Joseph Garbarino, John G. Jones, Peter R. Stevenson, Cynthia T. Bowers, Krishnamurthy Mahalingam, and Lyuba Kuznetsova
Electrically tunable TiN/SiO2/TiN epsilon-near-zero photonic structures with various parameters were fabricated using the reactive DC magnetron sputtering approach. Effective medium approximation was used to predict the optical permittivity of a multilayered TiN/SiO2 metamaterial and guide the design/fabrication. Experimental reflectance measurements for tunable TiN/SiO2/TiN structures were obtained using the ellipsometer technique in the visible and near-infrared spectral ranges. Results show that reflectance for biased (12 V) and un-biased bulk TiN/SiO2/TiN structure changes up to ∼ 2% with the spectral shift at the ENZ spectral point ∼ 10 nm for samples with an optimal SiO2 dielectric layer (thickness d=10 nm). Reflectance measurements for multilayered tunable TiN/SiO2/TiN structures show strong variation in reflectance change for s- polarized light at epsilon-near-zero wavelengths due to applied voltage (12 V). We expect that the results of this research study of the tunable TiN/SiO2/TiN epsilon-near-zero photonic structures will potentially be useful for the photonic density of states engineering, surface sensing, and metamaterial-based super-resolution imaging.
{"title":"Engineering electrically tunable TiN/SiO2 epsilon-near-zero metamaterials","authors":"Joseph Garbarino, John G. Jones, Peter R. Stevenson, Cynthia T. Bowers, Krishnamurthy Mahalingam, and Lyuba Kuznetsova","doi":"10.1364/ome.519794","DOIUrl":"https://doi.org/10.1364/ome.519794","url":null,"abstract":"Electrically tunable TiN/SiO<sub>2</sub>/TiN epsilon-near-zero photonic structures with various parameters were fabricated using the reactive DC magnetron sputtering approach. Effective medium approximation was used to predict the optical permittivity of a multilayered TiN/SiO<sub>2</sub> metamaterial and guide the design/fabrication. Experimental reflectance measurements for tunable TiN/SiO<sub>2</sub>/TiN structures were obtained using the ellipsometer technique in the visible and near-infrared spectral ranges. Results show that reflectance for biased (12 V) and un-biased bulk TiN/SiO<sub>2</sub>/TiN structure changes up to ∼ 2% with the spectral shift at the ENZ spectral point ∼ 10 nm for samples with an optimal SiO<sub>2</sub> dielectric layer (thickness d=10 nm). Reflectance measurements for multilayered tunable TiN/SiO<sub>2</sub>/TiN structures show strong variation in reflectance change for s- polarized light at epsilon-near-zero wavelengths due to applied voltage (12 V). We expect that the results of this research study of the tunable TiN/SiO<sub>2</sub>/TiN epsilon-near-zero photonic structures will potentially be useful for the photonic density of states engineering, surface sensing, and metamaterial-based super-resolution imaging.","PeriodicalId":19548,"journal":{"name":"Optical Materials Express","volume":null,"pages":null},"PeriodicalIF":2.8,"publicationDate":"2024-04-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140573343","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Au nanoplates with tunable in-plane dipolar localized surface plasmon resonance peaks in a broad range from the visible to near-infrared region were obtained in high yield using a seedless wet chemical growth method after purification. Cetyltrimethylammonium chloride was used as a surfactant, while hydrogen peroxide and sodium borohydride were used as the weak and strong reducing agents, respectively. The edge length and in-plane dipolar localized surface plasmon resonance peak of the Au nanoplates could be adjusted by varying the amounts of hydrogen peroxide and sodium borohydride. The Au nanoplates were further used as the saturable absorber to generate pulsed laser output in a passively Q-switched solid-state laser at approximately 2 µm. Our study offers a new method for obtaining Au nanoplates with tunable plasmonic peaks over a broad range.
