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Impacts of emerging and novel plastic waste variants on marine and coastal ecosystems: Challenges and implications on the circular economy 新兴和新型塑料废物对海洋和沿海生态系统的影响:对循环经济的挑战和影响
IF 6.1 3区 工程技术 Q2 ENERGY & FUELS Pub Date : 2023-05-09 DOI: 10.1002/wene.480
P. Roy Chowdhury, Himani Medhi, K. Bhattacharyya, C. Hussain
The twenty‐first century is confronted with the consequences of enormous amounts of global emerging plastic waste resulting from an excessive use of plastic, which has been imparting several negative impacts on the environment and human health. Moreover, some novel variants have also been reported in some coastal environments, so far, as a result of mixing of plastic waste with various other matrices. As a result, the problem of various forms of plastic waste within the marine ecosystem has emerged as a major concern in recent years. The current review is focused on the detrimental implications of various emerging and novel plastic variants, with an emphasis on coastal and marine environments. This review highlights the fate and transportation patterns of plastic waste, along with the contemporary examples of its implications on marine biota. Additionally, this work also examines the impacts of marine plastic waste on the environment. The review further highlights the importance of circular economy of plastic waste for sustainability. Then in the end, the growing anxieties about the impacts of plastic waste on coastal as well as marine environment, along with the strategies for reducing its impacts on ecological sustainability are discussed.
二十一世纪面临着全球因过度使用塑料而产生的大量塑料垃圾的后果,这对环境和人类健康产生了一些负面影响。此外,到目前为止,由于塑料垃圾与各种其他基质的混合,在一些沿海环境中也报告了一些新的变体。因此,近年来,海洋生态系统中各种形式的塑料垃圾问题已成为一个主要问题。目前的审查重点是各种新兴和新型塑料变体的有害影响,重点是沿海和海洋环境。这篇综述强调了塑料垃圾的命运和运输模式,以及其对海洋生物群影响的当代例子。此外,这项工作还考察了海洋塑料垃圾对环境的影响。该审查进一步强调了塑料垃圾循环经济对可持续性的重要性。最后,讨论了人们对塑料垃圾对沿海和海洋环境影响的日益担忧,以及减少其对生态可持续性影响的策略。
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引用次数: 0
Density functional theory modeling of critical properties of perovskite oxides for water splitting applications 钙钛矿氧化物水分解关键性质的密度泛函理论建模
IF 6.1 3区 工程技术 Q2 ENERGY & FUELS Pub Date : 2023-05-08 DOI: 10.1002/wene.476
K. Ghose, Joshua J. Brown, T. Frankcombe, A. Page, A. Bayon
Water splitting (WS) driven by solar energy is considered as a promising strategy to produce renewable hydrogen from water with minimal environmental impact. Realization of large‐scale hydrogen production by this approach requires cost‐effective, efficient and stable materials to drive the WS reaction. Perovskite oxides have recently attracted widespread attention in WS applications due to their unique structural features, such as compositional and structural flexibility allowing them to achieve desired sunlight absorption capability, precise control of electrocatalytic and redox activity to drive the chemical reaction, tuneable bandgaps and band edges, and earth‐abundance. However, perovskite oxides contain a large family of metal oxides and experimental exploration of novel perovskites without a priori knowledge of their properties could be costly and time‐consuming. First‐principles approaches such as density functional theory (DFT) are a useful and cost‐effective alternative towards this end. In this review, DFT‐based calculations for accurate prediction of the critical properties of ABO3 perovskite oxides relevant to WS processes are surveyed. Structural, electronic, optical, surface, and thermal properties are grouped according to their relevance to photocatalytic (PC), electrochemical (EC), photo‐electrochemical (PEC), and solar thermal water splitting (STWS) processes. The challenges associated with the choice of exchange‐correlation (XC) functional in DFT methods for precise prediction of these properties are discussed and specific XC functionals have been recommended where experimental comparisons are possible.
