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Alkyl derivative of p-terphenyl as an activator of polysiloxane-based scintillator 对三苯基的烷基衍生物作为聚硅氧烷基闪烁体的活化剂
IF 0.3 Q4 Physics and Astronomy Pub Date : 2022-09-25 DOI: 10.15407/jnpae2022.03.212
P. Zhmurin, D.A. Yelisieiev, V. Alekseev, O.V. Yelisieieva, Yu.О. Нurkalenko
One of the problems in creating a radiation-hard scintillation composition on a polysiloxane base is the search for a radiation-hard activator capable of dissolving in such a base in sufficient quantity. In this work, in order to improve the solubility of p-terphenyl molecules in a polysiloxane base, its structure was modified with tert-butyl substituents. The obtained alkyl derivative of p-terphenyl was used as an activator of polysiloxane-based scintillators. The optical and scintillation properties of the obtained polysiloxane-based scintillators were studied, and their radiation hardness was determined.
在聚硅氧烷碱上制造抗辐射闪烁组合物的问题之一是寻找一种能够充分溶解在这种碱中的抗辐射活化剂。为了提高对terphenyl分子在聚硅氧烷碱中的溶解度,本文采用叔丁基取代基对其结构进行了修饰。得到的对三苯基的烷基衍生物被用作聚硅氧烷基闪烁体的活化剂。研究了所制备的聚硅氧烷基闪烁体的光学性能和闪烁性能,并测定了其辐射硬度。
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引用次数: 0
Preliminary safety analysis at the decommissioning of the WWR-M research reactor WWR-M研究堆退役安全性初步分析
IF 0.3 Q4 Physics and Astronomy Pub Date : 2022-06-25 DOI: 10.15407/jnpae2022.02.107
Y. Lobach, Sergiy Y. Lobach, V. M. Shevel
Following the demands established by the current Ukrainian legislation, the Decommissioning Concept for the WWR-M research reactor was recently approved. The Concept envisages a strategy of immediate dismantling; it identifies and justifies the main technical and organizational measures for the preparation and implementation of decommissioning, the sequence of planned works and activities, as well as the necessary conditions and infrastructure. Decommissioning requires proper planning and demonstration that all planned dismantling works will be carried out safely. Presented safety assessment is a mandatory component of the Concept and the most important element of the overarching technological scheme. The purpose of the safety analysis is to provide input for detailed planning on how to ensure safety during decommissioning. Based on the results of the safety analysis, the measures to ensure radiation protection are defined while justifying their necessity and sufficiency.
根据乌克兰现行立法规定的要求,WWR-M研究堆的退役概念最近获得核准。该概念设想了一项立即拆除的战略;它确定并证明准备和执行退役的主要技术和组织措施、计划的工作和活动的顺序以及必要的条件和基础设施是合理的。拆除工程需要适当的规划和证明所有计划的拆卸工程将安全进行。提出的安全评估是该概念的强制性组成部分,也是总体技术方案的最重要组成部分。安全分析的目的是为如何确保退役期间的安全提供详细规划。根据安全分析的结果,确定了确保辐射防护的措施,同时证明了这些措施的必要性和充分性。
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引用次数: 1
Representative and highly sensitive express method of measurement of f-activity 具有代表性的高灵敏度的f-活度测定方法
IF 0.3 Q4 Physics and Astronomy Pub Date : 2022-06-25 DOI: 10.15407/jnpae2022.02.140
Y. Shchepkin, N. Mazina, V. I. Slisenko, D. Stratilat
The method for determination of f-activity (spontaneous fission) of samples based on a combination of multiplicity spectrometry, measurement of radiation energy, and registration of time of long-range fission products is considered. The method is representative, highly sensitive, and fast. The minimum determined value of the specific activity is 1.4⋅10-3 Bq/g.
