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High-precision fluidic Kirigami morphing surface for ultrasonic holographic lensing and haptic interfacing 用于超声全息透镜和触觉接口的高精度流体基里伽米变形表面
IF 4.5 3区 工程技术 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-12-01 Epub Date: 2025-11-17 DOI: 10.1016/j.eml.2025.102424
Ardalan Kahak , Moustafa Sayed Ahmed , Nahid Kalantaryardebily , Hrishikesh Kulkarni , Netta Gurari , Shima Shahab , Suyi Li
Morphing surfaces provide a versatile tool to advance the functionalities of high-performance aircraft, soft robots, biomedical devices, and human–machine interfaces. However, achieving precise shape transformation and mechanical property control remains challenging due to nonlinearity, design constraints, and the difficulty of coordinating multiple constituent materials across a continuous surface. To this end, this study unveils that Kirigami art can inspire novel solutions. More specifically, the geometric principles of Kirigami can be exploited to design and fabricate fluidic morphing surfaces capable of highly accurate shape morphing and output force control, all via a single pressure input. This study presents a systematic approach to designing Kirigami for tuning the local deformation and force output through extensive nonlinear modeling and experiment validation on two archetypal patterns: concentric square and circular cuts. The potentials of this approach are demonstrated via two multiphysics case studies: (1) an acoustic holography lens for ultrasonic wave steering, achieving highly accurate deformation control under a single global pressure input, and (2) a haptic device with a small volume, constant contact area, and high-resolution output force. The fluidic Kirigami concept allows for simple yet effective adaptation to different shape and stiffness requirements, paving the way for a new family of scalable and programmable morphing surfaces.
变形表面为高性能飞机、软体机器人、生物医学设备和人机界面提供了一种多功能工具。然而,由于非线性、设计限制以及在连续表面上协调多个组成材料的困难,实现精确的形状转换和机械性能控制仍然具有挑战性。为此,本研究揭示了Kirigami艺术可以激发新的解决方案。更具体地说,Kirigami的几何原理可以用于设计和制造流体变形表面,这些表面能够通过单一压力输入实现高精度的形状变形和输出力控制。本研究提出了一种系统的方法来设计Kirigami,通过广泛的非线性建模和实验验证两种原型模式:同心正方形和圆形切割,以调整局部变形和力输出。通过两个多物理场案例研究证明了这种方法的潜力:(1)用于超声波转向的声全息透镜,在单一全局压力输入下实现高精度的变形控制,以及(2)具有小体积,恒定接触面积和高分辨率输出力的触觉设备。流体Kirigami概念允许简单而有效地适应不同的形状和刚度要求,为一系列新的可扩展和可编程变形表面铺平了道路。
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引用次数: 0
Exploring conformational landscapes of two-dimensional macromolecules via well-tempered metadynamics 通过调质元动力学探索二维大分子的构象景观
IF 4.5 3区 工程技术 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-12-01 Epub Date: 2025-11-15 DOI: 10.1016/j.eml.2025.102421
Yanyan Zhao , Ke Zhou , Yan Chen , Yilun Liu
Exploring conformational landscape of two-dimensional (2D) macromolecules poses a profound challenge due to their intrinsically complex free energy surfaces. Conventional computational approaches based on equilibrium molecular dynamics (MD) suffer from limited ergodic exploration, failing to adequately explore energy landscapes and transition pathways between metastable conformations. In this study, we employ well-tempered Metadynamics simulations with carefully designed collective variables to comprehensively map conformational space of 2D macromolecules. Our systematic exploration reveals three distinct metastable states, i.e., flat, fold and scroll conformations. Through detailed free energy analysis, we elucidate the delicate interplay between bending rigidity and interlayer adhesion that govern free energy surfaces of these conformations. Furthermore, we propose a temperature-modulated strategy to regulate conformational transitions among the three states. By decomposing the total free energy into entropic and enthalpic contributions, we quantitatively characterize the temperature-dependent thermodynamic driving forces underlying conformational transformations. This research establishes a robust computational framework for quantifying free energy and entropy associated with metastable conformations in 2D macromolecule systems. Our findings advance fundamental understanding of conformational transitions, regulation processes, and self-assembly behaviors in 2D macromolecular systems.