{"title":"Seedless synthesis of Au nanoplates with tunable plasmonic peaks","authors":"Yuhao Zheng, Min Li, and Deyuan Shen","doi":"10.1364/ome.522159","DOIUrl":"https://doi.org/10.1364/ome.522159","url":null,"abstract":"Au nanoplates with tunable in-plane dipolar localized surface plasmon resonance peaks in a broad range from the visible to near-infrared region were obtained in high yield using a seedless wet chemical growth method after purification. Cetyltrimethylammonium chloride was used as a surfactant, while hydrogen peroxide and sodium borohydride were used as the weak and strong reducing agents, respectively. The edge length and in-plane dipolar localized surface plasmon resonance peak of the Au nanoplates could be adjusted by varying the amounts of hydrogen peroxide and sodium borohydride. The Au nanoplates were further used as the saturable absorber to generate pulsed laser output in a passively Q-switched solid-state laser at approximately 2 µm. Our study offers a new method for obtaining Au nanoplates with tunable plasmonic peaks over a broad range.","PeriodicalId":19548,"journal":{"name":"Optical Materials Express","volume":null,"pages":null},"PeriodicalIF":2.8,"publicationDate":"2024-04-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140573186","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
R. E. López-Romero, G. G. Pérez-Sánchez, I. Aldaya, D. Y. Medina, E. L. Martínez-Piñeiro, I. A. Figueroa, and R. Escudero
Erbium is well-recognized as a key element for optical amplification at the 1550 nm operation band. However, the limited solubility of this material in vitreous matrices sets a critical constraint to the achievable optical gain, which limits its applicability in photonic integrated platforms. One of the solutions to increase the concentration of erbium is to employ a crystalline structure instead of a glass. In this paper, we characterize samples of erbium and erbium-ytterbium oxalate single crystals synthesized using the gel diffusion method. X-ray diffraction spectra and thermogravimetric analyses reveal that the synthesis method indeed generated the expected compound, and the pump-and-probe experiments demonstrate an on-off gain coefficient of ≈ 6.5 dB/mm, making this material a high-potential candidate for the implementation of integrated optical amplifiers.
{"title":"Characterization of the optical gain at 1550 nm of erbium-oxalate single crystals","authors":"R. E. López-Romero, G. G. Pérez-Sánchez, I. Aldaya, D. Y. Medina, E. L. Martínez-Piñeiro, I. A. Figueroa, and R. Escudero","doi":"10.1364/ome.515335","DOIUrl":"https://doi.org/10.1364/ome.515335","url":null,"abstract":"Erbium is well-recognized as a key element for optical amplification at the 1550 nm operation band. However, the limited solubility of this material in vitreous matrices sets a critical constraint to the achievable optical gain, which limits its applicability in photonic integrated platforms. One of the solutions to increase the concentration of erbium is to employ a crystalline structure instead of a glass. In this paper, we characterize samples of erbium and erbium-ytterbium oxalate single crystals synthesized using the gel diffusion method. X-ray diffraction spectra and thermogravimetric analyses reveal that the synthesis method indeed generated the expected compound, and the pump-and-probe experiments demonstrate an on-off gain coefficient of ≈ 6.5 dB/mm, making this material a high-potential candidate for the implementation of integrated optical amplifiers.","PeriodicalId":19548,"journal":{"name":"Optical Materials Express","volume":null,"pages":null},"PeriodicalIF":2.8,"publicationDate":"2024-04-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140573016","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Hirofumi Morisawa, Atsushi Ono, Koki Ikegami, Wataru Inami, and Yoshimasa Kawata
We measured the photoelectron emission efficiency of aluminum (Al) nanohole arrays fabricated by colloidal lithography and demonstrated the enhancement of photoelectron emission in the deep-UV region via surface plasmon resonances. The Al nanohole arrays for increasing absorption in the deep-UV region were designed using the finite-difference time-domain method and used as photocathodes to enhance the photoelectron emission efficiency. The enhancement factor improved by up to 3.5 times for the optimized nanohole array. Using a two-dimensional mapping system, we demonstrated that the photoelectron emission depended on the uniformity of the sample and diameter of the nanohole arrays. Al nanohole arrays fabricated by colloidal lithography can be used to develop highly sensitive surface-detecting optical sensors and highly efficient surface-emitting electron sources. The two-dimensional mapping system can facilitate the development of highly efficient photocathodes.
