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2019 Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)最新文献

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Modifying the Optical Phonon Response of Nanocrystals inside Terahertz Plasmonic Nanocavities 修改太赫兹等离子体纳米腔内纳米晶体的光学声子响应
Xin Jin, A. Cerea, G. Messina, A. Rovere, R. Piccoli, F. De Donato, Francisco Palazón, A. Perucchi, P. Di Pietro, R. Morandotti, S. Lupi, F. De Angelis, M. Prato, A. Toma, L. Razzari
Phonons are quantized lattice vibrations that represent a major energy dissipation channel in solid-state systems [1], both at the macro- and at the nano-scale. Although the phonon response of a specific nanomaterial is usually considered as its intrinsic fingerprint, here we show how it can be altered by exploiting the unique properties of terahertz (THz) plasmonic nanocavities [2]. Specifically, we obtained such nanocavities from the end-to-end coupling (30-nm gap size) of few-μm-long plasmonic gold nanoantennas. We fabricated a series of plasmonic arrays featuring different nanoantenna lengths, spanning from 4.75 μm to 6.75 μm, thus tuning their resonances between approximately 7 and 9 THz. We tested our approach on cadmium sulphide (CdS) nanocrystals (NCs), spin-coated over the array surfaces (Fig. 1a), since these NCs feature a dipole-active (Fröhlich) phonon mode at 7.85 THz. We performed THz transmission measurements using a Fourier-transform THz microscope coupled to synchrotron light (ELETTRA, Trieste), showing the splitting of the nanoantenna resonance into two new vibro-polariton bands, as shown in Fig. 1b. This anti-crossing behaviour represents a distinctive signature of the strong coupling between the plasmon and phonon modes, the splitting (Rabi) at the crossing point being directly related to the coupling strength. More intriguingly, we also observed the phonon resonance modification without any THz illumination, just exploiting the vacuum electric field of the nanocavities [3] (estimated to be as high as 4.6× 105 V/m). To this end, we performed a series of micro-Raman measurements on individual nanocavity areas, finding evidence of the two new hybrid states (P− and P+ in Fig. 1c) even in THz "dark" conditions. The evidence of phonon mode splitting both in THz and Raman characterizations confirms the possibility of altering the intrinsic phonon response of a nanomaterial using properly tailored plasmonic resonators, which could open new avenues for the manipulation of energy dissipation in nanodevices. Novel cavity geometries that promise to further boost the strong vibrational coupling in these systems will be presented on site.
声子是一种量子化的晶格振动,在宏观和纳米尺度上都是固态系统中主要的能量耗散通道[1]。虽然特定纳米材料的声子响应通常被认为是其固有的指纹,但在这里,我们展示了如何通过利用太赫兹(THz)等离子体纳米腔的独特特性来改变它[2]。具体来说,我们通过几μm长的等离子体金纳米天线的端到端耦合(间隙尺寸为30 nm)获得了这种纳米空腔。我们制作了一系列具有不同纳米天线长度(从4.75 μm到6.75 μm)的等离子体阵列,从而在大约7到9太赫兹之间调谐它们的共振。我们在硫化镉(CdS)纳米晶体(nc)上测试了我们的方法,这些纳米晶体在阵列表面上进行了自旋涂层(图1a),因为这些nc具有7.85太赫兹的偶极子活性(Fröhlich)声子模式。我们使用傅立叶变换太赫兹显微镜耦合同步加速器(ELETTRA, Trieste)进行太赫兹透射测量,显示纳米天线共振分裂成两个新的振动极化子带,如图1b所示。这种反交叉行为代表了等离子体和声子模式之间强耦合的独特特征,交叉点的分裂(Rabi)与耦合强度直接相关。更有趣的是,我们还观察到在没有任何太赫兹照明的情况下,仅利用纳米腔的真空电场(估计高达4.6× 105 V/m)进行声子共振修饰[3]。为此,我们对单个纳米腔区域进行了一系列微拉曼测量,发现即使在太赫兹“黑暗”条件下也存在两种新的杂化态(图1c中的P−和P+)的证据。在太赫兹和拉曼表征中声子模式分裂的证据证实了使用适当定制的等离子体谐振器改变纳米材料的固有声子响应的可能性,这可能为操纵纳米器件中的能量耗散开辟新的途径。新的空腔几何形状有望进一步增强这些系统中的强振动耦合,将在现场展示。
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引用次数: 1
Active Control of Femtosecond Soliton Molecules 飞秒孤子分子的主动控制
F. Kurtz, C. Ropers, G. Herink
Mode-locked lasers are a paramount example of dissipative nonlinear systems that support bound-states of multiple solitons, often referred as "soliton molecules" [1,2,3]. Previously hidden, internal dynamics can now be accessed by employing the time-stretch dispersive Fourier transform (TS-DFT) and spectral interferometry — enabling the tracking of pulse separations and relative phases in real-time [4,5]. Oscillatory internal motions, akin to molecular vibrations, have previously been tracked — prompting the question whether such internal oscillations can be externally excited and ultimately be controlled.
