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Underground oil shale mine surveying using handheld mobile laser scanners 使用手持式移动激光扫描仪测量地下油页岩矿
IF 1.9 4区 工程技术 Q4 ENERGY & FUELS Pub Date : 2021-01-01 DOI: 10.3176/OIL.2021.1.03
A. Ellmann, S. Kanter, E. Väli
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引用次数: 0
Aspects of kerogen oxidative dissolution in subcritical water using oxygen from air 利用空气中的氧气在亚临界水中氧化溶解干酪根的几个方面
IF 1.9 4区 工程技术 Q4 ENERGY & FUELS Pub Date : 2021-01-01 DOI: 10.3176/oil.2021.3.02
K. Kaldas, A. Niidu, Gert Preegel, J. Uustalu, K. Muldma, M. Lopp
. Society’s growing demands on everyday products and materials are increasingly difficult to meet in an environment that seeks to avoid petroleum-based processes. Instead of abandoning fossil materials altogether, more research should be done on their efficient and clean conversion. One option for this is the oxidative dissolution of kerogen in water under conditions that satisfy the subcritical range (T = 150–200 °C, pO 2 = 0.5–4 MPa). The resulting mixture contains a substantial amount of various aliphatic carboxylic and dicarboxylic acids. Both batch and semi-continuous processes were set up to find the main factors and optimal conditions for the kerogen dissolution process. The rate of transformation of organic carbon to dissolved organic compounds was mainly influenced by elevated temperature and oxygen partial pressure. To obtain high yields of organic carbon dissolution and to avoid the formation of excess CO 2 , the oxidation of kerogen should be carried out fast (< 1 h) and under high oxygen pressure. By employing a temperature of 175 °C and O 2 pressure of 2 MPa, over 65% of the initial organic carbon dissolves in about one hour. Prolonged reaction times or harsher oxidation conditions resulted in a rapid degradation of dissolved matter and also of the valuable products formed. The organic matter content of the initial oil shale had a direct effect on the further degradation of dicarboxylic acid and consequently on the overall yield. The suitability of using a trickle-bed reactor for kerogen dissolution is discussed in detail on the basis of experimental results.
. 社会对日常产品和材料日益增长的需求越来越难以在一个寻求避免以石油为基础的过程的环境中得到满足。与其完全放弃化石材料,还不如对它们的高效和清洁转换进行更多的研究。其中一个选择是在满足亚临界范围(T = 150-200°C, p_2 = 0.5-4 MPa)的条件下,干酪根在水中的氧化溶解。所得到的混合物含有大量的各种脂肪族羧酸和二羧酸。建立了间歇式和半连续式两种工艺,找出了影响干酪根溶解的主要因素和最佳工艺条件。有机碳向溶解有机物转化的速率主要受温度升高和氧分压的影响。为了获得较高的有机碳溶解收率和避免过量co2的形成,干酪根的氧化应在高氧压下快速(< 1 h)进行。在175°C的温度和2mpa的o2压力下,超过65%的初始有机碳在大约一个小时内溶解。延长反应时间或严酷的氧化条件导致溶解物质和形成的有价值产品的迅速降解。初始油页岩的有机质含量直接影响二羧酸的进一步降解,从而影响总体产量。在实验结果的基础上,详细讨论了采用滴床反应器进行干酪根溶解的适宜性。
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引用次数: 2
The composition and properties of ash in the context of the modernisation of oil shale industry 油页岩工业现代化背景下灰分的组成和性质
IF 1.9 4区 工程技术 Q4 ENERGY & FUELS Pub Date : 2021-01-01 DOI: 10.3176/OIL.2021.2.04
T. Hain, R. Kuusik, L. Raado, J. Reinik, P. Somelar, Kadriann Tamm, A. Trikkel, M. Uibu, R. Viires
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引用次数: 3
Carbon dioxide sequestration in power plant Ca-rich ash waste deposits 电厂富钙灰废物沉积物中的二氧化碳封存
IF 1.9 4区 工程技术 Q4 ENERGY & FUELS Pub Date : 2021-01-01 DOI: 10.3176/OIL.2021.1.04
K. Kirsimäe, A. Konist, K. Leben, R. Mõtlep, T. Pihu
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引用次数: 5
Composition of gas from pyrolysis of Estonian oil shale with various sweep gases 爱沙尼亚油页岩热解气体组成与各种扫气
IF 1.9 4区 工程技术 Q4 ENERGY & FUELS Pub Date : 2021-01-01 DOI: 10.3176/oil.2021.3.03
Z. Baird, O. Järvik, S. Mozaffari
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引用次数: 2
The characteristics and kinetics of co-pyrolysis of furfural residue with oil shale semi-coke 糠醛渣油与油页岩半焦共热解特性及动力学研究
IF 1.9 4区 工程技术 Q4 ENERGY & FUELS Pub Date : 2021-01-01 DOI: 10.3176/OIL.2021.1.02
Y. Chen, J. Xuanyu, Y. Yang
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引用次数: 2
Numerical study of the flow, heat transfer and pyrolysis process in the gas full circulation oil shale retort 天然气全循环油页岩反应器内流动、传热及热解过程的数值研究
