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Crystal structure and magnetism of actinide oxides: a review. 锕系元素氧化物的晶体结构和磁性:综述。
Pub Date : 2024-05-16 DOI: 10.1088/1361-6633/ad38cb
Binod K Rai, Alex Bretaña, Gregory Morrison, Rosalie Greer, Krzysztof Gofryk, Hans-Conrad Zur Loye

In actinide systems, the 5felectrons experience a uniquely delicate balance of effects and interactions having similar energy scales, which are often difficult to properly disentangle. This interplay of factors such as the dual nature of 5f-states, strong electronic correlations, and strong spin-orbit coupling results in electronically unusual and intriguing behavior such as multi-k antiferromagnetic ordering, multipolar ordering, Mott-physics, mixed valence configurations, and more. Despite the inherent allure of their exotic properties, the exploratory science of even the more basic, binary systems like the actinide oxides has been limited due to their toxicity, radioactivity, and reactivity. In this article, we provide an overview of the available synthesis techniques for selected binary actinide oxides, including the actinide dioxides, sesquioxides, and a selection of higher oxides. For these oxides, we also review and evaluate the current state of knowledge of their crystal structures and magnetic properties. In many aspects, substantial knowledge gaps exist in the current body of research on actinide oxides related to understanding their electronic ground states. Bridging these gaps is vital for improving not only a fundamental understanding of these systems but also of future nuclear technologies. To this end, we note the experimental techniques and necessary future investigations which may aid in better elucidating the nature of these fascinating systems.

在锕系元素系统中,5f 电子经历了独特的微妙平衡效应和相互作用 ,这些效应和相互作用具有相似的能量尺度,通常很难正确地将其分开。5f态的双重特性、相互竞争的相互作用以及强自旋轨道耦合等因素的相互作用,导致了磁学上不同寻常、引人入胜的行为:多k反铁磁有序、多极有序、混合价态等。尽管锕系元素具有与生俱来的诱人奇特性质,但由于其毒性、放射性和反应性,即使是更基本的二元系统(如锕系元素氧化物)的探索性科学研究也极为有限。本文概述了部分二元锕系元素氧化物的现有合成技术,包括锕系元素二氧化物、倍半氧化物和部分高级氧化物。对于这些氧化物,我们回顾并评估了有关其晶体结构和磁性能的知识现状。在了解锕系元素氧化物的磁基态方面,目前的研究还存在许多知识空白。缩小这些差距不仅对增进对这些系统的基本了解,而且对未来的核 技术都至关重要 。为此,我们指出了实验技术和必要的未来研究 ,它们可能有助于更好地阐明这些迷人系统的本质。
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引用次数: 0
Acoustic manipulation of multi-body structures and dynamics. 多体结构和动力学的声学操纵。
Pub Date : 2024-05-15 DOI: 10.1088/1361-6633/ad43f9
Melody X Lim, Bryan VanSaders, Heinrich M Jaeger

Sound can exert forces on objects of any material and shape. This has made the contactless manipulation of objects by intense ultrasound a fascinating area of research with wide-ranging applications. While much is understood for acoustic forcing of individual objects, sound-mediated interactions among multiple objects at close range gives rise to a rich set of structures and dynamics that are less explored and have been emerging as a frontier for research. We introduce the basic mechanisms giving rise to sound-mediated interactions among rigid as well as deformable particles, focusing on the regime where the particles' size and spacing are much smaller than the sound wavelength. The interplay of secondary acoustic scattering, Bjerknes forces, and micro-streaming is discussed and the role of particle shape is highlighted. Furthermore, we present recent advances in characterizing non-conservative and non-pairwise additive contributions to the particle interactions, along with instabilities and active fluctuations. These excitations emerge at sufficiently strong sound energy density and can act as an effective temperature in otherwise athermal systems.

