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3D imaging lipidometry in single cell by in-flow holographic tomography 流式全息体层析单细胞三维成像血脂测定
IF 14.1 1区 物理与天体物理 Q1 OPTICS Pub Date : 2022-01-01 DOI: 10.29026/oea.2023.220048
D. Pirone, Daniele G Sirico, L. Miccio, V. Bianco, M. Mugnano, D. D. Giudice, G. Pasquinelli, S. Valente, Silvia Lemma, L. Iommarini, I. Kurelac, P. Memmolo, P. Ferraro
The most recent discoveries in the biochemical field are highlighting the increasingly important role of lipid droplets (LDs) in several regulatory mechanisms in living cells. LDs are dynamic organelles and therefore their complete characterization in terms of number, size, spatial positioning and relative distribution in the cell volume can shed light on the roles played by LDs. Until now, fluorescence microscopy and transmission electron microscopy are assessed as the gold standard methods for identifying LDs due to their high sensitivity and specificity. However, such methods generally only provide 2D assays and partial measurements. Furthermore, both can be destructive and with low productivity, thus limiting analysis of large cell numbers in a sample. Here we demonstrate for the first time the capability of 3D visualization and the full LD characterization in high-throughput with a tomographic phase-contrast flow-cytometer, by using ovarian cancer cells and monocyte cell lines as models. A strategy for retrieving significant parameters on spatial correlations and LD 3D positioning inside each cell volume is reported. The information gathered by this new method could allow more in depth understanding and lead to new discoveries on how LDs are correlated to cellular functions. 3D D. Pirone, P. Memmolo, V. Bianco, L. Iom- marini and P. Ferraro analyzed and discussed the tomographic reconstruc-tions and data. I. Kurelac, S. Lemma and L. Iommarini performed FM ex- periments and data analysis; G. Pasquinelli and S. Valente performed the TEM; all the authors contributed to critical discussion of the results and contributed to write the manuscript. P. Ferraro supervised the research.
生物化学领域的最新发现强调了脂滴(ld)在活细胞的几种调节机制中的重要作用。ld是动态细胞器,因此它们在细胞体积中的数量、大小、空间定位和相对分布方面的完整表征可以揭示ld所起的作用。到目前为止,荧光显微镜和透射电子显微镜因其高灵敏度和特异性被评价为鉴定ld的金标准方法。然而,这种方法通常只提供二维分析和部分测量。此外,两者都具有破坏性且生产率低,因此限制了样品中大量细胞的分析。本文首次以卵巢癌细胞和单核细胞系为模型,利用层析相衬流式细胞仪展示了高通量的3D可视化和全LD表征能力。一种策略,检索显著参数的空间相关性和LD三维定位在每个细胞体积。通过这种新方法收集的信息可以让我们更深入地了解ld如何与细胞功能相关,并导致新的发现。3D D. Pirone, P. Memmolo, V. Bianco, L. Iom- marini和P. Ferraro对层析重建和数据进行了分析和讨论。I. Kurelac、S. Lemma和L. Iommarini进行调频实验和数据分析;G. Pasquinelli和S. Valente进行透射电镜观察;所有作者都参与了对结果的批判性讨论,并参与了论文的撰写。P. Ferraro监督了这项研究。
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引用次数: 14
Confocal laser speckle autocorrelation imaging of dynamic flow in microvasculature 微血管动态血流的激光共聚焦散斑自相关成像
IF 14.1 1区 物理与天体物理 Q1 OPTICS Pub Date : 2022-01-01 DOI: 10.29026/oea.2022.210045
E. Du, Shuhao Shen, Anqi Qiu, Nanguang Chen
Laser speckle imaging has been widely used for in-vivo visualization of blood perfusion in biological tissues. However, existing laser speckle imaging techniques suffer from limited quantification accuracy and spatial resolution. Here we report a novel design and implementation of a powerful laser speckle imaging platform to solve the two critical limitations. The core technique of our platform is a combination of line scan confocal microscopy with laser speckle autocorrelation imaging, which is termed Line Scan Laser Speckle Autocorrelation Imaging (LS-LSAI). The technical advantages of LS-LSAI include high spatial resolution (~4.4 μm) for visualizing and quantifying blood flow in microvessels, as well as video-rate imaging speed for tracing dynamic flow
激光散斑成像已广泛应用于生物组织血液灌注的体内可视化。然而,现有的激光散斑成像技术存在定量精度和空间分辨率有限的问题。在这里,我们报告了一个新颖的设计和实现一个强大的激光散斑成像平台,以解决这两个关键的限制。我们平台的核心技术是线扫描共聚焦显微镜与激光散斑自相关成像的结合,称为线扫描激光散斑自相关成像(LS-LSAI)。LS-LSAI的技术优势包括高空间分辨率(~4.4 μm),用于微血管血流的可视化和量化,以及视频速率成像速度,用于跟踪动态血流
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引用次数: 9
