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Does Haze Pollution Inhibit Innovation Efficiency in China? The Mediating Role of Human Capital and the Moderating Role of Government Attention 雾霾污染是否抑制了中国的创新效率?人力资本的中介作用和政府关注的调节作用
IF 11.1 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Pub Date : 2024-11-19 DOI: 10.1016/j.jclepro.2024.144261
Qian Wang, Songzi Zhang, Shuming Ren
The problem of low innovation efficiency in developing countries has gained increasing attention, although there is little empirical evidence to examine this issue, especially from a haze pollution perspective. To fill this critical gap, this paper employs a series of empirical methods to investigate the impact of haze pollution on innovation efficiency and takes a panel dataset covering 30 provincial-level regions in China over 2010∼2018 as a case study. Results show that: (1) An increase in haze pollution has an inhibitory effect on China’s provincial innovation efficiency, whether for the overall, R&D, and commercialization efficiency. (2) Such a negative effect is exacerbated in provinces with low levels of urbanization and financial development, presenting a preference for poor territories. (3) Regarding spatial spillover effects, innovation efficiency in a given province is negatively correlated with haze pollution from neighboring provinces. (4) Regarding mediating factors, haze pollution reduces human capital and subsequently can inhibit innovation efficiency, i.e., the “human capital loss effect”. (5) Regarding moderating factors, rather than a “cost following effect”, government attention mitigates the inhibiting effect of haze pollution on innovation efficiency through an “innovation compensation effect”. In general, policymakers should seek a win-win situation between innovation activities and environmental protection.
发展中国家创新效率低下的问题日益受到关注,但研究这一问题的实证证据却很少,尤其是从雾霾污染的角度研究这一问题。为填补这一重要空白,本文采用一系列实证方法研究雾霾污染对创新效率的影响,并以 2010∼2018 年中国 30 个省级地区的面板数据集为研究案例。结果表明(1)雾霾污染的增加对中国省级创新效率有抑制作用,无论是整体效率、研发效率还是商业化效率。(2)在城市化水平和金融发展水平较低的省份,这种负面影响会加剧,呈现出对贫困地区的偏好。(3)在空间溢出效应方面,某一省份的创新效率与周边省份的雾霾污染呈负相关。(4)在中介因素方面,雾霾污染会降低人力资本,进而抑制创新效率,即 "人力资本损失效应"。(5) 在调节因素方面,政府关注通过 "创新补偿效应 "而非 "成本追随效应 "缓解了雾霾污染对创新效率的抑制作用。总之,决策者应在创新活动与环境保护之间寻求双赢。
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引用次数: 0
Efficient degradation of chloroquine via pyrite-modified electro-Fenton yielding •OH and O2•- 通过产生-OH和O2的黄铁矿改性电-芬顿高效降解氯喹
IF 11.1 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Pub Date : 2024-11-19 DOI: 10.1016/j.jclepro.2024.144256
Yuehua Zhang, Yinghui Lin, Yuanji Shi, Linyan Yang, Bing-Jie Ni, Xueming Chen
In the face of the mass production and consumption of chloroquine (CLQ), the presence of CLQ has posed a significant threat to the water environment and living organisms due to its bio-accumulative and persistent nature. In this work, a heterogeneous electro-Fenton system using a pyrite-modified carbon felt as the cathode (EF-FeS2-CF) was constructed to remove CLQ. EF-FeS2-CF was found to achieve 92.4±0.1% removal of 5 mg/L CLQ after 30 min at 20 mA and exhibited an outstanding catalytic performance for CLQ removal in wide ranges of operating conditions, excellent recyclability with low iron leaching (> 90% 30-min CLQ removal efficiency for all five cyclic experiments which led to only an accumulative Fe loss of < 0.3%) and remarkable application potential in different aqueous environments without any pH adjustment. Both O2•- and OH were found to greatly contribute to CLQ degradation while the latter played a major role (> 50% CLQ removal). To describe CLQ degradation towards complete mineralization in EF-FeS2-CF, three CLQ degradation paths were proposed based on the main degradation intermediates identified with generally lower ecotoxicities. Such an EF-FeS2-CF system therefore presents promising application potential to treat CLQ-laden waters.
