Pub Date : 2025-11-27DOI: 10.1038/s44160-025-00963-9
Wenying Cao, Jie Yang, Benke Hong
{"title":"Author Correction: Discovery and engineering of the biosynthesis of rotenoids","authors":"Wenying Cao, Jie Yang, Benke Hong","doi":"10.1038/s44160-025-00963-9","DOIUrl":"10.1038/s44160-025-00963-9","url":null,"abstract":"","PeriodicalId":74251,"journal":{"name":"Nature synthesis","volume":"5 1","pages":"151-151"},"PeriodicalIF":20.0,"publicationDate":"2025-11-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.nature.comhttps://www.nature.com/articles/s44160-025-00963-9.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145609587","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2025-11-25DOI: 10.1038/s44160-025-00939-9
Zichao Rong, Zihao Chen, Felix Luong, Saumil Chheda, H. T. Nhan Luong, Zhiling Zheng, Kevin Greco, Abdullah A. Alghamdi, K. Huyen Bui, Théo Jaffrelot Inizan, Tung Nguyen-Dang, H. Hieu Pham, Dung D. Le, Joachim Sauer, Viet Bac T. Phung, Jennifer T. Chayes, Christian Borgs, Mario Boley, Laurent El Ghaoui, Omar M. Yaghi
The discovery of crystalline reticular materials remains largely trial-and-error despite their societal importance. We introduce our algorithmic iterative reticular synthesis (AIRES) cycle, which integrates automated synthesis, image recognition, single-crystal X-ray diffraction and, crucially, customized algorithmic decision-making, to maximize distinct crystal discoveries rather than optimizing single targets. Demonstrated on zeolitic imidazolate frameworks (ZIFs), AIRES achieves twice the discovery rate of random exploration, crystallizing 10 new linkers into diverse ZIF topologies and expanding the single-linker Zn-ZIF library by one-third. By transforming reticular synthesis from an empirical process to a systematic exploration, AIRES provides a scalable and efficient blueprint for accelerating materials discovery.
{"title":"Algorithmic iterative reticular synthesis of zeolitic imidazolate framework crystals","authors":"Zichao Rong, Zihao Chen, Felix Luong, Saumil Chheda, H. T. Nhan Luong, Zhiling Zheng, Kevin Greco, Abdullah A. Alghamdi, K. Huyen Bui, Théo Jaffrelot Inizan, Tung Nguyen-Dang, H. Hieu Pham, Dung D. Le, Joachim Sauer, Viet Bac T. Phung, Jennifer T. Chayes, Christian Borgs, Mario Boley, Laurent El Ghaoui, Omar M. Yaghi","doi":"10.1038/s44160-025-00939-9","DOIUrl":"https://doi.org/10.1038/s44160-025-00939-9","url":null,"abstract":"The discovery of crystalline reticular materials remains largely trial-and-error despite their societal importance. We introduce our algorithmic iterative reticular synthesis (AIRES) cycle, which integrates automated synthesis, image recognition, single-crystal X-ray diffraction and, crucially, customized algorithmic decision-making, to maximize distinct crystal discoveries rather than optimizing single targets. Demonstrated on zeolitic imidazolate frameworks (ZIFs), AIRES achieves twice the discovery rate of random exploration, crystallizing 10 new linkers into diverse ZIF topologies and expanding the single-linker Zn-ZIF library by one-third. By transforming reticular synthesis from an empirical process to a systematic exploration, AIRES provides a scalable and efficient blueprint for accelerating materials discovery.","PeriodicalId":74251,"journal":{"name":"Nature synthesis","volume":"1 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-11-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145593789","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2025-11-24DOI: 10.1038/s44160-025-00932-2
Yangwoo Lee, Hyung-Jun Koo
Liquid gallium is employed as a reaction medium to synthesize uniquely structured solid–liquid–solid core–shell–shell nanoparticles, enabling the fabrication of diverse metallic nanostructures with excellent electrocatalytic performance.
{"title":"Liquid metal nanoreactors forge dynamic and stable nanocatalysts","authors":"Yangwoo Lee, Hyung-Jun Koo","doi":"10.1038/s44160-025-00932-2","DOIUrl":"10.1038/s44160-025-00932-2","url":null,"abstract":"Liquid gallium is employed as a reaction medium to synthesize uniquely structured solid–liquid–solid core–shell–shell nanoparticles, enabling the fabrication of diverse metallic nanostructures with excellent electrocatalytic performance.","PeriodicalId":74251,"journal":{"name":"Nature synthesis","volume":"4 12","pages":"1477-1478"},"PeriodicalIF":20.0,"publicationDate":"2025-11-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145583126","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2025-11-24DOI: 10.1038/s44160-025-00928-y
Rhys W. Hughes, Brent S. Sumerlin
Electrolysis enables selective dual C–H functionalization for transforming inert polyolefin deconstruction products into dynamic recyclable networks.
电解使选择性双碳氢功能化转化惰性聚烯烃解构产品为动态可回收的网络。
{"title":"Electrochemical upcycling of polyolefins into adaptable networks","authors":"Rhys W. Hughes, Brent S. Sumerlin","doi":"10.1038/s44160-025-00928-y","DOIUrl":"10.1038/s44160-025-00928-y","url":null,"abstract":"Electrolysis enables selective dual C–H functionalization for transforming inert polyolefin deconstruction products into dynamic recyclable networks.","PeriodicalId":74251,"journal":{"name":"Nature synthesis","volume":"4 12","pages":"1483-1484"},"PeriodicalIF":20.0,"publicationDate":"2025-11-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145583127","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2025-11-20DOI: 10.1038/s44160-025-00940-2
Weijin Wang, Xinjian Ji, Pol Gorrea-Acín, Kelvin Lau, Florence Pojer, Thomas R. Ward, Xile Hu
{"title":"Construction of dual-cofactor artificial metalloenzymes for synergistic and enantiodivergent catalysis of Michael addition reactions","authors":"Weijin Wang, Xinjian Ji, Pol Gorrea-Acín, Kelvin Lau, Florence Pojer, Thomas R. Ward, Xile Hu","doi":"10.1038/s44160-025-00940-2","DOIUrl":"https://doi.org/10.1038/s44160-025-00940-2","url":null,"abstract":"","PeriodicalId":74251,"journal":{"name":"Nature synthesis","volume":"8 1","pages":""},"PeriodicalIF":0.0,"publicationDate":"2025-11-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"145554626","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
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