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Generation and measurement of ultrashort free electron laser pulses in ultraviolet and soft-x-ray spectral regions 紫外和软x射线光谱区超短自由电子激光脉冲的产生和测量
Pub Date : 2023-06-09 DOI: 10.1117/12.2665832
N. Mirian
Over the last few years, tremendous progress has been gained in the generation and application of ultrashort radiation pulses. Recently, free-electron lasers generating ultrashort pulses with high peak power from the extreme ultraviolet (EUV) to the soft-x-ray region are opening a wide range of new scientific opportunities. Taking advantage of this short timescale permits probing ultrafast, out-of-equilibrium dynamics and the high intensities are key for nonlinear optics. The core structure of the extremely important light elements carbon, nitrogen, and oxygen can be accessed by soft-x-ray wavelengths by providing chemical sensitivity. Externally seeded free-electron lasers generate coherent pulses with the ability to be synchronized with femtosecond accuracy. In this contribution, we present new achievements in the generation of coherent ultrashort pulses in the range of EUV to the soft-x-ray in externally seeded FELs. In particular, we present the recently successful robust experiment at FERMI in Trieste, where few-femtosecond extreme-ultraviolet pulses were generated and characterized in terms of energy, and duration via autocorrelation.
近年来,超短辐射脉冲的产生和应用取得了巨大的进展。近年来,从极紫外光(EUV)到软x射线区域产生峰值功率高的超短脉冲的自由电子激光器正在开辟广泛的新的科学机会。利用这种短时间尺度可以探测超快,非平衡动力学和高强度是非线性光学的关键。极其重要的轻元素碳、氮和氧的核心结构可以通过提供化学灵敏度的软x射线波长获得。外部播种的自由电子激光器产生具有飞秒精度同步能力的相干脉冲。在这篇贡献中,我们介绍了在外部种子加速器中产生EUV到软x射线范围内的相干超短脉冲的新成就。特别地,我们介绍了最近在里雅斯特费米成功的鲁棒实验,在那里产生了几飞秒极紫外脉冲,并通过自相关在能量和持续时间方面进行了表征。
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引用次数: 0
Influence of crystal orientation on Ho:YAP microchip laser generation 晶体取向对Ho:YAP微芯片激光产生的影响
Pub Date : 2023-06-09 DOI: 10.1117/12.2665634
J. Šulc, M. Jelínek, M. Němec, H. Jelínková, K. Nejezchleb, S. Uxa
The goal of this work was an investigation of Ho:YAP (Ho:YAlO3) crystal as an active medium of resonantly longitudinally pumped multi-watt microchip laser operating at 2.1 ¹m spectral region. Three Ho:YAP crystals,a"-cut, b"-cut, and c"-cut Pbnm, with the same dimensions (7mm long, 3mm in diameter) and Ho-doping concentration (1.06 at.% Ho/Y) were compared. Resonator mirrors were deposited directly on the crystals faces. The output coupler transmission for desired laser emission wavelength range 2.1 µm was 11% and T = 3% @ 1.94 µm. The pumping mirror was highly reflecting at 2.1 µm and T = 89% @ 1.94 µm. Samples were fixed in air-cooled Cu-heatsink and longitudinally pumped by a CW Tm-fibre laser with the maximum output power amplitude of 12W @ 1939.2nm behind a focusing lens (f = 200 mm). The laser output power, emission wavelength, and output beam profile were measured in respect to incident pumping power. All three lasers had similar input-output power characteristics with the laser threshold close to 1.5W and slope efficiencies reaching quantum limit in respect to the incident pumping power. The best result (slope efficiency 79 %, laser threshold 1.54W, max output power 8.2W in an almost diffraction-limited, linearly polarized beam) was reached for microchip laser using b"-cut Ho:YAP crystal. Laser emission wavelength was 2119nm for a"-cut and b"-cut Ho:YAP and 2132nm for c"-cut Ho:YAP-based microchip laser. The designed lasers can serve as compact wavelength converters for laser radiation and could be used to expand capabilities of current Tm-fibre lasers used in medicine and industry preserving the overall system efficiency.
