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Fluorescence characteristics of organic tracer molecules for planar laser-induced fluorescence studies in internal combustion engines, part A: non-aromatics 用于内燃机平面激光诱导荧光研究的有机示踪分子的荧光特性,A 部分:非芳香族化合物
IF 2 3区 物理与天体物理 Q3 OPTICS Pub Date : 2024-08-21 DOI: 10.1007/s00340-024-08272-3
Soumyanil Nayek, Mayank Mittal

Tracer based planar laser-induced fluorescence (PLIF) has emerged as a powerful in-situ measurement technique with a considerable spatial and temporal resolution for Internal combustion (IC) engines. In PLIF, the emitted fluorescence signals from a tracer molecule are processed to determine distribution of temperature, fuel, residual gases etc. However, it is imperative to have a thorough understanding of the tracer physical properties and its fluorescence intensity dependencies on excitation wavelength, pressure, temperature, and bath gas composition existing inside the combustor for accurate quantitative interpretation. This work consists of a series of two articles providing a detailed review of the existing literature of fluorescence characteristics of various molecules used as tracers in IC engine applications. Due to the overwhelming usage of organic compounds in IC engine environment, the work is restricted to them. Part A of this work is focussed on non-aromatic compounds (acetone, 3-pentanone and biacetyl) whereas part B will focus on aromatics. Due to a small energy gap between the excited singlet and triplet states of ketones, they experience rapid inter-system crossing making them far less sensitive to oxygen quenching effects than aromatic molecules. Addition of tracers to surrogate fuel can lead to difficulties related to co-evaporation, azeotrope formation and stability of tracer molecules in terms of photolysis and pyrolysis effects when subjected to intense laser irradiation and harsh engine environment. In this work, fluorescence signal variation of tracer molecules is divided into variations in absorption cross-section and fluorescence quantum yield (FQY). Absorption cross-section normally increases with temperature but is insensitive to pressure changes. FQY reduces with increase in temperature but increases with pressure for ketones for non-oxygen containing bath gases. The pressure sensitivity increases with the number of atoms in a collider molecule. FQY values decrease with decreasing laser excitation wavelength whereas the temperature and pressure sensitivity of FQY reduce with increasing wavelengths. For simultaneous high pressure and temperature conditions, the pressure sensitivity of FQY is found to reduce due to a reduction in the effective number of collisions with bath gas molecules. Among the three tracers, acetone has been widely used for marking gaseous fuels and 3-pentanone and biacetyl for liquid fuels like iso-octane. Acetone and 3-pentanone have received significant attention for fluorescence studies due to their widespread usage in IC engine applications. Biacetyl on the other hand has recently started to receive attention due to its application in high repetition rates PLIF measurements and requires more fluorescence studies to fully characterise its fluorescence behaviour and construct fluorescence models over the complete pressure and temperature range required in IC engine applications.

