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Two-dimensional material/group-III nitride hetero-structures and devices. 二维材料/III 族氮化物异质结构和器件的最新进展。
Pub Date : 2025-04-04 DOI: 10.1088/1361-6633/adb6bc
Tingting Lin, Yi Zeng, Xinyu Liao, Jing Li, Changjian Zhou, Wenliang Wang

Two-dimensional (2D) material (graphene, MoS2, WSe2, MXene,etc)/group-III nitride (GaN, AlN, and their compounds) hetero-structures have been given special attention, on account of their prospective applications in remarkable performance broadband photodetectors, light-emitting diodes, solar cells, memristors, hydrogen sensors,etc. The utilization of advantages of the above two kind materials provides a solution to the dilemma of the degradation of device performance and reliability caused by carrier mobility, contact resistance, lattice mismatch, interface, and other factors. Therefore, the summary of the recent progress of 2D material/group-III nitride hetero-structures is urgent. In this work, it elaborates on interface interaction and stimulation, growth mechanism and device physic of 2D material/group-III nitride hetero-structures. Initially, it investigates the properties of the hetero-structures, combining the theoretical calculations on interface interaction of the heterojunction with experimental study, particularly emphasizing on interface effects on the performance of hetero-materials. The structure modification (band alignments, band edge position, synergetic work function and so on) at interface contributes to the outstanding properties of these hetero-structures. Subsequently, the growth of 2D material/group-III nitride hetero-structures is introduced in detail. The problems solved by the advancing synthesis strategies and the corresponding formation mechanisms are discussed in particular. Afterwards, based on the 2D material/group-III nitride hetero-structures, extending from optoelectronics, electronics, to photocatalyst and sensors,etc, are reviewed. Finally, the prospect of 2D material/group-III nitride hetero-structures is speculated to pave the way for further promotion.

二维(2D)材料(石墨烯,MoS2, MXene等)/ iii族氮化物(GaN, AlN及其化合物)异质结构由于其在高性能宽带光电探测器,发光二极管,太阳能电池等方面的潜在应用而受到特别关注。利用上述两种材料的优点,解决了载流子迁移率、晶格失配、界面等导致器件性能和可靠性下降的困境。因此,总结二维材料/ iii族氮化物异质结构和器件的研究进展迫在眉睫。本文阐述了二维材料/ iii族氮化物异质结构的界面相互作用和激发、生长和器件。首先,将异质结界面相互作用的理论计算与实验研究相结合,研究了异质结的性能,特别强调了界面效应对异质结性能的影响。随后,详细介绍了二维材料/ iii族氮化物异质结构的生长。重点讨论了先进的合成策略所解决的问题和形成机理。然后,基于二维材料/ iii族氮化物异质结构,从光电子学、电子学到光催化剂、传感器等器件进行了综述。最后,对二维材料/ iii族氮化物异质结构及器件的发展前景进行了展望,为进一步推广铺路。
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引用次数: 0
Fundamental concepts, design rules and potentials in radiative cooling. 辐射冷却的基本概念、设计规则和潜力。
Pub Date : 2025-03-28 DOI: 10.1088/1361-6633/adc69d
Zhuning Wang, Sijie Pian, Yulei Zhang, Yaoguang Ma

Amidst the escalating environmental concerns driven by global warming and the detrimental impacts of extreme climates, energy consumption and greenhouse gas emissions associated with refrigeration have reached unprecedented levels. Radiative cooling, as an emerging renewable cooling technology, has been positioned as a pivotal strategy in the fight against global warming. This review examines the theoretical model of radiative cooling emitters and complex practical environment. We first investigate the thermodynamic interactions between environmental factors and the cooling surface, followed by an examination of innovative modulation techniques such as asymmetric/non-reciprocal radiative heat transfer mechanisms. Additionally, we summarize the latest advancements in structural design and simulation methodologies for radiative cooling materials at the device level. We then delve into potential applications of radiative cooling materials in various scenarios including energy-efficient construction, personal thermal management, photovoltaic cooling, and dynamic PDRC materials with seasonal adaptability. In conclusion, we provide a comprehensive overview of this technology's strengths and current challenges to inspire further research and application development in radiative cooling technology with a focus on contributing towards energy conservation objectives and promoting a sustainable society.

