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Insights into the spatial distribution of global, national, and subnational greenhouse gas emissions in the Emissions Database for Global Atmospheric Research (EDGAR v8.0) 洞察全球大气研究排放数据库(EDGAR v8.0)中全球、国家和国家以下各级温室气体排放的空间分布情况
IF 11.4 1区 地球科学 Q1 Earth and Planetary Sciences Pub Date : 2024-06-14 DOI: 10.5194/essd-16-2811-2024
Monica Crippa, Diego Guizzardi, Federico Pagani, Marcello Schiavina, Michele Melchiorri, Enrico Pisoni, Francesco Graziosi, Marilena Muntean, Joachim Maes, Lewis Dijkstra, Martin Van Damme, Lieven Clarisse, Pierre Coheur
Abstract. To mitigate the impact of greenhouse gas (GHG) and air pollutant emissions, it is of utmost importance to understand where emissions occur. In the real world, atmospheric pollutants are produced by various human activities from point sources (e.g. power plants and industrial facilities) but also from diffuse sources (e.g. residential activities and agriculture). However, as tracking all these single sources of emissions is practically impossible, emission inventories are typically compiled using national-level statistics by sector, which are then downscaled at the grid-cell level using spatial information. In this work, we develop high-spatial-resolution proxies for use in downscaling the national emission totals for all world countries provided by the Emissions Database for Global Atmospheric Research (EDGAR). In particular, in this paper, we present the latest EDGAR v8.0 GHG, which provides readily available emission data at different levels of spatial granularity, obtained from a consistently developed GHG emission database. This has been achieved through the improvement and development of high-resolution spatial proxies that allow for a more precise allocation of emissions over the globe. A key novelty of this work is the potential to analyse subnational GHG emissions over the European territory and also over the United States, China, India, and other high-emitting countries. These data not only meet the needs of atmospheric modellers but can also inform policymakers working in the field of climate change mitigation. For example, the EDGAR GHG emissions at the NUTS 2 level (Nomenclature of Territorial Units for Statistics level 2) over Europe contribute to the development of EU cohesion policies, identifying the progress of each region towards achieving the carbon neutrality target and providing insights into the highest-emitting sectors. The data can be accessed at https://doi.org/10.2905/b54d8149-2864-4fb9-96b9-5fd3a020c224 specifically for EDGAR v8.0 (Crippa et al., 2023a) and https://doi.org/10.2905/D67EEDA8-C03E-4421-95D0-0ADC460B9658 for the subnational dataset (Crippa et al., 2023b).
摘要要减轻温室气体(GHG)和空气污染物排放的影响,最重要的是要了解排放发生在哪里。在现实世界中,点源(如发电厂和工业设施)和扩散源(如住宅活动和农业)等各种人类活动都会产生大气污染物。然而,由于跟踪所有这些单一排放源实际上是不可能的,因此排放清单通常采用按部门划分的国家级统计数据进行编制,然后利用空间信息在网格单元级别进行缩减。在这项工作中,我们开发了高空间分辨率代用指标,用于缩减全球大气研究排放数据库(EDGAR)提供的世界各国的国家排放总量。特别是在本文中,我们介绍了最新的 EDGAR v8.0 GHG,它提供了不同空间粒度级别的现成排放数据,这些数据都是从持续开发的温室气体排放数据库中获得的。这是通过改进和开发高分辨率空间代用指标实现的,可以更精确地分配全球范围内的排放量。这项工作的一个主要创新点是可以分析欧洲领土以及美国、中国、印度和其他高排放国家的次国家温室气体排放量。这些数据不仅能满足大气建模人员的需求,还能为气候变化减缓领域的政策制定者提供信息。例如,EDGAR 提供的欧洲 NUTS 2 级(第二级统计领土单位术语)温室气体排放数据有助于欧盟制定凝聚力政策,确定各地区在实现碳中和目标方面的进展情况,并深入分析排放最高的部门。这些数据可在以下网站获取:https://doi.org/10.2905/b54d8149-2864-4fb9-96b9-5fd3a020c224,特别是 EDGAR v8.0(Crippa 等人,2023a)和 https://doi.org/10.2905/D67EEDA8-C03E-4421-95D0-0ADC460B9658,用于国家以下数据集(Crippa 等人,2023b)。
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引用次数: 0
LamaH-Ice: LArge-SaMple DAta for Hydrology and Environmental Sciences for Iceland LamaH-Ice:冰岛水文和环境科学实验室(LArge-SaMple DAta for Hydrology and Environmental Sciences for Iceland
IF 11.4 1区 地球科学 Q1 Earth and Planetary Sciences Pub Date : 2024-06-13 DOI: 10.5194/essd-16-2741-2024
Hordur Bragi Helgason, Bart Nijssen
Abstract. Access to mountainous regions for monitoring streamflow, snow and glaciers is often difficult, and many rivers are thus not gauged and hydrological measurements are limited. Consequently, cold-region watersheds, particularly heavily glacierized ones, are poorly represented in large-sample hydrology (LSH) datasets. We present a new LSH dataset for Iceland, termed LamaH-Ice (LArge-SaMple DAta for Hydrology and Environmental Sciences for Iceland). Glaciers and ice caps cover about 10 % of Iceland and, while streamflow has been measured for several decades, these measurements have not previously been published in a consistent manner. The dataset provides daily and hourly hydrometeorological time series and catchment characteristics for 107 river basins in Iceland, covering an area of almost 46 000 km2 (45 % of Iceland's area), with catchment sizes ranging from 4 to 7500 km2. LamaH-Ice conforms to the structure of existing LSH datasets and includes most variables contained in these datasets as well as additional information relevant to cold-region hydrology, e.g., time series of snow cover, glacier mass balance and albedo. LamaH-Ice also includes dynamic catchment characteristics to account for changes in land cover, vegetation and glacier extent. A large majority of the watersheds in LamaH-Ice are not subject to human activities, such as diversions and flow regulations. Streamflow measurements under natural flow conditions are highly valuable to hydrologists seeking to model and comprehend the natural hydrological cycle or estimate climate change trends. The LamaH-Ice dataset (Helgason and Nijssen, 2024) is intended for the research community to improve the understanding of hydrology in cold-region environments. LamaH-Ice is publicly available on HydroShare at https://doi.org/10.4211/hs.86117a5f36cc4b7c90a5d54e18161c91 (Helgason and Nijssen, 2024).
