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Investigating the suitability of pristine and defective C3N monolayer as supercapacitor electrodes: DFT calculations 研究原始和缺陷 C3N 单层作为超级电容器电极的适用性:DFT 计算
IF 1.6 3区 物理与天体物理 Q3 PHYSICS, FLUIDS & PLASMAS Pub Date : 2024-09-02 DOI: 10.1016/j.hedp.2024.101154
Maher Ali Rusho , Ihsan A. Alduhan , Adil Ismael Mohammed , Hayder Hamid Abbas Al-Anbari , Aseel Salah Mansoor , Usama Kadem Radi , Amir H. Idean , Ahmad J. Obaidullah , Hala Bahair , Anupam Yadav

The possibility of utilizing defected C3N monolayers as the electrodes of supercapacitors (SCs) was investigated in the current study by performing DFT computations. A single-vacancy C3N monolayer (SC3NML), a double-vacancy C3N monolayer (DC3NM) and a pure C3N monolayer (PC3NML) were investigated. The charge plots, quantum capacitance (QC) and the density of state of SC3NML, DC3NM and PC3NML were also studied. Based on the results, the QC of SC3NML and DC3NM at voltages between -0.80 and 0.80 V was more compared to the QC of PC3NML. It was possible to use SC3NML as a negative electrode and DC3NM as a positive electrode, both of which were p-type semi-conductors. The stored charge in the SC3NML and DC3NM was higher compared to the stored charge in PC3NML at voltages 0 to 0.8 V. The charge stored in DC3NM was higher than the stored charge in SC3NML and PC3NML. Finally, DC3NML layer can be regarded as an encouraging electrode for application in SCs.

本研究通过 DFT 计算探讨了利用有缺陷的 C3N 单层作为超级电容器 (SC) 电极的可能性。研究了单空位 C3N 单层(SC3NML)、双空位 C3N 单层(DC3NM)和纯 C3N 单层(PC3NML)。还研究了 SC3NML、DC3NM 和 PC3NML 的电荷图、量子电容(QC)和状态密度。结果表明,与 PC3NML 的量子电容相比,SC3NML 和 DC3NM 在-0.80 至 0.80 V 电压下的量子电容更大。可以使用 SC3NML 作为负极,DC3NM 作为正极,它们都是 p 型半导体。在电压为 0 至 0.8 V 时,SC3NML 和 DC3NM 中存储的电荷高于 PC3NML 中存储的电荷。最后,DC3NML 层可被视为一种令人鼓舞的电池电极。
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引用次数: 0
Propagation of circularly polarized electromagnetic wave in magnetized spin plasma 磁化自旋等离子体中圆极化电磁波的传播
IF 1.6 3区 物理与天体物理 Q3 PHYSICS, FLUIDS & PLASMAS Pub Date : 2024-09-02 DOI: 10.1016/j.hedp.2024.101155
Qiang-Lin Hu , Yan-Chao She , Wen Hu , Jin-Peng Xiao , Zheng-Guo Xiao

The spin effects on the propagation characteristic of circularly polarized electromagnetic (EM) wave in high density strongly magnetized plasma are discussed based on the the classical hydrodynamical model of relativistic spin plasma. The dielectric coefficients for right-hand circularly polarized (RCP) and left-hand circularly polarized (LCP) waves are obtained. Results show that the spin effects can affect the propagation characteristic of circularly polarized EM wave dramatically. Provided the spin effect is strong enough, LCP waves can also propagate in the magnetized over-dense plasma, while RCP waves may not. The strength of spin effects can be enhanced by increasing the plasma density or/and EM wave intensity.

基于相对论自旋等离子体的经典流体力学模型,讨论了自旋对圆极化电磁波在高密度强磁化等离子体中传播特性的影响。得到了右旋圆极化(RCP)和左旋圆极化(LCP)波的介电系数。结果表明,自旋效应会显著影响圆极化电磁波的传播特性。只要自旋效应足够强,LCP 波也能在磁化过密等离子体中传播,而 RCP 波则不能。提高等离子体密度或/和电磁波强度可以增强自旋效应的强度。
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引用次数: 0
Technique for an improved and time-resolved carbon areal density measurement with a single channel diagnostic for inertial confinement fusion 利用单通道诊断技术改进惯性约束聚变的时间分辨碳等值密度测量技术
IF 1.6 3区 物理与天体物理 Q3 PHYSICS, FLUIDS & PLASMAS Pub Date : 2024-09-02 DOI: 10.1016/j.hedp.2024.101145
Hermann Geppert-Kleinrath , Robert Dwyer , Kevin Meaney , Cathleen Fry , Yongho Kim