{"title":"Enhanced photoelectron emission in a large area aluminum nanohole array via a deep-UV surface plasmon","authors":"Hirofumi Morisawa, Atsushi Ono, Koki Ikegami, Wataru Inami, and Yoshimasa Kawata","doi":"10.1364/ome.522182","DOIUrl":"https://doi.org/10.1364/ome.522182","url":null,"abstract":"We measured the photoelectron emission efficiency of aluminum (Al) nanohole arrays fabricated by colloidal lithography and demonstrated the enhancement of photoelectron emission in the deep-UV region via surface plasmon resonances. The Al nanohole arrays for increasing absorption in the deep-UV region were designed using the finite-difference time-domain method and used as photocathodes to enhance the photoelectron emission efficiency. The enhancement factor improved by up to 3.5 times for the optimized nanohole array. Using a two-dimensional mapping system, we demonstrated that the photoelectron emission depended on the uniformity of the sample and diameter of the nanohole arrays. Al nanohole arrays fabricated by colloidal lithography can be used to develop highly sensitive surface-detecting optical sensors and highly efficient surface-emitting electron sources. The two-dimensional mapping system can facilitate the development of highly efficient photocathodes.","PeriodicalId":19548,"journal":{"name":"Optical Materials Express","volume":null,"pages":null},"PeriodicalIF":2.8,"publicationDate":"2024-04-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140573018","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Xin Chang, Mike Pivnenko, Angadjit Singh, Weijie Wu, Pawan Shrestha, and Daping Chu
Metasurface technology is progressing rapidly towards commercialization and productization, due to its unparallelled advantages over conventional optical solutions. The reconfigurable metasurface, exhibiting more flexibility and capacity than its static counterpart, has been one of the most pursued features of metasurface. In this work, we present liquid crystal-based dynamic metasurface by immersing metasurface in nematic liquid crystal environment. No alignment material was used, and liquid crystal was aligned directly by metasurface. The alignment quality was characterized and the intensity contrast of 33 was obtained. Optical amplitude modulation was achieved with the modulation depth of 91% at the wavelength of 1375 nm. Moreover, sub-micrometre cell gap of 875 nm was realized, and the response time was measured to be sub-millisecond at room temperature, translating to > 1KHz operation frequency. The higher operation frequency of > 3.4 KHz was recorded at elevated temperature. The key performance indicators demonstrated in this work showcase the promising future of liquid crystal – based reconfigurable metasurface, especially for fast light modulator applications.//Metasurface technology is progressing rapidly toward commercialization and productization due to its unparalleled advantages over conventional optical solutions. The reconfigurable metasurface, exhibiting more flexibility and capacity than its static counterpart, has been one of the most pursued features of the metasurface. In this work, we present a liquid crystal-based dynamic metasurface by immersing the metasurface in a nematic liquid crystal environment. No alignment material was used, and liquid crystal was aligned directly by metasurface. The alignment quality was characterized, and the intensity contrast of 33 was obtained. Optical amplitude modulation was achieved with a modulation depth of 91% at the wavelength of 1375 nm. Moreover, a sub-micrometer cell gap of 875 nm was realized, and the response time was measured to be sub-millisecond at room temperature, translating to > 1KHz operation frequency. The higher operation frequency of > 3.4 KHz was recorded at elevated temperatures. The key performance indicators demonstrated in this work showcase the promising future of liquid crystal-based reconfigurable metasurface, especially for fast light modulator applications.
{"title":"Fast-switching reconfigurable metadevice with metasurface-induced liquid crystal alignment for light modulator applications","authors":"Xin Chang, Mike Pivnenko, Angadjit Singh, Weijie Wu, Pawan Shrestha, and Daping Chu","doi":"10.1364/ome.520326","DOIUrl":"https://doi.org/10.1364/ome.520326","url":null,"abstract":"Metasurface technology is progressing rapidly towards commercialization and productization, due to its unparallelled advantages over conventional optical solutions. The reconfigurable metasurface, exhibiting more flexibility and capacity than its static counterpart, has been one of the most pursued features of metasurface. In this work, we present liquid crystal-based dynamic metasurface by immersing metasurface in nematic liquid crystal environment. No alignment material was used, and liquid crystal was aligned directly by metasurface. The alignment quality was characterized and the intensity contrast of 33 was obtained. Optical amplitude modulation was achieved with the modulation depth of 91% at the wavelength of 1375 nm. Moreover, sub-micrometre cell gap of 875 nm was realized, and the response time was measured to be sub-millisecond at room temperature, translating to > 1KHz operation frequency. The higher operation frequency of > 3.4 KHz was recorded at elevated temperature. The key performance indicators demonstrated in this work showcase the promising future of liquid crystal – based reconfigurable metasurface, especially for fast light modulator applications.//Metasurface technology is progressing rapidly toward commercialization and productization due to its unparalleled advantages over conventional optical solutions. The reconfigurable metasurface, exhibiting more flexibility and capacity than its static counterpart, has been one of the most pursued features of the metasurface. In this work, we present a liquid crystal-based dynamic metasurface by immersing the metasurface in a nematic liquid crystal environment. No alignment material was used, and liquid crystal was aligned directly by metasurface. The alignment quality was characterized, and the intensity contrast of 33 was obtained. Optical amplitude modulation was achieved with a modulation depth of 91% at the wavelength of 1375 nm. Moreover, a sub-micrometer cell gap of 875 nm was realized, and the response time was measured to be sub-millisecond at room temperature, translating to > 1KHz operation frequency. The higher operation frequency of > 3.4 KHz was recorded at elevated temperatures. The key performance indicators demonstrated in this work showcase the promising future of liquid crystal-based reconfigurable metasurface, especially for fast light modulator applications.","PeriodicalId":19548,"journal":{"name":"Optical Materials Express","volume":null,"pages":null},"PeriodicalIF":2.8,"publicationDate":"2024-03-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140322478","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Photonic time interfaces, as the temporal analogue of spatial interfaces between two media, consist of a rapid change of the electromagnetic properties of a material (such as permittivity, ε, and permeability, μ) while the wave is present in the material. Here we exploit cascading of such time interfaces in spatially cascaded guided-wave structures such as slab waveguides and ring resonators by considering that the relative permittivity of the cladding of dielectric waveguides is rapidly changed at different moments of time from εclad_1 to εclad_2, while the material of the core remains unchanged in time. It is shown how such time-dependent cladding can enable frequency conversion within the space-time dielectric ring resonator and slab waveguides due to an induced modification of the effective refractive index of the mode propagating within such photonic device. Cascaded frequency conversion is achieved in such cascaded space-time dielectric waveguides and ring resonators, showing how the combination of space and time interfaces can offer further opportunities for manipulation of light-matter interaction using four-dimensional (4D) photonic structures.