由于二维(2D)大分子的自由能表面本质上是复杂的,因此探索其构象景观带来了深刻的挑战。基于平衡分子动力学(MD)的传统计算方法的遍历探索有限,无法充分探索亚稳构象之间的能量景观和转变途径。在这项研究中,我们采用了精心设计的集体变量的良好调质元动力学模拟来全面绘制二维大分子的构象空间。我们的系统探索揭示了三种不同的亚稳态,即平面、折叠和涡旋构象。通过详细的自由能分析,我们阐明了支配这些构象的自由能表面的弯曲刚度和层间附着力之间微妙的相互作用。此外,我们提出了一种温度调制策略来调节三种状态之间的构象转变。通过将总自由能分解为熵和焓贡献,我们定量地描述了构象转化背后的温度依赖的热力学驱动力。本研究建立了一个强大的计算框架,用于量化二维大分子体系中与亚稳构象相关的自由能和熵。我们的发现促进了对二维大分子系统的构象转变、调节过程和自组装行为的基本理解。
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引用次数: 0
Viscoelasticity and crack growth in tanglemers 缠结物的粘弹性和裂纹扩展
IF 4.5 3区 工程技术 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-12-01 Epub Date: 2025-11-11 DOI: 10.1016/j.eml.2025.102418
Yu Zhou , Xianyang Bao , Zhigang Suo
A tanglemer is a polymer network in which chains are long, and entanglements greatly outnumber crosslinks. In a tanglemer, each chain is divided by crosslinks into many strands, and each strand is divided by entanglements into many segments. In synthesizing tanglemers, the crosslink density is readily varied, but the entanglement density is set by the chemistry of the polymer. Here we investigate how crosslink density affects the mechanical behavior of tanglemers. We find that viscoelasticity is unaffected by crosslink density when tanglemers are subject to stretches small enough without breaking strands. We then study crack growth in tanglemers under a static load. A load exists, called the slow-crack threshold, below which the crack does not grow. The threshold is high in a tanglemer of low crosslink density. Fast crack growth, however, is insensitive to crosslink density. We discuss how molecular mechanisms affect mechanical behavior.
缠结物是一种聚合物网络,其中的链很长,缠结远远超过交联。在缠结器中,每条链通过交联被分成许多股,每条股又通过缠结被分成许多片段。在合成缠结剂时,交联密度是容易变化的,但缠结密度是由聚合物的化学性质决定的。在这里,我们研究了交联密度如何影响缠结物的力学行为。我们发现,当缠结剂受到足够小的拉伸而不断裂链时,粘弹性不受交联密度影响。然后研究了静载荷作用下缠结材料的裂纹扩展。存在一个荷载,称为慢裂阈值,低于此荷载,裂纹不会扩展。在交联密度低的缠结物中,阈值较高。然而,快速裂纹扩展对交联密度不敏感。我们讨论分子机制如何影响力学行为。
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引用次数: 0
When and where do large cracks grow? Griffith energy competition constrained by material strength 大裂缝何时何地出现?格里菲斯能源竞争受材料强度制约
IF 4.5 3区 工程技术 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-12-01 Epub Date: 2025-11-01 DOI: 10.1016/j.eml.2025.102417
Oscar Lopez-Pamies, Farhad Kamarei
An abundance of comparisons with experimental evidence has long settled that the Griffith energy competition along a known crack path — commonly expressed as a criticality condition on the energy release rate — describes when a large crack grows in a nominally elastic brittle material that is subjected to quasi-static loading. However, the answer to the question of where — that is, in which direction — a large crack grows remains unresolved. A slew of criteria have been proposed over the decades, but comparisons with experiments have indicated that none of such criteria apply in general.
Directly guided by the mathematical structure of the regularized phase-field theory of fracture initiated by Kumar, Francfort, and Lopez-Pamies (J. Mech. Phys. Solids 112 (2018), 523–551), and motivated by the wide range of experiments that this theory has been validated against, this Letter introduces a new criterion to describe when and where large cracks grow in elastic brittle materials under quasi-static loading conditions. In a nutshell: the growth of a large crack takes place within and only within regions where the strength surface of the material has been exceeded, this in a manner such that the sum of the potential (that is, the elastic energy minus the work of the external loads) and surface energies are minimized. Importantly, this strength-constrained Griffith-energy-competition criterion is general in the sense that it applies to materials with any elasticity (linear or nonlinear) and any material symmetry (isotropic or anisotropic). In this Letter, for simplicity of presentation, attention is restricted to the most basic of settings, that of isotropic linear elastic brittle materials. Following its raison d’etre by means of a simple example and then general introduction, the proposed criterion is confronted with a set of classical experiments on glass.
