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Performance of an Open-Source Image-Based History Matching Framework for CO(_2) Storage CO (_2)存储中基于开源图像的历史匹配框架的性能研究
IF 2.6 3区 工程技术 Q3 ENGINEERING, CHEMICAL Pub Date : 2026-01-07 DOI: 10.1007/s11242-025-02275-0
David Landa-Marbán, Tor H. Sandve, Jakub W. Both, Jan M. Nordbotten, Sarah E. Gasda

We present a history matching (HM) workflow applied to the International FluidFlower benchmark study dataset, which features high-resolution images of CO(_2) storage in a meter-scale, geologically complex reservoir. The dataset provides dense spatial and temporal observations of fluid displacement, offering a rare opportunity to validate and enhance HM techniques for geological carbon storage (GCS). The combination of detailed experimental data and direct visual observation of flow behavior at this scale is novel and valuable. This study explores the potential and limitations of using experimental data to calibrate standard models for GCS simulation. By leveraging high-resolution images and resulting interpretations of fluid phase distributions, we adjust uncertain parameters and reduce the mismatch between simulation results and observed data. Simulations are performed using the open-source OPM Flow simulator, while the open-source Everest decision-making tool is employed to conduct the HM. After the HM process, the final simulation results show good agreement with the experimental CO(_2) storage data. This suggests that the system can be effectively described using standard flow equations, conventional saturation functions, and typical PVT properties for CO(_2)–brine mixtures. Our results demonstrate that the Wasserstein distance is a particularly effective metric for matching multi-phase, multi-component flow data. The entire workflow is implemented in a Python package named pofff (Python OPM Flow FluidFlower), which organizes all functionality through a single input file. This design ensures reproducibility and facilitates future extensions of the study.

我们提出了一种历史匹配(HM)工作流程,应用于国际FluidFlower基准研究数据集,该数据集具有高分辨率图像,可以在米尺度、地质复杂的储层中存储CO (_2)。该数据集提供了流体位移的密集时空观测,为验证和增强地质碳储存(GCS)的HM技术提供了难得的机会。详细的实验数据和在这种尺度下流动行为的直接视觉观察相结合是新颖而有价值的。本研究探讨了使用实验数据校准GCS模拟标准模型的潜力和局限性。通过利用高分辨率图像和对流体相分布的解释,我们调整了不确定的参数,减少了模拟结果与观测数据之间的不匹配。仿真使用开源的OPM Flow模拟器进行,同时使用开源的Everest决策工具进行HM。经过HM处理后,最终的模拟结果与实验CO (_2)存储数据吻合较好。这表明,该体系可以使用标准流动方程、常规饱和度函数和CO (_2) -盐水混合物的典型PVT特性来有效描述。我们的结果表明,Wasserstein距离是匹配多相、多组分流动数据的一个特别有效的度量。整个工作流是在一个名为pofff (Python OPM Flow FluidFlower)的Python包中实现的,它通过一个输入文件组织所有功能。这种设计确保了再现性,并有利于未来研究的扩展。
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引用次数: 0
On the Stability of Foam Displacement Simulations in Porous Media 多孔介质中泡沫位移模拟的稳定性研究
IF 2.6 3区 工程技术 Q3 ENGINEERING, CHEMICAL Pub Date : 2026-01-07 DOI: 10.1007/s11242-025-02277-y
P. Z. S. Paz, F. A. N. Obiang, F. F. de Paula, G. Chapiro

Foam injection in porous media is a promising technique for enhanced recovery and other industrial applications, but its modeling is complicated by instabilities in the computed foam apparent viscosity. This study investigates oscillations observed during foam displacement simulations. Mesh refinement demonstrates that increasing discretization reduces the amplitude of global oscillations in the average apparent viscosity; however, sharp local peaks persist at shock fronts and may intensify over time. These instabilities are not solely numerical artifacts but are linked to the mathematical structure of the foam model, particularly the presence of steep saturation fronts. We show that numerical diffusion, unavoidable in simulation frameworks, can amplify such effects. To address this issue, we introduce a filtering technique that reconstructs the water saturation profile in the vicinity of the shock without affecting convergence. The method effectively suppresses viscosity oscillations while maintaining physical accuracy near discontinuities.