锁模激光器是耗散非线性系统的一个重要例子,它支持多孤子的束缚态,通常被称为“孤子分子”[1,2,3]。以前隐藏的内部动态现在可以通过使用时间拉伸色散傅立叶变换(TS-DFT)和光谱干涉术来访问-能够实时跟踪脉冲分离和相对相位[4,5]。振荡的内部运动,类似于分子振动,之前已经被跟踪了,这引发了一个问题,即这种内部振荡是否可以被外部激发并最终被控制。
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引用次数: 0
Comparative Study of Harmonic Generation in Air and Argon in Light Filaments Driven by Circularly Polarized Mid-IR Pulses 圆偏振中红外脉冲驱动灯丝中空气和氩气谐波产生的比较研究
V. Shumakova, C. Gollner, A. Voronin, A. Mitrofanov, D. Sidorov-Biryukov, A. Zheltikov, D. Kartashov, A. Baltuska, A. Pugžlys
A generation of optical harmonics by circularly polarized light, which is in general forbidden in an isotropic medium, was recently observed in molecular gases where molecules were aligned and oriented by another linearly polarized laser pulse [1] or by pulses with twisted polarization [2]. In order to generate nth-harmonic with circularly polarized light, a molecule has to "absorb" n photons, having the same handedness, and to emit a single nth harmonic photon while fulfilling the energy and the momentum conservation laws, meaning a necessity to excite the molecule to appropriate rotational state. One can do this by means of intrapulse rotational Raman scattering, which prepares the molecule in the excited state through a subsequent absorption of (n-1) same-handed photons [1]. All previously reported experimental studies on circular harmonic generation in molecular gases were performed with visible/near-IR drivers, in either gas jets or in standing cells and with pre-alignment of molecules by an additional laser pulses. Here we report on the studies of self-action of elliptically polarized mid-IR pulses on the generation of low-order harmonics in filaments ignited in air and in argon, representing a molecular and an atomic gas respectively. The harmonics were driven by 20-mJ, sub-100 fs mid-IR pulses, centred at 3.9 pm wavelength. In the experiments filamentation was assisted by focusing light with a spherical mirror of ROC=-2500 mm into an open-end tube, through which Ar gas was flown at slight overpressure. Polarization of the pulses was controlled by a broadband quarter wave plate (QWP). Spectra of 5th and 7th harmonics were recorded after the filaments with a grating spectrometer (HR4000, OceanOptics). Polarization state of the generated harmonics was analysed with a Glan-Taylor polarizer.
