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A Framework for Developing Tools to Predict PFAS Physical–Chemical Properties and Mass-Partitioning Parameters 开发全氟辛烷磺酸物理化学特性和质量分配参数预测工具的框架
Pub Date : 2024-08-02 DOI: 10.3390/environments11080164
Mark L. Brusseau
A framework for developing predictive models for PFAS physical–chemical properties and mass-partitioning parameters is presented. The framework is based on the objective of developing tools that are of sufficient simplicity to be used rapidly and routinely for initial site investigations and risk assessments. This is accomplished by the use of bespoke PFAS-specific QSPR models. The development of these models entails aggregation and curation of measured data sets for a target property or parameter, supplemented by estimates produced with quantum–chemical ab initio predictions. The application of bespoke QSPR models for PFAS is illustrated with several examples, including partitioning to different interfaces, uptake by several fish species, and partitioning to four different biological materials. Reasonable correlations to molar volume were observed for all systems. One notable observation is that the slopes of all of the regression functions are similar. This suggests that the partitioning processes in all of these systems are to some degree mediated by the same mechanism, namely hydrophobic interaction. Special factors and elements requiring consideration in the development of predictive models are discussed, including differences in bulk-phase versus interface partitioning processes.
本文介绍了一个用于开发全氟辛烷磺酸物理化学特性和质量分配参数预测模型的框架。该框架的目标是开发足够简单的工具,以便快速、常规地用于初步现场调查和风险评估。这是通过使用定制的 PFAS 专用 QSPR 模型来实现的。这些模型的开发需要对目标属性或参数的测量数据集进行汇总和整理,并辅以量子化学非初始预测得出的估计值。本文以几个实例说明了定制 QSPR 模型在全氟辛烷磺酸中的应用,包括不同界面的分配、几种鱼类的吸收以及四种不同生物材料的分配。在所有系统中都观察到了与摩尔体积的合理相关性。一个值得注意的现象是,所有回归函数的斜率都很相似。这表明,所有这些系统中的分配过程在某种程度上都是由相同的机制(即疏水作用)介导的。讨论了在开发预测模型时需要考虑的特殊因素和要素,包括体相分配过程与界面分配过程的差异。
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引用次数: 0
Impact of the September 2023 Storm Daniel and Subsequent Flooding in Thessaly (Greece) on the Natural and Built Environment and on Infectious Disease Emergence 希腊塞萨利 2023 年 9 月丹尼尔风暴及随后的洪水对自然环境和建筑环境以及传染病发生的影响
Pub Date : 2024-08-02 DOI: 10.3390/environments11080163
Spyridon Mavroulis, Maria Mavrouli, Efthymios Lekkas, Athanasios Tsakris
The storm Daniel and subsequent floods hit the Region of Thessaly (Greece) in early September 2023, causing extensive damage to the built environment (buildings, networks, and infrastructure), the natural environment (water bodies and soil), and the population (fatalities, injured, homeless, and displaced people). Additionally, the conditions and factors favorable for indirect public health impact (infectious diseases) emerged in the flood-affected communities. The factors had to do with infectious diseases from rodents and vectors, injuries, respiratory infections, water contamination, flood waste and their disposal sites as well as structural damage to buildings and the failures of infrastructure. The conditions that evolved necessitated the mobilization of the Civil Protection and Public Health agencies not only to cope with the storm and subsequent floods but also to avoid and manage indirect public health impact. The instructions provided to affected residents, health experts, and Civil Protection staff were consistent with the best practices and lessons learned from previous disasters. The emphasis should be on training actions for competent agencies, as well as education and increasing the awareness of the general population. Non-structural and structural measures should be implemented for increasing the climate resilience of infrastructures including the health care systems within a One Health approach.
