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Interatomic and intermolecular decay processes in quantum fluid clusters. 量子流体团簇中的原子间和分子间衰变过程。
Pub Date : 2024-11-19 DOI: 10.1088/1361-6633/ad8fbb
A C LaForge, L Ben Ltaief, S R Krishnan, N Sisourat, M Mudrich

In this comprehensive review, we explore interatomic and intermolecular correlated electronic decay phenomena observed in superfluid helium nanodroplets subjected to extreme ultraviolet radiation. Helium nanodroplets, known for their distinctive electronic and quantum fluid properties, provide an ideal environment for examining a variety of non-local electronic decay processes involving the transfer of energy, charge, or both between neighboring sites and resulting in ionization and the emission of low-kinetic energy electrons. Key processes include interatomic or intermolecular Coulombic decay and its variants, such as electron transfer-mediated decay. Insights gained from studying these light-matter interactions in helium nanodroplets enhance our understanding of the effects of ionizing radiation on other condensed-phase systems, including biological matter. We also emphasize the advanced experimental and computational techniques that make it possible to resolve electronic decay processes with high spectral and temporal precision. Utilizing ultrashort pulses from free-electron lasers, the temporal evolution of these processes can be followed, significantly advancing our comprehension of the dynamics within quantum fluid clusters and non-local electronic interactions in nanoscale systems.

在这篇综述中,我们探讨了在受到极紫外线(XUV)辐射的超流体氦纳米液滴中观察到的原子间和分子间相关电子衰变现象。氦纳米液滴以其独特的电子和量子流体特性而闻名,为研究各种非局部电子衰变过程提供了理想的环境,这些过程涉及相邻位点之间的能量、电荷或两者的转移,并导致电离和低动能电子的发射。主要过程包括原子间或分子间库仑衰变(ICD)及其变体,如电子转移介导的衰变(ETMD)。通过研究氦纳米微滴中的这些光物质相互作用,我们可以加深对电离辐射对其他凝聚相系统(包括生物物质)影响的理解。我们还强调了先进的实验和计算技术,这些技术使得高光谱和高时间精度地解析电子衰变过程成为可能。利用自由电子激光器发出的超短脉冲,可以跟踪这些过程的时间演变,极大地推动了我们对量子流体团簇内部动力学和纳米尺度系统中非局部电子相互作用的理解。
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引用次数: 0
Superscattering of light: fundamentals and applications. 光的超散射:基础与应用。
Pub Date : 2024-11-18 DOI: 10.1088/1361-6633/ad8eda
Chan Wang, Xuhuinan Chen, Zheng Gong, Ruoxi Chen, Hao Hu, Huaping Wang, Yi Yang, Low Tony, Baile Zhang, Hongsheng Chen, Xiao Lin

Superscattering, theoretically predicted in 2010 and experimentally observed in 2019, is an exotic scattering phenomenon of light from subwavelength nanostructures. In principle, superscattering allows for an arbitrarily large total scattering cross section, due to the degenerate resonance of eigenmodes or channels. Consequently, the total scattering cross section of a superscatterer can be significantly enhanced, far exceeding the so-called single-channel limit. Superscattering offers a unique avenue for enhancing light-matter interactions and can enable numerous practical applications, ranging from sensing, light trapping, bioimaging, and communications to optoelectronics. This paper provides a comprehensive review of the recent progress and developments in the superscattering of light, with a specific focus on elucidating its theoretical origins, experimental observations, and manipulations. Moreover, we offer an outlook on future research directions in superscattering, including potential realizations of directional superscattering, scattering-free plasmonic superscattering, enhancement of free-electron radiation and the Purcell effect via superscatterers, inelastic superscattering, and superscattering of non-electromagnetic waves.