太阳能驱动的水分解(WS)被认为是一种很有前途的策略,可以在对环境影响最小的情况下从水中生产可再生氢气。通过这种方法实现大规模氢气生产需要成本有效、高效和稳定的材料来驱动WS反应。钙钛矿氧化物最近在WS应用中引起了广泛关注,因为它们具有独特的结构特征,如成分和结构灵活性,使它们能够实现所需的阳光吸收能力,精确控制电催化和氧化还原活性以驱动化学反应,可调带隙和带边,以及地球丰度。然而,钙钛矿氧化物包含一大类金属氧化物,在不事先了解其性质的情况下对新型钙钛矿进行实验探索可能既昂贵又耗时。密度泛函理论(DFT)等第一性原理方法是实现这一目标的有用且成本有效的替代方法。在这篇综述中,调查了用于准确预测与WS工艺相关的ABO3钙钛矿氧化物的临界性质的基于DFT的计算。结构、电子、光学、表面和热性能根据其与光催化(PC)、电化学(EC)、光电化学(PEC)和太阳能热水分解(STWS)过程的相关性进行分组。讨论了在DFT方法中选择交换相关(XC)泛函以精确预测这些性质的挑战,并在可能进行实验比较的情况下推荐了特定的XC泛函。
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引用次数: 0
An alternative approach to capture uncertainties embedded in the estimation of social cost of carbon 捕捉碳社会成本估算中不确定性的替代方法
IF 6.1 3区 工程技术 Q2 ENERGY & FUELS Pub Date : 2023-04-18 DOI: 10.1002/wene.475
Desy Caesary, Hana Kim, M. Nam
The continuous increase in global surface temperature, which has been triggered by the increase in atmospheric CO2 concentration from anthropogenic activity, results in damage not only in the short term but also in the long term. This damage, called the social cost of carbon (SCC), has been widely estimated using integrated assessment models (IAMs). A large range of estimated SCC values have been observed because of uncertainties in IAMs' parameters. This study provides a comprehensive review of these uncertainties after dividing IAM modules into four categories: climate sensitivity, damage function, discount rate, and regional–sectoral validation. The review was conducted by comparing key ideas considered by various IAMs: socioeconomic conditions in relation to projected CO2 emissions, estimation of the atmospheric concentration of CO2, estimation of total radiative forcing, parameters of the temperature function, parameters of the damage function, and discount rate value. In addition, this study presents an alternative approach to capture the uncertainties embedded in the SCC estimation, using a machine learning approach. This enables a probabilistic evaluation of a specific level of SCC and improves our comprehension of the implication of the calculated SCC using IAMs. This alternative approach provides a basis for further study of SCC.
由人为活动导致的大气二氧化碳浓度增加引发的全球地表温度的持续升高,不仅在短期内,而且在长期内都会造成损害。这种损害被称为碳的社会成本(SCC),已经使用综合评估模型(IAM)进行了广泛的估计。由于IAM参数的不确定性,已经观察到了大范围的SCC估计值。本研究将IAM模块分为四类后,对这些不确定性进行了全面审查:气候敏感性、损害函数、贴现率和区域-部门验证。该审查是通过比较各种IAM考虑的关键思想进行的:与预计二氧化碳排放量有关的社会经济条件、二氧化碳大气浓度的估计、总辐射强迫的估计、温度函数的参数、损害函数的参数和贴现率值。此外,本研究提出了一种使用机器学习方法来捕捉SCC估计中嵌入的不确定性的替代方法。这使得能够对特定水平的SCC进行概率评估,并提高我们对使用IAM计算的SCC含义的理解。这种替代方法为SCC的进一步研究提供了基础。
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引用次数: 0
Direct gas heating in linear concentrating solar collectors for power and industrial process heat production: Applications and challenges 用于电力和工业过程热生产的线性聚光太阳能集热器的直接气体加热:应用和挑战
IF 6.1 3区 工程技术 Q2 ENERGY & FUELS Pub Date : 2023-04-10 DOI: 10.1002/wene.471
A. Lecuona-Neumann, A. Famiglietti
Parabolic trough collectors and linear Fresnel collectors are mature technologies for power production, and they are being recently applied to provide solar heat for industrial needs. Conventionally, they use a liquid as heat transfer fluid, either thermal oil or water, to carry heat from the receivers up to the point of conversion or delivery. Although liquids offer excellent thermal properties, they show technical limitations, besides environmental concerns, which have encouraged the research on alternative solutions. This work reviews the main research works on the use of gases as heat transfer fluid in linear concentrating collectors, including solar power and heat production, highlighting the potential applications and technical challenges. The review indicates: first, gases offer potential to replace liquids, and second, there is a need for more research and development to define the best technical compromises to reach practical application in every sector.