由于全球变暖和极端气候的不利影响,环境问题日益严重,与制冷相关的能源消耗和温室气体排放达到了前所未有的水平。辐射冷却作为一种新兴的可再生冷却技术,已被定位为应对全球变暖的关键战略。本文综述了辐射冷却源的理论模型和复杂的实际环境。我们首先研究了环境因素与冷却表面之间的热力学相互作用,然后研究了创新的调制技术,如不对称/非互反辐射传热机制。此外,我们总结了辐射冷却材料在器件级的结构设计和模拟方法的最新进展。然后,我们深入研究了辐射冷却材料在各种场景中的潜在应用,包括节能建筑、个人热管理、光伏冷却和具有季节性适应性的动态PDRC材料。最后,我们对辐射冷却技术的优势和当前面临的挑战进行了全面的概述,以激励辐射冷却技术的进一步研究和应用开发,重点是为实现节能目标和促进可持续社会做出贡献。
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引用次数: 0
Perturbative framework for engineering arbitrary Floquet Hamiltonian. 工程任意Floquet hamilton量的微扰框架。
Pub Date : 2025-02-21 DOI: 10.1088/1361-6633/adb072
Yingdan Xu, Lingzhen Guo

We develop a systematic perturbative framework to engineer an arbitrary target Hamiltonian in the Floquet phase space of a periodically driven oscillator based on Floquet-Magnus expansion. The high-order errors in the engineered Floquet Hamiltonian are mitigated by adding high-order driving potentials perturbatively. We introduce a transformation method that allows us to obtain an analytical expression of the leading-order correction drive for engineering a target Hamiltonian with discrete rotational and chiral symmetries in phase space. We also provide a numerically efficient procedure to calculate high-order correction drives and apply it to engineer the target Hamiltonian with degenerate eigenstates of multi-component cat states that are important for fault-tolerant hardware-efficiency bosonic quantum computation.

基于Floquet- magnus展开,建立了一个系统微扰框架,在周期驱动振荡器的Floquet相空间中构造任意目标哈密顿量。通过扰动加入高阶驱动势,减小了工程Floquet hamilton算符的高阶误差。我们介绍了一种变换方法,使我们能够得到在相空间中具有离散旋转和手性对称的工程目标哈密顿量的一阶修正驱动的解析表达式。我们还提供了一个数值上有效的程序来计算高阶校正驱动器,并将其应用于设计具有多分量cat状态的退化特征态的目标哈密顿量,这对于容错硬件效率玻色子量子计算非常重要。
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引用次数: 0
Liquid-liquid crystalline phase separation of filamentous colloids and semiflexible polymers: experiments, theory and simulations. 丝状胶体和半柔性聚合物的液-液相分离:实验、理论和模拟。
Pub Date : 2025-02-20 DOI: 10.1088/1361-6633/adb441
Hamed Almohammadi, Sayyed Ahmad Khadem, Paride Azzari, Ye Yuan, André Guerra, Alejandro D Rey, Raffaele Mezzenga

Liquid-liquid crystalline phase separation (LLCPS) is the process by which an initially homogenous single-phase solution composed of a solvent-most frequently water- and a solute-typically rigid or semiflexible macromolecules, polymers, supramolecular aggregates, or filamentous colloids-demixes into two (or more) distinct phases in which one phase is depleted by the solute and features properties of isotropic solutions, whereas the other is enriched by the solute and exhibits liquid crystalline anisotropic properties. Differently from the more common liquid-liquid phase separation (LLPS) of flexible macromolecules, which is a trade-off between entropy and enthalpy, LLCPS is mostly an entropy-controlled process in which the morphology, composition and properties of the new phases depend primarily on kinetics and thermodynamic factors and, unexpectedly, on the history followed to reach a specific point in the phase diagram. This review aims to comprehensively discuss the process of LLCPS from experimental, theoretical, and simulation standpoints. We discuss the main systems and experimental approaches followed over the past decades to induce and control LLCPS, then we delve into the main theoretical and modeling approaches available to rationalize this process, and finally, we expand on how numerical simulations can significantly enrich the understanding of LLCPS. A final section touches on possible applications and the significance of LLCPS beyond pure physics, that is, in the broader context of biology, nanotechnology, and everyday life.