摘要要进入山区监测溪流、积雪和冰川往往很困难,因此许多河流都没有测站,水文测量也很有限。因此,寒冷地区的流域,尤其是冰川化严重的流域,在大样本水文(LSH)数据集中的代表性很差。我们为冰岛提供了一个新的 LSH 数据集,名为 LamaH-Ice(冰岛水文和环境科学 LArge-SaMple DAta)。冰川和冰盖覆盖了冰岛约 10% 的面积,虽然对溪流的测量已有数十年历史,但这些测量数据此前并未以一致的方式发布。该数据集提供了冰岛 107 个河流流域的每日和每小时水文气象时间序列以及流域特征,覆盖面积近 46000 平方公里(占冰岛国土面积的 45%),流域面积从 4 到 7500 平方公里不等。LamaH-Ice 符合现有 LSH 数据集的结构,包括这些数据集中的大多数变量以及与寒冷地区水文相关的附加信息,如雪覆盖、冰川质量平衡和反照率的时间序列。LamaH-Ice 还包括动态流域特征,以反映土地覆盖、植被和冰川范围的变化。LamaH-Ice 中的大部分流域不受人类活动的影响,如分流和流量调节。在自然水流条件下进行的水流测量对于水文学家模拟和理解自然水文循环或估计气候变化趋势非常有价值。LamaH-Ice 数据集(Helgason 和 Nijssen,2024 年)旨在帮助研究界更好地了解寒冷地区环境中的水文情况。LamaH-Ice 可在水文共享网站 https://doi.org/10.4211/hs.86117a5f36cc4b7c90a5d54e18161c91 上公开获取(Helgason 和 Nijssen,2024 年)。
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引用次数: 0
State of Wildfires 2023–24 2023-24 年野火状况
IF 11.4 1区 地球科学 Q1 Earth and Planetary Sciences Pub Date : 2024-06-13 DOI: 10.5194/essd-2024-218
Matthew W. Jones, Douglas I. Kelley, Chantelle A. Burton, Francesca Di Giuseppe, Maria Lucia F. Barbosa, Esther Brambleby, Andrew J. Hartley, Anna Lombardi, Guilherme Mataveli, Joe R. McNorton, Fiona R. Spuler, Jakob B. Wessel, John T. Abatzoglou, Liana O. Anderson, Niels Andela, Sally Archibald, Dolors Armenteras, Eleanor Burke, Rachel Carmenta, Emilio Chuvieco, Hamish Clarke, Stefan H. Doerr, Paulo M. Fernandes, Louis Giglio, Douglas S. Hamilton, Stijn Hantson, Sarah Harris, Piyush Jain, Crystal A. Kolden, Tiina Kurvits, Seppe Lampe, Sarah Meier, Stacey New, Mark Parrington, Morgane M. G. Perron, Yuquan Qu, Natasha S. Ribeiro, Bambang H. Saharjo, Jesus San-Miguel-Ayanz, Jacquelyn K. Shuman, Veerachai Tanpipat, Guido R. van der Werf, Sander Veraverbeke, Gavriil Xanthopoulos
Abstract. Climate change is increasing the frequency and intensity of wildfires globally, with significant impacts on society and the environment. However, our understanding of the global distribution of extreme fires remains skewed, primarily influenced by media coverage and regional research concentration. This inaugural State of Wildfires report systematically analyses fire activity worldwide, identifying extreme events from the March 2023–February 2024 fire season. We assess the causes, predictability, and attribution of these events to climate change and land use, and forecast future risks under different climate scenarios. During the 2023–24 fire season, 3.9 million km2 burned globally, slightly below the average of previous seasons, but fire carbon (C) emissions were 16 % above average, totaling 2.4 Pg C. This was driven by record emissions in Canadian boreal forests (over 9 times the average) and dampened by reduced activity in African savannahs. Notable events included record-breaking wildfire extent and emissions in Canada, the largest recorded wildfire in the European Union (Greece), drought-driven fires in western Amazonia and northern parts of South America, and deadly fires in Hawai’i (100 deaths) and Chile (131 deaths). Over 232,000 people were evacuated in Canada alone, highlighting the severity of human impact. Our analyses revealed that multiple drivers were needed to cause areas of extreme fire activity. In Canada and Greece a combination of high fire weather and an abundance of dry fuels increased the probability of fires by 4.5-fold and 1.9–4.1-fold, respectively, whereas fuel load and direct human suppression often modulated areas with anomalous burned area. The fire season in Canada was predictable three months in advance based on the fire weather index, whereas events in Greece and Amazonia had shorter predictability horizons. Formal attribution analyses indicated that the probability of extreme events has increased significantly due to anthropogenic climate change, with a 2.9–3.6-fold increase in likelihood of high fire weather in Canada and a 20.0–28.5-fold increase in Amazonia. By the end of the century, events of similar magnitude are projected to occur 2.22–9.58 times more frequently in Canada under high emission scenarios. Without mitigation, regions like Western Amazonia could see up to a 2.9-fold increase in extreme fire events. For the 2024–25 fire season, seasonal forecasts highlight moderate positive anomalies in fire weather for parts of western Canada and South America, but no clear signal for extreme anomalies is present in the forecast. This report represents our first annual effort to catalogue extreme wildfire events, explain their occurrence, and predict future risks. By consolidating state-of-the-art wildfire science and delivering key insights relevant to policymakers, disaster management services, firefighting agencies, and land managers, we aim to enhance society’s resilien
