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Relation between the Actual and Estimated Maximum Ground Level Concentration of Air Pollutant and Its Downwind Locations 大气污染物实际和估算的最大地面浓度与顺风位置的关系
Pub Date : 2020-06-30 DOI: 10.4236/ojap.2020.92003
K. Essa, S. Etman, M. El-Otaify
In this work we used the Gaussian plume model to calculate the actual maximum ground level concentration (MGLC) of air pollutant and its downwind location by using different systems of dispersion parameters and for different stack heights. An approximate formula for the prediction of downwind position that produces the MGLC of a pollutant based on the Gaussian formula was derived for different diffusion parameters. The derived formula was used to calculate the approximate MGLC. The actual and estimated values are presented in tables. The comparison between the actual and estimated values was investigated through the calculation of the relative errors. The values of the relative errors between the actual and estimated MGLC lie in the range from: 0 to 70.2 and 0 to 1.6 for Pasquill Gifford system and Klug system respectively. The errors between the actual and estimated location of the MGLC lies in the range from: 0.2 to 227 and 0.7 to 9.4 for Pasquill Gifford system and Klug system respectively.
在这项工作中,我们使用高斯羽流模型,通过使用不同的分散参数系统和不同的烟囱高度来计算空气污染物的实际最大地面浓度及其下风位置。基于高斯公式,针对不同的扩散参数,推导了产生污染物MGLC的顺风位置的近似预测公式。导出的公式用于计算近似MGLC。表中列出了实际值和估计值。通过相对误差的计算,对实际值和估计值之间的比较进行了研究。Pasquill-Giford系统和Klug系统的实际和估计MGLC之间的相对误差值分别在0到70.2和0到1.6的范围内。Pasquill-Giford系统和Klug系统的MGLC的实际位置和估计位置之间的误差分别在0.2到227和0.7到9.4之间。
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引用次数: 5
Seasonal Behavior of Aerosol Vertical Concentration in Dakar and Role Played by the Sea-Breeze 达喀尔气溶胶垂直浓度的季节特征及海风的作用
Pub Date : 2020-02-04 DOI: 10.4236/ojap.2020.91002
H. Senghor, E. Machu, L. Durán, G. Jenkins, A. Gaye
The Westward transport of mineral dust from the North Africa continent to Atlantic Ocean can produce poor air quality, low visibilities, and negatively impacting respiratory and cardiac health due to the optical and physical properties of aerosols. The dynamical impact of the sea-breeze on the dust vertical distribution in West Africa remains unknown. To investigate this issue, we have used in-situ measurements from lidar. We have focused on the attenuated backscatter of aerosols to study the effect of the local circulation on the vertical profile of mineral dust at land-sea transition. The results highlight a strong diurnal cycle of mineral dust associated with the nocturnal low-level jet (NLLJ). The jet is located between 500 m and 1000 m and crucially affected by the dynamic of the sea-breeze circulation.
