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Equilibrium status of naturally occurring 226Ra with radon daughters and estimation of 238U activity from 235U using natural radioactivity ratio of 238U/235U in soil around Rawatbhata, Rajasthan Rajasthan Rawatbhata地区土壤中自然存在的226Ra与氡子体的平衡状态及238U/235U自然放射性比值估算235U的活度
Pub Date : 2022-07-01 DOI: 10.4103/rpe.rpe_9_23
Ajay Gocher, Mohit Sisodia, S. Tiwari, I. Saradhi, A. Kumar
Equilibrium status among 226Ra and radon daughters was studied in soil samples around Rawatbhata, Rajasthan. It was found that the increase in radioactivity of 214Bi (radon daughter) due to complete radon buildup in the sealed container is within 15% which establishes that 226Ra remains in equilibrium with radon daughter in soil of Rawatbhata. Radioactivity of 238U was estimated from the radioactivity of 235U using natural uranium isotopic radioactivity ratio (238U/235U) of 21.5. 238U radioactivity in soil was found in the range 25.8–49.5 Bq/kg with an average of 36.7 Bq/kg which is comparable to the global average of 35 Bq/kg.
研究了拉贾斯坦邦拉瓦特巴塔周围土壤样品中226Ra和氡子体的平衡状态。研究发现,由于密封容器中氡的完全积聚,214Bi(氡子体)的放射性增加在15%以内,这表明226Ra与Rawatbhata土壤中的氡子体保持平衡。使用21.5的天然铀同位素放射性比(238U/235U),根据235U的放射性估算238U的放射性。在土壤中发现238U放射性,范围为25.8–49.5 Bq/kg,平均值为36.7 Bq/kg。这与全球平均值35 Bq/kg相当。
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引用次数: 0
Assessment of environmental radioactivity and groundwater quality around Tummalapalle uranium mining site, Andhra Pradesh, India 印度安得拉邦Tummalapalle铀矿场周围环境放射性和地下水质量评价
Pub Date : 2022-07-01 DOI: 10.4103/rpe.rpe_10_23
Barendra Rana, S. Jha, Samim Molla, M. Dhumale, M. Kulkarni
A comprehensive background radiological status in the surrounding environment of the Tummalapalle U mining and processing facilities was evaluated. Radioactivity in soil and rock was estimated by high-resolution gamma spectroscopy with a high-purity p-type germanium detector. The external gamma radiation level, outdoor 222Rn concentration, radioactivity in the groundwater, and water quality parameters around the Tummalapalle site were studied. The terrestrial radioactivity in soil was higher than the national and global averages in the study region. Radium equivalent activity (Raeq) in soil and rock was much lower than the safe limit of 370 Bq/kg and therefore safe to use as a construction material. Hydrogeochemical analysis indicated that the groundwater in the study region is neutral to medium basic, oxic, fresh to brackish, and predominantly Ca2+-Mg2+-HCO3− (62.5%) type. The hydrogeochemistry of groundwater was primarily governed by rock-aquifer interaction in this region. The data generated in this study can serve as the baseline for this region to understand the change in environmental conditions, if any, due to prolonged anthropogenic activities.
