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Moiré metalens-based fluorescence optical sectioning microscopy 基于超构透镜的荧光光学切片显微镜
Yu-hsin Chia, C. H. Chu, S. Vyas, Yi-You Huang, D. Tsai, Yuan Luo
Microscopy is an essential tool for biomedical research and clinical diagnosis. Nevertheless, conventional wide-field imaging system lacks optical sectioning ability, restricting applications in thick tissues. Recently, HiLo microscopy improved sectioning efficiency but still requires axial movement. Here, we propose the Moiré metalens to develop the varifocal metalens based fluorescence optical sectioning microscopy. It leveraging metasurfaces capabilities to control optical properties. Our system enables optical sectioning and 3D imaging capability. We demonstrate multiplane HiLo optically sectioned images of fluorescent microspheres and ex-vivo mouse brain tissues. This technique opens new possibilities for high-contrast microscopy in biomedical research and clinical diagnosis.
显微镜是生物医学研究和临床诊断的重要工具。然而,传统的宽视场成像系统缺乏光学切片能力,限制了在厚组织中的应用。最近,HiLo显微镜提高了切片效率,但仍然需要轴向运动。在此,我们提出了moir超透镜来发展基于变焦超透镜的荧光光学切片显微镜。它利用超表面功能来控制光学特性。我们的系统具有光学切片和3D成像能力。我们展示了荧光微球和离体小鼠脑组织的多平面HiLo光学切片图像。这项技术为高对比度显微镜在生物医学研究和临床诊断方面开辟了新的可能性。
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引用次数: 0
Plasmonic response of a random metasurface based on gold nano-islands in attenuated total reflectance configuration 衰减全反射结构下基于金纳米岛的随机超表面的等离子体响应
J. P. Cuanalo, Irving Gazga, I. Cosme-Bolanos, N. Korneev, Rebeca Lugo, Rubén Ramos, S. Mansurova
In this work, we investigate the plasmonic response of a random metasurface based on gold nano-islands (AuNI) in an attenuated total reflectance (ATR) configuration. AuNI structures were obtained by thermal annealing of an ultrathin gold film deposited on a glass substrate. The samples exhibited a wide range of sizes and particle densities, varying the nominal gold thickness. For p polarization, a well-defined localized surface plasmon resonance (LSPR) dip was observed in all samples, while for s polarization, only AuNI with the smallest radii showed this dip. Some samples exhibited nearly zero reflection at the resonance wavelength. The highest sensitivity among all tested samples was achieved in these samples, providing potential for optimizing LSPR transducers in sensing applications. Notably, the resonance wavelength exhibited a nonlinear dependence on the refractive index in sensitivity measurements displaying a blue shift.
在这项工作中,我们研究了基于金纳米岛(AuNI)的随机超表面在衰减全反射(ATR)配置下的等离子体响应。通过在玻璃衬底上沉积超薄金膜的热退火获得了aui结构。样品的尺寸和颗粒密度范围很广,标称金的厚度也有所不同。对于p极化,在所有样品中都观察到一个明确的局部表面等离子体共振(LSPR)倾角,而对于s极化,只有半径最小的AuNI有这种倾角。有些样品在共振波长处的反射几乎为零。在所有测试样品中,这些样品的灵敏度最高,为优化传感应用中的LSPR传感器提供了潜力。值得注意的是,共振波长表现出非线性依赖于折射率在灵敏度测量显示蓝移。
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引用次数: 0
Plasmonic sensor for house wastewater monitoring 用于家庭污水监测的等离子体传感器
G. S. Sánchez Guerrero, P. V. Viera González, Edgar Martinez Guerra, K. Acuña Askar, Rodolfo Cortés Martínez
Wastewater quality monitoring is essential as an effective pandemic management tool. Domestic water is one of the leading causes of wastewater pollution. Domestic water originates from urban centers and contains substances from human activity consisting of organic matter such as food remains, feces, oils, detergents, and soaps. Different ways of sensing are used to maintain the water quality, like pH, conductivity, and turbidity sensors. Alternative methods are optical sensors because these offer great potential for wastewater monitoring, allowing massive, easy and low-cost acquisitions of a wide range of measures in real-time, at any flow conditions, and with high spatial resolution. Plasmonic sensors are optical sensors used for detection, which could realize rapid recognition, real-time analysis, and sensitive and selecting sensing. These devices exploit the interaction of light with matter using the SPR as a method based on the optoelectronic phenomenon. When light hits a metal surface (typically a gold surface) at a certain angle, part of the light energy pairs through the metal coating with the electrons in the metal surface layer, which then move due to excitation, called surface plasmon resonance. We use the Kretschmann configuration and the matrix transfer method to analyze the performance numerically to achieve the optime parameters of design for the sensor’s performance. In this work, we design and build a plasmonic sensor for house wastewater monitoring by tracking contaminants along a continuous flow of artisanal water.
