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Effect of the Spatially-Varied Electron Mean Free Path on Vortex Matter in a Superconducting Pb Island Grown on Si (111) 空间变化电子平均自由程对硅上超导铅岛中涡旋物质的影响(111)
IF 1.7 Q3 PHYSICS, CONDENSED MATTER Pub Date : 2023-09-05 DOI: 10.3390/condmat8030077
Jesús González, Jader González, F. Durán, Carlos Salas, Jorge Gómez
In this work we report theoretical calculations of a superconducting island in a strong vortex confinement regime. The obtained results reveal the evolution of the superconducting condensate with an applied magnetic field, depending on the spatial profile of the electron mean-free path in the sample. The results of this study provide an insight about the emergent superconducting properties under such conditions, using the Ginzburg-Landau numerical simulations where spatial variation of thickness of the island and the corresponding variation of the mean free path, omnipresent in similar structures of Pb grown on Si (111), are taken into account. These results offer a new route to tailor superconducting circuits by nanoengineered mean free path, using for example the controlled ion-bombardment on thin films, benefiting from the here shown impact of the spatially-varying mean free path on the vortex distribution, phase of superconducting order parameter, and the critical fields.
在这项工作中,我们报道了在强涡旋约束条件下超导岛的理论计算。所获得的结果揭示了超导冷凝物随外加磁场的演变,这取决于样品中电子平均自由程的空间分布。这项研究的结果提供了关于在这种条件下涌现的超导性质的见解,使用Ginzburg-Landau数值模拟,其中考虑了岛厚度的空间变化和平均自由程的相应变化,这些变化在Si(111)上生长的Pb的类似结构中普遍存在。这些结果提供了一种通过纳米工程平均自由程定制超导电路的新途径,例如使用薄膜上的受控离子轰击,受益于这里所示的空间变化的平均自由程对涡流分布、超导阶参数的相位和临界场的影响。
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引用次数: 0
Hubbard Bands and Exotic States in Doped and Undoped Mott Systems: The Kotliar–Ruckenstein Representation 掺杂和未掺杂莫特系统中的哈伯德带和奇异态:Kotlyar-Ruckenstein表示
IF 1.7 Q3 PHYSICS, CONDENSED MATTER Pub Date : 2023-08-28 DOI: 10.3390/condmat8030075
V. Irkhin
The slave–particle representation is a promising method to treat the properties of exotic strongly correlated systems. We develop a unified approach to describe both the paramagnetic state with possible spin–liquid features and states with strong long-range or short-range magnetic order. Combining the Kotliar–Ruckenstein representation and fractionalized spin–liquid deconfinement picture, the Mott transition and Hubbard subbands are considered. The spectrum in the insulating state is significantly affected by the presence of the spinon spin–liquid spectrum and a hidden Fermi surface. Presenting a modification of the Kotliar–Ruckenstein representation in the spin–wave region, we treat the case of magnetic order, with special attention being paid to the half-metallic ferromagnetic state. The formation of small and large Fermi surfaces for doped current carriers in the antiferromagnetic state is also discussed.
从粒子表示是处理奇异强相关系统性质的一种很有前途的方法。我们开发了一种统一的方法来描述具有可能的自旋-液体特征的顺磁状态和具有强长程或短程磁序的状态。结合Kotlyar–Ruckenstein表示和分数化自旋-液体去约束图,考虑了Mott跃迁和Hubbard子带。绝缘状态下的光谱受到旋子自旋-液体光谱和隐藏费米表面的存在的显著影响。提出了对自旋波区Kotlyar–Ruckenstein表示的修改,我们处理了磁序的情况,特别注意半金属铁磁态。还讨论了反铁磁状态下掺杂电流载流子的小费米表面和大费米表面的形成。
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引用次数: 0
Properties of Blue Phosphorene Nanoribbon-P3HT Polymer Heterostructures: DFT First Principles Calculations 蓝色磷纳米带- p3ht聚合物异质结构的性质:DFT第一性原理计算
IF 1.7 Q3 PHYSICS, CONDENSED MATTER Pub Date : 2023-08-22 DOI: 10.3390/condmat8030074
Benita Turiján-Clara, J. Correa, M. Mora-Ramos, C. Duque
Recently, 2D phosphorus allotropes have arisen as possible candidates for technological applications among the family of the so-called Xene layered materials. In particular, the energy band structure of blue phosphorene (BP) exhibits a medium-size semiconductor gap that tends to widen in the case of using this material in the form of ribbons. BP nanoribbons have attracted recent interest for their implication in the improvement in efficiency of novel solar cells. On the other hand, compound poly (3-hexylthiophene) (P3HT) is used as the semiconducting core of organic field effect transistors owing to such useful features as high carrier mobility. Here, we theoretically investigate the electronic properties of a heterostructure combination of BP—in the form of nanoribbons—with a P3HT polymer chain on top in order to identify the features of band alignment. The work is performed using first principles calculations via DFT, employing different exchange correlation approaches for comparison: PBE, HSE06 and DFT-1/2. It is found that, under DFT-1/2, such a heterostructure has a type-II band alignment.