本文的目的是研究Ho:YAP (Ho:YAlO3)晶体作为2.1¹m光谱区共振纵向泵浦多瓦微芯片激光器的有效介质。三颗Ho:YAP晶体,分别为“-”型、“b”型和“c”型pnm,具有相同的尺寸(长7mm,直径3mm)和Ho掺杂浓度(1.06 at。% Ho/Y)进行比较。谐振镜直接沉积在晶体表面。在2.1µm波长范围内,输出耦合器的透射率为11%,T = 3% @ 1.94µm。泵送镜在2.1µm和T = 89% @ 1.94µm处具有高反射率。样品被固定在空气冷却的cu散热器中,在聚焦透镜(f = 200 mm)后,用最大输出功率幅值为12W @ 1939.2nm的连续tm光纤激光器纵向泵浦。测量了激光输出功率、发射波长和输出光束轮廓与入射泵浦功率的关系。三种激光器的输入输出功率特性相似,激光阈值接近1.5W,斜率效率达到入射泵浦功率的量子极限。采用b”型切割Ho:YAP晶体的微芯片激光器,获得了最佳效果(斜率效率79%,激光阈值为1.54W,在几乎衍射受限的线偏光光束中最大输出功率为8.2W)。a”型和b”型Ho:YAP芯片激光器的发射波长为2119nm, c”型Ho:YAP芯片激光器的发射波长为2132nm。所设计的激光器可作为激光辐射的紧凑波长转换器,并可用于扩展当前用于医学和工业的tm光纤激光器的能力,同时保持系统的整体效率。
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引用次数: 0
Laser-diode-pumped Cr:ZnSe CW laser tunable in mid-IR range of 2.05-2.65μm 激光二极管泵浦的Cr:ZnSe连续激光器可在2.05 ~ 2.65μm的中红外范围内调谐
Pub Date : 2023-06-09 DOI: 10.1117/12.2665334
A. Říha, H. Jelínková, M. Doroshenko, M. Němec, J. Šulc, M. Čech, V. Badikov
The spectral and laser characteristics of two anti-reflection (AR) coated Cr:ZnSe single crystals 3 mm and 5 mm long were investigated under ~1.7 μm laser diode pumping. The crystals were assembled in a copper holder actively cooled by circulating water. Room temperature absorption and fluorescence spectra were measured, together with the fluorescence lifetime of Cr2+ ions were measured. The influence of the pump pulse durations on the output laser power was investigated. The mean output power of ~2.7 W in CW mode at the wavelength of ~2.4 μm (~24% slope efficiency) was obtained with the 5 mm thick AR coated sample. In this case the M2 beam parameter of ~1.1±0.1 and the beam waist diameter of ~42±4 μm which corresponds to the maximum (in the beam waist) laser power density of ~200 kW/cm2. Furthermore, using a MgF2 birefringent plate, the laser output was tuned from ~2.05 μm up to ~2.65 μm with a spectral linewidth of ~5-10 nm and a Gaussian beam profile. The mean laser output power in the broad mid-infrared range of ~2.1-2.52 μm exceeded 1 W, which corresponds to a power density of at least ~73.5 kW/cm2.
在~1.7 μm激光二极管泵浦下,研究了两种增透膜(AR)涂层的3 mm和5 mm Cr:ZnSe单晶的光谱和激光特性。这些晶体被组装在一个由循环水主动冷却的铜容器中。测量了室温吸收光谱和荧光光谱,并测量了Cr2+离子的荧光寿命。研究了泵浦脉冲持续时间对输出激光功率的影响。在~2.4 μm波长处,平均输出功率为~2.7 W,斜率效率为~24%。在这种情况下,光束M2参数为~1.1±0.1,束腰直径为~42±4 μm,对应于最大(束腰)激光功率密度为~200 kW/cm2。此外,利用MgF2双折射板,激光输出从~2.05 μm调谐到~2.65 μm,谱线宽度为~5 ~ 10 nm,光束轮廓为高斯分布。在~2.1 ~ 2.52 μm宽中红外范围内,激光平均输出功率超过1w,对应的功率密度至少为~73.5 kW/cm2。
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引用次数: 0
Angle resolved photo electron spectrometer for hard x-ray photon diagnostics at the European XFEL 角度分辨光电子能谱仪在欧洲自由电子激光器的硬x射线光子诊断
Pub Date : 2023-06-09 DOI: 10.1117/12.2665732
J. Laksman, F. Dietrich, J. Liu, T. Maltezopoulos, N. Kujala, M. Planas, W. Freund, S. Francoual, J. Grünert
We have developed and commissioned an angle-resolved photoelectron spectrometer, based on the electron time-of-flight concept, for hard x-ray photon diagnostics at the European Free-Electron Laser. The instrument provides users and operators with pulse-resolved, non-invasive spectral distribution diagnostics, which in the hard x-ray regime is a challenge due to the poor cross-section and high kinetic energy of photoelectrons for the available target gases. We report on the performance of this instrument as obtained using hard x-rays at the PETRA III synchrotron at DESY and the SASE1 beamline at the European XFEL. We demonstrate a resolving power of 10 eV at incident photon energies up to 20 keV.