由于气溶胶的光学和物理特性,矿物尘从北非大陆向西输送到大西洋可能会导致空气质量差、能见度低,并对呼吸和心脏健康产生负面影响。海风对西非沙尘垂直分布的动力影响尚不清楚。为了研究这个问题,我们使用了激光雷达的原位测量。我们专注于气溶胶的衰减后向散射,以研究局部环流对海陆过渡期矿物尘垂直剖面的影响。研究结果强调了与夜间低空急流(NLLJ)相关的矿物尘的强烈日循环。喷流位于500米至1000米之间,受到海风环流动态的严重影响。
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引用次数: 5
Exposure to PM2.5 Related to Road Traffic: Comparison between Crossroads and Outside of Crossroads at Cotonou, Benin 与道路交通相关的PM2.5暴露:贝宁科托努十字路口与十字路口外的比较
Pub Date : 2019-11-07 DOI: 10.4236/ojap.2019.84006
P. Houngbégnon, Gloria Ayivi-Vinz, H. Lawin, K. Houessionon, Fadel Tanimomon, M. Kedote, B. Fayomi, S. Dossou-Gbété, V. Agueh
Background: Several studies have analysed the pollution issues owing to road traffic in Cotonou, Benin. Concentration levels of particles are higher on high traffic than a low traffic. The exposure of human populations to air pollution is more intense on the roads. In Benin, the density of traffic on the crossroads is indeed more important. Are traffic locations such as crossroads, areas where the level of exposure PM2.5 is increased? Methods: This study was conducted along the 5 km high-traffic road in the city of Cotonou. It is a high traffic lane with two crossroads. Sampling and measurements were carried out in dry sea-son (January and February) and rainy season (June and July). For each season the measurements were made over two months from 7 am to 9 pm. PM2.5 measurements were made at different locations at crossroads and also along the track. To compare concentrations of PM2.5 at crossroads and outside of roundabout, we used the Generalized Linear Mixed Model. Results: In the rainy season the PM2.5 hourly concentrations ranged between 400 μg/m3 and 500 μg/m3 while in the dry season 100 μg/m3 and 300 μg/m3. In the rainy season, the average of PM2.5 concentration was 463.25 ± 66.21 μg/m3 at crossroads and 264.75 ± 50.97 μg/m3 outside of crossroads. In the dry season, the average of PM2.5 concentration was 232.75 ± 97.29 μg/m3 at crossroads and 123.31 ± 63.79 μg/m3 outside of crossroads. Both in dry and rainy seasons, PM2.5 concentration level peaks are observed from 7 am to 9 am and from 7 pm to 9 pm. The Generalized Linear Mixed Model showed that there is high significant difference between concentrations of PM2.5 at crossroads compared to outside of crossroads. Occupation of the roadside (in particular crossroads) for various economic activities is common practice in Cotonou thus health risk for people working around crossroads increases. Conclusion: Locations such as crossroads are areas where the level of exposure PM2.5 is highest on road traffics.
背景:几项研究分析了贝宁科托努道路交通造成的污染问题。交通繁忙时颗粒物的浓度水平比交通繁忙时高。在道路上,人们对空气污染的暴露更为严重。在贝宁,十字路口的交通密度确实更为重要。十字路口等交通场所是PM2.5暴露水平增加的区域吗?方法:本研究在科托努市5公里高速公路沿线进行。这是一条交通繁忙的车道,有两个十字路口。在旱季(1月和2月)和雨季(6月和7月)进行采样和测量。每个季节的测量都是在两个月内从早上7点到晚上9点进行的。PM2.5的测量是在十字路口和轨道沿线的不同地点进行的。为了比较十字路口和环岛外的PM2.5浓度,我们使用了广义线性混合模型。结果:雨季PM2.5时浓度在400 ~ 500 μg/m3之间,旱季PM2.5时浓度在100 ~ 300 μg/m3之间。雨季,十字路口PM2.5浓度平均值为463.25±66.21 μg/m3,十字路口外PM2.5浓度平均值为264.75±50.97 μg/m3。旱季,十字路口PM2.5浓度均值为232.75±97.29 μg/m3,十字路口外PM2.5浓度均值为123.31±63.79 μg/m3。在旱季和雨季,PM2.5浓度峰值出现在早上7点到9点以及晚上7点到9点。广义线性混合模型表明,十字路口PM2.5浓度与十字路口外存在高度显著性差异。占领路边(特别是十字路口)进行各种经济活动是科托努的普遍做法,因此在十字路口附近工作的人的健康风险增加。结论:十字路口等地点是道路交通中PM2.5暴露水平最高的区域。
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引用次数: 4
Climatological Analysis of Aerosols Optical Properties by Airborne Sensors and in Situ Measurements in West Africa: Case of the Sahelian Zone 基于机载传感器和实地测量的西非气溶胶光学特性的气候分析:以萨赫勒地区为例
Pub Date : 2019-11-07 DOI: 10.4236/ojap.2019.84007
Nébon Bado, A. Ouedraogo, H. Guengane, T. S. M. Ky, S. D. Bazyomo, B. Korgo, M. Drame, S. Sall, F. Kiéno, D. Bathiébo
