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Confined gas transport in low-dimensional materials 低维材料中的封闭气体输送
IF 3.9 3区 材料科学 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-01-07 DOI: 10.1080/19475411.2023.2300348
Hongwei Duan, Zeyu Zhuang, Jing Yang, Shengping Zhang, Luda Wang
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引用次数: 0
The rate dependence of the dielectric strength of dielectric elastomers 介电弹性体介电强度的速率依赖性
IF 3.9 3区 材料科学 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-01-03 DOI: 10.1080/19475411.2023.2299411
Xianghe Zheng, Jianyou Zhou, Pan Jia, Zheng Zhong
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引用次数: 0
Multi-stable straw-like carbon nanotubes for mechanical programmability at microscale 用于微尺度机械可编程性的多稳定稻草状碳纳米管
IF 3.9 3区 材料科学 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2023-12-21 DOI: 10.1080/19475411.2023.2296901
Jia Liu, Yong Ma, Wanjie Ren, Fei Pan, Shu Guo, Yuli Chen, Bin Ding
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引用次数: 0
Selective and asymmetric ion transport in covalent organic framework-based two-dimensional nanofluidic devices 基于共价有机框架的二维纳米流体设备中的选择性和非对称离子传输
IF 3.9 3区 材料科学 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2023-12-06 DOI: 10.1080/19475411.2023.2288954
Li-Qiu Huang, Shuang Chen, Ri-Jian Mo, Zhong-Qiu Li, Xing-Hua Xia
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引用次数: 0
Nanodiamond reinforced self-healing and transparent poly(urethane–urea) protective coating for scratch resistance 纳米金刚石增强型自愈合透明聚(尿烷-尿素)保护涂层,具有抗划伤性能
IF 3.9 3区 材料科学 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2023-12-03 DOI: 10.1080/19475411.2023.2289608
Zhuochao Wang, Wenxin Cao, Chunqiang Sun, Dongchao Ji, Kunlong Zhao, Gang Gao, Xingchun Xu, Yingqi Liu, Tianyu Zhang, Jiaqi Zhu, Jiecai Han
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引用次数: 0
Analysis of nonlinear multi-field coupling responses of piezoelectric semiconductor rods via machine learning 通过机器学习分析压电半导体棒的非线性多场耦合响应
IF 3.9 3区 材料科学 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2023-11-17 DOI: 10.1080/19475411.2023.2282780
Chuwei Wu, Zhengguang Xiao, Yuting Guo, Chunli Zhang
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引用次数: 0
SMA-origami coupling: online configuration switches and stability property modulation sma -折纸耦合:在线配置开关和稳定性调制
3区 材料科学 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2023-10-28 DOI: 10.1080/19475411.2023.2271584
Hai Zhou, Hongbin Fang, Zuolin Liu, Jian Xu
Active folding is a crucial requirement for practical applications of multi-stable origami structures. However, research on integrating active materials with origami structures to enable quick configuration switching and modulation of stability properties is still in its early stages. To advance the state-of-the-art, we designed a coupled structure comprising a stacked Miura-origami (SMO) structure and two Shape Memory Alloy (SMA) actuators. One actuator is used for extruding the SMO structure while the other is used for retracting, thereby realizing bidirectional reversible active folding of the coupled structure. Modeling the potential energy of the coupled structure shows that it can be switched between monostable and bistable by heating the SMA actuators. The above findings are also confirmed by experiments conducted on a delicate SMO-SMA coupled structure prototype. The activation of different actuators induces rapid configuration switching of the coupled structure, and the stability profile is qualitatively adjusted by designing the current loading profile to achieve steady-state temperature fluctuations. Overall, this study provides a new approach to coupling origami structures with smart materials for active folding and presents a novel method to regulate the stability property of origami structures, thus promoting their practical applications.
