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International Conference on Nanoscience, Engineering and Technology (ICONSET 2011)最新文献

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Dielectric nanoantenna stickers for photoluminescence control 用于光致发光控制的介电纳米天线贴纸
S. Murai, Yuto Inoue, TienYang Lo, Katsuhisa Tanaka
We fabricated dielectric nanoantenna stickers comprising a periodic array of TiO2 nanoparticles embedded inside the polydimethylsiloxane (PDMS). For the fabrication, we first used a nanoimprint to make a square lattice of TiO2 nanoparticles on the SiO2 glass substrate, and then covered it with a PDMS film. Finally, the nanoantenna was transferred from the substrate to the PDMS by dissolving the sacrifice layer between the nanoantenna and the substrate. We found that poly(sodium-4-styrene sulfonate) was suitable as the water-soluble sacrifice layer for the transfer of TiO2 nanoantenna. As a demonstration, we placed the TiO2 nanoantenna sticker on top of the light-emitting layer. The emission from the emitter layer was enhanced directionally following the dispersion of lattice resonances excited in the sticker.
我们在聚二甲基硅氧烷(PDMS)中制备了包含TiO2纳米粒子周期性阵列的介电纳米天线贴纸。在制作过程中,我们首先使用纳米压印在SiO2玻璃基板上制作TiO2纳米颗粒的方形晶格,然后在其上覆盖PDMS薄膜。最后,通过溶解纳米天线与衬底之间的牺牲层,将纳米天线从衬底转移到PDMS中。我们发现聚4-苯乙烯磺酸钠适合作为TiO2纳米天线转移的水溶性牺牲层。作为演示,我们将TiO2纳米天线粘贴在发光层的顶部。随着贴片中激发的晶格共振的色散,发射层的发射有方向性地增强。
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引用次数: 0
Validation of stable p-type phosphorus (P) doped ZnO thin films formation by investigating the photoresponse properties of P:ZnO/Ga2O3 heterojunctions 通过研究P:ZnO/Ga2O3异质结的光响应特性,验证P型磷(P)掺杂ZnO薄膜形成的稳定性
Archishman Saha, M. Mishra, R. Saha, A. Dalal, Ankita Sengupta, A. Mondal, S. Chattopadhyay, S. Chakrabarti
The formation of reproducible p-type conductivity in ZnO thin films is highly challenging now a days for the fabrication of several homo/heterojunction based fully transparent opto-electronic devices. In this study, p-type P: ZnO thin films are deposited by cost-effective SOD process and then intrinsically n-type Ga2O3 films are deposited on it to validate the p-type conductivity of ZnO by making vertical heterojunction with n-Ga2O3. The ZnO thin films are deposited by RF sputtering and subsequent P-doping is done by using the SOD technique on it. This involves proximity diffusing dopants into a spin-coated film by stacking the dopant source during thermal annealing at 800◦C for four hours in the furnace. Ga2O3 films are deposited on the P: ZnO films by using RF sputtering technique, for making the heterojunction. The electrical measurements are performed by using current-voltage (I-V) measurements under illuminated and dark conditions. The photo-switching and responsivity are also measured on the fabricated device. It is observed that the P: ZnO/Ga2O3 heterojunction exhibits the photoresponse in the dual wavelength region. The corresponding two peaks of responsivity are found around 200 nm and 390 nm with the values of 68.03 A/W and 7.93 A/W (at 5 V), respectively. Such two peaks originated due to the ultra-wide bandgaps of Ga2O3 (4.7eV) and P: ZnO (3.1 eV). Also, such heterojunction shows a rapid switching speed under white light at 5 V (rise time: 230 ms, fall time: 163 ms) and −5 V (rise time: 83 ms, Fall time: 169 ms), which is comparable with the other reported results. Therefore, the current study demonstrates the development of highly stable and reproducible p-type P: ZnO thin films by employing SOD technique and the validation of p-type formation by fabricating P: ZnO/Ga2O3 heterojunctions for dual-wavelength selector UV detector application and such detectors can be a potential candidate for various optoelectronic devices.