超散射是亚波长纳米结构对光的一种奇特散射现象,2010 年进行了理论预测,2019 年进行了实验观测。从原理上讲,超散射可以产生任意大的总散射截面,这是由于特征模式或通道的退化共振所致。因此,超散射器的总散射截面可以显著增强,远远超过所谓的单通道极限。超散射为增强光与物质的相互作用提供了一条独特的途径,并可实现从传感、光捕获、生物成像、通信到光电子学等众多实际应用。本文全面回顾了光的超散射方面的最新进展和发展,重点阐述了其理论起源、实验观察和操作方法。此外,我们还展望了超散射的未来研究方向,包括定向超散射的潜在实现、无散射质子超散射、通过超散射体增强自由电子辐射和珀塞尔效应、非弹性超散射以及非电磁波的超散射。
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引用次数: 0
Topological phase transitions via attosecond x-ray absorption spectroscopy. 通过阿秒 X 射线吸收光谱实现拓扑相变。
Pub Date : 2024-10-29 DOI: 10.1088/1361-6633/ad889f
Juan F P Mosquera, Giovanni Cistaro, Mikhail Malakhov, Emilio Pisanty, Alexandre Dauphin, Luis Plaja, Alexis Chacón, Maciej Lewenstein, Antonio Picón

We present a numerical experiment that demonstrates the possibility to capture topological phase transitions via an x-ray absorption spectroscopy scheme. We consider a Chern insulator whose topological phase is tuned via a second-order hopping. We perform time-dynamics simulations of the out-of-equilibrium laser-driven electron motion that enables us to model a realistic attosecond spectroscopy scheme. In particular, we use an ultrafast scheme with a circularly polarized IR pump pulse and an attosecond x-ray probe pulse. A laser-induced dichroism-type spectrum shows a clear signature of the topological phase transition. We are able to connect these signatures with the Berry structure of the system. This work extend the applications of attosecond absorption spectroscopy to systems presenting a non-trivial topological phase.

我们提出了一个数值实验,证明了通过 X 射线吸收光谱方案捕捉拓扑相变的可能性。我们考虑了一个通过二阶跳变调整拓扑相位的切尔绝缘体。我们对失衡激光驱动的电子运动进行了时间动力学模拟,从而建立了一个现实的阿秒光谱方案模型。特别是,我们使用了一种具有圆偏振红外泵浦脉冲和阿秒 x 射线探针脉冲的超快方案。激光诱导的二色性光谱显示了拓扑相变的明显特征。我们能够将这些特征与系统的贝里结构联系起来。这项工作将阿秒吸收光谱的应用扩展到了呈现非三维拓扑相位的系统。
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引用次数: 0
Quantum algorithms for scientific computing. 科学计算的量子算法。
Pub Date : 2024-10-29 DOI: 10.1088/1361-6633/ad85f0
R Au-Yeung, B Camino, O Rathore, V Kendon

Quantum computing promises to provide the next step up in computational power for diverse application areas. In this review, we examine the science behind the quantum hype, and the breakthroughs required to achieve true quantum advantage in real world applications. Areas that are likely to have the greatest impact on high performance computing (HPC) include simulation of quantum systems, optimization, and machine learning. We draw our examples from electronic structure calculations and computational fluid dynamics which account for a large fraction of current scientific and engineering use of HPC. Potential challenges include encoding and decoding classical data for quantum devices, and mismatched clock speeds between classical and quantum processors. Even a modest quantum enhancement to current classical techniques would have far-reaching impacts in areas such as weather forecasting, aerospace engineering, and the design of 'green' materials for sustainable development. This requires significant effort from the computational science, engineering and quantum computing communities working together.

量子计算有望为各种应用领域提供更强的计算能力。在这篇综述中,我们将研究量子炒作背后的科学,以及在现实应用中实现真正量子优势所需的突破。可能对高性能计算(HPC)产生最大影响的领域包括量子系统模拟、优化和机器学习。我们以电子结构计算和计算流体力学为例,这两个领域在当前科学和工程领域对高性能计算的使用中占有很大比例。潜在的挑战包括为量子设备编码和解码经典数据,以及经典和量子处理器之间不匹配的时钟速度。即使对当前的经典技术进行适度的量子改进,也会在天气预报、工程、航空航天、药物设计以及可持续发展的 "绿色 "材料设计等领域产生深远影响。这需要计算科学界、工程界和量子计算界共同努力。
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引用次数: 0
Observation of quantum entanglement in top quark pair production in proton-proton collisions ats=13 TeV. 在 √s = 13 TeV 的质子-质子对撞中观测到顶夸克对产生的量子纠缠。
Pub Date : 2024-10-23 DOI: 10.1088/1361-6633/ad7e4d
The Cms Collaboration