抛物线槽集热器和线性菲涅耳集热器是成熟的发电技术,它们最近被应用于为工业需要提供太阳能。传统上,它们使用液体作为传热流体,导热油或水,将热量从接收器携带到转换或输送点。尽管液体具有优异的热性能,但它们也存在技术限制,此外还有环境问题,这鼓励了对替代解决方案的研究。本文综述了在线性聚光集热器中使用气体作为传热流体的主要研究工作,包括太阳能发电和产热,重点介绍了潜在的应用和技术挑战。该报告指出:首先,气体有可能取代液体;其次,需要更多的研究和开发,以确定最佳的技术折衷方案,以便在每个领域实现实际应用。
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引用次数: 1
Machine learning for design and optimization of organic Rankine cycle plants: A review of current status and future perspectives 用于有机兰金循环工厂设计和优化的机器学习:现状和未来展望
IF 6.1 3区 工程技术 Q2 ENERGY & FUELS Pub Date : 2023-04-02 DOI: 10.1002/wene.474
J. Oyekale, B. Oreko
The organic Rankine cycle (ORC) is widely acknowledged as a sustainable power cycle. However, the traditional approach commonly adopted for its optimal design involves sequential consideration of working fluid selection, plant configuration, and component types, before the optimization of state parameters. This way, the design process fails to achieve an optimal design in most cases, since the process relies heavily on empirical judgments. To improve the design process, researchers have been exploring lately the suitability of machine learning techniques. It is however not clear yet if data‐driven designs of ORC plants are practically viable and accurate. To bridge this gap, this article reviews literature studies in the field. Overviews were first presented on the ORC technology and machine learning modeling approaches. Next, studies that applied machine‐learning methods for the design and performance prediction of ORC plants were discussed. Furthermore, studies that focused on ORC machine learning optimizations were discussed. The artificial neural network (ANN) approach was observed as the technique most frequently applied for ORC design and optimization. Additionally, researchers agree in general that machine‐learning methods can achieve accurate results, with significant reductions of computational time and cost. However, there is the risk of using inadequate data size in the machine learning design approach, or insufficient data set training time, all of which can affect accuracy. It is hoped that this effort would spur the practical implementation of machine learning techniques in the future design and optimization of ORC plants, toward the achievement of more sustainable energy technology.
