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Development and Validation of a Simultaneous Analytical Method for Six Anions in Drinking Water by Liquid Chromatography/Mass Spectrometry (LC/MS) 液相色谱/质谱(LC/MS)同时分析饮用水中6种阴离子的方法建立及验证
Pub Date : 2022-01-01 DOI: 10.2965/jswe.45.51
Norihiro Kobayashi, S. Takagi, Teruaki Kinoshita, Fumi Nakano, K. Furukawa, T. Kasuya, Shuhei Matsuhaba, Ikuo Teranaka, Tuyoshi Yamamoto, J. Yonekubo, Seiya Tanaka, Hiroyuki Niwa, Yuji Aita, Reika Takahara, Kaori Saito, Y. Ikarashi
1) Division of Environmental Chemistry, National Institute of Health Sciences, 3-25-26 Tonomachi, Kawasaki-ku, Kawasaki, Kanagawa 210-9501, Japan 2) Osaka Institute of Public Health, 1-3-69 Nakamichi, Higashinari-ku, Osaka 537-0025, Japan 3) Tokyo Metropolitan Institute of Public Health, 3-24-1 Hyakunincho, Shinjuku-ku, Tokyo 169-0073, Japan 4) Kanagawa Prefectural Institute of Public Health, 1-3-1 Shimomachiya, Chigasaki, Kanagawa 253-0087, Japan 5) Mie Prefecture Environmental Conservation Agency, 3258 Ueno, Kawage-cho, Tsu-shi, Mie 510-0304, Japan 6) Chiba Pharmaceutical Association, 1-12-11 Chuoko, Chuo-ku, Chiba-shi, Chiba 260-0024, Japan 7) Gifu Research Center for Public Health, 4-6 Akebono-cho, Gifu-shi, Gifu 500-8148, Japan 8) Saitama Prefectural Water Quality Management Center, 1632 Kobari, Gyoda City, Saitama 361-0024, Japan 9) Yonago City Waterworks Bureau, 1047-1 Fukuichi, Yonago, Tottori 683-0011, Japan 10) Nihon Waters K.K., 1-3-12 Kitashinagawa, Shinagawa-ku, Tokyo 140-0001, Japan 11) Agilent Technologies Japan, Ltd., 9-1 Takakura-cho, Hachioji-shi, Tokyo 192-8510, Japan 12) Shimadzu Corporation, 1 Nishinokyo Kuwabara-cho, Nakagyo-ku, Kyoto 604-8511, Japan 13) K.K. AB Sciex, Gotenyama Trust Tower 21/F, 4-7-35 Kita Shinagawa, Shinagawa-ku, Tokyo 140-0001, Japan 14) GL Sciences Inc., 237-2 Sayamagahara, Iruma, Saitama 358-0032, Japan 15) Thermo Fisher Scientific K.K., 3-9 Moriya-cho, Kanagawa-ku, Yokohama-shi, Kanagawa 221-0022, Japan
1)国立健康科学研究所环境化学研究室,日本神奈川川市川崎区钟町3-25-26,日本神奈川县2100 -9501;2)大阪公共卫生研究所,大阪东成区中道1-3-69,日本大阪537-0025;3)东京都公共卫生研究所,东京新宿区百国町3-24-1,日本东京169-0073;4)神奈川县公共卫生研究所,神奈川市下町町1-3-1,日本神奈川县253-0087;日本5)Mie县环境保护厅,3258上野,川崎町,津市,Mie 5100304;日本6)千叶县医药协会,1-12-11,中部,千叶市,千叶市,260-0024;日本7)岐阜市公共卫生研究中心,4-6,岐阜市,岐阜500-8148;日本8)埼玉县水质管理中心,日本361-0024;日本9)Yonago市自来水局,1047-1,Yonago, Fukuichi, Tottori, 683-0011;10)日本水公司,日本东京品川区北川1-3-12,日本东京140-0001;11)安捷科技日本有限公司,日本东京八良市高仓町9-1,日本东京192-8510;12)岛津公司,日本京都中古区东原町1号,日本京都604-8511;13)K.K. AB Sciex,日本御山信托大厦21楼,日本品川区北品川4-7-35,日本东京140-0001;14)GL科学公司,日本埼玉县入间市香原237-2,日本358-0032;15)赛默飞世尔科学公司,日本森谷町3-9;日本神奈川县横滨市神奈川区221-0022
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引用次数: 0
Long Term Trends of Dissolved Oxygen in Bottom Layer on the Vertical Distribution of Water Quality in Tokyo Bay 东京湾水质垂直分布中底层溶解氧的长期变化趋势
Pub Date : 2022-01-01 DOI: 10.2965/jswe.45.239
Satoko Yokoyama, Akira Iimura
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引用次数: 1
Estimation of Basic Unit Pollution Load of an Urban Area in the Lake Biwa Basin 琵琶湖流域城市区域基本单位污染负荷估算
Pub Date : 2022-01-01 DOI: 10.2965/jswe.45.21
K. Wada, H. Tsuno, N. Takei
