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Health risk assessment of municipal solid waste incineration emissions based on regression analysis 基于回归分析的城市固体废物焚烧排放健康风险评估
Pub Date : 2024-02-17 DOI: 10.1016/j.eehl.2024.01.009

This study examined the potential health risks posed by the operation of 96 waste-to-energy (WtE) plants in 30 cities in the Bohai Rim of China. Utilizing a sophisticated simulation approach, the Weather Research and Forecasting (WRF) model coupled with the California Puff (CALPUFF) model, we obtained the spatial distribution of pollutants emitted by WtE plants in the atmosphere. Hazard indices (HI) and cancer risks (CR) were calculated for each plant using the United States Environmental Protection Agency's recommended methodologies. The results indicated that both HIs and CRs were generally low, with values below the accepted threshold of 1.0 and 1.0 × 10−6, respectively. Specifically, the average HI and CR values for the entire study area were 2.95 × 10−3 and 3.43 × 10−7, respectively. However, some variability in these values was observed depending on the location and type of WtE plant. A thorough analysis of various parameters, such as waste composition, moisture content, and operating conditions, was conducted to identify the factors that influence the health risks associated with incineration. The findings suggest that proper waste sorting and categorization, increased cost of construction, and elevated height of chimneys are effective strategies for reducing the health risks associated with incineration. Overall, this study provides valuable insights into the potential health risks associated with WtE plants in the Bohai Rim region of China. The findings can serve as useful guidelines for law enforcement wings and industry professionals seeking to minimize the risks associated with municipal solid waste (MSW) management and promote sustainable development.

本研究探讨了中国环渤海地区 30 个城市的 96 家垃圾焚烧发电厂的运行对健康造成的潜在风险。利用复杂的模拟方法--气象研究与预报 (WRF) 模型与加州浮肿 (CALPUFF) 模型相结合,我们获得了垃圾焚烧发电厂排放的污染物在大气中的空间分布。采用美国环境保护局推荐的方法计算了每个工厂的危害指数 (HI) 和致癌风险 (CR)。结果表明,HI 和 CR 值普遍较低,分别低于 1.0 和 1.0 × 10-6 的公认阈值。具体来说,整个研究区域的 HI 和 CR 平均值分别为 2.95 × 10-3 和 3.43 × 10-7。然而,根据不同地点和不同类型的 WtE 工厂,这些值也存在一些差异。对废物成分、水分含量和运行条件等各种参数进行了全面分析,以确定影响焚烧相关健康风险的因素。研究结果表明,适当的垃圾分类和分级、增加建设成本和提高烟囱高度是降低焚烧相关健康风险的有效策略。总之,本研究为了解中国环渤海地区与热电联产工厂相关的潜在健康风险提供了宝贵的见解。研究结果可为执法部门和行业专业人士提供有用的指导,以最大限度地降低城市固体废物(MSW)管理的相关风险,促进可持续发展。
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引用次数: 0
Associations of short-term ambient temperature exposure with lung function in middle-aged and elderly people: A longitudinal study in China 短期环境温度暴露与中老年人肺功能的关系:中国的一项纵向研究
Pub Date : 2024-02-10 DOI: 10.1016/j.eehl.2024.01.008
Weihong Qiu , Bin Wang , Xiaobing Feng , Heng He , Lieyang Fan , Zi Ye , Xiuquan Nie , Ge Mu , Wei Liu , Dongming Wang , Min Zhou , Weihong Chen

