This paper investigates the microstructural mechanism that triggers diffuse instability in two-dimensional granular materials, utilizing directional statistics and Discrete Element Method simulations. Hill’s second-order work criterion is employed to identify the onset of diffuse instability at macroscale. A second-order work expression, formulated in terms of micro-variables, is derived based on a Stress-rate Force Fabric function and a Strain-rate Displacement Fabric function proposed for two-dimensional granular systems. The second-order work is theoretically originated from three independent aspects: contact density variation due to contact loss/gain and volume change, microstructure anisotropy evolution caused by rearrangement of the contact network and the contact force networks, and alteration of directional average normal contact force. The microstructure anisotropy and the directional average of the normal contact force are connected with the fabric anisotropy in the strong and weak sub-networks. Two dual mechanisms underlying diffuse instability are identified, including: (a) degradation of the microstructure characterized by a diminished peak in microstructure anisotropy combined with a volumetric dilating regime; (b) degradation of directional average normal contact force or buckling of the weak sub-network, which ultimately leads to the collapse of the entire microstructure. Moreover, these processes are associated with the contact density and coordination number approaching their critical thresholds.
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