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Determination of the nonlinear thermal expansion coefficient of an epoxy used as expander and its effects over a Fabry-Perot cavity filled with a polymer. 测定用作膨胀剂的环氧树脂的非线性热膨胀系数及其对填充聚合物的法布里-珀罗空腔的影响。
IF 2.8 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-07-02 DOI: 10.1364/ome.533001
Everardo Vargas-Rodríguez, A. Guzmán-Chávez, Raja Zaman
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引用次数: 0
Enhanced p-type conductivity of hexagonal boron nitride by an efficient two-step doping strategy 通过高效的两步掺杂策略增强六方氮化硼的 p 型电导率
IF 2.8 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-06-27 DOI: 10.1364/ome.523859
Yuang Cheng, Yang Chen, Bingchen Lv, Zhiming Shi, Yuanyuan Yue, Yuping Jia, Ke Jiang, Xiaoyu Wei, Dabing Li, Shanli Zhang, Xiaojuan Sun
The present study proposes a two-step doping strategy for achieving efficient Mg doping of h-BN, involving an additional post-annealing treatment. This approach leads to ∼108-fold enhancement in conductivity of h-BN, compared with the as-doped h-BN grown by low-pressure chemical vapor deposition. The mechanism for large enhancement in h-BN doping efficiency after post-annealing was investigated, providing evidence that this treatment not only facilitates the nanoparticle decomposition and incorporation of Mg atoms into h-BN, but also restores its lattice defects. The efficient two-step doping strategy for p-type h-BN in this study enlightens its promising prospects for ultraviolet optoelectronic devices.
本研究提出了一种两步掺杂策略,以实现 h-BN 的高效镁掺杂,其中包括额外的退火后处理。与通过低压化学气相沉积法生长的原掺杂 h-BN 相比,这种方法使 h-BN 的电导率提高了~108 倍。研究表明,后退火处理不仅能促进纳米粒子的分解和镁原子在 h-BN 中的掺入,还能恢复 h-BN 的晶格缺陷。本研究中针对 p 型 h-BN 的高效两步掺杂策略启示了其在紫外光电子器件中的广阔前景。
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引用次数: 0
Femtosecond laser synthesis of YAG:Ce3+ nanoparticles in liquid 飞秒激光合成液态 YAG:Ce3+ 纳米粒子
IF 2.8 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-06-24 DOI: 10.1364/ome.530234
Pan Liang, Xin Jia, Hua Zhao, Rongrong Hu, Kai Jiang
YAG:Ce3+ nanocrystals are promising bio-labeling materials due to their low toxicity and high photostability. It is in demand to efficiently synthesize YAG:Ce3+ nanocrystals of a small size. Pulse laser ablation is an approach to produce nanoparticles directly from bulk materials with the advantages of smaller particle sizes and lower production costs. Here, we present the synthesis of YAG:Ce3+ nanocrystals from bulk crystal using the femtosecond laser ablation method in liquid. Comparing the liquid environment, we demonstrated that the lauryl dimethylaminoacetic acid betain (LDA) aqueous solution is preferred for the formation of smaller-sized YAG:Ce3+ nanoparticles than deionized water due to the attractiveness between the LDA molecules and the YAG:Ce3+ nanoparticles. We also verified that the high laser repetition rate had no effect on the average size of YAG:Ce3+ nanocrystals, where the fragmentation process is saturated under a high laser repetition rate. This study provides a simple and effective method to synthesize small size YAG:Ce3+ nanoparticles by femtosecond laser ablation in liquid.