From field surveys of roof runoff conducted in general residential houses in the Lake Biwa basin, the pollution loads of buildings in an urban area were evaluated. The samples were collected from the total roof drainage during a rainfall event, and the water pollutants investigated were total organic carbon ( TOC ) , total nitrogen ( TN ) , and total phosphorus ( TP ) . As a result, it was estimated that 67.7% of the total precipitation flowed out as roof wastewater, and it was clarified that the proportion of dissolved components was high in all cases. The calculated loads of TOC, TN, and TP from buildings were 60.4, 18.1, and 0.64 g ha -1 day -1 , respectively. By applying these loads and roadway loads in the Lake Biwa basin, the basic unit pollution loads of TOC, TN, and TP in the urban area of the Lake Biwa basin were estimated to be 140, 24.2, and 1.1 g ha -1 day -1 , respectively.
通过对琵琶湖流域普通住宅屋顶径流的实地调查,评价了城区建筑物的污染负荷。样品采集于某次降雨过程中屋面总排水中,水污染物主要为总有机碳(TOC)、总氮(TN)和总磷(TP)。结果表明,总降水中有67.7%以顶板废水的形式流出,并且在所有情况下,溶解成分的比例都很高。建筑物TOC、TN和TP的计算负荷分别为60.4、18.1和0.64 g ha -1 day -1。在琵琶湖流域应用这些荷载和道路荷载,估算出琵琶湖流域城区TOC、TN和TP的基本单位污染荷载分别为140、24.2和1.1 g ha -1 day -1。
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引用次数: 0
Development of Marine Fertilizer Made from Ripened Chicken Manure Compost 熟鸡粪堆肥制海用肥料的研制
Pub Date : 2022-01-01 DOI: 10.2965/jswe.45.67
Tomotaka Ueno, Tamiji Yamamoto, K. Fukuoka
In the Seto Inland Sea, oligotrophication due to the long-term reduction measures of nitrogen and phosphorus, which is evidenced by the discoloration of nori laver and a decrease in fishery production, is pointed out. In this study, we developed a fertilizer that can elute nutrients required for the growth of marine organisms. The main ingredient of this fertilizer is chicken manure, to which steel slag and hardener were added, followed by pressing to form a solid fertilizer. To establish the proper N/P/Fe elution ratio for the growth of microalgae, elution tests using 500 L flasks were carried out with fertilizer pieces of different ingredient mixed ratios. A long-term elution test was also performed using the actual size fertilizer (25 cm diameter and 23 cm height) in 100 L containers under flow-through seawater systems. Elution of nutrients continued for longer than 5 months. It is concluded that the fertilizer developed in this study is useful for enhancing the growth of marine organisms.
指出濑户内海由于长期采取减少氮、磷的措施而出现了富营养化现象,其表现为紫菜变色和渔业产量减少。在这项研究中,我们开发了一种肥料,可以洗脱海洋生物生长所需的营养。这种肥料的主要成分是鸡粪,加入钢渣和硬化剂,然后压成固体肥料。为确定适宜微藻生长的N/P/Fe洗脱比例,采用500 L烧瓶进行了不同配比肥料块的洗脱试验。同时,采用实际尺寸的肥料(直径25 cm,高度23 cm)在100 L容器中进行了长期洗脱试验。营养物质的洗脱持续时间超过5个月。结果表明,本研究开发的肥料对促进海洋生物的生长有一定的作用。
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引用次数: 1
A Case Study for the Change in Antibiotic-Resistant Ratios of Escherichia coli Taken from Rivers in the Suburbs 郊区河流中大肠杆菌耐药率变化的个案研究
Pub Date : 2022-01-01 DOI: 10.2965/jswe.45.83
T. Urase, Yuito Kawano, Mio Sato
The antibiotic-resistant ratios of Escherichia coli taken from rivers in Kanagawa prefecture were investigated to clarify their changes since the early 2000s. A considerable number of isolates taken from urbanized rivers carried resistance to cefotaxime, indicating human-related sources such as combined sewer overflows and companion animals. On the other hand, some of the isolates from rivers in the suburbs carried simultaneous resistances to tetracycline and to sulfamethoxazole, which were associated with livestock farming. A comparison of resistant ratios in 2019 with those in the early 2000s shows a significant decrease in the resistance associated with livestock farming and an increase in the resistance to levofloxacin and to gentamicin, although this increase was not statistically significant.
