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On the Evaluation of Higher-Harmonic-Current Responses for High-Field Spectroscopies in Disordered Superconductors 无序超导体高场光谱高次电流响应的评价
Q3 PHYSICS, CONDENSED MATTER Pub Date : 2023-11-13 DOI: 10.3390/condmat8040095
Götz Seibold
We discuss a formalism that allows for the calculation of a higher-harmonic-current response to a strong applied electric field for disordered superconducting systems described on the basis of tight-binding models with on- and/or intersite interactions. The theory is based on an expansion of the density matrix in powers of the field amplitudes, where we solve the equation of motion for the individual components. This allows the evaluation of higher-order response functions on significantly larger lattices than one can achieve with a previously used approach, which is based on a direct temporal integration of the equation of motion for the complete density matrix. In the case of small lattices, where both methods can be applied by including also the contribution of collective modes, we demonstrate the agreement of the corresponding results.
我们讨论了一种形式,该形式允许计算高谐波电流响应对强电场的无序超导系统的响应,该响应基于具有场上和/或场间相互作用的紧密结合模型。该理论是基于密度矩阵的场振幅幂的展开,其中我们解决了单个分量的运动方程。这允许在更大的格上评估高阶响应函数,而不是使用以前使用的方法,该方法基于完整密度矩阵的运动方程的直接时间积分。在小格的情况下,两种方法都可以通过包括集体模态的贡献来应用,我们证明了相应结果的一致性。
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引用次数: 0
Experimental and Numerical Investigations on the Parameters of a Synchronous Machine Prototype with High-Temperature Superconductor Armature Windings 高温超导电枢绕组同步电机样机参数的实验与数值研究
Q3 PHYSICS, CONDENSED MATTER Pub Date : 2023-11-09 DOI: 10.3390/condmat8040094
Hocine Menana, Yazid Statra
In their applications in electrical machines, high-temperature superconductors (HTSs) are mainly used as inductors in synchronous machines due to the AC losses which can lead to high cryogenic costs. In this work, we show the possibility of their use as armature windings, handling some precautions. The approach is based on the combined use of modeling and measurements. The construction and the preliminary tests of a handmade prototype of an axial field HTS synchronous machine are presented. Several tests have been conducted at liquid nitrogen temperature. The measurements have been confirmed by modeling results. The preliminary tests on the prototype, in both modeling and measurements, are very promising.
高温超导体(HTSs)在电机中的应用主要是作为同步电机的电感,因为高温超导体的交流损耗会导致较高的低温成本。在这项工作中,我们展示了它们用作电枢绕组的可能性,并处理了一些注意事项。该方法基于建模和测量的结合使用。介绍了轴向磁场高温超导同步电机的手工样机的结构和初步试验。在液氮温度下进行了几次试验。模拟结果证实了测量结果。对原型机的初步测试,无论是建模还是测量,都非常有希望。
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引用次数: 0
Vortex Dynamics and Pinning in CaKFe4As4 Single Crystals from DC Magnetization Relaxation and AC Susceptibility 基于直流磁化弛豫和交流磁化率的CaKFe4As4单晶的涡旋动力学和钉钉
Q3 PHYSICS, CONDENSED MATTER Pub Date : 2023-10-29 DOI: 10.3390/condmat8040093
Alina M. Ionescu, Ion Ivan, Corneliu F. Miclea, Daniel N. Crisan, Armando Galluzzi, Massimiliano Polichetti, Adrian Crisan
Among various “families” of iron-based superconductors, the quite recently discovered AeAFe4As4 (where Ae is an alkali-earth metal and A is an alkali metal) has high critical current density, a very high upper critical field, and a low anisotropy, and has recently received much interest for the possibility of high magnetic field applications at the liquid hydrogen temperature. We have performed DC magnetization relaxation and frequency-dependent AC susceptibility measurements on high-quality single crystals of CaKFe4As4 with the aim of determining the pinning potential U*. The temperature dependence of U* displays a clear crossover between elastic creep and plastic creep. At temperatures around 27–28 K, U* has a very high value, up to 1200 K, resulting in an infinitesimally small probability of thermally activated flux jumps. From the dependence of the normalized pinning potential on irreversible magnetization, we have determined the creep exponents in the two creep regimes, which are in complete agreement with theoretical models. The estimation of the pinning potential from multifrequency AC susceptibility measurements was possible only near the critical temperature due to equipment limitations, and the resulting value is very close to the one that resulted from the magnetization relaxation data. Magnetic hysteresis loops revealed a second magnetization peak and very high values of the critical current density.