对Tummalapalle铀矿开采和加工设施周围环境的综合本底辐射状况进行了评价。用高纯度p型锗探测器,用高分辨率伽玛能谱法测定了土壤和岩石中的放射性。研究了Tummalapalle场址周围的外部伽马辐射水平、室外222Rn浓度、地下水放射性以及水质参数。研究区土壤陆源放射性水平高于全国和全球平均水平。土壤和岩石中的镭当量活度(Raeq)远低于370 Bq/kg的安全限值,因此可以安全用作建筑材料。水文地球化学分析表明,研究区地下水为中性~中碱性、含氧、鲜~半咸淡水,以Ca2+-Mg2+-HCO3−为主(62.5%)。该区地下水水文地球化学主要受岩石-含水层相互作用支配。本研究产生的数据可以作为该地区了解由于长期人为活动而导致的环境条件变化的基线。
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引用次数: 0
Estimation of aquatic dilution factor for liquid effluent discharges from Kaiga Generating Station using tritium as a tracer 用氚作示踪剂估算海贺电站液体出水水中稀释系数
Pub Date : 2022-07-01 DOI: 10.4103/rpe.rpe_37_22
T. Reji, R. Joshi, T. Ajith, Sanyam Jain, M. Vishnu, I. Saradhi, A. Vinodkumar
Very low-level radioactive liquid effluents much below the approved discharge limits are discharged to Kadra reservoir after dilution with condenser cooling water at Kaiga Generating Station. In addition, further dilution occurs from the discharge point to the nearest public utilization point in Kadra reservoir (Hartuga). The dilution obtained in Kadra reservoir is estimated by simultaneous measurements of tritium at the discharge point and at Hartuga. The on-site measurement indicates a dilution factor of 12.2 ± 2.4 for tritium. A dilution factor of 13.3 ± 3.4 was obtained using aquatic dispersion model.
远低于批准排放限值的极低放射性液体流出物经Kaiga发电站的冷凝器冷却水稀释后排放到Kadra水库。此外,从排放点到Kadra水库(Hartuga)最近的公共利用点发生进一步稀释。通过在排放点和Hartuga同时测量氚来估计Kadra水库中获得的稀释。现场测量表明,氚的稀释系数为12.2±2.4。采用水生分散模型得到的稀释系数为13.3±3.4。
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引用次数: 0
Evolution of beryllium safety standards over the last 70 years and challenges ahead 铍安全标准在过去70年中的演变和未来的挑战
Pub Date : 2022-07-01 DOI: 10.4103/rpe.rpe_6_23
Munish Kumar, A. Srivastava
Beryllium (Be), its alloys, and ceramics are widely used in high-tech applications such as electronics, space, atomic energy, and other day-to-day items of use. Initially, Be-based phosphors such as ZnBeSiO4 were being used in the lamp industry during the 1930s onward but were soon abandoned due to lung-related diseases and deaths of workers in the phosphor industry which was attributed to the highly toxic nature of Be. Typical effects associated with Be inhalation are chronic and acute Be diseases (CBD and ABD) and the main target organ being affected is the lung although effects on other human body organs are also well documented. Such diseases were observed not only in occupational workers handling Be but also in the members of the public residing in the neighborhood of Be manufacturing and processing facilities, especially in the USA. The CBD in occupational workers may depend on many factors such as individual's sensitivity to Be, amount of Be exposure, nature of Be compound, and types of Be operations and processes being performed. All this led to safety concerns about the toxicity of Be and recommendations regarding Be air concentration in the workplace and public environment were issued by the Department of Energy, USA in 1949 as occupational exposure limit (OEL)/threshold limit values (TLVs) which were 2.0 μg/m3 and 0.01 μg/m3 for occupational Be workers and public environment, respectively. It is worth to mention that these recommendations were adopted by various countries and organizations either as it is or with small changes. Later, different organizations recommended changes in the value of TLV for occupational workplaces, but such changes were never adopted as they were lacking sound epidemiological basis. The OEL/TLV of 2.0 μg/m3 continued for nearly 70 years until Occupational Safety and Health Administration (OSHA) in 2017 reduced the Be air concentration (BeAir-Conc) limit for occupational workers to 0.20 μg/m3 as the value of 2.00 