研究了基于多重光谱法、辐射能量测量和远程裂变产物时间记录相结合的样品自发裂变活性测定方法。该方法具有代表性,灵敏度高,速度快。比活度最小测定值为1.4⋅10-3 Bq/g。
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引用次数: 0
Effect of high energy electron exposure of the saline solution on physicochemical properties and cytotoxic activity of doxorubicin 高能电子暴露盐水溶液对阿霉素理化性质和细胞毒活性的影响
IF 0.3 Q4 Physics and Astronomy Pub Date : 2022-06-25 DOI: 10.15407/jnpae2022.02.131
M. A. Zabolotnyy, L. Aslamova, G. Dovbeshko, O. Gnatyuk, V. Neimash, V. Povarchuk, V. Orel, D. Kolesnyk, L. M. Kirkilevska, G.I. Solyanyk
The effect of preliminary irradiation of an aqueous solution of sodium chloride (saline) with 1 MeV high-energy electron beams on optical and cytotoxic/cytostatic properties of the dissolved Doxorubicin cancer drug is studied. With the use of Lewis lung carcinoma cell culture, it has been shown that the said treatment results in an increased cytotoxic/cytostatic action of the Doxorubicin, being the most pronounced in the range of low concentrations of the drug. The delivered dose of ionizing radiation on the saline ranged from 4 to 80 kGy. The maximum changes in the IR absorption spectra of Doxorubicin have been observed for the solutions irradiated with 10 kGy. The possible causes of the observed effects are discussed.
研究了1兆电子伏特高能电子束初照射氯化钠(生理盐水)对溶解的阿霉素抗癌药光学性能和细胞毒/细胞抑制性能的影响。使用Lewis肺癌细胞培养,已经表明,上述治疗结果增加了阿霉素的细胞毒性/细胞抑制作用,在药物低浓度范围内最为明显。在生理盐水上释放的电离辐射剂量为4至80千戈瑞。在10 kGy辐照下,阿霉素的红外吸收光谱变化最大。讨论了所观察到的效应的可能原因。
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引用次数: 1
Model of reactivity accident of the RBMK-1000 reactor RBMK-1000反应堆反应性事故模型
IF 0.3 Q4 Physics and Astronomy Pub Date : 2022-06-25 DOI: 10.15407/jnpae2022.02.099
V. Borysenko, V. Goranchuk
The reactor model was used to study the accident that destroyed the RBMK-1000 reactor at Unit 4 of the Chornobyl nuclear power plant on 26 April 1996. The model of reactivity accident of the RBMK-1000 reactor is based on equations of nuclear reactor kinetics, taking into account feedback in reactor reactivity. Reactivity changes as a result of both external influences – the movement of regulatory organs, changes in the reactor inlet coolant temperature, – and as a result of feedback by core parameters – changes in fuel temperature, coolant density, and 135Хе concentration. The model takes into account steam generation in the reactor core, which corresponds to the real physics of processes at the RBMK reactor, and allows obtaining simulation results that best match the recorded data and the consequences of the accident process. The study of reactivity accident on RBMK-1000 reactor is carried out for different combinations of values of control rods efficiency; reactivity coefficients by fuel temperature and coolant density; changes in the reactor inlet coolant temperature; the emergency protection time, as well as the reactor power level before closing the turbine generator stop valve. Different reactivity accident scenarios at RBMK-1000 reactor allow us to determine the most unfavorable combinations of external influences on the course of reactivity accident, namely: start time of main coolant pump rundown, time of activation of emergency protection, power level before the closing of turbine generator stop valves. In most reactivity accident scenarios, first of all, the critical values of fuel enthalpy are reached, at which the process of fuel destruction in the fuel element, destruction of the fuel assembly, and assembly channel start. Important results of studies are 1 – determination of the fact that time of activation of emergency protection after the closing of stop valves of turbine generator significantly affects the value of the maximum neutron power that is achieved during a reactivity accident; 2 – determination of the effect of reactor power before the closing of turbine generator stop valves on the course of the accident; 3 – it is not necessary to achieve supercritical on instantaneous neutrons, supercritical on delayed neutrons is enough to start fuel destruction.