Measurement of the areal density and velocity of the carbon ablator shell during peak burn in inertial confinement fusion give powerful information on the state of the ablator and where in the trajectory of implosion it reaches peak burn. Detailed comparison of the absolute densities and velocities of the carbon in implosions has been prevented by the limited ability to resolve shot-to-shot variation within a shot series or within a campaign. A new approach using a single, ultra fast (10 ps) gamma ray channel can massively reduce uncertainties and will provide insights on improvements to target and drive variables. Small improvements in these experimental design parameters may result in much greater yields.

在惯性约束聚变中,测量燃烧峰值期间碳烧蚀器外壳的平均密度和速度,可以获得有关烧蚀器状态以及在内爆运动轨迹中何处达到燃烧峰值的有力信息。由于在一系列射击或一次活动中分辨射击间变化的能力有限,因此无法对内爆中碳的绝对密度和速度进行详细比较。使用单个超快(∼10 ps)伽马射线通道的新方法可以大量减少不确定性,并为改进目标和驱动变量提供启示。这些实验设计参数的微小改进都可能带来更高的产量。
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引用次数: 0
2D kinetic-ion simulations of inverted corona fusion targets 倒日冕聚变目标的二维动能离子模拟
IF 1.6 3区 物理与天体物理 Q3 PHYSICS, FLUIDS & PLASMAS Pub Date : 2024-08-28 DOI: 10.1016/j.hedp.2024.101146
William Riedel , Nathan Meezan , Drew Higginson , Matthias Hohenberger , Mark Cappelli

Laser-driven “inverted corona” fusion targets have attracted interest as a low-convergence neutron source and platform for studying kinetic physics. The scheme consists of a hollow or gas-filled spherical shell made of deuterated plastic. The shell has one or more laser entrance holes (LEH), resembling a spherical hohlraum. The laser passes through the LEH’s and illuminates the interior surface of the shell, ablating a plasma that travels inward towards the target center. Long ion mean free paths in the converging plasma can lead to significant interpenetration, atomic mix, and other kinetic effects. In this work we report on numerical simulations of inverted corona targets using the kinetic-ion, fluid–electron hybrid particle-in-cell (PIC) approach in 2D RZ geometry. 2D simulations suggest that shape effects do not have a significant impact on plasma evolution and observed yield trends are primarily the result of 1D kinetic mix mechanisms. Simulations are also compared against available experimental data recorded at the OMEGA laser facility. In particular, synthetic x-ray emission images show good qualitative agreement with experimental results, albeit with an apparent timing discrepancy for the two-sided vacuum target. More generally, we demonstrate the potential of hybrid-PIC simulations for full-system modeling and experimental design, including collisional absorption of laser energy, plasma evolution, mix, and fusion burn.

激光驱动的 "倒日冕 "聚变目标作为一种低聚合中子源和研究动力学物理的平台,引起了人们的兴趣。该方案包括一个由氚化塑料制成的空心或充满气体的球形外壳。外壳上有一个或多个激光入口孔(LEH),类似于球形霍尔姆。激光穿过激光入口孔,照射到外壳内表面,烧蚀等离子体,等离子体向目标中心内移动。在会聚等离子体中,离子的平均自由路径较长,会导致明显的相互穿透、原子混合和其他动力学效应。在这项工作中,我们报告了在二维 RZ 几何结构中使用动力学-离子、流体-电子混合粒子入胞(PIC)方法对倒电晕目标进行的数值模拟。二维模拟表明,形状效应不会对等离子体的演化产生重大影响,观察到的产量趋势主要是一维动力学混合机制的结果。模拟结果还与 OMEGA 激光设备记录的现有实验数据进行了比较。特别是,合成 X 射线发射图像与实验结果显示出良好的定性一致,尽管双面真空靶存在明显的时间差异。更广泛地说,我们展示了混合 PIC 模拟在全系统建模和实验设计方面的潜力,包括激光能量的碰撞吸收、等离子体演变、混合和聚变燃烧。
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引用次数: 0
Electron impact ionization in dense plasmas 致密等离子体中的电子碰撞电离
IF 1.6 3区 物理与天体物理 Q3 PHYSICS, FLUIDS & PLASMAS Pub Date : 2024-08-28 DOI: 10.1016/j.hedp.2024.101153
Walter R. Johnson , Joseph Nilsen , K.T. Cheng