随着氯喹(CLQ)的大量生产和消费,由于其生物累积性和持久性,CLQ 的存在对水环境和生物体构成了严重威胁。本研究以黄铁矿改性碳毡(EF-FeS2-CF)为阴极,构建了一个异相电-芬顿系统来去除 CLQ。结果表明,EF-FeS2-CF 在 20 mA 电流下 30 分钟后对 5 mg/L CLQ 的去除率为 92.4±0.1%,在各种操作条件下对 CLQ 的去除均表现出卓越的催化性能,并且具有极低的铁浸出率和良好的可回收性(所有五次循环实验的 30 分钟 CLQ 去除率均为 90%,累计铁损耗仅为 0.3%),在不同水环境中具有显著的应用潜力,无需调节 pH 值。研究发现,O2--和-OH 对 CLQ 的降解都有很大的促进作用,而后者起着主要作用(CLQ 去除率达 50%)。为了描述CLQ在EF-FeS2-CF中完全矿化的降解过程,根据生态毒性通常较低的主要降解中间体,提出了三种CLQ降解途径。因此,这种 EF-FeS2-CF 系统在处理含有 CLQ 的水体方面具有广阔的应用前景。
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引用次数: 0
Operational Energy Savings in Greenhouses by Retrofitting Covering Plastics with Photothermal Antimony Tin Oxide Nanocoating 用光热氧化锑纳米涂层改装覆盖塑料,节约温室运行能耗
IF 11.1 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Pub Date : 2024-11-19 DOI: 10.1016/j.jclepro.2024.144242
Mohammad Elmi, Enhe Zhang, Anwar Jahid, Julian Wang
Energy management in greenhouses is crucial as they demand high energy consumption to keep a desirable environment for products. In this study, a novel greenhouse covering coating is introduced based on photothermal plasmonic nanoparticles to reduce energy consumption in greenhouses. Antimony tin oxide nanoparticles were used as plasmonic nanoparticles and were deposited on polyethylene greenhouse coverings. Thermal and optical properties of the Antimony Tin Oxide-coated covering were characterized, and a comprehensive seasonal greenhouse energy analysis was performed to investigate the energy performance of the developed greenhouse covering. The photosynthetically active radiation (PAR) transmittance of the developed covering is 0.746, and the PAR-to-Solar-Transmittance (PST) value increased about 75% by the new covering. Based on the results, developed greenhouse covering with photothermal plasmonic nanoparticles drops greenhouse heating load by 70% and reduces total greenhouse energy consumption up to 49% in very cold climates. Antimony Tin Oxide nanocoating itself increases greenhouse energy saving by 11.4% in comparison with uncoated-double-layer polyethylene covering. Greenhouse energy savings in this study were achieved without any compromise in photosynthetically active radiation (PAR) and crop growth. A greenhouse covering utilization guideline is provided for each climate zone based on the results of this study to optimize the energy use in the greenhouse. This study opens a new window to innovative material applications in greenhouses to make greenhouses more sustainable and energy-efficient.
温室的能源管理至关重要,因为温室需要高能耗来为产品保持理想的环境。本研究介绍了一种基于光热质子纳米粒子的新型温室覆盖涂层,以降低温室的能耗。该研究采用锑锡氧化物纳米粒子作为质子纳米粒子,并将其沉积在聚乙烯温室覆盖物上。对氧化锑锡涂层覆盖物的热性能和光学性能进行了表征,并进行了全面的季节性温室能源分析,以研究开发的温室覆盖物的能源性能。所开发覆盖物的光合有效辐射(PAR)透射率为 0.746,PAR-太阳透射率(PST)值在新覆盖物的作用下提高了约 75%。根据研究结果,所开发的带有光热质子纳米粒子的温室覆盖物可将温室加热负荷降低 70%,在极寒气候条件下可将温室总能耗降低 49%。与未涂层的双层聚乙烯覆盖物相比,纳米氧化锑锡涂层本身可使温室节能效果提高 11.4%。这项研究在不影响光合有效辐射(PAR)和作物生长的情况下实现了温室节能。根据这项研究的结果,为每个气候区提供了温室覆盖物利用指南,以优化温室的能源利用。这项研究为创新材料在温室中的应用打开了一扇新窗口,使温室更具可持续性和能源效率。
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引用次数: 0
Facilitating lignocellulose fractionation of Moringa oleifera Lam. husk by pretreatment with a novel 1-tetradecyl-3-carboxymethylimidazolium bromide-based deep eutectic solvent 使用新型 1-十四烷基-3-羧甲基溴化咪唑鎓深共晶溶剂进行预处理,促进油辣木籽壳的木质纤维素分馏
IF 11.1 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Pub Date : 2024-11-18 DOI: 10.1016/j.jclepro.2024.144249
Jiabo Cheng, Yuan Gao, Jie Liu, Yuting Zhang, Mengfei Tian, Mengying Zhang, Yaru Zhang, Chunjian Zhao, Chunying Li