有机朗肯循环(ORC)被广泛认为是一种可持续的动力循环。然而,通常用于其优化设计的传统方法包括在优化状态参数之前,依次考虑工作流体的选择、设备配置和部件类型。这样,设计过程在大多数情况下都无法实现最佳设计,因为该过程在很大程度上依赖于经验判断。为了改进设计过程,研究人员最近一直在探索机器学习技术的适用性。然而,目前尚不清楚ORC工厂的数据驱动设计是否切实可行和准确。为了弥补这一差距,本文回顾了该领域的文献研究。首先概述了ORC技术和机器学习建模方法。接下来,讨论了将机器学习方法应用于ORC工厂设计和性能预测的研究。此外,还讨论了专注于ORC机器学习优化的研究。人工神经网络(ANN)方法被认为是ORC设计和优化中最常用的技术。此外,研究人员普遍认为,机器学习方法可以获得准确的结果,显著减少计算时间和成本。然而,在机器学习设计方法中存在数据大小不足的风险,或者数据集训练时间不足,所有这些都会影响准确性。希望这一努力将推动机器学习技术在未来ORC工厂的设计和优化中的实际应用,以实现更可持续的能源技术。
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引用次数: 0
A comprehensive review on how ionic liquids enhance the pyrolysis of cellulose, lignin, and lignocellulose toward a circular economy 离子液体如何促进纤维素、木质素和木质纤维素的热解以实现循环经济的综合综述
IF 6.1 3区 工程技术 Q2 ENERGY & FUELS Pub Date : 2023-03-25 DOI: 10.1002/wene.473
Mohammad Eqbalpour, Amirhossein Andooz, E. Kowsari, S. Ramakrishna, Zahra Ansari Cheshmeh, A. Chinnappan
The sustainable use of plant biomass (PB) to produce new valuable compounds helps alleviate the world's excessive reliance on fossil fuels. Among the different processes available, pyrolysis has drawn significant attention for its efficiency in converting PB (including lignin, hemicellulose, and cellulose) into solid, liquid, and gas products by thermal degradation. Moreover, the participation of ionic liquids (ILs) in the pyrolysis process can further facilitate this process, improve the quality of pyrolysis products, and enhance the operational parameters. This review article presents an in‐depth examination of how ILs enhance the pyrolysis of lignin, cellulose, and lignocellulose toward sustainability and circular economy (CE). The structural chemistry of the components of PB, namely cellulose, lignin, and hemicellulose, is first discussed. Furthermore, the role of ILs in the pyrolysis of cellulose, lignin, and lignocellulose is thoroughly investigated. These roles include pre‐treating agent before pyrolysis, catalyst after or during pyrolysis, template during pyrolysis, and extractant after pyrolysis. In the following, the sustainability of PB pyrolysis with the participation of ILs is examined from three aspects: environmental, social, and economical. Finally, the PB pyrolysis was investigated from the CE aspect. There is no doubt that the participation of ILs in the pyrolysis process positively affects the operating conditions and product quality, so the whole process is only one step away from complete sustainability.
可持续利用植物生物质生产新的有价值的化合物有助于缓解世界对化石燃料的过度依赖。在现有的不同工艺中,热解因其通过热降解将PB(包括木质素、半纤维素和纤维素)转化为固体、液体和气体产品的效率而备受关注。此外,离子液体(ILs)参与热解过程可以进一步促进这一过程,提高热解产物的质量,并提高操作参数。这篇综述文章深入研究了离子液体如何促进木质素、纤维素和木质纤维素的热解,以实现可持续性和循环经济(CE)。首先讨论了PB中纤维素、木质素和半纤维素的结构化学。此外,还深入研究了离子液体在纤维素、木质素和木质纤维素热解中的作用。这些作用包括热解前的预处理剂、热解后或热解期间的催化剂、热解期间的模板和热解后的萃取剂。在下文中,从环境、社会和经济三个方面考察了有离子液体参与的PB热解的可持续性。最后,从CE的角度对PB的热解进行了研究。毫无疑问,离子液体参与热解过程对操作条件和产品质量产生了积极影响,因此整个过程距离完全可持续性只有一步之遥。
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引用次数: 2
Hybrid zinc‐air battery (ZAB) with transition metal‐based electrocatalysts—A step toward next‐generation electrochemical energy storage 具有过渡金属基电催化剂的混合锌-空气电池(ZAB)——迈向下一代电化学储能的一步
IF 6.1 3区 工程技术 Q2 ENERGY & FUELS Pub Date : 2023-03-15 DOI: 10.1002/wene.472
S. Tharani, D. Durgalakshmi, Aruna K. Kunhiraman, S. Balakumar, R. A. Rakkesh
Zinc air batteries (ZABs) are gaining popularity as a viable substitute for lithium‐based batteries in recent years because of their availability of raw materials, high energy density, affordability, and renewability. However, there remain challenges that have not been solved, like the lack of bifunctional catalysts that would increase the kinetics of oxygen reduction and oxygen evolution reactions (ORR and OER) in the cathodic layer of ZABs. Transition metal‐based catalyst (TMBCs) credited with high activity, stability and affordability are researched as a potential bifunctional catalyst. The review that is being presented intend to provide an overview of ZABs, specific information about TMBC types utilized in ZABs, as well as an explanation of the functions of artificial intelligence (AI) and machine learning (ML).
