Pub Date : 2022-08-07DOI: 10.1080/09506608.2022.2107372
Iva Milisavljevic, M. J. Pitcher, Jianqiang Li, S. Chenu, M. Allix, Yiquan Wu
ABSTRACT Latest advancements in transparent ceramics development have ensured a mainstream research interest in this family of materials. Crystallization of glass into transparent ceramics has emerged recently as an alternative but complementary trajectory for obtaining transparent ceramics, which circumvents some of the long-standing technical difficulties associated with traditional transparent ceramics processing. The full bulk glass crystallization allows for the synthesis of high-density/low-porosity transparent ceramics of stable and metastable phases or even non-cubic structures, which are difficult to obtain using the traditional processing methods. This article presents a brief survey of the science of the transparency of ceramics and a detailed overview of the materials systems and techniques used for the preparation of transparent ceramics through the glass crystallization route. Finally, the review provides authors' insights into the future trends and research directions aimed to encourage a widespread application of glass crystallization into transparent ceramics in the fabrication of next-generation materials.
{"title":"Crystallization of glass materials into transparent optical ceramics","authors":"Iva Milisavljevic, M. J. Pitcher, Jianqiang Li, S. Chenu, M. Allix, Yiquan Wu","doi":"10.1080/09506608.2022.2107372","DOIUrl":"https://doi.org/10.1080/09506608.2022.2107372","url":null,"abstract":"ABSTRACT Latest advancements in transparent ceramics development have ensured a mainstream research interest in this family of materials. Crystallization of glass into transparent ceramics has emerged recently as an alternative but complementary trajectory for obtaining transparent ceramics, which circumvents some of the long-standing technical difficulties associated with traditional transparent ceramics processing. The full bulk glass crystallization allows for the synthesis of high-density/low-porosity transparent ceramics of stable and metastable phases or even non-cubic structures, which are difficult to obtain using the traditional processing methods. This article presents a brief survey of the science of the transparency of ceramics and a detailed overview of the materials systems and techniques used for the preparation of transparent ceramics through the glass crystallization route. Finally, the review provides authors' insights into the future trends and research directions aimed to encourage a widespread application of glass crystallization into transparent ceramics in the fabrication of next-generation materials.","PeriodicalId":14427,"journal":{"name":"International Materials Reviews","volume":"68 1","pages":"648 - 676"},"PeriodicalIF":16.1,"publicationDate":"2022-08-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"48727103","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2022-07-13DOI: 10.1080/09506608.2022.2097411
Shi-Hao Li, Punith Kumar, S. Chandra, U. Ramamurty
ABSTRACT Amongst the many additive manufacturing (AM) techniques, directed energy deposition (DED) is a prominent one, which can also be used for the repair of damaged components. In this paper, we provide an overview on it, with emphasis on the typical microstructures of DED alloys and discuss the processing-microstructure-mechanical property correlations. Comparison is made with those manufactured using the conventional techniques and those obtained with laser beam powder bed fusion (LB-PBF). The characteristic solidification rates and thermal histories in DED result in distinct micro- and meso-structural features and mechanical performance, which are succinctly summarized. The potential of DED for manufacturing graded materials and for component repair is elaborated while highlighting the key-associated challenges and possible solutions. Modelling and simulation studies that facilitate an in-depth understanding of the DED technique are summarized. Finally, some critical issues and research directions that would help develop DED further and extend its application potential are identified.