在多孔介质中注入泡沫是一种很有前途的提高采收率和其他工业应用的技术,但由于计算泡沫表观粘度的不稳定性,其建模很复杂。本研究调查了泡沫位移模拟过程中观察到的振荡。网格细化表明,离散化程度的增加降低了平均表观粘度的全局振荡幅度;然而,剧烈的局部峰值在冲击前沿持续存在,并可能随着时间的推移而加剧。这些不稳定性不仅仅是数值上的人工产物,而且与泡沫模型的数学结构有关,特别是陡峭饱和锋面的存在。我们表明,在模拟框架中不可避免的数值扩散可以放大这种影响。为了解决这个问题,我们引入了一种滤波技术,在不影响收敛的情况下重建激波附近的含水饱和度剖面。该方法有效地抑制了粘度振荡,同时保持了不连续点附近的物理精度。
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引用次数: 0
Double-diffusive convection of a vertical through flow in a saturated porous layer by a power-law fluid with effect of variable gravity 变重力作用下幂律流体在饱和多孔层中垂直直流的双扩散对流
IF 2.6 3区 工程技术 Q3 ENGINEERING, CHEMICAL Pub Date : 2026-01-07 DOI: 10.1007/s11242-025-02273-2
Ambica Kolipaka, Anjanna Matta

This study investigates the thermosolutal convection of a power-law fluid with variable gravity in a vertical through flow that is heated and salted from below. Linear instability analysis investigates the growth of small disturbances in a system. After non-dimensionalizing the governing equations, they are linearized around a base state. The normal mode method applied for solving the perturbation equations. It gives the exponential form to solve stability criteria. The complete study was analyzed by using linear stability analysis; the influence of variable gravity is studied. This theoretical study investigates double-diffusive convection within a porous media filled by power-law fluid. It mainly examines how gravity and concentration gradients influence on thermal solutal convection behavior. The focus is on vertical through flow and its role in the onset and effect of instability.

本研究研究了一种变重力幂律流体在垂直通流中从下面加热和加盐的热溶质对流。线性不稳定性分析研究的是系统中小扰动的增长。在对控制方程进行无量纲化后,它们围绕一个基本状态进行线性化。采用正态法求解微扰方程。给出了稳定性判据的指数形式。采用线性稳定性分析对整个研究进行分析;研究了重力变化的影响。本理论研究探讨了幂律流体填充多孔介质中的双扩散对流。它主要考察重力和浓度梯度对热溶质对流行为的影响。重点是垂直通流及其在不稳定的开始和影响中的作用。
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引用次数: 0
Predicting Air Flow in Calendered Paper Sheets from μ-CT Data: Combining Physics with Morphology 利用μ-CT数据预测压延纸中的气流:结合物理与形态学
IF 2.6 3区 工程技术 Q3 ENGINEERING, CHEMICAL Pub Date : 2026-01-07 DOI: 10.1007/s11242-025-02250-9
Phillip Gräfensteiner, Andoni Rodriguez, Peter Leitl, Ekaterina Baikova, Maximilian Fuchs, Eduardo Machado Charry, Ulrich Hirn, André Hilger, Ingo Manke, Robert Schennach, Matthias Neumann, Volker Schmidt, Karin Zojer

Predicting the macroscopic properties of thin fiber-based porous materials from their microscopic morphology remains challenging because of the structural heterogeneity of these materials. In this study, computational fluid dynamics simulations were performed to compute volume air flow based on tomographic image data of uncompressed and compressed paper sheets. To reduce computational demands, a pore network model was employed, allowing volume air flow to be approximated with less computational effort. To improve prediction accuracy, geometric descriptors of the pore space, such as porosity, surface area, median pore radius, and geodesic tortuosity, were combined with predictions of the pore network model. This integrated approach significantly improves the predictive power of the pore network model and indicates which aspects of the pore space morphology are not accurately represented within the pore network model. In particular, we illustrate that a high correlation among descriptors does not necessarily imply redundancy in a combined prediction.