IF 1.9 4区 工程技术 Q4 ENERGY & FUELS Pub Date : 2021-01-01 DOI: 10.3176/oil.2021.4.03
F. Dai, J. Huang, H. Lu, L. Pan, S. Pei, Q. Wu
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引用次数: 3
General geology and geochemistry of the Lokpanta Formation oil shale, Nigeria 尼日利亚Lokpanta组油页岩一般地质地球化学特征
IF 1.9 4区 工程技术 Q4 ENERGY & FUELS Pub Date : 2021-01-01 DOI: 10.3176/OIL.2021.1.01
S. Ofili, A. Soesoo
. A detailed geochemical and mineralogical study was carried out on the Lokpanta oil shale (OS), Nigeria. Samples from three drill cores and several outcrops were studied in order to understand OS general geochemistry and reconstruct tectonic and depositional settings as well as paleoredox conditions. The mineral phases in OS include calcite, quartz, dolomite, feldspar, illite, kaolinite, halloysite, pyrite and gypsum, as well as a trace amount of anatase. The Lokpanta oil shale shows little variation in geochemistry. It is depleted in trace elements Ba and Rb and major compounds except CaO, and is enriched in trace elements Mo, Sb, As, V, Zn, Ni and U with reference to the Post-Archean Australian Shale (PAAS). These enrichments are, however, in most cases lower than those in the Estonian graptolite argillite (GA). Trace element ratios (U/Th, Ni/Co, V/Ni, V/(V + Ni) V/(V + Cr)) indicate that the Lokpanta oil shale was deposited in an anoxic environment. Discriminant diagrams also suggest its deposition in an active continental margin setting and a transitional to marine environment. The geochemical and paleoenvironmental features of the Lokpanta oil shale were compared with those of the Estonian graptolite argillite .
。对尼日利亚Lokpanta油页岩(OS)进行了详细的地球化学和矿物学研究。研究了三个岩心和几个露头样品,以了解OS的一般地球化学特征,重建构造和沉积环境以及古氧化还原条件。OS中的矿物相包括方解石、石英、白云石、长石、伊利石、高岭石、高岭石、黄铁矿和石膏,以及微量锐钛矿。Lokpanta油页岩地球化学特征变化不大。后太古宙澳大利亚页岩(PAAS)中微量元素Ba、Rb及除CaO外的主要化合物均富集,微量元素Mo、Sb、As、V、Zn、Ni、U富集。然而,在大多数情况下,这些富集程度低于爱沙尼亚笔石泥质岩的富集程度。微量元素比值(U/Th、Ni/Co、V/Ni、V/(V + Ni) V/(V + Cr))表明Lokpanta油页岩沉积于缺氧环境。判别图还表明其沉积于活动大陆边缘环境,并向海洋环境过渡。对比了Lokpanta油页岩与爱沙尼亚笔石泥岩的地球化学和古环境特征。
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引用次数: 8
Study on the permeability of oil shale during in situ pyrolysis 油页岩原位热解过程渗透率研究
IF 1.9 4区 工程技术 Q4 ENERGY & FUELS Pub Date : 2021-01-01 DOI: 10.3176/OIL.2021.2.02
Y. Geng, L. Li, Jianguo Liu
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引用次数: 2
Current status of co-pyrolysis of oil shale and biomass 油页岩与生物质共热解研究现状
IF 1.9 4区 工程技术 Q4 ENERGY & FUELS Pub Date : 2021-01-01 DOI: 10.3176/oil.2021.3.04
A. Cerón, A. Konist, H. Lees, O. Järvik
. The use of biomass (BM) and oil shale (OS) blends for the production of cleaner and improved fuels and chemicals through co-pyrolysis has recently attracted attention. The potential benefits, synergetic effects, interactions and promotion and inhibition effects of co-pyrolysis of BM and OS are reviewed and analyzed in this article based on an overview of various recent studies of co-pyrolysis, including the experimental and operational parameters and the yield and composition of the products. The effects of co-pyrolysis on different feedstock blends are discussed to guide future research on BM and OS copyrolysis. The effects of different pyrolysis parameters that can improve the pyrolysis process and quality of products are also reviewed. These parameters include CO 2 and steam atmospheres, heating rate, reaction temperature and particle size. Overall, in most cases reviewed, co-pyrolysis can enhance the yields of bio-oils, producer gas and chars as well as improve their properties while reducing the environmental effects of fossil fuels.
. 利用生物质(BM)和油页岩(OS)混合物通过共热解生产更清洁和改进的燃料和化学品最近引起了人们的关注。本文在综述近年来各种共热解研究的基础上,对BM和OS共热解的潜在效益、协同效应、相互作用以及促进和抑制作用进行了综述和分析,包括实验和操作参数、产物的产率和组成。讨论了共热解对不同原料共热解的影响,为今后BM和OS共热解的研究提供了指导。综述了不同热解参数对改善热解过程和产品质量的影响。这些参数包括二氧化碳和蒸汽气氛,加热速率,反应温度和颗粒大小。总的来说,在大多数情况下,共热解可以提高生物油、生产者气和木炭的产量,并改善其性能,同时减少化石燃料对环境的影响。
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引用次数: 4
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