摘要气候变化正在增加全球野火的频率和强度,对社会和环境造成了重大影响。然而,我们对全球极端火灾分布情况的了解仍然存在偏差,主要受到媒体报道和地区研究集中度的影响。这份首次发布的《野火状况报告》系统分析了全球范围内的火灾活动,确定了 2023 年 3 月至 2024 年 2 月火灾季节的极端事件。我们评估了这些事件的起因、可预测性以及与气候变化和土地利用的关系,并预测了不同气候情景下的未来风险。在 2023-24 火灾季期间,全球有 390 万平方公里的土地被烧毁,略低于以往火灾季的平均水平,但火灾碳排放量却比平均水平高出 16%,总计达 2.4 Pg C。值得注意的事件包括加拿大破纪录的野火范围和排放量、欧盟(希腊)有记录以来最大的野火、亚马孙西部和南美洲北部干旱引发的火灾,以及夏威夷(100 人死亡)和智利(131 人死亡)的致命火灾。仅在加拿大就有超过 23.2 万人撤离,这凸显了人类影响的严重性。我们的分析表明,造成极端火灾活动的地区需要多种驱动因素。在加拿大和希腊,高火险天气和大量干燥燃料的结合使火灾发生的概率分别增加了 4.5 倍和 1.9-4.1 倍,而燃料负荷和人类的直接压制往往会调节异常燃烧区域。根据火灾气象指数,加拿大的火灾季节可提前三个月预测,而希腊和亚马孙地区的火灾可预测时间较短。正式的归因分析表明,由于人为气候变化,极端事件发生的概率显著增加,加拿大发生大火天气的可能性增加了 2.9-3.6 倍,亚马孙地区增加了 20.0-28.5 倍。预计到本世纪末,在高排放情景下,加拿大发生类似规模事件的频率将增加 2.22-9.58 倍。如果不采取减排措施,西亚马孙等地区的极端火灾事件可能会增加 2.9 倍。对于 2024-25 火灾季节,季节性预测强调加拿大西部和南美洲部分地区的火灾天气将出现中等程度的积极异常,但预测中没有出现极端异常的明确信号。本报告是我们首次对极端野火事件进行编目、解释其发生原因并预测未来风险的年度报告。通过整合最先进的野火科学知识,并提供与政策制定者、灾害管理部门、消防机构和土地管理者相关的重要见解,我们旨在提高社会对野火的适应能力,并促进备灾、减灾和适应方面的进步。
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引用次数: 0
A new multi-resolution bathymetric dataset of the Gulf of Naples (Italy) from complementary multi-beam echosounders 那不勒斯湾(意大利)新的多分辨率测深数据集(来自互补多波束回声测深仪
IF 11.4 1区 地球科学 Q1 Earth and Planetary Sciences Pub Date : 2024-06-13 DOI: 10.5194/essd-2024-135
Federica Foglini, Marzia Rovere, Renato Tonielli, Giorgio Castellan, Mariacristina Prampolini, Francesca Budillon, Marco Cuffaro, Gabriella Di Martino, Valentina Grande, Sara Innangi, Maria Filomena Loreto, Leonardo Langone, Fantina Madricardo, Alessandra Mercorella, Paolo Montagna, Camilla Palmiotto, Claudio Pellegrini, Antonio Petrizzo, Lorenzo Petracchini, Alessandro Remia, Marco Sacchi, Daphnie Sanchez Galvez, Anna Nora Tassetti, Fabio Trincardi
Abstract. High-resolution bathymetry provides critical information to marine geoscientists. Bathymetric big data help characterise the seafloor and its benthic habitats, understand sedimentary records, and support the development of offshore engineering infrastructures. From September 27th to October 20th, 2022, the new CNR Research Vessel GAIA BLU explored the seafloor of the Naples and Pozzuoli Gulfs, and the Amalfi coastal area (Tyrrhenian Sea, Italy) from 50 to more than 2000 m water depth, acquiring about 5000 km2 of multi beam echosounder data. This area is particularly vulnerable to abrupt changes driven by the dynamics of several volcanic complexes, active in the area, and by human-induced impacts reflecting the proximity to the highly populated and touristic coastal area of Naples and nearby famous islands. For these reasons, the seafloor of the area needs to be known and constantly monitored. The digital bathymetric data previously available are restricted to the shallow highly dynamic area of the Gulf of Naples and appear fragmented as they were acquired in successive years, with different goals thereby using a variety of devices, with markedly different spatial resolutions. In this paper, we present bathymetric maps of the Gulf of Naples and adjacent slope basins at unprecedented resolution using three state-of-the-art multi beam echosounders. These high-resolution data highlight the technological advances of geophysical surveys achieved over the last 20 years and contribute to assessing the most dynamic areas where changes in the seafloor over time can be quantified. The new digital multi-resolution bathymetric products are openly accessible via Marine Geosciences Data System MGDS (refer to section Data Availability, Table 8, for datasets and products DOIs), perfectly matching the FAIR (Findable, Accessible, Interoperable and Reusable) and Open Science Principles.