The distorted-wave with exchange (DWE) method is employed to evaluate electron impact ionization cross sections in dense electron–ion plasmas. Bound and continuum electron wave functions are obtained from a non-relativistic average-atom code. Plots of DWE cross sections are presented for 1s electrons in Li and Be plasmas and 2p electrons in Na and Mg plasmas. For each of these elements, cross sections are evaluated at metallic density in a range of temperatures from 10 to 100 eV and at their respective melting points. Resonances in the cross sections appear near the incident energy threshold at high temperatures. The origin of these resonances is discussed. In general, the distorted wave (DW) method without exchange is found to be a good approximation to the DWE method for electron impact ionization calculations. In the resonance region, however, exchange effects are found to be very important and cannot be neglected.

采用带交换的扭曲波(DWE)方法来评估致密电子-离子等离子体中的电子碰撞电离截面。束缚和连续电子波函数是从非相对论平均原子代码中获得的。图中给出了 Li 和 Be 等离子体中 1s 电子以及 Na 和 Mg 等离子体中 2p 电子的 DWE 截面图。在 10 到 100 eV 的温度范围内,对每种元素的横截面都是在金属密度和各自的熔点下进行评估的。在高温入射能量阈值附近出现了截面共振。本文讨论了这些共振的起源。一般来说,在电子撞击电离计算中,无交换的扭曲波(DW)方法是 DWE 方法的良好近似方法。然而,在共振区,交换效应非常重要,不可忽视。
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引用次数: 0
Stable creation of a single plasma channel and collimated fast electrons using large-scale PIC simulations with new dynamic load-balancing technique 利用新型动态负载平衡技术进行大规模 PIC 模拟,稳定创建单个等离子体通道和准直快速电子
IF 1.6 3区 物理与天体物理 Q3 PHYSICS, FLUIDS & PLASMAS Pub Date : 2024-08-26 DOI: 10.1016/j.hedp.2024.101147
Hideaki Habara , Yoshinori Ueyama , Yutaka Nakamura , Hitoshi Sakagami

We developed a PIC code using new load balancing technique, in which the lower load processes help the higher load processes. A test calculation indicates more than 10 times faster than that without load balancing. Large scale 3-d calculations indicate the formation of central current whose density is close to critical density, supported by the magnetic field inside the channel.

我们利用新的负载平衡技术开发了 PIC 代码,其中低负载进程帮助高负载进程。测试计算表明,速度比没有负载平衡的情况下快 10 倍以上。大规模三维计算表明,在通道内磁场的支持下,形成了密度接近临界密度的中心电流。
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引用次数: 0
Mykonos: A pulsed power driver for science and innovation 米克诺斯岛促进科学和创新的脉冲功率驱动器
IF 1.6 3区 物理与天体物理 Q3 PHYSICS, FLUIDS & PLASMAS Pub Date : 2024-08-24 DOI: 10.1016/j.hedp.2024.101144
Jens Schwarz , Brian Hutsel , Thomas Awe , Bruno Bauer , Jacob Banasek , Eric Breden , Joe Chen , Michael Cuneo , Katherine Chandler , Karen DeZetter , Mark Gilmore , Matthew Gomez , Hannah Hasson , Maren Hatch , Nathan Hines , Trevor Hutchinson , Deanna Jaramillo , Christine Kalogeras Loney , Ian Kern , Derek Lamppa , Kevin Yates

Sandia National Laboratories has been operating the Mykonos linear transformer driver (LTD) in a five-cavity configuration since 2014. The machine operates at 1 MA output current, 500 kV output voltage, with a 10–90% current rise time of 85 ns, which enables small scale physics and engineering pulsed power experiments. Mykonos provides hands-on pulsed power experimental training for students and staff alongside senior Sandia scientists in an environment that is more accessible than the Z Facility. Over the years, we have fielded and accumulated a wide variety of optical, x-ray and electrical diagnostics and we are preparing to open this facility to outside users. Here, we are presenting the pulsed power and diagnostic capability of Mykonos as well as some recent experiments that have been performed on the facility. The goal of this publication is to attract researchers across the pulsed power and high energy density (HED) community to collaborate with Sandia on exciting, innovative science and to train the next generation of researchers for the National Nuclear Security Agency (NNSA) and the nation. As such, we have established a Mykonos Academic Access Program (MAAP) as part of ZNetUS to enable academic utilization of the Mykonos Pulsed Power Facility.