在ZnO薄膜中形成可复制的p型电导率是目前几种基于异质结的全透明光电器件的制造极具挑战性的。本研究通过低成本的SOD工艺沉积P型P: ZnO薄膜,然后在其上沉积本质n型Ga2O3薄膜,通过与n-Ga2O3形成垂直异质结来验证ZnO的P型导电性。采用射频溅射法制备ZnO薄膜,并利用超氧化物歧化酶技术对其进行p掺杂。这涉及通过在炉中800°C热退火过程中堆叠掺杂源,将邻近扩散的掺杂剂扩散到自旋涂层薄膜中。采用射频溅射技术在P: ZnO薄膜上沉积Ga2O3薄膜,形成异质结。电气测量是通过在照明和黑暗条件下使用电流-电压(I-V)测量来完成的。测量了器件的光开关性能和响应性。观察到P: ZnO/Ga2O3异质结在双波长区域表现出光响应。对应的两个响应峰分别出现在200 nm和390 nm附近,值分别为68.03 A/W和7.93 A/W (5 V时)。这两个峰源于Ga2O3 (4.7eV)和P: ZnO (3.1 eV)的超宽带隙。此外,该异质结在5 V(上升时间:230 ms,下降时间:163 ms)和- 5 V(上升时间:83 ms,下降时间:169 ms)的白光下显示出快速的切换速度,这与其他报道的结果相当。因此,目前的研究表明,利用超氧化物歧化酶技术开发出高度稳定和可重复的P型P: ZnO薄膜,并通过制造P: ZnO/Ga2O3异质结来验证P型形成,用于双波长选择紫外探测器的应用,这种探测器可以成为各种光电器件的潜在候选。
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引用次数: 0
Synthesis of VS2/N-rGO nanocomposite material for energy storage application 用于储能的VS2/N-rGO纳米复合材料的合成
A. Mandal, S. K. Pandey, Kantimay Das Gupta, S. Chakrabarti
Vanadium disulfide (VS2), which belongs to transition metal dichalcogenides (TMDs) group, is a prominent material for energy storage application. On the other hand, graphene like carbon-based nanomaterials offer improved electrochemical performance due to high specific surface area, excellent conductivity, good chemical, and mechanical stability. Therefore, composite of graphene like material with TMD have shown better electrochemical performance till date. In this work, we have synthesized VS2/N-rGO composite material, which can be applicable for energy storage device. At first, we have synthesized graphene oxide (GO) using Tour method. Then we reduced GO along with nitrogen doping using hydrothermal route. After that, we have synthesized VS2/N-rGO by hydrothermal method. The X-ray diffraction (XRD) spectrum of GO shows a prominent peak at 10.2°, which implies the interlayer spacing in GO of 8.7 Å. After reduction and doping with nitrogen (N), two peaks are obtained at 24.7° (d = 3.6 Å), and 42.3° (d = 2.1 Å) in the XRD pattern which corresponds to N-rGO. RAMAN spectrum of composite shows the characteristics peaks of VS2 at 141.6, 194.5, 286.4, 404.1, 680.1 and 997.2 cm-1 along with D and G bands coming from the N-rGO. We have also performed the Fourier-transform infrared-spectroscopy (FTIR) and Field-emission gun-scanning electron-microscopy (FEG-SEM) characterizations to investigate the bonding vibration and surface morphology of the materials. The synthesized material is suitable for energy storage applications.