基于示踪剂的平面激光诱导荧光(PLIF)已成为一种强大的现场测量技术,对内燃机(IC)具有相当高的空间和时间分辨率。在 PLIF 中,通过处理示踪分子发射的荧光信号,可以确定温度、燃料、残余气体等的分布情况。然而,为了准确地进行定量分析,必须全面了解示踪剂的物理特性及其荧光强度与燃烧器内激发波长、压力、温度和浴气成分的关系。这项工作包括两篇系列文章,对集成电路发动机应用中用作示踪剂的各种分子的荧光特性的现有文献进行了详细综述。由于有机化合物在集成电路发动机环境中的使用量非常大,因此本工作仅限于有机化合物。这项工作的 A 部分侧重于非芳香族化合物(丙酮、3-戊酮和生物乙酰基),而 B 部分将侧重于芳香族化合物。由于酮类化合物激发的单线态和三线态之间的能隙较小,它们会经历快速的系统间交叉,因此对氧淬灭效应的敏感性远低于芳香族分子。在代用燃料中添加示踪剂可能会导致协同蒸发、共沸物形成以及示踪剂分子在强激光照射和恶劣发动机环境下的光解和热解效应稳定性等方面的困难。在这项工作中,示踪剂分子的荧光信号变化分为吸收截面和荧光量子产率(FQY)的变化。吸收截面通常随温度升高而增大,但对压力变化不敏感。FQY 随温度的升高而减小,但对非含氧浴气中的酮类来说,则随压力的升高而增大。压力敏感性随对撞机分子中原子数的增加而增加。FQY 值随着激光激发波长的减少而降低,而 FQY 的温度和压力敏感性则随着波长的增加而降低。在高压和高温同时存在的条件下,由于与浴槽气体分子碰撞的有效次数减少,FQY 的压力敏感性也会降低。在这三种示踪剂中,丙酮被广泛用于标记气体燃料,3-戊酮和生物乙酰则用于标记异辛烷等液体燃料。由于丙酮和 3-戊酮在集成电路发动机中的广泛应用,它们在荧光研究中备受关注。另一方面,双乙酰基最近因其在高重复率 PLIF 测量中的应用而开始受到关注,需要进行更多的荧光研究,以充分描述其荧光特性,并在集成电路发动机应用所需的完整压力和温度范围内构建荧光模型。
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引用次数: 0
A high peak power and low peak-to-peak instability mid-infrared optical parametric oscillator pumped by a 1064 nm electro-optic cavity-dumped pulsed laser 由 1064 nm 电光腔倾销脉冲激光器泵浦的高峰值功率和低峰-峰不稳定性中红外光参量振荡器
IF 2 3区 物理与天体物理 Q3 OPTICS Pub Date : 2024-08-20 DOI: 10.1007/s00340-024-08304-y
Guozhen Wang, Yang Bai, Yi Li, Shunyu Yang, Xiaoying Zhang, Wenrui Duan, Baole Lu

In this paper, we demonstrate a tunable mid-infrared (mid-IR) optical parametric oscillator (OPO) using an MgO: PPLN crystal with a polarization period of 29.8 μm, which was end-pumped by a 1064 nm electro-optic cavity-dumped all-solid-state laser (1064 nm EOCD-laser) with a pulse repetition frequency range of 100 Hz to 1 kHz. Thanks to the use of 808 nm pulsed laser diode (LD) side-pumping Nd: YAG crystal, transverse electro-optic modulating (TEOM) MgO: LN crystal, and birefringent crystal (BC) filtering in the 1064 nm cavity-dumped cavity, both the 1064 nm EOCD-laser and the idler light output by the OPO exhibited high peak power and low peak-to-peak instability in both pulse width and single pulse energy. By combining temperature tuning of the MgO: PPLN crystal from 30 °C to 200 °C, wavelength tuning of the idler light from 3705.2 to 3424.3 nm was achieved. For the first time, a pulsed idler light at 3705.2 nm with a high peak power of 1.224 MW, a narrow pulse width of 4.97 ns, and an optical-to-optical (1064 nm to 3705.2 nm) conversion efficiency of 38.1% was obtained, corresponding to a tuning temperature of 30 °C and a pulse repetition frequency of 100 Hz. The peak-to-peak instability for both pulse width and single pulse energy was only ± 1.04% and ± 1.41%, respectively.

在本文中,我们展示了一种可调谐中红外(mid-IR)光参量振荡器(OPO),它采用了偏振周期为 29.8 μm 的 MgO:PPLN 晶体,其偏振周期为 29.8 μm,由脉冲重复频率范围为 100 Hz 至 1 kHz 的 1064 nm 电光腔倾销全固态激光器(1064 nm EOCD-激光器)端泵浦。由于使用了 808 nm 脉冲激光二极管(LD)侧泵浦 Nd:YAG 晶体、横向电光调制(TEOM)MgO:LN 晶体和双折射晶体(BC)滤波的 1064 nm 腔倾销腔中,1064 nm EOCD 激光和 OPO 输出的惰极光在脉冲宽度和单脉冲能量方面都表现出峰值功率高、峰-峰不稳定性低的特点。通过将 MgO:PPLN 晶体的温度从 30 °C 调整到 200 °C,实现了惰极光波长从 3705.2 纳米到 3424.3 纳米的调整。在调谐温度为 30 ℃、脉冲重复频率为 100 Hz 的条件下,首次获得了峰值功率为 1.224 MW、窄脉宽为 4.97 ns、光-光(1064 nm 至 3705.2 nm)转换效率为 38.1%的 3705.2 nm 脉冲惰极光。脉冲宽度和单脉冲能量的峰-峰不稳定性分别仅为 ± 1.04% 和 ± 1.41%。
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引用次数: 0
Influence of external magnetic field on electromagnetically induced grating in a degenerate two-level atomic medium 外磁场对退化两级原子介质中电磁诱导光栅的影响
IF 2 3区 物理与天体物理 Q3 OPTICS Pub Date : 2024-08-20 DOI: 10.1007/s00340-024-08301-1
Nguyen Huy Bang, Luong Thi Yen Nga, Ho Hai Quang, Nguyen Van Ai, Phan Van Thuan, Nguyen Thi Thu Hien, Hoang Minh Dong, Le Van Doai

