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Anomalous Purcell decay of strongly driven inhomogeneous emitters coupled to a cavity 与空腔耦合的强驱动非均质发射器的反常珀塞尔衰变
Pub Date : 2024-04-10 DOI: 10.1364/opticaq.520843
Michael T. Solomon, Martin Koppenhöfer, Mikhail Mamaev, Cheng Ji, Gregory Grant, Ignas Masiulionis, Sean E. Sullivan, F. Joseph Heremans, Supratik Guha, David D. Awschalom, Aashish A. Clerk, Alan M. Dibos
We perform resonant fluorescence lifetime measurements on a nanocavity-coupled erbium ensemble as a function of cavity-laser detuning and pump power. Our measurements reveal an anomalous three-fold suppression of the ensemble Purcell factor at zero cavity detuning and high pump fluence. We capture qualitative aspects of this decay rate suppression using a Tavis–Cummings model of non-interacting spins coupled to a common cavity.
我们对纳米腔耦合铒集合进行了共振荧光寿命测量,并将其作为腔激光失谐和泵浦功率的函数。我们的测量结果表明,在腔体失谐为零和高泵浦通量的情况下,集合珀塞尔因子会受到三倍的异常抑制。我们利用与共腔耦合的非相互作用自旋的 Tavis-Cummings 模型来捕捉这种衰减率抑制的定性方面。
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引用次数: 0
Gain-compensated metal cavity modes and a million-fold improvement of Purcell factors 增益补偿金属腔模式和普赛尔因子的百万倍改进
Pub Date : 2024-03-26 DOI: 10.1364/opticaq.504834
Becca VanDrunen, Juanjuan Ren, Sebastian Franke, and Stephen Hughes
Using a rigorous mode theory for gain-compensated plasmonic dimers, we demonstrate how quality factors and Purcell factors can be dramatically increased, improving the quality factors from 10 to over 26,000 and the peak Purcell factors from approximately 3000 to over 10 billion. Full three-dimensional calculations are presented for gold dimers in a finite-size gain medium, which allows one to easily surpass fundamental Purcell factor limits of lossy media. Within a regime of linear system response, we show how the Purcell factors are modified by the contributions from the projected local density of states as well as a non-local gain. Further, we show that the effective mode volume and radiative beta factors remain relatively constant, despite the significant enhancement of the Purcell factors.
利用增益补偿质子二聚体的严格模式理论,我们展示了如何显著提高品质因数和普赛尔因子,将品质因数从 10 提高到 26,000 以上,将普赛尔因子峰值从大约 3000 提高到 100 亿以上。我们介绍了有限尺寸增益介质中金二聚体的全三维计算,这使得我们可以轻松超越有损介质的基本普赛尔因子限制。在线性系统响应机制中,我们展示了珀塞尔因子是如何被投影局部态密度和非局部增益的贡献所改变的。此外,我们还展示了尽管普赛尔因子显著增强,但有效模式体积和辐射贝塔因子仍保持相对恒定。
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引用次数: 0
Traceable localization enables accurate integration of quantum emitters and photonic structures with high yield 可追踪定位技术实现了量子发射器和光子结构的高产能精确集成
Pub Date : 2024-03-18 DOI: 10.1364/opticaq.502464
Craig R. Copeland, Adam L. Pintar, Ronald G. Dixson, Ashish Chanana, Kartik Srinivasan, Daron A. Westly, B. Robert Ilic, Marcelo I. Davanco, and Samuel M. Stavis
In a popular integration process for quantum information technologies, localization microscopy of quantum emitters guides lithographic placement of photonic structures. However, a complex coupling of microscopy and lithography errors degrades registration accuracy, severely limiting device performance and process yield. We introduce a methodology to solve this widespread but poorly understood problem. A new foundation of traceable localization enables rapid characterization of lithographic standards and comprehensive calibration of cryogenic microscopes, revealing and correcting latent systematic effects. Of particular concern, we discover that scale factor deviation and complex optical distortion couple to dominate registration errors. These novel results parameterize a process model for integrating quantum dots and bullseye resonators, predicting higher yield by orders of magnitude, depending on the Purcell factor threshold as a quantum performance metric. Our foundational methodology is a key enabler of the lab-to-fab transition of quantum information technologies and has broader implications to cryogenic and correlative microscopy.