二硫化钒(VS2)属于过渡金属二硫族(TMDs),是一种重要的储能材料。另一方面,石墨烯类碳基纳米材料由于其高比表面积、优异的导电性、良好的化学和机械稳定性而提供了改进的电化学性能。因此,到目前为止,类石墨烯材料与TMD的复合材料表现出较好的电化学性能。在这项工作中,我们合成了VS2/N-rGO复合材料,可以应用于储能装置。首先,我们用Tour法合成了氧化石墨烯(GO)。然后采用水热法通过氮掺杂还原氧化石墨烯。然后,我们用水热法合成了VS2/N-rGO。氧化石墨烯的x射线衍射(XRD)谱在10.2°处有一个突出的峰,表明氧化石墨烯的层间间距为8.7 Å。还原后掺杂氮(N), XRD谱图中分别在24.7°(d = 3.6 Å)和42.3°(d = 2.1 Å)处得到两个峰,对应于N- rgo。复合材料的RAMAN光谱显示,VS2的特征峰位于141.6、194.5、286.4、404.1、680.1和997.2 cm-1, D和G波段来自N-rGO。我们还进行了傅里叶变换红外光谱(FTIR)和场发射枪扫描电子显微镜(fg - sem)表征,以研究材料的键合振动和表面形貌。该合成材料适合于储能应用。
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引用次数: 0
High-performance sensor based on bound states in the continuum 基于连续体束缚态的高性能传感器
Guodong Zhu, Sen Yang, J. Ndukaife
The bound states in the continuum (BIC) were first discovered by von Neumann and Wigner in quantum mechanics. It was subsequently identified in photonics. BIC represents an embedded eigenmode that can perfectly confine light. The optical resonators that support this mode can have very large field enhancements and infinite Q factor in theory. Considering these advantages as well as the negligible heat generation, the dielectric metasurface using BIC mode is a more promising platform for sensor applications. Nevertheless, their performance is quite constrained by factors such as inevitable fabrication imperfections, the array size of chips, and up-down symmetry breaking. To mitigate these challenges, we construct merging BICs with the accessible electric field distribution in a Lieb lattice. Meanwhile, we integrated this system with a lateral photonic crystal mirror to enhance its performance in compact conditions. The design we propose remains robust, sustaining a very high Q factor (up to 105) even when the up-down symmetry is broken, which provides a potential platform for optical trapping and biomedical sensing applications.
连续统中的束缚态是由量子力学中的冯·诺伊曼和维格纳首次发现的。它随后在光子学中被发现。BIC代表了一种可以完美地限制光的嵌入式特征模。支持这种模式的光学谐振器理论上可以有非常大的场增强和无限的Q因子。考虑到这些优点以及可以忽略不计的热量产生,使用BIC模式的介电超表面是一个更有前途的传感器应用平台。然而,它们的性能受到诸如不可避免的制造缺陷、芯片阵列尺寸和上下对称破坏等因素的限制。为了缓解这些挑战,我们在Lieb晶格中构造了具有可达电场分布的合并bic。同时,我们将该系统与横向光子晶体反射镜集成在一起,以提高其在紧凑条件下的性能。我们提出的设计保持稳健,即使在上下对称被打破时也能保持非常高的Q因子(高达105),这为光学捕获和生物医学传感应用提供了一个潜在的平台。
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引用次数: 0
Giant circular dichroic SHG behavior of double SP resonant chiral aluminum nanorod dimer structures 双SP共振手性铝纳米棒二聚体结构的巨圆二向色SHG行为
A. Sugita, Kenshin Muroi, Sota Tamotsu
This paper reports on the giant circular dichroic second-harmonic generation (CD-SHG) behavior of double SP resonant chiral Al nanorod (AlNR) dimer structures. The two AlNRs are aligned in a straight line. It becomes chiral, when one of the AlNRs is shifted laterally from it. We obtained CD-SHG signals up to 0.5 for the corresponding amount of the shift. Additionally, the sign of the CD-SHG was reversed, when the sign of the shift was reversed. The amount of the CD-SHG was flexibly tunable by changing the amount of the shift, which was the uniqueness of the present chiral plasmonic nanostructure.
本文报道了双SP共振手性铝纳米棒二聚体结构的巨圆二向色次谐波产生(CD-SHG)行为。这两个alnr排成一条直线。当其中一个alnr从它旁边移开时,它就变成手性的。我们得到相应位移量的CD-SHG信号高达0.5。此外,CD-SHG的符号被反转,当移位的符号被反转。通过改变位移量可以灵活地调节CD-SHG的量,这是目前手性等离子体纳米结构的独特性。
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引用次数: 0
Optical fiber and the microscopic interactions of light with matter 光纤和光与物质的微观相互作用
H. H. Cerecedo-Núñez, P. Padilla-Sosa
Microscopic laser light interaction with matter has many consequences. That result depends on many factors: the medium, the matter involved, the light intensity, the wavelength, and the many ways of light, among others. In this contribution, we are going to discuss several results observed when light interacts with matter under different conditions. The observation did use a standard optical fiber and near-infrared radiation. We are going to discuss the basic linear and angular momentum transference, optical trapping; light energy conversions, such as absorption, heating, photochemical reactions, and micro-thermocavitation.
