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Assessments of radiological and toxicological risks from the use of groundwater and surface water in the zone of influence of the uranium production legacy site 评估铀生产遗留场址影响区内使用地下水和地表水的辐射和毒理学风险
IF 0.3 Q4 Physics and Astronomy Pub Date : 2022-12-25 DOI: 10.15407/jnpae2022.04.271
B. Zanoz, D. O. Bugai, D. Koliabina, R. Avila
Radioactive and chemical contamination of groundwater and surface water (Konoplyanka and Dnipro Rivers) in the zone of influence of the soviet era uranium production legacy site - Prydniprovsky Chemical Plant (PChP, Kamianske) is a source of radiological and toxicological risks for the population. Modeled water use scenarios included drinking water consumption, crop irrigation, fishing, and usage of the river beaches for recreation. According to the assessment results, the radiological risks of water usage in current conditions are low. At the same time, a conservative assessment indicates potential future toxicological risks from uranium (use of groundwater for drinking) and from manganese (due to accumulation in river fish). In the long term, risks from groundwater may increase significantly due to the dispersion of contaminated groundwater plumes outside the industrial site, or due to unrestricted access of the population to the territory of the PChP. To reduce uncertainty in the risk assessment results, it is important to improve the groundwater monitoring network downstream from the PChP site and to collect site-specific data on manganese transfer coefficients to fish.
苏联时代铀生产遗留地点——Prydniprovsky化工厂(PChP, Kamianske)影响区内的地下水和地表水(Konoplyanka河和第聂伯罗河)受到放射性和化学污染,对人口构成放射性和毒理学风险。模拟的水使用场景包括饮用水消耗、作物灌溉、捕鱼和河滩娱乐的使用。根据评价结果,在目前条件下,用水的放射性风险较低。与此同时,一项保守的评估表明,铀(使用地下水饮用)和锰(由于河鱼体内的积累)可能带来未来的毒理学风险。从长远来看,由于受污染的地下水扩散到工业场地外,或由于人口不受限制地进入卫生防护中心的领土,地下水的风险可能会大大增加。为减少风险评估结果的不确定性,有必要完善PChP站点下游的地下水监测网络,并收集特定站点的锰向鱼类转移系数数据。
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引用次数: 0
Evaluation of gamma-ray buildup factors for some waste paper and natural rubber composites 某些废纸和天然橡胶复合材料的射线积累因子评价
IF 0.3 Q4 Physics and Astronomy Pub Date : 2022-12-25 DOI: 10.15407/jnpae2022.04.280
M. A. El-Sarraf, A. El-Sayed Abdo
In this work, four waste paper composites were studied in terms of several photon interaction parameters over the energy region from 0.015 to 15.0 MeV. The waste paper and natural rubber (WP/NR) composites of different densities ranging from ρ = 0.894 to 1.16 gm⋅cm-3 were used for shielding radioactive rubble at different time period stages. Some additives were also used including high-abrasion furnace black, paraffin wax, B4C, as well as magnetite. The deduced parameters of photon interaction: equivalent atomic number Zeq, exposure buildup factor and energy absorption buildup factor have been studied as a function of incident photon energy, WP/NR elemental composition, and for penetration depths, up to 40 mean free path. The Zeq numbers have shown slight variation over the selected incident energy range and buildup factors were found to be modest at low and high photon energy meanwhile their values increase widely over the intermediate energy region. In addition, kerma relative to air for photon energies from 1 to 20 MeV were computed and show dependence upon equivalent atomic numbers. In this work, it was clear that filled samples offer better shielding capabilities than unfilled ones. The obtained data could be useful for radiation physicists and scientists in estimating the γ-irradiation received after applying such shields.