在量子信息技术流行的集成工艺中,量子发射器的定位显微镜可指导光子结构的光刻放置。然而,显微镜和光刻误差的复杂耦合降低了配准精度,严重限制了器件性能和工艺产量。我们介绍了一种方法来解决这一普遍存在但却鲜为人知的问题。可追踪定位的新基础可实现光刻标准的快速表征和低温显微镜的全面校准,揭示并纠正潜在的系统效应。特别值得关注的是,我们发现比例因子偏差和复杂光学失真共同主导了套准误差。这些新成果为量子点和牛眼谐振器的集成工艺模型提供了参数,根据作为量子性能指标的珀塞尔因子阈值,预测产量将提高几个数量级。我们的基础方法是量子信息技术从实验室向实验室过渡的关键推动因素,对低温显微镜和相关显微镜具有更广泛的影响。
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引用次数: 0
High-rate multiplexed entanglement source based on time-bin qubits for advanced quantum networks 基于时宾量子比特的高速率多路复用纠缠源,用于先进量子网络
Pub Date : 2024-03-12 DOI: 10.1364/opticaq.509335
Andrew Mueller, Samantha I. Davis, Boris Korzh, Raju Valivarthi, Andrew D. Beyer, Rahaf Youssef, Neil Sinclair, Cristián Peña, Matthew D. Shaw, and Maria Spiropulu
Entanglement distribution based on time-bin qubits is an attractive option for emerging quantum networks. We demonstrate a 4.09-GHz repetition rate source of photon pairs entangled across early and late time bins separated by 80 ps. Simultaneous high rates and high visibilities are achieved through frequency multiplexing the spontaneous parametric down conversion output into eight time-bin entangled channel pairs. We demonstrate entanglement visibilities as high as 99.4%, total entanglement rates up to 3.55×106 coincidences/s, and predict a straightforward path towards achieving up to an order of magnitude improvement in rates without compromising visibility. Finally, we resolve the density matrices of the entangled states for each multiplexed channel and express distillable entanglement rates in ebit/s, thereby quantifying the trade-off between visibility and coincidence rates that contributes to useful entanglement distribution. This source is a fundamental building block for high-rate entanglement-based quantum key distribution systems or advanced quantum networks.
对于新兴的量子网络而言,基于时间带量子比特的纠缠分发是一种极具吸引力的选择。我们展示了一种 4.09 千兆赫重复频率的光子对纠缠源,其早期和晚期时间分段相隔 80 ps。通过将自发参量下变频输出复用为八个时间带纠缠通道对,实现了同时的高速率和高可见度。我们展示了高达 99.4% 的纠缠可见度,总纠缠率高达 3.55×106 个重合/秒,并预测了在不影响可见度的情况下实现高达数量级速率改进的直接途径。最后,我们解析了每个多路复用通道的纠缠态密度矩阵,并以 ebit/s 为单位表达了可提炼的纠缠率,从而量化了能见度和重合率之间的权衡,这有助于有用的纠缠分布。该源是基于高速率纠缠的量子密钥分发系统或先进量子网络的基本构件。
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引用次数: 0
Harnessing quantum emitter rings for efficient energy transport and trapping 利用量子发射环实现高效能量传输和捕获
Pub Date : 2024-03-07 DOI: 10.1364/opticaq.510021
Raphael Holzinger, Jonah S. Peter, Stefan Ostermann, Helmut Ritsch, and Susanne Yelin
Efficient transport and harvesting of excitation energy under low light conditions is an important process in nature and quantum technologies alike. Here we formulate a quantum optics perspective to excitation energy transport in configurations of two-level quantum emitters with a particular emphasis on efficiency and robustness against disorder. We study a periodic geometry of emitter rings with subwavelength spacing, where collective electronic states emerge due to near-field dipole–dipole interactions. The system gives rise to collective subradiant states that are particularly suited to excitation transport and are protected from energy disorder and radiative decoherence. Comparing ring geometries with other configurations shows that the former are more efficient in absorbing, transporting, and trapping incident light. Because our findings are agnostic as to the specific choice of quantum emitters, they indicate general design principles for quantum technologies with superior photon transport properties and may elucidate potential mechanisms resulting in the highly efficient energy transport efficiencies in natural light-harvesting systems.