废水质量监测作为一种有效的大流行管理工具至关重要。生活用水是污水污染的主要原因之一。生活用水来自城市中心,含有人类活动产生的有机物质,如食物残渣、粪便、油脂、洗涤剂和肥皂。不同的传感方式用于维持水质,如pH值,电导率和浊度传感器。替代方法是光学传感器,因为它们为废水监测提供了巨大的潜力,可以在任何流量条件下以高空间分辨率实时获取大量、简单和低成本的测量数据。等离子体传感器是一种用于检测的光学传感器,具有快速识别、实时分析、灵敏和选择性传感等特点。这些装置利用SPR作为基于光电现象的方法,利用光与物质的相互作用。当光线以一定角度照射到金属表面(通常是金表面)时,部分光能与金属表层的电子配对,然后由于激发而移动,称为表面等离子体共振。采用Kretschmann组态和矩阵传递法对传感器性能进行了数值分析,得到了传感器性能的最优设计参数。在这项工作中,我们设计并构建了一个等离子体传感器,通过跟踪沿着连续流动的手工水的污染物来监测家庭废水。
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引用次数: 0
Investigation of electronic and optical behavior of Ag-based novel double perovskite MA2AgBiCl6 for photovoltaic applications 银基新型双钙钛矿MA2AgBiCl6光电性能研究
Neelu Neelu, Nivedita Pandey, S. Chakrabarti
High-performance semiconductors for optoelectronic device applications based on hybrid perovskites have been extensively investigated by the research community. However, their degradability and toxicity problem is a serious challenge that should be addressed effectively. Nowadays, double perovskites have been introduced as a promising lead-free alternative which is a combination of two single perovskites in which lead is replaced by monovalent and trivalent cation. Herein, we have chemically prepared a promising, stable, and novel organic-inorganic hybrid lead-free methyl ammonium (MA) based double perovskite material MA2AgBiCl6 by one-pot hydrothermal method. Structural characterization using x-ray diffraction (XRD) experiment confirms the formation of the orthorhombic crystalline phase of MA2AgBiCl6. Further, the examination of the Ultra-violet (UV-vis) spectroscopy characterization of MA2AgBiCl6 affirms the excellent absorbance behavior with a direct and indirect bandgap of 3.58 eV and 2.8 eV respectively. To investigate the optical characteristics of MA2AgBiCl6, photoluminescence (PL) spectroscopy experiment was performed and it is found that the material is reflecting good photoluminescence nature having a sharp peak at 320 nm which occur due to the band to band transition and carrier recombination of phonons. Furthermore, we performed a scanning electron microscopy (SEM) experiment on synthesized material to see its surface properties and we have observed the uniform nanotubes like fine and dense structure. Also, the Fourier transform infrared (FTIR) spectroscopy measurement reflect the transmittance nature of the prepared material. This detailed investigation on novel double perovskite MA2AgBiCl6 opens a new window for the emerging category of halide-based double perovskites for their possible utility in photovoltaics.
