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Ultrafast control of exciton dynamics by optically-induced thermionic carrier injection in a metal-semiconductor heterojunction 金属半导体异质结中光诱导热离子载流子注入对激子动力学的超快控制
Pub Date : 2023-06-09 DOI: 10.1117/12.2665677
K. Keller, R. Rojas-Aedo, Huiqin Zhang, P. Schweizer, J. Allerbeck, D. Brida, D. Jariwala, N. Maccaferri
Interface effects in metals-semiconductors heterojunctions are subject of intense research due to the possibility to exploit the synergy between their electronic and optical properties in next-generation opto-electronic devices. In this framework, understanding the carrier dynamics at the metal-semiconductor interface, as well as achieving a coherent control of charge and energy transfer in metal-semiconductor heterostructures, are crucial and yet quite unexplored aspects. Here, we experimentally show that thermionically injected carriers from a gold substrate can drastically affect the dynamics of excited carriers in bulk WS2. By employing a pump-push-probe scheme, where a push pulse excites direct transitions in the WS2, and another delayed pump pulse induces thermionic injection of carriers from the gold substrate into the semiconductor, we can control both the formation and annihilation of excitons. Our findings might foster the development of novel opto-electronic approaches to control charge dynamics using light at ultrafast timescales.
金属-半导体异质结中的界面效应是研究的热点,因为在下一代光电器件中有可能利用其电子和光学特性之间的协同作用。在这个框架中,理解金属-半导体界面的载流子动力学,以及实现金属-半导体异质结构中电荷和能量转移的相干控制,是至关重要的,但尚未被探索的方面。在这里,我们实验表明,从金衬底热注入载流子可以极大地影响体WS2中激发载流子的动力学。通过采用泵浦-推-探方案,其中一个推脉冲激发WS2中的直接跃迁,另一个延迟泵浦脉冲诱导载流子从金衬底注入半导体,我们可以控制激子的形成和湮灭。我们的发现可能会促进利用超快时间尺度的光来控制电荷动力学的新型光电方法的发展。
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引用次数: 0
Design of a compact time-delay-compensated monochromator for femtosecond pulses in the extreme-ultraviolet 用于极紫外飞秒脉冲的紧凑型延时补偿单色仪的设计
Pub Date : 2023-06-09 DOI: 10.1117/12.2665826
F. Frassetto, L. Poletto
Table-top beamlines based on high-order laser harmonics (HHs) are nowadays lab-based facilities commonly used both for ultrafast experiments on its own sake and in preparatory experiments conceived, ab initio, for large-scale facilities such as FELs. Differently from FELs, HHs are emitted in a broad spectral range, requiring for most experiments the selection of a single harmonic. The monochromatization should preserve the temporal structure of the femtosecond pulse in a so-called time-delay-compensated monochromator (TDCM), where a couple of gratings is used in a configuration to compensate for the pulse-front tilt. At present, TDCMs in the extreme ultraviolet (15–100 eV) are realized using six optics at grazing incidence: two plane gratings and four toroidal mirrors. The gratings are illuminated by a collimated beam and the mirrors are used to collimate and focus the beam in the two sections of the monochromator: intermediate slit and target area. Here we present the design of a TDCM with four optical elements: two gratings, a cylindrical(spherical) mirror and a toroidal mirror. The gratings are used in the off-plane geometry and are illuminated by a divergent beam. The optical design is discussed in detail giving all the parameters for the definition of the configuration. We present the design of a TDCM for the 15-60 eV region, being a physical realization in progress. The main topics discussed are the beam size at the target area, the residual temporal broadening, the error budget for the alignment and the expected throughput. The design has advantages in terms of costs, compactness, alignment stability and throughput.