反应堆模型用于研究1996年4月26日毁坏切尔诺贝利核电站4号机组RBMK-1000反应堆的事故。RBMK-1000反应堆的反应性事故模型以核反应堆动力学方程为基础,考虑了反应堆反应性中的反馈。反应性的变化是由于两种外部影响——调节机构的移动、反应堆入口冷却剂温度的变化,以及堆芯参数反馈的结果——燃料温度、冷却剂密度和135Хе浓度的变化。该模型考虑了反应堆堆芯中的蒸汽产生,这与RBMK反应堆过程的真实物理特性相对应,并允许获得与记录数据和事故过程后果最匹配的模拟结果。采用不同的控制棒效率值组合,对RBMK-1000反应堆的反应性事故进行了研究;按燃料温度和冷却剂密度计算的反应性系数;反应堆进口冷却剂温度的变化;紧急保护时间,以及电抗器功率水平前关闭汽轮发电机截止阀。通过RBMK-1000反应堆不同的反应性事故情景,我们确定了外部影响对反应性事故过程最不利的组合,即:主冷却剂泵熄火开始时间、应急保护启动时间、汽轮发电机截止阀关闭前的功率水平。在大多数反应性事故场景中,首先达到燃料焓的临界值,此时开始燃料元件内燃料的破坏、燃料组件的破坏和组件通道的破坏过程。研究的重要结果是:1 .确定了汽轮发电机截止阀关闭后应急保护启动的时间对反应性事故中达到的最大中子功率值有显著影响;2 -确定涡轮发电机截止阀关闭前反应堆功率对事故进程的影响;没有必要达到瞬时中子的超临界,延迟中子的超临界足以开始燃料破坏。
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引用次数: 0
Degradation and recovery features of irradiated GAP LEDs 辐照GAP led的降解和恢复特性
IF 0.3 Q4 Physics and Astronomy Pub Date : 2022-06-25 DOI: 10.15407/jnpae2022.02.116
O. Budnyk, R. Vernydub, O. Kyrylenko, P. Lytovchenko, O. Radkevych, D. Stratilat, V. Tartachnyk
The homo-transitional original and irradiated by electrons with E = 2 MeV; F = 5.9⋅1014 cm-2 ÷ 8.2⋅1016 cm-2 GaP LEDs were studied. The effect of radiation treatment on their electrical and optical characteristics was studied; the results of isochronous annealing of irradiated samples are given; the consequences of high-temperature annealing of output diodes are analyzed. Peculiarities of the formation of the current-voltage characteristics of red LEDs doped with Zn, O, and green LEDs doped with N under reverse bias, as well as features of the recovery of the reverse current during annealing of both types of LEDs, are revealed.
经E = 2 MeV的电子辐照后的同质跃迁原态;F = 5.9⋅1014 cm-2 ÷ 8.2⋅1016 cm-2研究了辐照处理对其电学和光学特性的影响;给出了辐照样品的等时退火结果;分析了输出二极管高温退火的后果。揭示了掺杂Zn、O的红色led和掺杂N的绿色led在反向偏置下电流-电压特性形成的特点,以及两种led在退火过程中反向电流恢复的特点。
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引用次数: 0
Characteristics of the territory of the Rivne region according to the value of radon flux density out of the soil 根据土壤中氡通量密度的值来确定Rivne地区的领土特征
IF 0.3 Q4 Physics and Astronomy Pub Date : 2022-06-25 DOI: 10.15407/jnpae2022.02.122
M. Klymenko, O. Klymenko, O. Lebed, L. Klymenko, I.I. Zaleskiy, O.V. Varzhel
This article presents features of pre-Mesozoic Quaternary sediments and soil variations for the territory of the region. Middle-Upper Riphean sediments (sandstones) of the Lower Vendus (tuffs, basalts), represent the Polissia zone on the territory. The Lisostep zone is represented by Devonian sediments (interlayers of argillites, siltstones, and limestones). The soils of the Polissia area formed the mellow sand and moraine deposits and represent the soddy podzolic of the different levels of soil gleying. The soils of Lisostep formed less and loamy soils and they represent mainly grey forest podzolic and low humus chernozem with the marks of soil podzolization. The scale of quantitative and qualitative estimation of constrained ecological risk for the region population is set from lower to a high level with the value of radon current density out of the soil from 0 to 25 mBq/(m2⋅s), medium – from 25.1 to 50 mBq/(m2⋅s), higher than medium from 50.1 to 75 mBq/(m2⋅s), higher than 75 mBq/(m2⋅s). Notably, in the Polissia area, 46.3 % of the population suffers from a medium level of risk and in the area of Lisostep, 23.4 % of the population suffers from higher than medium risk and 4.6 % suffers from high-constrained ecological risk.