Entanglement is an intrinsic property of quantum mechanics and is predicted to be exhibited in the particles produced at the Large Hadron Collider. A measurement of the extent of entanglement in top quark-antiquark (tt¯) events produced in proton-proton collisions at a center-of-mass energy of 13 TeV is performed with the data recorded by the CMS experiment at the CERN LHC in 2016, and corresponding to an integrated luminosity of 36.3 fb-1. The events are selected based on the presence of two leptons with opposite charges and high transverse momentum. An entanglement-sensitive observableDis derived from the top quark spin-dependent parts of thett¯production density matrix and measured in the region of thett¯production threshold. Values ofD<-1/3are evidence of entanglement andDis observed (expected) to be-0.480-0.029+0.026(-0.467-0.029+0.026) at the parton level. With an observed significance of 5.1 standard deviations with respect to the non-entangled hypothesis, this provides observation of quantum mechanical entanglement withintt¯pairs in this phase space. This measurement provides a new probe of quantum mechanics at the highest energies ever produced.

纠缠是量子力学的固有特性,据预测在大型强子对撞机产生的粒子中也会表现出这种特性。我们利用欧洲核子研究中心大型强子对撞机的CMS实验在2016年记录的数据,测量了在质心能量为13 TeV的质子-质子对撞中产生的顶夸克-反夸克($mathrm{tbar{t}}$)事件中的纠缠程度,对应的综合光度为36.3 fb$^{-1}$。这些事件是根据存在两个带相反电荷和高横向动量的轻子来选择的。从 $mathrm{tbar{t}}$ 产生密度矩阵的顶夸克自旋相关部分导出了纠缠敏感观测值 $D$,并在 $mathrm{tbar{t}}$ 产生阈值区域进行了测量。$Dlt-$1/3的值是纠缠的证据,在粒子水平上,$D$被观测到(预期)为$-$0.480$^{+0.026}_{-0.029}$($-$0.467$^{+0.026}_{-0.029}$)。与非纠缠假说相比,观察到的显著性为 5.1 个标准偏差,这就提供了在这个相空间的 $mathrm{tbar{t}}$ 对中对量子力学纠缠的观察。这一测量为量子力学在迄今为止最高能量下的发展提供了新的探针。
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引用次数: 0
Continuously tunable single-photon level nonlinearity with Rydberg state wave-function engineering. 利用雷德贝格态波函数工程实现连续可调的单光子级非线性。
Pub Date : 2024-10-23 DOI: 10.1088/1361-6633/ad847e
Biao Xu, Gen-Sheng Ye, Yue Chang, Tao Shi, Lin Li

Extending optical nonlinearity into the extremely weak light regime is at the heart of quantum optics, since it enables the efficient generation of photonic entanglement and implementation of photonic quantum logic gate. Here, we demonstrate the capability for continuously tunable single-photon level nonlinearity, enabled by precise control of Rydberg interaction over two orders of magnitude, through the use of microwave-assisted wave-function engineering. To characterize this nonlinearity, light storage and retrieval protocol utilizing Rydberg electromagnetically induced transparency is employed, and the quantum statistics of the retrieved photons are analyzed. As a first application, we demonstrate our protocol can speed up the preparation of single photons in low-lying Rydberg states by a factor of up to∼40. Our work holds the potential to accelerate quantum operations and to improve the circuit depth and connectivity in Rydberg systems, representing a crucial step towards scalable quantum information processing with Rydberg atoms.