In this work, the external magnetic field is employed as a “knob” to transfer the light energy from the zero-order diffraction to the high-order diffractions of electromagnetically induced grating in a degenerate two-level atomic medium. Under a standing-wave coupling field, the diffraction of the probe beam is created with the diffraction pattern including zero-, first- and second-order diffractions. When the magnetic field is not applied, the absorption grating is formed based on amplitude modulation of the transmission function; most of the probe light energy is focused on the zero-order diffraction (about 70%) and only about 6% of the first-order diffraction. However, when the external magnetic field is applied, the phase grating is formed based on the phase modulation of transmission function; the probe light energy is transferred from zero-order diffraction to first- and second-order diffractions, in which the first-order diffraction efficiency can be obtained about 32% with proper magnetic field strength. Moreover, the probe light energy can also be transferred from zero-order diffraction to first- and second-order diffractions by adjusting the frequency and/or the intensity of the coupling and probe fields in the presence of external magnetic field.

在这项工作中,外部磁场被用作 "旋钮",将光能从零阶衍射转移到退化两级原子介质中电磁诱导光栅的高阶衍射。在驻波耦合场下,探针光束会产生衍射,衍射图样包括零阶、一阶和二阶衍射。在未施加磁场时,根据透射函数的振幅调制形成吸收光栅;探针光的大部分能量(约 70%)都集中在零阶衍射上,只有约 6% 的一阶衍射。然而,当施加外磁场时,基于透射函数的相位调制会形成相位光栅;探针光能量会从零阶衍射转移到一阶和二阶衍射,其中一阶衍射效率在适当的磁场强度下可达到约 32%。此外,在有外磁场的情况下,通过调整耦合场和探针场的频率和/或强度,也可将探针光能从零阶衍射转移到一阶和二阶衍射。
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引用次数: 0
Characterizing quantum correlations dynamics in Heisenberg system with Dzyaloshinskii–Moriya interaction 表征具有 Dzyaloshinskii-Moriya 相互作用的海森堡系统中的量子关联动力学
IF 2 3区 物理与天体物理 Q3 OPTICS Pub Date : 2024-08-19 DOI: 10.1007/s00340-024-08305-x
Rachid Ben hammou, Noureddine Benrass, Khadija El Anouz, Nabil Habiballah, Abderrahim El Allati

In this paper, we investigate the dynamics of quantum correlation using a Heisenberg spin system in the presence of the Dzyaloshinskii–Moriya interaction (DM) and an external magnetic field. Indeed, quantum discord and its geometrical aspects, namely the trace and Hellinger distances, have been exploited in order to study quantum correlation evolution using the Lindblad master equation. A substantial enhancement in geometric quantum discord (GQD) is observed when the values of DM increase. Moreover, our results show that the geometric quantum discord undergoes a decrease in function of the external magnetic field; except for the small values, its maximum is reached. However, we find that strong values of the temperature have a destructive effect on the behavior of GQD.