The short-term associations of ambient temperature exposure with lung function in middle-aged and elderly Chinese remain obscure. The study included 19,128 participants from the Dongfeng-Tongji cohort's first (2013) and second (2018) follow-ups. The lung function for each subject was determined between April and December 2013 and re-assessed in 2018, with three parameters (forced vital capacity [FVC], forced expiratory volume in 1 s [FEV1], and peak expiratory flow [PEF]) selected. The China Meteorological Data Sharing Service Center provided temperature data during the study period. In the two follow-ups, a total of 25,511 records (average age: first, 64.57; second, 65.80) were evaluated, including 10,604 males (41.57%). The inversely J-shaped associations between moving average temperatures (lag01–lag07) and FVC, FEV1, and PEF were observed, and the optimum temperatures at lag04 were 16.5 °C, 18.7 °C, and 16.2 °C, respectively. At lag04, every 1 °C increase in temperature was associated with 14.07 mL, 9.78 mL, and 62.72 mL/s increase in FVC, FEV1, and PEF in the low-temperature zone (<the optimum temperatures), whereas 5.72 mL, 2.01 mL, and 11.64 mL/s decrease in the high-temperature zone (≥the optimum temperatures), respectively (all P < 0.05). We observed significant effect modifications of gender, age, body mass index, body surface area, smoking status, drinking status, and physical activity on the associations (all Pmodification < 0.05). Non-optimal temperatures may cause lung function decline. Several individual characters and lifestyles have effect modification on the temperature effects.

环境温度暴露与中国中老年人肺功能的短期关系仍不明确。该研究纳入了东风-同济队列第一次(2013年)和第二次(2018年)随访的19128名参与者。每个受试者的肺功能在2013年4月至12月期间测定,并于2018年重新评估,选取了三个参数(用力肺活量[FVC]、1 s内用力呼气容积[FEV1]和呼气峰流速[PEF])。中国气象数据共享服务中心提供了研究期间的气温数据。在两次随访中,共评估了 25,511 份记录(平均年龄:第一次,64.57 岁;第二次,65.80 岁),其中包括 10,604 名男性(41.57%)。移动平均温度(lag01-lag07)与 FVC、FEV1 和 PEF 呈反向 J 型关系,lag04 时的最佳温度分别为 16.5 °C、18.7 °C 和 16.2 °C。在滞后 04 期,温度每升高 1 °C,低温区(最佳温度)的 FVC、FEV1 和 PEF 分别增加 14.07 mL、9.78 mL 和 62.72 mL/s,而高温区(≥最佳温度)则分别减少 5.72 mL、2.01 mL 和 11.64 mL/s(所有 P 均为 0.05)。我们观察到性别、年龄、体重指数、体表面积、吸烟状况、饮酒状况和体力活动对相关性有明显的影响修正(所有 Pmodification < 0.05)。非最佳温度可能导致肺功能下降。一些个体特征和生活方式会对温度效应产生影响。
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引用次数: 0
Characterizing the photodegradation-induced release of volatile organic compounds from bottled water containers 描述光降解诱导瓶装水容器释放挥发性有机化合物的特征
Pub Date : 2024-02-08 DOI: 10.1016/j.eehl.2024.01.005
Ruijuan Liu , Zhianqi Liao , Jing Zheng , Xinni Wu , Zongyi Tan , Huase Ou

While plastic water bottles are known to potentially release various volatile organic compounds (VOCs) when exposed to light, existing knowledge in this field remains limited. In this study, we systematically examined the composition, yield, and toxicity of VOCs released from six plastic containers obtained from different continents under UV-A and solar irradiation. After light exposure, all containers released VOCs, including alkanes, alkenes, alcohols, aldehydes, carboxylic acids, aromatics, etc. The 1#, 3#, 4#, 5#, and 6# containers exhibited 35, 32, 19, 24 and 37 species of VOCs, respectively. Specifically, the 2# container released 28 and 32 series of VOCs after 1-day (short-term) and 7-day (long-term) UV-A irradiation, respectively, compared to 30 and 32 species under solar irradiation. Over half of the VOCs identified were oxidized compounds alongside various short-chain hydrocarbons. Significant differences in VOC compositions among the containers were observed, potentially originating from light-induced aging and degradation of the polyethylene terephthalate structure in the containers. Toxicological predictions unveiled distinctive toxic characteristics of VOCs from each container. For example, among the various VOCs produced by the 2# container, straight-chain alkanes like n-hexadecane (544-76-3) were identified as the most toxic compounds. After long-term irradiation, the yield of these toxic VOCs from the 2# container ranged from 0.11 ng/g to 0.79 ng/g. Considering the small mass of a single bottle, the volatilization of VOCs from an individual container would be insignificant. Even after prolonged exposure to light, the potential health risks associated with inhaling VOCs when opening and drinking bottled water appear manageable.

