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Engineering electrically tunable TiN/SiO2 epsilon-near-zero metamaterials 电子可调 TiN/SiO2 epsilon-near-zero 超材料工程学
IF 2.8 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-04-08 DOI: 10.1364/ome.519794
Joseph Garbarino, John G. Jones, Peter R. Stevenson, Cynthia T. Bowers, Krishnamurthy Mahalingam, and Lyuba Kuznetsova
Electrically tunable TiN/SiO2/TiN epsilon-near-zero photonic structures with various parameters were fabricated using the reactive DC magnetron sputtering approach. Effective medium approximation was used to predict the optical permittivity of a multilayered TiN/SiO2 metamaterial and guide the design/fabrication. Experimental reflectance measurements for tunable TiN/SiO2/TiN structures were obtained using the ellipsometer technique in the visible and near-infrared spectral ranges. Results show that reflectance for biased (12 V) and un-biased bulk TiN/SiO2/TiN structure changes up to ∼ 2% with the spectral shift at the ENZ spectral point ∼ 10 nm for samples with an optimal SiO2 dielectric layer (thickness d=10 nm). Reflectance measurements for multilayered tunable TiN/SiO2/TiN structures show strong variation in reflectance change for s- polarized light at epsilon-near-zero wavelengths due to applied voltage (12 V). We expect that the results of this research study of the tunable TiN/SiO2/TiN epsilon-near-zero photonic structures will potentially be useful for the photonic density of states engineering, surface sensing, and metamaterial-based super-resolution imaging.
利用反应式直流磁控溅射方法制造了具有各种参数的电可调 TiN/SiO2/TiN epsilon-near-zero 光子结构。利用有效介质近似法预测了多层 TiN/SiO2 超材料的光导率,并为设计/制造提供了指导。利用椭偏仪技术在可见光和近红外光谱范围内对可调 TiN/SiO2/TiN 结构进行了反射率实验测量。结果表明,对于具有最佳 SiO2 介电层(厚度 d=10 nm)的样品,偏压(12 V)和非偏压块状 TiN/SiO2/TiN 结构的反射率随 ENZ 光谱点 ∼ 10 nm 处的光谱偏移变化可达 ∼ 2%。多层可调谐 TiN/SiO2/TiN 结构的反射率测量结果表明,在ε-近零波长处,s 偏振光的反射率变化因施加电压(12 V)而变化很大。我们希望这项关于可调谐 TiN/SiO2/TiN ε-近零光子结构的研究成果能在光子态密度工程、表面传感和基于超材料的超分辨率成像方面发挥潜在作用。
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引用次数: 0
Seedless synthesis of Au nanoplates with tunable plasmonic peaks 无籽合成具有可调等离子峰的金纳米板
IF 2.8 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-04-08 DOI: 10.1364/ome.522159
Yuhao Zheng, Min Li, and Deyuan Shen
Au nanoplates with tunable in-plane dipolar localized surface plasmon resonance peaks in a broad range from the visible to near-infrared region were obtained in high yield using a seedless wet chemical growth method after purification. Cetyltrimethylammonium chloride was used as a surfactant, while hydrogen peroxide and sodium borohydride were used as the weak and strong reducing agents, respectively. The edge length and in-plane dipolar localized surface plasmon resonance peak of the Au nanoplates could be adjusted by varying the amounts of hydrogen peroxide and sodium borohydride. The Au nanoplates were further used as the saturable absorber to generate pulsed laser output in a passively Q-switched solid-state laser at approximately 2 µm. Our study offers a new method for obtaining Au nanoplates with tunable plasmonic peaks over a broad range.
采用无籽湿化学生长法,在纯化后获得了具有可调谐面内双极性局域表面等离子体共振峰的金纳米板,其峰值范围从可见光到近红外。十六烷基三甲基氯化铵用作表面活性剂,过氧化氢和硼氢化钠分别用作弱还原剂和强还原剂。通过改变过氧化氢和硼氢化钠的用量,可以调节金纳米板的边长和面内双极性局域表面等离子体共振峰。金纳米板被进一步用作可饱和吸收体,在约 2 µm 的被动 Q 开关固体激光器中产生脉冲激光输出。我们的研究为获得具有大范围可调等离子峰的金纳米板提供了一种新方法。
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引用次数: 0
Characterization of the optical gain at 1550 nm of erbium-oxalate single crystals 1550 纳米波长铒-草酸盐单晶体光学增益的表征
IF 2.8 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-04-05 DOI: 10.1364/ome.515335
R. E. López-Romero, G. G. Pérez-Sánchez, I. Aldaya, D. Y. Medina, E. L. Martínez-Piñeiro, I. A. Figueroa, and R. Escudero
Erbium is well-recognized as a key element for optical amplification at the 1550 nm operation band. However, the limited solubility of this material in vitreous matrices sets a critical constraint to the achievable optical gain, which limits its applicability in photonic integrated platforms. One of the solutions to increase the concentration of erbium is to employ a crystalline structure instead of a glass. In this paper, we characterize samples of erbium and erbium-ytterbium oxalate single crystals synthesized using the gel diffusion method. X-ray diffraction spectra and thermogravimetric analyses reveal that the synthesis method indeed generated the expected compound, and the pump-and-probe experiments demonstrate an on-off gain coefficient of ≈ 6.5 dB/mm, making this material a high-potential candidate for the implementation of integrated optical amplifiers.