最近,2D磷同素异形体已经成为所谓Xene层状材料家族中技术应用的可能候选者。特别地,蓝色磷光体(BP)的能带结构表现出中等尺寸的半导体间隙,在以带的形式使用这种材料的情况下,该半导体间隙倾向于加宽。BP纳米带最近因其在提高新型太阳能电池效率方面的作用而引起人们的兴趣。另一方面,化合物聚(3-己基噻吩)(P3HT)由于高载流子迁移率等有用特性而被用作有机场效应晶体管的半导体核心。在这里,我们从理论上研究了纳米带形式的BP与顶部的P3HT聚合物链的异质结构组合的电子性质,以确定能带排列的特征。这项工作是通过DFT使用第一性原理计算进行的,使用不同的交换相关方法进行比较:PBE、HSE06和DFT-1/2。研究发现,在DFT-1/2下,这种异质结构具有II型能带排列。
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引用次数: 0
PbF2–CdF2–SrF2 Ternary Solid Solution: Crystal Growth and Investigation PbF2–CdF2–SrF2三元固溶体的晶体生长与研究
IF 1.7 Q3 PHYSICS, CONDENSED MATTER Pub Date : 2023-08-16 DOI: 10.3390/condmat8030073
I. I. Buchinskaya, I. O. Goryachuk, N. Sorokin, V. Sokolov, D. Karimov
Crystals based on alkaline earth metal difluorides are widely used optical materials. In this study, in order to expand the range of optical matrices, multicomponent Pb1−x−yCdxSryF2 (0.27 < x < 0.55, 0.06 < y < 0.18) solid solution crystals with a fluorite structure (sp. gr. Fm-3m) were grown from melt using the vertical directional crystallization technique for the first time. The densities and refractive indices of the grown crystals vary depending on the quantitative content components (x and y) in the ranges of 6.6039(5)–7.5232(5) g/cm3 and 1.6403–1.7084, respectively. The optical transmission and electrochemical impedance spectra were studied. The homogenous composition regions of non-cellular crystallization of this ternary solid solution at a crystallization rate of 6 mm/h and an interface temperature gradient of 80 deg/cm were experimentally determined as 0.30 < x < 0.35, 0 < y < 0.6. These grown crystalline materials may be of interest as high-density highly refractive cubic isomorphic hosts and low-temperature ionic conductors (~2 × 10−5 S/cm at room temperature) for various applications.