μg/m3 was inadequate to protect occupational workers from CBD. This is a major change in the Be-related safety standards recommended recently and is/being adopted by many countries. The present article provides details about the evolution of Be safety standards over the last 70 years, the notion behind the recent revision of Be permissible exposure limit (PEL) value from 2.0 μg/m3 to 0.20 μg/m3 by OSHA and the associated safety challenges ahead. The information from literature about Be safety and related safety standards adopted in India is also given. The article also provides details about TLVs for BeAir-Conc being followed in various countries in the world and various challenges for the implementation of a revised PEL value of 0.20 μg/m3 as suggested by OSHA i.e., reduction in PEL value by a factor of 10 or recommendation of revised TLV of 0.05 μg/m3 by American Conference of Governmental Industrial Hygienists as compared to the previous value of 2.0 μg/m3. In view of different notations and limit
铍(Be)及其合金和陶瓷广泛用于高科技应用,如电子、太空、原子能和其他日常用品。最初,Be基磷光体,如ZnBeSiO4,在20世纪30年代以后被用于灯具行业,但由于Be的剧毒性质,磷光体行业工人的肺部相关疾病和死亡,很快被放弃。与吸入Be相关的典型影响是慢性和急性Be疾病(CBD和ABD),受影响的主要靶器官是肺,尽管对其他人体器官的影响也有充分的记录。这种疾病不仅在处理Be的职业工人中观察到,而且在Be制造和加工设施附近的公众中也观察到,尤其是在美国。职业工人的CBD可能取决于许多因素,如个人对Be的敏感性、Be暴露量、Be化合物的性质,以及正在执行的Be操作和过程的类型。所有这些都导致了对Be毒性的安全担忧,美国能源部于1949年发布了关于工作场所和公共环境中Be空气浓度的建议,作为职业暴露限值(OEL)/阈值限值(TLV),对职业Be工人和公共环境分别为2.0μg/m3和0.01μg/m3。值得一提的是,这些建议是由各个国家和组织通过的,要么是按现状通过,要么是稍作修改。后来,不同的组织建议改变职业工作场所的TLV值,但这些改变从未被采纳,因为它们缺乏健全的流行病学基础。2.0μg/m3的OEL/TLV持续了近70年,直到职业安全与健康管理局(OSHA)在2017年将职业工人的Be空气浓度(BeAir-Conc)限值降至0.20μg/m3,因为2.00μg/m3的值不足以保护职业工人免受CBD的影响。这是最近推荐的Be相关安全标准的一个重大变化,许多国家正在采用。本文详细介绍了过去70年来Be安全标准的演变,OSHA最近将Be允许暴露限值(PEL)从2.0μg/m3修订为0.20μg/m3的概念,以及未来的相关安全挑战。还提供了有关Be安全和印度采用的相关安全标准的文献信息。文章还详细介绍了世界各国对BeAir Conc的TLV的遵守情况,以及OSHA建议的0.20μ。,PEL值降低了10倍,或者美国政府工业卫生学家会议建议将TLV修正为0.05微克/立方米,而之前的值为2.0微克/立方米。鉴于各机构推荐的BeAir Conc的不同符号和限制,以及Be安全相关细节的有限信息,本文包含了过去70年Be安全标准的演变过程中有关Be安全的所有相关信息。这对个人在职业工作场所的安全以及环境安全都是一个重要问题,从标准制定到今天,它的汇编对于提供关于Be安全的全面信息是非常必要的。
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引用次数: 0
Theoretical evaluation of calibration factor for LR-115 cellulose nitrate solid state nuclear track detectors: A model for determining alpha radioactivity level in natural water LR-115硝酸纤维素固体核径迹探测器标定系数的理论评价:测定天然水中α放射性水平的模型
Pub Date : 2022-07-01 DOI: 10.4103/rpe.rpe_26_22
Biswajit Das, A. Deb
Alpha-sensitive solid-state nuclear track detectors (SSNTDs) are used successively for decades for determining the alpha-radiation level in various environmental materials. A model for measurement of total alpha-radioactivity in natural water by using alpha-sensitive LR-115 type II cellulose nitrate (CN) film SSNTDs has been developed in the present work. The LR-115 CN films in bare mode are assumed to be immersed into a water sample for alpha-exposure. During the exposure time period, the alpha-particles that are emitted from the alpha-emitters present in the water sample will interact with the CN film and create their latent trails in the film. These latent trails will be manifested as pits of alpha-tracks after chemical etching of the exposed film. For alpha-radioactivity measurement, calibration factor (CF) for LR-115 type II SSNTDs has been evaluated theoretically by using the range of alpha-particles of residual energies situated between 1.6 MeV and 4.7 MeV in natural water and the actual geometry of experimental setup for alpha-exposure. The evaluated CF is found to be 204.93 Bq.l − 1.(tracks. cm − 2.h − 1)−1. The evaluated CF and experimental procedure can reliably be utilized in monitoring the alpha-radioactivity of natural water and in other radioactivity field measurements.
