首页 > 最新文献

Advanced Sensor Research最新文献

英文 中文
Smart Hydrogel Sensors for Health Monitoring and Early Warning (Adv. Sensor Res. 9/2024) 用于健康监测和预警的智能水凝胶传感器(传感器研究进展 9/2024)
Pub Date : 2024-09-10 DOI: 10.1002/adsr.202470026
Kang Wang, Junhui Zhang, Heng Li, Jingzhi Wu, Qiwu Wan, Taiju Chen, Wenjing Liu, Hai Peng, Hong Zhang, Yang Luo

Smart Monitoring Hydrogel Sensors

In article 2400003, Hong Zhang, Yang Luo, and co-workers report advancements in smart hydrogel sensors for health monitoring and early warning. Leveraging the biocompatible properties of hydrogels, these sensors facilitate continuous, precise monitoring of various physiological parameters. The review highlights the mechanisms of these sensors, their benefits for medical diagnostics, and directions for future research. It also explores their potential in various medical scenarios, such as disease monitoring and management, underscoring the need for further clinical validation.

智能监测水凝胶传感器在第 2400003 号文章中,张宏、罗扬及其合作者报告了用于健康监测和预警的智能水凝胶传感器的研究进展。利用水凝胶的生物相容性,这些传感器可对各种生理参数进行连续、精确的监测。综述重点介绍了这些传感器的作用机制、它们在医疗诊断方面的优势以及未来的研究方向。文章还探讨了它们在疾病监测和管理等各种医疗场景中的潜力,强调了进一步临床验证的必要性。
{"title":"Smart Hydrogel Sensors for Health Monitoring and Early Warning (Adv. Sensor Res. 9/2024)","authors":"Kang Wang,&nbsp;Junhui Zhang,&nbsp;Heng Li,&nbsp;Jingzhi Wu,&nbsp;Qiwu Wan,&nbsp;Taiju Chen,&nbsp;Wenjing Liu,&nbsp;Hai Peng,&nbsp;Hong Zhang,&nbsp;Yang Luo","doi":"10.1002/adsr.202470026","DOIUrl":"https://doi.org/10.1002/adsr.202470026","url":null,"abstract":"<p><b>Smart Monitoring Hydrogel Sensors</b></p><p>In article 2400003, Hong Zhang, Yang Luo, and co-workers report advancements in smart hydrogel sensors for health monitoring and early warning. Leveraging the biocompatible properties of hydrogels, these sensors facilitate continuous, precise monitoring of various physiological parameters. The review highlights the mechanisms of these sensors, their benefits for medical diagnostics, and directions for future research. It also explores their potential in various medical scenarios, such as disease monitoring and management, underscoring the need for further clinical validation.\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":100037,"journal":{"name":"Advanced Sensor Research","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2024-09-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/adsr.202470026","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142170190","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Masthead (Adv. Sensor Res. 9/2024) 桅杆头(第 9/2024 号传感器预案)
Pub Date : 2024-09-10 DOI: 10.1002/adsr.202470027
{"title":"Masthead (Adv. Sensor Res. 9/2024)","authors":"","doi":"10.1002/adsr.202470027","DOIUrl":"https://doi.org/10.1002/adsr.202470027","url":null,"abstract":"","PeriodicalId":100037,"journal":{"name":"Advanced Sensor Research","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2024-09-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/adsr.202470027","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142170191","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Integrated Microwave Photonic Sensors Based on Microresonators (Adv. Sensor Res. 8/2024) 基于微谐振器的集成微波光子传感器(传感器研究进展 8/2024)
Pub Date : 2024-08-08 DOI: 10.1002/adsr.202470025
Xiaoyi Tian, Liwei Li, Linh Nguyen, Xiaoke Yi

Integrated Microwave Photonic Sensors

Sensors stand as pivotal cornerstones of technologies. In article 2300145, Xiaoke Yi and co-workers demonstrate integrated microwave photonic sensors using microresonators for ultra-sensitive, high-resolution, and rapid detection. These compact sensors, enhanced through integration techniques and artificial intelligence, offer great potential across various applications, representing a significant advancement in modern sensing technologies.