This paper deals with the climatology of aerosols in West Africa based on satellite and in situ measurements between 2001 and 2016 and covers four sites in the Sahelian zone. There are indeed Banizoumbou (13.541°N, 02.665°E), Cinzana (13.278°N, 05.934°W), Dakar (14.394°N, 16.959°W) and Ouagadougou (12.20°N, 1.40°W) located respectively in Niger, Mali, Senegal and Burkina Faso. Thus, an intercomparison between the satellite observations and the in situ measurements shows a good correlation between MODIS and AERONET with a correlation coefficient R = 0.86 at Cinzana, R = 0.85 at Banizounbou, R = 0.84 at Ouagadougou and a low correlation coefficient R = 0.66 calculated on the Dakar site. Like MODIS, SeaWiFS shows a very good correspondence with measurements of the ground photometer especially for Banizoumbou (R = 0.89), Cinzana (R = 0.88) and Dakar (R = 0.75) followed by a low correlation coefficient calculated on the Ouagadougou site (R = 0.64). The performance of these airborne sensors is also corroborated by the calculation of root mean square error (RMSE) and the mean absolute error (MAE). Following this validation, a climatological analysis based on aerosol optical depth (AOD) shows the seasonality of aerosols in West Africa strongly influenced by the climate dynamics illustrated by the MERRA model reanalysis. This seasonal spatial distribution of aerosols justifies the temporal variability of the particles observed at the different sites in the Sahel. In addition, a combined analysis of AOD and Angstrom coefficient indicates the aerosol period in the Sahel in spring (March-April-May) and summer (June-July-August). However, these aerosols are strongly dominated by desert dust whose main sources are located north in the Sahara and Sahel.
本文基于2001年至2016年间的卫星和现场测量,研究了西非气溶胶的气候学,涵盖了萨赫勒地区的四个地点。尼日尔、马里、塞内加尔和布基纳法索分别有巴尼祖姆布(13.541°N,02.665°E)、辛扎纳(13.278°N,05.934°W)、达喀尔(14.394°N,16.959°W)和瓦加杜古(12.20°N,1.40°W)。因此,卫星观测和现场测量之间的相互比较显示,MODIS和AERONET之间具有良好的相关性,Cinzana的相关系数R=0.86,Banizounbou的相关系数R=0.85,瓦加杜古的相关系数P=0.84,达喀尔现场计算的相关系数低,R=0.66。与MODIS一样,SeaWiFS与地面光度计的测量结果显示出非常好的一致性,尤其是Banizoumbou(R=0.89),Cinzana(R=0.88)和Dakar(R=0.75),然后在瓦加杜古现场计算出低相关系数(R=0.64)。这些机载传感器的性能也通过均方根误差(RMSE)和平均绝对误差(MAE)的计算得到证实。在此验证之后,基于气溶胶光学深度(AOD)的气候分析显示,西非气溶胶的季节性受到MERRA模型再分析所示气候动力学的强烈影响。气溶胶的这种季节性空间分布证明了在萨赫勒地区不同地点观测到的颗粒物的时间变异性。此外,AOD和Angstrom系数的综合分析表明,萨赫勒地区春季(3月至4月至5月)和夏季(6月至7月至8月)的气溶胶期。然而,这些气溶胶主要由沙漠尘埃主导,其主要来源位于撒哈拉以北和萨赫勒地区。
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引用次数: 3
Contribution of Hydrofluorocarbons (HFCs) and Hydrofluoro-Olefins (HFOs) Atmospheric Breakdown Products to Acidification (“Acid Rain”) in the EU at Present and in the Future 氢氟碳化合物(hfc)和氢氟烯烃(hfo)大气分解产品对欧盟目前和未来酸化("酸雨")的贡献
Pub Date : 2019-11-07 DOI: 10.4236/ojap.2019.84004
A. Lindley, A. Mcculloch, Tim Vink
While hydrogen fluoride (HF) and hydrogen chloride (HCl) are not considered main air-pollutants in the EU, they have the potential to contribute to acidification. Hydrofluorocarbons (HFCs), hydrofluoro-olefins (HFOs) and hydrochlorofluoro-olefins (HCFOs) are used as refrigerants and for other applications. They break down in the atmosphere to produce HF and HCl (for HCFOs) and some of these fluorocarbons also break down to produce trifluoroacetic acid (TFA). For the emissions of these fluorocarbons in the EU, a worst-case scenario estimates their theoretical potential contribution to acidification and compares it to the acidification potential for the main air pollutants contributing to acidification, which are nitrous oxides (NOx), sulphur oxides (mainly SO2), and ammonia (NH3). The Acidification Potential from these fluorocarbons in 2016 is estimated at 2, NOx, NH3, and it can be concluded that this is insignificant in the context of the main acidification air-pollutants. Assuming that the EU targets for emissions of SO2, NOx and NH3 by 2030 are achieved, the Acidification Potential from HFCs, HFOs and HCFOs in 2030 is also estimated at 2, NOx, NH3 and will remain insignificant.