微观激光与物质的相互作用有许多后果。这一结果取决于许多因素:介质、所涉及的物质、光强度、波长、光的多种方式等等。在这篇文章中,我们将讨论光在不同条件下与物质相互作用时观察到的几个结果。这次观测确实使用了标准光纤和近红外辐射。我们将讨论基本的线性和角动量传递,光捕获;光能转换,如吸收、加热、光化学反应、微热空化等。
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引用次数: 0
Spectrally selective thermal emission from graphene decorated with silver nanodisks 用银纳米片修饰石墨烯的光谱选择性热发射
J. Craft, Muhammad Waqas Shabbir, D. Englund, R. Osgood, M. N. Leuenberger
We show that graphene decorated with Ag nanodisks realizes spectrally selective thermal emission by means of acoustic graphene plasmons (AGPs) localized between graphene and the Ag nanodisks inside a dielectric material. Our finite-difference time domain (FDTD) calculations show that the spectrally selective thermal radiation emission can be tuned by means of a gate voltage into two different wavelength regimes, namely the atmospherically opaque regime between λ = 5 μm and λ = 8 μm or the atmospherically transparent regime between λ = 8 μm and λ = 12 μm. This allows for electrical switching between a radiative heat trapping mode for the former regime and a radiative cooling mode for the latter regime.
研究表明,在介质材料中,用银纳米片修饰的石墨烯通过石墨烯和银纳米片之间的声石墨烯等离子体(AGPs)实现了光谱选择性热发射。时域有限差分(FDTD)计算表明,通过栅极电压可以将光谱选择性热辐射发射调谐到两个不同的波长范围,即λ = 5 μm和λ = 8 μm之间的大气不透明区域或λ = 8 μm和λ = 12 μm之间的大气透明区域。这允许在前一种状态的辐射吸热模式和后一种状态的辐射冷却模式之间进行电气切换。
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引用次数: 0
Protocol to design plasmonic sensors for the characterization of materials at the atomic scale 原子尺度材料表征等离子体传感器设计方案
P. Viera-González, G. Sánchez-Guerrero, Edgar Martínez-Guerra, Eduardo Martínez-Guerra, Rodolfo Cortés Martínez
Materials characterization is essential since it is the basis for understanding materials’ physical and chemical properties before being used in any application. Nowadays, expensive equipment such as scanning electron microscopy and X-ray diffraction for thin film characterization at atomic layers are used. Atomic layer deposition (ALD) is a technique for growing thin films with a wide range of applications. The film thickness range is usually 1-500 nm. Plasmonic sensors are a low-cost technique for material characterization, including inorganic and organic thin films. The thickness resolution ranges from a fraction of a nanometer (monolayers) to several micrometers. These devices exploit the interaction of light with matter using surface plasmon resonance as a method based on the optoelectronic phenomenon. Kretschmann geometry continues to be a configuration widely used as an experimental setup to excite surface plasmon resonance in the characterization of different materials. It consists of a coupler prism with a thin metal film. The incident light in the total internal reflection at a specific angle, the evanescent wave transfers the energy to the electrons plasma of metal giving place surface plasmon resonance (SPR). The SPR effect in metals is highly sensitive to variations in the optical properties of the interface. We use the Kretschmann configuration and the matrix transfer method to analyze the performance numerically to achieve the optime parameters of design for the sensor’s performance. In this work, we developed a protocol to design and build a plasmonic sensor for the characterization of materials at the atomic layer level.