从神奈川县的河流中提取的大肠杆菌的抗生素耐药比率进行了调查,以阐明其自21世纪初以来的变化。从城市化河流中提取的相当数量的分离株对头孢噻肟具有耐药性,这表明与人类有关的来源,如联合下水道溢流和伴侣动物。另一方面,来自郊区河流的一些分离株同时对四环素和磺胺甲恶唑具有耐药性,这与畜牧业有关。将2019年的耐药率与21世纪初的耐药率进行比较后发现,与畜牧业相关的耐药率显著下降,对左氧氟沙星和庆大霉素的耐药率上升,尽管这种上升没有统计学意义。
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引用次数: 0
Appropriate Construction Volume of Granulated Coal Ash for Suppression of Hydrogen Sulfide Generation from Dredged Pit in Lake Nakaumi 抑制中海湖疏浚坑硫化氢生成适宜颗粒粉煤灰施工体积
Pub Date : 2022-01-01 DOI: 10.2965/jswe.45.207
Tamiji Yamamoto, Shunsuke Nakahara, T. Kuwabara, K. Nakamoto, Tadashi Saito, K. Hino
{"title":"Appropriate Construction Volume of Granulated Coal Ash for Suppression of Hydrogen Sulfide Generation from Dredged Pit in Lake Nakaumi","authors":"Tamiji Yamamoto, Shunsuke Nakahara, T. Kuwabara, K. Nakamoto, Tadashi Saito, K. Hino","doi":"10.2965/jswe.45.207","DOIUrl":"https://doi.org/10.2965/jswe.45.207","url":null,"abstract":"","PeriodicalId":16300,"journal":{"name":"Journal of Japan Society on Water Environment","volume":null,"pages":null},"PeriodicalIF":0.0,"publicationDate":"2022-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"77110066","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Behavior of Biopolymers in Integrated Membrane System for Reclamation of Municipal Wastewater Effluent 生物聚合物在城市污水综合膜系统中的性能研究
Pub Date : 2022-01-01 DOI: 10.2965/jswe.45.159
Mifuyu Harada, Tasuma Suzuki, Y. Wada, Shigetoshi Ichimura
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引用次数: 0
Impact of Variation in Nutrient Concentration on Ecosystem, Biomass, and Production in a Semi-enclosed Embayment: Osaka Bay 半封闭港湾大阪湾营养物浓度变化对生态系统、生物量和产量的影响
Pub Date : 2022-01-01 DOI: 10.2965/jswe.45.145
T. Fujiwara, Kentaro Suzuki, Naoko Kimura, Motoharu Suzuki, M. Nakajima, K. Tadokoro, K. Abo
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引用次数: 3
Nitrogen Removal from Real Sewage Pretreated with Anaerobic Membrane Bioreactors Using One-Stage Partial Nitritation-Anammox Process with Hydroxyapatite Crystallization and Partial Nitritation-Anammox Granule 厌氧膜生物反应器预处理真实污水的部分亚硝化-厌氧氨氧化-羟基磷灰石结晶-部分亚硝化-厌氧氨氧化颗粒法脱氮研究
Pub Date : 2022-01-01 DOI: 10.2965/jswe.45.1
S. Nitta, Riku Izumida, Runda Du, Yisong Hu, Y. Li
To apply the one-stage partial nitritation-anammox (PNA) process to municipal mainstream wastewater, an experiment on continuous nitrogen removal using hydroxyapatite crystallization and partial nitritation-anammox (HAP-PNA) granule was conducted at 25 °C using real sewage pretreated with anaerobic membrane bioreactors (AnMBR). In the sewage adaptation period, the ammonium concentration of the sewage was firstly adjusted to 150 mg-N L and then gradually decreased to 100 and then to 50 mg-N L. Finally, the real sewage treatment with the ammonium concentration of 33 mg-N L for long-term operation at HRT of 2 h. Results of the continuous feeding tests for the real sewage treatment, showed that a nitrogen removal efficiency of 87% was obtained at HRT of 2 h, and the rates of ammonium oxidation and nitrogen removal by anammox bacteria were 0.20 and 0.34 kg-N (m d), respectively. From the results of microbial analysis, the top two dominant species were the anammox bacteria and AOB, with relative abundances of 30.2% (Candidatus Kuenenia stuttgartiensis) and 13.6% (Nitrosomonas sp.), respectively. Therefore, it was shown that AOB and anammox bacteria involved in the PNA process could be maintained during the real sewage treatment. This is the first demonstration of the successful operation and stable high performance of the PNA process with HAP-PNA granule for treating mainstream sewage.