众所周知,塑料水瓶在光照下可能会释放出各种挥发性有机化合物(VOC),但该领域的现有知识仍然有限。在这项研究中,我们系统地研究了在紫外线-A 和太阳光照射下,从不同大陆获取的六个塑料容器释放的挥发性有机化合物的成分、产量和毒性。光照后,所有容器都释放出挥发性有机化合物,包括烷烃、烯烃、醇、醛、羧酸、芳烃等。1#、3#、4#、5#和 6#容器分别释放出 35、32、19、24 和 37 种挥发性有机化合物。具体来说,2# 容器在经过 1 天(短期)和 7 天(长期)紫外线-A 照射后,分别释放出 28 和 32 个系列的挥发性有机化合物,而在太阳光照射下则分别释放出 30 和 32 个系列的挥发性有机化合物。已确定的挥发性有机化合物中有一半以上是氧化化合物和各种短链碳氢化合物。据观察,不同容器中的挥发性有机化合物成分存在显著差异,这可能是由于光引起的容器聚对苯二甲酸乙二醇酯结构老化和降解所致。毒理学预测揭示了每个容器中挥发性有机化合物的独特毒性特征。例如,在 2#容器产生的各种挥发性有机化合物中,正十六烷(544-76-3)等直链烷烃被确定为毒性最强的化合物。经过长期辐照,2# 容器产生的这些有毒挥发性有机化合物的产量介于 0.11 纳克/克到 0.79 纳克/克之间。考虑到单个瓶子的质量较小,单个容器中挥发性有机化合物的挥发量微乎其微。即使长时间暴露在光线下,打开和饮用瓶装水时吸入挥发性有机化合物对健康造成的潜在风险似乎也是可控的。
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引用次数: 0
Associating prenatal phthalate exposure with childhood autistic traits: Investigating potential adverse outcome pathways and the modifying effects of maternal vitamin D 产前接触邻苯二甲酸盐与儿童自闭症特征的关系:研究潜在的不良后果途径和母体维生素 D 的调节作用
Pub Date : 2024-02-07 DOI: 10.1016/j.eehl.2024.01.007
The association between prenatal phthalate mixture exposure and the risk of autism spectrum disorder (ASD) in children, as well as the potential mechanism and impact of maternal vitamin D, remains unclear. We analyzed data from 3209 mother–child pairs. The associations between prenatal phthalate exposure and autistic traits in children aged 1.5, 3, 5, and 6 years were explored. Furthermore, the modifying effects of maternal vitamin D and the adverse outcome pathway, which elucidates the contribution of phthalates to ASD, were estimated. Exposure to a phthalate mixture was associated with an increased risk of ASD in children aged 1.5–6 years. For mothers with 25(OH)D deficiency, an exposure‒response relationship was observed between phthalate mixtures in early to mid-pregnancy and autistic traits in children aged 3 years. However, this association was not observed for mothers with sufficient prenatal 25(OH)D levels. The potential mechanism of action of di(2-ethylhexyl) phthalate (DEHP) exposure may involve affecting GRIN2B, inhibiting NMDAR in the postsynaptic membrane, disrupting synaptic function, and impairing learning and memory, ultimately leading to ASD development. Importantly, maternal vitamin D supplementation was demonstrated to mitigate the risk of ASD associated with phthalate exposure. Reducing phthalate exposure during pregnancy may be associated with a decreased risk of autistic traits in children. Furthermore, adequate vitamin D supplementation could potentially mitigate the impact of phthalates on these traits. Additionally, the proposed biological mechanism provides insight into how phthalate exposure may contribute to the development of ASD.
产前接触邻苯二甲酸盐混合物与儿童自闭症谱系障碍(ASD)风险之间的关系以及母体维生素 D 的潜在机制和影响仍不清楚。我们分析了 3209 对母子的数据。我们探讨了产前邻苯二甲酸盐暴露与 1.5、3、5 和 6 岁儿童自闭症特征之间的关联。此外,还估算了母体维生素 D 和不良后果途径的调节作用,从而阐明了邻苯二甲酸盐对自闭症的影响。接触邻苯二甲酸盐混合物与1.5-6岁儿童患ASD的风险增加有关。对于缺乏 25(OH)D 的母亲来说,在孕早期至孕中期接触邻苯二甲酸盐混合物与 3 岁儿童的自闭症特征之间存在暴露-反应关系。然而,产前 25(OH)D 水平充足的母亲则没有观察到这种关系。接触邻苯二甲酸二(2-乙基己基)酯(DEHP)的潜在作用机制可能包括影响GRIN2B,抑制突触后膜上的NMDAR,破坏突触功能,损害学习和记忆,最终导致自闭症的发展。重要的是,母体补充维生素 D 被证明可降低与邻苯二甲酸盐暴露相关的 ASD 风险。减少孕期接触邻苯二甲酸盐可能与降低儿童患自闭症的风险有关。此外,补充充足的维生素 D 有可能减轻邻苯二甲酸盐对这些特征的影响。此外,所提出的生物学机制还有助于人们深入了解接触邻苯二甲酸盐是如何导致自闭症的发展的。
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引用次数: 0
A new ChatGPT-empowered, easy-to-use machine learning paradigm for environmental science 为环境科学提供全新的、由 ChatGPT 支持的、易于使用的机器学习范例
Pub Date : 2024-02-03 DOI: 10.1016/j.eehl.2024.01.006
Haoyuan An , Xiangyu Li , Yuming Huang , Weichao Wang , Yuehan Wu , Lin Liu , Weibo Ling , Wei Li , Hanzhu Zhao , Dawei Lu , Qian Liu , Guibin Jiang