基于碱土金属二氟化物的晶体是广泛使用的光学材料。在本研究中,为了扩大光学基质的范围,首次使用垂直定向结晶技术从熔体中生长出具有萤石结构的多组分Pb1−x−yCdxSryF2(0.27<x<0.55,0.06<y<0.18)固溶体晶体(sp.gr.Fm-3m)。生长晶体的密度和折射率根据定量含量组分(x和y)的不同而变化,分别在6.6039(5)–7.5232(5)g/cm3和1.6403–1.7084的范围内。研究了其光透射光谱和电化学阻抗谱。该三元固溶体在6 mm/h的结晶速率和80°/cm的界面温度梯度下的非细胞结晶的均匀组成区域被实验确定为0.30
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引用次数: 0
Electric and Magnetic Fields Effects in Vertically Coupled GaAs/AlxGa1−xAs Conical Quantum Dots 垂直耦合GaAs/AlxGa1-xAs锥形量子点中的电场和磁场效应
IF 1.7 Q3 PHYSICS, CONDENSED MATTER Pub Date : 2023-08-15 DOI: 10.3390/condmat8030071
Ana María López Aristizábal, Fernanda Mora Rey, Á. Morales, J. A. Vinasco, C. Duque
Vertically coupled quantum dots have emerged as promising structures for various applications such as single photon sources, entangled quantum pairs, quantum computation, and quantum cryptography. We start with a structure composed of two vertically coupled GaAs conical quantum dots surrounded by AlxGa1−x, and the effects of the applied electric and magnetic fields on the energies are evaluated using the finite element method. In addition, the effects are evaluated by including the presence of a shallow-donor impurity. The electron binding energy behavior is analyzed, and the effects on the photoionization cross-section are studied. Calculations are carried out in the effective mass and parabolic conduction band approximations. Our results show a notable dependence on the electric and magnetic fields applied to the photoionization cross-section. In general, it has been observed that both the electric and magnetic fields are useful parameters for inducing blueshifts of the resonant photoionization cross-section structure, which is accompanied by a drop in its magnitude.
垂直耦合量子点在单光子源、纠缠量子对、量子计算和量子密码学等领域的应用前景十分广阔。我们从两个由AlxGa1−x包围的垂直耦合GaAs锥形量子点组成的结构开始,并使用有限元方法评估了外加电场和磁场对能量的影响。此外,通过包括浅层供体杂质的存在来评估效果。分析了电子结合能行为,并研究了其对光离截面的影响。计算是在有效质量和抛物线传导带近似下进行的。我们的研究结果表明,光电离截面与电场和磁场有显著的关系。总的来说,电场和磁场都是引起共振光电离截面结构蓝移的有用参数,蓝移的幅度会随之下降。
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引用次数: 0
Superlattices, Bonding-Antibonding, Fermi Surface Nesting, and Superconductivity 超晶格、键合反键、费米表面嵌套和超导性
IF 1.7 Q3 PHYSICS, CONDENSED MATTER Pub Date : 2023-08-15 DOI: 10.3390/condmat8030072
J. Alarco, I. Mackinnon
Raman and synchrotron THz absorption spectral measurements on MgB2 provide experimental evidence for electron orbital superlattices. In earlier work, we have detected THz spectra that show superlattice absorption peaks with low wavenumbers, for which spectral density evolves and intensifies after cooling below the superconducting transition temperature for MgB2. In this work, we show how these observations indicate a direct connection to superconducting properties and mechanisms. Bonding–antibonding orbital character is identified in calculated electronic band structures and Fermi surfaces consistent with superlattice structures along the c-axis. DFT calculations show that superlattice folding of reciprocal space generates Brillouin zone boundary reflections, Umklapp processes, and substantially enhances nesting relationships. Tight binding equations are compared with expected charge density waves from nesting relationships and adjusted to explicitly accommodate these linked processes. Systematic analysis of electronic band structures and Fermi surfaces allows for direct identification of Cooper pairing and the superconducting gap, particularly when the k-grid resolution of a calculation is suitably calibrated to structural parameters. Thus, we detail a robust and accurate DFT re-interpretation of BCS superconductivity for MgB2.