摘要。高分辨率测深为海洋地球科学家提供了关键信息。测深大数据有助于描述海底及其底栖生物栖息地的特征、了解沉积记录并支持近海工程基础设施的开发。2022 年 9 月 27 日至 10 月 20 日,新的 CNR 研究船 GAIA BLU 号探索了那不勒斯湾、波祖利湾和阿马尔菲沿海地区(意大利第勒尼安海)水深 50 米至 2000 多米的海底,获取了约 5000 平方公里的多波束回声测深仪数据。这一地区特别容易受到该地区活跃的几个火山群的动态变化和人类活动的影响而发生突变,这反映了该地区毗邻那不勒斯人口密集的旅游沿海地区和附近著名的岛屿。因此,需要了解并持续监测该地区的海底情况。以前可用的数字测深数据仅限于那不勒斯湾的浅海高动态区域,而且显得支离破碎,因为这些数据是在连续几年中获得的,目标各不相同,因此使用了各种设备,空间分辨率也明显不同。在本文中,我们使用三台最先进的多波束回声测深仪,以前所未有的分辨率绘制了那不勒斯湾及邻近斜坡盆地的测深图。这些高分辨率数据彰显了过去 20 年地球物理勘测技术的进步,有助于评估最具活力的区域,在这些区域可以量化海底随时间发生的变化。新的数字多分辨率测深产品可通过海洋地球科学数据系统 MGDS 公开获取(数据集和产品 DOI 参见表 8 "数据可用性 "部分),完全符合 FAIR(可查找、可获取、可互操作和可重用)和开放科学原则。
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引用次数: 0
IPB-MSA&SO4: a daily 0.25° resolution dataset of in situ-produced biogenic methanesulfonic acid and sulfate over the North Atlantic during 1998–2022 based on machine learning IPB-MSA&SO4:基于机器学习的 1998-2022 年北大西洋上空每日 0.25° 分辨率生物源甲烷磺酸和硫酸盐数据集
IF 11.4 1区 地球科学 Q1 Earth and Planetary Sciences Pub Date : 2024-06-12 DOI: 10.5194/essd-16-2717-2024
Karam Mansour, Stefano Decesari, Darius Ceburnis, Jurgita Ovadnevaite, Lynn M. Russell, Marco Paglione, Laurent Poulain, Shan Huang, Colin O'Dowd, Matteo Rinaldi
Abstract. Accurate long-term marine-derived biogenic sulfur aerosol concentrations at high spatial and temporal resolutions are critical for a wide range of studies, including climatology, trend analysis, and model evaluation; this information is also imperative for the accurate investigation of the contribution of marine-derived biogenic sulfur aerosol concentrations to the aerosol burden, for the elucidation of their radiative impacts, and to provide boundary conditions for regional models. By applying machine learning algorithms, we constructed the first publicly available daily gridded dataset of in situ-produced biogenic methanesulfonic acid (MSA) and non-sea-salt sulfate (nss-SO4=) concentrations covering the North Atlantic. The dataset is of high spatial resolution (0.25° × 0.25°) and spans 25 years (1998–2022), far exceeding what observations alone could achieve both spatially and temporally. The machine learning models were generated by combining in situ observations of sulfur aerosol data from Mace Head Atmospheric Research Station, located on the west coast of Ireland, and from the North Atlantic Aerosols and Marine Ecosystems Study (NAAMES) cruises in the northwestern Atlantic with the constructed sea-to-air dimethylsulfide flux (FDMS) and ECMWF ERA5 reanalysis datasets. To determine the optimal method for regression, we employed five machine learning model types: support vector machines, decision tree, regression ensemble, Gaussian process regression, and artificial neural networks. A comparison of the mean absolute error (MAE), root-mean-square error (RMSE), and coefficient of determination (R2) revealed that Gaussian process regression (GPR) was the most effective algorithm, outperforming the other models with respect to simulating the biogenic MSA and nss-SO4= concentrations. For predicting daily MSA (nss-SO4=), GPR displayed the highest R2 value of 0.86 (0.72) and the lowest MAE of 0.014 (0.10) µg m−3. GPR partial dependence analysis suggests that the relationships between predictors and MSA and nss-SO4= concentrations are complex rather than linear. Using the GPR algorithm, we produced a high-resolution daily dataset of in situ-produced biogenic MSA and nss-SO4= sea-level concentrations over the North Atlantic, which we named “In-situ Produced Biogenic Methanesulfonic Acid and Sulfate over the North Atlantic” (IPB-MSA&SO4). The obtained IPB-MSA&SO4 data allowed us to analyze the spatiotemporal patterns of MSA and nss-SO4= as well as the ratio between them (MSA:nss-SO4=). A comparison with the existing Copernicus Atmosphere Monitoring Service ECMWF Atmospheric Composition Reanalysis 4 (CAMS-EAC4) reanalysis suggested that our high-resolution dataset reproduces the spatial and temporal patterns of the biogenic sulfur aerosol concentration with high accuracy and has high consistency with independent measurements in the Atlantic Ocean. IPB-MSA&SO4 is publicly available at https://doi.org/10.17632/j8bzd5dvpx.1 (Mansour et al., 2023b)
摘要。准确的高时空分辨率海洋生物源硫气溶胶长期浓度对于气候学、趋势分析和模式评估等广泛研究至关重要;这些信息对于准确调查海洋生物源硫气溶胶浓度对气溶胶负荷的贡献、阐明其辐射影响以及为区域模式提供边界条件也是必不可少的。通过应用机器学习算法,我们构建了首个可公开获取的覆盖北大西洋的原地产生的生物源甲磺酸(MSA)和非海盐硫酸盐(nss-SO4=)浓度的日网格数据集。该数据集空间分辨率高(0.25°×0.25°),时间跨度长达 25 年(1998-2022 年),在空间和时间上都远远超过了单靠观测所能达到的水平。机器学习模型是通过将爱尔兰西海岸梅斯海德大气研究站和西北大西洋北大西洋气溶胶和海洋生态系统研究(NAAMES)巡航的硫气溶胶原位观测数据与构建的海气二甲基硫通量(FDMS)和 ECMWF ERA5 再分析数据集相结合而生成的。为了确定最佳回归方法,我们采用了五种机器学习模型类型:支持向量机、决策树、回归集合、高斯过程回归和人工神经网络。通过比较平均绝对误差(MAE)、均方根误差(RMSE)和判定系数(R2)发现,高斯过程回归(GPR)是最有效的算法,在模拟生物源 MSA 和 nss-SO4= 浓度方面优于其他模型。在预测每日 MSA(nss-SO4=)时,GPR 的 R2 值最高,为 0.86(0.72),MAE 最低,为 0.014(0.10) µg m-3。GPR 部分依存分析表明,预测因子与 MSA 和 nss-SO4= 浓度之间的关系是复杂的,而非线性的。利用 GPR 算法,我们生成了北大西洋上空原位生成的生物甲烷磺酸和 nss-SO4= 海平面浓度的高分辨率日数据集,并将其命名为 "北大西洋上空原位生成的生物甲烷磺酸和硫酸盐"(IPB-MSA&SO4)。利用获得的 IPB-MSA&SO4 数据,我们可以分析 MSA 和 nss-SO4= 的时空模式以及它们之间的比例(MSA:nss-SO4=)。与现有的哥白尼大气监测服务 ECMWF 大气成分再分析 4(CAMS-EAC4)再分析的比较表明,我们的高分辨率数据集高度准确地再现了生物源硫气溶胶浓度的时空模式,并与大西洋的独立测量结果高度一致。IPB-MSA&SO4 可在 https://doi.org/10.17632/j8bzd5dvpx.1 上公开获取(Mansour 等,2023b)。