Refining lignocellulose into fermentable monosaccharides remains a challenging endeavor. In this study, we employed a novel deep eutectic solvent (DES) composed of 1-tetradecyl-3-carboxymethylimidazolium bromide (C14CIMBr) and lactic acid (LA) for the pretreatment of Moringa oleifera Lam. husk (M. oleifera husk), aiming to enhance lignocellulose fractionation. The optimal conditions identified were 165°C, 43.9 minutes, and a molar ratio of C14CIMBr to LA at 1:4.8, resulting in the removal of 93.8% of lignin and 96.8% of hemicellulose. Following enzymatic hydrolysis of the pretreated M. oleifera husk, yields of glucose and xylose reached 94.3% and 86.1%, respectively, representing significant increases by factors of 7.0-fold and 10.3-fold compared to untreated M. oleifera husk. Molecular simulations indicated that the novel DES effectively disrupts the original internal hydrogen bonding network while reconstructing new DES-lignocellulosic hydrogen bonds, it also demonstrates excellent solubilization capabilities for lignin cleavage products. Finally, the yield of regenerated lignin reached 81.3%, exhibiting notable bactericidal activity under blue light irradiation.
将木质纤维素提炼成可发酵单糖仍然是一项具有挑战性的工作。在这项研究中,我们采用了由 1-十四烷基-3-羧甲基溴化咪唑(C14CIMBr)和乳酸(LA)组成的新型深共晶溶剂(DES)来预处理油橄榄树皮(M. oleifera husk),旨在提高木质纤维素的分馏能力。确定的最佳条件是:165°C、43.9 分钟、C14CIMBr 与 LA 的摩尔比为 1:4.8,从而去除 93.8% 的木质素和 96.8% 的半纤维素。经酶水解预处理的油橄榄果壳后,葡萄糖和木糖的产量分别达到 94.3% 和 86.1%,与未经处理的油橄榄果壳相比,分别显著增加了 7.0 倍和 10.3 倍。分子模拟表明,新型 DES 能有效地破坏原有的内部氢键网络,同时重建新的 DES-木质纤维素氢键,它还对木质素裂解产物具有出色的增溶能力。最后,再生木质素的产率达到 81.3%,在蓝光照射下具有显著的杀菌活性。
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引用次数: 0
What affects consumer’s participation in vehicle scrappage programmes? An empirical study on scrapping intentions 是什么影响了消费者参与汽车报废计划?关于报废意向的实证研究
IF 11.1 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Pub Date : 2024-11-18 DOI: 10.1016/j.jclepro.2024.144254
, Sarada Prasad Sarmah, Nikesh Nayak
This study examines consumer intentions toward scrapping End-of-Life vehicles (ELVs) to understand how vehicle scrappage policies might alleviate environmental deterioration caused by emissions from outdated vehicles. The research objective is to assess the factors influencing consumer decisions regarding vehicle scrappage, using a model grounded in the Theory of Planned Behavior (TPB). Data was collected from 403 valid responses and analyzed using exploratory factor analysis, confirmatory factor analysis, and structural equation modeling.The findings reveal that the original TPB model accounts for 58.3% of the variance in consumer intentions to scrap vehicles. However, incorporating sociodemographic variables into the model increases the explained variance to 80.6%, with perceived behavioral control as the most influential factor, followed by consumer attitudes. We found that subjective norms do not influence consumers' intentions to participate in scrappage programs. Younger consumers were more likely to support vehicle scrappage, while environmental concerns alone did not foster a positive attitude toward scrappage.In conclusion, while consumer intentions to scrap vehicles are primarily influenced by control and attitude, targeted interventions are needed to enhance policy adoption. Key managerial implications include: promoting acceptance through tailored advertisements, offering differentiated subsidies, engaging younger audiences through awareness campaigns, and redefining promotional strategies to encourage ELV scrappage effectively.