虽然氟化氢(HF)和氯化氢(HCl)在欧盟不被认为是主要的空气污染物,但它们有可能导致酸化。氢氟碳化合物(HFCs)、氢氟烯烃(HFO)和氢氯氟烯烃(HCFO)用作制冷剂和用于其他应用。它们在大气中分解产生HF和HCl(用于HCFO),其中一些氟碳化合物也分解产生三氟乙酸(TFA)。对于欧盟这些氟碳化合物的排放,最坏的情况估计了它们对酸化的理论潜在贡献,并将其与导致酸化的主要空气污染物的酸化潜力进行比较,这些污染物是一氧化二氮(NOx)、硫氧化物(主要是SO2)和氨(NH3)。2016年,这些氟碳化合物的酸化潜力估计为2,NOx,NH3,可以得出结论,在主要酸化空气污染物的背景下,这是微不足道的。假设欧盟到2030年实现了二氧化硫、氮氧化物和氨的排放目标,2030年氢氟碳化合物、氢氟碳化合物和氟氯烃的酸化潜力估计也为2,氮氧化物和NH3,并且仍然微不足道。
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引用次数: 6
Seasonal Influence in Traffic-Related Air Pollutants Concentrations in Urban Parks from Porto Alegre, Brazil 巴西阿雷格里港城市公园交通相关空气污染物浓度的季节性影响
Pub Date : 2019-11-07 DOI: 10.4236/ojap.2019.84005
Bruna Marmett, R. Carvalho, Fernanda Ramos Rhoden, C. Rhoden
Traffic-related air pollution is an alarming source of pollutants exposure and consequently to the development of several adverse health effects. Otherwise, green spaces are reported to improve health status. Although, in an urban scenario most of these areas are located near air pollutants sources, as vehicle fleet. Thus, the aim of the present study was to determine, during one year, the levels of nitrogen dioxide (NO2) and ozone (O3) in the main parks from Porto Alegre—Brazil. This study focused on three urban parks: Germania, Moinhos de Vento and Marinha do Brasil Park. Nitrogen dioxide and ozone measurements were accessed by passive monitoring in four campaigns including all seasons and performed at distances of 0 m, 15 m, 30 m, 45 m, 60 m and 75 m from the main road at each park. NO2 and O3 concentration among the parks was not different (p > 0.05), as well as the mean concentration of NO2 and O3 of all parks in the six sites did not differ (p > 0.05). However, season 1 and 3 showed increased NO2 and O3 concentration. Temperature were decreased in season 1 and 3 (p p > 0.05). Traffic flow was higher in Moinhos de Vento Park and Marinha do Brasil Park compared to Germania Park (p 2 and O3 concentration in urban parks from Porto Alegre.