铒是公认的 1550 nm 工作波段光放大的关键元素。然而,这种材料在玻璃基质中的溶解度有限,对可实现的光学增益造成了严重制约,从而限制了其在光子集成平台中的应用。提高铒浓度的解决方案之一是采用晶体结构代替玻璃。在本文中,我们对使用凝胶扩散法合成的铒和草酸铒镱单晶样品进行了表征。X 射线衍射光谱和热重分析表明,这种合成方法确实产生了预期的化合物,而且泵浦和探针实验表明,这种材料的通断增益系数≈ 6.5 dB/mm,使其成为实现集成光放大器的一种极具潜力的候选材料。
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引用次数: 0
Enhanced photoelectron emission in a large area aluminum nanohole array via a deep-UV surface plasmon 通过深紫外表面等离子体增强大面积铝纳米孔阵列的光电子发射
IF 2.8 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-04-04 DOI: 10.1364/ome.522182
Hirofumi Morisawa, Atsushi Ono, Koki Ikegami, Wataru Inami, and Yoshimasa Kawata
We measured the photoelectron emission efficiency of aluminum (Al) nanohole arrays fabricated by colloidal lithography and demonstrated the enhancement of photoelectron emission in the deep-UV region via surface plasmon resonances. The Al nanohole arrays for increasing absorption in the deep-UV region were designed using the finite-difference time-domain method and used as photocathodes to enhance the photoelectron emission efficiency. The enhancement factor improved by up to 3.5 times for the optimized nanohole array. Using a two-dimensional mapping system, we demonstrated that the photoelectron emission depended on the uniformity of the sample and diameter of the nanohole arrays. Al nanohole arrays fabricated by colloidal lithography can be used to develop highly sensitive surface-detecting optical sensors and highly efficient surface-emitting electron sources. The two-dimensional mapping system can facilitate the development of highly efficient photocathodes.
我们测量了通过胶体光刻法制造的铝(Al)纳米孔阵列的光电子发射效率,并证明了通过表面等离子体共振增强了深紫外区的光电子发射。利用有限差分时域法设计了可增加深紫外区吸收的铝(Al)纳米孔阵列,并将其用作光电阴极以提高光电子发射效率。优化后的纳米孔阵列的增强系数提高了 3.5 倍。利用二维绘图系统,我们证明了光电子发射取决于样品的均匀性和纳米孔阵列的直径。利用胶体光刻技术制作的铝纳米孔阵列可用于开发高灵敏度表面检测光学传感器和高效表面发射电子源。二维绘图系统可促进高效光电阴极的开发。
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引用次数: 0
Fast-switching reconfigurable metadevice with metasurface-induced liquid crystal alignment for light modulator applications 用于光调制器应用的具有元表面诱导液晶对准功能的快速开关可重构元器件
IF 2.8 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-03-29 DOI: 10.1364/ome.520326
Xin Chang, Mike Pivnenko, Angadjit Singh, Weijie Wu, Pawan Shrestha, and Daping Chu
Metasurface technology is progressing rapidly towards commercialization and productization, due to its unparallelled advantages over conventional optical solutions. The reconfigurable metasurface, exhibiting more flexibility and capacity than its static counterpart, has been one of the most pursued features of metasurface. In this work, we present liquid crystal-based dynamic metasurface by immersing metasurface in nematic liquid crystal environment. No alignment material was used, and liquid crystal was aligned directly by metasurface. The alignment quality was characterized and the intensity contrast of 33 was obtained. Optical amplitude modulation was achieved with the modulation depth of 91% at the wavelength of 1375 nm. Moreover, sub-micrometre cell gap of 875 nm was realized, and the response time was measured to be sub-millisecond at room temperature, translating to > 1KHz operation frequency. The higher operation frequency of > 3.4 KHz was recorded at elevated temperature. The key performance indicators demonstrated in this work showcase the promising future of liquid crystal – based reconfigurable metasurface, especially for fast light modulator applications.//Metasurface technology is progressing rapidly toward commercialization and productization due to its unparalleled advantages over conventional optical solutions. The reconfigurable metasurface, exhibiting more flexibility and capacity than its static counterpart, has been one of the most pursued features of the metasurface. In this work, we present a liquid crystal-based dynamic metasurface by immersing the metasurface in a nematic liquid crystal environment. No alignment material was used, and liquid crystal was aligned directly by metasurface. The alignment quality was characterized, and the intensity contrast of 33 was obtained. Optical amplitude modulation was achieved with a modulation depth of 91% at the wavelength of 1375 nm. Moreover, a sub-micrometer cell gap of 875 nm was realized, and the response time was measured to be sub-millisecond at room temperature, translating to > 1KHz operation frequency. The higher operation frequency of > 3.4 KHz was recorded at elevated temperatures. The key performance indicators demonstrated in this work showcase the promising future of liquid crystal-based reconfigurable metasurface, especially for fast light modulator applications.