圆偏振光产生光谐波,这在各向同性介质中通常是禁止的,最近在分子气体中被观察到,其中分子被另一个线偏振激光脉冲[1]或扭曲偏振脉冲[2]排列和定向。为了用圆偏振光产生n次谐波,分子必须“吸收”n个具有相同手性的光子,并在满足能量和动量守恒定律的同时发射单个n次谐波光子,这意味着必须将分子激发到适当的旋转状态。我们可以通过脉冲内旋转拉曼散射来做到这一点,它通过随后吸收(n-1)同手光子来使分子处于激发态[1]。所有先前报道的关于分子气体中圆谐波产生的实验研究都是在可见/近红外驱动下进行的,无论是在气体射流中还是在站立的细胞中,并通过额外的激光脉冲对分子进行预校准。本文报道了椭圆偏振中红外脉冲对在空气和氩气中点燃的细丝产生低次谐波的自作用,分别代表分子气体和原子气体。谐波由20兆焦耳、低于100 fs的中红外脉冲驱动,以3.9 pm波长为中心。在实验中,用ROC=-2500 mm的球面反射镜将光聚焦到一个开口管中,氩气在轻微的超压下流过该管,以辅助灯丝的形成。脉冲的偏振由宽带四分之一波片(QWP)控制。用光栅光谱仪(HR4000, OceanOptics)记录了灯丝的5次和7次谐波光谱。用Glan-Taylor偏振器分析了产生的谐波的偏振态。
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引用次数: 0
Ultimate Quantum Noise Limit of Frequency Comb Measurements 频率梳测量的量子噪声极限
Ruoyu Liao, Youjian Song, G. Steinmeyer
Frequency comb measurements have enormously progressed in the last decade, with 10−18 precisions coming into reach [1]. Similar to Moore's law, the precision in frequency metrology measurements has improved by about 3 orders of magnitude in a little bit more than a decade. Along these lines, the question may arise whether there will be continuous improvements for decades to come — or whether, at one point, an ultimate limitation to further improvement arises. Moreover, frequency metrology has proven superior to other methods to evince a drift of fundamental physical constants, e.g., the fine-structure constants, yet no such drift has ever been convincingly proven using either optical [2] or cosmological methods [3]. So the question is: how low can we go before quantum effects impose an ultimate limit for precision frequency metrology?
频率梳测量在过去十年中取得了巨大进展,达到了10 - 18的精度[1]。与摩尔定律类似,频率计量测量的精度在十多年的时间里提高了大约3个数量级。沿着这些路线,可能会出现这样的问题:在未来的几十年里,是否会有持续的改进——或者,在某一点上,是否会出现进一步改进的最终限制。此外,频率计量已被证明优于其他方法来证明基本物理常数的漂移,例如,精细结构常数,然而,使用光学[2]或宇宙学方法[3]都没有令人信服地证明这种漂移。所以问题是:在量子效应对精确频率测量施加最终限制之前,我们能降到多低?
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引用次数: 0
Laser Printing of a Nano-Imager to Perform Full Optical Machine Learning 实现全光学机器学习的纳米成像仪激光打印
E. Goi, M. Gu
Applications of artificial intelligence techniques, specifically machine learning and more recently deep learning [1], are transforming several fields ranging from clinical medicine to optical computing. Integrating full-optical neuromorphic architectures in opto-electronic devices (Fig. 1a) will lead to the near-term availability of clinically and industrially relevant applications such as real-time features detection and classification, image processing and optical implementation of computational intensive tasks such as matrix multiplication with low-power consumption, high-accuracy and ultra-fast processing speed [2].