将光学非线性扩展到极微弱的光环境是量子光学的核心,因为它能有效地产生光子纠缠和实现光子量子逻辑门。在这里,我们展示了连续可调单光子级非线性的能力,通过使用微波辅助波函数工程,精确控制雷德堡相互作用超过两个数量级。为了描述这种非线性,我们采用了利用雷德贝格电磁诱导透明度的光存储和检索协议,并对检索光子的量子统计进行了分析。作为首次应用,我们展示了我们的协议可以将低洼雷德贝格态单光子的制备速度提高约 40 倍。我们的工作有望加速量子操作,并改善雷德贝格系统中的电路深度和连通性,这是用雷德贝格原子实现可扩展量子信息处理的关键一步。
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引用次数: 0
Expressibility-induced Concentration of Quantum Neural Tangent Kernels. 量子神经切线核的可表达性诱导浓度。
Pub Date : 2024-10-03 DOI: 10.1088/1361-6633/ad82cf
Li-Wei Yu, Weikang Li, Qi Ye, Zhide Lu, Zizhao Han, Dong-Ling Deng

Quantum tangent kernel methods provide an efficient approach to analyzing the performance of quantum machine learning models in the infinite-width limit, which is of crucial importance in designing appropriate circuit architectures for certain learning tasks. Recently, they have been adapted to describe the convergence rate of training errors in quantum neural networks in an analytical manner. Here, we study the connections between the expressibility and value concentration of quantum tangent kernel models. In particular, for global loss functions, we rigorously prove that high expressibility of both the global and local quantum encodings can lead to exponential concentration of quantum tangent kernel values to zero. Whereas for local loss functions, such issue of exponential concentration persists owing to the high expressibility, but can be partially mitigated. We further carry out extensive numerical simulations to support our analytical theories. Our discoveries unveil a fundamental feature of quantum neural tangent kernels, indicating that the issue of their concentration cannot be bypassed merely by transitioning to a local encoding scheme while maintaining high expressibility. This offers valuable insights for the design of wide quantum variational circuit models in practical applications.

量子切核方法为分析量子机器学习模型在无限宽极限下的性能提供了一种有效方法,这对于为某些学习任务设计适当的电路架构至关重要。最近,这些方法被用于分析描述量子神经网络中训练误差的收敛速率。在这里,我们研究了量子切核模型的可表达性和值集中之间的联系。特别是,对于全局损失函数,我们严格证明了全局和局部量子编码的高可表达性会导致量子正切核值以指数形式集中为零。而对于局部损失函数,由于可表达性高,指数集中的问题依然存在,但可以得到部分缓解。我们进一步进行了大量的数值模拟,以支持我们的分析理论。我们的发现揭示了量子神经切核的一个基本特征,表明在保持高可表达性的同时,仅仅过渡到局部编码方案无法绕过其集中问题。这为在实际应用中设计宽量子变分电路模型提供了宝贵的启示。
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引用次数: 0
Exact results of the one-dimensional repulsive Hubbard model. 一维斥力哈伯德模型的精确结果
Pub Date : 2024-10-03 DOI: 10.1088/1361-6633/ad7b70
Jia-Jia Luo, Han Pu, Xi-Wen Guan

We present analytical results of the fundamental properties of the one-dimensional (1D) Hubbard model with a repulsive interaction. The new model results with arbitrary external fields include: (I) using the exact solutions of the Bethe ansatz equations of the Hubbard model, we first rigorously calculate the gapless spin and charge excitations, exhibiting exotic features of fractionalized spinons and holons. We then investigate the gapped excitations in terms of the spin string and thek-Λstring bound states at arbitrary driving fields, showing subtle differences in spin magnons and chargeη-pair excitations. (II) For a high-density and high spin magnetization region, i.e. near the quadruple critical point, we further analytically obtain the thermodynamic properties, dimensionless ratios and scaling functions near quantum phase transitions. (III) Importantly, we give the general scaling functions at quantum criticality for arbitrary filling and interaction strength. These can directly apply to other integrable models. (IV) Based on the fractional excitations and the scaling laws, the spin-incoherent Luttinger liquid (SILL) with only the charge propagation mode is elucidated by the asymptotic of the two-point correlation functions with the help of conformal field theory. We also, for the first time, obtain the analytical results of the thermodynamics for the SILL. (V) Finally, to capture deeper insights into the Mott insulator and interaction-driven criticality, we further study the double occupancy and propose its associated contact and contact susceptibilities, through which an adiabatic cooling scheme based upon quantum criticality is proposed. In this scenario, we build up general relations among arbitrary external- and internal-potential-driven quantum phase transitions, providing a comprehensive understanding of quantum criticality. Our methods offer rich perspectives of quantum integrability and offer promising guidance for future experiments with interacting electrons and ultracold atoms, both with and without a lattice.