Carnivorous plants inspired shape-morphing slippery surfaces 食肉植物激发了变形光滑表面的灵感
IF 14.1 1区 物理与天体物理 Q1 OPTICS Pub Date : 2022-01-01 DOI: 10.29026/oea.2023.210163
Dongdong Han, Yong‐Lai Zhang, Zhao-Di Chen, Ji-chao Li, Jia‐Nan Ma, J. Mao, Hao Zhou, Hongjiang Sun
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引用次数: 11
Dynamic phase assembled terahertz metalens for reversible conversion between linear polarization and arbitrary circular polarization 动态相位组合太赫兹超构透镜在线偏振和任意圆偏振之间可逆转换
IF 14.1 1区 物理与天体物理 Q1 OPTICS Pub Date : 2022-01-01 DOI: 10.29026/oea.2022.210062
Jitao Li, Guo-cui Wang, Zhen Yue, Jingyu Liu, Jie Li, Chenglong Zheng, Yating Zhang, Yan Zhang, Jianquan Yao
If a metalens integrates the circular polarization (CP) conversion function, the focusing lens together with circular-polariz-ing lens (CPL) in traditional cameras may be replaced by a metalens. However, in terahertz (THz) band, the reported metalenses still do not obtain the perfect and strict single-handed CP, because they were constructed via Pancharatnam-Berry phase so that CP conversion contained both left-handed CP (LCP) and right-handed CP (RCP) components. In this paper, a silicon based THz metalens is constructed using dynamic phase to obtain single-handed CP conversion. Also, we can rotate the whole metalens at a certain angle to control the conversion of multi-polarization states, which can simply manipulate the focusing for incident linear polarization (LP) THz wave in three polarization conversion states, including LP without conversion, LCP and RCP. Moreover, the polarization conversion behavior is reversible, that is, the THz metalens can convert not only the LP into arbitrary single-handed CP, but also the LCP and RCP into two perpendicular LP, respectively. The metalens is expected to be used in advanced THz camera, as a great candidate for traditional CPL and focusing lens group, and also shows potential application in polarization imaging with discriminating LCP and RCP.
如果一个超透镜集成了圆偏振光转换函数,那么传统相机中的聚焦透镜和圆偏振光透镜就可以被一个超透镜所取代。然而,在太赫兹(THz)波段,所报道的超构透镜仍然没有获得完美和严格的单手CP,因为它们是通过Pancharatnam-Berry相构建的,使得CP转换同时包含左手CP (LCP)和右手CP (RCP)成分。本文利用动态相位构造了硅基太赫兹超构透镜,实现了单手CP转换。此外,我们还可以将整个超透镜以一定角度旋转来控制多极化状态的转换,从而可以简单地控制入射线性偏振(LP)太赫兹波在不转换的LP、LCP和RCP三种偏振转换状态下的聚焦。此外,太赫兹超透镜的极化转换行为是可逆的,即既可以将LP转化为任意单手CP,也可以将LCP和RCP分别转化为两个垂直的LP。超透镜作为传统CPL和聚焦透镜组的重要候选,有望应用于先进的太赫兹相机,并在分辨LCP和RCP的偏振成像中显示出潜在的应用前景。
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引用次数: 53
Beyond Lambertian light trapping for large-area silicon solar cells: fabrication methods 超越大面积硅太阳能电池的朗伯氏光捕获:制造方法
IF 14.1 1区 物理与天体物理 Q1 OPTICS Pub Date : 2021-12-31 DOI: 10.29026/oea.2022.210086
J. Maksimovic, Jingwen Hu, S. Ng, T. Katkus, G. Seniutinas, T. P. Rivera, M. Stuiber, Y. Nishijima, S. John, S. Juodkazis
Light trapping photonic crystal (PhC) patterns on the surface of Si solar cells provides a novel opportunity to approach the theoretical efficiency limit of 32.3%, for light-to-electrical power conversion with a single junction cell. This is beyond the efficiency limit implied by the Lambertian limit of ray trapping 29%. The interference and slow light effects are harnessed for collecting light even at the long wavelengths near the Si band-gap. We compare two different methods for surface patterning, that can be extended to large area surface patterning: 1) laser direct write and 2) step-&-repeat 5-times reduction projection lithography. Large area throughput limitations of these methods are compared with the established electron beam lithography (EBL) route, which is conventionally utilised but much slower than the presented methods. Spectral characterisation of the PhC light trapping is compared for samples fabricated by different methods. Reflectance of Si etched via laser patterned mask was 7% at visible wavelengths and was comparable with Si patterned via EBL made mask. The later pattern showed a stronger absorbance than the Lambertian limit (M.-L. Hsieh et al., Sci. Rep. 10, 11857 (2020)).