为将一期部分亚硝化-厌氧氨氧化(PNA)工艺应用于城市主流废水,采用厌氧膜生物反应器(AnMBR)预处理的真实污水,在25℃条件下进行了羟基磷灰石结晶-部分亚硝化-厌氧氨氧化(HAP-PNA)颗粒连续脱氮实验。在污水适应期,污水的氨浓度先调整到150 mg-N L,然后逐渐降低到100 mg-N L,再降到50 mg-N L,最后以氨浓度为33 mg-N L的实际污水处理,在HRT 2 h下长期运行。对实际污水处理的连续投料试验结果表明,在HRT 2 h下,脱氮效率为87%。厌氧氨氧化菌的氨氧化和脱氮速率分别为0.20和0.34 kg-N (m d)。微生物分析结果显示,厌氧氨氧化菌和AOB的相对丰度最高,分别为30.2% (Candidatus Kuenenia stuttgartiensis)和13.6% (Nitrosomonas sp.)。因此,在实际的污水处理过程中,参与PNA过程的AOB和厌氧氨氧化菌是可以维持的。这是采用HAP-PNA颗粒处理主流污水的PNA工艺成功运行和稳定高性能的首次演示。
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引用次数: 0
Comparative Analysis of Plastic Pieces in Basin, River and Coast: Case Study in the Hikiji River Basin, Kanagawa Prefecture 盆地、河流和海岸塑料碎片的比较分析——以神奈川县志地河流域为例
Pub Date : 2022-01-01 DOI: 10.2965/jswe.45.11
S. Mishima, Kenji Ozawa, S. Nakayama, Hiromi Kikuchi, Ayumi Namba, T. Kataoka, Y. Nihei
Research on plastic debris in the ocean and rivers is being vigorously conducted, but there is little research on the dynamics of plastic from the basin, which is one of the sources of plastic waste, to rivers and coasts. In this study, we conducted a field survey of basins ( roads ), rivers, and coasts in the Hikichi River basin, Kanagawa Prefecture, with the aim of clarifying the dynamics of plastic pieces in the basin, river, and coast. From the results of the sample particle recovery test, the target size of the plastic piece in this study was set to be > 1 mm. The results indicated that the numerical and mass concentration of plastic pieces in the road dust between districts considered were significantly higher in the commercial and residential areas, respectively, mainly because of the difference in plastic piece size distribution. A comparison of plastic materials on roads, rivers, and coasts showed that polyethylene ( PE ), polypropylene ( PP ), and polystyrene ( PS ), which have low specific gravity, were predominant in the river and materials washed up on the coast, but not significant in the road dust.
对海洋和河流中的塑料碎片的研究正在大力进行,但对塑料从盆地(塑料废物的来源之一)到河流和海岸的动态研究却很少。在本研究中,我们对神奈川县日知河流域的盆地(道路)、河流和海岸进行了实地调查,目的是澄清盆地、河流和海岸中塑料碎片的动态。从样品颗粒回收试验的结果来看,本研究中塑料片的目标尺寸设定为>.1 mm。结果表明:城区道路粉尘中塑料碎片的数量和质量浓度均显著高于居民区,这主要是由于塑料碎片尺寸分布的差异造成的。对道路、河流和海岸的塑料材料进行了比较,结果表明,聚乙烯(PE)、聚丙烯(PP)和聚苯乙烯(PS)的比重较低,在河流和海岸冲上岸的材料中占主导地位,但在道路粉尘中不显著。
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引用次数: 0
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Journal of Japan Society on Water Environment
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