在弱光条件下高效传输和收集激发能量是自然界和量子技术的一个重要过程。在这里,我们从量子光学的角度阐述了两级量子发射器配置中的激发能量传输,并特别强调了效率和对无序的鲁棒性。我们研究了一种具有亚波长间距的发射环周期性几何结构,在这种结构中,由于近场偶极子-偶极子相互作用,出现了集体电子态。该系统产生的集体亚辐射态特别适合于激发传输,并能防止能量无序和辐射退相干。将环形几何结构与其他配置进行比较后发现,前者能更有效地吸收、传输和捕获入射光。由于我们的研究结果与量子发射器的具体选择无关,因此它们指出了具有卓越光子传输特性的量子技术的一般设计原则,并可能阐明导致自然光收集系统高效能量传输效率的潜在机制。
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引用次数: 0
Single-photon sub-Rayleigh precision measurements of a pair of incoherent sources of unequal intensity 对一对强度不等的非相干光源进行单光子亚瑞利精密测量
Pub Date : 2024-02-22 DOI: 10.1364/opticaq.505457
Luigi Santamaria, Fabrizio Sgobba, and Cosmo Lupo
Interferometric methods have been recently investigated to achieve sub-Rayleigh imaging and precision measurements of faint incoherent sources up to the ultimate quantum limit. Here we consider single-photon imaging of two point-like emitters of unequal intensity. This is motivated by the fact that pairs of natural emitters typically have unequal brightness, for example, binary star systems and exoplanets. We address the problem of estimating the transverse separation d or the relative intensity epsilon. Our theoretical analysis shows that the associated statistical errors are qualitatively different from the case of equal intensity. We employ multi-plane light conversion technology to implement Hermite–Gaussian (HG) spatial-mode demultiplexing (SPADE), and demonstrate sub-Rayleigh measurement of two emitters with a Gaussian point-spread function. The experimental errors are comparable with the theoretical bounds. The latter are benchmarked against direct imaging, yielding an epsilon ^{-1/2} improvement in the signal-to-noise ratio, which may be significant when the primary source is much brighter than the secondary one, for example, as for imaging of exoplanets.
最近研究了干涉测量方法,以实现亚雷利光成像和对微弱非相干光源的精确测量,直至量子极限。在这里,我们考虑对两个不等强度的点状发射体进行单光子成像。这是因为成对的自然发射体通常具有不等的亮度,例如双星系统和系外行星。我们要解决的问题是估计横向间隔 d 或相对强度 epsilonepsilon。我们的理论分析表明,相关的统计误差与等强度的情况有本质的区别。我们采用多平面光转换技术来实现赫米特-高斯(HG)空间模式解复用(SPADE),并演示了两个具有高斯点扩散函数的发射器的亚雷利测量。实验误差与理论限值相当。后者以直接成像为基准,在信噪比方面得到了 epsilon ^{-1/2}epsilon ^{-1/2} 的改善,当主源比副源亮得多时,例如系外行星成像时,信噪比可能会显著提高。
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引用次数: 0
Practical tests for sub-Rayleigh source discriminations with imperfect demultiplexers 使用不完善的解复用器进行亚瑞利光源判别的实际测试
Pub Date : 2024-01-30 DOI: 10.1364/opticaq.502459
Konrad Schlichtholz, Tomasz Linowski, Mattia Walschaers, Nicolas Treps, Łukasz Rudnicki, and Giacomo Sorelli
Quantum-optimal discrimination between one and two closely separated light sources can be theoretically achieved by ideal spatial-mode demultiplexing, simply monitoring whether a photon is detected in a single antisymmetric mode. However, we show that for any imperfections of the demultiplexer, no matter how small, this simple statistical test becomes practically useless. While we identify a class of separation-independent tests with vanishing error probabilities in the limit of large numbers of detected photons, they are generally unreliable beyond that very limit. As a practical alternative, we propose a simple semi-separation-independent test, which provides a method for designing reliable experiments, through arbitrary control over the maximal probability of error.