The quantity and complexity of environmental data show exponential growth in recent years. High-quality big data analysis is critical for performing a sophisticated characterization of the complex network of environmental pollution. Machine learning (ML) has been employed as a powerful tool for decoupling the complexities of environmental big data based on its remarkable fitting ability. Yet, due to the knowledge gap across different subjects, ML concepts and algorithms have not been well-popularized among researchers in environmental sustainability. In this context, we introduce a new research paradigm—“ChatGPT + ML + Environment”, providing an unprecedented chance for environmental researchers to reduce the difficulty of using ML models. For instance, each step involved in applying ML models to environmental sustainability, including data preparation, model selection and construction, model training and evaluation, and hyper-parameter optimization, can be easily performed with guidance from ChatGPT. We also discuss the challenges and limitations of using this research paradigm in the field of environmental sustainability. Furthermore, we highlight the importance of “secondary training” for future application of “ChatGPT + ML + Environment”.

近年来,环境数据的数量和复杂性呈指数级增长。高质量的大数据分析对于复杂的环境污染网络进行精密的特征描述至关重要。机器学习(ML)凭借其卓越的拟合能力,已被用作一种强大的工具,用于解耦环境大数据的复杂性。然而,由于不同学科之间存在知识鸿沟,机器学习的概念和算法在环境可持续发展领域的研究人员中尚未得到广泛普及。在此背景下,我们引入了一种新的研究范式--"ChatGPT + ML + 环境",为环境研究人员提供了一个前所未有的机会,以降低使用 ML 模型的难度。例如,在 ChatGPT 的指导下,将 ML 模型应用于环境可持续性的每个步骤,包括数据准备、模型选择和构建、模型训练和评估以及超参数优化,都可以轻松完成。我们还讨论了在环境可持续性领域使用这种研究范式所面临的挑战和局限性。此外,我们还强调了 "二次训练 "对于 "ChatGPT + ML + 环境 "未来应用的重要性。
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引用次数: 0
Comprehensive evaluation framework for intervention on health effects of ambient temperature 环境温度对健康影响干预措施综合评估框架(CEFI-HEAT)
Pub Date : 2024-01-28 DOI: 10.1016/j.eehl.2024.01.004
Jiaming Wang , Peng Wang , Beibei Liu , Patrick L. Kinney , Lei Huang , Kai Chen