自 2014 年以来,桑迪亚国家实验室一直在运行五腔配置的 Mykonos 线性变压器驱动器 (LTD)。该设备的输出电流为 1 MA,输出电压为 500 kV,10-90% 的电流上升时间为 85 ns,可进行小规模物理和工程脉冲功率实验。与 Z 设施相比,Mykonos 为学生和员工提供了更方便的脉冲功率实验培训环境,让他们与桑迪亚的资深科学家一起进行实验。多年来,我们已经实地使用并积累了各种光学、X 射线和电气诊断设备,我们正准备向外部用户开放该设施。在此,我们将介绍米克诺斯设施的脉冲功率和诊断能力,以及最近在该设施上进行的一些实验。该出版物的目的是吸引脉冲功率和高能量密度 (HED) 领域的研究人员与桑迪亚合作,共同开展激动人心的创新科学研究,并为美国国家核安全局(NNSA)和国家培养下一代研究人员。因此,我们制定了米克诺斯学术访问计划 (MAAP),作为 ZNetUS 的一部分,使学术界能够利用米克诺斯脉冲功率设施。
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引用次数: 0
A hybrid simulation integrating molecular dynamics and particle-in-cell methods for improved laser-target interaction 集成分子动力学和粒子入胞法的混合模拟,用于改进激光与目标的相互作用
IF 1.6 3区 物理与天体物理 Q3 PHYSICS, FLUIDS & PLASMAS Pub Date : 2024-08-24 DOI: 10.1016/j.hedp.2024.101148
Harihara Sudhan Kumar , Masayuki Takahashi , Yasuhiro Kuramitsu , Takumi Minami , Hiromitsu Kiriyama , Yuji Fukuda , Naofumi Ohnishi

Ultra-thin targets (less than 10 nm), such as graphene, can be irradiated with relativistic intensity lasers to generate energetic ions. However, the laser prepulse can prematurely destroy these targets and significantly influence the final ion energies. Due to the limitations of the conventional hydrodynamic model, simulating the interaction between ultra-thin targets and a prepulse is infeasible. To overcome this issue, we propose a hybrid simulation technique in this study. This technique involves simulating the target-prepulse interaction using molecular dynamics (MD) simulation, which is then combined with the particle-in-cell simulation for the target-main pulse interaction, in order to accurately model the entire laser-target interaction dynamics. A realistic, experimentally measured laser intensity profile for the prepulse is used for the MD simulation, and the particle energies from this hybrid simulation are found to be in good agreement with the experiment.

石墨烯等超薄目标(小于 10 纳米)可通过相对论强度激光照射产生高能离子。然而,激光预脉冲会过早地破坏这些目标,并严重影响最终离子能量。由于传统流体力学模型的局限性,模拟超薄靶和预脉冲之间的相互作用是不可行的。为了克服这一问题,我们在本研究中提出了一种混合模拟技术。该技术包括使用分子动力学(MD)模拟来模拟目标与预脉冲的相互作用,然后再结合粒子入胞模拟来模拟目标与主脉冲的相互作用,从而精确地模拟整个激光与目标相互作用的动力学过程。在 MD 模拟中使用了实验测得的真实的预脉冲激光强度曲线,结果发现这种混合模拟得出的粒子能量与实验结果非常吻合。
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引用次数: 0
Extension of the SpK atomic physics code to generate global equation of state data 扩展 SpK 原子物理代码以生成全局状态方程数据
IF 1.6 3区 物理与天体物理 Q3 PHYSICS, FLUIDS & PLASMAS Pub Date : 2024-08-21 DOI: 10.1016/j.hedp.2024.101136
Adam R. Fraser , A.J. Crilly , N.-P.L. Niasse , D.A. Chapman , J.D. Pecover , S.J. O’Neill , J.P. Chittenden