本文研究了4种废纸复合材料在0.015 ~ 15.0 MeV能量范围内的光子相互作用参数。在ρ = 0.894 ~ 1.16 gm⋅cm-3范围内,采用不同密度的废纸与天然橡胶(WP/NR)复合材料,在不同时间段对放射性碎石进行屏蔽。还使用了高磨耗炉黑、石蜡、B4C和磁铁矿等添加剂。研究了光子相互作用的等效原子序数Zeq、暴露累积因子和能量吸收累积因子与入射光子能量、WP/NR元素组成和穿透深度(平均自由程可达40)的关系。Zeq值在选定的入射能量范围内变化不大,在低光子和高光子能量范围内积聚因子不大,而在中间能量范围内积聚因子的值则大幅度增加。此外,计算了光子能量从1到20 MeV的相对于空气的kerma,并显示出与等效原子序数的依赖关系。在这项工作中,很明显,填充的样品比未填充的样品提供更好的屏蔽能力。所获得的数据可用于辐射物理学家和科学家估计施加这种屏蔽后所受到的γ辐照。
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引用次数: 1
Properties of the diffusion and drift kinetic coefficients in momentum space for a cold Fermi system 冷费米系统动量空间中扩散和漂移动力学系数的性质
IF 0.3 Q4 Physics and Astronomy Pub Date : 2022-10-27 DOI: 10.15407/jnpae2023.01.005
S. V. Lukyanov
Using the methods of kinetic theory, expressions for the diffusion and drift coefficients for a cold Fermi system are obtained. Their dependencies on the momentum are calculated for the step distribution function as well as in the case of excitation of a particle-hole pair.
利用动力学方法,得到了冷费米系统的扩散系数和漂移系数的表达式。对于阶跃分布函数以及粒子-空穴对的激励情况,计算了它们对动量的依赖关系。
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引用次数: 0
Potentials of interaction of 10,11,12,13B isotopes with 12C 10、11、12、13B同位素与12C的相互作用势
IF 0.3 Q4 Physics and Astronomy Pub Date : 2022-09-25 DOI: 10.15407/jnpae2022.03.164
S. Mezhevych, A. Rudchik, O. Ponkratenko, K. Rusek, K. Kemper, V.M. Kyrianchuk, A. A. Rudchik, Y. Stepanenko, V. Uleshchenko
A comparative analysis of calculations for the 12С(10В,10В)12С elastic scattering at Еlab(10B) = 41.3 MeV, the 12С(11В,11В)12С elastic scattering at Еlab(11B) = 40.0 MeV, transfer reactions 13С(11В,12С)12В and 14С(11В,12С)13В at Еlab(11B) = 45.0 МеВ was performed within the coupled-reaction-channels method (CRC) using previously deduced Woods-Saxon potentials for the interaction of 10,11,12,13В + 12С nuclei in the exit reaction channels, as well as potentials for these systems of nuclei generated by means of the double-folding method using theoretically modeled shapes for the distributions of protons and neutrons in 10,11,12,13В and 12С. The relationship of isotopic effects (differences of the calculated CRC cross sections when replacing the potential for a given pair of nuclei by interaction potential for one nucleus with the isotope of another nucleus) with the internal structure, e.g. the shapes of nucleon density distributions in the interacting nuclei, is investigated. The shapes (radial dependence) of recently deduced Woods-Saxon potentials and potentials calculated by means of the double-folding methods for the systems of 10,11,12,13В + 12С nuclei are compared. Based on the results of the analysis of experimental data, an assumption is made about the possible differences in the shapes of surface nucleon density distributions from the ones modeled theoretically in 10,11B isotopes.