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引用次数: 0
Global biogeography of N2-fixing microbes: nifH amplicon database and analytics workflow 固氮微生物的全球生物地理学:nifH 扩增子数据库和分析工作流程
IF 11.4 1区 地球科学 Q1 Earth and Planetary Sciences Pub Date : 2024-06-12 DOI: 10.5194/essd-2024-163
Michael Morando, Jonathan Magasin, Shunyan Cheung, Matthew M. Mills, Jonathan P. Zehr, Kendra A. Turk-Kubo
Abstract. Marine nitrogen (N) fixation is a globally significant biogeochemical process carried out by a specialized group of prokaryotes (diazotrophs), yet our understanding of their ecology is constantly evolving. Although marine dinitrogen (N2)-fixation is often ascribed to cyanobacterial diazotrophs, indirect evidence suggests that non-cyanobacterial diazotrophs (NCDs) might also be important. One widely used approach for understanding diazotroph diversity and biogeography is polymerase chain reaction (PCR)-amplification of a portion of the nifH gene, which encodes a structural component of the N2-fixing enzyme complex, nitrogenase. An array of bioinformatic tools exists to process nifH amplicon data, however, the lack of standardized practices has hindered cross-study comparisons. This has led to a missed opportunity to more thoroughly assess diazotroph biogeography, diversity, and their potential contributions to the marine N cycle. To address these knowledge gaps a bioinformatic workflow was designed that standardizes the processing of nifH amplicon datasets originating from high-throughput sequencing (HTS). Multiple datasets are efficiently and consistently processed with a specialized DADA2 pipeline to identify amplicon sequence variants (ASVs). A series of customizable post-pipeline stages then detect and discard spurious nifH sequences and annotate the subsequent quality-filtered nifH ASVs using multiple reference databases and classification approaches. This newly developed workflow was used to reprocess nearly all publicly available nifH amplicon HTS datasets from marine studies, and to generate a comprehensive nifH ASV database containing 7909 ASVs aggregated from 21 studies that represent the diazotrophic populations in the global ocean. For each sample, the database includes physical and chemical metadata obtained from the Simons Collaborative Marine Atlas Project (CMAP). Here we demonstrate the utility of this database for revealing global biogeographical patterns of prominent diazotroph groups and highlight the influence of sea surface temperature. The workflow and nifH ASV database provide a robust framework for studying marine N2 fixation and diazotrophic diversity captured by nifH amplicon HTS. Future datasets that target understudied ocean regions can be added easily, and users can tune parameters and studies included for their specific focus. The workflow and database are available, respectively, in GitHub (https://github.com/jdmagasin/nifH-ASV-workflow; Morando et al., 2024) and Figshare (https://doi.org/10.6084/m9.figshare.23795943.v1; Morando et al., 2024).
摘要海洋固氮(N)是一个具有全球意义的生物地球化学过程,由一组专门的原核生物(重氮营养体)进行,但我们对其生态学的了解却在不断发展。尽管海洋二氮(N2)固定过程通常是由蓝藻重氮营养体完成的,但间接证据表明,非蓝藻重氮营养体(NCD)可能也很重要。为了解重氮营养体的多样性和生物地理学,一种广泛使用的方法是聚合酶链式反应(PCR)--扩增 nifH 基因的一部分。目前有一系列生物信息学工具可用于处理 nifH 扩增子数据,但由于缺乏标准化方法,妨碍了跨研究比较。这导致我们错失了更全面地评估重氮营养生物地理学、多样性及其对海洋氮循环的潜在贡献的机会。为了填补这些知识空白,我们设计了一套生物信息学工作流程,对源自高通量测序(HTS)的 nifH 扩增子数据集进行标准化处理。利用专门的 DADA2 管道对多个数据集进行高效一致的处理,以识别扩增子序列变异(ASV)。然后,一系列可定制的后管道阶段会检测并剔除虚假的 nifH 序列,并利用多个参考数据库和分类方法对随后经过质量过滤的 nifH ASV 进行注释。这个新开发的工作流程被用于重新处理海洋研究中几乎所有公开的 nifH 扩增子 HTS 数据集,并生成一个全面的 nifH ASV 数据库,其中包含从 21 项研究中汇总的 7909 个 ASV,这些研究代表了全球海洋中的重氮营养种群。对于每个样本,数据库都包含从西蒙斯海洋图集合作项目(CMAP)中获得的物理和化学元数据。在此,我们展示了该数据库在揭示全球主要重氮营养群生物地理模式方面的实用性,并强调了海面温度的影响。该工作流程和 nifH ASV 数据库为研究海洋 N2 固定和 nifH 扩增子 HTS 捕获的重氮营养体多样性提供了一个强大的框架。未来,针对研究不足的海洋区域的数据集可以很容易地添加进来,用户可以根据自己的具体侧重点调整参数和研究内容。工作流程和数据库可分别在 GitHub (https://github.com/jdmagasin/nifH-ASV-workflow; Morando et al., 2024) 和 Figshare (https://doi.org/10.6084/m9.figshare.23795943.v1; Morando et al., 2024) 上查阅。
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引用次数: 0
Global nitrous oxide budget (1980–2020) 全球一氧化二氮预算(1980-2020 年)
IF 11.4 1区 地球科学 Q1 Earth and Planetary Sciences Pub Date : 2024-06-11 DOI: 10.5194/essd-16-2543-2024