在各种铁基超导体“家族”中,最近发现的AeAFe4As4(其中Ae是碱土金属,A是碱金属)具有高临界电流密度,非常高的上临界场和低各向异性,并且最近因在液氢温度下高磁场应用的可能性而引起了人们的极大兴趣。我们对高质量的CaKFe4As4单晶进行了直流磁化弛豫和频率相关的交流磁化率测量,目的是确定钉钉电位U*。U*的温度依赖性在弹性蠕变和塑性蠕变之间表现出明显的交叉。在27-28 K左右的温度下,U*具有非常高的值,高达1200 K,导致热激活通量跳变的概率无穷小。根据归一化钉钉电位对不可逆磁化的依赖关系,我们确定了两种蠕变状态下的蠕变指数,这与理论模型完全一致。由于设备的限制,多频交流磁化率测量只能在临界温度附近估计钉钉电位,结果值与磁化弛豫数据的结果非常接近。磁滞回线显示出第二个磁化峰和很高的临界电流密度值。
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引用次数: 0
Obtaining Boron Carbide and Nitride Matrix Nanocomposites for Neutron-Shielding and Therapy Applications 制备用于中子屏蔽和治疗的碳化硼和氮基纳米复合材料
Q3 PHYSICS, CONDENSED MATTER Pub Date : 2023-10-28 DOI: 10.3390/condmat8040092
Levan Chkhartishvili, Shio Makatsaria, Nika Gogolidze, Otar Tsagareishvili, Tamaz Batsikadze, Matlab Mirzayev, Shalva Kekutia, Vladimer Mikelashvili, Jano Markhulia, Tamaz Minashvili, Ketevan Davitadze, Natia Barbakadze, Tamar Dgebuadze, Ketevan Kochiashvili, Rusudan Tsiskarishvili, Roin Chedia
The very high capture cross-section of (epi)thermal neutrons by the boron isotope 10B makes elemental boron and its compounds and composites prospective for serving as materials intensively interacting with neutron irradiation. In their nanostructured form, boron-rich materials reveal properties that improve their radiation-performance characteristics. In this regard, new technologies have been proposed for the synthesis of nanocomposites with matrices of boron carbide B4C and hexagonal boron nitride h-BN. For the first time, boron carbide-tungsten and hexagonal boron nitride–(iron,magnetite) composites were obtained, respectively, in the form of layered/sandwich structures of components B4C and W and h-BN nanopowders coated/intercalated with magnetic nanoclusters of iron Fe or magnetite Fe3O4. Studying of their chemical/phase composition, structure/morphology, and some other properties leads to the conclusion that the developed B4C–W and h-BN–(Fe,Fe3O4) composites would be useful for solving important problems of boron-based neutron shielding and BNCT (Boron Neutron Capture Therapy), such as attenuating the gamma-radiation accompanying the absorption of neutrons by 10B nuclei and targeted delivery of 10B nuclei, as BNCT therapeutic agents, to tumor tissues using control by an external magnetic field, respectively.