集成微波光子传感器传感器是技术的重要基石。在第 2300145 号文章中,Xiaoke Yi 及其合作者展示了利用微谐振器实现超灵敏、高分辨率和快速检测的集成微波光子传感器。这些小巧的传感器通过集成技术和人工智能得到了增强,在各种应用中具有巨大的潜力,是现代传感技术的一大进步。
{"title":"Integrated Microwave Photonic Sensors Based on Microresonators (Adv. Sensor Res. 8/2024)","authors":"Xiaoyi Tian,&nbsp;Liwei Li,&nbsp;Linh Nguyen,&nbsp;Xiaoke Yi","doi":"10.1002/adsr.202470025","DOIUrl":"https://doi.org/10.1002/adsr.202470025","url":null,"abstract":"<p><b>Integrated Microwave Photonic Sensors</b></p><p>Sensors stand as pivotal cornerstones of technologies. In article 2300145, Xiaoke Yi and co-workers demonstrate integrated microwave photonic sensors using microresonators for ultra-sensitive, high-resolution, and rapid detection. These compact sensors, enhanced through integration techniques and artificial intelligence, offer great potential across various applications, representing a significant advancement in modern sensing technologies.\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":100037,"journal":{"name":"Advanced Sensor Research","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2024-08-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/adsr.202470025","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141967760","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Masthead (Adv. Sensor Res. 8/2024) 桅杆头(传感器推进决议 8/2024)
Pub Date : 2024-08-08 DOI: 10.1002/adsr.202470024
{"title":"Masthead (Adv. Sensor Res. 8/2024)","authors":"","doi":"10.1002/adsr.202470024","DOIUrl":"https://doi.org/10.1002/adsr.202470024","url":null,"abstract":"","PeriodicalId":100037,"journal":{"name":"Advanced Sensor Research","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2024-08-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/adsr.202470024","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141967779","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Development of Kirigami-Patterned Stretchable Tactile Sensor Array with Soft Hinges for Highly Sensitive Force Detection (Adv. Sensor Res. 8/2024) 开发具有软铰链的桐木图案可伸缩触觉传感器阵列,实现高灵敏度力检测(传感器研究进展 8/2024)
Pub Date : 2024-08-08 DOI: 10.1002/adsr.202470023
Chenhao Mao, Jie Jin, Deqing Mei, Yancheng Wang

Deformation-Insensitivity

Flexible sensor array using kirigami structural and soft-hinge design enables deformation-insensitive pressure detection. The sensitivity of sensor is enhanced by the modification with micropillars on conductive rubber. Characterization tests verify the almost negligible effects to sensor caused by 40% stretching and 180° bending interferences. The proposed sensor array is capable of functioning on the deformable surfaces with stable detection signals. More details can be found in article 2400012 by Yancheng Wang and co-workers.