Hanqin Tian, Naiqing Pan, Rona L. Thompson, Josep G. Canadell, Parvadha Suntharalingam, Pierre Regnier, Eric A. Davidson, Michael Prather, Philippe Ciais, Marilena Muntean, Shufen Pan, Wilfried Winiwarter, Sönke Zaehle, Feng Zhou, Robert B. Jackson, Hermann W. Bange, Sarah Berthet, Zihao Bian, Daniele Bianchi, Alexander F. Bouwman, Erik T. Buitenhuis, Geoffrey Dutton, Minpeng Hu, Akihiko Ito, Atul K. Jain, Aurich Jeltsch-Thömmes, Fortunat Joos, Sian Kou-Giesbrecht, Paul B. Krummel, Xin Lan, Angela Landolfi, Ronny Lauerwald, Ya Li, Chaoqun Lu, Taylor Maavara, Manfredi Manizza, Dylan B. Millet, Jens Mühle, Prabir K. Patra, Glen P. Peters, Xiaoyu Qin, Peter Raymond, Laure Resplandy, Judith A. Rosentreter, Hao Shi, Qing Sun, Daniele Tonina, Francesco N. Tubiello, Guido R. van der Werf, Nicolas Vuichard, Junjie Wang, Kelley C. Wells, Luke M. Western, Chris Wilson, Jia Yang, Yuanzhi Yao, Yongfa You, Qing Zhu
Abstract. Nitrous oxide (N2O) is a long-lived potent greenhouse gas and stratospheric ozone-depleting substance that has been accumulating in the atmosphere since the preindustrial period. The mole fraction of atmospheric N2O has increased by nearly 25 % from 270 ppb (parts per billion) in 1750 to 336 ppb in 2022, with the fastest annual growth rate since 1980 of more than 1.3 ppb yr−1 in both 2020 and 2021. According to the Sixth Assessment Report of the Intergovernmental Panel on Climate Change (IPCC AR6), the relative contribution of N2O to the total enhanced effective radiative forcing of greenhouse gases was 6.4 % for 1750–2022. As a core component of our global greenhouse gas assessments coordinated by the Global Carbon Project (GCP), our global N2O budget incorporates both natural and anthropogenic sources and sinks and accounts for the interactions between nitrogen additions and the biogeochemical processes that control N2O emissions. We use bottom-up (BU: inventory, statistical extrapolation of flux measurements, and process-based land and ocean modeling) and top-down (TD: atmospheric measurement-based inversion) approaches. We provide a comprehensive quantification of global N2O sources and sinks in 21 natural and anthropogenic categories in 18 regions between 1980 and 2020. We estimate that total annual anthropogenic N2O emissions have increased 40 % (or 1.9 Tg N yr−1) in the past 4 decades (1980–2020). Direct agricultural emissions in 2020 (3.9 Tg N yr−1, best estimate) represent the large majority of anthropogenic emissions, followed by other direct anthropogenic sources, including fossil fuel and industry, waste and wastewater, and biomass burning (2.1 Tg N yr−1), and indirect anthropogenic sources (1.3 Tg N yr−1) . For the year 2020, our best estimate of total BU emissions for natural and anthropogenic sources was 18.5 (lower–upper bounds: 10.6–27.0) Tg N yr−1, close to our TD estimate of 17.0 (16.6–17.4) Tg N yr−1. For the 2010–2019 period, the annual BU decadal-average emissions for both natural and anthropogenic sources were 18.2 (10.6–25.9) Tg N yr−1 and TD emissions were 17.4 (15.8–19.20) Tg N yr−1. The once top emitter Europe has reduced its emissions by 31 % since the 1980s, while those of emerging economies have grown, making China the top emitter since the 2010s. The observed atmospheric N2O concentrations in recent years have exceeded projected levels under all scenarios in the Coupled Model Intercomparison Project Phase 6 (CMIP6), underscoring the importance of reducing anthropogenic N2O emissions. To evaluate mitigation efforts and contribute to the Global Stocktake of the United Nations Framework Convention on Climate Change, we propose the establishment of a global network for monitoring and modeling N2O from the surface through to the stratosphere. The data presented in this work can be downloaded from https://doi.org/10.18160/RQ8P-2Z4R (Tian et al., 2023).
摘要一氧化二氮(N2O)是一种长寿命的强效温室气体和平流层臭氧消耗物质,自前工业化时期以来一直在大气中累积。大气中氧化亚氮的摩尔分数从 1750 年的 270 ppb(十亿分之一)增加到 2022 年的 336 ppb,增加了近 25%,其中 2020 年和 2021 年的年增长率超过 1.3 ppb-1,是自 1980 年以来最快的年增长率。根据《政府间气候变化专门委员会第六次评估报告》(IPCC AR6),1750-2022 年期间,一氧化二氮对温室气体总的增强有效辐射强迫的相对贡献率为 6.4%。作为全球碳项目(GCP)协调的全球温室气体评估的核心组成部分,我们的全球一氧化二氮预算包含了自然和人为源和汇,并考虑了氮添加和控制一氧化二氮排放的生物地球化学过程之间的相互作用。我们采用了自下而上(BU:清单、通量测量的统计外推法以及基于过程的陆地和海洋建模)和自上而下(TD:基于大气测量的反演)的方法。我们对 1980-2020 年间全球 18 个地区 21 个自然和人为类别的一氧化二氮源和汇进行了全面量化。我们估计,在过去 40 年(1980-2020 年)中,每年的人为一氧化二氮排放总量增加了 40%(或每年 1.9 兆吨氮)。2020 年的直接农业排放(3.9 Tg N yr-1,最佳估计值)占人为排放的绝大部分,其次是其他直接人为排放源,包括化石燃料和工业、废物和废水以及生物质燃烧(2.1 Tg N yr-1),以及间接人为排放源(1.3 Tg N yr-1)。对于 2020 年,我们对自然源和人为源的生物量总排放量的最佳估计值为 18.5(下限-上限:10.6-27.0)兆吨氮年-1,接近于我们的技术发展估算值 17.0(16.6-17.4)兆吨氮年-1。2010-2019 年期间,自然源和人为源的年均 BU 排放量为 18.2(10.6-25.9)兆吨氮年-1,TD 排放量为 17.4(15.8-19.20)兆吨氮年-1。曾经的最大排放国欧洲自 20 世纪 80 年代以来已减少了 31%的排放量,而新兴经济体的排放量却在增加,中国自 2010 年代以来已成为最大排放国。近年来观测到的大气中一氧化二氮浓度超过了耦合模式相互比较项目第六阶段(CMIP6)中所有情景下的预测水平,这凸显了减少人为一氧化二氮排放的重要性。为了评估减排工作并为《联合国气候变化框架公约》的全球评估做出贡献,我们建议建立一个全球网络,对从地表到平流层的一氧化二氮进行监测和建模。本研究中的数据可从 https://doi.org/10.18160/RQ8P-2Z4R 下载(Tian 等人,2023 年)。