本研究探讨了消费者对报废报废汽车(ELV)的意向,以了解汽车报废政策可如何缓解过时汽车尾气排放造成的环境恶化。研究的目的是利用基于计划行为理论(TPB)的模型,评估影响消费者决定报废车辆的因素。研究从 403 份有效回复中收集了数据,并使用探索性因素分析、确认性因素分析和结构方程模型对数据进行了分析。研究结果表明,原始 TPB 模型占消费者报废车辆意向变异的 58.3%。然而,将社会人口变量纳入模型后,解释方差增加到了 80.6%,其中感知行为控制是影响最大的因素,其次是消费者态度。我们发现,主观规范并不影响消费者参与报废汽车计划的意愿。总之,虽然消费者报废车辆的意愿主要受控制和态度的影响,但需要采取有针对性的干预措施来促进政策的采纳。主要的管理意义包括:通过量身定制的广告促进消费者的接受度,提供差异化的补贴,通过宣传活动吸引年轻受众,以及重新定义推广策略以有效鼓励电子学习车辆的报废。
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引用次数: 0
Data-driven ship typical operational conditions: a benchmark tool for assessing ship emissions 数据驱动的船舶典型运行条件:评估船舶排放的基准工具
IF 11.1 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Pub Date : 2024-11-17 DOI: 10.1016/j.jclepro.2024.144252
Ailong Fan, Xuelong Fan, Mingyang Zhang, Liu Yang, Yuqi Xiong, Xiao Lang, Chenxing Sheng, Yapeng He
Analysing operational conditions of ships presents a novel approach to assessing emission levels, motivated by the inadequacy of traditional static weighting factors, such as ISO 8178-E3 cycle, to capture the dynamic and complex operating characteristics of ships at sea. This study introduces a data-driven method to construct and validate ship typical operational conditions. The method encompasses identifying ship motion states, extracting features, compressing time series data based on these features, and performing cluster analysis. It has been applied to process over 12.6 million data points, demonstrating its applicability to a large dataset. The results indicate that by using actual measurement data and the proposed methodology, three typical operational conditions for ships were successfully established. There are significant differences in the feature parameters among these conditions, highlighting the distinct characteristics of each operational state. The validity of the constructed typical operational conditions was confirmed through a validation process, which involved analysing the differences in feature parameters and comparing the probability distributions of speed and acceleration to the overall dataset. Additionally, energy consumption and emission levels calculated using the typical conditions were validated through comparison with real-world data from upstream and downstream voyages. This study providing a novel tool for assessing emissions in the maritime industry.
由于传统的静态加权因子(如 ISO 8178-E3 周期)不足以捕捉船舶在海上动态和复杂的运行特征,因此对船舶运行条件进行分析是评估排放水平的一种新方法。本研究介绍了一种数据驱动方法,用于构建和验证船舶典型运行条件。该方法包括识别船舶运动状态、提取特征、根据这些特征压缩时间序列数据并进行聚类分析。该方法已用于处理超过 1260 万个数据点,证明了其对大型数据集的适用性。结果表明,通过使用实际测量数据和建议的方法,成功建立了三种典型的船舶运行条件。这些工况的特征参数存在明显差异,凸显了每种运行状态的不同特点。构建的典型运行状态的有效性通过验证过程得到了确认,验证过程包括分析特征参数的差异,并将速度和加速度的概率分布与整个数据集进行比较。此外,通过与上游和下游航程的实际数据进行比较,还验证了使用典型工况计算出的能耗和排放水平。这项研究为评估海运业的排放提供了一种新工具。
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引用次数: 0
The cost of sustainability in the construction sector – the case of family houses in Belgium 建筑行业可持续性的成本--以比利时家庭住宅为例
IF 11.1 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Pub Date : 2024-11-17 DOI: 10.1016/j.jclepro.2024.144240
J. Douhard, B. Van Pottelsberghe de la Potterie
The housing sector is a major contributor to greenhouse gas emissions and a large body of literature has focused on measuring the environmental impact of houses, using the Life Cycle Assessment (LCA) methodology. This literature reaches the conclusion that alternative construction materials should be used to reduce the environmental impact of buildings. While such research provides essential knowledge on the carbon footprint of the housing sector, few studies take into account the economic side of the issue. This paper addresses this gap by calculating the Life Cycle Cost (LCC) of houses and matching the results with the LCA stages. The methodology is developed for two reference houses in Belgium. Considering all elements and materials used in the construction process, this approach allows a comparison of each house’s elements based on the required investment to abate their carbon footprint. The most striking results are that (1) the operational stage (i.e., the use of houses) accounts for about 65% of the total carbon impact of a house; (2) a 1€ investment in sustainable materials induces a drop of 1 to 1.3 kgCO2eq; (3) this effect is heterogeneous across materials, with the highest returns obtained for external walls (-6 KgCO2eq) and windows (-3 to -6 kgCO2eq) and the lowest returns obtained for ground floor (-0.3 kgCO2eq).