形变敏感性采用叽里格米结构和软铰链设计的柔性传感器阵列可实现形变敏感性压力检测。通过对导电橡胶上的微柱进行改性,提高了传感器的灵敏度。特性测试证明,40% 的拉伸和 180° 的弯曲干扰对传感器的影响几乎可以忽略不计。所提出的传感器阵列能够在可变形表面上正常工作,并提供稳定的检测信号。更多详情,请参阅王彦成及其合作者撰写的文章 2400012。
{"title":"Development of Kirigami-Patterned Stretchable Tactile Sensor Array with Soft Hinges for Highly Sensitive Force Detection (Adv. Sensor Res. 8/2024)","authors":"Chenhao Mao,&nbsp;Jie Jin,&nbsp;Deqing Mei,&nbsp;Yancheng Wang","doi":"10.1002/adsr.202470023","DOIUrl":"https://doi.org/10.1002/adsr.202470023","url":null,"abstract":"<p><b>Deformation-Insensitivity</b></p><p>Flexible sensor array using kirigami structural and soft-hinge design enables deformation-insensitive pressure detection. The sensitivity of sensor is enhanced by the modification with micropillars on conductive rubber. Characterization tests verify the almost negligible effects to sensor caused by 40% stretching and 180° bending interferences. The proposed sensor array is capable of functioning on the deformable surfaces with stable detection signals. More details can be found in article 2400012 by Yancheng Wang and co-workers.\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":100037,"journal":{"name":"Advanced Sensor Research","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2024-08-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/adsr.202470023","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141967778","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Flexible Tribo-Enhanced Piezoelectric Nanogenerator Based on Aluminium Ferrite Electrospun Hybrid Nanofibers for Energy Harvesting and Patient Rehabilitation Application 基于铝铁氧体电纺混合纳米纤维的柔性三相增强压电纳米发电机,用于能量收集和患者康复应用
Pub Date : 2024-07-29 DOI: 10.1002/adsr.202400023
Nishat Kumar Das, Sushmee Badhulika

Mechanical energy harvesters have recently emerged as promising options for self-powering sensors and small electronic devices. In this work, aluminum ferrite (AlFeO3)/PVDF hybrid perovskite electrospun nanofiber-based tribo-enhanced piezoelectric nanogenerators (TPENGs) are developed for energy harvesting. The as-fabricated TPENG achieves an average voltage output of 52.3 V and an average current output of 1.23 µA. Additionally, the power density of the TPENG is calculated to be 0.085 W.m−2 at an 80 MΩ external resistance load. A 3D-printed device is fabricated, containing nylon fabric (tribo-positive) as a rotor attached to printed fins, while six (AlFeO3)/PVDF hybrid perovskite electrospun nanofiber piezoelectric nanogenerators (PENGs) wrapped with Kapton tape (tribo-negative) serve as the stator. The three printed fins of the device are moved by a string-based pulley, generating an open circuit voltage of 200 V and a short circuit current of 4.5 µA. The as-fabricated 3D-printed device with TPENGs is used to power small electronics (e.g., LEDs and watch) and an exercise setup, allowing patients to generate power by pulling the attached string, thereby estimating the level of impairment. Integrating energy harvesting into rehabilitation motivates patients to move impaired body parts, enhancing TPENG's application in healthcare as a practical and engaging tool for patient rehabilitation.