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引用次数: 0
Multifrequency radar observations of marine clouds during the EPCAPE campaign EPCAPE 运动期间对海洋云层的多频雷达观测
IF 11.4 1区 地球科学 Q1 Earth and Planetary Sciences Pub Date : 2024-06-10 DOI: 10.5194/essd-16-2701-2024
Juan M. Socuellamos, Raquel Rodriguez Monje, Matthew D. Lebsock, Ken B. Cooper, Robert M. Beauchamp, Arturo Umeyama
Abstract. The Eastern Pacific Cloud Aerosol Precipitation Experiment (EPCAPE) was a year-round campaign conducted by the US Department of Energy at the Scripps Institution of Oceanography in La Jolla, CA, USA, with a focus on characterizing atmospheric processes at a coastal location. The ground-based prototype of a new Ka-, W-, and G-band (35.75, 94.88, and 238.8 GHz) profiling atmospheric radar, named CloudCube, which was developed at the Jet Propulsion Laboratory, took part in the experiment during 6 weeks in March and April 2023. This article describes the unique data sets that were obtained during the field campaign from a variety of marine clouds and light precipitation. These are, to the best of the authors' knowledge, the first observations of atmospheric clouds using simultaneous multifrequency measurements including 238.8 GHz. These data sets therefore provide an exceptional opportunity to study and analyze hydrometeors with diameters in the millimeter- and submillimeter size range that can be used to better understand cloud and precipitation structure, formation, and evolution. The data sets referenced in this article are intended to provide a complete, extensive, and high-quality collection of G-band data in the form of Doppler spectra and Doppler moments. In addition, Ka-band and W-band reflectivity and Ka-, W-, and G-band reflectivity ratio profiles are included for several cases of interest on 6 different days. The data sets can be found at https://doi.org/10.5281/zenodo.10076227 (Socuellamos et al., 2024).
摘要东太平洋云雾气溶胶降水实验(EPCAPE)是美国能源部在美国加利福尼亚州拉霍亚斯克里普斯海洋学研究所开展的一项全年活动,重点是描述沿海地区的大气过程特征。喷气推进实验室开发的新型 Ka 波段、W 波段和 G 波段(35.75、94.88 和 238.8 千兆赫)剖面大气雷达(名为 CloudCube)的地基原型参与了 2023 年 3 月和 4 月为期 6 周的实验。本文介绍了在实地活动期间从各种海洋云层和小降水中获得的独特数据集。据作者所知,这是首次使用包括 238.8 GHz 在内的多频同步测量对大气云层进行观测。因此,这些数据集为研究和分析直径在毫米和亚毫米范围内的水介质提供了难得的机会,可用于更好地了解云和降水的结构、形成和演变。本文引用的数据集旨在以多普勒光谱和多普勒矩的形式提供完整、广泛和高质量的 G 波段数据集。此外,还包括 6 个不同天的 Ka 波段和 W 波段反射率以及 Ka、W 和 G 波段反射率比剖面图。数据集见 https://doi.org/10.5281/zenodo.10076227(Socuellamos 等,2024 年)。
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引用次数: 0
GEST: Accurate global ocean surface current reconstruction withmulti-scale dynamics-informed neural network GEST:利用多尺度动态信息神经网络进行精确的全球洋面洋流重建
IF 11.4 1区 地球科学 Q1 Earth and Planetary Sciences Pub Date : 2024-06-10 DOI: 10.5194/essd-2024-190
Linyao Ge, Guiyu Wang, Baoxiang Huang, Chuanchuan Cao, Xiaoyan Chen, Ge Chen
Abstract. Exceptional precision and excellent resolution reconstruction of sea surface currents are beneficial for exploring complex oceanic dynamic processes. Normally, this required physical inversion models for global or regional oceans are constructed to reconstruct oceanic currents. These models are based on the analysis of sea surface geostrophic and Ekman currents derived from satellite observations of sea level and wind stress fields. Nevertheless, the presence of various typical dynamic processes in marine environments, such as mesoscale eddies and small-scale waves, continues to pose challenges in accurately reconstructing oceanic currents. Meanwhile, any product of surface current that neglects the contribution of wave motion would, at best, be incomplete. Therefore, in this paper, we introduce an accurate sea surface current product at a depth of 15 m, named GEST (Geostrophic-Ekman-Stokes-Tide). This product is produced by a multi-scale dynamics-informed neural network that learns the intricate representation of concealed characteristics in Ekman, geostrophic currents, wave-induced Stokes drift, and TPXO9 tidal currents. Its structure design is predicated upon the intricate coupling relationships between various ocean surface components and the veritable currents discerned by the deployment of drift buoys, with each ocean surface component correlating to discrete physical processes. Compared with the prevailing product, the GEST confers an elevation in precision by approximately 9.2 cm/s over the traditional multinomial fitting method, 10.4 cm/s beyond the OSCAR, and 8.81 cm/s surpassing GlobCurrent.