{"title":"Directed energy deposition of metals: processing, microstructures, and mechanical properties","authors":"Shi-Hao Li, Punith Kumar, S. Chandra, U. Ramamurty","doi":"10.1080/09506608.2022.2097411","DOIUrl":"https://doi.org/10.1080/09506608.2022.2097411","url":null,"abstract":"ABSTRACT Amongst the many additive manufacturing (AM) techniques, directed energy deposition (DED) is a prominent one, which can also be used for the repair of damaged components. In this paper, we provide an overview on it, with emphasis on the typical microstructures of DED alloys and discuss the processing-microstructure-mechanical property correlations. Comparison is made with those manufactured using the conventional techniques and those obtained with laser beam powder bed fusion (LB-PBF). The characteristic solidification rates and thermal histories in DED result in distinct micro- and meso-structural features and mechanical performance, which are succinctly summarized. The potential of DED for manufacturing graded materials and for component repair is elaborated while highlighting the key-associated challenges and possible solutions. Modelling and simulation studies that facilitate an in-depth understanding of the DED technique are summarized. Finally, some critical issues and research directions that would help develop DED further and extend its application potential are identified.","PeriodicalId":14427,"journal":{"name":"International Materials Reviews","volume":"68 1","pages":"605 - 647"},"PeriodicalIF":16.1,"publicationDate":"2022-07-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"45331900","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2022-06-18DOI: 10.1080/09506608.2022.2086388
Gillian F. Hawes, Sarish Rehman, Yverick Rangom, M. Pope
ABSTRACT Advancements in electrochemical energy storage devices such as batteries and supercapacitors are vital for a sustainable energy future. Significant progress has been made in developing novel materials for these devices, but less attention has focused on developments in electrode and device manufacturing. While electrodes are traditionally made through slurry casting of electrochemically active material, advanced manufacturing techniques enable patterning of novel electrode architectures and control of device geometries in real-time, which can potentially result in electrodes with increased loading, improved electrochemical performance, and added functionality, such as flexibility and wearability. These inexpensive methods are particularly suited for lab-scale research and start-up companies, as they enable rapid prototyping without a full device production line. The present review describes three main methods of advanced manufacturing (inkjet printing, direct ink writing, and laser-induced graphene techniques) and evaluates the performance of batteries and supercapacitors fabricated via these methods in comparison to traditionally manufactured devices.
{"title":"Advanced manufacturing approaches for electrochemical energy storage devices","authors":"Gillian F. Hawes, Sarish Rehman, Yverick Rangom, M. Pope","doi":"10.1080/09506608.2022.2086388","DOIUrl":"https://doi.org/10.1080/09506608.2022.2086388","url":null,"abstract":"ABSTRACT Advancements in electrochemical energy storage devices such as batteries and supercapacitors are vital for a sustainable energy future. Significant progress has been made in developing novel materials for these devices, but less attention has focused on developments in electrode and device manufacturing. While electrodes are traditionally made through slurry casting of electrochemically active material, advanced manufacturing techniques enable patterning of novel electrode architectures and control of device geometries in real-time, which can potentially result in electrodes with increased loading, improved electrochemical performance, and added functionality, such as flexibility and wearability. These inexpensive methods are particularly suited for lab-scale research and start-up companies, as they enable rapid prototyping without a full device production line. The present review describes three main methods of advanced manufacturing (inkjet printing, direct ink writing, and laser-induced graphene techniques) and evaluates the performance of batteries and supercapacitors fabricated via these methods in comparison to traditionally manufactured devices.","PeriodicalId":14427,"journal":{"name":"International Materials Reviews","volume":"68 1","pages":"323 - 364"},"PeriodicalIF":16.1,"publicationDate":"2022-06-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"49100912","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2022-06-16DOI: 10.1080/09506608.2022.2079367
Xiao Lin, Saijilafu, Xiexing Wu, Kang Wu, Jianquan Chen, L. Tan, F. Witte, Huilin Yang, D. Mantovani, Huan Zhou, Chunyong Liang, Qiang Yang, Ke Yang, Lei Yang
ABSTRACT Mg-based alloys as revolutionary implantable biomaterials have increasingly attracted considerable attention, owing to their biodegradability in vivo and beneficial effects on biological systems. The degradation process and products of Mg-based alloys have been reported to exhibit significant biological effects on host-tissue responses. However, these effects have not yet been fully understood. This review systemically summarizes and analyses the current understandings and recent research progress in this area. The primary focal points are the biological effects and related mechanisms associated with the degradation behaviour of Mg-based alloys. The biological impacts of the degradation products are elucidated and the arguable or controversial issues are also discussed, providing a pathway toward a greater understanding of the biological implications of Mg-based alloys. Furthermore, based on these biological implications, the restorative potential of Mg-based alloys for applications in tissue repair and regeneration is summarized. Finally, outlooks on biosafety evaluation and design strategies for Mg-based alloy implants are briefly discussed.