与传统光学解决方案相比,元表面技术具有无可比拟的优势,因此正朝着商业化和产品化的方向快速发展。与静态元表面相比,可重新配置的元表面具有更大的灵活性和容量,这一直是元表面最受追捧的特性之一。在这项工作中,我们通过将元表面浸入向列液晶环境,提出了基于液晶的动态元表面。没有使用对准材料,液晶直接由元表面对准。对准质量进行了表征,并获得了 33 的强度对比度。在波长为 1375 nm 时,实现了光学振幅调制,调制深度达到 91%。此外,还实现了 875 纳米的亚微米单元间隙,室温下的响应时间为亚毫秒级,工作频率为 1KHz。在高温条件下,工作频率更高,达到 3.4 千赫兹。这项工作中展示的关键性能指标表明,基于液晶的可重构元表面技术前景广阔,特别是在快速光调制器应用方面。与静态元表面相比,可重新配置的元表面具有更高的灵活性和容量,这一直是元表面最受追捧的特性之一。在这项工作中,我们通过将元表面浸入向列液晶环境,展示了一种基于液晶的动态元表面。没有使用对准材料,液晶直接由元表面对准。对准质量进行了表征,并获得了 33 的强度对比度。在波长为 1375 nm 时,实现了光学振幅调制,调制深度达到 91%。此外,还实现了 875 nm 的亚微米单元间隙,室温下的响应时间为亚毫秒级,工作频率为 1KHz。在高温条件下,工作频率更高,达到 3.4 千赫兹。这项工作中展示的关键性能指标展示了基于液晶的可重构元表面的美好前景,尤其是在快速光调制器应用方面。
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引用次数: 0
Spatiotemporal cascading of dielectric waveguides [Invited] 介质波导的时空级联 [特邀]
IF 2.8 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-03-28 DOI: 10.1364/ome.516262
Victor Pacheco-Peña and Nader Engheta
Photonic time interfaces, as the temporal analogue of spatial interfaces between two media, consist of a rapid change of the electromagnetic properties of a material (such as permittivity, ε, and permeability, μ) while the wave is present in the material. Here we exploit cascading of such time interfaces in spatially cascaded guided-wave structures such as slab waveguides and ring resonators by considering that the relative permittivity of the cladding of dielectric waveguides is rapidly changed at different moments of time from εclad_1 to εclad_2, while the material of the core remains unchanged in time. It is shown how such time-dependent cladding can enable frequency conversion within the space-time dielectric ring resonator and slab waveguides due to an induced modification of the effective refractive index of the mode propagating within such photonic device. Cascaded frequency conversion is achieved in such cascaded space-time dielectric waveguides and ring resonators, showing how the combination of space and time interfaces can offer further opportunities for manipulation of light-matter interaction using four-dimensional (4D) photonic structures.