基于高阶激光谐波(HHs)的桌面光束线目前是基于实验室的设施,通常用于超快实验本身,也用于为大型设施(如FELs)从头开始构思的预备实验。与fel不同的是,HHs的发射光谱范围很宽,因此大多数实验都需要选择单一谐波。在所谓的延迟补偿单色器(TDCM)中,单色化应保留飞秒脉冲的时间结构,其中一对光栅用于补偿脉冲前倾斜的配置。目前,在极紫外波段(15-100 eV), TDCMs采用6种掠射光学器件:2个平面光栅和4个环面反射镜实现。光栅由准直光束照射,反射镜用于准直和聚焦单色器的两个部分:中间狭缝和目标区域。在这里,我们提出了一种具有四个光学元件的TDCM的设计:两个光栅,一个圆柱(球面)反射镜和一个环面反射镜。光栅用于离平面几何,并由发散光束照射。详细讨论了光学设计,给出了定义结构的所有参数。我们提出了一个用于15-60 eV区域的TDCM的设计,是一个正在进行的物理实现。主要讨论了目标区域的波束尺寸、剩余时间展宽、对准误差预算和期望吞吐量。该设计在成本、紧凑性、对准稳定性和吞吐量方面具有优势。
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引用次数: 0
Electron injection on steep ramp-up plasma density profiles in high repetition rate laser-plasma wake-field accelerators 高重复率激光等离子体尾迹场加速器中陡坡上升等离子体密度曲线的电子注入
Pub Date : 2023-06-09 DOI: 10.1117/12.2660115
V. Petržílka, P. Gajdos, M. Krus
Electron acceleration by laser pulses with high repetition rate can be used for technical applications. To reach conditions for the wake-field laser acceleration, it was demonstrated recently in experiments that it is beneficial to use near single cycle laser drive pulses with sub-4 fs duration, with narrow waists. To explore possible electron density ramp-up injection as an alternative to ramp-down and ionization injections, we performed numerical simulations of electron bunches generation in the ramp-up region. The PIC code Epoch2D and input parameters near to experiments were used. We assumed thin plasma slabs with super Gaussian density profiles of order 4-80, FWHM about 30 µm. We found that density ramp-up injected bunches can have charges several times higher than those obtained by ionization injection. There can be created a group of up to ten bunches in a sequence of bubbles, with not too mutually different maximum energy and charges. At oblique incidence of drive pulses on steep ramp up profiles, we find significant enhancement of the first bunch charge. For large slant angles -45 or 45 degrees, the bunch charge enhancement is about twenty times. We conclude that the ramp-up injection can be a useful alternative injection on steep enough density profiles.
高重复频率激光脉冲的电子加速可以用于技术应用。为了达到尾流场激光加速的条件,最近的实验证明,使用持续时间小于4秒的窄束近单周期激光驱动脉冲是有益的。为了探索可能的电子密度上升注入作为斜坡下降和电离注入的替代方案,我们在斜坡区域进行了电子束产生的数值模拟。采用PIC代码Epoch2D,输入参数接近实验值。我们假设薄等离子体板的超高斯密度分布为4-80阶,FWHM约为30µm。我们发现密度增加注入的束比电离注入获得的束具有高几倍的电荷。在一系列气泡中可以产生一组多达10束的气泡,它们的最大能量和电荷不会太大不同。当驱动脉冲斜入射在陡坡上时,我们发现第一束电荷显著增强。对于大倾角-45度或45度,束荷增强约为20倍。我们得出结论,在足够陡峭的密度剖面上,升压注入是一种有用的替代注入方法。
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引用次数: 0
Optimization of PMP films’ production and mechanical properties based on ZnO nanoparticles addition ZnO纳米颗粒对PMP薄膜制备及力学性能的优化
Pub Date : 2023-06-09 DOI: 10.1117/12.2665616
Amalia D'Avino, D. Sagnelli, A. Vestri, M. Rippa, V. Marchesano, V. Ambrogi, Anna De Girolamo, F. Loffredo, F. Villani, G. Nenna, L. Petti
In the last decade, smart materials have been developed in the fields of optical machines, sensors, motors, robots, and energy harvesting. This is due to their capability to respond to external stimuli or environmental changes. Among smart materials, photo-mobile polymers (PMPs) based on liquid crystals are the most promising in the field of photo-responsive actuators. These polymers are made with a mixture of liquid crystals containing azobenzene moieties that can undergo photoisomerization from trans to cis under UV light. This process leads to a macroscopic bending of the PMPs, which transforms light into mechanical energy. To enhance the PMPs' actuation, a novel liquid crystal nanocomposite is proposed. In our work, the nanocomposites are prepared with different concentrations of ZnO nanoparticles (NPs) embedded in the cross-linked polymer matrix. We have demonstrated that ZnO NPs improve the actuation and mechanical properties of the PMP, and the main aim of this assay is to optimize such effect as a function of the nanoparticles concentration. We also show the lowest and highest amounts of ZnO needed to enhance the bending behavior of the PMP. Optical, mechanical, and thermal analyses were performed to characterize the PMPs. Spectral characterization in UV/vis range of the bare and doped films, optical and atomic force microscopy, were used to comprehend the role of ZnO nanoparticles and their distribution among the liquid crystals. To study the dynamic response of the PMPs and their mechanical properties, lasers at different wavelengths were used.