{"title":"Biodegradable Mg-based alloys: biological implications and restorative opportunities","authors":"Xiao Lin, Saijilafu, Xiexing Wu, Kang Wu, Jianquan Chen, L. Tan, F. Witte, Huilin Yang, D. Mantovani, Huan Zhou, Chunyong Liang, Qiang Yang, Ke Yang, Lei Yang","doi":"10.1080/09506608.2022.2079367","DOIUrl":"https://doi.org/10.1080/09506608.2022.2079367","url":null,"abstract":"ABSTRACT Mg-based alloys as revolutionary implantable biomaterials have increasingly attracted considerable attention, owing to their biodegradability in vivo and beneficial effects on biological systems. The degradation process and products of Mg-based alloys have been reported to exhibit significant biological effects on host-tissue responses. However, these effects have not yet been fully understood. This review systemically summarizes and analyses the current understandings and recent research progress in this area. The primary focal points are the biological effects and related mechanisms associated with the degradation behaviour of Mg-based alloys. The biological impacts of the degradation products are elucidated and the arguable or controversial issues are also discussed, providing a pathway toward a greater understanding of the biological implications of Mg-based alloys. Furthermore, based on these biological implications, the restorative potential of Mg-based alloys for applications in tissue repair and regeneration is summarized. Finally, outlooks on biosafety evaluation and design strategies for Mg-based alloy implants are briefly discussed.","PeriodicalId":14427,"journal":{"name":"International Materials Reviews","volume":"68 1","pages":"365 - 403"},"PeriodicalIF":16.1,"publicationDate":"2022-06-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"44521671","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2022-06-10DOI: 10.1080/09506608.2022.2084670
S. K. Nayak, Anil Kumar, T. Laha
ABSTRACT Among various materials available for alleviating the corrosion-related degradation, thermal sprayed Fe-based metallic glass coatings (MGCs) have received huge attention from the scientific community due to the exceptional combination of mechanical and corrosion properties, along with commercially attractive low material cost of this particular alloy system. Emerging reports on the thermal sprayed Fe-based MGCs outperforming conventional corrosion-resistant materials and coatings have accelerated further exploration of this domain, resulting in an immense increase of research activities over the last few decades producing fascinating results. This review takes a holistic approach encompassing an in-depth assessment of all the relevant salient work till date, including corrosion properties, corresponding degradation mechanisms, metallurgical and environmental factors with reference to passive film dynamics and/or formation of corrosion products. Moreover, various strategies for improved corrosion properties and recent research progress have been reviewed with an attempt to identify the present knowledge gaps and the future research directions. GRAPHICAL ABSTRACT
{"title":"Fe-based metallic glass coatings by thermal spraying: a focused review on corrosion properties and related degradation mechanisms","authors":"S. K. Nayak, Anil Kumar, T. Laha","doi":"10.1080/09506608.2022.2084670","DOIUrl":"https://doi.org/10.1080/09506608.2022.2084670","url":null,"abstract":"ABSTRACT Among various materials available for alleviating the corrosion-related degradation, thermal sprayed Fe-based metallic glass coatings (MGCs) have received huge attention from the scientific community due to the exceptional combination of mechanical and corrosion properties, along with commercially attractive low material cost of this particular alloy system. Emerging reports on the thermal sprayed Fe-based MGCs outperforming conventional corrosion-resistant materials and coatings have accelerated further exploration of this domain, resulting in an immense increase of research activities over the last few decades producing fascinating results. This review takes a holistic approach encompassing an in-depth assessment of all the relevant salient work till date, including corrosion properties, corresponding degradation mechanisms, metallurgical and environmental factors with reference to passive film dynamics and/or formation of corrosion products. Moreover, various strategies for improved corrosion properties and recent research progress have been reviewed with an attempt to identify the present knowledge gaps and the future research directions. GRAPHICAL ABSTRACT","PeriodicalId":14427,"journal":{"name":"International Materials Reviews","volume":"68 1","pages":"404 - 485"},"PeriodicalIF":16.1,"publicationDate":"2022-06-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"47486832","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2022-05-20DOI: 10.1080/09506608.2022.2047419