最近,机械能收集器已成为自供电传感器和小型电子设备的理想选择。本研究开发了用于能量收集的铝铁氧体 (AlFeO3)/PVDF 混合包晶电纺纳米纤维基三相增强压电纳米发电机 (TPENG)。制作完成的 TPENG 实现了 52.3 V 的平均电压输出和 1.23 µA 的平均电流输出。此外,经计算,在 80 MΩ 外部电阻负载下,TPENG 的功率密度为 0.085 W.m-2。三维打印设备包含尼龙织物(三极正极)作为转子,连接到打印鳍片上,而六个用 Kapton 胶带(三极负极)包裹的 (AlFeO3)/PVDF 混合包晶电纺纳米纤维压电纳米发电机(PENG)作为定子。该装置的三个印刷鳍片通过一个基于线的滑轮移动,可产生 200 V 的开路电压和 4.5 µA 的短路电流。带有 TPENGs 的 3D 打印设备可用于为小型电子设备(如 LED 和手表)和运动装置供电,让患者通过拉动连接的绳索来发电,从而估算损伤程度。将能量收集融入康复治疗可激励患者移动受损的身体部位,从而提高 TPENG 在医疗保健领域的应用,使其成为患者康复治疗的实用而有吸引力的工具。
{"title":"Flexible Tribo-Enhanced Piezoelectric Nanogenerator Based on Aluminium Ferrite Electrospun Hybrid Nanofibers for Energy Harvesting and Patient Rehabilitation Application","authors":"Nishat Kumar Das,&nbsp;Sushmee Badhulika","doi":"10.1002/adsr.202400023","DOIUrl":"https://doi.org/10.1002/adsr.202400023","url":null,"abstract":"<p>Mechanical energy harvesters have recently emerged as promising options for self-powering sensors and small electronic devices. In this work, aluminum ferrite (AlFeO<sub>3</sub>)/PVDF hybrid perovskite electrospun nanofiber-based tribo-enhanced piezoelectric nanogenerators (TPENGs) are developed for energy harvesting. The as-fabricated TPENG achieves an average voltage output of 52.3 V and an average current output of 1.23 µA. Additionally, the power density of the TPENG is calculated to be 0.085 W.m<sup>−2</sup> at an 80 MΩ external resistance load. A 3D-printed device is fabricated, containing nylon fabric (tribo-positive) as a rotor attached to printed fins, while six (AlFeO<sub>3</sub>)/PVDF hybrid perovskite electrospun nanofiber piezoelectric nanogenerators (PENGs) wrapped with Kapton tape (tribo-negative) serve as the stator. The three printed fins of the device are moved by a string-based pulley, generating an open circuit voltage of 200 V and a short circuit current of 4.5 µA. The as-fabricated 3D-printed device with TPENGs is used to power small electronics (e.g., LEDs and watch) and an exercise setup, allowing patients to generate power by pulling the attached string, thereby estimating the level of impairment. Integrating energy harvesting into rehabilitation motivates patients to move impaired body parts, enhancing TPENG's application in healthcare as a practical and engaging tool for patient rehabilitation.</p>","PeriodicalId":100037,"journal":{"name":"Advanced Sensor Research","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2024-07-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/adsr.202400023","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142170272","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Masthead (Adv. Sensor Res. 7/2024) 桅杆头(传感器推进决议 7/2024)
Pub Date : 2024-07-12 DOI: 10.1002/adsr.202470022
{"title":"Masthead (Adv. Sensor Res. 7/2024)","authors":"","doi":"10.1002/adsr.202470022","DOIUrl":"https://doi.org/10.1002/adsr.202470022","url":null,"abstract":"","PeriodicalId":100037,"journal":{"name":"Advanced Sensor Research","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2024-07-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/adsr.202470022","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141624323","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Direct Fabrication of Electronic Circuits on Wooden Surfaces (Adv. Sensor Res. 7/2024) 在木质表面直接制作电子电路(传感器研究进展 7/2024)
Pub Date : 2024-07-12 DOI: 10.1002/adsr.202470021
Florian Egger, David Schiller, Thomas Stockinger, Claudia Pretschuh, Uwe Müller, Martin Kaltenbrunner

Interactive Wood

Sensors fabricated directly onto wooden surfaces allow to detect humidity and temperature changes or monitor the curing of varnishes. They enable structural integrity monitoring in construction or turn furniture into interactive touch panels, all in a sustainable fashion. More details can be found in article number 2400010 by Martin Kaltenbrunner and co-workers.

交互式木材传感器可直接安装在木材表面,用于检测湿度和温度变化,或监测清漆的固化情况。它们可以监测建筑结构的完整性,或将家具变成交互式触摸屏,所有这些都是可持续的。更多详情,请参阅马丁-卡尔特布伦纳(Martin Kaltenbrunner)及其合作者撰写的第 2400010 号文章。
{"title":"Direct Fabrication of Electronic Circuits on Wooden Surfaces (Adv. Sensor Res. 7/2024)","authors":"Florian Egger,&nbsp;David Schiller,&nbsp;Thomas Stockinger,&nbsp;Claudia Pretschuh,&nbsp;Uwe Müller,&nbsp;Martin Kaltenbrunner","doi":"10.1002/adsr.202470021","DOIUrl":"https://doi.org/10.1002/adsr.202470021","url":null,"abstract":"<p><b>Interactive Wood</b></p><p>Sensors fabricated directly onto wooden surfaces allow to detect humidity and temperature changes or monitor the curing of varnishes. They enable structural integrity monitoring in construction or turn furniture into interactive touch panels, all in a sustainable fashion. More details can be found in article number 2400010 by Martin Kaltenbrunner and co-workers.\u0000\u0000 <figure>\u0000 <div><picture>\u0000 <source></source></picture><p></p>\u0000 </div>\u0000 </figure></p>","PeriodicalId":100037,"journal":{"name":"Advanced Sensor Research","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2024-07-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/adsr.202470021","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141624321","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Platinum Decorated Palladium Nanowires for Room-Temperature Hydrogen Detection 用于室温氢探测的铂装饰钯纳米线
Pub Date : 2024-06-24 DOI: 10.1002/adsr.202400013
Abhishek Kumar, Yaoli Zhao, Sadaf Mohsenifard, Vaishali Maheshkar, Thomas Thundat, Mark T. Swihart