我们已经开发并委托了一个角度分辨光电子光谱仪,基于电子飞行时间的概念,用于硬x射线光子诊断在欧洲自由电子激光器。该仪器为用户和操作人员提供了脉冲分辨、非侵入性的光谱分布诊断,这在硬x射线条件下是一个挑战,因为可用目标气体的光电子截面差,动能高。我们报告了该仪器在DESY的PETRA III同步加速器和欧洲XFEL的SASE1光束线上获得的硬x射线的性能。我们展示了在入射光子能量高达20 keV时的10 eV的分辨能力。
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引用次数: 0
Amplification of HOH carrying orbital angular momentum in plasma-based amplifiers 等离子体放大器中携带轨道角动量的HOH的放大
Pub Date : 2023-06-08 DOI: 10.1117/12.2665543
Santiago López, A. Alonso, Elena de la Fuente, A. Pandey, O. Guilbaud, E. Oliva
After 30 years since the discovery of the intrinsic orbital angular momentum (OAM) possessed by certain beams, a plethora of applications have been developed in diverse fields such as communications, astrophysics, and biochemistry. Meanwhile, injecting high-order harmonics (HOH) into krypton amplifier plasmas has emerged as a promising alternative to Free Electron Lasers (FEL) for generating table-top, XUV coherent radiation sources. This work brings together these two concepts and asks the following question: what happens when an HOH with OAM is injected into a plasma? Does the amplified beam retain the same OAM, or is this property affected? Understanding the OAM response to this process lays the foundation for new applications. Simulations using the 3D, time-dependent, Maxwell-Bloch code Dagon show that OAM is conserved in low-density plasmas. However, at higher densities, although the OAM is still preserved, the density profiles leave increasing footprints in phase patterns in the form of phase jumps curvature. Finally, a study has been conducted for a plasma with a waveguide, further supporting the potential of OAM for plasma diagnosis.
自某些光束所具有的固有轨道角动量(OAM)被发现30年后,在通信、天体物理学和生物化学等不同领域得到了大量的应用。与此同时,向氪放大器等离子体注入高次谐波(HOH)已成为自由电子激光器(FEL)的一种有前途的替代方案,用于产生桌面XUV相干辐射源。这项工作将这两个概念结合在一起,并提出了以下问题:当将带有OAM的HOH注入等离子体时会发生什么?放大后的光束是否保持相同的OAM,或者这种特性是否受到影响?理解OAM对这个过程的响应为开发新的应用程序奠定了基础。使用三维时间相关麦克斯韦-布洛赫码的模拟显示,OAM在低密度等离子体中是守恒的。然而,在更高的密度下,尽管OAM仍然被保留,但密度剖面在相模式中以相跳曲率的形式留下了越来越多的足迹。最后,对等离子体波导进行了研究,进一步支持了OAM在等离子体诊断中的潜力。
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引用次数: 0
Radiation generation during laser and particle beam interactions in particle-in-cell codes 粒子细胞码中激光与粒子束相互作用时的辐射产生
Pub Date : 2023-06-08 DOI: 10.1117/12.2665680
Patrik Puškáš, Dominika Mašlárová, R. Babjak, M. Krůs
Radiation reaction can severely affect the motion of ultra-relativistic particles in intense electromagnetic fields. Here, we study particle-in-cell (PIC) methods of kinetic modeling of radiation reaction in classical and quantum regimes. We test the methods of photon emission from highly energetic particles moving in strong electromagnetic field in two open-source PIC codes Smilei and EPOCH. We benchmark the codes and discuss the differences.