硅太阳能电池表面的光捕获光子晶体(PhC)图案为单结电池的光-电功率转换提供了一个接近32.3%理论效率极限的新机会。这超出了光线捕获29%的朗伯极限所暗示的效率极限。干涉和慢光效应被用来收集光,即使在Si带隙附近的长波长下也是如此。我们比较了两种不同的表面图案化方法,这两种方法可以扩展到大面积表面图案:1)激光直接写入和2)分步重复5次缩小投影光刻。将这些方法的大面积吞吐量限制与已建立的电子束光刻(EBL)路线进行比较,后者是传统使用的,但比所提出的方法慢得多。比较了不同方法制备的样品的PhC光捕获的光谱特征。通过激光图案化掩模蚀刻的Si在可见波长下的反射率为7%,并且与通过EBL制造的掩模图案化的Si相当。后一种模式显示出比朗伯极限更强的吸光度(M.-L.Hieh等人,Sci.Rep.1011857(2020))。
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引用次数: 6
Laser-induced periodic surface structured electrodes with 45% energy saving in electrochemical fuel generation through field localization 激光诱导周期性表面结构电极,通过场定位实现电化学燃料发电节能45%
IF 14.1 1区 物理与天体物理 Q1 OPTICS Pub Date : 2021-12-13 DOI: 10.29026/oea.2022.210105
C. S. Saraj, S. Singh, Gopal Verma, R. Rajan, Wei Li, Chunlei Guo
Electrochemical oxidation/reduction of radicals is a green and environmentally friendly approach to generate fuels. These reactions, however, suffer from sluggish kinetics due to a low local concentration of radicals around the electrocatalyst. A large electrode potential can enhance the fuel generation efficiency via enhancing the radical concentration around the electrocatalyst sites, but this comes at the cost of electricity. Here, we report about 45 % saving in energy to achieve an electrochemical hydrogen generation rate of 3×1016 molecules cm-2s-1 (current density: 10 mA/cm2) through localized electric field-induced enhancement in the reagent concentration (LEFIRC) at laser-induced periodic surface structured (LIPSS) electrodes. The finite element model is used to simulate the spatial distribution of the electric field to understand the effects of LIPSS geometric parameters in field localization. When the LIPSS patterned electrodes are used as substrates to support Pt/C and RuO2 electrocatalysts, the 10 overpotentials for HER and OER are decreased by 40 and 25 %, respectively. Moreover, the capability of the LIPSS-patterned electrodes to operate at significantly reduced energy is also demonstrated in a range of electrolytes including alkaline, acidic, neutral, and seawater. Importantly, when two LIPSS patterned electrodes were assembled as the anode and cathode into a cell, it requires 330 mVs of lower electric potential with enhanced stability over a similar cell made of pristine electrodes to drive a current density of 10 mA/cm2. This work demonstrates a physical and versatile approach of electrode surface patterning to boost electrocatalytic fuel generation performance and can be applied to any metal and semiconductor catalysts for a range of electrochemical reactions.
自由基的电化学氧化/还原是一种绿色环保的燃料生产方法。然而,由于电催化剂周围自由基的低局部浓度,这些反应的动力学缓慢。大的电极电势可以通过提高电催化剂位点周围的自由基浓度来提高燃料产生效率,但这是以电为代价的。在这里,我们报道了通过在激光诱导的周期性表面结构(LIPSS)电极处的局部电场诱导的试剂浓度(LEFIRC)的增强,实现3×1016分子cm-2s-1(电流密度:10mA/cm2)的电化学氢生成率,从而节省了约45%的能量。有限元模型用于模拟电场的空间分布,以了解LIPSS几何参数在场定位中的影响。当LIPSS图案化电极用作支撑Pt/C和RuO2电催化剂的衬底时HER和OER的10个过电位分别降低了40%和25%。此外,在包括碱性、酸性、中性和海水在内的一系列电解质中,也证明了LIPSS图案化电极在显著降低的能量下工作的能力。重要的是,当将两个LIPSS图案化电极作为阳极和阴极组装到电池中时,与由原始电极制成的类似电池相比,需要330mV的较低电势和增强的稳定性来驱动10mA/cm2的电流密度。这项工作展示了一种物理和通用的电极表面图案化方法,以提高电催化燃料生成性能,并可应用于任何金属和半导体催化剂,用于一系列电化学反应。
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引用次数: 4
Intelligent metaphotonics empowered by machine learning 机器学习赋予的智能变形学
IF 14.1 1区 物理与天体物理 Q1 OPTICS Pub Date : 2021-10-22 DOI: 10.29026/oea.2022.210147
S. Krasikov, Aaron D Tranter, A. Bogdanov, Y. Kivshar
In the recent years, we observe a dramatic boost of research in photonics empowered by the concepts of machine learning and artificial intelligence. The corresponding photonic systems, to which this new methodology is applied, can range from traditional optical waveguides to nanoantennas and metasurfaces, and these novel approaches underpin the fundamental principles of light-matter interaction developed for a smart design of intelligent photonic devices. Concepts and approaches of artificial intelligence and machine learning penetrate rapidly into the fundamental physics of light, and they provide effective tools for the study of the field of metaphotonics driven by optically-induced electric and magnetic resonances. Here, we introduce this new field with its application to metaphotonics and also present a summary of the basic concepts of machine learning with some specific examples developed and demonstrated for metasystems and metasurfaces.