基于混合钙钛矿的光电子器件应用的高性能半导体已经被研究界广泛研究。然而,它们的可降解性和毒性问题是一个需要有效解决的严峻挑战。目前,双钙钛矿是一种很有前途的无铅替代品,它是两种单钙钛矿的组合,其中铅被一价和三价阳离子取代。本文采用一锅水热法制备了一种稳定的新型有机-无机杂化无铅甲基铵(MA)基双钙钛矿材料MA2AgBiCl6。x射线衍射(XRD)实验证实了MA2AgBiCl6形成了正交晶相。此外,对MA2AgBiCl6的紫外-可见光谱表征证实了其良好的吸光度行为,其直接带隙和间接带隙分别为3.58 eV和2.8 eV。为了研究MA2AgBiCl6的光学特性,进行了光致发光(PL)光谱实验,发现该材料具有良好的光致发光特性,在320 nm处由于声子的带间跃迁和载流子的复合而产生尖峰。此外,我们对合成材料进行了扫描电子显微镜(SEM)实验,观察其表面性能,我们观察到纳米管的均匀,如精细和致密的结构。傅里叶变换红外光谱(FTIR)测量也反映了所制备材料的透光性。对新型双钙钛矿MA2AgBiCl6的详细研究为新兴的卤化物基双钙钛矿在光伏领域的潜在应用打开了一扇新的窗口。
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引用次数: 0
Effects of laser induced shockwave on neurons from an Alzheimer’s mouse model 激光诱导冲击波对阿尔茨海默氏症小鼠模型神经元的影响
Veronica Gomez Godinez, Steven Zheng, Matthew Hsin-De Tran, Chengbiao Wu, Linda Z. Shi
Neuronal responses to injury are of interest to the development of methods to mitigate damage and stimulate repair. We utilized a single pulse from a 1030nm laser to create a laser induced shockwave (LIS) to subject neuronal cells to injury and compare the effects of injury on neurons from an Alzheimer’s Disease (AD) mouse model and wild type (WT) mice. We found differences in the calcium response to LIS in AD versus WT neurons. Additionally, we found that LIS induced cell death led to a calcium elevation which differed from that in cells that stayed alive. Therefore, the calcium response can be utilized to separate dead cells from live cells.
神经元对损伤的反应对减轻损伤和刺激修复的方法的发展很感兴趣。我们利用1030nm激光的单脉冲产生激光诱导冲击波(LIS),使神经元细胞受到损伤,并比较损伤对阿尔茨海默病(AD)小鼠模型和野生型(WT)小鼠神经元的影响。我们发现AD和WT神经元对LIS的钙反应存在差异。此外,我们发现LIS诱导的细胞死亡导致钙升高,这与存活的细胞不同。因此,钙反应可以用来分离死细胞和活细胞。
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引用次数: 0
Multilayer broadband switchable absorbers based on phase-change materials 基于相变材料的多层宽带可切换吸收体
Md. Tanvir Emrose, Emily L. Payne, Chenglong You, G. Veronis
We introduce multilayer structures with the phase-change material germanium-antimony-tellurium (GST) for use as broadband switchable absorbers in the infrared wavelength range. We use a memetic optimization algorithm coupled with the transfer-matrix method to optimize both the material composition and the layer thicknesses of the multilayer structures. We show that in the optimized structures near perfect absorption can be switched to very low absorption in a broad wavelength range by switching GST from its crystalline to its amorphous phase. Our results could pave the way to a new class of broadband switchable absorbers and thermal sources in the infrared wavelength range.
我们介绍了用相变材料锗锑碲(GST)作为红外波段宽带可切换吸收器的多层结构。我们使用模因优化算法结合传递矩阵方法来优化多层结构的材料组成和层厚度。我们表明,在优化的结构中,通过将GST从晶体相转换为非晶态相,可以在宽波长范围内将接近完美的吸收转换为非常低的吸收。我们的研究结果可以为在红外波长范围内的新型宽带可切换吸收器和热源铺平道路。
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引用次数: 0
End-to-end optimization of meta-lens doublet for high-quality wide-angle imaging 端到端优化元透镜双透镜,实现高质量广角成像
Yeong-Su Park, Byoungho Lee, Yoonchan Jeong
In this paper, we propose an advanced method to jointly optimize doublet metalens and deep learning-based postprocessing networks for wide-angle and full-color imaging with high fidelity. The optical image formation module in the spatially-variant system and a reconstruction network module are implemented in a differentiable manner. By premitigating coma aberration with doublet metalens, the proposed model outperforms both cases of singlet structure and analogous electronic implementations in terms of reconstruction accuracy.