硼同位素10B对(epi)热中子的高捕获截面使得元素硼及其化合物和复合材料有望成为与中子辐照强烈相互作用的材料。在其纳米结构形式下,富硼材料显示出改善其辐射性能特征的特性。在此基础上,提出了以碳化硼B4C和六方氮化硼h-BN为基体制备纳米复合材料的新工艺。首次制备了碳化硼-钨复合材料和六方氮化硼-(铁、磁铁矿)复合材料,分别为B4C和W组分的层状/夹层结构,h-BN纳米粉末包被铁Fe或磁铁矿Fe3O4磁性纳米团簇。通过对B4C-W和h-BN - (Fe,Fe3O4)复合材料的化学/物相组成、结构/形貌及其它性能的研究,认为所制备的B4C-W和h-BN - (Fe,Fe3O4)复合材料可作为BNCT治疗剂,用于解决硼基中子屏蔽和BNCT(硼中子俘获治疗)的重要问题,如衰减伴随中子被10B核吸收的伽马辐射和靶向递送10B核等。分别利用外部磁场控制肿瘤组织。
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引用次数: 0
The Depairing Current Density of a Fe(Se,Te) Crystal Evaluated in Presence of Demagnetizing Factors 存在退磁因素时铁(硒,碲)晶体的依赖电流密度评估
Q3 PHYSICS, CONDENSED MATTER Pub Date : 2023-10-23 DOI: 10.3390/condmat8040091
Armando Galluzzi, Krastyo Buchkov, Vihren Tomov, Elena Nazarova, Antonio Leo, Gaia Grimaldi, Adrian Crisan, Massimiliano Polichetti
The effect of the demagnetizing factor, regarding the determination of the de-pairing current density Jdep, has been studied in the case of a Fe(Se,Te) crystal, using DC magnetic measurements as a function of a magnetic field (H) at different temperatures (T). First, the lower critical field Hc1(T) values were obtained, and the demagnetization effects acting on them were investigated after calculating the demagnetizing factor. The temperature behaviors of both the original Hc1 values and the ones obtained after considering the demagnetization effects (Hc1demag) were analyzed, and the temperature dependence of the London penetration depth λL(T) was obtained in both cases. In particular, the λL(T) curves were fitted with a power law dependence, indicating the presence of low-energy quasiparticle excitations. Furthermore, by plotting λL−2 as a function of T, we found that our sample behaves as a multigap superconductor, which is similar to other Fe-11 family iron-based compounds. After that, the coherence length ξ values were extracted, starting with the Hc2(T) curve. The knowledge of λL and ξ allowed us to determine the Jdep values and to observe how they are influenced by the demagnetizing factor.
本文以Fe(Se,Te)晶体为研究对象,在不同温度(T)下,利用直流磁测量值作为磁场(H)的函数,研究了退磁因子对解偶电流密度jdeep的影响。首先,得到了较低的临界场Hc1(T)值,计算出退磁因子后,研究了作用于其上的退磁效应。分析了原始Hc1值和考虑退磁效应后得到的Hc1值(Hc1demag)的温度行为,得到了两种情况下伦敦穿透深度λL(T)与温度的关系。特别是λL(T)曲线具有幂律依赖性,表明存在低能准粒子激发。此外,通过绘制λL−2作为T的函数,我们发现我们的样品表现为多隙超导体,这与其他Fe-11家族铁基化合物相似。之后,从Hc2(T)曲线开始提取相干长度ξ值。λL和ξ的知识使我们能够确定jdeep值,并观察它们如何受到退磁因素的影响。
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引用次数: 0
Effects of the Exciton Fine Structure Splitting on the Entanglement-Based Quantum Key Distribution 激子精细结构分裂对基于纠缠态的量子密钥分配的影响
Q3 PHYSICS, CONDENSED MATTER Pub Date : 2023-10-10 DOI: 10.3390/condmat8040090
Adrián Felipe Hernández-Borda, María Paula Rojas-Sepúlveda, Hanz Yecid Ramírez-Gómez
The reliable transmission of secure keys is one of the essential tasks to be efficiently accomplished by quantum information processing, and the use of entangled particles is a very important tool toward that goal. However, efficient production of maximally entangled states is still a challenge for further progress in quantum computing and quantum communication. In the search for optimal sources of entanglement, quantum dots have emerged as promising candidates, but the presence of dephasing in the generated entangled states raises questions about their real usefulness in large-scale quantum networks. In this work, we evaluate the effects of the exciton fine structure splitting, present in most quantum dot samples, on the fidelity of the BBM92 protocol for quantum key distribution. We find that the protocol’s performance is heavily impacted by such splitting and establish an upper limit for the product between the energy splitting and the exciton lifetime to have a dependable distributed key.
安全密钥的可靠传输是量子信息处理要高效完成的重要任务之一,而使用纠缠粒子是实现这一目标的重要工具。然而,最大纠缠态的高效产生仍然是量子计算和量子通信进一步发展的挑战。在寻找最佳纠缠源的过程中,量子点已经成为有希望的候选者,但是在产生的纠缠态中存在的去相态提出了它们在大规模量子网络中真正有用的问题。在这项工作中,我们评估了存在于大多数量子点样品中的激子精细结构分裂对量子密钥分发BBM92协议保真度的影响。我们发现这种分裂严重影响了协议的性能,并建立了能量分裂与激子寿命之间的乘积的上限,以获得可靠的分布式密钥。
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引用次数: 0
Suppression of Stacking Order with Doping in 1T-TaS2−xSex 掺杂对1T-TaS2−xSex层序的抑制
Q3 PHYSICS, CONDENSED MATTER Pub Date : 2023-10-10 DOI: 10.3390/condmat8040089
Sharon S. Philip, Despina Louca, Matthew B. Stone, Alexander I. Kolesnikov
In 1T-TaS2−xSex, the charge density wave (CDW) state features a star of David lattice that expands across layers as the system becomes commensurate upon cooling. The layers can also order along the c-axis, and different stacking orders have been proposed. Using neutron scattering on powder samples, we compared the stacking order previously observed in 1T-TaS2 when the system is doped with Se. While at low temperature, a 13c layer sequence stacking was observed in TaS2; this type of ordering was not evident with doping. Doping with Se results in a metallic state in which the Mott transition is suppressed, which may be linked to the absence of layer stacking.