YAG:Ce3+ 纳米晶体具有低毒性和高光稳定性,是一种前景广阔的生物标记材料。目前需要高效合成小尺寸的 YAG:Ce3+ 纳米晶体。脉冲激光烧蚀是一种直接从块状材料中生产纳米颗粒的方法,具有颗粒尺寸更小、生产成本更低的优点。在此,我们介绍了利用飞秒激光烧蚀法在液体中从块状晶体合成 YAG:Ce3+ 纳米晶体的过程。通过比较液体环境,我们证明月桂基二甲基氨基乙酸甜菜碱(LDA)水溶液比去离子水更适合形成较小尺寸的 YAG:Ce3+ 纳米粒子,这是由于 LDA 分子与 YAG:Ce3+ 纳米粒子之间存在吸引力。我们还验证了高激光重复率对 YAG:Ce3+ 纳米晶体的平均尺寸没有影响,在高激光重复率下,碎裂过程达到饱和。本研究提供了一种在液体中利用飞秒激光烧蚀合成小尺寸 YAG:Ce3+ 纳米粒子的简单而有效的方法。
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引用次数: 0
Silicon nanohole based enhanced light absorbers for thin film solar cell applications 应用于薄膜太阳能电池的基于硅纳米孔的增强型光吸收器
IF 2.8 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-06-24 DOI: 10.1364/ome.528499
Rony Das, Badhan Golder, Dip Sarker, Arif Ahammad
We proposed a nanohole-based silicon (Si) absorber structure to enhance the light absorption of thin-film Si solar cells. Our proposed structures exhibited excellent performances harnessing the light-matter interaction phenomenon with a few microns of thick Si (3 µm). We employed the finite-difference time-domain method to analyze the optical properties and solved Poisson’s, continuity, and heat transfer equations to analyze the electrical and thermal properties of our proposed structures, operating in the wavelength range from 300 to 1100 nm. We obtained a maximum average absorption of 72.6% for our proposed square hole Si absorber structure. The power conversion efficiency and short circuit current density were calculated to be 20.74% and 39.91 mA/cm2. We achieved polarization-insensitive performance due to the symmetrical nature of the structure. The temperature of our proposed structure was increased by ∼10 K due to light absorption for different ambient temperatures. Moreover, we found our proposed structure was thermally stable over time. Our proposed structures can enhance the absorption of Si nanostructures, which can be conducive to designing Si-thin solar cells for energy harvesting.
我们提出了一种基于纳米孔的硅吸收器结构,以增强薄膜硅太阳能电池的光吸收能力。我们提出的结构在几微米厚的硅片(3 微米)上就能利用光-物质相互作用现象,表现出卓越的性能。我们采用有限差分时域法分析了光学特性,并求解了泊松方程、连续性方程和传热方程,分析了我们提出的结构在 300 至 1100 纳米波长范围内的电学和热学特性。我们提出的方孔硅吸收器结构的最大平均吸收率为 72.6%。经计算,功率转换效率和短路电流密度分别为 20.74% 和 39.91 mA/cm2。由于结构的对称性,我们实现了对极化不敏感的性能。在不同的环境温度下,由于光吸收,我们提出的结构的温度升高了 10 K。此外,我们还发现我们提出的结构具有长期的热稳定性。我们提出的结构可以增强硅纳米结构的吸收能力,有利于设计用于能量收集的硅-薄太阳能电池。
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引用次数: 0
On the thermal stability of multilayer optics for use with high X-ray intensities 关于用于高强度 X 射线的多层光学器件的热稳定性
IF 2.8 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-06-24 DOI: 10.1364/ome.527226
Margarita Zakharova, Zlatko Rek, Božidar Šarler, Saša Bajt
High-intensity X-ray free electron laser (XFEL) beams require optics made of materials with minimal radiation absorption, high diffraction efficiency, and high radiation hardness. Multilayer Laue lenses (MLLs) are diffraction-based X-ray optics that can focus XFEL beams, as already demonstrated with tungsten carbide/silicon carbide (WC/SiC)-based MLLs. However, high atomic number materials such as tungsten strongly absorb X-rays, resulting in high heat loads. Numerical simulations predict much lower heat loads in MLLs consisting of low atomic number Z materials, although such MLLs have narrower rocking curve widths. In this paper, we first screen various multilayer candidates and then focus on Mo2C/SiC multilayer due to its high diffraction efficiency. According to numerical simulations, the maximum temperature in this multilayer should remain below 300°C if the MLL made out of this multilayer is exposed to an XFEL beam of 17.5 keV photon energy, 1 mJ energy per pulse and 10 kHz pulse repetition rate. To understand the thermal stability of the Mo2C/SiC multilayer, we performed a study on the multilayers of three different periods (1.5, 5, and 12 nm) and different Mo2C to SiC ratios. We monitored their periods, crystallinity, and stress as a function of annealing temperature for two different heating rates. The results presented in this paper indicate that Mo2C/SiC-based MLLs are viable for focusing XFEL beams without being damaged under these conditions.
