magnitude and decay time. An advanced model explaining the observed deviation of fluorescence kinetics from single exponential decay is presented. The method was tested with pure and contaminated Freon-113 samples, chloroform, acetone and n-heptane.

研究了有机溶剂中氧的激光诱导荧光作为一种潜在的非接触定量方法。在1270 nm的氧吸收波段,用二极管激光直接激发荧光。溶剂中既没有添加敏化剂,也没有添加单线态氧阱。一个未冷却的光电二极管被用作检测器。用一个简单的动力学模型从信号大小和衰减时间来评估氧浓度。提出了一种先进的模型来解释观察到的荧光动力学偏离单指数衰减。用纯氟利昂-113、氯仿、丙酮和正庚烷样品对该方法进行了测试。
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引用次数: 0
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Applied Physics B
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