2023 年 9 月初,丹尼尔风暴和随后的洪水袭击了希腊塞萨利大区,对建筑环境(建筑、网络和基础设施)、自然环境(水体和土壤)和人口(死亡、受伤、无家可归和流离失所者)造成了广泛破坏。此外,受洪灾影响的社区还出现了有利于间接影响公众健康(传染病)的条件和因素。这些因素涉及啮齿动物和病媒引起的传染病、受伤、呼吸道感染、水污染、洪水垃圾及其处理场所,以及建筑物结构性损坏和基础设施故障。在这种情况下,民防和公共卫生机构必须动员起来,不仅要应对暴风雨和随后的洪水,还要避免和管理对公众健康的间接影响。向受灾居民、卫生专家和民防人员提供的指示与以往灾害中的最佳做法和经验教训是一致的。重点应放在对主管机构的培训行动以及教育和提高普通民众的认识上。应采取非结构性和结构性措施,在 "一个健康 "方法中提高包括医疗保健系统在内的基础设施的气候适应能力。
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引用次数: 0
Enhancing Swine Wastewater Treatment: A Sustainable and Systematic Approach through Optimized Chemical Oxygen Demand/Sulfate Mass Ratio in Attached-Growth Anaerobic Bioreactor 加强猪废水处理:附着生长厌氧生物反应器中优化化学需氧量/硫酸盐质量比的可持续系统方法
Pub Date : 2024-08-01 DOI: 10.3390/environments11080162
Mehdi Lamssali, Shobha Mantripragada, Dongyang Deng, Lifeng Zhang
The swine industry generates millions of gallons (thousands of cubic meters) of wastewater every day, posing significant environmental risk due to high concentrations of organics and nutrients. This study aims to investigate the effectiveness of attached-growth anaerobic bioreactors for treating swine wastewater by utilizing sulfate-reducing bacteria, focusing on the impact of chemical oxygen demand (COD)/sulfate mass ratios on organics degradation. A series of lab-scale anaerobic bioreactors were employed to treat swine wastewater for a 14-day period. The study evaluated changes in pH, acidity, alkalinity, COD, sulfate, and various nutrients along with total suspended solids (TSS) and volatile suspended solids (VSS) before and after treatment. At a COD/sulfate mass ratio of 2:1, the bioreactors achieved optimum removal efficiencies of 80% for TSS, 83% for VSS, 86–88% for COD, 82–87% for sulfate, 73% for sulfide, and 73% for sulfite. The nutrient removal efficiency was 67% for nitrate and 72% for nitrite. The acidity and alkalinity were effectively controlled, with alkalinity values reaching up to 2161 ± 92.5 mg/L and pH within the range of 7–7.24. The findings demonstrated that anaerobic bioreactor at a COD/sulfate mass ratio of 2:1 significantly enhanced the degradation of organic matter coupling with sulfate reduction in swine wastewater, providing an efficient and sustainable treatment method.
养猪业每天产生数百万加仑(数千立方米)的废水,由于含有高浓度的有机物和营养物质,对环境造成了严重危害。本研究旨在调查附着生长厌氧生物反应器利用硫酸盐还原菌处理猪场废水的效果,重点关注化学需氧量(COD)/硫酸盐质量比对有机物降解的影响。一系列实验室规模的厌氧生物反应器被用来处理猪废水,为期 14 天。研究评估了处理前后 pH 值、酸度、碱度、化学需氧量、硫酸盐、各种营养物质以及总悬浮固体 (TSS) 和挥发性悬浮固体 (VSS) 的变化。在化学需氧量/硫酸盐质量比为 2:1 时,生物反应器对总悬浮固体的最佳去除率为 80%,挥发性悬浮固体为 83%,化学需氧量为 86-88%,硫酸盐为 82-87%,硫化物为 73%,亚硫酸盐为 73%。硝酸盐和亚硝酸盐的营养物去除率分别为 67% 和 72%。酸度和碱度得到了有效控制,碱度值达到 2161 ± 92.5 mg/L,pH 值在 7-7.24 范围内。研究结果表明,在 COD/硫酸盐质量比为 2:1 的条件下,厌氧生物反应器能显著提高猪场废水中有机物的降解和硫酸盐的还原,提供了一种高效、可持续的处理方法。
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引用次数: 0
Honeybees and the One Health Approach 蜜蜂与 "统一健康方案
Pub Date : 2024-07-26 DOI: 10.3390/environments11080161
Joana C. Prata, Paulo Martins da Costa
The One Health approach recognizes the interconnectedness between human, animal, and environmental health. Honeybees (Apis mellifera) embody this framework due to their crucial role in ecosystems, food production, and susceptibility to contaminants. Despite their suitability for a One Health approach, there is a lack of research showcasing the multidisciplinary impacts and contributions of bees. The objective of this work is to explore the application of the One Health approach to bees through a narrative review. This work highlights the contribution of bees to history and culture, economy, medicine, nutrition, food security, and the functioning of ecosystems. It also demonstrates that bee health is affected by land management, agricultural practices, environmental contaminants, nutritional resource availability, predators and diseases, weather, climate patterns, and beekeeping practices. This complex system is highly influenced by policy and beekeeping practices, which will benefit animal health directly and environmental and human health indirectly. Thus, the protection of bees should be prioritized.