我们提出了具有斥力相互作用的一维(1D)哈伯德模型基本性质的分析结果。 该模型在任意外场下的新结果包括: I)利用哈伯德模型贝特安萨特方程的精确解,我们首先严格计算了无间隙自旋和电荷激发,展示了分数化自旋子和全子的奇异特征。然后,我们研究了任意驱动场下自旋弦和 $k-Lambda$ 弦束缚态的间隙激发,显示了自旋磁子和电荷 $eta$ 对激发的微妙差异。III)重要的是,我们给出了任意填充 和相互作用强度下量子临界点的一般缩放函数。这些可以直接应用于其他可积分模型。 IV) 基于分数激元和缩放定律,在共形场理论的帮助下,通过两点相关函数的渐近,阐明了只有电荷传播模式的自旋相干鲁丁格液体(SILL)。最后,为了更深入地了解莫特绝缘体和相互作用驱动临界,我们进一步研究了双占位,并提出了与之相关的接触和接触感性,从而提出了基于量子临界的绝热冷却方案。在这种情况下,我们建立了任意外部和内部势驱动量子相变之间的一般关系,提供了对量子临界的全面理解。我们的方法为量子可集成性提供了丰富的视角,并为未来有晶格和无晶格的相互作用电子和超冷原子实验提供了有前途的指导。
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引用次数: 0
70 years of hyperon spectroscopy: a review of strange Ξ, Ω baryons, and the spectrum of charmed and bottom baryons. 超重子光谱学 70 年:奇异Ξ重子、Ω重子以及粲重子和底重子的光谱回顾。
Pub Date : 2024-09-30 DOI: 10.1088/1361-6633/ad7610
Volker Crede, John Yelton

The first hyperon was discovered about 70 years ago, but the nature of these particles, particularly with regard to multistrange hyperons, and many of their properties can still be considered to be literally strange. A dedicated and successful global spectroscopy program in the 1960s and 1970s usingK-beams revealed many multistrange candidates, but the available evidence of their existence is statistically limited. For this reason, there is still much to learn about the systematics of the spectrum of excited hyperon states and what they have in common with their non-strange companions, or how they differ from the nucleon and Δ resonances. Results from photo- and electroproduction experiments off the proton and neutron using polarized beams and targets have provided intriguing evidence for new nucleon excitations and shed light on the structure of some of the known nucleon and Δ states. Recent years have also seen a great deal of progress in the field of charmed and bottom baryon spectroscopy. Unprecedented data from the Large Hadron Collider in particular indicate continued rapid progress in the field of bottom baryons. On the theoretical side, baryons with one heavy quarkQand a lightqqsystem serve as an ideal laboratory for studying lightqq(diquark) correlations and the dynamics of the light quarks in the colour environment of a heavy quark. In this review, we discuss the status of doubly and triply strange Ξ as well as Ω baryons, and the properties of all the known charmed and bottom states. The comparison of the two heavy sectors reveals many similarities as predicted by heavy-quark symmetries, together with differences in mass splittings easily understood by potential models. The multi-strange hyperons bridge the under-explored gap between the light- and the heavy-flavour baryons. How do the properties of a singly charmedQ-qqsystem change with decreasing mass of the heavy quark in the transition to a doubly strangeq-QQsystem with a heavier quark-quark system relative to one light quark? Significant progress towards understanding hyperon resonances is expected in coming years from the ongoing experiments at the high-energy collider facilities and planned experiments usingKbeams at Jefferson Laboratory and J-PARC.