高强度 X 射线自由电子激光器(XFEL)光束需要由辐射吸收最小、衍射效率高和辐射硬度高的材料制成的光学器件。多层劳厄透镜(MLL)是一种基于衍射的 X 射线光学器件,可以聚焦 XFEL 光束,基于碳化钨/碳化硅(WC/SiC)的多层劳厄透镜已经证明了这一点。然而,钨等高原子序数材料会强烈吸收 X 射线,从而导致高热负荷。数值模拟预测,由低原子序数 Z 材料组成的 MLL 的热负荷要低得多,尽管这种 MLL 的摇摆曲线宽度较窄。在本文中,我们首先筛选了各种候选多层材料,然后重点研究了具有高衍射效率的 Mo2C/SiC 多层材料。根据数值模拟,如果将该多层膜制成的 MLL 暴露在光子能量为 17.5 keV、每脉冲能量为 1 mJ、脉冲重复率为 10 kHz 的 XFEL 光束中,该多层膜的最高温度应保持在 300°C 以下。为了了解 Mo2C/SiC 多层的热稳定性,我们对三种不同周期(1.5、5 和 12 nm)和不同 Mo2C 与 SiC 比率的多层进行了研究。在两种不同的加热速率下,我们监测了它们的周期、结晶度和应力与退火温度的函数关系。本文介绍的结果表明,基于 Mo2C/SiC 的 MLL 可用于聚焦 XFEL 光束,而不会在这些条件下受到损坏。
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引用次数: 0
Temperature dependence of THz generation efficiency, THz refractive index, and THz absorption in lithium-niobate around 275 GHz 275 GHz 附近铌酸锂中太赫兹产生效率、太赫兹折射率和太赫兹吸收的温度依赖性
IF 2.8 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-06-18 DOI: 10.1364/ome.528491
Umit Demirbas, Christian Rentschler, Zhelin Zhang, Mikhail Pergament, Nicholas H. Matlis, Franz X. Kärtner
In this study, we demonstrate the capabilities of the pulse train excitation approach in determining key material properties of nonlinear crystals, such as refractive index, thermo-optic coefficient, and absorption. The method provides reliable results even at relatively low THz frequencies, where other characterization methods, such as THz time-domain spectroscopy, have difficulties. To illustrate the capabilities of our approach, we used pulse trains with 800-fs long pulses and adjustable time delay to investigate the material properties of periodically poled lithium niobate (PPLN) crystal with a poling period of 400 µm. Via scanning the incident pulse-train frequency, we measured the frequency response of the crystal at different temperatures (78-350 K), which enabled us to determine the temperature dependence of the refractive index and thermo-optic coefficient of the PPLN crystal around 275 GHz with very high precision. We further studied the variation of THz generation efficiency with temperature in detail to understand the temperature dependence of THz absorption in PPLN material. The technique employed is quite general and could be applied to both other frequency ranges and nonlinear crystals.