声音可以对任何材料和形状的物体施加力。因此,通过强烈的超声波对物体进行非接触式操纵成为一个具有广泛应用的迷人研究领域。虽然人们对单个物体的声学作用力已经有了很多了解,但近距离内多个物体之间以声音为媒介的相互作用却产生了一系列丰富的结构和动力学,而人们对这些结构和动力学的探索还比较少,这些结构和动力学正在成为研究的前沿领域。我们介绍了刚性颗粒和可变形颗粒之间以声音为媒介的相互作用的基本机制,重点是颗粒尺寸和间距远小于声音波长的情况。我们讨论了二次声散射、Bjerknes 力和微流的相互作用,并强调了颗粒形状的作用。此外,我们还介绍了在描述粒子相互作用的非守恒和非成对相加贡献以及不稳定性和活跃波动方面的最新进展。这些激发在足够强的声能密度下出现,并能在其他非热系统中充当有效温度。
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引用次数: 0
Learning dynamical models of single and collective cell migration: a review. 学习单细胞和集体细胞迁移的动力学模型:综述。
Pub Date : 2024-04-04 DOI: 10.1088/1361-6633/ad36d2
David B Brückner, Chase P Broedersz

Single and collective cell migration are fundamental processes critical for physiological phenomena ranging from embryonic development and immune response to wound healing and cancer metastasis. To understand cell migration from a physical perspective, a broad variety of models for the underlying physical mechanisms that govern cell motility have been developed. A key challenge in the development of such models is how to connect them to experimental observations, which often exhibit complex stochastic behaviours. In this review, we discuss recent advances in data-driven theoretical approaches that directly connect with experimental data to infer dynamical models of stochastic cell migration. Leveraging advances in nanofabrication, image analysis, and tracking technology, experimental studies now provide unprecedented large datasets on cellular dynamics. In parallel, theoretical efforts have been directed towards integrating such datasets into physical models from the single cell to the tissue scale with the aim of conceptualising the emergent behaviour of cells. We first review how this inference problem has been addressed in both freely migrating and confined cells. Next, we discuss why these dynamics typically take the form of underdamped stochastic equations of motion, and how such equations can be inferred from data. We then review applications of data-driven inference and machine learning approaches to heterogeneity in cell behaviour, subcellular degrees of freedom, and to the collective dynamics of multicellular systems. Across these applications, we emphasise how data-driven methods can be integrated with physical active matter models of migrating cells, and help reveal how underlying molecular mechanisms control cell behaviour. Together, these data-driven approaches are a promising avenue for building physical models of cell migration directly from experimental data, and for providing conceptual links between different length-scales of description.

从胚胎发育、免疫反应到伤口愈合和癌症转移,单细胞和集体细胞迁移都是对各种生理现象至关重要的基本过程。为了从物理角度理解细胞迁移,人们开发了各种各样的模型来研究支配细胞运动的基本物理机制。建立此类模型的一个关键挑战是如何将模型与实验观察结果联系起来,而实验观察结果往往表现出复杂的随机行为。在本综述中,我们将讨论数据驱动理论方法的最新进展,这些方法可直接与实验数据连接,从而推断出随机细胞迁移的动力学模型。利用纳米制造、图像分析和跟踪技术的进步,实验研究现在提供了前所未有的细胞动态大数据集。与此同时,理论界也在努力将这些数据集整合到从单细胞到组织尺度的物理模型中,目的是将细胞的突发行为概念化。我们首先回顾了如何在自由迁移和封闭细胞中解决这一推理问题。接下来,我们将讨论为什么这些动力学通常采用欠阻尼随机运动方程的形式,以及如何从数据中推断出这种方程。然后,我们回顾了数据驱动推理和机器学习方法在细胞行为异质性、亚细胞自由度以及多细胞系统集体动力学方面的应用。在这些应用中,我们强调数据驱动方法如何与迁移细胞的物理活性物质模型相结合,并帮助揭示潜在的分子机制如何控制细胞行为。总之,这些数据驱动方法是直接从实验数据中建立细胞迁移物理模型,并在不同描述长度尺度之间提供概念联系的大有可为的途径。
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引用次数: 0
Charge density waves in two-dimensional transition metal dichalcogenides. 二维过渡金属二卤化物中的电荷密度波。
Pub Date : 2024-04-02 DOI: 10.1088/1361-6633/ad36d3
Jinwoong Hwang, Wei Ruan, Yi Chen, Shujie Tang, Michael F Crommie, Zhi-Xun Shen, Sung-Kwan Mo

Charge density wave (CDW is one of the most ubiquitous electronic orders in quantum materials. While the essential ingredients of CDW order have been extensively studied, a comprehensive microscopic understanding is yet to be reached. Recent research efforts on the CDW phenomena in two-dimensional (2D) materials provide a new pathway toward a deeper understanding of its complexity. This review provides an overview of the CDW orders in 2D with atomically thin transition metal dichalcogenides (TMDCs) as the materials platform. We mainly focus on the electronic structure investigations on the epitaxially grown TMDC samples with angle-resolved photoemission spectroscopy and scanning tunneling microscopy/spectroscopy as complementary experimental tools. We discuss the possible origins of the 2D CDW, novel quantum states coexisting with them, and exotic types of charge orders that can only be realized in the 2D limit.