比较分析计算的12个С(10В10В)12С弹性散射Е实验室(10 b) = 41.3兆电子伏,12个С(11ВВ11日)12С弹性散射Е实验室(11 b) = 40.0兆电子伏,转移反应13С(11В12С)12В和14С(11В12С)13ВЕ实验室(11 b) = 45.0МеВcoupled-reaction-channels内执行方法(CRC)使用之前推断Woods-Saxon潜力10的交互,11日12日13日В+ 12С原子核在反应退出渠道,以及利用理论模拟的质子和中子在10、11、12、13В和12С的分布的形状,用双折叠方法产生的这些核系统的势。研究了同位素效应(用一个原子核与另一个原子核的同位素相互作用势代替一对给定原子核的势时计算出的CRC截面的差异)与内部结构(如相互作用原子核中核子密度分布的形状)的关系。比较了10、11、12、13В + 12С核系最近推导的Woods-Saxon势和用双折叠方法计算的势的形状(径向依赖)。根据实验数据的分析结果,对10、11B同位素表面核子密度分布的形状与理论模型可能存在的差异作了假设。
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引用次数: 0
Determination of 63Ni activity in NPP construction materials 核电厂建筑材料中63Ni活性的测定
IF 0.3 Q4 Physics and Astronomy Pub Date : 2022-09-25 DOI: 10.15407/jnpae2022.03.207
V. O. Zheltonozhskyi, D. E. Myznikov, A. M. Savrasov, V. I. Slisenko
The γ-spectra were measured of the structural materials of the 2nd unit of the Chornobyl NPP which were irradiated by bremsstrahlung with end-point energy 37 MeV. Using the ratio of the 57Co and 58Co activities, the nickel and cobalt masses ratio was determined. Using the obtained data and the measured 60Co activity in the studied samples, a method for determining of the 63Ni activity was developed. Radiochemical validation of the created method was performed and good quantitative agreement of 63Ni activities obtained by spectroscopic and radiochemical methods was obtained.
用末端能量为37mev的轫致辐射,测量了切尔诺贝利核电站2号机组结构材料的γ-能谱。利用57Co和58Co活性比,确定了镍和钴的质量比。利用所得数据和样品中60Co活性的测定,建立了一种测定63Ni活性的方法。对所建立的方法进行了放射化学验证,并获得了光谱和放射化学方法获得的63Ni活度的良好定量一致性。
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引用次数: 1
Elastic and inelastic scattering of 15N ions by 10B at energy 81 MeV. Isotopic effects in scattering of 15N + 10В, 15N + 11В, 14N + 10В nuclei 81mev下10B对15N离子的弹性和非弹性散射。15N + 10В, 15N + 11В, 14N + 10В核散射中的同位素效应
IF 0.3 Q4 Physics and Astronomy Pub Date : 2022-09-25 DOI: 10.15407/jnpae2022.03.153
A. Rudchik, A. A. Rudchik, V.V. Khejlo, K. Rusek, K. Kemper, E. Piasecki, A. Stolarz, A. Trzcińska, Val. M. Pirnak, O. Ponkratenko, E. I. Koshchy, O. E. Kutsyk, S. Mezhevych, A. P. Ilyin, Y. Stepanenko, V. Uleshchenko, Yu. O. Shyrma
New experimental data of angular distributions for the elastic and inelastic scattering of 15N ions by 10B nuclei were obtained at the energy Elab(15N) = 81 MeV. The experimental data were analyzed within the coupled-reaction channels method (CRC). The Woods - Saxon optical potentials were used for nuclei interactions in the calculations. The potential's parameters for the interaction of 15N + 10В nuclei were deduced as well as it was measured the angular distribution of the elastic scattering for these nuclei. The experimental data of the 15N + 10В elastic scattering are compared with data of the 15N + 11В and 14N + 10В scatterings. It was discovered isotopic effects in the scatterings of these three nuclear couples due to the difference in the optical potentials of the interaction of these nuclei and their structure. New experimental data of inelastic scattering of 15N + 10В nuclei for 0.718 - 3.587 МеV states of 10В nucleus and for 5.270 - 6.324 МеV states of 15N nucleus were measured. These data were analyzed within the CRC method using the translation-invariant shell model for collective excitations of 15N and 10B nuclei. Information about deformations of these nuclei was obtained.