光子时间界面是两种介质之间空间界面的时间类似物,由材料的电磁特性(如介电常数ε和磁导率μ)的快速变化组成,同时波存在于材料中。在这里,我们利用空间级联导波结构(如板坯波导和环形谐振器)中的这种时间界面级联,考虑到介质波导包层的相对介电常数在不同时刻从εclad_1 快速变化到εclad_2,而核心材料在时间上保持不变。图中展示了这种随时间变化的包层如何在时空介质环谐振器和板坯波导中实现频率转换,这是因为在这种光子器件中传播的模式的有效折射率发生了诱导性改变。在这种级联时空介质波导和环形谐振器中实现了级联频率转换,展示了空间和时间界面的结合如何为利用四维(4D)光子结构操纵光物质相互作用提供更多机会。
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引用次数: 0
Localization landscape of optical waves in multifractal photonic membranes 多分形光子膜中光波的定位景观
IF 2.8 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-03-21 DOI: 10.1364/ome.520201
Tornike Shubitidze, Yilin Zhu, Hari Sundar, and Luca Dal Negro
In this paper, we investigate the localization properties of optical waves in disordered systems with multifractal scattering potentials. In particular, we apply the localization landscape theory to the classical Helmholtz operator and, without solving the associated eigenproblem, show accurate predictions of localized eigenmodes for one- and two-dimensional multifractal structures. Finally, we design and fabricate nanoperforated photonic membranes in silicon nitride (SiN) and image directly their multifractal modes using leaky-mode spectroscopy in the visible spectral range. The measured data demonstrate optical resonances with multiscale intensity fluctuations in good qualitative agreement with numerical simulations. The proposed approach provides a convenient strategy to design multifractal photonic membranes, enabling rapid exploration of extended scattering structures with tailored disorder for enhanced light-matter interactions.
本文研究了具有多分形散射势的无序系统中光波的局域化特性。特别是,我们将局域景观理论应用于经典亥姆霍兹算子,并在不解决相关特征问题的情况下,准确预测了一维和二维多分形结构的局域特征模式。最后,我们在氮化硅(SiN)中设计并制造了纳米穿孔光子膜,并在可见光谱范围内使用漏模光谱法直接对其多分形模式进行成像。测量数据显示了具有多尺度强度波动的光学共振,与数值模拟具有良好的定性一致性。所提出的方法为设计多分形光子膜提供了一种便捷的策略,能够快速探索具有定制无序性的扩展散射结构,从而增强光物质之间的相互作用。
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引用次数: 0
Passively harmonic mode-locked erbium-doped fiber laser with a gold nanofilm saturable absorber 带有金纳米薄膜可饱和吸收器的被动谐波模式锁定掺铒光纤激光器
IF 2.8 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-03-20 DOI: 10.1364/ome.521096
Changjian Lv, Fanchao Meng, Tianqi Zhang, Junjie Wang, Qi Yan, Zhixu Jia, Weiping Qin, and Guanshi Qin
We demonstrate a 1.5 GHz harmonic mode-locked erbium-doped fiber laser by incorporating gold nanofilm as a saturable absorber (SA). The high-quality gold nanofilm SA fabricated by the physical vapor deposition method possesses a high modulation depth of 12.9% and a low saturation intensity of 1.69 MW/cm2 at 1.56 µm, facilitating the generation of harmonic mode-locking. The fundamental mode-locked operation was obtained at 1564.7 nm, with a pulse duration of 586 fs and a repetition rate of 34.235 MHz. At the pump power of 610 mW, 44th-order harmonic mode-locking with a repetition rate of 1.506 GHz was achieved, which is the highest yet reported in mode-locked fiber lasers using gold nanomaterials as SAs. Moreover, the gold nanofilm-based harmonic mode-locked fiber laser shows relatively high signal-to-noise ratios, high output power, and good stability. These results highlight the advantage of the gold nanofilm-based SA in realizing high repetition rate laser sources.
我们展示了一种将纳米金薄膜作为可饱和吸收体(SA)的 1.5 GHz 谐波锁模掺铒光纤激光器。采用物理气相沉积法制造的高质量纳米金膜 SA 具有 12.9% 的高调制深度和 1.56 µm 处 1.69 MW/cm2 的低饱和强度,有利于产生谐波锁模。在 1564.7 nm 波长处实现了基本锁模操作,脉冲持续时间为 586 fs,重复频率为 34.235 MHz。在 610 mW 的泵浦功率下,实现了重复率为 1.506 GHz 的 44 阶谐波锁模,这是迄今为止使用金纳米材料作为 SA 的锁模光纤激光器中的最高值。此外,基于金纳米薄膜的谐波锁模光纤激光器显示出相对较高的信噪比、较高的输出功率和良好的稳定性。这些结果凸显了基于金纳米薄膜的 SA 在实现高重复率激光源方面的优势。
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引用次数: 0
Surface wave control via unidirectional surface magnetoplasmon waveguide arrays 通过单向表面磁谱仪波导阵列控制表面波
IF 2.8 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-03-20 DOI: 10.1364/ome.518730
Shiqing Li, Weipu Tu, Hang Zhang, Jinhua Yan, and Linfang Shen
Freely tailoring the wavefronts of surface waves (SWs), including surface plasmon polaritons (SPPs) and their equivalent counterparts, holds significant importance in the field of on-chip photonics. However, conventional diffraction-optics based devices often suffer from limited functionalities and low working efficiencies. Here, we present a novel concept of a unidirectional surface magnetoplasmon (USMP) waveguide array composed of carefully engineered subwavelength-spaced unidirectional waveguide slits. By utilizing the unique propagation properties of USMPs within these waveguides, the USMP waveguide array efficiently converts USMPs into SWs with predetermined wavefronts. As proof of the concept, we numerically demonstrate this new principle through the design of two microwave USMP waveguide arrays using a metal-air-YIG structure, which directly converts USMPs into SWs with the wavefronts of Bessel beam and focusing. Additionally, we extend this concept to the terahertz regime and achieve beam deflection of SWs using a metal-air-semiconductor waveguide array. These findings may inspire the development of highly miniaturized on-chip devices for integrated photonics applications.