由于纤维基多孔材料的结构不均匀性,从微观形貌预测其宏观性能仍然具有挑战性。在本研究中,基于未压缩和压缩纸张的层析成像数据,进行了计算流体动力学模拟来计算体积空气流量。为了减少计算需求,采用了孔隙网络模型,从而可以用较少的计算量来近似计算体积气流。为了提高预测精度,孔隙空间的几何描述符,如孔隙度、表面积、中位孔隙半径和测地线扭曲度,与孔隙网络模型的预测相结合。这种综合方法显著提高了孔隙网络模型的预测能力,并指出孔隙空间形态的哪些方面在孔隙网络模型中没有得到准确的表示。特别地,我们说明了描述符之间的高相关性并不一定意味着组合预测中的冗余。
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引用次数: 0
Maas (2007) Problem Revisited: Rigorous Derivation and Extension of the Elliptical Interface of Fresh Recharge Water and Upward Seeping Fresh or Saline Water Maas(2007)重新审视的问题:淡水回灌与淡水或咸水向上渗透椭圆界面的严格推导与推广
IF 2.6 3区 工程技术 Q3 ENGINEERING, CHEMICAL Pub Date : 2025-12-10 DOI: 10.1007/s11242-025-02245-6
D. van de Craats, C. J. van Duijn, P. A. C. Raats

This study revisits and extends the analytical model presented by Maas (J Hydrol 347:223–228, 2007), which describes simultaneous downward infiltration of fresh water and upward seepage of fresh or saline groundwater beneath an elongated island. Under steady-state conditions and using the sharp interface approximation, the interface between the two types of water forms a semi-elliptical shape. Notably, the unusual y-linearity of the flow potential provides an analytical advantage, enabling a direct and elegant extension from a one-phase to a two-phase system. For transient conditions, Maas (J Hydrol 347:223–228, 2007) employed a successive steady-state approach based on elliptical shapes. We demonstrate that this approach is physically inconsistent, as the tip of the lens must possess a finite derivative to allow for movement. Instead, we introduce an interface motion equation to track this front dynamically. Additionally, we identify potentially unstable configurations during outward lens migration, where denser salt water temporarily overlays fresh water near the lens tip. To address this, we incorporate diffusion, moving beyond the sharp interface assumption. Finally, we assess the applicability of Maas’s elliptical approximation for interface motion and find it remains robust as long as the approximation that lens thickness is negligible compared to its width is used with caution. These findings broaden the analytical understanding of fresh water lens dynamics in island aquifers and refine the conditions under which simplified models remain valid.

本研究重新审视并扩展了Maas (J Hydrol 347:223 - 228,2007)提出的分析模型,该模型描述了在细长岛屿下方淡水同时向下渗透和淡水或咸水同时向上渗透的情况。在稳态条件下,采用锐界面近似,两种水之间的界面形成半椭圆形状。值得注意的是,不同寻常的流势y线性提供了分析优势,使从单相系统直接扩展到两相系统成为可能。对于瞬态条件,Maas (J Hydrol 347:223 - 228,2007)采用了基于椭圆形状的连续稳态方法。我们证明这种方法在物理上是不一致的,因为透镜的尖端必须具有有限的导数以允许运动。相反,我们引入了一个界面运动方程来动态跟踪这一锋面。此外,在晶状体向外迁移过程中,我们发现了潜在的不稳定结构,其中密度较大的盐水暂时覆盖了晶状体尖端附近的淡水。为了解决这个问题,我们结合了扩散,超越了尖锐界面假设。最后,我们评估了Maas的椭圆近似对界面运动的适用性,并发现只要谨慎使用透镜厚度与宽度相比可以忽略不计的近似,它仍然是稳健的。这些发现拓宽了对岛屿含水层淡水透镜体动力学的分析理解,并改进了简化模型有效的条件。
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引用次数: 0
Revisiting Darcy–Brinkman Flow Through an Elliptic Tube 通过椭圆管重新审视达西-布林克曼流
IF 2.6 3区 工程技术 Q3 ENGINEERING, CHEMICAL Pub Date : 2025-12-07 DOI: 10.1007/s11242-025-02268-z
André Borries Lopes, Mohammad Erfan Fahim Far, Vinícius Coutinho da Silva