近年来,我们观察到在机器学习和人工智能概念的推动下,光子学的研究取得了巨大的进步。这种新方法所应用的相应光子系统可以从传统的光波导到纳米天线和超表面,这些新方法巩固了为智能光子器件的智能设计而开发的光-物质相互作用的基本原理。人工智能和机器学习的概念和方法迅速渗透到光的基础物理学中,它们为光感应电和磁共振驱动的变光子学领域的研究提供了有效的工具。在这里,我们介绍了这一新的领域及其在元光子学中的应用,并对机器学习的基本概念进行了总结,并给出了一些针对元系统和元表面开发和演示的具体示例。
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引用次数: 54
Ultrashort pulsed laser induced complex surface structures generated by tailoring the melt hydrodynamics 通过调整熔体流体力学产生超短脉冲激光诱导的复杂表面结构
IF 14.1 1区 物理与天体物理 Q1 OPTICS Pub Date : 2021-04-27 DOI: 10.29026/oea.2022.210052
F. Fraggelakis, G. Tsibidis, E. Stratakis
We present a novel approach for tailoring the laser induced surface topography upon femtosecond (fs) pulsed laser irradiation. The method employs spatially controlled double fs laser pulses to actively regulate the hydrodynamic microfluidic motion of the melted layer that gives rise to the structures formation. The pulse train used, in particular, consists of a previously unexplored spatiotemporal intensity combination including one pulse with Gaussian and another with periodically modulated intensity distribution created by Direct Laser Interference Patterning (DLIP). The interpulse delay is appropriately chosen to reveal the contribution of the microfluidic melt flow, while it is found that the sequence of the Gaussian and DLIP pulses remarkably influences the surface profile attained. Results also demonstrate that both the spatial intensity of the double pulse and the effective number of pulses per irradiation spot can further be modulated to control the formation of complex surface morphologies. The underlying physical processes behind the complex patterns’ generation were interpreted in terms of a multiscale model combining electrodynamic excitation with melt hydrodynamics. We believe that this work can constitute a significant step forward towards producing laser induced surface structures on demand by tailoring the melt microfluidic phenomena.
我们提出了一种在飞秒(fs)脉冲激光照射下调整激光诱导表面形貌的新方法。该方法采用空间控制的双fs激光脉冲来主动调节熔化层的流体动力学微流体运动,从而形成结构。特别地,所使用的脉冲串由先前未探索的时空强度组合组成,包括一个具有高斯的脉冲和另一个具有由直接激光干涉图案化(DLIP)创建的周期性调制强度分布的脉冲。适当选择脉冲间延迟来揭示微流体熔体流动的贡献,同时发现高斯脉冲和DLIP脉冲的顺序显著影响所获得的表面轮廓。结果还表明,可以进一步调节双脉冲的空间强度和每个照射点的有效脉冲数,以控制复杂表面形貌的形成。根据将电动激励与熔体流体力学相结合的多尺度模型,解释了复杂图案生成背后的潜在物理过程。我们相信,这项工作可以通过定制熔体微流体现象,朝着按需生产激光诱导的表面结构迈出重要一步。
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引用次数: 24
Cylindrical vector beams reveal radiationless anapole condition in a resonant state 圆柱矢量光束在谐振状态下显示无辐射拟极点状态
IF 14.1 1区 物理与天体物理 Q1 OPTICS Pub Date : 2021-04-22 DOI: 10.29026/oea.2022.210014
Yudong Lu, Yi Xu, Ouyang Xu, Mingcong Xian, Yaoyu Cao, Kai Chen, Xiangping Li
Nonscattering optical anapole condition is corresponding to the excitation of radiationless field distributions in open resonators, which offers new degrees of freedom for tailoring light-matter interaction. Conventional mechanisms for achieving such a condition relies on sophisticated manipulation of electromagnetic multipolar moments of all orders to guarantee superpositions of vanished moment strengths at the same wavelength. In contrast, here we report on the excitation of optical radiationless anapole hidden in a resonant state of a Si nanoparticle utilizing tightly focused radially polarized (RP) beam. The coexistence of magnetic resonant state and anapole condition at the same wavelength further enables the triggering of resonant state by tightly focused azimuthally polarized (AP) beam whose corresponding electric multipole coefficient could be zero. As a result, high contrast inter-transition between radiationless anapole condition and ideal magnetic resonant scattering can be achieved experimentally in visible spectrum. The proposed mechanism is general which can be realized in different types of nanostructures. Our results showcase that the unique combination of structured light and structured Mie resonances could provide new degrees of freedom for tailoring light-matter interaction, which might shed new light on functional meta-optics.