在Elab(15N) = 81 MeV的能量下,获得了10B核对15N离子弹性和非弹性散射角分布的新实验数据。采用耦合反应通道法(CRC)对实验数据进行分析。计算中采用Woods - Saxon光势描述原子核相互作用。推导了15N + 10В核相互作用的势参数,并测量了这些核的弹性散射角分布。将15N + 10В弹性散射实验数据与15N + 11В和14N + 10В弹性散射实验数据进行了比较。由于这三种核对相互作用的光势及其结构的不同,在散射中发现了同位素效应。测量了15N + 10В核在10В核的0.718 ~ 3.587 МеV态和15N核的5.270 ~ 6.324 МеV态的非弹性散射的新实验数据。这些数据在CRC方法中使用15N和10B核集体激发的平移不变壳层模型进行了分析。获得了这些核的变形信息。
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引用次数: 1
Zoning of radioactively contaminated territories after the Chornobyl accident 切尔诺贝利事故后放射性污染地区的分区
IF 0.3 Q4 Physics and Astronomy Pub Date : 2022-09-25 DOI: 10.15407/jnpae2022.03.182
V. Kashparov, D. Holiaka, S. Levchuk, V. Berkovskyy
The radiological zoning of Chornobyl contaminated areas was one of the essential elements of social and radiation protection. The zoning was based on estimates of annual committed effective doses to members of the public and on the levels of radionuclide deposition density. In 1991, 86 settlements were classified as associated with the zone of unconditional (mandatory) resettlement, and 841 settlements were assigned to the zone of guaranteed voluntary resettlement. The status of these settlements has been preserved until now. The assessments showed that as of 2022, for all settlements located outside the Chornobyl Exclusion Zone the radiological conditions do not exceed the current legislative criteria for inclusion in the zone of unconditional (mandatory) resettlement. It is also shown that in 2022, the zone of guaranteed voluntary resettlement can be assigned for: only 38 settlements, according to the legislative criterion "90Sr density of contamination" and only 17 settlements, according to the legislative criterion "137Cs density of contamination". The work also indicates and analyses the provisions of current legislation that require clarification.
切尔诺贝利污染地区的辐射区划是社会和辐射保护的基本要素之一。分区是根据对公众每年承诺有效剂量的估计和放射性核素沉积密度的水平确定的。1991年,86个定居点被划归无条件(强制)重新安置区,841个定居点被划归有保证的自愿重新安置区。这些定居点的地位一直保持到现在。评估表明,截至2022年,位于切尔诺贝利禁区以外的所有定居点的辐射条件不超过目前列入无条件(强制)重新安置区的立法标准。根据立法标准“污染密度90Sr”和立法标准“污染密度137Cs”,到2022年,自愿安置保障区只能分配给38个定居点和17个定居点。这项工作还指出和分析了需要澄清的现行立法的规定。
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引用次数: 0
The nuclear safety monitoring system for fuel-containing materials located in destroyed unit No. 4 of the Chornobyl NPP and proposals for its modernization 位于被毁的切尔诺贝利核电站4号机组的含燃料材料核安全监测系统及其现代化建议
IF 0.3 Q4 Physics and Astronomy Pub Date : 2022-09-25 DOI: 10.15407/jnpae2022.03.172
M. V. Saveliev, R. L. Godun, M. Pantin, I. Skiter, K. Sushchenko
The paper presents a brief description of the Nuclear Safety Monitoring System (NSMS), which is a part of the Integrated Automated Monitoring System of the "Shelter" object (a facility that covers the destroyed Unit No. 4 of the Chornobyl NPP). Further development of the NSMS is proposed by introducing algorithms for automatic identification of neutron anomalies with a help of fuzzy logic and statistical methods; digital filtering of specific irregular impulse interferences leading to metrological system failures; algorithms for predicting changes in neutron flux density and assessing changes in the nuclear hazard of fuel containing materials accumulations.