Despite the existence of many interventions to mitigate or adapt to the health effects of climate change, their effectiveness remains unclear. Here, we introduce the Comprehensive Evaluation Framework for Intervention on Health Effects of Ambient Temperature to evaluate study designs and effects of intervention studies. The framework comprises three types of interventions: proactive, indirect, and direct, and four categories of indicators: classification, methods, scope, and effects. We trialed the framework by an evaluation of existing intervention studies. The evaluation revealed that each intervention has its own applicable characteristics in terms of effectiveness, feasibility, and generalizability scores. We expanded the framework's potential by offering a list of intervention recommendations in different scenarios. Future applications are then explored to establish models of the relationship between study designs and intervention effects, facilitating effective interventions to address the health effects of ambient temperature under climate change.

尽管存在许多旨在减轻或适应气候变化对健康影响的干预措施,但其效果仍不明确。在此,我们介绍环境温度对健康影响干预综合评估框架,以评估干预研究的设计和效果。该框架包括三类干预措施:主动、间接和直接,以及四类指标:分类、方法、范围和效果。我们通过对现有干预研究的评估试用了该框架。评估结果表明,每种干预措施在有效性、可行性和可推广性方面都有自己的适用特点。我们通过提供不同情况下的干预建议清单,扩大了该框架的潜力。我们还探讨了未来的应用,以建立研究设计与干预效果之间的关系模型,促进采取有效干预措施,应对气候变化下环境温度对健康的影响。
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引用次数: 0
Unraveling the nuclear isotope tapestry: Applications, challenges, and future horizons in a dynamic landscape 揭开核同位素的面纱:动态环境中的应用、挑战和未来前景
Pub Date : 2024-01-12 DOI: 10.1016/j.eehl.2024.01.001
Hang Yang , Qi Feng , Weixiang Xu , Yadong Tang , Guoliang Bai , Yunli Liu , Zisen Liu , Shibin Xia , Zhenbin Wu , Yi Zhang

Nuclear isotopes, distinct atoms characterized by varying neutron counts, have profoundly influenced a myriad of sectors, spanning from medical diagnostics and therapeutic interventions to energy production and defense strategies. Their multifaceted applications have been celebrated for catalyzing revolutionary breakthroughs, yet these advancements simultaneously introduce intricate challenges that warrant thorough investigation. These challenges encompass safety protocols, potential environmental detriments, and the complex geopolitical landscape surrounding nuclear proliferation and disarmament. This comprehensive review embarks on a deep exploration of nuclear isotopes, elucidating their nuanced classifications, wide-ranging applications, intricate governing policies, and the multifaceted impacts of their unintended emissions or leaks. Furthermore, the study meticulously examines the cutting-edge remediation techniques currently employed to counteract nuclear contamination while projecting future innovations in this domain. By weaving together historical context, current applications, and forward-looking perspectives, this review offers a panoramic view of the nuclear isotope landscape. In conclusion, the significance of nuclear isotopes cannot be understated. As we stand at the crossroads of technological advancement and ethical responsibility, this review underscores the paramount importance of harnessing nuclear isotopes' potential in a manner that prioritizes safety, sustainability, and the greater good of humanity.