本文介绍了该地区前中生代第四纪沉积特征和土壤变化。中上Riphean沉积物(砂岩)的下Vendus(凝灰岩,玄武岩),代表领土上的Polissia带。流步带以泥盆纪沉积物(泥质岩、粉砂岩和灰岩夹层)为代表。Polissia地区的土壤形成了成熟的砂和冰碛沉积,代表了不同程度的土壤滑脱的碳酸灰化期。利索阶的土壤形成较少的壤质土,主要为灰色森林灰化土和低腐殖黑钙土,具有土壤灰化土的标志。区域人口约束生态风险的定量和定性评价尺度由低到高,土壤中氡电流密度为0 ~ 25 mBq/(m2·s),中至25.1 ~ 50 mBq/(m2·s),中高至50.1 ~ 75 mBq/(m2·s),中高至75 mBq/(m2·s)。值得注意的是,在波利西亚地区,46.3%的人口面临中等程度的风险,在利索step地区,23.4%的人口面临中等以上的风险,4.6%的人口面临高度受限的生态风险。
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引用次数: 0
Elastic and inelastic form factors of the 10B nuclei with the large-basis shell model 大基壳模型下10B核的弹性和非弹性形状因子
IF 0.3 Q4 Physics and Astronomy Pub Date : 2022-06-25 DOI: 10.15407/jnpae2022.02.093
Bashair H. Jawed, A. D. Salman, S.M. Imran Hossain
In this study, inelastic and elastic form factors for the low-lying excited states of 10B nucleus were calculated utilizing the nuclear shell model theory. We employed a large-basis psd model space with psdmwk interaction and the harmonic oscillator potential in the form factors calculation. The calculated results with the effective charge are in acceptable agreement with experimental results.
本研究利用核壳模型理论计算了10B核低洼激发态的非弹性和弹性形状因子。在形状因子计算中,我们采用了具有psdmwk相互作用和谐振子势的大基psd模型空间。计算结果与实验结果吻合较好。
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引用次数: 0
Assessment of the possibility of a return to the original use of pastures and hayfields abandoned after the Chornobyl accident 评估重新使用切尔诺贝利事故后废弃的牧场和草场的可能性
IF 0.3 Q4 Physics and Astronomy Pub Date : 2022-03-25 DOI: 10.15407/jnpae2022.01.047
Y. Khomutinin, O. V. Kosarchuk, S. Polishchuk, M. Lazarev, S. Levchuk, V. V. Pavliuchenko
A radiological assessment of hayfields and pastures (Narodychy district, Zhytomyr region), which were taken out of economic use due to contamination after the Chornobyl accident, was performed. The possibility and ways of returning the lands to original use were considered. Maps of 137Cs and 90Sr soil contamination densities for the field were made and the corresponding statistical characteristics of the contamination were estimated. Estimates of 137Cs and 90Sr activity concentration in natural grasses, cow milk, and meat as well as the risks of exceeding by the values the permissible levels have been calculated. The possibility of using the land for the production of milk and meat has been shown in the example of the considered radioactively contaminated pastures.