本文简要介绍了核安全监测系统(NSMS),该系统是“庇护所”对象(覆盖被摧毁的切尔诺贝利核电站4号机组的设施)综合自动监测系统的一部分。通过引入基于模糊逻辑和统计方法的中子异常自动识别算法,提出了NSMS的进一步发展方向;导致计量系统故障的特殊不规则脉冲干扰的数字滤波预测中子通量密度变化和评估含燃料材料聚集体核危害变化的算法。
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引用次数: 0
Effect of forest fires on forest plant complexes contaminated by radionuclides 森林火灾对受放射性核素污染的森林植物复合体的影响
IF 0.3 Q4 Physics and Astronomy Pub Date : 2022-09-25 DOI: 10.15407/jnpae2022.03.195
L. Romanchuck, V. Ustymenko
Among the most pressing threats to the existence of forest plant complexes of the nature reserve fund is the pyrogenic danger, which is exacerbated by changes in the natural hydrolytic regime and global climate change, the driving effects of which are currently difficult to fully assess. The article highlights the results of a study of the forest plant complexes and soil state of the nature reserve "Drevlyanskyi" in Zhytomyr region after the fires. The results of the field survey of plantations, agrochemical and radiological analysis of soil indicators are presented. Studies show a change in the composition of forest plant complexes, a reduction in the number of herbaceous species, and a decrease in the area of moss and lichen cover. The surveyed area is characterized by significant spatial heterogeneity of the main agrochemical and physicochemical parameters of the soil. There was a slight increase in the content of heavy metals in the soil, however, the indicators did not exceed the maximum allowable concentrations in these areas. To assess the radiation situation after fires on the territory of the nature reserve, the indicators of the density of soil pollution with 137Cs and 90Sr were determined. The authors recommended a set of measures to improve the efficiency of nature reserves. Adherence to the recommendations will help to increase the environmental sustainability of forest plant complexes and will minimize the occurrence of fires and their consequences.
自然保护区森林植物复合体生存面临的最紧迫威胁是热原性危险,自然水解机制的变化和全球气候变化加剧了热原性危险,而热原性危险的驱动效应目前难以充分评估。本文重点介绍了日托米尔地区“德雷夫利扬斯基”自然保护区火灾后森林植物复合体和土壤状态的研究结果。介绍了人工林的野外调查结果、土壤指标的农化和放射性分析结果。研究表明,森林植物复合体的组成发生了变化,草本物种的数量减少,苔藓和地衣覆盖的面积减少。调查区土壤主要农化和理化参数具有显著的空间异质性。土壤中重金属含量略有增加,但各项指标均未超过最大允许浓度。为评价自然保护区火灾后的辐射状况,测定了137Cs和90Sr土壤污染密度指标。作者提出了一套提高自然保护区效率的措施。遵守这些建议将有助于提高森林植物综合体的环境可持续性,并将尽量减少火灾的发生及其后果。
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引用次数: 0
Improved parametrization of inclusive proton spectra from 3H(α,p)6He reaction using data obtained in a correlation experiment 利用相关实验数据改进了3H(α,p)6He反应包涵质子谱的参数化
IF 0.3 Q4 Physics and Astronomy Pub Date : 2022-09-25 DOI: 10.15407/jnpae2022.03.159
O. Povoroznyk, O. K. Gorpinich
The new analysis of inclusive proton spectra from 3H(α,p)6He reaction was performed. The existence of two new excited levels of 6He with energy parameters E2ex.s.*= 2.4 MeV, Γ = 0.4 MeV; E3ex.s.*= 3.0 MeV, Γ = 0.6 MeV was confirmed as a result of new parameterization performed using energy parameters obtained from the correlation kinematic-incomplete experimental study of 3H(α,pα)nn reactions at Eα = 27.2 MeV and Eα = 67.2 MeV in contrast to the initial analysis, in which the resonance observed above the known first excited 6He level E1ex.s. = 1.8 MeV was treated as the second broad excited level E2ex.s. = 2.98 (0.17) MeV, Γ2ex.s. = 2.39 (0.27) MeV.
对3H(α,p)6He反应的包涵质子谱进行了新的分析。能级参数为e2exs的6He的两个新激发态的存在性。*= 2.4 MeV, Γ = 0.4 MeV;E3ex.s。在Eα = 27.2 MeV和Eα = 67.2 MeV的3H(α,pα)nn反应的相关运动学不完全实验研究中获得的能量参数进行了新的参数化,与初始分析相比,证实了*= 3.0 MeV, Γ = 0.6 MeV,其中在已知第一激发6He能级e1exs以上观察到的共振。= 1.8 MeV作为第二宽激发能级e2exs。= 2.98 (0.17) MeV, Γ2ex.s。= 2.39 (0.27) MeV。
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引用次数: 0
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Nuclear Physics and Atomic Energy
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