The use of hydrogen as an energy carrier will require low-cost, low-power hydrogen sensors. Toward this goal, penta-twinned palladium nanowires (Pd NWs) are synthesized and fabricated sensors from them by drop-casting. Pd NWs drop-cast onto an interdigitated electrode (IDE) gave a response of 0.3% to 1 vol.% H2, with response and recovery times of 12 and 20 s, respectively. However, they exhibited a negative response (decreased resistance) at low H2 concentrations. Pd NWs on a paper substrate provided a tenfold higher response to 1 vol.% H2, with response and recovery times of 10 s each, but still exhibited negative response at low H2 concentration. Exposing the Pd NW-on-paper sensor to ozone-generating UV light degraded the PVP used in Pd NW synthesis, eliminating the reverse sensing response, and providing a response of 5% to 1 vol.% H2, with response and recovery times of 15 s. This allowed reliable H2 detection down to 100 ppm H2. Finally, coating the Pd NWs with a small amount of Pt (<5%) reduced the response and recovery times to 5 s by catalyzing H2 dissociation. This work provides a path to low-cost sensors to enable the safe use of H2 as an energy carrier.

使用氢作为能源载体需要低成本、低功耗的氢传感器。为了实现这一目标,我们合成了五孪晶钯纳米线(Pd NWs),并通过滴铸方法将其制成了传感器。将钯纳米线滴铸到互斥电极(IDE)上可产生 0.3% 至 1 vol.% H2 的响应,响应时间和恢复时间分别为 12 秒和 20 秒。然而,在低浓度 H2 时,它们表现出负响应(电阻下降)。纸基底上的钯碳纳米管对 1 vol.% H2 的响应提高了十倍,响应和恢复时间分别为 10 秒,但在低 H2 浓度时仍表现出负响应。将纸基钯碳氧化物传感器暴露在产生臭氧的紫外线下,会使钯碳氧化物合成过程中使用的 PVP 降解,从而消除反向感应反应,对 1 Vol.% H2 的响应为 5%,响应和恢复时间均为 15 秒。最后,通过催化 H2 解离,在钯碳氮化物上镀上少量铂(5%),可将响应和恢复时间缩短至 5 秒。这项工作为低成本传感器提供了一条途径,使人们能够安全地将 H2 用作能量载体。
{"title":"Platinum Decorated Palladium Nanowires for Room-Temperature Hydrogen Detection","authors":"Abhishek Kumar,&nbsp;Yaoli Zhao,&nbsp;Sadaf Mohsenifard,&nbsp;Vaishali Maheshkar,&nbsp;Thomas Thundat,&nbsp;Mark T. Swihart","doi":"10.1002/adsr.202400013","DOIUrl":"https://doi.org/10.1002/adsr.202400013","url":null,"abstract":"<p>The use of hydrogen as an energy carrier will require low-cost, low-power hydrogen sensors. Toward this goal, penta-twinned palladium nanowires (Pd NWs) are synthesized and fabricated sensors from them by drop-casting. Pd NWs drop-cast onto an interdigitated electrode (IDE) gave a response of 0.3% to 1 vol.% H<sub>2</sub>, with response and recovery times of 12 and 20 s, respectively. However, they exhibited a negative response (decreased resistance) at low H<sub>2</sub> concentrations. Pd NWs on a paper substrate provided a tenfold higher response to 1 vol.% H<sub>2</sub>, with response and recovery times of 10 s each, but still exhibited negative response at low H<sub>2</sub> concentration. Exposing the Pd NW-on-paper sensor to ozone-generating UV light degraded the PVP used in Pd NW synthesis, eliminating the reverse sensing response, and providing a response of 5% to 1 vol.% H<sub>2</sub>, with response and recovery times of 15 s. This allowed reliable H<sub>2</sub> detection down to 100 ppm H<sub>2</sub>. Finally, coating the Pd NWs with a small amount of Pt (&lt;5%) reduced the response and recovery times to 5 s by catalyzing H<sub>2</sub> dissociation. This work provides a path to low-cost sensors to enable the safe use of H<sub>2</sub> as an energy carrier.</p>","PeriodicalId":100037,"journal":{"name":"Advanced Sensor Research","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2024-06-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/adsr.202400013","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141968109","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Electrochemical Surface Plasmon Resonance Sensing using a van der Waals Heterostructure 使用范德华异质结构的电化学表面等离子体共振传感技术
Pub Date : 2024-06-17 DOI: 10.1002/adsr.202400028
Robert Jungnickel, Kannan Balasubramanian