在过去的十年中,智能材料在光学机器、传感器、电机、机器人和能量收集领域得到了发展。这是由于它们对外部刺激或环境变化的反应能力。在智能材料中,基于液晶的光移动聚合物(pmp)是光响应致动器领域中最有前途的材料。这些聚合物是由含有偶氮苯基团的液晶混合物制成的,这些液晶可以在紫外线下从反式到顺式进行光异构化。这个过程导致pmp的宏观弯曲,将光转化为机械能。为了提高pmp的驱动性能,提出了一种新型的液晶纳米复合材料。在我们的工作中,将不同浓度的ZnO纳米粒子(NPs)嵌入交联聚合物基体中制备了纳米复合材料。我们已经证明ZnO纳米粒子改善了PMP的驱动和力学性能,本实验的主要目的是优化纳米粒子浓度对PMP的影响。我们还显示了提高PMP弯曲性能所需的最低和最高氧化锌量。进行了光学、机械和热分析来表征pmp。利用光学显微镜和原子力显微镜对裸膜和掺杂膜的紫外/可见光谱进行了表征,以了解ZnO纳米颗粒在液晶中的作用及其分布。为了研究pmp的动态响应和力学性能,使用了不同波长的激光。
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引用次数: 0
Transition of electron beams between vacuum and plasma in the external injection into a laser wakefield accelerator 激光尾场加速器外注入过程中电子束在真空和等离子体间的跃迁
Pub Date : 2023-06-09 DOI: 10.1117/12.2665683
David Gregocki, Dominika Mašlárová, M. Krůs
Laser wakefield acceleration is a remarkably efficient method for relativistic electron acceleration that ensures high electric field gradients generated by plasma waves. In this approach, an ultra-short, high-intensity laser pulse propagates through a plasma medium. It has already proven its potential by reaching gradients up to hundreds of GV/m. To further stabilize and control the process of acceleration, a separate source of electrons is widely considered. In order to address this problem, we have performed 3D particle-in-cell simulations using the Smilei code. Several plasma density profiles with different vacuum-plasma transition region and their effect on the external injection were analysed.