统一健康 "方法承认人类、动物和环境健康之间的相互联系。蜜蜂(Apis mellifera)在生态系统、食品生产和易受污染物影响方面发挥着至关重要的作用,因此体现了这一框架。尽管蜜蜂适用于 "同一健康 "方法,但目前缺乏展示蜜蜂的多学科影响和贡献的研究。这项工作的目的是通过叙述性综述探索 "同一健康 "方法在蜜蜂中的应用。这项工作强调了蜜蜂对历史和文化、经济、医药、营养、粮食安全以及生态系统功能的贡献。它还表明,蜜蜂的健康受到土地管理、农业实践、环境污染物、营养资源可用性、天敌和疾病、天气、气候模式以及养蜂实践的影响。这一复杂系统受政策和养蜂实践的影响很大,这将直接有利于动物健康,间接有利于环境和人类健康。因此,应优先保护蜜蜂。
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引用次数: 0
A Novel eDNA-Based Approach for the Monitoring and Management of the Endangered Beluga (Huso huso, Linnaeus, 1758) and Adriatic (Acipenser naccarii, Bonaparte, 1836) Sturgeon 基于 eDNA 的监测和管理濒危白鲟(Huso huso,林尼厄斯,1758 年)和亚得里亚海鲟(Acipenser naccarii,波拿巴,1836 年)的新方法
Pub Date : 2024-07-23 DOI: 10.3390/environments11080160
Caterina Maria Antognazza, Fausto Ramazzotti, Antonia Bruno, Andrea Galimberti, Monica Di Francesco, Serena Zaccara
Beluga sturgeon (Huso huso Linnaeus, 1758, acipenseridae) and Adriatic sturgeon (Acipenser naccarii, Bonaparte, 1836, acipenseridae) within the Po River basin have been recently assessed for the IUCN Red List of Threatened Species and were found to be Extinct in the Wild and Critically Endangered, respectively. Significant declines in both species’ abundance have spurred major research efforts and management actions in recent decades. Recently, specific actions have been conducted to recover habitat connectivity through projects of river defragmentation and reintroduction plans have been implemented for both sturgeon species. To manage effective conservation efforts, knowledge of a species’ distribution and abundance is critical, especially for adult sturgeon that are able to move hundreds of kilometers away from release sites. Here, two new quantitative PCR (qPCR) assays to detect beluga sturgeon and Adriatic sturgeon environmental DNA (eDNA) in water samples have been developed with the goal of providing an alternative method to monitor their presence. Two Taqman-based assays targeting the mitochondrial cytochrome b region were developed and showed no amplification of other related and co-occurring fishes. A mesocosm within the Ticino Park on the Ticino River (a main tributary of the Po River), where both species are bred, was used to develop and validate the assays. The LOQ for H. huso assay corresponded to Ct = 41 (7.33 × 107 DNA counts/µL of reaction) and for A. naccarrii it was Ct = 37 (2.23 × 1016 DNA counts/µL of reaction). Additionally, water samples were taken from the discard drainage, which flows directly into the Ticino River, testing positive detection of eDNA within a distance of up to 2 km. Overall, the results suggested that the two assays developed in this study could represent a promising new tool for monitoring both beluga and Adriatic sturgeon.