We revisit the classical problem of fully developed Darcy–Brinkman flow through a tube with elliptic cross section. Building upon the exact velocity field originally derived by Narasimhacharyulu and Pattabhiramacharyulu (Proc. Indian Acad. Sci. Sect. A 87:79–83, 1978), we find, for the first time, an exact series expression for the Poiseuille number in this regime. Our results match the earlier Ritz-based approximations and are in close agreement with the finite-element solutions presented here.

我们重新讨论了完全发展的达西-布林克曼流通过椭圆截面管的经典问题。在Narasimhacharyulu和Pattabhiramacharyulu (Proc. Indian academy Sci.)最初推导的精确速度场的基础上。(A节87:79-83,1978),我们第一次发现了在这种状态下泊泽维尔数的精确级数表达式。我们的结果与先前的基于ritz的近似相匹配,并且与本文提出的有限元解非常一致。
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引用次数: 0
Pore Network Model for Study of Biofilm Growth Limitations in Porous Substrata 多孔基质中生物膜生长限制研究的孔隙网络模型
IF 2.6 3区 工程技术 Q3 ENGINEERING, CHEMICAL Pub Date : 2025-12-03 DOI: 10.1007/s11242-025-02261-6
Emad Aamer, Felix Faber, Supriya Bhaskaran, Robert Dürr, Katja Bettenbrock, Achim Kienle, Nicole Vorhauer-Huget

We present a pore network approach for the simulation and study of biofilm growth inside porous structures under various limiting conditions. The proposed pore-scale model allows us to resolve the interrelationship between growth and diffusive transport based on the solution of coupled ordinary differential equations. Special focus of this study is on diffusion as well as on metabolically limited conditions, which is realized with different second Damköhler numbers. Instead of relying on idealized geometries, the pore network structures are generated using the effective transport properties of thin sintered particles and fibrous felt porous layers derived from high-resolution X-ray micro-CT scans. The great differences in pore sizes and porosities of the regarded structures result in significantly different effective diffusivities. In addition to that, competitive substrate consumption and inhibition is achieved using the experiment-based kinetic model for S. oneidensis from Tang et al. (Tang et al., Biotechnol. Bioeng. 96:125–133, 2007). The primary nutrients are lactate and oxygen. Acetate is both, a by-product and a potential substrate, theoretically enabling dynamic shifts in substrate utilization. With the chosen parameters and conditions, the second Damköhler number can be varied with a significant impact on biomass distribution inside of the two selected pore networks, especially in dependence on oxygen availability in single pores. The simulation results show that biofilm growth is limited by the transport of dissolved oxygen. Interestingly, significantly more biomass per m3 is produced in the sintered structure because of the generally higher pore utilization degree.