人工智能技术的应用,特别是机器学习和最近的深度学习[1],正在改变从临床医学到光学计算等多个领域。在光电器件中集成全光学神经形态架构(图1a)将导致临床和工业相关应用的近期可用性,如实时特征检测和分类、图像处理和计算密集型任务的光学实现,如低功耗、高精度和超快处理速度的矩阵乘法[2]。
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引用次数: 2
All-Fiber Mode-Locked Thulium Doped Fiber Laser using a Novel Femtosecond Laser Inscribed 45° Tilted Fiber Grating 采用45°倾斜光纤光栅的新型飞秒激光器实现全光纤锁模掺铥光纤激光器
A. Theodosiou, J. Aubrecht, Nithyanandan Kanagaraj, P. Peterka, K. Kalli, I. Kašík, P. Honzátko
The recent development of mode-locked fiber lasers operating at ∼2μm is accelerating, driven by industrial and medical applications, particularly in the so-called "eye-safe" applications of laser surgery, biomedical imaging, medicine and sensing [1]. While being practical devices, given reproducible experimental conditions, fiber lasers continue to be an excellent research avenue to unveil a plethora of complex ultrafast dynamics. Developments on versatile all-fiber laser sources are attractive, due to their increased efficiency, robust and compact configurations. The development of artificial saturable absorbers, such as nonlinear polarization rotation (NPR) based on the optical Kerr effect, has enabled the realization of all-fiber formats. However, in hybrid laser designs, the use of bulk polarizers reduces the perceived advantage of the fiber-based format. In this communication, we employ a recently developed 45° tilted fiber grating (TFG) inscribed using femtosecond laser [2] as an in-line fiber polarizer in an all-fiber laser [3]. This grating inscription process offer advantages over traditional 45°-TFG UV-laser inscription, and is based on plane-by-plane, direct writing using a femtosecond laser, as it neither requires a phase mask nor a hydrogen loading process, as is usually the case.
在工业和医疗应用的推动下,特别是在激光手术、生物医学成像、医学和传感等所谓的“眼睛安全”应用中,工作在~ 2μm的锁模光纤激光器的最新发展正在加速[1]。光纤激光器虽然是实用的设备,但在可重复的实验条件下,它仍然是揭示大量复杂超快动力学的良好研究途径。多用途全光纤激光源的发展是有吸引力的,因为它们提高了效率,坚固和紧凑的配置。人工饱和吸收器的发展,如基于光学克尔效应的非线性偏振旋转(NPR),使全光纤格式的实现成为可能。然而,在混合激光设计中,使用大块偏振器降低了基于光纤格式的感知优势。在本次通信中,我们采用了最近开发的45°倾斜光纤光栅(TFG),该光栅使用飞秒激光器[2]作为全光纤激光器中的直线光纤偏振器[3]。这种光栅刻字工艺比传统的45°-TFG紫外激光刻字具有优势,并且基于使用飞秒激光的逐平面直接书写,因为它既不需要相位掩模,也不需要氢气加载过程,这通常是情况。
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引用次数: 0
The Optical Properties of AuZr Intermetallic Alloys AuZr金属间合金的光学性能
Hugh Littlehailes, W. Hendren, Stacey Drakeley, R. Bowman, F. Huang
Intermetallic alloys are increasingly attracting attention as important alternative plasmonic materials, due to their high melting temperatures and strong mechanical strength [1]. They are potential candidate materials in applications in harsh environments, such as heat-assisted magnetic recording (HAMR) and photothermal photovoltaics [2,3].
金属间合金因其熔点高、机械强度强等优点,作为一种重要的等离子体材料越来越受到人们的关注。它们是在恶劣环境下应用的潜在候选材料,如热辅助磁记录(HAMR)和光热光伏[2,3]。
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引用次数: 0
Femtosecond-Laser-Written Waveguide Lasers at ∼2 μm 飞秒激光写入波导激光器在~ 2 μm
X. Mateos, E. Kifle, P. Loiko, C. Romero, J. D. de Aldana, A. Ródenas, S. Y. Choi, J. Bae, F. Rotermund, U. Griebner, V. Petrov, M. Aguiló, F. Díaz
In this work, we review our recent results on fabrication, optical characterization and continuous-wave and passively Q-switched 2μm laser operation of active waveguides (WGs) produced by femtosecond direct laser writing (fs-DLW) in thulium and holmium doped low-symmetry (monoclinic) crystals. Fs-DLW was performed by 120-fs / 1-kHz pulses at 795 nm [1]. Various depressed-index photonic micro-structures were fabricated, Fig. 1, such as buried channel WGs with circular and hexagonal (lattice-like) cladding, surface WGs with a half-ring cladding, and straight WGs and Y-branch splitters with a rectangular cross-section. The WG core size was in the range 40–100 μm, comprising both fundamental- and multi-mode WGs.