最近,世界自然保护联盟(IUCN)濒危物种红色名录对波河流域的白鲟(Huso huso Linnaeus, 1758, acipenseridae)和亚得里亚海鲟(Acipenser naccarii, Bonaparte, 1836, acipenseridae)进行了评估,发现它们分别处于野外灭绝和极度濒危状态。近几十年来,这两个物种数量的显著下降促使了大量的研究工作和管理行动。最近,已采取具体行动,通过河流破碎化项目恢复栖息地的连通性,并为这两种鲟鱼实施了重新引入计划。要管理有效的保护工作,了解物种的分布和丰度至关重要,尤其是对于能够从释放地点移动数百公里的成年中华鲟而言。在此,我们开发了两种新的定量 PCR(qPCR)检测方法来检测水样中的白鲟和亚得里亚海鲟环境 DNA(eDNA),目的是提供一种替代方法来监测它们的存在。针对线粒体细胞色素 b 区开发了两种基于 Taqman 的检测方法,结果表明没有对其他相关鱼类和共生鱼类进行扩增。在提契诺河(波河的一条主要支流)上的提契诺公园内的一个中观生态环境中,这两种鱼类都在此繁衍生息。H. huso 的最低检测限为 Ct = 41(7.33 × 107 DNA 计数/微升反应),A. naccarrii 的最低检测限为 Ct = 37(2.23 × 1016 DNA 计数/微升反应)。此外,还从直接流入提契诺河的废弃排水沟中采集了水样,检测到 2 公里范围内的 eDNA 检测呈阳性。总之,研究结果表明,本研究中开发的两种检测方法是监测白鲟和亚得里亚海鲟鱼的一种很有前途的新工具。
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引用次数: 0
A Review of Grease Trap Waste Management in the US and the Upcycle as Feedstocks for Alternative Diesel Fuels 美国油脂分离器废物管理及作为替代柴油燃料原料的再循环回顾
Pub Date : 2024-07-23 DOI: 10.3390/environments11080159
Andres Mata, Junsong Zhang, Joshua Pridemore, Kevin Johnson, Nathan Holliday, Art Helmstetter, Mingming Lu
As byproducts generated by commercial and domestic food-related processes, FOGs (fats, oils, and grease) are the leading cause of sewer pipe blockages in the US and around the world. Grease trap waste (GTW) is a subcategory of FOG currently disposed of as waste, resulting in an economic burden for GTW generators and handlers. This presents a global need for both resource conservation and carbon footprint reduction, particularly through increased waste upcycling. Therefore, it is critical to better understand current GTW handling practices in the context of the urban food–energy–water cycle. This can be accomplished with firsthand data collection, such as onsite visits, phone discussions, and targeted questionnaires. GTW disposal methods were found to be regional and correspond to key geographical locations, with landfill operations mostly practiced in the Midwest regions, incineration mainly in the Northeast and Mid-Atlantic regions, and digestion mainly in the West of the US. Select GTW samples were analyzed to evaluate their potential reuse as low-cost feedstocks for biodiesel or renewable diesel, which are alternatives to petroleum diesel fuels. Various GTW lipid extraction technologies have been reviewed, and more studies were found on converting GTW into biodiesel rather than renewable diesel. The challenges for these two pathways are the high sulfur content in biodiesel and the metal contents in renewable diesel, respectively. GTW lipid extraction technologies should overcome these issues while producing minimum-viable products with higher market values.