在本文中,我们利用一个海森堡自旋系统,在杜扎洛辛斯基-莫里亚相互作用(DM)和外部磁场的作用下,研究了量子相关性的动力学。事实上,量子不和及其几何方面,即痕量距离和海灵格距离,已被用来利用林德布拉德主方程研究量子相关性的演化。当 DM 值增大时,几何量子不和谐(GQD)会显著增强。此外,我们的研究结果表明,几何量子不和随外部磁场的变化而减小;除了很小的数值外,几何量子不和达到了最大值。然而,我们发现温度值过高会对 GQD 的行为产生破坏性影响。
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引用次数: 0
Skew information correlations and coherence in the Ising-XYZ diamond chain under an external magnetic field 外磁场下 Ising-XYZ 金刚石链的偏斜信息相关性和相干性
IF 2 3区 物理与天体物理 Q3 OPTICS Pub Date : 2024-08-17 DOI: 10.1007/s00340-024-08298-7
Aicha Chouiba, Essalha Chaouki, Youssef Khedif, Mostafa Mansour

This research investigates the interplay between coherence and skew information correlations in the Ising-({textbf {XYZ}}) diamond chain, which includes both Ising and Heisenberg spin particles in the presence of an external magnetic field. The initial step involves determining the reduced density matrix using the transfer matrix approach (TMA). Following this, quantum correlations and coherence in the Ising-({textbf {XYZ}}) diamond chain are quantified using uncertainty-induced nonlocality (UIN), local quantum uncertainty (LQU), and the (ell _1) norm of coherence ((C_{ell _1})). The study examines the impact of thermal noise and various system parameters, such as the xy-anisotropy (alpha), Heisenberg interaction (Gamma) among interstitial sites, Ising spin exchange (J_1), and magnetic field strength, on the dynamics of quantum resources within the system. The results indicate that both temperature and magnetic field negatively affect these quantum properties. Conversely, values of the xy-anisotropy parameter enhance quantum correlation and coherence, mitigating the detrimental impact of absolute temperature. This research offers significant insights into the behavior of quantum resources in this specific system.

本研究调查了 Ising-({textbf {XYZ}})金刚石链中相干性和倾斜信息相关性之间的相互作用,该金刚石链包括在外部磁场存在下的 Ising 和 Heisenberg 自旋粒子。第一步是使用转移矩阵方法(TMA)确定还原密度矩阵。随后,利用不确定性诱导的非位置性(UIN)、局部量子不确定性(LQU)和相干性的(ell _1)规范((C_ell _1}))量化了 Ising-({textbf {XYZ}})金刚石链中的量子相关性和相干性。研究考察了热噪声和各种系统参数,如 xy-各向异性(xy-anisotropy (α))、间隙位点之间的海森堡相互作用(Heisenberg interaction (γ))、伊星自旋交换(Ising spin exchange (J_1))和磁场强度对系统内量子资源动态的影响。结果表明,温度和磁场都会对这些量子特性产生负面影响。相反,xy-各向异性参数值增强了量子相关性和相干性,减轻了绝对温度的不利影响。这项研究为了解这一特定系统中量子资源的行为提供了重要启示。
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引用次数: 0
Beating of dark hollow laser beams in magnetized plasma under the influence of D.C. electric field to generate THz radiation 在直流电场的影响下,暗空心激光束在磁化等离子体中跳动以产生太赫兹辐射
IF 2 3区 物理与天体物理 Q3 OPTICS Pub Date : 2024-08-14 DOI: 10.1007/s00340-024-08296-9
Vishal Thakur, Sandeep Kumar

In the present theoretical analysis, a new scheme of terahertz (THz) generation is proposed by beating of the two dark hollow laser beams (DHLBs) in the magnetized plasma under the influence of a D.C. electric field. The D.C. electric and static magnetic fields are applied mutually perpendicular to each other as well as to the direction of propagation of DHLBs. The nonlinear current density becomes strong due to the coupling between the nonlinear density and D.C. drift velocity of the electrons of magnetized plasma which is further responsible for THz generation. The normalized THz amplitude shows enhancement with the increase of D.C. electric and static magnetic fields. The dark-size parameter and beam order also play a significant role in the enhancement of the THz generation. The present scheme is capable of generating THz radiation at laser intensities ( ,10^{14} ;{text{W}}/{text{cm}}^2), the magnetic field ( 38;{text{kG}}), D.C. electric field (45;{text{kV}}/{text{cm}},) and electron temperature ( ,6;{text{keV}}.) We have also considered the mutual interactions between the DHLBs and emitted THz radiation with magnetized plasma to provide more practical and accurate results. This scheme can be proved to be very effective and helpful in developing a proper tunable THz source for the investigation of histopathological samples, Bessel cell carcinoma tissues, and the treatment of tumors.