在这项研究中,我们展示了脉冲串激发方法在确定非线性晶体的关键材料特性(如折射率、热光学系数和吸收)方面的能力。该方法即使在相对较低的太赫兹频率下也能提供可靠的结果,而其他表征方法(如太赫兹时域光谱法)在这方面存在困难。为了说明我们方法的能力,我们使用了 800 fs 长脉冲和可调时间延迟的脉冲序列来研究极化周期为 400 µm 的周期性极化铌酸锂(PPLN)晶体的材料特性。通过扫描入射脉冲序列频率,我们测量了晶体在不同温度(78-350 K)下的频率响应,从而能够非常精确地确定 PPLN 晶体在 275 GHz 附近的折射率和热光学系数的温度依赖性。我们进一步详细研究了太赫兹产生效率随温度的变化,以了解 PPLN 材料的太赫兹吸收与温度的关系。所采用的技术非常通用,可应用于其他频率范围和非线性晶体。
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引用次数: 0
Ultrafast carrier dynamics and nonlinear optical absorption of two dimensional NiPS3 nanosheets 二维 NiPS3 纳米片的超快载流子动力学和非线性光学吸收
IF 2.8 3区 材料科学 Q2 Materials Science Pub Date : 2024-06-04 DOI: 10.1364/ome.525626
Ziyao Gong, Lei Yan, Qinyong He, Dechao Shen, Yunqi Yang, Anping Ge, Liaoxin Sun, Guohong ma, Saifeng Zhang
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引用次数: 0
Inkjet-printed waveguide-coupled passive wedge-shaped microdisk resonator with refractive index tunability 具有折射率可调性的喷墨打印波导耦合无源楔形微盘谐振器
IF 2.8 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-05-31 DOI: 10.1364/ome.528582
Frederik van Schoonhoven, Yoshitaka Tomishige, Adrian Abazi, Alejandro Sánchez-Postigo, Jinghan Chen, Yuya Mikami, Naoya Tate, Yuji Oki, Carsten Schuck, Hiroaki Yoshioka
We incorporate a passive wedge-shaped organic microdisk supporting spatially separated whispering gallery modes into an SU-8 photonic integrated circuit (PIC) by using direct inkjet printing. This innovative method allows the mixing of multiple organic materials, enabling tunability of the refractive index of microdisks, thereby overcoming limitations of single-material resonators from conventional lithography. In this study, the microdisk resonator, with a refractive index matching that of SU-8 by mixing hyperbranched polymers, is mounted horizontally to an optical waveguide, achieving directional coupling between the microdisk and PIC at a wavelength of 1550 nm. Geometrical conditions for successful coupling were obtained by measuring the cross-sectional profile of the fabricated structure’s surface via atomic force microscopy, determining ways to adjust the coupling efficiency.
我们利用直接喷墨打印技术,将支持空间分离的耳语画廊模式的无源楔形有机微盘集成到 SU-8 光子集成电路 (PIC) 中。这种创新方法可以混合多种有机材料,实现微盘折射率的可调性,从而克服了传统光刻技术中单一材料谐振器的局限性。在这项研究中,通过混合超支化聚合物使微盘谐振器的折射率与 SU-8 匹配,并将其水平安装到光波导上,从而实现了微盘与波长为 1550 nm 的 PIC 之间的定向耦合。通过原子力显微镜测量制造结构表面的横截面轮廓,获得了成功耦合的几何条件,从而确定了调整耦合效率的方法。
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引用次数: 0
Wide-mode-area slow light waveguides in valley photonic crystal heterostructures 山谷光子晶体异质结构中的宽模区慢光波导
IF 2.8 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-05-31 DOI: 10.1364/ome.525349
Chengkun Zhang, Yasutomo Ota, Satoshi Iwamoto
We designed slow-light waveguides with a wide mode area based on slab-type valley photonic crystal (VPhC) heterostructures which are composed of a graphene-like PhC sandwiched by two topologically distinct VPhCs. The group velocity of the topological guided mode hosted in a VPhC heterostructure can be slowed down by shifting the VPhC lattice toward the graphene-like PhC at the domain interfaces. Simultaneously, the mode width of the slow-light topological guided mode can be widened by increasing the size of the graphene-like PhC domain. We found that employing the graphene-like structure at the center domain is crucial for realizing a topological single-guided mode in such heterostructures. Furthermore, the impact of random fluctuations in air-hole size in the graphene-like domain was numerically investigated. Our simulation results demonstrate that the transmittance for the slow-light states can be kept high as far as the size fluctuation is small although it drops faster than that for fast-light states when the disorder level increases. The designed wide-mode-area slow-light waveguides are based on hole-based PhCs, offering novel on-chip applications of topological waveguides.
