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Temperature measurement and morphological/crystalline differences in the laser-induced carbonization of polydimethylsiloxane 聚二甲基硅氧烷激光诱导碳化过程中的温度测量和形态/晶体差异
IF 2.8 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-03-14 DOI: 10.1364/ome.514788
Masato Kai, Shuichiro Hayashi, Ken Kashikawa, and Mitsuhiro Terakawa
Laser-induced carbonization, which allows for the facile generation of graphitic carbon, is considered a promising technique for fabricating arbitrary conductive microstructures. The morphology and crystallinity of the resulting product are acknowledged to be significantly influenced by laser irradiation conditions. However, unlike discussions pertaining to furnaces where detailed considerations of applied temperature and resulting products are common, discussions on the process of laser-induced carbonization are limited. In recent years, reports have shown that using polydimethylsiloxane (PDMS) as a precursor material not only produces graphitic carbon but also results in the formation of silicon carbide. In this study, we utilized a thermographic camera to measure temperature changes during laser-induced carbonization, aiming to elucidate the correlation between PDMS temperature fluctuations and the morphology and crystallinity of the resulting graphitic carbon. The results demonstrate that the morphology and crystallinity of the graphitic carbon formed through laser-induced carbonization are not solely determined by the maximum temperature in the laser-irradiated area. The temperature changes during laser irradiation play a crucial role in the selective generation of these materials.
激光诱导碳化技术可以方便地生成石墨碳,被认为是制造任意导电微结构的一种有前途的技术。众所周知,激光辐照条件对所产生产品的形态和结晶度有很大影响。然而,与炉子的讨论不同的是,对应用温度和生成物的详细考虑很常见,而对激光诱导碳化过程的讨论却很有限。近年来,有报告显示,使用聚二甲基硅氧烷(PDMS)作为前驱体材料不仅能产生石墨碳,还能形成碳化硅。在本研究中,我们利用热成像摄像机测量激光诱导碳化过程中的温度变化,旨在阐明 PDMS 温度波动与所生成石墨碳的形态和结晶度之间的相关性。结果表明,通过激光诱导碳化形成的石墨碳的形态和结晶度并不完全取决于激光照射区域的最高温度。激光照射过程中的温度变化对这些材料的选择性生成起着至关重要的作用。
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引用次数: 0
High-throughput speckle spectrometers based on multifractal scattering media 基于多分形散射介质的高通量斑点光谱仪
IF 2.8 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-03-14 DOI: 10.1364/ome.511275
Bhupesh Kumar, Yilin Zhu, Luca Dal Negro, and Sebastian A. Schulz
We present compact integrated speckle spectrometers based on monofractal and multifractal scattering media in a silicon-on-insulator platform. Through both numerical and experimental studies we demonstrate enhanced optical throughput, and hence signal-to-noise ratio, for a number of random structures with tailored multifractal geometries without affecting the spectral decay of the speckle correlation functions. Moreover, we show that the developed multifractal media outperform traditional scattering spectrometers based on uniform random distributions of scattering centers. Our findings establish the potential of low-density random media with multifractal correlations for integrated on-chip applications beyond what is possible with uncorrelated random disorder.
我们在硅-绝缘体平台上展示了基于单分形和多分形散射介质的紧凑型集成斑点光谱仪。通过数值和实验研究,我们证明了在不影响斑点相关函数光谱衰减的情况下,采用定制多分形几何结构的随机结构可提高光学吞吐量和信噪比。此外,我们还发现所开发的多分形介质优于基于均匀随机散射中心分布的传统散射光谱仪。我们的研究结果确立了具有多分形相关性的低密度随机介质在片上集成应用的潜力,超越了无相关随机无序介质的应用范围。
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引用次数: 0
UV-VIS-NIR absorber to harvest energy for solar thermophotovoltaics 紫外-可见-近红外吸收器为太阳能光热发电收集能量
IF 2.8 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-03-14 DOI: 10.1364/ome.517791
Sumbel Ijaz, Muhammad Qasim Mehmood, Khaled A. Aljaloud, Rifaqat Hussain, Ali H. Alqahtani, and Akram Alomainy
Ideal ultraviolet-visible-infrared (UV-VIS-NIR) absorbers with consistent performance at elevated temperatures and severe climate conditions are crucial to harvest energy for solar-thermophotovoltaic systems (STPVs). As solar energy promises to fulfill the power demands, its efficient utilization through high-performing light-absorbing devices is inevitable. The requirement of high-temperature durability makes conventional plasmonics an infeasible choice, and those highly thermostable refractory metals/their derivatives suitable ones. In this work, a lossy refractory plasmonic material i.e. Zirconium-Nitride-based subwavelength, ultra-broadband, wide-angle, polarization-insensitive, and free-space impedance-matched metasurface absorber in a three-level Pythagorean fractal structure is demonstrated. A comprehensive investigative study is conducted with the successful attainment of more than 90% absorption between ∼ 500–900 nm with a peak of more than 98% at 655 nm. The mean absorption for wideband (200–2500 nm) is 86.01% and it is 91.37% for visible range. The proposed study provides an efficient choice of meta-absorbers for realizing highly efficient STPVs.