在本理论分析中,提出了一种新的太赫兹(THz)产生方案,即在直流电场的影响下,两束暗空心激光束(DHLB)在磁化等离子体中跳动。直流电场和静态磁场相互垂直,也相互垂直于 DHLB 的传播方向。由于磁化等离子体电子的非线性密度和直流漂移速度之间的耦合作用,非线性电流密度变得很强,这进一步导致了太赫兹的产生。归一化太赫兹振幅随着直流电场和静态磁场的增加而增强。暗尺寸参数和光束阶次对太赫兹产生的增强也起着重要作用。本方案能够在激光强度( ,10^{14} ;{text{W}}/ {text{cm}}^2)、磁场( 38;{text{kG}}), D.C.我们还考虑了DHLBs和发射的太赫兹辐射与磁化等离子体之间的相互作用,以提供更实用、更准确的结果。该方案可以证明是非常有效的,有助于开发一种合适的可调谐太赫兹源,用于组织病理学样本、贝塞尔细胞癌组织的研究和肿瘤的治疗。
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引用次数: 0
Enhanced emission in the NIR range by Nd3+ doped borosilicate glass for lasing applications 掺杂钕3+的硼硅玻璃在近红外范围内的增强发射,用于激光应用
IF 2 3区 物理与天体物理 Q3 OPTICS Pub Date : 2024-08-12 DOI: 10.1007/s00340-024-08294-x
Yasha Tayal, Rupesh A. Talewar, Sk. Mahamuda, Kartika Maheshwari, Sheetal Kumari, Mohit Kumar, Ravita Pilania, Aman Prasad, A. S. Rao

Borosilicate glasses were prepared via melt quench technique with different concentration of Nd3+ ions. X-ray diffraction (XRD) was performed for the prepared glass to study the amorphous structure. The glass stability was studied by Thermo-gravimetric Analysis (TGA). Spectroscopic analysis of the prepared glasses was done through absorption, excitation, emission and decay measurements. Absorption spectra was used to evaluate the J-O parameters. Radiative parameters are evaluated with the help of application of J-O theory. Emission spectra show three prominent bands in NIR region arising from 4F3/2 → 4I9/2, 4I11/2 and 4I13/2 centered around 910, 1068 and 1339 nm accordingly, with the most intense being the one at 1068 nm. Stimulated emission cross section, branching ratio and quantum efficiency for 4F3/2 → 4I11/2 transition is very high and is suitable for lasing applications. Dipole–dipole interaction is observed among activator ions on the basis of Dexter theory. The optimized Nd3+ doped glass (NBS10) possess maximum value for all radiative parameters and hence can be best suited for applications in the area of lasers and fiber amplifiers.

通过熔体淬火技术,使用不同浓度的 Nd3+ 离子制备了硼硅玻璃。对制备的玻璃进行了 X 射线衍射 (XRD),以研究其无定形结构。通过热重分析法(TGA)研究了玻璃的稳定性。通过吸收、激发、发射和衰变测量对制备的玻璃进行了光谱分析。吸收光谱用于评估 J-O 参数。借助 J-O 理论的应用评估了辐射参数。发射光谱显示,在近红外区域,4F3/2 → 4I9/2、4I11/2 和 4I13/2 产生了三个突出的波段,分别位于 910、1068 和 1339 纳米波段,其中波段最长的是 1068 纳米波段。4F3/2 → 4I11/2 转变的受激发射截面、支化比和量子效率都非常高,适合激光应用。根据 Dexter 理论,活化剂离子之间存在偶极-偶极相互作用。优化后的掺钕玻璃(NBS10)的所有辐射参数都达到了最大值,因此最适合应用于激光器和光纤放大器领域。
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引用次数: 0
Multiphoton absorption with Laguerre-Gaussian beams 拉盖尔-高斯光束的多光子吸收
IF 2 3区 物理与天体物理 Q3 OPTICS Pub Date : 2024-08-09 DOI: 10.1007/s00340-024-08297-8
Ferhat Kessi