激光尾场加速是一种非常有效的相对论性电子加速方法,可以保证等离子体波产生的高电场梯度。在这种方法中,超短、高强度激光脉冲通过等离子体介质传播。它已经通过达到数百GV/m的梯度证明了它的潜力。为了进一步稳定和控制加速过程,人们普遍考虑使用单独的电子源。为了解决这个问题,我们使用Smilei代码进行了三维细胞内粒子模拟。分析了不同真空等离子体过渡区的几种等离子体密度分布及其对外部注入的影响。
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引用次数: 0
Effect of cryogenic temperature on spectroscopic and laser properties of Tm:SrF2 crystal 低温对Tm:SrF2晶体光谱和激光性能的影响
Pub Date : 2023-06-09 DOI: 10.1117/12.2665636
Karel Veselský, M. Jelínek, V. Kubecek, J. Šulc, H. Jelínková, Yangxiao Wang, Zhonghan Zhang, L. Su
We present a temperature influence (in range from 78 up to 300 K) on the spectroscopic and laser properties of Tm:SrF2 crystal doped with 2 at. % of Tm3+. The sample was grown using the temperature gradient technique in shape of a single-crystal fiber (d= 2 mm, l = 5 mm) with plane-parallel face-polished without any AR coating. The Tm:SrF2 crystal was mounted in a temperature-controlled copper holder of the liquid nitrogen cryostat. The measured absorption and emission spectra remained broad even at low temperature. The fluorescence lifetime was fitted with a double exponential function, and the measured lifetime changed significantly with temperature decrease. The 147 mm long semi-hemispherical laser resonator consisted of a flat pumping mirror (T < 95 % @ 763 nm, HR @ 1750-2100 nm) placed inside the cryostat and a curved output coupler (r=150 mm, R=97.5 % @ 1750-2100 nm) placed outside the cryostat. For longitudinal pumping, a fiber coupled laser diode was used. The diode was operating in the pulse regime (5 ms pulse length, 10 Hz repetition rate) at wavelength 763 nm. At room temperature, the laser emission was achieved at 1949 nm with a high 38 % slope efficiency. With a temperature decrease, the slope efficiency increased, and the laser threshold decreased, and the laser output wavelength shifted.
我们研究了温度对掺杂2at的Tm:SrF2晶体的光谱和激光特性的影响(范围从78到300 K)。% Tm3+。样品采用温度梯度法生长成单晶纤维形状(d= 2 mm, l = 5 mm),并在无AR涂层的情况下进行平面平行表面抛光。将Tm:SrF2晶体安装在液氮低温恒温器的温控铜支架中。测得的吸收和发射光谱即使在低温下也保持宽广。荧光寿命符合双指数函数,随温度的降低,荧光寿命变化显著。147mm长的半球形激光谐振器由放置在低温恒温器内部的平面泵浦反射镜(T < 95% @ 763 nm, HR @ 1750-2100 nm)和放置在低温恒温器外部的弯曲输出耦合器(r=150 mm, r= 97.5% @ 1750-2100 nm)组成。纵向泵浦采用光纤耦合激光二极管。二极管在763 nm波长的脉冲状态下工作(5 ms脉冲长度,10 Hz重复率)。在室温下,激光发射波长为1949 nm,斜率效率高达38%。随着温度的降低,斜率效率增加,激光阈值降低,激光输出波长发生偏移。
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引用次数: 0
Exposed interfaces and fast mixing in XFEL-friendly liquid sheets 暴露的界面和快速混合在xfl友好的液体片
Pub Date : 2023-06-09 DOI: 10.1117/12.2669141
David J. Hoffman, H. Bechtel, Diego A. Huyke, J. Santiago, D. DePonte, J. Koralek
Microfluidic liquid sheet jets have rapidly grown in popularity for extreme ultraviolet and soft x-ray spectroscopies as they are vacuum stable, constantly refreshing, and are easily able to reach sub-micron optical path lengths required for transmission measurements. We have recently demonstrated the generation of a new class of sheet jet comprised of two liquids (a “liquid heterostructure”) by colliding two jets of one liquid onto opposite sides of third jet of another liquid. The resulting structure is a layered sheet jet where a thin sheet of one liquid is completely enveloped by a larger sheet of a separate liquid. If the component liquids are miscible, the thin component layers result in fast diffusive mixing on submillisecond time scales based on measurements using FTIR microscopy. If the component liquids are immiscible, the resulting structure contains well-defined, large-area liquid-liquid interfaces with a minimized bulk liquid background as determined from ellipsometry and FTIR microscopy measurements. The inner liquid layer in these structures was found to be as thin as tens of nanometers, comparable to the thinnest sheet jets that can be produced. These new heterostructures provide the same benefits as conventional sheet jets for XUV and SXR spectroscopy and could enable new mix-and-probe spectroscopic techniques or support developing methods such as XUV/SXR second harmonic generation for examining buried liquid interfaces.