在本文中,我们提出了一种先进的方法来联合优化双重超透镜和基于深度学习的后处理网络,以实现高保真的广角和全彩成像。空间变系统中的光学成像模块和重建网络模块以可微方式实现。通过用双重超透镜预校正彗差,所提出的模型在重建精度方面优于单重态结构和类似的电子实现。
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引用次数: 0
Phase identification on infiltrated thermal barrier materials by 2D Raman spectroscopy 二维拉曼光谱对渗透热障材料的物相识别
Ivan F. Bedoya-Trujillo, A. Herrera-Rodríguez, Sebastian Pérez-Bedoya, Natalia Brizuela-Colmenares, J. Zárate-Medina, J. Muñoz-Saldaña
Thermochemical degradation of thermal barrier coatings generated by the infiltration of siliceous debris at high temperatures is considered a serious threat by aircraft industry due to phase destabilization of the thermal barrier material induces changes on its properties. Most materials-based strategies to mitigate the infiltration aim to promote the reactive crystallization of phases such as apatite. In this work, 2D Raman spectroscopy was carried out over the cross sections of lanthanum-gadolinium zirconate ceramic samples infiltrated by Colima and Popocatepetl volcanic ashes at 1250 °C for 10 h to identify the phases reprecipitated after infiltration. Raman mappings showed the characteristic peaks and the distribution of reprecipitated phases such as rare-earth apatite, monoclic and tetragonal zirconia. Additionally, rare-earth zirconate ceramics were identified by the characteristic F2g band of the pyrochlore structure. At the reaction layer, two zones were observed. Zirconia phases reprecipitating right at the upper zone while rare-earth apatite reprecipitating at the lower zone. For apatite, the peak corresponding to stretching vibrations of Si-O tetrahedra shows shifting to higher wavenumber values as gadolinium content increases in the rare-earth zirconate infiltrated. The 2D Raman spectroscopy was very effective to observe the distribution of the reprecipitated phases in addition to correlate the influence of gadolinium in the formed apatite. A correlation between infiltration depth and bands were confirmed.
硅质碎屑在高温下渗透产生的热障涂层的热化学降解被认为是航空工业的一个严重威胁,因为热障材料的相不稳定会引起其性能的变化。大多数以材料为基础的减缓渗透的策略旨在促进相的反应结晶,如磷灰石。本文采用二维拉曼光谱对Colima和Popocatepetl火山灰在1250℃下浸渍10 h的锆酸镧钆陶瓷样品的横截面进行了二维拉曼光谱分析,以确定浸渍后再沉淀的相。拉曼映射显示了稀土磷灰石、单晶和四方形氧化锆等再析出相的特征峰和分布。此外,利用焦绿石结构的特征F2g波段对稀土锆酸盐陶瓷进行了识别。在反应层,观察到两个区。氧化锆相在上带再沉淀,稀土磷灰石在下带再沉淀。对于磷灰石,随着稀土锆酸盐中钆含量的增加,Si-O四面体拉伸振动对应的峰向更高的波数值移动。二维拉曼光谱非常有效地观察了再析出相的分布,并关联了形成的磷灰石中钆的影响。证实了入渗深度与波段之间的相关性。
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引用次数: 0
Optical anisotropy of NbOCl2 NbOCl2的光学各向异性
Shuin Jian Wu, Y. Ho, Isa Ahmadalidokht, G. Eda, Alexander Ling
Guo et al, 2023, report that NbOCl2 is a novel thin-material SPDC source, but further optical measurements on thicker samples of the material suggest that NbOCl2 does not behave like conventional SPDC producing materials. In this paper, we report the following: (1) NbOCl2 is not completely transparent at the reported pump wavelength of 404 nm, (2) NbOCl2 behaves as a polarizer at 405 nm, (3) coincidences above noise level around 810 nm were obtained when pumping NbOCl2 at 405 nm and varied with pump polarization, and (4) pumping at the more transparent wavelength of 780 nm fails to yield any detectable SPDC photon pairs.
Guo等人,2023报道,NbOCl2是一种新型的薄材料SPDC源,但对材料较厚样品的进一步光学测量表明,NbOCl2的行为不像传统的SPDC产生材料。在本文中,我们报告了以下几个方面:(1)在404 nm的泵浦波长下,NbOCl2不是完全透明的;(2)在405 nm的泵浦波长下,NbOCl2表现为偏振器;(3)在405 nm泵浦时,NbOCl2在810 nm左右的噪声级以上得到了一致性,并且随着泵浦偏振的变化而变化;(4)在780 nm更透明的波长下泵浦时,没有产生任何可检测的SPDC光子对。
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引用次数: 0
Deposition and characterization of distributed Bragg feedback resonant-cavities with complex index active layers 具有复指数有源层的分布式Bragg反馈谐振腔的沉积与表征
Angelica Drees, Peter R. Stevensen, A. Sarangan
We demonstrate a novel approach to designing a distributed Bragg reflector consisting of a complex-index material (i.e., gold and VO2). The design with a gold center layer has been fabricated and characterized. The field enhancement is used to reduce the optical limiting threshold and increase nonlinearity.
我们展示了一种设计由复折射率材料(即金和VO2)组成的分布式布拉格反射器的新方法。制备了具有金中心层的设计并对其进行了表征。光场增强可以降低光限阈值,增加非线性。
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引用次数: 0
期刊
International Conference on Nanoscience, Engineering and Technology (ICONSET 2011)
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