住房部门是温室气体排放的主要贡献者,大量文献都集中在使用生命周期评估(LCA)方法来衡量住房对环境的影响。这些文献得出的结论是,应使用替代建筑材料来减少建筑物对环境的影响。虽然这些研究提供了有关住房领域碳足迹的基本知识,但很少有研究考虑到这一问题的经济方面。本文通过计算房屋的生命周期成本 (LCC),并将结果与生命周期评估阶段相匹配,填补了这一空白。该方法是针对比利时的两栋参考房屋开发的。考虑到建造过程中使用的所有元素和材料,这种方法可以根据减少碳足迹所需的投资对每栋房屋的元素进行比较。最显著的结果是:(1) 运行阶段(即房屋的使用)约占房屋总碳影响的 65%;(2) 在可持续材料上投资 1 欧元可减少 1 至 1.3 千克 CO2eq;(3) 不同材料的效果不同,外墙(-6 千克 CO2eq)和窗户(-3 至-6 千克 CO2eq)的回报率最高,底层(-0.3 千克 CO2eq)的回报率最低。
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引用次数: 0
Education for Sustainable Development (ESD) through Participatory Research (PR): A systematic review 通过参与式研究(PR)开展可持续发展教育(ESD):系统回顾
IF 11.1 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Pub Date : 2024-11-17 DOI: 10.1016/j.jclepro.2024.144237
Alexa Ray R. Fernando, Gizelle P. Tajan
With less than a decade left to achieve the SDGs, developing human capacity and promoting transformative learning is crucial to encourage as many people as possible to become agents of change toward achieving these goals. The literature suggests that Participatory Research (PR)—a host of methods, designs, and collaborative frameworks—has the potential to facilitate inclusive, participatory, and bottom-up approaches to knowledge co-generation and transformative learning in various communities. Using a systematic review approach, this study explored the use of PR in ESD in the recent global literature on education. PR’s efficacy as a participatory tool for ESD among collegiate and adult learners was analyzed. PR’s use and effectiveness in ESD to various stakeholders were also examined. The reviewed studies emphasized the potential of PR in promoting inclusive and participatory approaches to transformative learning and knowledge co-generation among many stakeholders. It highlights the need for academic institutions to adopt participatory and collaborative research methods to enhance their contributions towards achieving the SDGs through ESD. Furthermore, the study investigated how ESD through PR enables individuals to become active social agents and decision-makers in the quest for transformative change and sustainable development. Implications to curriculum and pedagogy enhancement and future directions for using PR in ESD were also presented.
距离实现可持续发展目标只剩下不到十年的时间,发展人的能力和促进变革性学习对于鼓励尽可能多的人成为实现这些目标的变革推动者至关重要。文献表明,参与式研究(PR)--一系列方法、设计和合作框架--具有促进包容性、参与性和自下而上的方法的潜力,从而在各个社区实现知识的共同生成和变革性学习。本研究采用系统回顾的方法,探讨了近期全球教育文献中可持续发展教育中公关的使用情况。分析了公关作为可持续发展教育的参与式工具在大学生和成人学习者中的有效性。还研究了可持续发展教育中公共关系对各相关方的使用情况和效果。所审查的研究强调了公共关系在促进包容性和参与性方法方面的潜力,以在许多有关各 方之间促进变革性学习和知识的共同生成。研究强调,学术机构需要采用参与性和合作性研究方法,通过可持续发展教育为实现可 持续发展目标做出更大贡献。此外,研究还探讨了可持续发展教育如何通过公共关系使个人成为积极的社会行动者和决策者,以寻求变革和可持续发展。还介绍了课程和教学法改进的意义以及在可持续发展教育中使用公关的未来方向。
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引用次数: 0
Corrigendum to “Circular economy in action: Transforming textile waste into sustainable soil additives - Physicochemical properties and biodegradability” [J. Clean. Prod. 480 (2024) 144093] 循环经济在行动:将纺织废物转化为可持续的土壤添加剂--物理化学特性和生物降解性"[J. Clean. Prod.