几十年来,固体核径迹探测器(SSNTDs)一直被用于测定各种环境材料中的α辐射水平。本文建立了一种利用α敏感的LR-115型II型硝酸纤维素(CN)薄膜SSNTDs测量天然水中总α -放射性的模型。假设裸露模式下的LR-115 CN薄膜浸入水样中进行α曝光。在曝光期间,水样中存在的α -发射器发射的α -粒子将与CN膜相互作用,并在膜中产生潜在的痕迹。这些隐迹经过曝光胶片的化学蚀刻后会表现为凹坑。在α放射性测量方面,利用自然水体中α粒子的残余能量在1.6 MeV ~ 4.7 MeV之间的范围和α暴露实验装置的实际几何形状,从理论上评估了LR-115型SSNTDs的校准因子(CF)。评价的CF值为204.93 Bq。L−1。Cm−2.h−1)−1。评价后的CF和实验方法可可靠地用于天然水体的α -放射性监测和其他放射性现场测量。
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引用次数: 0
The behavior of mill tailings produced from a uranium extraction plant adapted an indigenously developed alkaline leaching-assisted process 采用自主开发的碱性浸出辅助工艺的铀提取厂尾矿的行为
Pub Date : 2022-07-01 DOI: 10.4103/rpe.rpe_17_23
Barendra Rana, Samim Molla, M. Dhumale, S. Jha, M. Kulkarni
The potential impact of tailings with respect to uranium and its associated toxic metals in the surrounding environment is assessed by identifying their concentrations and physicochemical behavior in the tailings. Tessier's sequential extraction method was used to study the speciation of U, Co, Zn, Mn, Fe, Pb, Cr, and Cd in different geochemical fractions of the alkaline mill tailings of the Tummalapalle process plant. The study indicated that uranium and other toxic metals present in the tailings have different chemical forms. Most of the toxic elements are not readily available in an exchangeable phase; rather, they are present in the tailings in stable complex form. However, a few elements, such as Co, Pb, and Cd, showed significantly higher concentrations in the oxidizing phase. The elements present in the oxidizing phases can be labile after prolonged exposure to atmospheric conditions. U (nat.) and Fe associated with the tailings are indicated to be mostly distributed in the residual phase. Radioactive disequilibrium of 238U and 232Th series radionuclides in the ore, waste rock, and tailings were studied. Disequilibrium was mostly noticed in the 238U series radionuclides in these matrices; however, the 232Th series radionuclides showed a radioactive equilibrium between their parents and daughters.