Laguerre-Gaussian beams possess a unique transverse mode structure defined by the orbital (l) and radial (m) mode numbers, offering promising potential for controlling nonlinear optical interactions. This comprehensive study aims to elucidate the crucial influence of this transverse mode structure on the nonlinear absorption processes. We first established a rigorous theoretical framework by deriving analytical expressions describing the behavior of the Open Z-scan normalized optical transmittance for an arbitrary nth-order nonlinear process under the weak nonlinearity approximation, accounting for the transmitted optical intensity, power, and their dependency on the beam’s transverse mode profile. In the numerical simulations, we focused on the specific case of second-order ((n=2)) nonlinear absorption. Subsequently, detailed numerical simulations were employed to systematically analyze the intricate interplay between the (l) and (m) mode indices and their impact on the transmittance characteristics. By precisely varying these indices, we investigated how the observed transmission profiles were affected, revealing distinct behaviors for different Laguerre-Gaussian modes. When only (m) increases, absorption decreases due to the wider transverse energy spread, while varying (l) leads to a non-monotonic trend involving intense lobes. Remarkably, simultaneously increasing both (l) and (m) systematically enhances absorption through constructive interference of the helical and ring-like structures.

拉盖尔-高斯光束具有独特的横向模式结构,由轨道(l)和径向(m)模式数定义,为控制非线性光学相互作用提供了巨大潜力。这项综合研究旨在阐明这种横向模式结构对非线性吸收过程的关键影响。我们首先建立了一个严格的理论框架,在弱非线性近似条件下推导出了描述任意 n 阶非线性过程的 Open Z 扫描归一化光学透射率行为的分析表达式,并考虑了透射光强度、功率及其与光束横模剖面的关系。在数值模拟中,我们重点研究了二阶((n=2))非线性吸收的具体情况。随后,我们进行了详细的数值模拟,系统地分析了 (l) 和 (m) 模式指数之间错综复杂的相互作用及其对透射特性的影响。通过精确地改变这些指数,我们研究了观察到的透射曲线是如何受到影响的,揭示了不同拉盖尔-高斯模式的不同行为。如果只增加(m),由于横向能量散布更广,吸收就会减少,而改变(l)则会导致一种非单调的趋势,涉及强烈的裂片。值得注意的是,同时增加(l)和(m)会通过螺旋和环状结构的建设性干扰系统地增强吸收。
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引用次数: 0
Analysis of beat frequencies of transverse mode degeneracy in diode-pumped Nd:YVO4 laser 二极管泵浦 Nd:YVO4 激光器中横向模式退化的节拍频率分析
IF 2 3区 物理与天体物理 Q3 OPTICS Pub Date : 2024-08-07 DOI: 10.1007/s00340-024-08293-y
Jing Wang, Da Lin, Zhanglang Lin, Bingxuan Li, Wenbin Liao, Ge Zhang

This paper provides a detailed analysis of transverse mode degeneracy process of end-pumped Nd:(hbox {YVO}_4) laser. By observing the intersection of the beat frequency signals in the concave-plano cavity, the exact cavity length position of the transverse mode degeneracy can be clearly identified, which is also where transverse-mode locking occurs. Investigating the positions of the degeneracy of 1/3 and 2/7 reveals that transverse-mode locking occurs within the micrometer range. Our results give a simple and intuitive description of frequency degeneracy in a common solid-state laser

本文详细分析了端泵浦Nd:(hbox {YVO}_4)激光器的横向模式退化过程。通过观察凹面-平面腔中拍频信号的交点,可以清楚地确定横向模式退化的确切腔长位置,这也是横向模式锁定发生的位置。对 1/3 和 2/7 退化位置的研究表明,横向模式锁定发生在微米范围内。我们的研究结果简单直观地描述了普通固体激光器的频率退化现象
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引用次数: 0
InAs three quantum dots as working substance for quantum heat engines 作为量子热引擎工作物质的 InAs 三量子点
IF 2 3区 物理与天体物理 Q3 OPTICS Pub Date : 2024-08-05 DOI: 10.1007/s00340-024-08291-0
H. Ait Mansour, F. El Ayachi, M. Faqir, M. El Baz

Heat engines are considered a valuable resource for the modern society. The development of these systems leads to the production of heat engines with high efficiency despite their small size, called quantum heat engines. Among these, the quantum Otto cycle which is considered a fundamental thermodynamic cycle in classical heat engines, has also found applications in the realm of quantum heat engines. In this paper, we consider three InAs quantum dots as a working substance, which allows the engine to operate at very small scales, in the presence of an electric field, and the Förster mechanism, which describes the transfer of energy between quantum dots and thus affects the engine’s behavior. In this regard, we study the behavior of the work performed by the engine and the entanglement in the system as the Förster parameter is varied. We found a significant link between the engine’s work performance, the system’s entanglement, and the Förster interaction. At a critical Förster interaction value, which depends on the excitons frequencies, we observe a sharp inflection in work output. This transition coincides with the system reaching maximum entanglement after a separable state.