对在切尔诺贝利事故后因污染而停止经济使用的干草田和牧场(Narodychy区,日托米尔地区)进行了放射性评估。对土地恢复原状的可能性和途径进行了探讨。绘制了田间137Cs和90Sr土壤污染密度图,并估算了相应的污染统计特征。对天然草、牛奶和肉类中137Cs和90Sr活性浓度的估计值以及超过允许水平的风险进行了计算。利用这片土地生产牛奶和肉类的可能性在被认为受到放射性污染的牧场的例子中得到了证明。
{"title":"Assessment of the possibility of a return to the original use of pastures and hayfields abandoned after the Chornobyl accident","authors":"Y. Khomutinin, O. V. Kosarchuk, S. Polishchuk, M. Lazarev, S. Levchuk, V. V. Pavliuchenko","doi":"10.15407/jnpae2022.01.047","DOIUrl":"https://doi.org/10.15407/jnpae2022.01.047","url":null,"abstract":"A radiological assessment of hayfields and pastures (Narodychy district, Zhytomyr region), which were taken out of economic use due to contamination after the Chornobyl accident, was performed. The possibility and ways of returning the lands to original use were considered. Maps of 137Cs and 90Sr soil contamination densities for the field were made and the corresponding statistical characteristics of the contamination were estimated. Estimates of 137Cs and 90Sr activity concentration in natural grasses, cow milk, and meat as well as the risks of exceeding by the values the permissible levels have been calculated. The possibility of using the land for the production of milk and meat has been shown in the example of the considered radioactively contaminated pastures.","PeriodicalId":42588,"journal":{"name":"Nuclear Physics and Atomic Energy","volume":null,"pages":null},"PeriodicalIF":0.3,"publicationDate":"2022-03-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"78771409","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Cytogenetic studies of Myodes glareolus from the natural populations of the Chornobyl Exclusion Zone in the remote post-accident period 核事故后遥远时期切尔诺贝利隔离区自然种群中光柔米德的细胞遗传学研究
IF 0.3 Q4 Physics and Astronomy Pub Date : 2022-03-25 DOI: 10.15407/jnpae2022.01.039
N. M. Riabchenko, O. Burdo, A. Lypska
The results of cytogenetic studies of bank voles (Myodes glareolus) carried out during 2009 - 2016 in the areas of the Chornobyl Exclusion Zone with different levels of radionuclide contamination are presented. In the remote period after the Chornobyl accident features of chromosomal instability in somatic cells of examined animals, manifested as elevated levels of bone marrow cells with micronuclei, are observed. Probably, they can be caused by transgenerational radiation-induced chromosomal instability and changes in the ecological characteristics of the population under the combined impact of chronic low-intensity radiation and negative environmental factors.
本文介绍了2009年至2016年在放射性核素污染程度不同的切尔诺贝利隔离区开展的银行田鼠(Myodes glareolus)细胞遗传学研究的结果。在切尔诺贝利事故发生后的较长时期内,观察到受检动物体细胞的染色体不稳定特征,表现为带有微核的骨髓细胞水平升高。这可能是由于在慢性低强度辐射和负面环境因素共同作用下,辐射引起的跨代染色体不稳定性和种群生态特征的变化所引起的。
{"title":"Cytogenetic studies of Myodes glareolus from the natural populations of the Chornobyl Exclusion Zone in the remote post-accident period","authors":"N. M. Riabchenko, O. Burdo, A. Lypska","doi":"10.15407/jnpae2022.01.039","DOIUrl":"https://doi.org/10.15407/jnpae2022.01.039","url":null,"abstract":"The results of cytogenetic studies of bank voles (Myodes glareolus) carried out during 2009 - 2016 in the areas of the Chornobyl Exclusion Zone with different levels of radionuclide contamination are presented. In the remote period after the Chornobyl accident features of chromosomal instability in somatic cells of examined animals, manifested as elevated levels of bone marrow cells with micronuclei, are observed. Probably, they can be caused by transgenerational radiation-induced chromosomal instability and changes in the ecological characteristics of the population under the combined impact of chronic low-intensity radiation and negative environmental factors.","PeriodicalId":42588,"journal":{"name":"Nuclear Physics and Atomic Energy","volume":null,"pages":null},"PeriodicalIF":0.3,"publicationDate":"2022-03-25","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"86113149","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":0,"RegionCategory":"","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 1
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Nuclear Physics and Atomic Energy
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