在这项工作中,我们回顾了最近在掺铥和钬低对称(单斜)晶体中飞秒直接激光写入(fs-DLW)产生的有源波导(WGs)的制造、光学表征以及连续波和被动调q 2μm激光操作方面的研究成果。Fs-DLW采用120-fs / 1- khz脉冲,波长为795 nm[1]。我们制作了各种各样的低折射率光子微结构,如图1所示,如圆形和六边形(晶格状)包层的埋沟道光子光栅,半环形包层的表面光子光栅,以及矩形截面的直波导光子光栅和y分支分光器。WG芯尺寸在40-100 μm范围内,包括基模和多模WG。
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引用次数: 0
Following the Mechanisms of a Single Water Droplet Drying by Means of Photonic Resonant Structure 利用光子共振结构研究单水滴干燥机理
L. Garnier, H. Lhermite, V. Vié, H. Cormerais, Octave Pin, Quentin Liddell, B. Bêche
We have designed and fabricated integrated photonic micro-resonators (MRs) devices in polymer UV210 on a SiO2 substrate. UV210 is a positive resin that features an absorption band in the deep-UV domain. Such a property allows us to perform photolithography at lower wavelength than the traditional i-line photolithography so as to design smaller and more precise structures [1]. By using such MR as sensor [2,3], we have monitored the evaporation of a sessile water droplet by dynamically tracking its optical transduced signal. To do so, a broadband laser (λ = 790 nm, FWHM = 40 nm) is coupled to a set of MRs through the injection in a tapered access waveguide. The use of a broadband laser allows us to visualize several resonances on the same spectrum, which increases the precision of the data treatment. The water droplet is deposited on the MRs and the transduced signal is acquired during the whole drying process. The output optical signal is monitored by the mean of an optical spectrum analyser with a frequency of acquisition of about 1 Hz.
我们在SiO2衬底上设计并制造了基于聚合物UV210的集成光子微谐振器(MRs)器件。UV210是一种具有深紫外吸收带的正性树脂。这种特性使我们能够在比传统的i线光刻更低的波长下进行光刻,从而设计出更小、更精确的结构[1]。通过使用像传感器这样的MR[2,3],我们通过动态跟踪其光学转导信号来监测一个固定水滴的蒸发。为此,宽带激光器(λ = 790 nm, FWHM = 40 nm)通过注入锥形接入波导与一组MRs耦合。宽带激光的使用使我们能够在同一光谱上看到几个共振,这增加了数据处理的精度。在整个干燥过程中,水滴沉积在磁流变仪上,并获得转导信号。输出光信号由光谱分析仪的平均值监测,其采集频率约为1hz。
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引用次数: 2
Controllable Photon-Pair Spectral Correlations 可控光子对光谱关联
M. Cordier, B. Debord, F. Gérôme, P. Delaye, F. Benabid, I. Zaquine
Photon-pair states, whether spectrally correlated or separable, can all be very useful in quantum technology applications. For example, the former are used for improving the security of quantum key distribution, whilst the latter are the backbone in heralded single photon sources. It has been shown that the amount of spectral correlations is well-described by the shape of the Joint Spectral Amplitude function (JSA), which mostly depends on the relative group velocity relation between the pump, signal and idler photons within the source medium [1].
光子对状态,无论是光谱相关的还是可分离的,都可以在量子技术应用中非常有用。例如,前者用于提高量子密钥分发的安全性,而后者是预示的单光子源的骨干。研究表明,联合谱振幅函数(Joint spectral Amplitude function, JSA)的形状很好地描述了光谱相关性的数量,它主要取决于源介质中泵浦、信号和空闲光子之间的相对群速度关系[1]。
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引用次数: 0
期刊
2019 Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)
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