电荷密度波(CDW)是量子材料中最普遍的电子秩之一。虽然人们已经对CDW阶的基本成分进行了广泛研究,但尚未达成全面的微观认识。最近对二维(2D)材料中 CDW 现象的研究为深入了解其复杂性提供了一条新途径。本综述概述了以原子薄过渡金属二卤化物(TMDCs)为材料平台的二维 CDW 秩。我们主要关注外延生长的 TMDC 样品的电子结构研究,并以角分辨光发射光谱和扫描隧道显微镜/光谱作为补充实验工具。我们讨论了二维 CDW 的可能起源、与之共存的新型量子态以及只有在二维极限下才能实现的奇异类型电荷阶。
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引用次数: 0
The surface force balance: direct measurement of interactions in fluids and soft matter. 表面力平衡:直接测量流体和软物质中的相互作用。
Pub Date : 2024-03-19 DOI: 10.1088/1361-6633/ad2b9b
Hannah J Hayler, Timothy S Groves, Aurora Guerrini, Astrid Southam, Weichao Zheng, Susan Perkin

Over the last half-century, direct measurements of surface forces have been instrumental in the exploration of a multitude of phenomena in liquid, soft, and biological matter. Measurements of van der Waals interactions, electrostatic interactions, hydrophobic interactions, structural forces, depletion forces, and many other effects have checked and challenged theoretical predictions and motivated new models and understanding. The gold-standard instrument for these measurements is thesurface force balance(SFB), orsurface forces apparatus, where interferometry is used to detect the interaction force and distance between two atomically smooth planes, with 0.1 nm resolution, over separations from about 1 µm down to contact. The measured interaction forcevs.distance gives access to the free energy of interaction across the fluid film; a fundamental quantity whose general form and subtle features reveal the underlying molecular and surface interactions and their variation. Motivated by new challenges in emerging fields of research, such as energy storage, biomaterials, non-equilibrium and driven systems, innovations to the apparatus are now clearing the way for new discoveries. It is now possible to measure interaction forces (and free energies) with control of electric field, surface potential, surface chemistry; to measure time-dependent effects; and to determine structurein situ. Here, we provide an overview the operating principles and capabilities of the SFB with particular focus on the recent developments and future possibilities of this remarkable technique.

在过去的半个世纪里,对表面力的直接测量在探索液体、软物质和生物物质的多种现象中发挥了重要作用。对范德华相互作用、静电相互作用、疏水相互作用、结构力、损耗力和许多其他效应的测量,检验和挑战了理论预测,并激发了新的模型和理解。这些测量的黄金标准仪器是(textit{表面力天平},或(textit{表面力仪器},其中干涉测量法用于检测两个原子平滑平面之间的相互作用力和距离,分辨率为 0.1~nm,测量范围从大约 1~unit{um} 到接触。通过测量相互作用力与距离的关系,可以获得流体薄膜之间相互作用的自由能;这是一个基本量,其一般形式和微妙特征揭示了分子和表面相互作用的基本情况及其变化。在能量储存、生物材料、非平衡和驱动系统等新兴研究领域的新挑战的推动下,仪器的创新正在为新发现开辟道路。现在,我们可以通过控制电场、表面电位、表面化学来测量相互作用力(和自由能);测量随时间变化的效应;以及原位确定结构。在此,我们将概述表面力平衡的工作原理和功能,并特别关注这一非凡技术的最新发展和未来可能性。
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引用次数: 0
Bridging the gap between surface physics and photonics. 缩小表面物理学与光子学之间的差距。
Pub Date : 2024-03-06 DOI: 10.1088/1361-6633/ad2ac9
Pekka Laukkanen, Marko Punkkinen, Mikhail Kuzmin, Kalevi Kokko, Xiaolong Liu, Behrad Radfar, Ville Vähänissi, Hele Savin, Antti Tukiainen, Teemu Hakkarainen, Jukka Viheriälä, Mircea Guina