非散射光学拟极点条件对应于开放谐振腔中无辐射场分布的激发,为调整光-物质相互作用提供了新的自由度。实现这种条件的传统机制依赖于对所有阶的电磁多极矩的复杂操纵,以保证在同一波长上消失的矩强度的叠加。与此相反,本文报道了利用紧聚焦径向极化(RP)光束激发隐藏在硅纳米粒子共振状态下的无辐射光学拟极点。磁谐振态和拟极点条件在同一波长的共存,进一步使得紧密聚焦的方位角极化光束触发谐振态,其对应的电多极系数可以为零。实验结果表明,在可见光谱中可以实现无辐射拟极点条件与理想磁谐振散射之间的高对比度间跃迁。所提出的机制是通用的,可以在不同类型的纳米结构中实现。我们的研究结果表明,结构光和结构Mie共振的独特组合可以为定制光-物质相互作用提供新的自由度,这可能为功能元光学提供新的思路。
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引用次数: 15
Near-perfect fidelity polarization-encoded multilayer optical data storage based on aligned gold nanorods 基于对齐金纳米棒的近乎完美保真偏振编码多层光学数据存储
IF 14.1 1区 物理与天体物理 Q1 OPTICS Pub Date : 2021-04-13 DOI: 10.29026/oea.2021.210002
Linwei Zhu, Yaoyu Cao, Qiuqun Chen, Xueying Ouyang, Yi Xu, Zhongliang Hu, J. Qiu, Xiangping Li
Encoding information in light polarization is of great importance in facilitating optical data storage (ODS) for information security and data storage capacity escalation. However, despite recent advances in nanophotonic techniques vastly enhancing the feasibility of applying polarization channels, the data fidelity in reconstructed bits has been constrained by severe crosstalks occurring between varied polarization angles during data recording and reading process, which gravely hindered the utilization of this technique in practice. In this paper, we demonstrate an ultra-low crosstalk polarization-encoding multilayer optical data storage technique for high-fidelity data recording and retrieving by utilizing a nanofibre-based nanocomposite film involving highly aligned gold nanorods (GNRs). With parallelizing the gold nanorods in the recording medium, the information carrier configuration minimizes miswriting and misreading possibilities for information input and output, respectively, compared with its randomly self-assembled counterparts. The enhanced data accuracy has significantly improved the bit recall fidelity that is quantified by a correlation coefficient higher than 0.99. It is anticipated that the demonstrated technique can facilitate the development of multiplexing ODS for a greener future.
对光偏振信息进行编码对于促进光学数据存储(ODS)的信息安全和数据存储容量升级具有重要意义。然而,尽管纳米光子技术的最新进展大大提高了应用偏振通道的可行性,但在数据记录和读取过程中,不同偏振角之间发生的严重串扰限制了重建比特的数据保真度,这严重阻碍了该技术在实践中的应用。在本文中,我们展示了一种超低串扰偏振编码多层光学数据存储技术,通过利用包含高度排列的金纳米棒(GNRs)的基于纳米纤维的纳米复合薄膜,用于高保真数据记录和检索。通过在记录介质中并行化金纳米棒,与随机自组装的对应物相比,信息载体配置分别最大限度地减少了信息输入和输出的错误写入和误读可能性。增强的数据准确性显著提高了比特召回保真度,该保真度通过高于0.99的相关系数来量化。预计所展示的技术可以促进多路复用ODS的发展,以实现更绿色的未来。
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引用次数: 21
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Opto-Electronic Advances
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