第一个超子是在大约 70 年前被发现的,但这些粒子的性质,特别是多量程超子,以及它们的许多特性仍然可以被认为是非常奇怪的。20 世纪 60 年代和 70 年代,利用 K 光束开展的一项专门的全球光谱计划取得了成功,发现了许多多量程候选粒子,但从统计学角度来看,证明它们存在的现有证据非常有限。因此,关于激发超子态光谱的系统性,它们与非超子态的共同点,或者它们与核子和Δ共振的区别,还有很多东西需要了解。利用偏振光束和靶子对质子和中子进行的光子和电子产生实验的结果为新的核子激发态提供了引人入胜的证据,并揭示了一些已知核子和Δ态的结构。近年来,粲重子和底重子光谱学领域也取得了巨大进展。特别是来自大型强子对撞机的前所未有的数据表明,底重子领域继续取得快速进展。在理论方面,具有一个重夸克 Q 和一个轻 qq 系统的重子是研究轻 qq(二夸克)相关性和轻夸克在重夸克颜色环境中的动力学的理想实验室。在这篇综述中,我们讨论了双奇异Ξ和三奇异Ξ以及Ω重子的现状,以及所有已知粲态和底态的性质。通过对这两个重部门的比较,我们发现了重夸克对称性所预言的许多相似之处,以及潜在模型容易理解的质量分裂差异。多量程超子弥补了轻重子之间探索不足的差距。在过渡到双奇异q-QQ系统(相对于一个轻夸克,夸克-夸克系统更重)的过程中,单粲Q-qq系统的性质如何随着重夸克质量的降低而变化?高能对撞机设施正在进行的实验以及计划在杰斐逊实验室和 J-PARC 使用 K 波束进行的实验预计将在未来几年里为了解超子共振取得重大进展。
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引用次数: 0
Continuous gated first-passage processes. 连续的门控第一通道流程。
Pub Date : 2024-09-19 DOI: 10.1088/1361-6633/ad7530
Yuval Scher, Aanjaneya Kumar, M S Santhanam, Shlomi Reuveni

Gated first-passage processes, where completion depends on both hitting a target and satisfying additional constraints, are prevalent across various fields. Despite their significance, analytical solutions to basic problems remain unknown, e.g. the detection time of a diffusing particle by a gated interval, disk, or sphere. In this paper, we elucidate the challenges posed by continuous gated first-passage processes and present a renewal framework to overcome them. This framework offers a unified approach for a wide range of problems, including those with single-point, half-line, and interval targets. The latter have so far evaded exact solutions. Our analysis reveals that solutions to gated problems can be obtained directly from the ungated dynamics. This, in turn, reveals universal properties and asymptotic behaviors, shedding light on cryptic intermediate-time regimes and refining the notion of high-crypticity for continuous-space gated processes. Moreover, we extend our formalism to higher dimensions, showcasing its versatility and applicability. Overall, this work provides valuable insights into the dynamics of continuous gated first-passage processes and offers analytical tools for studying them across diverse domains.

门控第一通过过程的完成取决于撞击目标和满足其他约束条件,这种过程在各个领域都很普遍。尽管其重要性不言而喻,但基本问题的分析解决方案仍是未知数,例如扩散粒子被门控区间、圆盘或球体检测到的时间。在本文中,我们阐明了连续门控首次通过过程所带来的挑战,并提出了克服这些挑战的更新框架。该框架为包括单点、半线和区间目标在内的各种问题提供了统一的方法。迄今为止,后者一直无法精确求解。我们的分析表明,门控问题的解决方案可以直接从非门控动力学中获得。这反过来又揭示了普遍特性和渐近行为,揭示了隐秘的中间时态,并重新定义了连续空间门控过程的高隐秘性概念。此外,我们还将我们的形式主义扩展到了更高的维度,展示了它的多功能性和适用性。总之,这项工作为连续门控第一通道过程的动力学提供了宝贵的见解,并为在不同领域研究它们提供了分析工具。
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引用次数: 0
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