微流控液片射流在极紫外和软x射线光谱中迅速普及,因为它们是真空稳定的,不断刷新,并且很容易达到传输测量所需的亚微米光程长度。我们最近演示了一种新型的由两种液体组成的片状射流(一种“液体异质结构”),通过将一种液体的两股射流碰撞到另一种液体的第三股射流的相对两侧。由此产生的结构是层状片状射流,其中一种液体的薄板完全被另一种较大的单独液体的薄板包裹。如果组分液体是可混溶的,那么薄的组分层会导致在亚毫秒时间尺度上的快速扩散混合。如果组成液体是不混溶的,则所得结构包含定义良好的大面积液-液界面,并具有最小的体积液体背景,这是由椭偏仪和FTIR显微镜测量确定的。这些结构的内部液体层被发现只有几十纳米薄,与可以生产的最薄的薄片射流相当。这些新的异质结构为XUV和SXR光谱提供了与传统片状射流相同的好处,可以实现新的混合-探针光谱技术,或支持开发用于检测埋藏液体界面的XUV/SXR二次谐波产生等方法。
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引用次数: 0
Relativistic electron acceleration from nanotips 纳米尖端的相对论性电子加速
Pub Date : 2023-06-09 DOI: 10.1117/12.2669592
L. Veisz, A. de Andres, S. Bhadoria, A. Gonoskov, M. Marklund, T. Blackburn, J. Marmolejo, D. Hanstorp
Vacuum laser acceleration (VLA) of electrons has been an intense field of research for a long time due to the extremely high (>1 TV/m) accelerating fields. However, it is very challenging to realize and only a few promising experiments have been performed which have demonstrated the principle. Here, we report on the interaction of relativistic intensity (1020 Wcm-2) sub-two optical cycle (<5 fs) laser pulses with nanotips to realize and optimize VLA. Various properties of accelerated electrons (angular distribution, charge, and electron spectrum) are measured with different intensities and carrier envelope phases of the laser pulse. Among others, waveform dependence of the electron propagation direction is observed. Furthermore, comparable or even higher electron energies beyond 10 MeV are detected with lower laser intensity, i.e., longer focusing, than with high intensity. These surprising results are reproduced using particle-in-cell simulations, which indicate a nanophotonics electron emission from the nanotip followed by VLA. In fact, the unexpected observations are a direct proof of the VLA process and provide a way to optimize it towards higher energy, isolated, attosecond electron bunch generation.
电子的真空激光加速(VLA)由于具有极高的加速场(>1 TV/m)而长期以来一直是研究的热点。然而,实现起来非常困难,只有少数有希望的实验证明了这一原理。本文报道了相对论强度(1020 Wcm-2)亚二光周期(<5 fs)激光脉冲与纳米尖端的相互作用,以实现和优化VLA。用激光脉冲的不同强度和载流子包络相位测量了加速电子的各种特性(角分布、电荷和电子能谱)。其中,观察到电子传播方向的波形依赖性。此外,在较低的激光强度下,即比高强度下聚焦时间更长,可以检测到相当甚至更高的电子能量,超过10 MeV。这些令人惊讶的结果通过细胞内粒子模拟重现,这表明纳米尖端的纳米光子电子发射紧随其后的是VLA。事实上,这些意想不到的观测结果是VLA过程的直接证明,并提供了一种优化它的方法,使其朝着更高能量、隔离、阿秒电子束的方向发展。
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引用次数: 0
Numerical simulation studies of superconducting afterburner operation at SASE2 beamline of European XFEL 欧洲自由电子激光器SASE2束流超导加力燃烧室运行的数值模拟研究
Pub Date : 2023-06-09 DOI: 10.1117/12.2669177
C. Lechner, S. Casalbuoni, G. Geloni, E. Schneidmiller, S. Serkez, H. Sinn
European XFEL is a multi-beamline x-ray free-electron laser (FEL) user facility driven by a superconducting accelerator with a nominal photon energy range from 250 eV to 25 keV. To extend the photon range towards harder x-rays, an afterburner undulator based on superconducting undulator (SCU) technology is currently being planned. This afterburner undulator would be installed at the end of the already operating SASE2 hard x-ray FEL beamline. The electron bunch is microbunched by the FEL process in the SASE2 undulators and in the SCUs drives emission either at the same wavelength or at a harmonic of the upstream SASE2 undulator. In this contribution we describe numerical simulations of the potential photon output.