我们设计的慢光波导具有很宽的模式面积,它基于板状谷光子晶体(VPhC)异质结构,由两个拓扑不同的 VPhC 夹着一个类石墨烯 PhC 组成。通过在畴界面将 VPhC 晶格移向类石墨烯 PhC,可以减慢 VPhC 异质结构中寄存的拓扑导引模式的群速度。同时,通过增大类石墨烯 PhC 域的尺寸,可以拓宽慢光拓扑导引模式的模式宽度。我们发现,在中心畴采用类石墨烯结构是在此类异质结构中实现拓扑单导模的关键。此外,我们还在数值上研究了类石墨烯域中气孔尺寸随机波动的影响。我们的模拟结果表明,只要尺寸波动较小,慢光态的透射率就能保持较高水平,不过当无序度增加时,慢光态的透射率比快光态的透射率下降得更快。所设计的宽模区慢光波导基于孔基 PhC,为拓扑波导提供了新颖的片上应用。
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引用次数: 0
Design and fabrication of a porous prism film for display backlight applications 设计和制造用于显示器背光的多孔棱镜薄膜
IF 2.8 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-05-30 DOI: 10.1364/ome.528148
Fang-Hsuan Su, Ray-Hua Horng, Dong-Sing Wuu
This study demonstrates a fabrication method of a porous brightness enhancement film (pBEF) that offers brightness enhancement, light diffusion, color shift reduction, and improved thermal stability. During the ultraviolet imprinting and solvent evaporation processes, the nano/submicron-sized air pores are generated within the polymer prism structure, and micropatterns spontaneously form on the prism surface. The inner pores ranging from 30 to 450 nm can effectively scatter light to mitigate color shift, which is caused by multiple internal reflections within the prism structure. The micropatterns have multiple rings formed one around another with 5–15-µm diameter on the prism surface improve visual quality. Moreover, the obtained functions are achieved in a single film solution, obviating the need for using multiple materials, and the fabrication process is relatively simple and fast as it is conducted under ambient conditions. When the pBEF is integrated into a liquid-crystal display backlight, it provides the brightness enhancement performance and comparable viewing angle distribution of a regular BEF combined with an additional diffuser (two films) and increases brightness by ∼8% compared to a bead prism (particle-based BEF). Additionally, it reduces the redshift (Δxy) from 0.1605 to 0.1415. Furthermore, the pBEF exhibits a lower coefficient of thermal expansion than the regular BEF.
本研究展示了一种多孔增亮膜(pBEF)的制造方法,这种薄膜具有增亮、光扩散、减少色移和提高热稳定性等功能。在紫外线压印和溶剂蒸发过程中,聚合物棱镜结构内部会产生纳米/亚微米级的气孔,棱镜表面会自发形成微图案。内部 30 纳米到 450 纳米的气孔可有效散射光线,减轻棱镜结构内部多重反射造成的色移。在棱镜表面形成的直径为 5-15µm 的多个环状微图案提高了视觉质量。此外,所获得的功能只需一种薄膜溶液即可实现,无需使用多种材料,而且制作过程相对简单快捷,因为它是在环境条件下进行的。当 pBEF 集成到液晶显示器背光中时,它具有普通 BEF 的亮度增强性能和可比视角分布,并结合了额外的扩散器(两层薄膜),与珠棱镜(颗粒型 BEF)相比,亮度提高了 ∼ 8%。此外,它还将红移(Δxy)从 0.1605 降低到 0.1415。此外,pBEF 的热膨胀系数低于普通 BEF。
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引用次数: 0
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Optical Materials Express
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