Coupling surface plasmon resonance (SPR) sensing with electrochemistry (EC) is a promising analytical strategy to obtain information about interfacial phenomena in heterogeneous reactions. Typical EC-SPR sensors utilize a metal film both as the plasmonic material and as the working electrode. In this configuration, the eigenmodulation of the plasmonic properties of the metal film under applied potential results in a background signal, which hampers the unambiguous interpretation of the sensor response due to redox reactions. Here, a new strategy is presented to overcome this disadvantage by using a van der Waals heterostructure (vdW-HS) as the working electrode. The vdW-HS comprises of a graphene / hexagonal boron nitride (hBN) stack on a gold film of a standard SPR sensor. It is shown here that the background signal is completely suppressed enabling the unambiguous analysis of SPR sensor response due to electrochemical reactions. It is further observed that the potential dependent plasmonic signals are not just a reproduction of the electrochemical current and subtle differences can be traced back to the diffusive nature of the redox active species. Finally, it is demonstrated that EC-SPR can be used as a complementary method to distinguish if the electrochemical response is mainly surface-bound or due to diffusion.

将表面等离子体共振(SPR)传感与电化学(EC)相结合是一种很有前途的分析策略,可用于获取有关异相反应中界面现象的信息。典型的 EC-SPR 传感器利用金属薄膜作为等离子材料和工作电极。在这种结构中,金属膜的质子特性在外加电位下的特征调制会产生背景信号,从而妨碍对氧化还原反应引起的传感器响应做出明确的解释。本文提出了一种新策略,通过使用范德华异质结构(vdW-HS)作为工作电极来克服这一缺点。vdW-HS 由标准 SPR 传感器金膜上的石墨烯/六方氮化硼(hBN)叠层组成。研究表明,本底信号被完全抑制,从而能够准确分析电化学反应引起的 SPR 传感器响应。进一步观察还发现,与电位相关的等离子信号并不仅仅是电化学电流的再现,其细微差别可追溯到氧化还原活性物种的扩散性质。最后,研究表明,EC-SPR 可以作为一种补充方法,用于区分电化学反应主要是表面结合还是由于扩散。
{"title":"Electrochemical Surface Plasmon Resonance Sensing using a van der Waals Heterostructure","authors":"Robert Jungnickel,&nbsp;Kannan Balasubramanian","doi":"10.1002/adsr.202400028","DOIUrl":"https://doi.org/10.1002/adsr.202400028","url":null,"abstract":"<p>Coupling surface plasmon resonance (SPR) sensing with electrochemistry (EC) is a promising analytical strategy to obtain information about interfacial phenomena in heterogeneous reactions. Typical EC-SPR sensors utilize a metal film both as the plasmonic material and as the working electrode. In this configuration, the eigenmodulation of the plasmonic properties of the metal film under applied potential results in a background signal, which hampers the unambiguous interpretation of the sensor response due to redox reactions. Here, a new strategy is presented to overcome this disadvantage by using a van der Waals heterostructure (vdW-HS) as the working electrode. The vdW-HS comprises of a graphene / hexagonal boron