欧洲XFEL是由超导加速器驱动的多束线x射线自由电子激光器(FEL)用户设备,标称光子能量范围为250 eV至25 keV。为了将光子范围扩展到更硬的x射线,目前正在计划一种基于超导波动器(SCU)技术的加力燃烧器波动器。这个加力燃烧器波动器将安装在已经运行的SASE2硬x射线FEL光束线的末端。电子束通过FEL过程在SASE2波动器中微束化,在scu中驱动在相同波长或在上游SASE2波动器的谐波上发射。在这篇文章中,我们描述了潜在光子输出的数值模拟。
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引用次数: 1
ZnO nanorods as a piezoelectric energy harvester from light induced flexions ZnO纳米棒作为光致弯曲的压电能量收集器
Pub Date : 2023-06-09 DOI: 10.1117/12.2665540
M. Haras, M. Wlazło, W. Andrysiewicz, T. Skotnicki
Rapid growth is promoting the Internet of Things (IoT) to become one of the main branches of the semiconductor industry. Surprisingly, the IoT growth would have been even faster if economically attractive and reliable alternatives for batteries and wires had been available. Providing power supply to the IoT nodes is challenging regarding their: (i) quantity (close to 8x the human population), (ii) harsh operation environments, (iii) size (typical footprint much smaller than mm2) and (iv) hard-to-reach locations. Modern IoT node requires very small energy (less than 100μJ/cycle) to operate. Wire supply of energy is expensive and uncomfortable while using a battery requires periodic replacements/maintenance and produces tons of toxic waste. Energy Harvesting (EH) could be a solution to overcome the IoT supply difficulties offering self-supplied nodes enabling further IoT market growth. EH converts natural or waste energies (vibrations, heat losses, light, etc.) into useful energy. We present an innovative two-step conversion harvester capable of transforming light into electricity via the PieZoelectric (PZ) effect. Our approach uses a Photo- Mobile Polymer (PMP) integrated with the PZ material. PMP serves as light-to-movement transducer and PZ converts the light-induced PMP flexions into voltage. As a PZ material, a nanostructured ZnO nanorods were used as their fabrication is cheap and ready-to-use at industrial scale. ZnO performance characterization in a dedicated flexions simulator revealed energy as high as 80nJ during 55sec bending runs. This result encourages further PMP and ZnO optimization enabling extension of piezoelectrics onto light conversion.
快速增长正在推动物联网(IoT)成为半导体产业的主要分支之一。令人惊讶的是,如果有经济上有吸引力和可靠的电池和电线替代品,物联网的增长将会更快。为物联网节点提供电源具有挑战性,因为它们:(i)数量(接近人口的8倍),(ii)恶劣的操作环境,(iii)尺寸(典型占地面积远小于mm2)和(iv)难以到达的位置。现代物联网节点运行所需能量非常小(小于100μJ/cycle)。电线供电既昂贵又不舒服,而使用电池需要定期更换/维护,并产生大量有毒废物。能量收集(EH)可能是克服物联网供应困难的一种解决方案,提供自给自足的节点,使物联网市场进一步增长。EH将自然或废弃的能量(振动、热损失、光等)转化为有用的能量。我们提出了一种创新的两步转换收割机,能够通过压电(PZ)效应将光转化为电。我们的方法使用了与PZ材料集成的光移动聚合物(PMP)。PMP作为光到运动的传感器,PZ将光诱导的PMP弯曲转换为电压。作为PZ材料,纳米结构的ZnO纳米棒由于其制造成本低且可用于工业规模而被使用。在专用弯曲模拟器中对ZnO的性能进行了表征,结果表明,在55秒的弯曲过程中,ZnO的能量高达80nJ。这一结果鼓励进一步优化PMP和ZnO,使压电扩展到光转换。
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引用次数: 1
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Optics + Optoelectronics
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