大量与实验证据的比较早已确定了沿已知裂纹路径的格里菲斯能量竞争-通常表示为能量释放率的临界条件-描述了当名义上的弹性脆性材料受到准静态载荷时出现大裂纹时的情况。然而,一个大裂缝在哪里——也就是说,在哪个方向——生长的问题的答案仍然没有得到解决。几十年来,人们提出了一系列的标准,但与实验的比较表明,这些标准都不适用。在Kumar, Francfort, and Lopez-Pamies (J. Mech.)提出的裂缝正则相场理论的数学结构的直接指导下。理论物理。固体112(2018),523-551),并受到该理论已被验证的广泛实验的启发,这封信引入了一个新的标准来描述在准静态加载条件下弹性脆性材料中的大裂纹何时何地产生。简而言之:大裂纹的增长发生在且仅发生在材料强度表面已被超过的区域内,这种方式使得势能(即弹性能减去外部负载的功)和表面能的总和最小。重要的是,这种强度约束的格里菲斯-能量竞争准则在某种意义上是通用的,它适用于具有任何弹性(线性或非线性)和任何材料对称性(各向同性或各向异性)的材料。在这封信中,为了表述简单,注意力被限制在最基本的设置,即各向同性线弹性脆性材料。通过一个简单的例子和一般的介绍,给出了该准则的存在理由,并与一系列经典的玻璃实验进行了对比。
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引用次数: 0
Front cover CO1 前盖CO1
IF 4.5 3区 工程技术 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-11-01 Epub Date: 2025-10-29 DOI: 10.1016/S2352-4316(25)00127-0
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引用次数: 0
On failure mechanisms and load-parallel cracking in confined elastomeric layers 承压弹性体层破坏机制及荷载平行开裂研究
IF 4.5 3区 工程技术 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-11-01 Epub Date: 2025-09-20 DOI: 10.1016/j.eml.2025.102406
Aarosh Dahal, Aditya Kumar
Thin layers of elastomers bonded to two rigid plates demonstrate unusual failure response. Historically, it has been believed that strongly-bonded layers fail by two distinct mechanisms: (i) internal/external penny-shaped crack nucleation and propagation, and (ii) cavitation, that is, cavity growth leading to fibrillation and then failure. However, recent work has demonstrated that cavitation itself is predominantly a fracture process. While the equations describing cavitation from a macroscopic or top-down view are now known and validated with experiments, several aspects of the cavitation crack growth need to be better understood. Notably, cavitation often involves through-thickness crack growth parallel to the loading direction, raising questions about when it initiates instead of the more typical penny-shaped cracks perpendicular to the load. Understanding and controlling the two vertical and horizontal crack growth is key to developing tougher soft films and adhesives. The purpose of this Letter is to provide an explanation for the load-parallel crack growth through a comprehensive numerical analysis and highlight the role of various material and geometrical parameters.
粘接在两个刚性板上的薄层弹性体表现出不同寻常的失效响应。从历史上看,人们一直认为强粘结层的失效有两种不同的机制:(i)内部/外部便士形裂纹的形核和扩展,以及(ii)空化,即空腔的生长导致纤颤然后失效。然而,最近的研究表明,空化本身主要是一个破裂过程。虽然从宏观或自上而下的角度描述空化的方程现在已知并通过实验验证,但空化裂纹扩展的几个方面需要更好地理解。值得注意的是,空化通常涉及平行于加载方向的贯穿厚度裂纹扩展,这引起了关于何时开始的问题,而不是更典型的垂直于加载的便士形裂纹。了解和控制两种垂直和水平裂纹的扩展是开发更坚韧的软膜和胶粘剂的关键。这封信的目的是通过全面的数值分析来解释荷载平行裂纹扩展,并突出各种材料和几何参数的作用。
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引用次数: 0
Mechanics of bonded sensor layers in soft tubes: Suppressing instability and failure for sensing reliability 软管中键合传感器层的力学:抑制不稳定性和失效对传感可靠性的影响
IF 4.5 3区 工程技术 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-11-01 Epub Date: 2025-09-12 DOI: 10.1016/j.eml.2025.102405
Yi Jin , Christian A. Zorman , Changyong Chase Cao
Integrating sensors onto thin-walled tubular structures is of paramount importance for the advancement of smart infrastructures and facilities, enabling real-time detection of mechanical states and environmental conditions. This study systematically investigates the mechanics of bonded sensor layers in suppressing bending-induced ovalization, buckling, and failure in soft, thin-walled tubes, with the goal of enhancing sensing reliability. While significant progress has been made in understanding instability phenomena in tubular structures under mechanical loading, a critical gap remains in characterizing how bonded sensor layers influence deformation and failure mechanisms. To address this, a comprehensive parametric analysis—supported by finite element simulations and experimental validation—was conducted to evaluate the effects of four key parameters: length ratio, thickness ratio, wrapped angle, and relative stiffness. The results reveal that optimized configurations—specifically, length ratios exceeding 0.7, thickness ratios above 1.6, moderate wrapped angles (approximately 2π/3–4π/3), and relative stiffness greater than 0.03—can suppress ovalization to below 25 % in sensor-covered regions, redistribute deformation to uncovered segments, and trigger complex buckling behaviors involving multiple kinks and secondary instabilities. These thresholds mitigate localized strain concentrations, reduce the risk of sensor layer wrinkling or delamination, and preserve measurement fidelity under operational loading. The findings extend classical instability theories to hyperelastic, multilayered systems and provide practical design guidelines for sensor-integrated tubular structures. Applications include smart pipelines and conduits for structural health monitoring and environmental sensing in next-generation infrastructure systems.