MgB2的拉曼光谱和同步加速器太赫兹吸收光谱测量为电子轨道超晶格提供了实验证据。在早期的工作中,我们已经检测到太赫兹光谱,其显示出具有低波数的超晶格吸收峰,在冷却到MgB2的超导转变温度以下后,其光谱密度演变并增强。在这项工作中,我们展示了这些观测结果如何表明与超导性质和机制的直接联系。在计算的电子能带结构和沿c轴与超晶格结构一致的费米表面中确定了键合-反键轨道特征。DFT计算表明,倒易空间的超晶格折叠产生布里渊区边界反射、Umklapp过程,并显著增强了嵌套关系。将紧密结合方程与嵌套关系中的预期电荷密度波进行比较,并进行调整以明确适应这些关联过程。电子能带结构和费米表面的系统分析允许直接识别库珀配对和超导间隙,特别是当计算的k网格分辨率被适当地校准到结构参数时。因此,我们详细介绍了对MgB2的BCS超导性的稳健和准确的DFT重新解释。
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引用次数: 0
The Transport and Optical Characteristics of a Metal Exposed to High-Density Energy Fluxes in Compressed and Expanded States of Matter 在物质压缩和膨胀状态下暴露于高密度能量流的金属的输运和光学特性
IF 1.7 Q3 PHYSICS, CONDENSED MATTER Pub Date : 2023-08-11 DOI: 10.3390/condmat8030070
Nikolay B. Volkov, A. I. Lipchak
This article presents a theoretical study of the optical and transport properties of metals. Iron, as an example, was used to discuss, through a theoretical description, the peculiarities of these properties in the compressed and expanded states under the influence of high-density energy fluxes. By solving the semi-classical Boltzmann equation for conduction electrons for a broad range of densities and temperatures, the expressions of electrical conductivity, electronic thermal conductivity, and thermoelectric coefficient calculations were derived. The real and imaginary parts of the iron permittivity and the energy absorption coefficient for the first and second harmonics of Nd:YAG laser radiation were obtained. The calculation peculiarities of the metal’s optical characteristics of matter in an expanded state in a broad range of densities and temperatures were considered. The analysis of the obtained results shows their agreement with the theoretical description for cases of ideal non-degenerate and dense degenerate electron plasmas. It is shown that the behavior of the electrical conductivity and optical characteristics in the critical and supercritical regions of density and temperature are in agreement with the known experimental results.
本文对金属的光学性质和输运性质进行了理论研究。以铁为例,通过理论描述,讨论了在高密度能量通量影响下,压缩和膨胀状态下这些性质的特性。通过求解在宽密度和温度范围内传导电子的半经典Boltzmann方程,导出了电导率、电子热导率和热电系数的计算表达式。获得了Nd:YAG激光辐射一次谐波和二次谐波的铁介电常数和能量吸收系数的实部和虚部。考虑了在宽密度和温度范围内膨胀态物质的金属光学特性的计算特性。对所得结果的分析表明,它们与理想非简并和稠密简并电子等离子体的理论描述是一致的。结果表明,在密度和温度的临界和超临界区域,电导率和光学特性的行为与已知的实验结果一致。
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引用次数: 0
ETPTA Inverse Photonic Crystals for the Detection of Alcohols ETPTA逆光子晶体用于醇类的检测
IF 1.7 Q3 PHYSICS, CONDENSED MATTER Pub Date : 2023-08-08 DOI: 10.3390/condmat8030068
M. Ashurov, S. Kutrovskaya, A. Baranchikov, S. Klimonsky, A. Kavokin
We developed a comparatively simple and inexpensive approach for the determination of the concentration of alcohols in water. The method is based on the study of the optical properties of ethoxylate trimethylolpropane triacrylate (ETPTA) inverse photonic crystals (IPhCs). The position of the transmission minimum associated with the first photonic stop band (PSB) is used as the analytical signal. The PSB position depends on the swelling degree of ETPTA photoresist and the refractive index of the tested alcohols and their mixtures with water. The signal increases linearly with increasing concentration of ethylene glycol and increases nonlinearly but monotonically with the concentration of methanol and ethanol in water. Sensitivity to alcohols, in the case of the ethylene glycol–water mixtures, reached about 0.55 nm/v.% or 560 nm/RIU (refractive index unit), which is sufficient for various applications in bio/chemical detection and environmental monitoring.