Global microphysics models are required for the modelling of high-energy-density physics (HEDP) experiments, the improvement of which are critical to the path to inertial fusion energy. This work presents further developments to the atomic and microphysics code, SpK, part of the numerical modelling suite of Imperial College London and First Light Fusion. We extend the capabilities of SpK to allow the calculation of the equation of state (EoS). The detailed configuration accounting calculations are interpolated into finite-temperature Thomas–Fermi calculations at high coupling to form the electronic component of the model. The Cowan model provides the ionic contribution, modified to approximate the physics of diatomic molecular dissociation. By utilising bonding corrections and performing a Maxwell construction, SpK captures the EoS from states ranging from the zero-pressure solid, through the liquid–vapour coexistence region and into plasma states. This global approach offers the benefit of capturing electronic shell structure over large regions of parameter space, building highly-resolved tables in minutes on a simple desktop. We present shock Hugoniot and off-Hugoniot calculations for a number of materials, comparing SpK to other models and experimental data. We also apply EoS and opacity data generated by SpK in integrated simulations of indirectly-driven capsule implosions, highlighting physical sensitivities to the choice of EoS models.

高能量密度物理(HEDP)实验的建模需要全局微观物理模型,这些模型的改进对通向惯性聚变能的道路至关重要。这项工作展示了对原子和微观物理代码 SpK 的进一步开发,SpK 是伦敦帝国学院和 First Light Fusion 数值建模套件的一部分。我们扩展了 SpK 的功能,允许计算状态方程(EoS)。详细的构型核算计算被插值到高耦合的有限温度托马斯-费米计算中,形成模型的电子部分。考恩模型提供了离子部分,并对其进行了修改,以近似二原子分子解离的物理过程。通过利用成键修正和执行麦克斯韦构造,SpK 捕获了从零压固态到液气共存区再到等离子体态的 EoS。这种全局方法的优点是可以捕捉参数空间大范围内的电子壳结构,在简单的桌面上几分钟内就能建立高分辨率的表格。我们介绍了一些材料的休克休轰特和非休克休轰特计算,并将 SpK 与其他模型和实验数据进行了比较。我们还将 SpK 生成的 EoS 和不透明度数据应用于间接驱动的胶囊内爆的综合模拟中,强调了 EoS 模型的选择对物理的敏感性。
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引用次数: 0
Observation of ion species energy dependence on charge-to-mass ratio in laser-driven magnetic reconnection experiment 在激光驱动的磁重联实验中观测离子物种能量与电荷质量比的关系
IF 1.6 3区 物理与天体物理 Q3 PHYSICS, FLUIDS & PLASMAS Pub Date : 2024-08-19 DOI: 10.1016/j.hedp.2024.101137
K.F.F. Law , J. Dun , Y. Abe , A. Morace , Y. Arikawa , Ph. Korneev , J.J. Santos , S. Fujioka

Magnetic reconnection, a critical process in plasma physics, involves the reconnection of magnetic field lines, leading to the release of energy and acceleration of particles. This phenomenon is pivotal across various fields such as astrophysics, fusion energy research, and space weather forecasting. In this study, we conducted an experiment on magnetic reconnection using a laser-driven micro-coil to generate bi-directional currents. Analysis of the ion energy distribution from the reconnection outflow revealed that the maximum energy for each ion species correlates with a common gyroradius within the reconnection field, with spectral shapes across different ion species — excluding protons — showing uniformity after normalization by the square of their charge-to-mass ratio. These findings align with the hypothesis of large-scale magnetic field turbulence at the acceleration site, indicative of a strongly driven magnetic reconnection system.

磁再连接是等离子物理学中的一个关键过程,涉及磁场线的再连接,导致能量释放和粒子加速。这一现象在天体物理学、核聚变能源研究和空间天气预报等多个领域都举足轻重。在这项研究中,我们利用激光驱动的微型线圈产生双向电流,进行了磁重联实验。对来自再连接外流的离子能量分布的分析表明,每种离子的最大能量与再连接场内的共同回旋半径相关,不同离子种类(不包括质子)的光谱形状在按其电荷质量比的平方归一化后显示出一致性。这些发现与加速点的大尺度磁场湍流假说相吻合,表明存在一个强驱动的磁再连接系统。
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引用次数: 0
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High Energy Density Physics
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