辐射反应会严重影响超相对论粒子在强电磁场中的运动。在此,我们研究了经典和量子环境下辐射反应动力学建模的粒子胞内(PIC)方法。我们在两个开放源代码的PIC代码Smilei和EPOCH中测试了高能粒子在强电磁场中运动的光子发射方法。我们对代码进行基准测试并讨论其差异。
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引用次数: 0
High power commissioning of BELLA iP2 up to 17 J BELLA iP2高功率调试,最高可达17j
Pub Date : 2023-06-08 DOI: 10.1117/12.2669162
L. Obst-Huebl, K. Nakamura, S. Hakimi, J. De Chant, A. Jewell, B. Stassel, A. Snijders, A. Gonsalves, J. van Tilborg, Z. Eisentraut, Z. Harvey, L. Willingale, C. Tóth, C. Schroeder, C. Geddes, E. Esarey
The new short focal length experimental beamline at the BELLA PW, called iP2, was commissioned up to 17 J laser pulse energy, corresponding to a peak intensity of 1.2 × 1021 W/cm2 on target, based on a measured focal spot size with FWHM 2.7 μm and Gaussian equivalent pulse length of 40 fs. The ion acceleration performance was measured under variation of the laser pulse energy and length, and the laser spot size on target. A maximum proton energy of ∼ 40 MeV was observed in the target normal sheath acceleration regime using 13 μm thick Kapton foil targets. Surveys outside the radiation shielded accelerator cave showed very low radiation levels and there was no measurable activation of experimental installations after performing several tens of shots on target. Back reflections of the laser pulse from the target interaction were monitored and partially mitigated, but ultimately caused damage in the laser frontend. This prohibited further increase of the laser pulse energy beyond 17 J. Implementation of a double plasma mirror is expected to sufficiently suppress back reflections to allow for iP2 experiments at the full BELLA PW pulse energy.
BELLA PW上新的短焦距实验光束线,称为iP2,在FWHM为2.7 μm,高斯等效脉冲长度为40 fs的测量焦斑尺寸的基础上,获得了高达17 J的激光脉冲能量,对应于目标上的峰值强度为1.2 × 1021 W/cm2。测量了激光脉冲能量、脉冲长度和靶上光斑大小变化对离子加速性能的影响。使用13 μm厚的卡普顿箔靶,在靶正常鞘层加速状态下观察到的最大质子能量为~ 40 MeV。辐射屏蔽加速器洞穴外的调查显示,辐射水平非常低,在对目标进行了几十次射击后,实验装置没有可测量的激活。目标相互作用产生的激光脉冲的后反射被监测和部分减轻,但最终在激光前端造成损伤。这就禁止了激光脉冲能量超过17j的进一步增加,双等离子体镜的实现有望充分抑制反向反射,从而允许在BELLA PW脉冲能量下进行iP2实验。
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引用次数: 2
Noncollinear gating of laser-plasma-driven attosecond pulses without spectral filtering 无谱滤波激光等离子体驱动阿秒脉冲的非线性共线门控
Pub Date : 2023-06-08 DOI: 10.1117/12.2665631
M. Yeung, J. P. Kennedy, B. Dromey
Intense attosecond scale pulses of extreme-ultraviolet and soft X-ray light can be generated from plasma surfaces driven relativistically by intense laser pulses. The temporal profile consists of a train of pulses separated by the laser’s optical period and manifests in the spectral domain as harmonics of the laser frequency. Isolating individual attosecond pulses is a key challenge for applications of these sources to time-resolved experiments for attosecond science and plasma-based sources allow the use of ultra-high energies and intensities that can enable fully attosecond scale pump-probe measurements. Results are presented here for numerical Particle-In-Cell simulations of a scheme to angularly sweep the pulses so that one is temporally gated out from the others in the reflected direction. Using two identical laser pulses that are incident noncollinearly on the surface with a time delay causes the instantaneous wavefront to sweep between each of them with the attosecond pulses also being swept in their emission angle accordingly. This method naturally separates out the remaining reflected laser energy due to the angular gap between the incident pulses negating the need for spectral filtering after the interaction. We demonstrate clear gating of a single pulse along the reflected axis in both 2D and 3D simulations and discuss the effect of spectral isolation from the laser frequency. We extend the investigation to further examine techniques to improve the temporal gating by tailoring the laser and target properties.