理想的紫外-可见-红外(UV-VIS-NIR)吸收器在高温和恶劣的气候条件下仍能保持稳定的性能,这对太阳能热光电系统(STPV)的能量收集至关重要。由于太阳能有望满足电力需求,因此通过高性能的光吸收装置高效利用太阳能势在必行。对高温耐久性的要求使得传统的等离子体成为不可行的选择,而那些高耐热性难熔金属/其衍生物则是合适的选择。在这项工作中,展示了一种有损耐火质子材料,即基于锆氮化物的亚波长、超宽带、广角、偏振不敏感和自由空间阻抗匹配的元表面吸收器,具有三层毕达哥拉斯分形结构。研究人员进行了全面的调查研究,成功地实现了 ∼ 500-900 nm 波长范围内超过 90% 的吸收率,在 655 nm 波长处的吸收率峰值超过 98%。宽波段(200-2500 nm)的平均吸收率为 86.01%,可见光范围为 91.37%。这项研究为实现高效 STPV 提供了有效的元吸收剂选择。
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引用次数: 0
Unveiling the potentiality of a self-powered CGT chalcopyrite-based photodetector: theoretical insights 揭示基于黄铜矿的自供电 CGT 光电探测器的潜力:理论见解
IF 2.8 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-03-12 DOI: 10.1364/ome.519847
Md. Islahur Rahman Ebon, Md. Alamin Hossain Pappu, Sheikh Noman Shiddique, and Jaker Hossain
The article demonstrates the design and modelling of CuGaTe2 direct bandgap (1.18 eV) chalcopyrite-based photodetector (PD), which has superb optical and electronic characteristics and shows remarkable performance on the photodetector. The photodetector has been investigated throughout the work by switching width, carrier and defect densities of particular layers and also the interface defect density of particular interfaces. The various layers have been optimized for the higher performance of the PD. Also, the impression of various device resistances has been analyzed. The JSC and VOC of the heterostructure photodetector is found to be 38.27 mA/cm2 and 0.94 V, in turn. The maximum responsivity, R and detectivity, D* are found to be 0.663A/W and 1.367 × 1016 Jones at a wavelength of 920 nm. The spectral response has a very high value in the range of 800 to 1000 nm light wavelength, which confirmed that this device is capable of detecting the near infrared (NIR) region of light. This work gives important guidance for the manufacture of CGT material-based photodetectors with higher performance.
文章展示了基于黄铜矿的 CuGaTe2 直接带隙(1.18 eV)光电探测器(PD)的设计和建模,该光电探测器具有极佳的光学和电子特性,并在光电探测器上表现出卓越的性能。在整个研究过程中,我们通过切换特定层的宽度、载流子密度和缺陷密度,以及特定界面的界面缺陷密度,对该光电探测器进行了研究。为了提高光电探测器的性能,对各层进行了优化。此外,还分析了各种器件电阻的影响。异质结构光电探测器的 JSC 和 VOC 分别为 38.27 mA/cm2 和 0.94 V。波长为 920 nm 时,最大响应率 R 和检测率 D* 分别为 0.663A/W 和 1.367 × 1016 Jones。光谱响应在 800 到 1000 nm 的光波长范围内具有非常高的值,这证实该装置能够检测近红外(NIR)光区。这项工作为制造具有更高性能的 CGT 材料光电探测器提供了重要指导。
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引用次数: 0
Hybrid Photonics: Integration, Design and Devices feature issue: publisher’s note 混合光子学:集成、设计与器件》特刊:出版商说明
IF 2.8 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-03-11 DOI: 10.1364/ome.523203
Sébastien Cueff, Joyce Poon, Dries Van Thourhout, and Laurent Vivien
“Invited” was added to the title of a paper [Opt. Mater. Express 14, 862 (2024) [CrossRef] ] in error.