Graphical Abstract

我们提出了一种孔隙网络方法来模拟和研究不同限制条件下多孔结构内生物膜的生长。所提出的孔隙尺度模型使我们能够在求解耦合常微分方程的基础上解决生长与扩散输运之间的相互关系。本研究的重点是扩散和代谢限制条件,这是通过不同的秒Damköhler数来实现的。孔隙网络结构不是依赖于理想的几何形状,而是利用高分辨率x射线微ct扫描得出的薄烧结颗粒和纤维毡多孔层的有效传输特性生成的。不同孔隙结构的孔径和孔隙率差异较大,导致有效扩散系数差异较大。除此之外,竞争性底物消耗和抑制是使用基于实验的动力学模型,从唐等人(唐等人,生物技术。生物工程。96:125-133,2007)。主要的营养物质是乳酸盐和氧气。醋酸盐既是一种副产品,也是一种潜在的底物,理论上可以实现底物利用的动态变化。在选定的参数和条件下,第二个Damköhler数可以改变,这对两个选定的孔隙网络内的生物量分布有显著影响,特别是对单个孔隙中氧气可用性的依赖。模拟结果表明,生物膜的生长受到溶解氧运输的限制。有趣的是,由于孔隙利用率普遍较高,烧结结构中每立方米产生的生物量明显更多。图形抽象
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引用次数: 0
A Graph-Partitioning-Based Multiscale Preconditioner for Modeling Flow in Unstructured Pore Networks 基于图分割的非结构化孔隙网络流建模多尺度预调节器
IF 2.6 3区 工程技术 Q3 ENGINEERING, CHEMICAL Pub Date : 2025-12-03 DOI: 10.1007/s11242-025-02262-5
Alfredo Jaramillo, Bradley McCaskill, Mohammad Piri, Shehadeh Masalmeh

Multiphase flow simulation in porous media is a challenging task with significant industrial implications. Pore Network Modeling (PNM) is an effective method that provides accurate results within a reasonable computational timeframe. However, as the complexity of these systems increases, particularly when simulating whole-core-sized pore networks (Digital Plugs) with millions of elements, there is a growing demand to improve the computational efficiency of PNM. The primary computational bottleneck is the pressure field update process, which involves solving a linear system of balance equations. To address this issue, our research focuses on evaluating the performance of a recently developed multiscale preconditioner for solving this system. We compare its performance against a state-of-the-art algebraic multigrid (AMG) method. Networks where the multiscale preconditioner outperforms AMG are identified, and a multilevel strategy is implemented to extend the capabilities of the method to networks with up to 200 million pore bodies. This shows the multiscale method is a promising alternative to accelerate multiphase simulations in Pore Network Modeling.