材料表征是必不可少的,因为它是在任何应用中使用之前了解材料物理和化学性质的基础。目前,昂贵的设备,如扫描电子显微镜和x射线衍射表征薄膜在原子层使用。原子层沉积(ALD)是一种具有广泛应用的薄膜生长技术。薄膜厚度范围通常为1- 500nm。等离子体传感器是一种低成本的材料表征技术,包括无机和有机薄膜。厚度分辨率范围从纳米(单层)的一小部分到几微米。这些装置利用表面等离子体共振作为一种基于光电现象的方法,利用光与物质的相互作用。在不同材料的表征中,克雷茨曼几何仍然是一种广泛使用的结构,作为激发表面等离子体共振的实验装置。它由一个带有薄金属薄膜的耦合器棱镜组成。入射光以一定角度进行全内反射,倏逝波将能量传递给金属的电子等离子体,产生表面等离子体共振(SPR)。金属中的SPR效应对界面光学性质的变化高度敏感。采用Kretschmann组态和矩阵传递法对传感器性能进行了数值分析,得到了传感器性能的最优设计参数。在这项工作中,我们开发了一种协议来设计和构建一个等离子体传感器,用于在原子层水平上表征材料。
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引用次数: 0
Structured surface plasmon generated with interfered evanescent waves 由干涉消褪波产生的结构表面等离子体
Fabian C. Cubillos-Morales, G. Martínez Niconoff, I. I. Cazares Aguilar
This work introduces an interesting configuration for exciting structured surface plasmon-polaritons (SSPP) by analyzing wave propagation on a composite dielectric-metal surface. In particular, we focus on the coupling of interfered evanescent waves with structured SPP. This innovative approach unlocks new avenues for enhancing plasmon optics models, encompassing diffraction, interference, and focalization. By exploring the potential of this configuration, we improved the understanding and application of structured SPP in various optical phenomena.
本文通过分析波在复合介质-金属表面的传播,介绍了一种有趣的激发结构表面等离子体极化子(SSPP)的配置。特别地,我们专注于干涉倏逝波与结构SPP的耦合。这种创新的方法为增强等离子体光学模型开辟了新的途径,包括衍射、干涉和聚焦。通过探索这种结构的潜力,我们提高了对结构SPP在各种光学现象中的理解和应用。
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引用次数: 0
Topological darkness in random gold metasurfaces for high sensitivity detection using phase interrogation 基于相位询问的随机金超表面拓扑暗度高灵敏度检测
Juan Pablo Cuanalo Fernandez, N. Korneev, I. Cosme-Bolanos, María Beatriz de la Mora Mojica, Irving Gazga Gurrión, S. Mansurova, R. Ramos García
In this study, we investigate the phenomenon of nearly zero reflectance and associated phase singularity in a random array of gold nanoislands (Au NI) both theoretically and experimentally. The Au NI were produced via solid-state thermal dewetting of ultrathin gold films, which were magnetron sputtered onto a glass substrate. The morphology of the nanoislands was characterized using scanning electron microscopy and atomic force microscopy. To understand the plasmonic response of the random array of Au NI, we conducted reflectance measurements for both s and p polarized beams demonstrating the p. These measurements were performed using the attenuated total internal reflectance configuration. A partial state of topological darkness in a random array of Au NI was demonstrated by showing nearly zero reflection for the p polarization component. Additionally, we employed a common path spectral interferometer to measure the differential phase spectra. Our findings revealed that the differential phase spectra exhibited abrupt ±π phase jumps, indicating the presence of a phase singularity regime. Moreover, we demonstrated high bulk reflectance index sensitivity (RIS) within this regime. To validate our experimental results, we compared them with analytical reflectance and phase spectra obtained through the application of island film theory. The agreement between the experimental and theoretical predictions provided strong confirmation of our measurement technique.
在这项研究中,我们从理论上和实验上研究了金纳米岛(Au NI)随机阵列的近零反射率和相关的相位奇点现象。通过磁控溅射到玻璃衬底上的超薄金膜的固态热脱湿制备了Au NI。利用扫描电子显微镜和原子力显微镜对纳米岛的形貌进行了表征。为了了解Au NI随机阵列的等离子体响应,我们对s和p极化光束进行了反射率测量,以显示p。这些测量是使用衰减的总内反射配置进行的。通过对p偏振分量的反射接近于零,证明了随机Au NI阵列中拓扑黑暗的部分状态。此外,我们采用了共程光谱干涉仪来测量差分相位光谱。我们的研究结果表明,微分相谱表现出突然的±π相跃,表明存在相奇点区。此外,我们还证明了在该范围内具有较高的体反射指数灵敏度(RIS)。为了验证我们的实验结果,我们将其与应用岛膜理论得到的解析反射率和相谱进行了比较。实验和理论预测的一致性为我们的测量技术提供了强有力的证实。
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引用次数: 0
期刊
International Conference on Nanoscience, Engineering and Technology (ICONSET 2011)
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