"在一篇论文[Opt.Mater.Express 14, 862 (2024) [CrossRef] ] 错误。
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引用次数: 0
Independently regulating linearly and circularly polarized terahertz wave metasurface 独立调节线性和圆极化太赫兹波元表面
IF 2.8 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-03-11 DOI: 10.1364/ome.519712
Jiu-sheng Li, Ruo-tong Huang, and Ri-hui Xiong
We propose a terahertz metasurface that can independently regulate linearly circularly polarized waves. It consists of the top layer “O-O” metal pattern, polyimide layer, middle layer “I” shaped metal pattern, polyimide layer, and metal substrate from top to bottom. By using the phase principle of Pancharatnam Berry (PB) for encoding and arrangement, the metasurface generates vortex beams with different topological charges under circularly polarized terahertz wave incidence, and achieves focusing shift at different positions. Combining the convolution theorem for encoding arrangement, the metasurface can achieve focused vortex function under circularly polarized terahertz wave incidence. The designed metasurface can also generate Airy beam under linearly polarized terahertz wave incidence. The simulation results indicate that under different polarization (linear/circular polarization) terahertz wave incidence, the metasurface can achieve different functions, which provides a new approach for flexible control of terahertz waves.
我们提出了一种能独立调节线性圆极化波的太赫兹元表面。它由顶层 "O-O "型金属图案、聚酰亚胺层、中间层 "I "型金属图案、聚酰亚胺层和金属基板自上而下组成。利用 Pancharatnam Berry(PB)的相位原理进行编码和排列,元表面在圆极化太赫兹波入射下产生具有不同拓扑电荷的涡流束,并在不同位置实现聚焦偏移。结合卷积定理进行编码排列,元表面可在圆极化太赫兹波入射下实现聚焦涡旋功能。所设计的元表面还能在线性极化太赫兹波入射下产生艾里波束。仿真结果表明,在不同极化(线极化/圆极化)太赫兹波入射下,元表面可以实现不同的功能,这为灵活控制太赫兹波提供了一种新方法。
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引用次数: 0
Narrowband-seeded PPLN non-resonant optical parametric oscillator 窄带种子 PPLN 非共振光参量振荡器
IF 2.8 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-03-07 DOI: 10.1364/ome.517919
Tugba Temel, Robert T. Murray, Li Wang, Weidong Chen, André Schirrmacher, Ronan A. Battle, and Valentin Petrov
A PPLN non-resonant optical parametric oscillator injection-seeded by narrowband sub-100-mW CW radiation at the signal wavelength produces > 3 W idler average power at 2376 nm for a 20-kHz repetition rate, with a sub-2-nm spectral linewidth. The maximum quantum efficiency reaches 39.5%, roughly 1.4 times higher compared to narrowband operation achieved with a volume Bragg grating at the same pump level. Seed levels as low as 40 mW are sufficient to produce the desired spectral narrowing effect.
一个 PPLN 非共振光参量振荡器在信号波长处注入 100 毫瓦以下的窄带连续波辐射,在 2376 纳米波长处以 20 千赫的重复频率产生 3 瓦的惰极平均功率,光谱线宽为 2 纳米以下。最大量子效率达到 39.5%,与相同泵浦电平下使用体布拉格光栅实现的窄带操作相比,大约高出 1.4 倍。低至 40 mW 的种子电平就足以产生所需的光谱窄化效果。
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引用次数: 0
On the applicability of the Maxwell Garnett effective medium model to media with a high density of cylindrical pores 论麦克斯韦-加内特有效介质模型对高密度圆柱孔介质的适用性
IF 2.8 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-03-05 DOI: 10.1364/ome.516125
Julia Brandt, Guido Dittrich, Marc Thelen, Hagen Renner, Patrick Huber, Manfred Eich, and Alexander Petrov
The optical properties of dielectric materials with subwavelength cylindrical pores are commonly described by effective medium models. We compare the Maxwell Garnett and the Bruggeman effective medium models for porous silicon with simulations and experiments for the case of polarization orthogonal to the pore axis. The Maxwell Garnett model matches the results of the simulations even up to very high porosities. An experimental study of the effective permittivity of macroporous and mesoporous silicon is conducted by analyzing the Fabry-Pérot oscillations in the long-wavelength limit. These experimental results are also consistent with the Maxwell Garnett model. We advocate using this model for media with cylindrical pores in the future.