主动折叠是多稳定折纸结构实际应用的关键条件。然而,将活性材料与折纸结构相结合以实现构型快速切换和稳定性调制的研究仍处于早期阶段。为了推进最先进的技术,我们设计了一个由堆叠的三浦折纸(SMO)结构和两个形状记忆合金(SMA)致动器组成的耦合结构。一个驱动器用于挤压SMO结构,另一个驱动器用于收缩,从而实现耦合结构的双向可逆主动折叠。对耦合结构的势能建模表明,通过加热SMA致动器可以在单稳态和双稳态之间切换。上述发现也通过在精密的SMO-SMA耦合结构原型上的实验得到了证实。不同致动器的激活引起耦合结构的快速配置切换,通过设计电流加载曲线来定性调整稳定性曲线,以实现稳态温度波动。总之,本研究提供了一种将折纸结构与智能材料耦合进行主动折叠的新途径,并提出了一种调节折纸结构稳定性的新方法,从而促进了折纸结构的实际应用。
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引用次数: 0
Interplay between entanglement and crosslinking in determining mechanical behaviors of polymer networks 缠结和交联在决定聚合物网络力学行为中的相互作用
3区 材料科学 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2023-09-29 DOI: 10.1080/19475411.2023.2261777
Yuhao Liu, Weikang Xian, Jinlong He, Ying Li
In polymer physics, the concept of entanglement refers to the topological constraints between long polymer chains that are closely packed together. Both theory and experimentation suggest that entanglement has a significant influence on the mechanical properties of polymers. This indicates its promise for materials design across various applications. However, understanding the relationship between entanglement and mechanical properties is complex, especially due to challenges related to length scale constraints and the difficulties of direct experimental observation. This research delves into how the polymer network structure changes when deformed. We specifically examine the relationship between entanglement, crosslinked networks, and their roles in stretching both entangled and unentangled polymer systems. For unentangled polymers, our findings underscore the pivotal role of crosslinking bond strength in determining the system’s overall strength and resistance to deformation. As for entangled polymers, entanglement plays a pivotal role in load bearing during the initial stretching stage, preserving the integrity of the polymer network. As the stretching continues and entanglement diminishes, the responsibility for bearing the load increasingly shifts to the crosslinking network, signifying a critical change in the system’s behavior. We noted a linear correlation between the increase in entanglement and the rise in tensile stress during the initial stretching stage. Conversely, the destruction of the network correlates with a decrease in tensile stress in the later stage. The findings provide vital insights into the complex dynamics between entanglement and crosslinking in the stretching processes of polymer networks, offering valuable guidance for future manipulation and design of polymer materials to achieve desired mechanical properties.
在聚合物物理学中,缠结的概念是指紧密排列在一起的长聚合物链之间的拓扑约束。理论和实验都表明,缠结对聚合物的力学性能有重要影响。这表明了它在各种应用中的材料设计前景。然而,理解缠结和力学性能之间的关系是复杂的,特别是由于长度尺度限制和直接实验观察的困难。本研究探讨了聚合物网络结构在变形时的变化规律。我们特别研究了纠缠、交联网络之间的关系,以及它们在拉伸纠缠和非纠缠聚合物系统中的作用。对于未纠缠的聚合物,我们的研究结果强调了交联键强度在决定体系整体强度和抗变形能力方面的关键作用。对于缠结的聚合物,缠结在初始拉伸阶段的承载中起着关键作用,保持了聚合物网络的完整性。随着拉伸的继续和缠结的减少,承担载荷的责任越来越多地转移到交联网络,这标志着系统行为的关键变化。我们注意到,在初始拉伸阶段,缠结的增加与拉伸应力的上升之间存在线性相关。相反,网络的破坏与后期拉应力的降低相关。这些发现为聚合物网络拉伸过程中纠缠和交联之间的复杂动力学提供了重要的见解,为未来操作和设计聚合物材料提供了有价值的指导,以实现所需的机械性能。
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引用次数: 0
Failure mechanisms in flexible electronics 柔性电子的失效机制
3区 材料科学 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2023-09-27 DOI: 10.1080/19475411.2023.2261775
Zhehui Zhao, Haoran Fu, Ruitao Tang, Bocheng Zhang, Yunmin Chen, Jianqun Jiang
The rapid evolution of flexible electronic devices promises to revolutionize numerous fields by expanding the applications of smart devices. Nevertheless, despite this vast potential, the reliability of these innovative devices currently falls short, especially in light of demanding operation environment and the intrinsic challenges associated with their fabrication techniques. The heterogeneity in these processes and environments gives rise to unique failure modes throughout the devices’ lifespan. To significantly enhance the reliability of these devices and assure long-term performance, it is paramount to comprehend the underpinning failure mechanisms thoroughly, thereby enabling optimal design solutions. A myriad of investigative efforts have been dedicated to unravel these failure mechanisms, utilizing a spectrum of tools from analytical models, numerical methods, to advanced characterization methods. This review delves into the root causes of device failure, scrutinizing both the fabrication process and the operation environment. Next, We subsequently address the failure mechanisms across four commonly observed modes: strength failure, fatigue failure, interfacial failure, and electrical failure, followed by an overview of targeted characterization methods associated with each mechanism. Concluding with an outlook, we spotlight ongoing challenges and promising directions for future research in our pursuit of highly resilient flexible electronic devices.