nitride (hBN) stack on a gold film of a standard SPR sensor. It is shown here that the background signal is completely suppressed enabling the unambiguous analysis of SPR sensor response due to electrochemical reactions. It is further observed that the potential dependent plasmonic signals are not just a reproduction of the electrochemical current and subtle differences can be traced back to the diffusive nature of the redox active species. Finally, it is demonstrated that EC-SPR can be used as a complementary method to distinguish if the electrochemical response is mainly surface-bound or due to diffusion.</p>","PeriodicalId":100037,"journal":{"name":"Advanced Sensor Research","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2024-06-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/adsr.202400028","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"142170258","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
期刊
Advanced Sensor Research
全部 Acc. Chem. Res. ACS Applied Bio Materials ACS Appl. Electron. Mater. ACS Appl. Energy Mater. ACS Appl. Mater. Interfaces ACS Appl. Nano Mater. ACS Appl. Polym. Mater. ACS BIOMATER-SCI ENG ACS Catal. ACS Cent. Sci. ACS Chem. Biol. ACS Chemical Health & Safety ACS Chem. Neurosci. ACS Comb. Sci. ACS Earth Space Chem. ACS Energy Lett. ACS Infect. Dis. ACS Macro Lett. ACS Mater. Lett. ACS Med. Chem. Lett. ACS Nano ACS Omega ACS Photonics ACS Sens. ACS Sustainable Chem. Eng. ACS Synth. Biol. Anal. Chem. BIOCHEMISTRY-US Bioconjugate Chem. BIOMACROMOLECULES Chem. Res. Toxicol. Chem. Rev. Chem. Mater. CRYST GROWTH DES ENERG FUEL Environ. Sci. Technol. Environ. Sci. Technol. Lett. Eur. J. Inorg. Chem. IND ENG CHEM RES Inorg. Chem. J. Agric. Food. Chem. J. Chem. Eng. Data J. Chem. Educ. J. Chem. Inf. Model. J. Chem. Theory Comput. J. Med. Chem. J. Nat. Prod. J PROTEOME RES J. Am. Chem. Soc. LANGMUIR MACROMOLECULES Mol. Pharmaceutics Nano Lett. Org. Lett. ORG PROCESS RES DEV ORGANOMETALLICS J. Org. Chem. J. Phys. Chem. J. Phys. Chem. A J. Phys. Chem. B J. Phys. Chem. C J. Phys. Chem. Lett. Analyst Anal. Methods Biomater. Sci. Catal. Sci. Technol. Chem. Commun. Chem. Soc. Rev. CHEM EDUC RES PRACT CRYSTENGCOMM Dalton Trans. Energy Environ. Sci. ENVIRON SCI-NANO ENVIRON SCI-PROC IMP ENVIRON SCI-WAT RES Faraday Discuss. Food Funct. Green Chem. Inorg. Chem. Front. Integr. Biol. J. Anal. At. Spectrom. J. Mater. Chem. A J. Mater. Chem. B J. Mater. Chem. C Lab Chip Mater. Chem. Front. Mater. Horiz. MEDCHEMCOMM Metallomics Mol. Biosyst. Mol. Syst. Des. Eng. Nanoscale Nanoscale Horiz. Nat. Prod. Rep. New J. Chem. Org. Biomol. Chem. Org. Chem. Front. PHOTOCH PHOTOBIO SCI PCCP Polym. Chem.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1