作为商业和家庭食品相关流程产生的副产品,FOG(脂肪、油和油脂)是造成美国和世界各地下水管道堵塞的主要原因。隔油池废物 (GTW) 是目前作为废物处理的 FOG 的一个子类别,给隔油池废物的产生者和处理者造成了经济负担。这就提出了保护资源和减少碳足迹的全球需求,特别是通过增加废物的再循环利用。因此,在城市食品-能源-水循环的背景下,更好地了解当前 GTW 的处理方法至关重要。这可以通过收集第一手数据来实现,如现场访问、电话讨论和有针对性的问卷调查。研究发现,GTW 的处理方法具有区域性,并与主要地理位置相对应,其中填埋作业主要在美国中西部地区,焚烧作业主要在美国东北部和大西洋中部地区,而消化作业主要在美国西部地区。对部分 GTW 样品进行了分析,以评估其作为生物柴油或可再生柴油低成本原料的再利用潜力,生物柴油或可再生柴油是石油柴油燃料的替代品。对各种 GTW 脂肪提取技术进行了审查,发现更多的研究涉及将 GTW 转化为生物柴油而非可再生柴油。这两种途径所面临的挑战分别是生物柴油中的高硫含量和可再生柴油中的金属含量。GTW 脂质提取技术应克服这些问题,同时生产出具有更高市场价值的最低可行产品。
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引用次数: 0
Characterization of the Dominant Stages at Which Gas Flaring Is Introduced: Impacts and Policy Options to Ameliorate Them 天然气燃烧的主要阶段特征:影响及改善影响的政策选择
Pub Date : 2024-07-22 DOI: 10.3390/environments11070158
Nwabueze Emekwuru
Information on associated gas flaring in the Niger Delta is analyzed to characterize the various stages in the lifecycle of an oil exploration and production facility through which gas flaring is introduced into an area, leading to ecological, health, and economic impacts, and possible policies and implementation strategies for the reduction of the flared gas are offered. Gas flaring is currently occurring at a rate of 5318 million m3 per year in the Niger Delta region. The impacts of gas flaring on the ecological, human, and economic systems include poor air quality, acid rain, and soil degradation. Other impacts include decreased crop yield, increased incidences of respiratory diseases amongst inhabitants in the area, and losses of billions of USD yearly in economic costs. Three dominant stages in the introduction of gas flaring are characterized in this study, using the concept of the management of the invasion of non-native species into an ecosystem and it is determined that the cheapest method of minimizing gas flaring is to incorporate mitigation measures during the design stage of the oil exploration/production facility, rather than after flaring has commenced, as is the common emphasis. During the early periods of oil production, gas flaring is largely localized, and the gas utilization measures can still be implemented to good effect. However, once the facility is established, gas flaring becomes pervasive, stretching kilometers beyond the flare points. Current policies like the imposition of flare-out years on the oil producers have helped, but they have been insufficient as the intensity of gas flaring in the region continues at double the average global levels. Working with relevant stakeholders, a realistic flare-out deadline should be agreed upon, clear and specific gas flaring legislation should be drawn up that includes measures to mitigate gas flaring for each proposed oil facility, and proper data collection and management services would enable the implementation of the policies to be based on robust evidence. These policies would shift the costs of gas flaring away from the inhabitants of the region back to the operators of the facilities that are the sources of the flares.
对尼日尔三角洲伴生天然气燃烧的信息进行了分析,以确定石油勘探和生产设施生命周期各阶段的特点,通过这些阶段,天然气燃烧被引入一个地区,导致生态、健康和经济影响,并提出了减少天然气燃烧的可能政策和实施策略。目前,尼日尔三角洲地区的天然气燃烧率为每年 5.318 亿立方米。天然气燃烧对生态、人类和经济系统的影响包括空气质量差、酸雨和土壤退化。其他影响还包括农作物减产、该地区居民呼吸道疾病发病率上升以及每年数十亿美元的经济损失。本研究采用非本地物种入侵生态系统的管理概念,对引入天然气燃烧的三个主要阶段进行了描述,并确定最大限度减少天然气燃烧的最经济方法是在石油勘探/生产设施的设计阶段就纳入缓解措施,而不是像通常强调的那样在燃烧开始后才采取。在石油生产初期,天然气燃烧主要集中在局部地区,天然气利用措施的实施仍能取得良好效果。然而,一旦设施建成,天然气燃烧就会变得无处不在,甚至会延伸到燃烧点以外的数公里之外。对石油生产商规定燃烧年限等现行政策有所帮助,但还不够,因为该地区的天然气燃烧强度仍然是全球平均水平的两倍。应与相关利益攸关方合作,商定一个切实可行的天然气燃烧淘汰期限,制定明确具体的天然气燃烧立法,其中包括针对每个拟建石油设施减少天然气燃烧的措施,并提供适当的数据收集和管理服务,使政策的实施建立在可靠证据的基础上。这些政策将把天然气燃烧的成本从该地区居民身上转移回作为燃烧源的设施运营商身上。
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引用次数: 0