热机被认为是现代社会的宝贵资源。随着这些系统的发展,人们制造出了体积虽小但效率很高的热机,即量子热机。其中,量子奥托循环被认为是经典热机的基本热力学循环,在量子热机领域也有应用。在本文中,我们将三个砷化铟量子点视为工作物质,这使得发动机可以在电场存在的情况下,在非常小的尺度上运行,而弗斯特机制则描述了量子点之间的能量转移,从而影响了发动机的行为。在这方面,我们研究了随着佛斯特参数的变化,引擎所做的功和系统中纠缠的行为。我们发现,发动机的工作性能、系统的纠缠度和佛斯特相互作用之间存在重要联系。在一个取决于激子频率的临界佛斯特相互作用值上,我们观察到工作输出出现了一个急剧的拐点。这一转变与系统在可分离状态后达到最大纠缠度相吻合。
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引用次数: 0
期刊
Applied Physics B
全部 Acc. Chem. Res. ACS Applied Bio Materials ACS Appl. Electron. Mater. ACS Appl. Energy Mater. ACS Appl. Mater. Interfaces ACS Appl. Nano Mater. ACS Appl. Polym. Mater. ACS BIOMATER-SCI ENG ACS Catal. ACS Cent. Sci. ACS Chem. Biol. ACS Chemical Health & Safety ACS Chem. Neurosci. ACS Comb. Sci. ACS Earth Space Chem. ACS Energy Lett. ACS Infect. Dis. ACS Macro Lett. ACS Mater. Lett. ACS Med. Chem. Lett. ACS Nano ACS Omega ACS Photonics ACS Sens. ACS Sustainable Chem. Eng. ACS Synth. Biol. Anal. Chem. BIOCHEMISTRY-US Bioconjugate Chem. BIOMACROMOLECULES Chem. Res. Toxicol. Chem. Rev. Chem. Mater. CRYST GROWTH DES ENERG FUEL Environ. Sci. Technol. Environ. Sci. Technol. Lett. Eur. J. Inorg. Chem. IND ENG CHEM RES Inorg. Chem. J. Agric. Food. Chem. J. Chem. Eng. Data J. Chem. Educ. J. Chem. Inf. Model. J. Chem. Theory Comput. J. Med. Chem. J. Nat. Prod. J PROTEOME RES J. Am. Chem. Soc. LANGMUIR MACROMOLECULES Mol. Pharmaceutics Nano Lett. Org. Lett. ORG PROCESS RES DEV ORGANOMETALLICS J. Org. Chem. J. Phys. Chem. J. Phys. Chem. A J. Phys. Chem. B J. Phys. Chem. C J. Phys. Chem. Lett. Analyst Anal. Methods Biomater. Sci. Catal. Sci. Technol. Chem. Commun. Chem. Soc. Rev. CHEM EDUC RES PRACT CRYSTENGCOMM Dalton Trans. Energy Environ. Sci. ENVIRON SCI-NANO ENVIRON SCI-PROC IMP ENVIRON SCI-WAT RES Faraday Discuss. Food Funct. Green Chem. Inorg. Chem. Front. Integr. Biol. J. Anal. At. Spectrom. J. Mater. Chem. A J. Mater. Chem. B J. Mater. Chem. C Lab Chip Mater. Chem. Front. Mater. Horiz. MEDCHEMCOMM Metallomics Mol. Biosyst. Mol. Syst. Des. Eng. Nanoscale Nanoscale Horiz. Nat. Prod. Rep. New J. Chem. Org. Biomol. Chem. Org. Chem. Front. PHOTOCH PHOTOBIO SCI PCCP Polym. Chem.
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