多孔介质中多相流的模拟是一项具有重要工业意义的具有挑战性的任务。孔隙网络建模(PNM)是一种有效的方法,可以在合理的计算时间内提供准确的结果。然而,随着这些系统的复杂性的增加,特别是当模拟具有数百万个元素的全核大小的孔隙网络(数字插头)时,提高PNM的计算效率的需求日益增长。主要的计算瓶颈是压力场更新过程,这涉及到求解一个线性平衡方程组。为了解决这个问题,我们的研究重点是评估最近开发的多尺度预调节器的性能,以解决这个系统。我们将其性能与最先进的代数多网格(AMG)方法进行比较。确定了多尺度预调节器优于AMG的网络,并实施了多层次策略,将该方法的功能扩展到具有多达2亿个孔隙体的网络。这表明多尺度方法是一种很有前途的替代方法,可以加速孔隙网络建模中的多相模拟。
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引用次数: 0
Research and Application of the Unsteady Heat Transfer Analytical Model for SAGD SAGD非定常传热分析模型的研究与应用
IF 2.6 3区 工程技术 Q3 ENGINEERING, CHEMICAL Pub Date : 2025-11-28 DOI: 10.1007/s11242-025-02251-8
Guoqing Feng, Pan Wang, Xiangjin Liang, Junhui Zou, Aiping Zheng, Ning Li, Dong Song, Yang Liu, Wenzhi Song, Huan Liu, Haiyang Yu
<div><p>The thermal losses to overburden and underburden in Steam-Assisted Gravity Drainage (SAGD) arise from unsteady heat transfer as the steam chamber continuously changes shape. No accurate analytical solution currently exists. Here we enforce energy conservation, redefine the outer boundary, and reformulate the unsteady-conduction model, establishing a relation between heat-penetration depth and cumulative heat transfer per unit area, and propose a new solution pathway. This method first parameterizes heat-penetration depth, then integrates to obtain cumulative heat transfer, and finally differentiates to compute stratal heat loss. This workflow provides a quantitative route to overburden and underburden thermal losses in SAGD. Coupling the framework with Butler’s oil-rate formula yields closed-form expressions for key SAGD indicators—water production, steam-heat utilization, and oil–steam ratio—derived from unsteady heat conduction. Through axial discretization, the approach accommodates heterogeneity along the horizontal section in a typical SAGD well pattern. We also implement a production-grade program that ingests geological, thermodynamic, and operational inputs and rapidly evaluates multiple outputs, including stratal heat loss, steam-heat utilization, and oil–steam ratio. Against CMG thermal simulation, the overburden heat-loss deviation remains within 5%, substantially improving index-prediction efficiency. Using the Qigu Formation reservoir in the Liu-1 well area of the Karamay Oilfield, Xinjiang, as a case study, we apply the analytical model to optimize planar well spacing to 70 m. For a representative well pair (Well Group A), predictions show that thermal losses to both strata increase and then decline, peaking when the steam chamber reaches the boundary. Sensitivity analysis indicates negative correlations between heat loss and oil saturation, permeability, porosity, and oil-zone thickness, whereas overburden/underburden thermal diffusivity correlates positively with oil–steam ratio. The ranked sensitivity, from strong to weak, is: overburden/underburden thermal diffusivity, oil-zone thickness, oil saturation, permeability, and porosity. The results support index prediction, layout planning, parameter optimization, and measure selection in SAGD-developed heavy-oil reservoirs. The numerical implementation supports batch evaluation and scenario screening, enabling rapid sensitivity sweeps and uncertainty assessment without sacrificing interpretability. We validate the workflow by reproducing time histories of overburden heat loss and by checking consistency of derived indicators with field trends and CMG-STARS benchmarks under identical controls, grids, and rock–fluid properties. The discretized representation preserves mass and energy balances within each segment and allows segment-level attribution of heat sinks and production response. In addition, the program exposes intermediate variables, such as penetration depth and appa
蒸汽辅助重力泄放(SAGD)过程中,随着蒸汽室形状的不断变化,上覆土和下覆土的热损失是由非定常换热引起的。目前还没有准确的解析解。本文强化能量守恒,重新定义外边界,重新建立非定常传导模型,建立热侵彻深度与单位面积累积换热之间的关系,并提出新的求解途径。该方法首先参数化热侵彻深度,然后积分得到累积换热,最后微分计算地层热损失。该工作流程为SAGD的上覆层和下覆层热损失提供了定量的途径。将该框架与Butler的产油率公式相结合,可以得到SAGD关键指标的封闭表达式——产水量、蒸汽热利用率和由非稳态热传导得出的油蒸汽比。通过轴向离散化,该方法可以适应典型SAGD井网水平段的非均质性。我们还实施了一个生产级程序,该程序吸收地质、热力学和操作输入,并快速评估多种输出,包括地层热损失、蒸汽-热利用率和油蒸汽比。对比CMG热模拟,覆盖层热损失偏差控制在5%以内,大大提高了指标预测效率。以新疆克拉玛依油田六1井区七沽组储层为例,应用该分析模型对平面井距进行了优化,达到70 m。对于具有代表性的井对(a井组),预测表明两个地层的热损失先增加后下降,当蒸汽室到达边界时达到峰值。敏感性分析表明,热损失与含油饱和度、渗透率、孔隙度和油层厚度呈负相关,而上覆/下覆热扩散系数与油汽比呈正相关。敏感性由强到弱依次为:上覆岩/下覆岩热扩散系数、油层厚度、含油饱和度、渗透率、孔隙度。研究结果为sagd稠油油藏指标预测、布置规划、参数优化和措施选择提供了依据。数值实现支持批量评估和场景筛选,在不牺牲可解释性的情况下实现快速灵敏度扫描和不确定性评估。我们通过重现覆盖层热损失的时间历史,并在相同的控制、网格和岩石流体性质下,通过检查导出指标与现场趋势和CMG-STARS基准的一致性来验证工作流程。离散化的表示保留了每个区段内的质量和能量平衡,并允许区段级归因散热器和生产响应。此外,该程序还暴露了中间变量,如渗透深度和表观热容量,以便在早期测量可用时进行诊断检查和校准。这些特点使该方法适合于预feed研究以及操作监视和优化。
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引用次数: 0
Real-Time Microfluidic Visualization of Salt Scaling: Impact of Surface Wettability and Scaling Mechanisms in Heterogeneous Porous Media 盐结垢的实时微流控可视化:表面润湿性的影响和非均质多孔介质中的结垢机制
IF 2.6 3区 工程技术 Q3 ENGINEERING, CHEMICAL Pub Date : 2025-11-28 DOI: 10.1007/s11242-025-02260-7
Amélia de Santana Cartaxo, Antônio Demouthié de Sales Rolim Esmeraldo, Sérgio de Souza Camargo Jr., Tiago Albertini Balbino