与交通有关的空气污染是污染物暴露的一个令人担忧的来源,因此会对健康产生一些不利影响。否则,据报道,绿地可以改善健康状况。尽管如此,在城市场景中,这些区域大多位于空气污染源附近,如车队。因此,本研究的目的是在一年内确定巴西阿雷格里港主要公园的二氧化氮(NO2)和臭氧(O3)水平。这项研究的重点是三个城市公园:日耳曼尼亚,莫因霍斯德文托和马林哈巴西公园。二氧化氮和臭氧测量通过四次活动(包括所有季节)的被动监测进行,并在距离每个公园主干道0米、15米、30米、45米、60米和75米的距离处进行。公园间NO2和O3浓度无差异(p>0.05),6个地点所有公园的NO2和O3平均浓度也无差异(p>0.05)。第1季和第3季的气温有所下降(p>0.05)。与日耳曼尼亚公园相比,Moinhos de Vento公园和Marinha do Brasil公园的交通流量更高(阿雷格里港城市公园的P2和O3浓度)。
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引用次数: 5
Citizens and Air Quality: The Results of the First Survey Carried Out in the Po River Basin (Northern Italy) 公民与空气质量:波河流域(意大利北部)首次调查结果
Pub Date : 2019-09-19 DOI: 10.4236/ojap.2019.83003
E. Cancila, Irene Sabbadini, Marco Ottolenghi, M. Deserti, Sara Tessitore
The air quality survey investigated the level of perception and awareness of citizens on the air quality in the 42 cities (provincial capitals) of the Po basin in the north west of Italy. This study means that perceptions could then be compared between in the Po basin and other parts of Italy and Europe. This research was carried out as part of the Life15 IPE IT 013 PREPAIR Project (Po Regions Engaged to Policies of Air), which involves 18 national and international partners, and includes all the regions of the Po Basin. The survey involved around 7331 citizens that live in the Po basin that includes 42 cities (provincial capitals) and a total of 6.5 million inhabitants. A multivariate analysis was applied to identify the main citizens’ profiles concerning the topic of air quality and the availability to implement virtuous behaviours to reduce air pollution. Four different profiles emerge from the cluster analysis: “Committed and proactive”, “Willing but …”, “Hesitant”, “Not willing”.
空气质量调查调查了意大利西北部波河流域42个城市(省会)的公民对空气质量的感知和意识水平。这项研究意味着,可以将波河流域与意大利和欧洲其他地区的看法进行比较。这项研究是Life15 IPE IT 013 PREPAIR项目(参与空气政策的Po地区)的一部分,该项目涉及18个国家和国际合作伙伴,包括Po盆地的所有地区。这项调查涉及居住在Po流域的约7331名公民,该流域包括42个城市(省会)和650万居民。应用多元分析来确定主要公民关于空气质量主题的概况,以及实施良性行为以减少空气污染的可用性。聚类分析得出了四种不同的概况:“承诺和积极主动”、“愿意但…”、“犹豫不决”、“不愿意”。
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引用次数: 0
Geothermal, Oceanic, Wildfire, Meteorological and Anthropogenic Impacts on PM2.5 Concentrations in the Fairbanks Metropolitan Area 地热、海洋、野火、气象和人为因素对费尔班克斯都市区PM2.5浓度的影响
Pub Date : 2019-06-30 DOI: 10.4236/OJAP.2019.82002
N. Mölders, G. Fochesatto, S. Edwin, G. Kramm
The impacts of low and high-frequency variability from teleconnections between large scale atmospheric processes and local weather as well as emissions changes on concentrations of particulate matter of 2.5 μm or less in diameter ([PM2.5]) were examined for the Fairbanks Metropolitan Area (FMA). October to March and May to August mean [PM2.5] were 1.8 and 3.1 μg·m-3 higher for positive than negative annual mean Pacific Decadal Oscillation. Annual mean [PM2.5] were 3.8 μg·m-3 lower for positive than negative Southern Oscillation Index. On 1999-2018 average, [PM2.5] decreased 2.9 μg·m-3·decade-1. On average over October to March, decadal and inter-annual variability caused higher or similar differences in mean observed [PM2.5] and its species than emission-control measures. The 2006 implementation of Tier 2 for new vehicles decreased observed sulfate concentrations the strongest (~4.95 μg·m-3·decade-1) of all occurred emissions changes. On average, observed [PM2.5] showed elevated values at all sites when wind blew from directions of hot springs. The same was found for the sulfate, ammonium and non-metal components of PM2.5. Observations showed that these geothermal waters contain sulfate, ammonia, boric acid and non-metals. Hot springs of such composition are known to emit hydrogen sulfide and ammonia that can serve as precursors for ammonium and sulfate aerosols.