Vidushi Sharma, Sheetal Chowdhury, N. Keshavan, B. Basu
ABSTRACT Ultra-high molecular weight polyethylene (UHMWPE) materials have played a significant role in the field of reconstructive surgery, particularly as acetabular liners/sockets for total hip joint replacement (THR), and tibial inserts for total knee joint replacement (TKR). This review aims to provide a perspective on key elements regarding the processing–structure–property relationship of UHMWPE and derivatives. Much emphasis will be provided to discuss the clinically relevant properties of UHMWPE blend/composite formulation, Vitamin-E reinforced or highly crosslinked variants. In addition, we provide clinical insights into the role of wear debris in inflammation and osteolysis. The relatively unexplored domain of UHMWPE additive manufacturing. Finally, the relatively unexplored domain of UHMWPE additive manufacturing and the opportunities associated with the next generation of UHMWPE implants are highlighted. GRAPHICAL ABSTRACT
{"title":"Six decades of UHMWPE in reconstructive surgery","authors":"Vidushi Sharma, Sheetal Chowdhury, N. Keshavan, B. Basu","doi":"10.1080/09506608.2022.2047419","DOIUrl":"https://doi.org/10.1080/09506608.2022.2047419","url":null,"abstract":"ABSTRACT Ultra-high molecular weight polyethylene (UHMWPE) materials have played a significant role in the field of reconstructive surgery, particularly as acetabular liners/sockets for total hip joint replacement (THR), and tibial inserts for total knee joint replacement (TKR). This review aims to provide a perspective on key elements regarding the processing–structure–property relationship of UHMWPE and derivatives. Much emphasis will be provided to discuss the clinically relevant properties of UHMWPE blend/composite formulation, Vitamin-E reinforced or highly crosslinked variants. In addition, we provide clinical insights into the role of wear debris in inflammation and osteolysis. The relatively unexplored domain of UHMWPE additive manufacturing. Finally, the relatively unexplored domain of UHMWPE additive manufacturing and the opportunities associated with the next generation of UHMWPE implants are highlighted. GRAPHICAL ABSTRACT","PeriodicalId":14427,"journal":{"name":"International Materials Reviews","volume":"68 1","pages":"46 - 81"},"PeriodicalIF":16.1,"publicationDate":"2022-05-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"46739441","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2022-05-19DOI: 10.1080/09506608.2022.2077030
Cong Chen, Jinwei Gao, S. Feng
ABSTRACT Perovskite solar cells are promising candidates for next-generation photovoltaic devices with certified power-conversion efficiency for single-junction perovskite-based devices exceeded 25%. However, it remains challenging to fabricate a large-area and dense perovskite film using solution-based deposition methods. This is due to perovskite wet films being highly sensitive and unstable, and thus having only a narrow processing window. There is therefore a demand for ways to expand the processing window in the fabrication of perovskite films. Herein, we systematically review research on the role of precursor solutions and antisolvents during the perovskite formation process, and reveal the fundamental factors governing the width of the perovskite film-processing window. Then, we give an overview of current strategies for enlarging the processing window, which includes solvent and antisolvent engineering strategies. We conclude by summarizing current challenges in the development of perovskite solar modules with a wide processing window and provide perspectives for future development.