液-液结晶相分离(LLCPS)是一种由溶剂(通常是水)和溶质(通常是刚性或半柔性大分子、聚合物、超分子聚集体或丝状胶体)组成的初始均质单相溶液分解成两个(或更多)不同相的过程,其中一个相被溶质耗尽,并具有各向同性溶液的特性。而另一种则被溶质富集,表现出液晶的各向异性。与更常见的柔性大分子的液-液相分离(LLPS)不同,这是熵和焓之间的权衡,LLCPS主要是一个熵控制的过程,其中新相的形态、组成和性质主要取决于动力学和热力学因素,出乎意料的是,取决于达到相图中特定点的历史。本文旨在从实验、理论和模拟的角度全面讨论LLCPS的过程。我们讨论了过去几十年来诱导和控制LLCPS的主要系统和实验方法,然后我们深入研究了可用于合理化这一过程的主要理论和建模方法,最后,我们扩展了数值模拟如何显著丰富对LLCPS的理解。最后一节涉及到LLCPS在纯物理之外的可能应用和意义,即在生物学、纳米技术和日常生活的更广泛背景下。
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引用次数: 0
Transport resistance strikes back: unveiling its impact on fill factor losses in organic solar cells. 运输阻力反击:揭示其对有机太阳能电池中填充因子损失的影响。
Pub Date : 2025-02-17 DOI: 10.1088/1361-6633/adb20c
Maria Saladina, Carsten Deibel

The fill factor (FF) is a critical parameter for solar cell efficiency, but its analytical description is challenging due to the interplay between recombination and charge extraction processes. A significant factor contributing toFFlosses, beyond recombination, that has not received much attention is the influence of charge transport. In most state-of-the-art organic solar cells, the primary limitations of theFFdo not just arise from non-radiative recombination, but also from low conductivity of the organic semiconductors. A closer look reveals that even in the highest efficiency cells, performance losses due to transport resistance are significant. This finding highlights the need for refined models to predict theFFaccurately. Here, we extend the analytical model for transport resistance to a more general case by incorporating energetic disorder. We introduce a straightforward set of equations to predict theFFof a solar cell, enabling the differentiation of losses attributed to recombination and transport resistance. Our analytical model is validated with a large set of experimental current-voltage and light intensity-dependent open-circuit voltage data for a wide range of temperatures. Based on our findings, we provide valuable insights into strategies for mitigatingFFlosses, guiding the development of more efficient solar cell designs and optimisation strategies.

填充因子(FF)是太阳能电池效率的关键参数,但由于重组和电荷提取过程之间的相互作用,对其进行分析描述具有挑战性。除重组外,导致填充因子损失的一个重要因素是电荷传输的影响,但这一因素并未得到广泛关注。在大多数最先进的有机太阳能电池中,FF 的主要限制不仅来自非辐射重组,还来自有机半导体的低电导率。仔细观察就会发现,即使在效率最高的电池中,传输电阻造成的性能损失也很大。这一发现凸显了精确预测 FF 的精细模型的必要性。 在这里,我们通过系统地纳入能量无序,将传输电阻的分析模型扩展到了更一般的情况。我们引入了一套简单明了的方程来预测太阳能电池的 FF,从而能够区分归因于重组和输运电阻的损耗。我们的分析模型通过大量温度范围内的实验电流-电压数据和与光照强度相关的开路电压数据进行了验证。基于我们的研究结果,我们为减轻 FF 损耗的策略提供了宝贵的见解,为开发更高效的太阳能电池设计和优化策略提供了指导。
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引用次数: 0
A cordial introduction to double scaled SYK. 双尺度SYK的亲切介绍。
Pub Date : 2025-02-14 DOI: 10.1088/1361-6633/ada889
Micha Berkooz, Ohad Mamroud

We review recent progress regarding the double scaled Sachdev-Ye-Kitaev model and otherp-local quantum mechanical random Hamiltonians. These models exhibit an expansion using chord diagrams, which can be solved by combinatorial methods. We describe exact results in these models, including their spectrum, correlation functions, and Lyapunov exponent. In a certain limit, these techniques manifest the relation to the Schwarzian quantum mechanics, a theory of quantum gravity inAdS2. More generally, the theory is controlled by a rigid algebraic structure of a quantum group, suggesting a theory of quantum gravity on non-commutativeq-deformedAdS2. We conclude with discussion of related universality classes, and survey some of the current research directions.