自由定制表面波(SW)的波面,包括表面等离子体极化子(SPP)及其等效对应物,在片上光子学领域具有重要意义。然而,传统的衍射光学器件往往功能有限,工作效率低。在这里,我们提出了一个新颖的概念,即由精心设计的亚波长间距单向波导狭缝组成的单向表面磁共振(USMP)波导阵列。通过利用 USMP 在这些波导中的独特传播特性,USMP 波导阵列可有效地将 USMP 转换为具有预定波面的 SW。作为对这一概念的证明,我们使用金属-空气-YIG 结构设计了两个微波 USMP 波导阵列,直接将 USMP 转换为具有贝塞尔波束和聚焦波面的 SW。此外,我们还将这一概念扩展到太赫兹领域,利用金属-空气-半导体波导阵列实现了 SW 的波束偏转。这些发现可能有助于开发用于集成光子学应用的高度微型化片上器件。
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引用次数: 0
Core-shell diamond-graphene needles with silicon-vacancy color centers 具有硅空位色彩中心的核壳金刚石-石墨烯针
IF 2.8 3区 材料科学 Q3 MATERIALS SCIENCE, MULTIDISCIPLINARY Pub Date : 2024-03-18 DOI: 10.1364/ome.518724
Mariam Maku Quarshie, Sergei Malykhin, and Polina Kuzhir
Color centers in diamond nanostructures open new horizons in biomedicine, offering a biocompatible material platform for sensing temperature, pH, and magnetic field. Covering of the color centers enriched diamonds with graphene shell can essentially extend their application potential. Specifically, under irradiation with ultrashort laser pulses, the highly absorptive graphene shell can be used for excitation of a shock acoustic wave which can be used for cancer cell destruction or drug photoactivation through the Joule heating. In this study, we present a novel method for creating diamond-graphite core-shell structures. Through precise control of the growth of the graphitic layer on Single Crystal Diamond Needles (SCDNs) via vacuum annealing at 900°C for 30 minutes, we preserved 57% of the light emission from silicon-vacancy (SiV-) centers while maintaining their spectral peaks. Contrary to our expectations of reduced SiV- luminescence due to the presence of the graphitic shell, we observed that the initial high brightness of SiV- in the diamond needles persisted. This enabled us to detect SiV- luminescence spectrally, even within the core-shell structures. Our results underscore the tunability of these structures’ properties through temperature and duration control, suggesting promising prospects for their application in advanced biomedical tools with sensing capabilities.
金刚石纳米结构中的色彩中心为生物医学开辟了新天地,为感知温度、pH 值和磁场提供了一个生物相容性材料平台。在富含颜色中心的金刚石上覆盖石墨烯外壳,可以从根本上扩展其应用潜力。具体来说,在超短激光脉冲的照射下,高吸收性石墨烯外壳可用于激发冲击声波,通过焦耳加热破坏癌细胞或药物光活化。在这项研究中,我们提出了一种制造金刚石-石墨核壳结构的新方法。通过在 900°C 下真空退火 30 分钟,精确控制单晶金刚石针(SCDN)上石墨层的生长,我们保留了硅空穴(SiV-)中心 57% 的光发射,同时保持了它们的光谱峰。由于石墨外壳的存在,SiV- 发光减少,与我们的预期相反,我们观察到金刚石针中 SiV- 最初的高亮度持续存在。这使我们能够从光谱上检测到 SiV- 发光,即使在核壳结构中也是如此。我们的研究结果表明,这些结构的特性可通过温度和持续时间控制进行调整,这为其在具有传感功能的先进生物医学工具中的应用提供了广阔的前景。
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引用次数: 0
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Optical Materials Express
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