在1T-TaS2−xSex中,电荷密度波(CDW)态的特征是戴维星晶格,当系统在冷却时变得相称时,它会跨层扩展。层也可以沿c轴排列,并提出了不同的堆叠顺序。通过对粉末样品的中子散射,我们比较了掺杂Se时在1T-TaS2中观察到的堆积顺序。低温时,TaS2出现13c层序堆积;这种排序在服用兴奋剂的情况下并不明显。掺杂硒导致金属态莫特跃迁被抑制,这可能与层堆积的缺失有关。
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引用次数: 0
Ultrafast Pump–Probe Spectroscopy in Organic Dirac Electron Candidate α-(BETS)2I3 有机狄拉克电子候选物α-(BETS)2I3的超快泵浦探测光谱
Q3 PHYSICS, CONDENSED MATTER Pub Date : 2023-10-10 DOI: 10.3390/condmat8040088
Satoshi Tsuchiya, Masato Katsumi, Ryuhei Oka, Toshio Naito, Yasunori Toda
Photo-induced carrier dynamics were measured in the organic Dirac electron candidate α-(BETS)2I3 to investigate why resistivity increases below TMI = 50 K. We found a change in carrier dynamics due to an insulating gap formation below T′ = 50 K. On the other hand, the relaxation time and polarization anisotropy of the observed dynamics differ from those in the charge-ordering (CO) state of the isostructural salt α-(ET)2I3. Based on the difference, it can be concluded that the insulating phase has a different origin than the CO state.
测量了有机狄拉克候选电子α-(BETS)2I3的光致载流子动力学,探讨了在TMI = 50 K以下电阻率增加的原因。我们发现,在T ' = 50 K以下,由于绝缘间隙形成,载流子动力学发生了变化。另一方面,观察到的弛豫时间和极化各向异性与同构盐α-(ET)2I3的电荷有序(CO)态不同。根据这一差异,可以得出绝缘相与CO态来源不同的结论。
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引用次数: 0
Superconducting and Mechanical Properties of the Tl0.8Hg0.2Ba2Ca2Cu3O9−δ Superconductor Phase Substituted by Lanthanum and Samarium Fluorides 氟化镧和氟化钐取代Tl0.8Hg0.2Ba2Ca2Cu3O9−δ超导体相的超导性和力学性能
Q3 PHYSICS, CONDENSED MATTER Pub Date : 2023-10-07 DOI: 10.3390/condmat8040087
Rola F. Khattar, Mohammed Anas, Ramadan Awad, Khulud Habanjar
This study investigated the impact of samarium and lanthanum fluorides (SmF3 and LaF3) on the physical and mechanical properties of Tl0.8Hg0.2Ba2Ca2−xRxCu3O9−δ−yFy superconducting phases (specifically the (Tl, Hg)-1223 phase), where R = Sm and La, with 0.00 ≤ x ≤ 0.10. The superconducting samples were synthesized using the solid-state reaction method. X-ray diffraction (XRD) verified the formation of the (Tl, Hg)-1223 phase without altering its tetragonal structure. Scanning electron micrographs (SEM) reveal the improvement of the grain size and inter-grain connectivity as Sm and La contents increased up to x=0.025. The electrical properties of (Tl, Hg)-1223 were studied using I-V and electrical resistivity measurements. Improved superconducting transition temperature (Tc) and transport critical current density (Jc) were observed up to x=0.025, beyond which they decreased substantially. Vickers microhardness (Hv) measurements were performed at room temperature to investigate their mechanical performance with various applied loads (0.49–9.80 N) and times (10–90 s). For both substitutions, the mechanical properties were enhanced up to an optimal value at x=0.025. All samples exhibited normal indentation size effect (ISE) behavior. The proportional sample resistance (PSR) model best explained Hv values among five theoretical models. Dislocation creep was the primary creep mechanism in the samples, according to indentation creep studies.