我们开发了一种比较简单和便宜的方法来测定水中醇的浓度。该方法是基于对乙氧基酸三甲基丙烷三丙烯酸酯(ETPTA)逆光子晶体(IPhCs)光学性质的研究。利用与第一光子停止带(PSB)相关的传输最小值的位置作为分析信号。PSB的位置取决于ETPTA光刻胶的膨胀程度和被测醇及其与水的混合物的折射率。信号随乙二醇浓度的增加呈线性增加,随甲醇和乙醇浓度的增加呈非线性单调增加。在乙二醇-水混合物的情况下,对醇的灵敏度达到约0.55 nm/v。%或560nm /RIU(折射率单位),足以用于生物/化学检测和环境监测的各种应用。
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引用次数: 1
Effect of External Fields on the Electronic and Optical Properties in ZnTe/CdSe and CdSe/ZnTe Spherical Quantum Dots 外加场对ZnTe/CdSe和CdSe/ZnTe球形量子点电子和光学性质的影响
IF 1.7 Q3 PHYSICS, CONDENSED MATTER Pub Date : 2023-08-02 DOI: 10.3390/condmat8030066
Rafael G. Toscano-Negrette, José C. León-González, J. A. Vinasco, Á. Morales, M. Mora-Ramos, C. Duque
A theoretical analysis was conducted to examine the electronic and optical properties of a confined electron and a hole in a type-II core-shell spherical quantum dot composed of CdSe/ZnTe and ZnTe/CdSe. The Schrödinger equation for the electron and the hole was numerically solved using COMSOL-Multiphysics software in the 2D axisymmetric module, which employs the finite element method under the effective mass approximation. A Fortran code was utilized to calculate excitonic energy, specifically designed to solve the Coulomb integral. The calculations encompassed variations in the inner radius (R1), as well as variations in the electric (Fz) and magnetic (B) fields along the z-axis. The absorption coefficients were determined for transitions between the hole and electron ground states, considering z-polarized incident radiation. Including a magnetic field increases the transition energy, consequently causing the absorption peaks to shift toward the blue region of the spectrum. On the other hand, the electric field decreased the overlap of the electron and hole wavefunctions. As a result, the amplitude of the absorption peaks decreased with an increase in the electric field.
对由CdSe/ZnTe和ZnTe/CdSe组成的II型核壳球形量子点中的受限电子和空穴的电子和光学性质进行了理论分析。使用COMSOL Multiphysics软件在二维轴对称模块中对电子和空穴的薛定谔方程进行了数值求解,该模块采用有效质量近似下的有限元方法。使用Fortran代码计算激子能量,该代码专门用于求解库仑积分。计算包括内半径(R1)的变化,以及沿z轴的电场(Fz)和磁场(B)的变化。考虑z偏振入射辐射,确定了空穴基态和电子基态之间跃迁的吸收系数。包括磁场会增加跃迁能量,从而导致吸收峰向光谱的蓝色区域移动。另一方面,电场减少了电子和空穴波函数的重叠。结果,吸收峰的振幅随着电场的增加而减小。
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引用次数: 0
Influence of Frustration Effects on the Critical Current of DC SQUID 挫折效应对直流SQUID临界电流的影响
IF 1.7 Q3 PHYSICS, CONDENSED MATTER Pub Date : 2023-07-28 DOI: 10.3390/condmat8030065
I. Askerzade
In this paper, we conducted the calculation of the critical current of DC SQUID based on the Josephson junction on a multi-band superconductor with frustration effect. It is shown that the critical current of DC SQUID on the frustrated multi-band superconductor with a small geometrical inductance of the loop is determined by the supercurrent amplitude in different channels and by the external magnetic field. In the case of a DC SQUID with high inductance, frustration effects can be ignored.
本文基于具有受挫效应的多带超导体上的Josephson结,计算了直流SQUID的临界电流。结果表明,在小几何电感回路受挫多带超导体上,直流SQUID的临界电流由不同通道的超电流幅值和外加磁场决定。对于高电感的直流SQUID,可以忽略挫折效应。
{"title":"Influence of Frustration Effects on the Critical Current of DC SQUID","authors":"I. Askerzade","doi":"10.3390/condmat8030065","DOIUrl":"https://doi.org/10.3390/condmat8030065","url":null,"abstract":"In this paper, we conducted the calculation of the critical current of DC SQUID based on the Josephson junction on a multi-band superconductor with frustration effect. It is shown that the critical current of DC SQUID on the frustrated multi-band superconductor with a small geometrical inductance of the loop is determined by the supercurrent amplitude in different channels and by the external magnetic field. In the case of a DC SQUID with high inductance, frustration effects can be ignored.","PeriodicalId":10665,"journal":{"name":"Condensed Matter","volume":" ","pages":""},"PeriodicalIF":1.7,"publicationDate":"2023-07-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"41730557","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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Condensed Matter
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