IF 11.1 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Pub Date : 2024-11-17 DOI: 10.1016/j.jclepro.2024.144216
Daria Marczak, Krzysztof Lejcuś, Joanna Grzybowska-Pietras, Włodzimierz Biniaś, Ahmed Tamma
No Abstract
无摘要
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引用次数: 0
Performance of surfactant supplementation on alleviating membrane fouling in treatment of waste activated sludge: Experimental and modeling analyses 在处理废弃活性污泥时补充表面活性剂对减轻膜堵塞的作用:实验和模型分析
IF 11.1 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Pub Date : 2024-11-17 DOI: 10.1016/j.jclepro.2024.144248
Mohsen Taghavijeloudar, Bahman Nazari, Mahdokht Safaei
In this research, surfactant supplementation was investigated as a novel strategy for alleviation of membrane fouling in waste activated sludge (WAS) membrane filtration process. The effect of WAS pre-treatment with different surfactants on membrane performance were investigated in terms of flux variation, membrane rejection and fouling mechanisms. A generalization form of blocking law was developed to determine membrane fouling mechanism. According to the results, cationic surfactant below critical micelle concentration (CMC) values improved membrane performance, while anionic and non-ionic surfactant showed a negative impact at all dosages. It was observed that WAS pretreatment with 300 mg/L Cetyltrimethylammonium bromide (CTAB) could increase the water flux from 195 to 611 L/m2/h (LMH) and decrease the rejection rate from 93% to 85%, respectively. Although CTAB addition increased the total extracellular polymeric substances (EPSs) amount from 56.16 to 119.6 mg/L which was due to the surfactant solubilization property, the total resistance decreased from 0.33×1010 to 0.11×1010 m-1. This was attributed to the flock formation induced by CTAB through charge neutralization and bridging mechanism. Modeling simulation of the results indicated that CTAB addition transformed fouling mechanism from cake to intermediate-blocking model. The environmental risk assessment revealed that only 0.3 mg/L surfactant penetrated in permeate which was low ecological risk (risk quotients (RQ) < 0.5) to the aquatic environment. Our finding suggested CTAB treatment at low dosage (0.1 g/L) as a promising and efficient approach for fouling mitigation and improving membrane process for wastewater treatment.
在这项研究中,研究人员将表面活性剂作为一种新型策略,用于减轻废弃活性污泥(WAS)膜过滤过程中的膜污垢。从通量变化、膜排斥和污垢机理等方面研究了使用不同表面活性剂预处理 WAS 对膜性能的影响。为确定膜堵塞机理,建立了堵塞定律的一般化形式。结果表明,低于临界胶束浓度(CMC)值的阳离子表面活性剂可改善膜性能,而阴离子和非离子表面活性剂在所有用量下都会产生负面影响。观察发现,用 300 毫克/升十六烷基三甲基溴化铵(CTAB)预处理 WAS,可将水通量从 195 升/平方米/小时(LMH)提高到 611 升/平方米/小时(LMH),并将排斥率从 93% 降低到 85%。虽然由于表面活性剂的增溶特性,CTAB 使细胞外高分子物质(EPSs)总量从 56.16 mg/L 增加到 119.6 mg/L,但总阻力却从 0.33×1010 m-1 下降到 0.11×1010 m-1。这归因于 CTAB 通过电荷中和和架桥机制诱导形成的絮状物。模型模拟结果表明,CTAB 的加入使污垢机理从滤饼模式转变为中间阻塞模式。环境风险评估显示,渗透液中表面活性剂的渗透量仅为 0.3 mg/L,对水环境的生态风险较低(风险商数为 0.5)。我们的研究结果表明,低剂量(0.1 g/L)CTAB 处理是缓解污垢和改进废水处理膜过程的一种有效方法。
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引用次数: 0
期刊
Journal of Cleaner Production
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