将传感器集成到薄壁管状结构上对于智能基础设施和设施的发展至关重要,可以实时检测机械状态和环境条件。本研究系统地研究了在软薄壁管中粘结传感器层抑制弯曲引起的椭圆化、屈曲和失效的力学,目的是提高传感器的可靠性。虽然在理解管状结构在机械载荷下的不稳定现象方面取得了重大进展,但在表征粘结传感器层如何影响变形和破坏机制方面仍然存在关键差距。为了解决这个问题,在有限元模拟和实验验证的支持下,进行了全面的参数分析,以评估四个关键参数的影响:长度比、厚度比、包裹角和相对刚度。结果表明,优化后的结构——长度比大于0.7,厚度比大于1.6,包裹角适中(约2π/3 - 4π/3),相对刚度大于0.03——可以抑制传感器覆盖区域的椭圆化至25 %以下,将变形重新分配到未覆盖的部分,并触发包括多重扭结和二次失稳在内的复杂屈曲行为。这些阈值减轻了局部应变浓度,降低了传感器层起皱或分层的风险,并保持了工作负载下测量的保真度。这些发现将经典的不稳定性理论扩展到超弹性、多层系统,并为传感器集成管状结构提供了实用的设计指南。应用包括下一代基础设施系统中用于结构健康监测和环境传感的智能管道和导管。
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引用次数: 0
Precipitate response in GRCop-42 metallic microparticles under extreme impact conditions GRCop-42金属微粒在极端冲击条件下的沉淀响应
IF 4.5 3区 工程技术 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-11-01 Epub Date: 2025-09-29 DOI: 10.1016/j.eml.2025.102410
Jianxiong Li , Yuan Yao , Mostafa Hassani
GRCop-42 is a Cu-based alloy strengthened primarily through precipitation hardening by a single Cr2Nb phase. While its deformation mechanisms under quasi-static conditions have been extensively studied, the behavior of these precipitates under extreme strain rates remains poorly understood. In this study, we investigate the high-rate response of GRCop-42 powder using laser-induced microparticle impact testing (LIPIT), where individual alloy particles are impacted onto a pure Cu substrate at velocities ranging from 100 to 600 m/s. We observe a transition from rebound to impact-induced bonding at ∼490 ± 11 m/s. Cross-sectional microstructural analysis of bonded particles reveals that, although high strain rate impact does not lead to significant precipitate fracture or coarsening, the precipitates undergo shape changes. At higher velocities, the Cr2Nb precipitates exhibit increased aspect ratios, particularly near particle edges. This oblate deformation at the precipitate scale is attributed to localized temperature rise from adiabatic heating, driven by extreme plastic deformation. The effect is more pronounced at higher velocities and is spatially concentrated near the periphery of the particle–substrate interface.
GRCop-42是一种cu基合金,主要通过单个Cr2Nb相的沉淀硬化来强化。虽然其在准静态条件下的变形机制已经被广泛研究,但这些析出物在极端应变速率下的行为仍然知之甚少。在这项研究中,我们使用激光诱导微粒冲击测试(LIPIT)研究了GRCop-42粉末的高速率响应,其中单个合金颗粒以100至600 m/s的速度撞击纯Cu衬底。我们观察到在~ 490 ± 11 m/s的速度下从反弹到冲击诱导键的转变。结合颗粒的断面显微组织分析表明,虽然高应变速率冲击不会导致明显的析出相断裂或粗化,但析出相发生了形状变化。在较高的速度下,Cr2Nb析出物表现出增大的长径比,特别是在颗粒边缘附近。这种在沉淀尺度上的扁形变形归因于极端塑性变形驱动的绝热加热引起的局部温升。这种效应在较高的速度下更为明显,并且在空间上集中在颗粒-衬底界面的外围附近。
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引用次数: 0
Tracing back transient information from near-stationary random data 从近平稳随机数据追溯瞬态信息
IF 4.5 3区 工程技术 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-11-01 Epub Date: 2025-09-23 DOI: 10.1016/j.eml.2025.102408
Xi Chen , Xiaoling Jin , Yong Wang , Zhilong Huang
Tracing back the past and predicting the future are of equal importance, while compared to the prediction, the backtracking is far from receiving the attention it deserves. With the explosive advances of the diffusion models, backtracking has undergone a complete renaissance, especially for stochastic systems. This work addresses this issue, tracing back transient information from near-stationary random data. Different from the diffusion models, we aim for statistical information but not sample information, and we only need near-stationary sample segments for identification, but not a large number of full-time samples for learning. The core idea of this data-driven method is: embedding Fokker-Planck equation (as a priori physical knowledge), which portrays the evolution of probability density of state, and then identifying and solving it to trace back the transient probability density. The efficacy of this method is demonstrated by three typical examples, namely, a one-dimensional linear system, a two-dimensional linear system, and the van der Pol system.