通过确定尾矿中铀及其伴生有毒金属的浓度和物理化学行为,评价尾矿对周围环境的潜在影响。采用Tessier顺序萃取法研究了Tummalapalle厂碱矿尾矿不同地球化学组分中U、Co、Zn、Mn、Fe、Pb、Cr、Cd的形态。研究表明,尾矿中的铀和其他有毒金属具有不同的化学形态。大多数有毒元素在交换相中不容易得到;相反,它们以稳定的复合形式存在于尾矿中。而Co、Pb、Cd等元素在氧化相中浓度明显升高。氧化相中的元素在长时间暴露于大气条件后是不稳定的。与尾矿伴生的铀和铁主要分布在残余相中。研究了238U和232Th系列放射性核素在矿石、废石和尾矿中的放射性不平衡。在这些基质中,238U系列放射性核素主要存在不平衡;然而,232Th系列放射性核素在母体和子体之间表现出放射性平衡。
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引用次数: 0
A study on the level of terrestrial gamma and gross alpha activity in Gulf of Mannar, South coast of India, Tamil Nadu 印度泰米尔纳德邦南海岸马纳尔湾陆地伽玛和总α活动水平的研究
Pub Date : 2022-07-01 DOI: 10.4103/rpe.rpe_21_22
R. Krishnamoorthy, O. Basith, M. Mohamed Jaffer
This study presents the results of outdoor ambient gamma and gross alpha activity of Gulf of Mannar, and these measurements were carried out using Scintillation Counter (UR-705). Results showed that the terrestrial Gamma radiation levels of the Gulf of Mannar ranged from 4.10 μR/h to 76.33 μR/h. The Gross alpha radioactivity levels of the Gulf of Mannar ranged between 3.67 Bq/kg and 51.34 Bq/kg. The calculated ambient gamma and gross alpha activity were found to be lower than the world average. Gamma absorbed dose rates in air outdoors were calculated to be in the range between 35.67 nGy/h and 664.07 nGy/h with an arithmetic mean of 98.98 ± 20.54 nGy/h. This value is lower than the population-weighted world-averaged of 60 nGy/h. Inhabitants of Northern Gulf of Mannar are subjected to external gamma Annual dose exposure ranging between 0.30 and 5.65 mGy/y with an arithmetic mean of 0.84 ± 0.17 mGy/y.
本研究介绍了马纳尔湾室外环境伽马和总α活动的结果,这些测量是使用闪烁计数器(UR-705)进行的。结果表明:马纳尔湾陆地γ辐射水平在4.10 ~ 76.33 μR/h之间;马纳尔湾的总α放射性水平介于3.67 Bq/kg至51.34 Bq/kg之间。计算出的环境伽马和总α活动低于世界平均水平。室外空气中γ吸收剂量率在35.67 ~ 664.07 nGy/h之间,算术平均值为98.98±20.54 nGy/h。这个值低于人口加权的世界平均水平60 nGy/h。马纳尔湾北部居民遭受的外部γ年剂量暴露范围为0.30至5.65毫戈瑞/年,算术平均值为0.84±0.17毫戈瑞/年。
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引用次数: 0
Optimization of FLUKA detector model for HPGe array HPGe阵列FLUKA探测器模型的优化
Pub Date : 2022-07-01 DOI: 10.4103/rpe.rpe_35_22
C. Charubala, V. Santhanakrishnan, G. Ganesh, M. Kulkarni
Monte Carlo codes, such as FLUKA, are widely used to optimize calibration of spectrometric systems. HPGe detector array (HDA) for lung monitoring was modeled in FLUKA code using available information about their geometry and optimized for efficiency using 241Am point source at smaller distances (<10 cm) as in case of in-vivo monitoring scenarios. Thickness of dead layer (DL) on the top and lateral detector surfaces for low energy counting was determined by considering the experimental and simulated efficiency for various energies. Using trial and error method, optimized DL thickness was found out to be 2.5 μm on top surface and 1.8 mm on lateral surfaces for each HPGe detector in the array. For the optimized model, it was found that the simulated and experimental efficiency and the simulated and experimental spectra were in reasonable agreement. Optimization of the HDA was an important benchmarking step to reduce the simulation errors before they are implemented in complex numerical problems using computational phantoms.