柔性电子设备的快速发展有望通过扩展智能设备的应用来彻底改变许多领域。然而,尽管有巨大的潜力,这些创新设备的可靠性目前还不足,特别是考虑到苛刻的操作环境和与制造技术相关的内在挑战。这些过程和环境的异质性在设备的整个使用寿命中产生了独特的故障模式。为了显著提高这些设备的可靠性并确保长期性能,彻底了解基本故障机制至关重要,从而实现最佳设计解决方案。无数的调查工作已经致力于解开这些失效机制,利用一系列工具,从分析模型,数值方法,到先进的表征方法。这次审查深入到设备故障的根本原因,仔细检查制造过程和操作环境。接下来,我们随后讨论了四种常见模式的失效机制:强度失效、疲劳失效、界面失效和电气失效,然后概述了与每种机制相关的目标表征方法。最后,展望了我们在追求高弹性柔性电子器件的过程中所面临的挑战和未来研究的有希望的方向。
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引用次数: 0
Self-sensing magnetic actuators of bilayer hydrogels 双层水凝胶的自传感磁致动器
3区 材料科学 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2023-09-21 DOI: 10.1080/19475411.2023.2257616
Shengyuan Zhang, Huangsan Wei, Jingda Tang
Hard magnetic soft robots have been widely used in biomedical engineering. In these applications, it is crucial to sense the movement of soft robots and their interaction with target objects. Here, we propose a strategy to fabricate a self-sensing bilayer actuator by combining magnetic and ionic conductive hydrogels. The magnetic hydrogel containing NdFeB particles exhibits rapid response to magnetic field and achieve bending deformation. Meanwhile, the polyacrylamide (PAAm) hydrogel with lithium chloride (LiCl) allows for the sensing of deformation. The bending behavior of the bilayer under magnetic field is well captured by theoretical and simulated models. Additionally, the bilayer strain sensor shows good sensitivity, stability and can endure a wide-range cyclic stretching (0–300%). These merits qualify the self-sensing actuator to monitor the motion signals, such as bending of fingers and grasping process of an intelligent gripper. When subject to an external magnetic field, the gripper can grab a cube and sense the resistance change simultaneously to detect the object size. This work may provide a versatile strategy to integrate actuating and self-sensing ability in soft robots.
硬磁软机器人在生物医学工程中有着广泛的应用。在这些应用中,感知软体机器人的运动及其与目标物体的交互是至关重要的。在此,我们提出了一种结合磁性和离子导电水凝胶制备自传感双层致动器的策略。含钕铁硼的磁性水凝胶对磁场的响应速度快,可实现弯曲变形。同时,含有氯化锂(LiCl)的聚丙烯酰胺(PAAm)水凝胶可以感知变形。理论模型和模拟模型都很好地反映了双分子层在磁场作用下的弯曲行为。此外,双层应变传感器具有良好的灵敏度和稳定性,可以承受大范围的循环拉伸(0-300%)。这些优点使自传感作动器能够监测智能抓手的手指弯曲和抓取过程等运动信号。当受到外部磁场的影响时,抓手可以抓住一个立方体,同时感知电阻的变化,以检测物体的大小。这项工作为软机器人的驱动和自感知能力的集成提供了一种通用的策略。
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International Journal of Smart and Nano Materials
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