在费尔班克斯大都会区(FMA),研究了大规模大气过程与当地天气之间遥相关的低频和高频变化以及排放变化对直径小于或等于2.5μm的颗粒物浓度([PM2.5])的影响。10月至3月和5月至8月的平均PM2.5分别比负的年平均太平洋十年振荡高1.8和3.1μg·m-3。正南方涛动指数的年平均〔PM2.5〕比负南方涛动指标低3.8μg·m-3。在1999-2018年的平均水平上,[PM2.5]下降了2.9μg·m-3·decate-1。平均而言,10月至3月,十年和年际变化导致观测到的平均PM2.5及其种类的差异高于或类似于排放控制措施。2006年对新车实施Tier 2降低了观测到的硫酸盐浓度,这是所有发生的排放变化中最强的(~4.95μg·m-3·decate-1)。平均而言,当风从温泉方向吹来时,观测到的PM2.5在所有地点都显示出升高的值。PM2.5的硫酸盐、铵和非金属成分也是如此。观测表明,这些地热水中含有硫酸盐、氨、硼酸和非金属。已知这种成分的温泉会释放硫化氢和氨,这些硫化氢和氨可以作为铵和硫酸盐气溶胶的前体。
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引用次数: 3
Predictive Meteorological Factors for Elevated PM2.5 Levels at an Air Monitoring Station Near a Petrochemical Complex in Yunlin County, Taiwan 台湾云林县石化厂附近空气监测站PM2.5水平升高的预测气象因素
Pub Date : 2019-03-29 DOI: 10.4236/OJAP.2019.81001
Yee-Hsin Kao, Chih-Wen Lin, J. Chiang
Since 1991, air pollution has gained special attention in Taiwan after a petrochemical complex was constructed in Mailiao Township, Yunlin County. We explored the association between the magnitude of PM2.5 and meteorological factors during 2012-2016. Our findings revealed that 1) mean PM2.5 levels gradually decreased from 30.70 μg/m3 in 2013 to 25.36 μg/m3 in 2016; 2) wind speed is the main determinant of air quality—air quality significantly improved when it was faster than 4 m/sec; and 3) wind direction is another determinant of air quality—when the wind direction was southerly, air quality improved. Elevated PM2.5 levels were defined as those hourly levels higher than the third quartile (36 μg/m3). The significantly negative predictive factors for elevated PM2.5 levels were the summer or autumn seasons, rainfall, increased wind speed, and wind direction from 150° to 230° from the north. The significantly positive predictive factors for elevated PM2.5 levels were working hours from 6 a.m. to 2 p.m., a temperature between 11°C and 25°C, relative humidity between 40% and 68%, and wind direction (e.g., northerly wind, northeasterly wind, and easterly wind). The predictive formula is attached in the Appendix. Therefore, people should protect themselves on these high-risk days.
1991年以来,台湾云林县麦寮乡兴建石化厂后,空气污染问题日益受到重视。我们探讨了2012-2016年PM2.5的强度与气象因素之间的关系。我们的研究结果表明:1)PM2.5平均水平从2013年的30.70微克/立方米逐渐下降到2016年的25.36微克/立方米;2) 风速是空气质量的主要决定因素——风速超过4米/秒时,空气质量显著改善;3)风向是空气质量的另一个决定因素——当风向为南风时,空气质量有所改善。PM2.5水平升高被定义为高于第三个四分位数(36微克/立方米)的小时水平。PM2.5水平升高的显著负面预测因素是夏季或秋季、降雨、风速增加以及风向从150°到230°。PM2.5水平升高的显著积极预测因素是早上6点到下午2点的工作时间、11°C到25°C的温度、40%到68%的相对湿度以及风向(如北风、东北风和东风)。预测公式见附录。因此,人们应该在这些高风险的日子里保护自己。
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引用次数: 2
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Open journal of air pollution
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