蒙特卡罗代码,如FLUKA,被广泛用于优化光谱系统的校准。用于肺部监测的HPGe探测器阵列(HDA)在FLUKA代码中使用有关其几何形状的可用信息进行建模,并在体内监测场景中使用较小距离(<10 cm)的241Am点源进行效率优化。考虑不同能量下的实验效率和模拟效率,确定了低能量计数时探测器顶部和侧面的死层厚度。通过试错法确定了阵列中每个HPGe探测器的最优DL厚度为上表面2.5 μm,侧表面1.8 mm。结果表明,优化模型的模拟效率与实验效率、模拟光谱与实验光谱基本一致。HDA的优化是在复杂数值问题中使用计算幻影实现之前减少仿真误差的重要基准测试步骤。
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引用次数: 0
Studies on the contribution of the aquatic water body to the tritium flux in the atmosphere near the discharge point of Kakrapar Gujarat Site, India 印度Kakrapar Gujarat场址排放点附近水体对大气中氚通量贡献的研究
Pub Date : 2022-04-01 DOI: 10.4103/rpe.rpe_24_22
C. Joshi, A. Patra, D. P. Nankar, I. Saradhi, AVinod Kumar
The contribution of the aquatic water body to the tritium (3H) flux in the atmosphere near the discharge point of Kakrapar Gujarat Site has been assessed by collecting and analyzing the 3H activity in the air moisture and in the water sample near the aquatic discharge point. The observed air 3H activity near the discharge point was in the range of ≤0.20–19.8 Bq/m3, whereas the predicted 3H activity at the same location due to the atmospheric release through stack varied from 0.10 to 0.15 Bq/m3. The range of water 3H activity through the discharge point varied from ≤10 to 3482 Bq/l. The 3H flux (water to air transfer) was estimated and found to be in the range of ≤5.90E+01 – 2.05E+04 Bq/m2/s. The observation shows that during radioactive aquatic releases, there is an increase in the 3H activity levels in the water vapor near the aquatic discharge point. The observed 3H activity levels in air samples were extremely low to contribute any additional dose to the member of the public as compared to the public dose obtained from natural background sources.
通过收集和分析Kakrapar Gujarat站点排放点附近空气湿度和水样中的3H活度,评价了水体对排放点附近大气中氚(3H)通量的贡献。在排放点附近观测到的3H活度在≤0.20 ~ 19.8 Bq/m3之间,而在同一地点由于大气通过堆叠释放的3H活度预测值在0.10 ~ 0.15 Bq/m3之间。通过排放点的水3H活度范围为≤10 ~ 3482 Bq/l。3H通量(水到空气的传递)估计在≤5.90E+01 - 2.05E+04 Bq/m2/s范围内。观测结果表明,在放射性水体释放过程中,水体排放点附近水蒸气中的3H活性水平有所升高。与从自然本底来源获得的公众剂量相比,空气样本中观察到的3H活性水平极低,不会对公众产生任何额外剂量。
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引用次数: 0
Radiological safety during sodium diuranate dissolution process: A radiological data study 二铀酸钠溶解过程中的放射安全性:放射学资料研究
Pub Date : 2022-04-01 DOI: 10.4103/rpe.rpe_12_22
M. Shailesh, SK Suman, PK Malti, V. Pol, S. Manna, RV Kolekar, SK Satpati
The article presents an overview of the occupational radiation protection aspects of experimental sodium diuranate transferring and handling processes required for refining utilization. The health physics aspects and associated monitoring programs necessary to adequately measure and control radiological exposures to workers during the process is described here. A particle size distribution study was also carried out and estimated the activity median aerodynamic diameter (AMAD) for the process. The AMAD varied from 4.6 to 7.7 μm and geometric standard deviation ranged from 1.9 to 2.8. Obtained data serve the purpose of comparison for formulating a detailed radiological safety protocol during regular operation.
本文综述了炼化利用实验用重铀酸钠转移和处理工艺中职业辐射防护方面的问题。健康物理方面和相关的监测程序,以充分测量和控制辐射暴露的工人在这个过程中进行了描述。还进行了粒径分布研究,并估计了该工艺的活度中值气动直径(AMAD)。AMAD范围为4.6 ~ 7.7 μm,几何标准差范围为1.9 ~ 2.8。获得的数据用于比较,以便在正常操作时制定详细的放射安全方案。
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引用次数: 0
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Radiation Protection and Environment
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