理论上,通过理想的空间模式解复用,可以在一个和两个紧密分离的光源之间实现量子最佳分辨,只需监测光子是否在单个非对称模式中被检测到即可。然而,我们的研究表明,无论解复用器的缺陷有多小,这种简单的统计测试实际上都是无用的。虽然我们发现了一类与分离无关的检验方法,在检测到大量光子的情况下,它们的误差概率会消失,但超过这个极限后,它们通常就不可靠了。作为一种实用的替代方法,我们提出了一种简单的半分离无关检验方法,通过对最大误差概率的任意控制,为设计可靠的实验提供了一种方法。
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引用次数: 0
Storage of telecom wavelength heralded single photons in a fiber cavity quantum memory 在光纤腔量子存储器中存储电信波长预示单光子
Pub Date : 2024-01-09 DOI: 10.1364/opticaq.506601
Duncan England, R. Tannous, Kent Fisher, Daniel Poitras, Cyril Hnatovsky, Stephen Mihailov, P. Bustard, Benjamin Sussman
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引用次数: 0
High-Dimensional Path-Entangled Qudits on a Silicon Photonic Chip 硅光子芯片上的高维路径纠缠 Qudits
Pub Date : 2023-12-21 DOI: 10.1364/opticaq.500322
Evan Manfreda, J. D. Elliott, Matthew van Niekerk, Daniel Proctor, Mario Ciminelli, Thomas W. Palone, Christopher Tison, Michael Fanto, Stefan F Preble, Gregory Howland
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引用次数: 0
Transmission of light–matter entanglement over a metropolitan network 通过城域网传输光物质纠缠
Pub Date : 2023-12-18 DOI: 10.1364/opticaq.501048
Jelena V. Rakonjac, Samuele Grandi, Sören Wengerowsky, Dario Lago-Rivera, Félicien Appas, and Hugues de Riedmatten
We report on the transmission of telecom photons entangled with a multimode solid-state quantum memory over a deployed optical fiber in a metropolitan area. Photon pairs were generated through spontaneous parametric downconversion, with one photon stored in a rare-earth-based quantum memory, and the other, at telecommunication wavelengths, traveling through increasing distances of optical fiber, first in the laboratory and then outside in a deployed fiber loop. We measured highly non-classical correlations between the stored and the telecom photons for storage times up to 25 µs and for a fiber separation up to 50 km. We also report light–matter entanglement with a two-qubit fidelity up to 88%, which remains constant within error bars for all fiber lengths, showing that the telecom qubit does not suffer decoherence during the transmission. Finally, we moved the detection stage of the telecom photons to a different location placed 16 km away, and confirmed the non-classical correlations between the two photons. Our system was adapted to provide the transmission of precise detection times and synchronization signals over long quantum communication channels, providing the first steps for a future quantum network involving quantum memories and non-classical states.
我们报告了与多模固态量子存储器纠缠在一起的电信光子在大都会地区部署的光纤上的传输情况。光子对是通过自发参量降频转换产生的,其中一个光子存储在一个基于稀土的量子存储器中,另一个光子以电信波长通过光纤的传输距离不断增加,首先是在实验室中,然后是在室外部署的光纤环路中。我们测量了存储光子和电信光子之间的高度非经典相关性,存储时间长达 25 微秒,光纤间隔长达 50 千米。我们还报告了双量子比特保真度高达 88% 的光物质纠缠,在所有光纤长度范围内,该保真度在误差范围内保持不变,这表明电信量子比特在传输过程中不会发生退相干。最后,我们将电信光子的探测阶段移到了 16 千米之外的另一个地方,并证实了两个光子之间的非经典相关性。我们的系统适用于在长量子通信信道上传输精确的检测时间和同步信号,为未来涉及量子存储器和非经典状态的量子网络迈出了第一步。
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引用次数: 0
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Optica Quantum
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