在强激光脉冲的相对论驱动下,等离子体表面可以产生极紫外光和软x射线的强阿秒级脉冲。时间剖面由激光的光周期分隔的一系列脉冲组成,并在谱域中表现为激光频率的谐波。隔离单个阿秒脉冲是将这些源应用于阿秒科学的时间分辨实验的关键挑战,而基于等离子体的源允许使用超高能量和强度,可以实现完全阿秒尺度的泵浦探针测量。本文给出了一种脉冲角扫描方案的数值模拟结果,该方案可以使脉冲在反射方向上暂时从其他脉冲中门控出来。使用两个相同的激光脉冲,在一个时间延迟的情况下,以非线性方式入射到表面上,使得瞬时波前在它们之间扫过,而阿秒脉冲也相应地在它们的发射角上扫过。由于入射脉冲之间的角间隙,这种方法自然地分离出剩余的反射激光能量,从而消除了相互作用后对光谱滤波的需要。我们在二维和三维模拟中演示了沿反射轴的单脉冲的清晰门控,并讨论了光谱隔离对激光频率的影响。我们进一步研究了通过调整激光和目标特性来改善时间门控的技术。
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引用次数: 0
Development of the multidisciplinary x-ray sources at the ELI Beamlines facility 多学科x射线源在ELI光束线设施的发展
Pub Date : 2023-06-08 DOI: 10.1117/12.2665775
U. Chaulagain, M. Lamač, M. Raclavský, K. H. Rao, Orsolya Morvai, František Vaněk, K. Ta-Phuoc, S. V. Bulanov, J. Nejdl
One of the major objectives of the ELI Beamlines project is to employ the state-of-the-art high power lasers for the generation of ultra-short pulses of particles and X-rays with unprecedented parameters to deliver stable beamline capacity to serve the broad scientific and industrial user community. The development of laser plasma-based X-ray sources at ELI beamlines, especially the ELI Gammatron beamline based on the laser plasma accelerator (LPA) is presented here. The ELI Gammatron beamline is capable of providing X-ray pulses of energies from 1-100 keV in the Betatron scheme and up to few MeV’s in the inverse Compton scheme. A dedicated LPA-based Betatron X-ray source, developed at the ELI plasma physics platform (P3) will serve as an active diagnostic of the high energy density (HED) plasma and laboratory astrophysics multi-beam experiments. In addition to this, a novel scheme for enhancing the X-ray flux of the betratron sources was proposed based on nonlinear resonances in a two-colour laser field interaction. A high-sensitivity optical probing technique for characterizing gas targets for LPA was also developed in-house to support the beamline development.
ELI光束线项目的主要目标之一是采用最先进的高功率激光器,以前所未有的参数产生粒子和x射线的超短脉冲,以提供稳定的光束线容量,为广泛的科学和工业用户社区服务。本文介绍了激光等离子体x射线源在ELI束线上的发展,特别是基于激光等离子体加速器(LPA)的ELI伽玛管束线。ELI伽玛管光束线能够提供能量从1-100 keV的x射线脉冲在Betatron方案和高达几个MeV的反康普顿方案。由ELI等离子体物理平台(P3)开发的基于lpa的专用Betatron x射线源将作为高能量密度(HED)等离子体和实验室天体物理多束实验的主动诊断。在此基础上,提出了一种利用双色激光场相互作用中的非线性共振来提高辐射源x射线通量的新方案。一种用于LPA气体目标表征的高灵敏度光学探测技术也在内部开发,以支持光束线的发展。
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引用次数: 0
Effects of nanodiamonds layer in organic light emitting diode 纳米金刚石层对有机发光二极管的影响
Pub Date : 2023-06-08 DOI: 10.1117/12.2665070
G. Ong, H. Tan, T. Ong, T. Tou, C. Nee, S. Yap
Nanodiamonds (NDs) have attracted great interest due to their high refractive index and thermal conductivity. The unique properties of NDs, including high thermal conductivity, chemical stability, and tensile strength, make them a promising candidate for enhancing OLED efficiency. NDs were coated either beneath or above the PEDOT:PSS hole injection layer in a green-emitting OLEDs (ITO/ PEDOT:PSS/NPD/CBP:Ir(ppy)3/TPBi/Liq/Al). The best performance is obtained from the device with NDs layer beneath the PEDOT:PSS layer where the current efficiency (CE) is increased by 5.4%, power efficiency (PE) is increased by 17.7% and the external quantum efficiency (EQE) is increased by 4.5% at a luminance of 10000 cd/m2 as compared to a standard device without NDs layer.
纳米金刚石(NDs)由于其高折射率和导热性而引起了人们的广泛关注。nd的独特性质,包括高导热性、化学稳定性和抗拉强度,使其成为提高OLED效率的有希望的候选者。在绿色发光oled (ITO/ PEDOT:PSS/NPD/CBP:Ir(ppy)3/TPBi/Liq/Al)中,将nd涂覆在PEDOT:PSS空穴注入层的下方或上方。在PEDOT:PSS层下方有nd层的器件,在亮度为10000 cd/m2时,与没有nd层的标准器件相比,电流效率(CE)提高了5.4%,功率效率(PE)提高了17.7%,外量子效率(EQE)提高了4.5%。
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引用次数: 0
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Optics + Optoelectronics
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