The Impact of Air Pollution from Industrial Fires in Urban Settings: Monitoring, Modelling, Health, and Environmental Justice Perspectives 城市环境中工业火灾造成的空气污染的影响:监测、建模、健康和环境正义视角
Pub Date : 2024-07-21 DOI: 10.3390/environments11070157
Michael E. Deary, Simon D. Griffiths
Industrial fires at facilities including waste management sites, warehouses, factories, chemical works, and fuel storage depots are relatively frequent occurrences. Often, these fires occur adjacent to urban communities and result in ground-level airborne pollutant concentrations that are well above guideline values. Land, water, livestock, and crops may also be contaminated by the emissions and by firefighting activities. Moreover, impacted communities tend to have a higher proportion of minority ethnic populations as well as individuals with underlying health vulnerabilities and those of lower socio-economic status. Nevertheless, this is an aspect of air quality that is under-researched, and so this review aims to highlight the public health hazards associated with industrial fires and the need for an effective, coordinated, public health response. We also review the range of monitoring techniques that have been utilised in such fires and highlight the role of dispersion modelling in predicting plume trajectories and in estimating population exposure. We recommend establishing 1 h guideline values for particulate matter to facilitate timely public health interventions, and we highlight the need to review regulatory and technical controls for sites prone to fires, particularly in the waste sector.
包括废物管理场所、仓库、工厂、化工厂和燃料储存库在内的设施发生工业火灾的频率相对较高。这些火灾通常发生在城市社区附近,导致地面空气中的污染物浓度远高于指导值。土地、水、牲畜和农作物也可能受到排放物和灭火活动的污染。此外,受影响的社区往往有更多的少数民族人口、有潜在健康隐患的人和社会经济地位较低的人。尽管如此,这仍是空气质量研究不足的一个方面,因此本综述旨在强调与工业火灾相关的公共健康危害,以及采取有效、协调的公共健康应对措施的必要性。我们还回顾了在此类火灾中使用的各种监测技术,并强调了扩散模型在预测烟羽轨迹和估计人口暴露量方面的作用。我们建议制定颗粒物 1 h 指导值,以便及时采取公共卫生干预措施,并强调有必要审查对火灾易发地点的监管和技术控制措施,特别是在废物处理部门。
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引用次数: 0
Innovative Photocatalytic Reactor for Sustainable Industrial Water Decontamination: Utilizing 3D-Printed Components and Silica-Titania Trilayer Coatings 用于可持续工业用水净化的创新型光催化反应器:利用三维打印部件和二氧化硅-钛三层涂层
Pub Date : 2024-07-20 DOI: 10.3390/environments11070156
George V. Theodorakopoulos, Michalis K. Arfanis, Tadej Stepišnik Perdih, Simos Malamis, Dimitrios Iatrou, George Em. Romanos, Polycarpos Falaras
Industrial activities generate enormous quantities of polluted effluents, necessitating advanced methods of wastewater treatment to prevent potential environmental threats. Thus, the design of a novel photocatalytic reactor for industrial water decontamination, purification, and reuse is proposed as an efficient advanced oxidation technology. In this work, the development of the active reactor components is described, utilizing a two-step sol–gel technique to prepare a silica-titania trilayer coating on 3D-printed polymeric filters. The initial dip-coated SiO2 insulator further protects and enhances the stability of the polymer matrix, and the subsequent TiO2 layers endow the composite architecture with photocatalytic functionality. The structural and morphological characteristics of the modified photocatalytic filters are extensively investigated, and their performance is assessed by studying the photocatalytic degradation of the Triton X-100, a common and standard chemical surfactant, presented in the contaminated wastewater of the steel metal industry. The promising outcomes of the innovative versatile reactor pave the way for developing scalable, cost-effective reactors for efficient water treatment technologies.