Calcium carbonate scaling poses a significant challenge in oil and gas production, hindering recovery and impacting economic viability. This study utilizes microfluidic "reservoir-on-chip" platforms to visualize, quantify, and characterize CaCO3 precipitation in hydrophobic and hydrophilic porous media to elucidate scaling mechanisms. Traditional methods face limitations in observing the intricacies of scale formation at the pore scale. Microfluidic platforms, however, offer real-time, high-resolution visualization of flow dynamics and scale deposition, enabling the study of key parameters like temperature, solution concentration, and surface wettability. This research investigates the impact of these parameters on CaCO3 scaling, with a particular focus on wettability's influence on the nucleation process. By elucidating the interplay of different factors, this study aims to provide insights into mitigating and controlling scale formation in oil and gas production. Our findings demonstrate that the covered area by precipitates increased with increasing temperature and concentration for both hydrophobic and hydrophilic surfaces, with more substantial coverage observed on hydrophilic surfaces. Scanning electron microscopy and X-ray diffraction analysis confirmed the presence of calcite, vaterite, and aragonite polymorphs. Furthermore, the findings hold implications for advancing carbon capture, utilization, and storage (CCUS) technologies, particularly mineral carbonation, by providing a deeper understanding of carbonate formation dynamics at the pore scale.

Graphical abstract

碳酸钙结垢对油气生产构成了重大挑战,阻碍了采收率并影响了经济可行性。本研究利用微流体“片上储层”平台可视化、量化和表征CaCO3在疏水和亲水多孔介质中的沉淀,以阐明结垢机制。传统的方法在观察孔隙尺度上结垢形成的复杂性方面存在局限性。然而,微流控平台提供了实时、高分辨率的流动动力学和水垢沉积可视化,从而能够研究温度、溶液浓度和表面润湿性等关键参数。本研究探讨了这些参数对CaCO3结垢的影响,特别关注润湿性对成核过程的影响。通过阐明不同因素的相互作用,本研究旨在为缓解和控制油气生产中的结垢提供见解。我们的研究结果表明,无论是疏水表面还是亲水表面,沉淀的覆盖面积都随着温度和浓度的增加而增加,其中亲水表面的覆盖面积更大。扫描电子显微镜和x射线衍射分析证实了方解石、水晶石和文石多晶体的存在。此外,该研究结果通过提供对孔隙尺度碳酸盐形成动力学的更深入了解,对推进碳捕获、利用和封存(CCUS)技术,特别是矿物碳酸化具有重要意义。图形抽象
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Transport in Porous Media
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