摘要高精度和高分辨率的海面洋流重建有利于探索复杂的海洋动力过程。通常情况下,需要构建全球或区域海洋的物理反演模型来重建洋流。这些模型基于对卫星观测海平面和风应力场得出的海面地转和 Ekman 海流的分析。然而,由于海洋环境中存在各种典型的动态过程,如中尺度漩涡和小尺度波浪,准确重建洋流仍然面临挑战。同时,任何忽略波浪运动贡献的表层洋流产品充其量都是不完整的。因此,我们在本文中介绍了一种精确的 15 米深度海面洋流产品,命名为 GEST(Geostrophic-Ekman-Stokes-Tide)。该产品由一个多尺度动态信息神经网络生成,该网络可学习埃克曼、地营洋流、波浪诱导斯托克斯漂移和 TPXO9 潮汐中错综复杂的隐蔽特征表示。其结构设计基于各种海洋表面成分与漂流浮标探测到的真实海流之间错综复杂的耦合关系,每个海洋表面成分都与离散的物理过程相关联。与现有产品相比,GEST 的精度比传统的多项式拟合方法高出约 9.2 厘米/秒,比 OSCAR 高出 10.4 厘米/秒,比 GlobCurrent 高出 8.81 厘米/秒。
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引用次数: 0
Global Methane Budget 2000–2020 2000-2020 年全球甲烷预算
IF 11.4 1区 地球科学 Q1 Earth and Planetary Sciences Pub Date : 2024-06-06 DOI: 10.5194/essd-2024-115
Marielle Saunois, Adrien Martinez, Benjamin Poulter, Zhen Zhang, Peter Raymond, Pierre Regnier, Joseph G. Canadell, Robert B. Jackson, Prabir K. Patra, Philippe Bousquet, Philippe Ciais, Edward J. Dlugokencky, Xin Lan, George H. Allen, David Bastviken, David J. Beerling, Dmitry A. Belikov, Donald R. Blake, Simona Castaldi, Monica Crippa, Bridget R. Deemer, Fraser Dennison, Giuseppe Etiope, Nicola Gedney, Lena Höglund-Isaksson, Meredith A. Holgerson, Peter O. Hopcroft, Gustaf Hugelius, Akihito Ito, Atul K. Jain, Rajesh Janardanan, Matthew S. Johnson, Thomas Kleinen, Paul Krummel, Ronny Lauerwald, Tingting Li, Xiangyu Liu, Kyle C. McDonald, Joe R. Melton, Jens Mühle, Jurek Müller, Fabiola Murguia-Flores, Yosuke Niwa, Sergio Noce, Shufen Pan, Robert J. Parker, Changhui Peng, Michel Ramonet, William J. Riley, Gerard Rocher-Ros, Judith A. Rosentreter, Motoki Sasakawa, Arjo Segers, Steven J. Smith, Emily H. Stanley, Joel Thanwerdas, Hanquin Tian, Aki Tsuruta, Francesco N. Tubiello, Thomas S. Weber, Guido van der Werf, Doug E. Worthy, Yi Xi, Yukio Yoshida, Wenxin Zhang, Bo Zheng, Qing Zhu, Qiuan Zhu, Qianlai Zhuang
Abstract. Understanding and quantifying the global methane (CH4) budget is important for assessing realistic pathways to mitigate climate change. Emissions and atmospheric concentrations of CH4 continue to increase, maintaining CH4 as the second most important human-influenced greenhouse gas in terms of climate forcing after carbon dioxide (CO2). The relative importance of CH4 compared to CO2 for temperature change is related to its shorter atmospheric lifetime, stronger radiative effect, and acceleration in atmospheric growth rate over the past decade, the causes of which are still debated. Two major challenges in reducing uncertainties in the factors explaining the well-observed atmospheric growth rate arise from diverse, geographically overlapping CH4 sources and from the uncertain magnitude and temporal change in the destruction of CH4 by short-lived and highly variable hydroxyl radicals (OH). To address these challenges, we have established a consortium of multi-disciplinary scientists under the umbrella of the Global Carbon Project to improve, synthesise and update the global CH4 budget regularly and to stimulate new research on the methane cycle. Following Saunois et al. (2016, 2020), we present here the third version of the living review paper dedicated to the decadal CH4 budget, integrating results of top-down CH4 emission estimates (based on in-situ and greenhouse gas observing satellite (GOSAT) atmospheric observations and an ensemble of atmospheric inverse-model results) and bottom-up estimates (based on process-based models for estimating land-surface emissions and atmospheric chemistry, inventories of anthropogenic emissions, and data-driven extrapolations). We present a budget for the most recent 2010–2019 calendar decade (the latest period for which full datasets are available), for the previous decade of 2000–2009 and for the year 2020. The revision of the bottom-up budget in this edition benefits from important progress in estimating inland freshwater emissions, with better accounting of emissions from lakes and ponds, reservoirs, and streams and rivers. This budget also reduces double accounting across freshwater and wetland emissions and, for the first time, includes an estimate of the potential double accounting that still exists (average of 23 Tg CH4 yr-1). Bottom-up approaches show that the combined wetland and inland freshwater emissions average 248 [159–369] Tg CH4 yr-1 for the 2010–2019 decade. Natural fluxes are perturbed by human activities through climate, eutrophication, and land use. In this budget, we also estimate, for the first time, this anthropogenic component contributing to wetland and inland freshwater emissions. Newly available gridded products also allowed us to derive an almost complete latitudinal and regional budget based on
我们确定了改进 CH4 预算的五个主要优先事项:i) 根据对不同类型排放生态系统的可靠分类,绘制全球高分辨率水饱和土壤和淹没区 CH4 排放图;ii) 进一步开发基于过程的内陆水排放模型;iii) 加强地方(如 FLUXNET-CH4 测量、城市尺度监测、具有指向能力的卫星图像)到区域尺度的 CH4 观测(地表网络和卫星全球遥感测量),以制约自下而上的模型和全球遥感测量、iii) 加强从地方(如 FLUXNET-CH4 测量、城市尺度监测、带指向功能的卫星图像)到区域尺度 (地表网络和卫星全球遥感测量)的甲烷观测,以制约自下而上的模式和大气反演;iv) 在自上而下的反演中改进传输模型和光化学汇的表示方法,以及 v) 利用同位素和/或乙烷等共排放物以及遥感探测到的人为超级排放物(主要是石油和天然气部门,但也包括煤炭、农业和垃圾填埋场)的自下而上清单中的信息,整合三维可变反演系统,以改进源划分。本文提供的数据可从 https://doi.org/10.18160/GKQ9-2RHT 下载(Martinez 等人,2024 年)。
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