工业活动会产生大量的污染废水,因此需要采用先进的废水处理方法来防止潜在的环境威胁。因此,我们提出设计一种新型光催化反应器,作为一种高效的高级氧化技术,用于工业用水的去污、净化和回用。这项工作介绍了活性反应器组件的开发,利用两步溶胶-凝胶技术在 3D 打印聚合物过滤器上制备二氧化硅-钛三层涂层。最初浸涂的二氧化硅绝缘体可进一步保护和增强聚合物基体的稳定性,而随后的二氧化钛层则赋予了复合结构光催化功能。我们广泛研究了改性光催化过滤器的结构和形态特征,并通过研究钢铁金属工业污染废水中常见的标准化学表面活性剂 Triton X-100 的光催化降解来评估其性能。创新型多功能反应器取得的可喜成果为开发可扩展的、具有成本效益的高效水处理技术反应器铺平了道路。
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引用次数: 0
Heated Aeration for Nitrite-Oxidizing Bacteria (NOB) Control in Anammox-Integrated Membrane-Aerated Biofilm Reactors (MABR) 加热曝气用于亚硝酸盐氧化细菌(NOB)在氨氧化集成膜曝气生物膜反应器(MABR)中的控制
Pub Date : 2024-07-19 DOI: 10.3390/environments11070155
Natalia Shiu, Hui Guo, Younggy Kim
Nutrient removal in conventional wastewater treatment systems is expensive due to the high aeration costs. An alternative method for effective and sustainable nitrogen removal in wastewater treatment is anaerobic ammonium oxidation (Anammox) implemented with other innovative technologies, such as membrane-aerated biofilm reactors (MABRs). A major challenge associated with the Anammox process is effective control of nitrite-oxidizing bacteria (NOB). High temperature operation in wastewater treatment systems can promote Anammox bacterial growth and inhibit NOB activity. This research aims to investigate the feasibility of integrating Anammox processes with a lab-scale MABR and to examine the effects of high temperature aeration supplied to MABR systems on Anammox bacterial growth and NOB suppression. Experimental results indicate that the membrane’s air permeability was a critical parameter for the successful operation of Anammox-integrated MABR systems due to its influence on the system’s dissolved oxygen concentration (0.41 ± 0.39 mg O2/L). The ammonia removal by AOB and Anammox bacteria was determined to be 7.53 mg N/L·d (76.5%) and 2.12 mg N/L·d (23.5%), respectively. High temperature aeration in MABRs with the Anammox process shows a promising potential for improving energy consumption and sustainable nitrogen removal in wastewater treatment systems.
由于曝气成本高昂,传统废水处理系统中的营养物去除成本高昂。在废水处理中实现有效和可持续脱氮的另一种方法是厌氧氨氧化(Anammox),并与膜通气生物膜反应器(MABRs)等其他创新技术结合使用。与 Anammox 工艺相关的一个主要挑战是有效控制亚硝酸盐氧化细菌(NOB)。废水处理系统中的高温运行会促进 Anammox 细菌的生长,抑制 NOB 的活性。本研究旨在探讨将 Anammox 工艺与实验室规模的 MABR 相结合的可行性,并研究向 MABR 系统提供高温曝气对 Anammox 细菌生长和 NOB 抑制的影响。实验结果表明,由于膜的透气性对系统溶解氧浓度(0.41 ± 0.39 mg O2/L)的影响,因此膜的透气性是 Anammox 集成 MABR 系统成功运行的关键参数。经测定,AOB 和 Anammox 细菌的氨去除率分别为 7.53 mg N/L-d(76.5%)和 2.12 mg N/L-d(23.5%)。采用 Anammox 工艺的 MABRs 中的高温曝气在改善废水处理系统的能耗和可持续脱氮方面显示出巨大的潜力。
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引用次数: 0
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Environments
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