回顾过去和预测未来同样重要,但与预测相比,回溯远远没有得到应有的重视。随着扩散模型的爆炸式发展,回溯已经经历了一个完整的复兴,特别是对于随机系统。这项工作解决了这个问题,从接近平稳的随机数据中追溯瞬态信息。与扩散模型不同的是,我们的目标是统计信息而不是样本信息,我们只需要近平稳的样本段进行识别,而不需要大量的全职样本进行学习。这种数据驱动方法的核心思想是:嵌入描述状态概率密度演变的Fokker-Planck方程(作为先验的物理知识),然后对其进行识别和求解,追溯瞬时概率密度。通过一维线性系统、二维线性系统和van der Pol系统三个典型实例证明了该方法的有效性。
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引用次数: 0
Influence of additive–polymer interactions on the mechanical behaviors of cross-linked polymers 添加剂-聚合物相互作用对交联聚合物力学行为的影响
IF 4.5 3区 工程技术 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2025-11-01 Epub Date: 2025-09-02 DOI: 10.1016/j.eml.2025.102403
Wenjian Nie , Lan Xu , Wenjie Xia
Attaining an in-depth understanding of the underlying factors dictating mechanical and macroscopic properties is crucial for establishing structure–property relationships in cross-linked thermosetting polymers. The introduction of additives into these polymers can lead to significant alterations in topology, dynamic behavior, and mechanical properties. In this study, we employ a coarse-grained (CG) polymer model to systematically explore the influences of additive-polymer intermolecular interaction strength εap, additive mass fraction m, and cross-link density c on the temperature-dependent mechanical behaviors of a cross-linked glass-forming thermoset. Our results demonstrate that the mechanical characteristics, particularly the tensile and shear moduli, are predominantly affected by εap and m, with a clear temperature dependence across the glassy regime. The modulus outcomes reveal contrasting trends between the neutral interaction system εap=1 and the strong interaction system εap>1. Intriguingly, varying εap yields distinct scaling relationships between modulus and reduced temperature T/Tg, indicating a shift from the behavior typically observed in cross-linked thermosets without additives. Moreover, we identify a correlation between the moduli and the Debye–Waller parameter u2, providing insight into the local stiffness at the molecular level. Our results highlight the critical role of additives and their intermolecular interactions with polymers in governing the mechanical responses of cross-linked network, offering insights for molecular design of thin films, coatings, and nanocomposite systems.
深入了解决定机械和宏观性能的潜在因素对于建立交联热固性聚合物的结构-性能关系至关重要。在这些聚合物中加入添加剂会导致拓扑结构、动态行为和机械性能的显著改变。在本研究中,我们采用粗粒(CG)聚合物模型系统地探讨了添加剂-聚合物分子间相互作用强度εap、添加剂质量分数m和交联密度c对交联玻璃成型热固性材料的温度依赖力学行为的影响。我们的研究结果表明,力学特性,特别是拉伸和剪切模量,主要受εap和m的影响,在整个玻璃态中具有明显的温度依赖性。模量结果揭示了中性相互作用体系εap=1与强相互作用体系εap>;1之间的变化趋势。有趣的是,不同的εap在模量和还原温度T/Tg之间产生了不同的标度关系,这表明在没有添加剂的交联热固性材料中通常观察到的行为发生了转变。此外,我们确定了模量与Debye-Waller参数< u2 >之间的相关性,从而在分子水平上深入了解局部刚度。我们的研究结果强调了添加剂及其与聚合物的分子间相互作用在控制交联网络力学响应中的关键作用,为薄膜、涂层和纳米复合系统的分子设计提供了见解。
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引用次数: 0
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Extreme Mechanics Letters
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