{"title":"Spatiotemporal cascading of dielectric waveguides [Invited]","authors":"Victor Pacheco-Peña and Nader Engheta","doi":"10.1364/ome.516262","DOIUrl":"https://doi.org/10.1364/ome.516262","url":null,"abstract":"Photonic time interfaces, as the temporal analogue of spatial interfaces between two media, consist of a rapid change of the electromagnetic properties of a material (such as permittivity, <i>ε</i>, and permeability, <i>μ</i>) while the wave is present in the material. Here we exploit cascading of such time interfaces in spatially cascaded guided-wave structures such as slab waveguides and ring resonators by considering that the relative permittivity of the cladding of dielectric waveguides is rapidly changed at different moments of time from <i>ε<sub>clad_1</sub></i> to <i>ε<sub>clad_2</sub></i>, while the material of the core remains unchanged in time. It is shown how such time-dependent cladding can enable frequency conversion within the space-time dielectric ring resonator and slab waveguides due to an induced modification of the effective refractive index of the mode propagating within such photonic device. Cascaded frequency conversion is achieved in such cascaded space-time dielectric waveguides and ring resonators, showing how the combination of space and time interfaces can offer further opportunities for manipulation of light-matter interaction using four-dimensional (4D) photonic structures.","PeriodicalId":19548,"journal":{"name":"Optical Materials Express","volume":null,"pages":null},"PeriodicalIF":2.8,"publicationDate":"2024-03-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140322562","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
{"title":"Simulating 4D Quantum Hall Effect with Two Bosons in a 1D Quasicrystal","authors":"Zhaoxin Wu, Junkai Li, Tuo Wan, Zhaoju Yang","doi":"10.1364/ome.521685","DOIUrl":"https://doi.org/10.1364/ome.521685","url":null,"abstract":"","PeriodicalId":19548,"journal":{"name":"Optical Materials Express","volume":null,"pages":null},"PeriodicalIF":2.8,"publicationDate":"2024-03-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140373959","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
M. Sakamoto, Kuon Kawamura, Masato Suzuki, Kohei Noda, T. Unuma, T. Sasaki, N. Kawatsuki, Hiroshi Ono
{"title":"Design and fabrication of liquid crystal retarder for the mid and far infrared wavelength ranges","authors":"M. Sakamoto, Kuon Kawamura, Masato Suzuki, Kohei Noda, T. Unuma, T. Sasaki, N. Kawatsuki, Hiroshi Ono","doi":"10.1364/ome.521677","DOIUrl":"https://doi.org/10.1364/ome.521677","url":null,"abstract":"","PeriodicalId":19548,"journal":{"name":"Optical Materials Express","volume":null,"pages":null},"PeriodicalIF":2.8,"publicationDate":"2024-03-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140376716","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
K. Kiedrowski, M. Ferraro, R. Jauberteau, S. Wabnitz, M. C. Crocco, Vincenzo Formoso, M. Jupé, Detlev Ristau
{"title":"Comparing the Laser-Induced Damage Distribution in POFs with Raytracing Simulations","authors":"K. Kiedrowski, M. Ferraro, R. Jauberteau, S. Wabnitz, M. C. Crocco, Vincenzo Formoso, M. Jupé, Detlev Ristau","doi":"10.1364/ome.520782","DOIUrl":"https://doi.org/10.1364/ome.520782","url":null,"abstract":"","PeriodicalId":19548,"journal":{"name":"Optical Materials Express","volume":null,"pages":null},"PeriodicalIF":2.8,"publicationDate":"2024-03-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"140376285","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
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