Use and performance criteria of photonic devices increase in various application areas such as information and communication, lighting, and photovoltaics. In many current and future photonic devices, surfaces of a semiconductor crystal are a weak part causing significant photo-electric losses and malfunctions in applications. These surface challenges, many of which arise from material defects at semiconductor surfaces, include signal attenuation in waveguides, light absorption in light emitting diodes, non-radiative recombination of carriers in solar cells, leakage (dark) current of photodiodes, and light reflection at solar cell interfaces for instance. To reduce harmful surface effects, the optical and electrical passivation of devices has been developed for several decades, especially with the methods of semiconductor technology. Because atomic scale control and knowledge of surface-related phenomena have become relevant to increase the performance of different devices, it might be useful to enhance the bridging of surface physics to photonics. Toward that target, we review some evolving research subjects with open questions and possible solutions, which hopefully provide example connecting points between photonic device passivation and surface physics. One question is related to the properties of the wet chemically cleaned semiconductor surfaces which are typically utilized in device manufacturing processes, but which appear to be different from crystalline surfaces studied in ultrahigh vacuum by physicists. In devices, a defective semiconductor surface often lies at an embedded interface formed by a thin metal or insulator film grown on the semiconductor crystal, which makes the measurements of its atomic and electronic structures difficult. To understand these interface properties, it is essential to combine quantum mechanical simulation methods. This review also covers metal-semiconductor interfaces which are included in most photonic devices to transmit electric carriers to the semiconductor structure. Low-resistive and passivated contacts with an ultrathin tunneling barrier are an emergent solution to control electrical losses in photonic devices.

在信息与通信、照明和光伏等各种应用领域,光子设备的使用和性能标准不断提高。在许多当前和未来的光子设备中,半导体晶体表面是一个薄弱环节,会造成严重的光电损耗和应用故障。这些表面难题很多是由半导体表面的材料缺陷引起的,例如波导中的信号衰减、发光二极管中的光吸收、太阳能电池中载流子的非辐射重组、光电二极管的漏(暗)电流以及太阳能电池界面的光反射等。为了减少有害的表面效应,设备的光学和电学钝化技术已经发展了几十年,尤其是在半导体技术方面。由于原子尺度的控制和对表面相关现象的了解与提高不同设备的性能息息相关,因此加强表面物理学与光子学的衔接可能会有所帮助。为了实现这一目标,我们回顾了一些不断发展的研究课题,并提出了一些开放性问题和可能的解决方案,希望能为光子设备钝化与表面物理之间的联系提供一些实例。其中一个问题与湿化学清洗半导体表面的特性有关,半导体表面通常用于设备制造工艺中,但似乎与物理学家在超高真空中研究的晶体表面不同。在设备中,有缺陷的半导体表面通常位于由半导体晶体上生长的金属薄膜或绝缘体薄膜形成的嵌入式界面上,这就给测量其原子和电子结构带来了困难。要了解这些界面特性,必须结合量子力学模拟方法。本综述还涉及金属-半导体界面,这些界面包含在大多数光子设备中,用于向半导体结构传输载流子。具有超薄隧穿势垒的低电阻和钝化接触是控制光子设备电损耗的新兴解决方案。
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引用次数: 0
Coherent light scattering from cellular dynamics in living tissues. 活体组织中细胞动态的相干光散射。
Pub Date : 2024-03-04 DOI: 10.1088/1361-6633/ad2229
David D Nolte