近年来,锌-空气电池(ZABs)作为锂基电池的可行替代品越来越受欢迎,因为它们具有原材料可用性、高能量密度、可负担性和可再生性。然而,仍然存在尚未解决的挑战,例如缺乏会增加ZABs阴极层中氧还原和析氧反应(ORR和OER)动力学的双功能催化剂。过渡金属基催化剂(TMBCs)具有高活性、稳定性和可负担性,被认为是一种潜在的双功能催化剂。正在进行的综述旨在提供ZAB的概述、ZAB中使用的TMBC类型的具体信息,以及对人工智能(AI)和机器学习(ML)功能的解释。
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引用次数: 1
Indirect weather‐based approaches for increasing power transfer capabilities of electrical transmission networks 提高电力传输网络电力传输能力的基于天气的间接方法
IF 6.1 3区 工程技术 Q2 ENERGY & FUELS Pub Date : 2023-02-24 DOI: 10.1002/wene.470
B. Keyvani, E. Whelan, Eadaoin Doddy, Damian Flynn
Dynamic line rating (DLR) systems are recognized as a cost‐effective and socially accepted asset for relieving network congestion and uprating existing transmission systems, based upon accessing additional weather‐dependent capacity of overhead lines. Although direct and indirect DLR methods are available, utilization of indirect weather‐based approaches, that is, sensors are not installed on the conductor, are of increasing interest due to fast installation times, that is, no requirement for line outages and lower capital costs, with achievable potential for wide‐area implementation. An extensive review is presented on the components and requirements of such systems, including weather stations, forecasting models, downscaling and DLR calculations, overhead line and conductor thermal models, and communication platforms. In addition, the features of practical instances of these systems are briefly reviewed. Moreover, a systematic approach is introduced for statistical evaluation of the high‐level DLR potential across an entire region, as well as an assessment of the line‐level DLR ampacities within an electrical grid, based on (weather forecasting) reanalysis data. The proposed methodology can disclose available additional capacity as part of early‐stage planning for wide‐area DLR systems. The island of Ireland and the 110 kV network of the Republic of Ireland (ROI) power system are considered as the study cases, with comparison made against seasonal static ratings and ambient temperature adjusted line rating methods.
动态线路评级(DLR)系统是公认的具有成本效益和社会认可的资产,用于缓解网络拥堵和升级现有的输电系统,基于获取额外的天气依赖性架空线路容量。虽然直接和间接DLR方法都是可用的,但由于安装时间快,不需要线路中断和较低的资本成本,因此利用间接基于天气的方法(即传感器不安装在导体上)越来越受到人们的关注,并且具有在广域实施的潜力。对这些系统的组成部分和要求进行了广泛的审查,包括气象站、预报模型、缩小和DLR计算、架空线和导体热模型以及通信平台。此外,还简要介绍了这些系统实例的特点。此外,本文还介绍了一种系统的方法,用于统计评估整个地区的高水平DLR潜力,以及基于(天气预报)再分析数据的电网内线路级DLR容量的评估。所提出的方法可以揭示可用的额外容量,作为广域DLR系统早期规划的一部分。以爱尔兰岛和爱尔兰共和国(ROI)电力系统的110 kV网络为研究案例,与季节静态额定和环境温度调节线路额定方法进行了比较。
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引用次数: 0
A roadmap for required technological advancements to further reduce onshore wind turbine noise impact on the environment 为进一步减少陆上风力涡轮机噪音对环境的影响所需要的技术进步路线图
IF 6.1 3区 工程技术 Q2 ENERGY & FUELS Pub Date : 2023-02-02 DOI: 10.1002/wene.469
F. Bertagnolio, M. Herr, Kaj Dam Madsen
The noise emission of wind turbines and farms can be an important and limiting factor for future cost reductions and growth of wind energy. Closing scientific and technological gaps on wind turbine noise is thus directly supporting the further development of renewable energy while reducing adverse reactions toward wind farms. The present article is providing guidance on the most relevant research directions from an engineering perspective, namely: simulation methods, wind tunnel testing, and wind turbine design. Each topic is addressed separately and specific scientific challenges are identified. Future research directions that may improve our physical understanding of wind turbine noise, as well as facilitate the deployment of wind energy, are outlined. It is concluded that future scientific research on the topic of wind turbine noise should be conducted in a multidisciplinary context to maximize its impact. The suggested topics shall be seen as a collection of what is seen as the most relevant topics across research and product development but shall not be seen as exclusive or interlinked with specific development plans.