核同位素是以不同中子数为特征的独特原子,对从医疗诊断和治疗干预到能源生产和防御战略等众多领域产生了深远影响。它们的多方面应用因催化革命性突破而备受赞誉,但这些进步同时也带来了错综复杂的挑战,需要进行深入研究。这些挑战包括安全协议、潜在的环境危害以及围绕核扩散与核裁军的复杂地缘政治格局。本综述对核同位素进行了深入探讨,阐明了其细微的分类、广泛的应用、错综复杂的管理政策,以及意外排放或泄漏造成的多方面影响。此外,该研究还细致地探讨了目前用于应对核污染的尖端修复技术,同时预测了该领域未来的创新。通过将历史背景、当前应用和前瞻性观点交织在一起,本综述提供了核同位素领域的全景图。总之,核同位素的重要性不容低估。当我们站在技术进步和道德责任的十字路口时,本综述强调了以优先考虑安全、可持续性和人类更大利益的方式利用核同位素潜力的极端重要性。
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引用次数: 0
Mineral-mediated stability of organic carbon in soil and relevant interaction mechanisms 矿物介导的土壤有机碳稳定性及相关相互作用机制
Pub Date : 2024-01-03 DOI: 10.1016/j.eehl.2023.12.003
Zibo Xu , Daniel C.W. Tsang

Soil, the largest terrestrial carbon reservoir, is central to climate change and relevant feedback to environmental health. Minerals are the essential components that contribute to over 60% of soil carbon storage. However, how the interactions between minerals and organic carbon shape the carbon transformation and stability remains poorly understood. Herein, we critically review the primary interactions between organic carbon and soil minerals and the relevant mechanisms, including sorption, redox reaction, co-precipitation, dissolution, polymerization, and catalytic reaction. These interactions, highly complex with the combination of multiple processes, greatly affect the stability of organic carbon through the following processes: (1) formation or deconstruction of the mineral–organic carbon association; (2) oxidative transformation of the organic carbon with minerals; (3) catalytic polymerization of organic carbon with minerals; and (4) varying association stability of organic carbon according to the mineral transformation. Several pieces of evidence related to the carbon turnover and stability during the interaction with soil minerals in the real eco-environment are then demonstrated. We also highlight the current research gaps and outline research priorities, which may map future directions for a deeper mechanisms-based understanding of the soil carbon storage capacity considering its interactions with minerals.

土壤是最大的陆地碳库,是气候变化和环境健康相关反馈的核心。矿物质是土壤碳储存的重要组成部分,占土壤碳储存的 60% 以上。然而,人们对矿物质和有机碳之间的相互作用如何影响碳的转化和稳定性仍然知之甚少。在此,我们对有机碳与土壤矿物之间的主要相互作用及相关机制进行了严格的审查,包括吸附、氧化还原反应、共沉淀、溶解、聚合和催化反应。这些相互作用由多个过程组合而成,非常复杂,通过以下过程极大地影响了有机碳的稳定性:(1)矿物-有机碳关联的形成或解构;(2)有机碳与矿物的氧化转化;(3)有机碳与矿物的催化聚合;以及(4)有机碳的关联稳定性随矿物转化而变化。随后,我们展示了在真实生态环境中与土壤矿物相互作用过程中碳的转化和稳定性的几个相关证据。我们还强调了当前的研究空白,并概述了研究重点,这些研究重点可能为基于机制更深入地理解土壤碳储存能力(考虑其与矿物的相互作用)指明了未来的方向。
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引用次数: 0
Water decontamination by reactive high-valent iron species 活性高价铁物种对水的净化作用
Pub Date : 2023-12-14 DOI: 10.1016/j.eehl.2023.12.002
Yunhui Zhang , Logan Swaren , Wenbing Wang
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引用次数: 0
Free-range poultry eggs as an emerging tool for pollution bio-indication 散养禽蛋作为一种新兴的污染生物指示工具
Pub Date : 2023-12-12 DOI: 10.1016/j.eehl.2023.12.001
Anissa Zergui , Daniel Brice Nkontcheu Kenko
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引用次数: 0
期刊
Eco-Environment & Health
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