This review examines the biological physics of intracellular transport probed by the coherent optics of dynamic light scattering from optically thick living tissues. Cells and their constituents are in constant motion, composed of a broad range of speeds spanning many orders of magnitude that reflect the wide array of functions and mechanisms that maintain cellular health. From the organelle scale of tens of nanometers and upward in size, the motion inside living tissue is actively driven rather than thermal, propelled by the hydrolysis of bioenergetic molecules and the forces of molecular motors. Active transport can mimic the random walks of thermal Brownian motion, but mean-squared displacements are far from thermal equilibrium and can display anomalous diffusion through Lévy or fractional Brownian walks. Despite the average isotropic three-dimensional environment of cells and tissues, active cellular or intracellular transport of single light-scattering objects is often pseudo-one-dimensional, for instance as organelle displacement persists along cytoskeletal tracks or as membranes displace along the normal to cell surfaces, albeit isotropically oriented in three dimensions. Coherent light scattering is a natural tool to characterize such tissue dynamics because persistent directed transport induces Doppler shifts in the scattered light. The many frequency-shifted partial waves from the complex and dynamic media interfere to produce dynamic speckle that reveals tissue-scale processes through speckle contrast imaging and fluctuation spectroscopy. Low-coherence interferometry, dynamic optical coherence tomography, diffusing-wave spectroscopy, diffuse-correlation spectroscopy, differential dynamic microscopy and digital holography offer coherent detection methods that shed light on intracellular processes. In health-care applications, altered states of cellular health and disease display altered cellular motions that imprint on the statistical fluctuations of the scattered light. For instance, the efficacy of medical therapeutics can be monitored by measuring the changes they induce in the Doppler spectra of livingex vivocancer biopsies.

这篇综述探讨了通过光学厚活组织动态光散射的相干光学探测细胞内运输的生物物理学。细胞及其成分处于持续运动中,由跨越多个数量级的各种速度组成,反映了维持细胞健康的各种功能和机制。从数十纳米大小的细胞器开始,活体组织内部的运动是由生物能分子的水解作用和分子马达的作用力主动驱动的,而不是热驱动的。主动运输可模仿热布朗运动的随机行走,但平均位移远离热平衡,并可通过莱维或分数布朗行走显示异常扩散。尽管细胞和组织具有平均各向同性的三维环境,但单个光散射物体在细胞或细胞内的主动传输往往是伪一维的,例如,细胞器沿着细胞骨架轨道持续位移,或者细胞膜沿着细胞表面的法线位移,尽管在三维空间中是各向同性的。相干光散射是表征此类组织动力学的天然工具,因为持续的定向传输会引起散射光的多普勒频移。来自复杂动态介质的许多频移偏波相互干扰,产生动态斑点,通过斑点对比成像和波动光谱学揭示组织尺度过程。低相干干涉仪、动态光学相干断层扫描、扩散波光谱学、扩散相关光谱学、差分动态显微镜和数字全息技术提供的相干检测方法可揭示细胞内的过程。在医疗保健应用中,细胞健康和疾病状态的改变会显示出细胞运动的改变,而这些改变会影响散射光的统计波动。例如,可以通过测量活体癌症活检组织的多普勒光谱变化来监测医疗疗法的疗效。
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引用次数: 0
Nucleon-nucleon correlations inside atomic nuclei: synergies, observations and theoretical models. 原子核内的核子-核子相关性:协同、观测和理论模型。
Pub Date : 2024-02-29 DOI: 10.1088/1361-6633/ad27dd
Ranjeet Dalal, I J Douglas MacGregor

While the main features of atomic nuclei are well described by nuclear mean-field models, there is a large and growing body of evidence which indicates an important additional role played by spatially-correlated nucleon-nucleon structures. The role of nucleonic structures was first suggested by Heidmann in 1950 to explain the pick-up reactions of energetic nucleons. Since then, a steady flux of new experimental evidence has confirmed the presence of similar structures inside atomic nuclei, dominated by correlations between pairs of nucleons. The role of these internal nucleon-nucleon correlations has been established using various energetic probes like photons, pions, leptons and hadrons. These correlated structures are essential for understanding the interaction of particles with nuclei and their presence provides an explanation of many specific nuclear phenomena, including backscattered protons, copious deuteron production, sub-threshold particle production, neutrino interactions with nuclei and the European Muon Collaboration effect. On the theoretical side, these measurements have stimulated a large number of phenomenological models specifically devised to address these enigmatic observations. While reviews exist for specific interactions, there is currently no published commentary which systematically encompasses the wide range of experimental signatures and theoretical frameworks developed thus far. The present review draws together the synergies between a wide range of different experimental and theoretical studies, summarizes progress in this area and highlights outstanding issues for further study.