本文综述了双尺度Sachdev-Ye-Kitaev模型和其他p局部量子力学随机哈密顿量的最新进展。这些模型采用和弦图展开,可以用组合方法求解。我们描述了这些模型的精确结果,包括它们的谱、相关函数和李雅普诺夫指数。在一定限度内,这些技术显示了与Schwarzian量子力学的关系,这是AdS2中的量子引力理论。更一般地说,该理论是由量子群的刚性代数结构控制的,提出了非交换q-变形AdS2上的量子引力理论。最后对相关的普适性类进行了讨论,并对目前的一些研究方向进行了综述。
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引用次数: 0
Smoothed particle hydrodynamics for free-surface and multiphase flows: a review. 自由表面和多相流的光滑粒子流体力学研究进展。
Pub Date : 2025-02-11 DOI: 10.1088/1361-6633/ada80f
David Le Touzé, Andrea Colagrossi

The smoothed particle hydrodynamics (SPH) method is expanding and is being applied to more and more fields, particularly in engineering. The majority of current SPH developments deal with free-surface and multiphase flows, especially for situations where geometrically complex interface configurations are involved. The present review article covers the last 25 years of development of the method to simulate such flows, discussing the related specific features of the method. A path is drawn to link the milestone articles on the topic, and the main related theoretical and numerical issues are investigated. In particular, several SPH schemes have been derived over the years, based on different assumptions. The main ones are presented and discussed in this review underlining the different contexts and the ways in which they were derived, resulting in similarities and differences. In addition, a summary is provided of the recent corrections proposed to increase the accuracy, stability and robustness of SPH schemes in the context of free-surface and multiphase flows. Future perspectives of development are identified, placing the method within the panorama of Computational Fluid Dynamics.

光滑粒子流体力学(SPH)方法在越来越多的领域得到了扩展和应用,特别是在工程领域。目前大多数SPH开发都涉及自由表面和多相流,特别是涉及几何复杂界面配置的情况。这篇综述文章涵盖了过去25年来模拟这种流动的方法的发展,讨论了该方法的相关具体特征。绘制了一条路径来连接关于该主题的里程碑文章,并研究了主要的相关理论和数值问题。特别是,基于不同的假设,多年来推导了几种SPH格式。本文将介绍和讨论这些主要词汇,并强调它们的不同背景和产生方式,从而得出它们的异同。此外,总结了最近提出的修正,以提高SPH方案在自由表面和多相流背景下的准确性、稳定性和鲁棒性,并确定了将该方法置于计算流体动力学全景中的未来发展前景。
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引用次数: 0
Corrigendum: A review of UTe2at high magnetic fields (2023Rep. Prog. Phys.86 114501). 勘误:UTe2at高磁场的回顾(2023Rep.)。掠夺。Phys.86 114501)。
Pub Date : 2025-02-07 DOI: 10.1088/1361-6633/adb04d
Sylvia K Lewin, Corey E Frank, Sheng Ran, Johnpierre Paglione, Nicholas P Butch
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引用次数: 0
Interatomic Coulombic decay in lithium-doped large helium nanodroplets induced by photoelectron impact excitation. 光电子冲击激发下掺锂大氦纳米液滴的原子间库仑衰变。
Pub Date : 2025-02-07 DOI: 10.1088/1361-6633/ada9c6
L Ben Ltaief, K Sishodia, J D Asmussen, A R Abid, S R Krishnan, H B Pedersen, N Sisourat, M Mudrich