风力涡轮机和风电场的噪音排放可能是未来风能成本降低和增长的一个重要和限制因素。因此,缩小风力涡轮机噪音方面的科技差距直接支持可再生能源的进一步发展,同时减少对风电场的不利反应。本文从工程角度对最相关的研究方向提供指导,即:模拟方法、风洞试验和风力涡轮机设计。每个主题都单独讨论,并确定了具体的科学挑战。概述了未来的研究方向,这些方向可能会提高我们对风力涡轮机噪音的物理理解,并促进风能的部署。结论是,未来应在多学科背景下对风力涡轮机噪声进行科学研究,以最大限度地发挥其影响。建议的主题应视为研究和产品开发中最相关主题的集合,但不应视为与具体开发计划排他性或相互关联。
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引用次数: 1
Syngas production from thermochemical conversion of mixed food waste: A review 混合食物垃圾热化学转化制合成气的研究进展
IF 6.1 3区 工程技术 Q2 ENERGY & FUELS Pub Date : 2023-01-04 DOI: 10.1002/wene.468
S. Yadav, Priyanka Katiyar, M. Mesfer, M. Danish
Lately, the generation of leftover food or cooked food waste has turned out to be a critical issue and its disposal in an environmental friendly way has been a challenge. This food waste is being sent for incineration and landfilling which results in a significant contribution to environmental pollution. Therefore, alternative methods for processing food waste in an environmentally benign way have been explored by many researchers. Thermochemical methods are one of those methods and are found to be promising for not only handling the food waste in an ecological way but also producing renewable energy efficiently in the form of bio‐oil and syngas along with a solid byproduct, that is, biochar. However, the generation of syngas is favored by only two thermochemical processes, fast pyrolysis, and gasification. Some derived processes such as co‐pyrolysis, and co‐gasification can also generate syngas. All these processes for syngas generation differ from each other in terms of process conditions (temperature, reaction agents, and residence time) and syngas quality generated (amount of syngas produced, syngas composition, and heating capacity). Additionally, supercritical water gasification is the latest process developed for processing food waste to generate syngas with much higher hydrogen fraction; however, it produces syngas with less yield and involves high operational costs.
最近,剩饭剩菜或熟食垃圾的产生已经成为一个关键问题,以一种环保的方式处理剩饭剩菜已经成为一个挑战。这些食物垃圾被送去焚烧和填埋,这对环境污染造成了重大影响。因此,许多研究人员已经探索了以环境友好的方式处理食物垃圾的替代方法。热化学方法就是其中的一种方法,人们发现它不仅有希望以生态的方式处理食物垃圾,而且还能以生物油和合成气的形式有效地生产可再生能源,同时还能产生固体副产品,即生物炭。然而,合成气的产生只有两种热化学过程,快速热解和气化。一些衍生的过程,如共热解和共气化也可以产生合成气。所有这些合成气生成过程在工艺条件(温度、反应剂和停留时间)和生成的合成气质量(产生的合成气数量、合成气成分和加热能力)方面都有所不同。此外,超临界水气化是最新开发的处理食物垃圾的工艺,可以产生氢含量更高的合成气;然而,它生产的合成气产量较低,运营成本高。
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引用次数: 0
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