虽然原子核的主要特征可以用核平均场模型很好地描述,但大量且越来越多的证据表明,空间相关的核子-核子结构还发挥着重要作用。核子结构的作用最早是由海德曼于 1950 年提出的,用来解释高能核子的拾取反应。从那时起,不断涌现的新实验证据证实了原子核内部存在类似的结构,主要是核子对之间的相关性。利用光子、小离子、轻子和强子等各种高能探针,这些内部核子-核子关联的作用已经得到证实。这些相关结构对于理解粒子与原子核的相互作用至关重要,它们的存在为许多特定的核现象提供了解释,包括质子后向散射、大量氘核产生、亚阈值粒子产生、中微子与原子核的相互作用以及 EMC 效应。在理论方面,这些测量结果激发了大量的现象学模型,这些模型是专门针对这些神秘的观测结果而设计的。虽然已有针对特定相互作用的综述,但目前还没有发表系统地涵盖迄今为止广泛的实验特征和理论框架的评论。本评论汇集了大量不同实验和理论研究之间的协同作用,总结了这一领域的进展,并强调了有待进一步研究的未决问题。
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引用次数: 0
HoloTile light engine: new digital holographic modalities and applications. HoloTile 光引擎:新的数字全息模式和应用。
Pub Date : 2024-02-28 DOI: 10.1088/1361-6633/ad2aca
Jesper Glückstad, Andreas Erik Gejl Madsen

HoloTile is a patented computer generated holography approach with the aim of reducing the speckle noise caused by the overlap of the non-trivial physical extent of the point spread function in Fourier holographic systems from adjacent frequency components. By combining tiling of phase-only of rapidly generated sub-holograms with a PSF-shaping phase profile, each frequency component-or output 'pixel'- in the Fourier domain is shaped to a desired non-overlapping profile. In this paper, we show the high-resolution, speckle-reduced reconstructions that can be achieved with HoloTile, as well as present new HoloTile modalities, including an expanded list of PSF options with new key properties. In addition, we discuss numerous applications for which HoloTile, its rapid hologram generation, and the new PSF options may be an ideal fit, including optical trapping and manipulation of particles, volumetric additive printing, information transfer and quantum communication.

HoloTile 是一种已获专利的计算机生成全息方法,旨在减少傅里叶全息系统中相邻频率分量的点扩散函数非三维物理范围重叠所产生的斑点噪声。通过将快速生成的子全息图的纯相位平铺与 PSF 成型相位轮廓相结合,傅里叶域中的每个频率分量(或输出 "像素")都被成型为所需的非重叠轮廓。在本文中,我们展示了利用 HoloTile 可以实现的高分辨率、减少斑点的重建,并介绍了新的 HoloTile 模式,包括具有新关键特性的 PSF 扩展选项列表。此外,我们还讨论了 HoloTile、其快速全息图生成和新的 PSF 选项可能非常适合的众多应用,包括粒子的光学捕获和操纵、体积添加印刷、信息传输和量子通信。
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引用次数: 0
Further understanding the interaction between dark energy and dark matter: current status and future directions. 进一步了解暗能量与暗物质之间的相互作用:现状与未来方向。
Pub Date : 2024-02-23 DOI: 10.1088/1361-6633/ad2527
B Wang, E Abdalla, F Atrio-Barandela, D Pavón

The interaction between dark matter and dark energy (DE) can be incorporated into field theory models of DE that have proved successful in alleviating the coincidence problem. We review recent advances in this field, including new models and constraints from different astronomical data sets. We show that interactions are allowed by observations and can reduce the current tensions among different measurements of cosmological parameters. We extend our discussion to include constraints from non-linear effects and results from cosmological simulations. Finally, we discuss forthcoming multi-messenger data from current and future observational facilities that will help to improve our understanding of the interactions within the dark sector.

暗物质和暗能量之间的相互作用可以被纳入暗能量场论模型,这些模型已被证明成功地缓解了巧合问题。我们回顾了这一领域的最新进展,包括新模型和来自不同天文数据集的约束。我们表明,观测结果允许相互作用,并能缓解当前不同宇宙学参数测量之间的紧张关系。我们将讨论范围扩大到非线性效应的约束和宇宙逻辑模拟的结果。最后,我们讨论了即将从当前和未来的观测设施中获得的多信使数据,这些数据将有助于提高我们对暗区内部相互作用的理解。
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引用次数: 0
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