{"title":"The strategies for widening processing windows for perovskite solar cells: a mini review on the role of solvent/antisolvent","authors":"Cong Chen, Jinwei Gao, S. Feng","doi":"10.1080/09506608.2022.2077030","DOIUrl":"https://doi.org/10.1080/09506608.2022.2077030","url":null,"abstract":"ABSTRACT Perovskite solar cells are promising candidates for next-generation photovoltaic devices with certified power-conversion efficiency for single-junction perovskite-based devices exceeded 25%. However, it remains challenging to fabricate a large-area and dense perovskite film using solution-based deposition methods. This is due to perovskite wet films being highly sensitive and unstable, and thus having only a narrow processing window. There is therefore a demand for ways to expand the processing window in the fabrication of perovskite films. Herein, we systematically review research on the role of precursor solutions and antisolvents during the perovskite formation process, and reveal the fundamental factors governing the width of the perovskite film-processing window. Then, we give an overview of current strategies for enlarging the processing window, which includes solvent and antisolvent engineering strategies. We conclude by summarizing current challenges in the development of perovskite solar modules with a wide processing window and provide perspectives for future development.","PeriodicalId":14427,"journal":{"name":"International Materials Reviews","volume":"68 1","pages":"301 - 322"},"PeriodicalIF":16.1,"publicationDate":"2022-05-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"48023646","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2022-05-19DOI: 10.1080/09506608.2022.2077029
D. Dudina, K. Georgarakis, E. Olevsky
ABSTRACT Aluminium and magnesium matrix composites are attractive lightweight materials with strength surpassing that of the corresponding matrix metals. Recent years have seen extensive research aimed at finding ways to control the structure of metal matrix composites and obtaining materials with new sets of properties. This review aims to show that field-assisted sintering is a promising approach for the powder metallurgy processing of aluminium and magnesium matrix composites. The review focuses on the achievements in the compositional and microstructural design and properties of aluminium and magnesium matrix composites obtained by spark plasma sintering, microwave sintering and induction sintering. Issues related to the process scale-up in the field-assisted sintering technologies are also addressed. GRAPHICAL ABSTRACT
{"title":"Progress in aluminium and magnesium matrix composites obtained by spark plasma, microwave and induction sintering","authors":"D. Dudina, K. Georgarakis, E. Olevsky","doi":"10.1080/09506608.2022.2077029","DOIUrl":"https://doi.org/10.1080/09506608.2022.2077029","url":null,"abstract":"ABSTRACT Aluminium and magnesium matrix composites are attractive lightweight materials with strength surpassing that of the corresponding matrix metals. Recent years have seen extensive research aimed at finding ways to control the structure of metal matrix composites and obtaining materials with new sets of properties. This review aims to show that field-assisted sintering is a promising approach for the powder metallurgy processing of aluminium and magnesium matrix composites. The review focuses on the achievements in the compositional and microstructural design and properties of aluminium and magnesium matrix composites obtained by spark plasma sintering, microwave sintering and induction sintering. Issues related to the process scale-up in the field-assisted sintering technologies are also addressed. GRAPHICAL ABSTRACT","PeriodicalId":14427,"journal":{"name":"International Materials Reviews","volume":"68 1","pages":"225 - 246"},"PeriodicalIF":16.1,"publicationDate":"2022-05-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"41890832","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2022-05-12DOI: 10.1080/09506608.2022.2069451
Ayda Afshar, Merve Gultekinoglu, M. Edirisinghe
ABSTRACT Binary polymer systems provide significant advantages in the preparation of materials used in biomedical applications. To highlight the importance and need of binary polymer systems in biomedical applications; utilisations of nano-carrier and fibre are discussed in detail in terms of their use as biomaterial, and their potential for further development with focus on dual and sequential drug delivery applications. On the other hand, in fibre technology, creation of binary polymer systems have been investigated using spinning processes such as electrospinning and even more recently innovated pressurised gyration. How these methods can be used to promote the mass production of binary polymer systems with various morphologies and characteristics are elucidated. The effects of different polymer materials, including solvents, mechanical properties, and the rate of degradation of polymers, are discussed. Current polymer blending systems and manufacturing processes are analysed, and technologies for biomaterials are carefully considered with up to date details.