具有亚波长圆柱形孔隙的介电材料的光学特性通常用有效介质模型来描述。我们将多孔硅的麦克斯韦-加内特(Maxwell Garnett)和布鲁格曼(Bruggeman)有效介质模型与偏振与孔轴正交情况下的模拟和实验进行了比较。即使孔隙率非常高,麦克斯韦-加内特模型也能与模拟结果相匹配。通过分析长波长极限的法布里-佩罗特振荡,对大孔和介孔硅的有效介电常数进行了实验研究。这些实验结果也与麦克斯韦-加内特模型一致。我们主张今后将该模型用于具有圆柱形孔隙的介质。
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引用次数: 0
Random laser emission from dye-doped gain media with optically trapped scattering particles 带有光学捕获散射粒子的掺染增益介质的随机激光发射
IF 2.8 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-03-05 DOI: 10.1364/ome.510961
Takashi Okamoto, Naomichi Yokoi, and Takashi Kaku
In this study, an optical trapping technique is employed to manipulate the scatterer distribution within a random laser medium. By focusing the trapping beams into small regions within the three-dimensional scattering medium, the scattering particles around them are concentrated in those regions, resulting in an inhomogeneous scatterer distribution. The experimental results show that optical trapping increases the maximum spike intensity in the emission spectrum. Furthermore, the spectral spike intensity depends on the power of the trap spots. The relationship between the maximum and average spike intensities in the emission spectra exhibits a characteristic observed in other random lasers with inhomogeneous scatterer distributions.
本研究采用光学捕获技术来操纵随机激光介质中的散射体分布。通过将捕获光束聚焦到三维散射介质中的小区域,周围的散射粒子就会集中到这些区域,从而形成不均匀的散射体分布。实验结果表明,光学捕集增加了发射光谱中的最大尖峰强度。此外,光谱尖峰强度取决于陷阱光斑的功率。发射光谱中的最大尖峰强度和平均尖峰强度之间的关系显示了在其他具有不均匀散射体分布的随机激光器中观察到的特征。
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引用次数: 0
Effective medium metasurfaces using nanoimprinting of the refractive index: design, performance, and predictive tolerance analysis 利用纳米压印折射率的有效介质元表面:设计、性能和预测公差分析
IF 2.8 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-03-04 DOI: 10.1364/ome.515617
Matthew Panipinto and Judson D. Ryckman
Production of flat optics incorporating subwavelength features, particularly at visible frequencies, remains a significant challenge. Here, we establish a framework for the design of effective medium metasurfaces (EMM), relying on nanoimprinting of mesoporous silicon to realize a patterned refractive index n(x,y) corresponding to an arbitrary transmitted phase profile ϕ(x,y). The method is used to design the stamp profile required to produce a Fresnel lens and the theoretical performance of the metalens is examined using the finite-difference time-domain method. Additionally, we demonstrate neural network aided Monte Carlo analysis as a method to model the effects of metasurface fabrications errors on EMM performance and process yield.
生产具有亚波长特征的平面光学器件,尤其是在可见光频率下,仍然是一项重大挑战。在这里,我们建立了一个设计有效介质元表面(EMM)的框架,依靠介孔硅的纳米压印来实现与任意透射相位轮廓j(x,y)相对应的图案化折射率n(x,y)。该方法用于设计生产菲涅尔透镜所需的印章轮廓,并使用有限差分时域法检验了金属透镜的理论性能。此外,我们还演示了神经网络辅助蒙特卡洛分析法,该方法可用于模拟元表面制造误差对 EMM 性能和工艺产量的影响。
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引用次数: 0
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Optical Materials Express
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