Irradiation of condensed matter with ionizing radiation generally causes direct photoionization as well as secondary processes that often dominate the ionization dynamics. Here, large helium (He) nanodroplets with radius≳40nm doped with lithium (Li) atoms are irradiated with extreme ultraviolet (XUV) photons of energyhν⩾44.4 eV and indirect ionization of the Li dopants is observed in addition to direct photoionization of the He droplets. Specifically, Li ions are efficiently produced by an interatomic Coulombic decay (ICD) process involving metastable He∗atoms and He2∗excimers which are populated by elastic and inelastic scattering of photoelectrons in the nanodroplets as well as by electron-ion recombination. This type of indirect ICD, observed in large He nanodroplets in nearly the entire XUV range, turns out to be more efficient than Li dopant ionization by ICD following direct resonant photoexcitation athν=21.6eV and by charge-transfer ionization. Indirect ICD processes induced by scattering of photoelectrons likely play an important role in other condensed phase systems exposed to ionizing radiation as well, including biological matter.

用电离辐射照射凝聚态物质通常会引起直接的光电离以及通常主导电离动力学的二次过程。用能量为hν≥44.4 eV的极紫外(XUV)光子照射半径为≥40 nm的掺锂(Li)原子的氦(He)纳米液滴,在观察到Li掺杂剂的直接光离的同时,还观察到Li掺杂剂的间接电离。具体来说,Li离子是通过原子间库仑衰变(ICD)过程有效地产生的,该过程涉及亚稳态He*原子和He2*准分子,这些准分子由纳米液滴中光电子的弹性和非弹性散射以及电子-离子复合填充。在几乎整个XUV范围内的大He纳米液滴中观察到,这种类型的间接ICD比在hν = 21.6 eV的直接共振光激发下通过ICD和电荷转移电离的Li掺杂剂电离效率更高。由光电子散射引起的间接ICD过程可能在暴露于电离辐射的其他凝聚相系统中也发挥重要作用,包括生物物质。
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引用次数: 0
Search for light long-lived particles decaying to displaced jets in proton-proton collisions ats=13.6 TeV. 寻找在√s = 13.6 TeV的质子-质子碰撞中衰变为位移射流的轻长寿命粒子。
Pub Date : 2025-02-03 DOI: 10.1088/1361-6633/adaa13
The Cms Collaboration

A search for light long-lived particles (LLPs) decaying to displaced jets is presented, using a data sample of proton-proton collisions at a center-of-mass energy of 13.6 TeV, corresponding to an integrated luminosity of 34.7 fb-1, collected with the CMS detector at the CERN LHC in 2022. Novel trigger, reconstruction, and machine-learning techniques were developed for and employed in this search. After all selections, the observations are consistent with the background predictions. Limits are presented on the branching fraction of the Higgs boson to LLPs that subsequently decay to quark pairs or tau lepton pairs. An improvement by up to a factor of 10 is achieved over previous limits for models with LLP masses smaller than 60 GeV and proper decay lengths smaller than 1 m. The first constraints are placed on the fraternal twin Higgs (FTH) and folded supersymmetry (FSUSY) models, where the lower bounds on the top quark partner mass reach up to 350 GeV for the FTH model and 250 GeV for the FSUSY model.

利用CERN大型强子对撞机(CMS)探测器于2022年采集的质能为13.6 TeV的质子-质子碰撞数据样本(对应的综合光度为34.7 fb$^{-1}$),研究了衰变为位移射流的轻长寿命粒子。新的触发、重建和机器学习技术被开发并应用于这项研究。经过所有的选择,观测结果与背景预测是一致的。对希格斯玻色子分支分数的限制提出了长寿命粒子,随后衰变成夸克对或tau轻子对。对于长寿命粒子质量小于60 GeV和适当衰变长度小于1 m的模型,实现了比以前限制的10倍的改进。第一个约束条件是兄弟孪生希格斯和折叠超对称模型,其中兄弟孪生希格斯模型的顶夸克伴侣质量下界达到350 GeV,折叠超对称模型的下界达到250 GeV。
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引用次数: 0
期刊
Reports on progress in physics. Physical Society (Great Britain)
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