{"title":"Binary polymer systems for biomedical applications","authors":"Ayda Afshar, Merve Gultekinoglu, M. Edirisinghe","doi":"10.1080/09506608.2022.2069451","DOIUrl":"https://doi.org/10.1080/09506608.2022.2069451","url":null,"abstract":"ABSTRACT Binary polymer systems provide significant advantages in the preparation of materials used in biomedical applications. To highlight the importance and need of binary polymer systems in biomedical applications; utilisations of nano-carrier and fibre are discussed in detail in terms of their use as biomaterial, and their potential for further development with focus on dual and sequential drug delivery applications. On the other hand, in fibre technology, creation of binary polymer systems have been investigated using spinning processes such as electrospinning and even more recently innovated pressurised gyration. How these methods can be used to promote the mass production of binary polymer systems with various morphologies and characteristics are elucidated. The effects of different polymer materials, including solvents, mechanical properties, and the rate of degradation of polymers, are discussed. Current polymer blending systems and manufacturing processes are analysed, and technologies for biomaterials are carefully considered with up to date details.","PeriodicalId":14427,"journal":{"name":"International Materials Reviews","volume":"68 1","pages":"184 - 224"},"PeriodicalIF":16.1,"publicationDate":"2022-05-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"43358713","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
ABSTRACT In recent years, the hydrogen economy has been strongly favoured by governmental and industrial bodies worldwide. A tremendous number of papers are published every year on different aspects of protonic ceramic electrochemical cells (PCECs) due to their lower operation temperature, easier reversible operation, and brighter prospects for further development. While new progress is being made continuously, many critical challenges remain. The effort on PCEC investigation could be more aligned for greater collective impact, e.g. the academic community could devote more effort to overdue critical problems but less to incremental improvements. This review aims to provide some insightful perspectives on critical challenges facing the development of PCECs, to sort out priorities in future effort, and to suggest promising directions to pursue. In this way, it is hoped that the technical readiness level of PCECs might advance more quickly, toward field demonstrations and commercialization for a clean and sustainable energy era. GRAPHICAL ABSTRACT
{"title":"Protonic ceramic materials for clean and sustainable energy: advantages and challenges","authors":"Hanchen Tian, Zheyu Luo, Yufei Song, Yucun Zhou, Mingyang Gong, Wenyuan Li, Zongping Shao, Meilin Liu, Xingbo Liu","doi":"10.1080/09506608.2022.2068399","DOIUrl":"https://doi.org/10.1080/09506608.2022.2068399","url":null,"abstract":"ABSTRACT In recent years, the hydrogen economy has been strongly favoured by governmental and industrial bodies worldwide. A tremendous number of papers are published every year on different aspects of protonic ceramic electrochemical cells (PCECs) due to their lower operation temperature, easier reversible operation, and brighter prospects for further development. While new progress is being made continuously, many critical challenges remain. The effort on PCEC investigation could be more aligned for greater collective impact, e.g. the academic community could devote more effort to overdue critical problems but less to incremental improvements. This review aims to provide some insightful perspectives on critical challenges facing the development of PCECs, to sort out priorities in future effort, and to suggest promising directions to pursue. In this way, it is hoped that the technical readiness level of PCECs might advance more quickly, toward field demonstrations and commercialization for a clean and sustainable energy era. GRAPHICAL ABSTRACT","PeriodicalId":14427,"journal":{"name":"International Materials Reviews","volume":"68 1","pages":"272 - 300"},"PeriodicalIF":16.1,"publicationDate":"2022-05-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"41715747","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
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