本研究研究了钐和氟化镧(SmF3和LaF3)对Tl0.8Hg0.2Ba2Ca2−xRxCu3O9−δ−yFy超导相(特别是(Tl, Hg)-1223相)物理力学性能的影响,其中R = Sm和La, 0.00≤x≤0.10。采用固相反应法制备了超导样品。x射线衍射(XRD)证实(Tl, Hg)-1223相的形成没有改变其四方结构。扫描电镜(SEM)显示,Sm和La含量增加到x=0.025时,晶粒尺寸和晶粒间连通性有所改善。采用I-V和电阻率法研究了(Tl, Hg)-1223的电学性质。在x=0.025范围内,超导转变温度(Tc)和输运临界电流密度(Jc)均有提高,超过该温度和输运临界电流密度则显著降低。在室温下进行维氏显微硬度(Hv)测量,以研究不同施加载荷(0.49-9.80 N)和时间(10-90 s)下的力学性能。对于两种替代材料,在x=0.025时,力学性能都提高到最佳值。所有样品均表现出正常的压痕尺寸效应(ISE)行为。在五个理论模型中,比例样品电阻(PSR)模型最能解释Hv值。根据压痕蠕变的研究,位错蠕变是试样中主要的蠕变机制。
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引用次数: 0
Position-Dependent Effective Mass and Asymmetry Effects on the Electronic and Optical Properties of Quantum Wells with Improved Rosen–Morse Potential 位置相关的有效质量和不对称性对改进罗森-莫尔斯势量子阱的电子和光学性质的影响
Q3 PHYSICS, CONDENSED MATTER Pub Date : 2023-10-05 DOI: 10.3390/condmat8040086
Esin Kasapoglu, Melike Behiye Yücel, Carlos A. Duque
In this study, we investigated, for the first time, the effects of the spatially varying effective mass, asymmetry parameter, and well width on the electronic and optical properties of a quantum well which has an improved Rosen–Morse potential. Calculations were made within the framework of the effective mass and parabolic band approximations. We have used the diagonalization method by choosing a wave function based on the trigonometric orthonormal functions to find eigenvalues and eigenfunctions of the electron confined within the improved Rosen–Morse potential. Our results show that the position dependence mass, asymmetry, and confinement parameters cause significant changes in the electronic and optical properties of the structure we focus on since these effects create a significant increase in electron energies and a blue shift in the absorption spectrum. The increase in energy levels enables the development of optoelectronic devices that can operate at wider wavelengths and absorb higher-energy photons. Through an appropriate choice of parameters, the Rosen–Morse potential offers, among many advantages, the possibility of simulating heterostructures close to surfaces exposed to air or vacuum, thus giving the possibility of substantially enriching the allowed optical transitions given the breaking of the system´s symmetries. Similarly, the one-dimensional Rosen–Morse potential model proposed here can be extended to one- and zero-dimensional structures such as core/shell quantum well wires and quantum dots. This offers potential advancements in fields such as optical communication, imaging technology, and solar cells.
在这项研究中,我们首次研究了空间变化的有效质量、不对称参数和阱宽度对具有改进的罗森-莫尔斯势的量子阱的电子和光学性质的影响。在有效质量和抛物线带近似的框架内进行了计算。我们采用对角化的方法,选择一个基于三角标准正交函数的波函数来求出限制在改进的罗森-莫尔斯势内的电子的本征值和本征函数。我们的研究结果表明,位置依赖、质量、不对称性和约束参数会导致我们所关注的结构的电子和光学性质发生显著变化,因为这些影响会导致电子能量的显著增加和吸收光谱的蓝移。能级的增加使光电器件的发展能够在更宽的波长下工作并吸收更高能量的光子。通过适当选择参数,罗森-莫尔斯势提供了许多优点,其中包括模拟接近暴露于空气或真空表面的异质结构的可能性,从而提供了在系统对称性破坏的情况下大量丰富允许的光学跃迁的可能性。同样,本文提出的一维罗森-莫尔斯势模型也可以推广到核/壳量子阱线和量子点等一维和零维结构。这为光通信、成像技术和太阳能电池等领域提供了潜在的进步。
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引用次数: 0
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Condensed Matter
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