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Development of high intensity neutron source at the European Spallation Source 高强度中子源在欧洲散裂源的发展
IF 1.1 Q3 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2020-02-10 DOI: 10.3233/jnr-200159
V. Santoro, K. Andersen, D. Dijulio, E. Klinkby, T. Miller, D. Milstead, G. Muhrer, M.Stroble, A. Takibayev, L. Zanini, O. Zimmer
The European Spallation Source being constructed in Lund, Sweden will provide the user community with a neutron source of unprecedented brightness. By 2025, a suite of 15 instruments will be served by a high-brightness moderator system placed above the spallation target. The ESS infrastructure, consisting of the proton linac, the target station, and the instrument halls, allows for implementation of a second source below the spallation target. We propose to develop a second neutron source with a high-intensity moderator able to (1) deliver a larger total cold neutron flux, (2) provide high intensities at longer wavelengths in the spectral regions of Cold (4–10 Å), Very Cold (10–40 Å), and Ultra Cold (several 100 Å) neutrons, as opposed to Thermal and Cold neutrons delivered by the top moderator. Offering both unprecedented brilliance, flux, and spectral range in a single facility, this upgrade will make ESS the most versatile neutron source in the world and will further strengthen the leadership of Europe in neutron science. The new source will boost several areas of condensed matter research such as imaging and spin-echo, and will provide outstanding opportunities in fundamental physics investigations of the laws of nature at a precision unattainable anywhere else. At the heart of the proposed system is a volumetric liquid deuterium moderator. Based on proven technology, its performance will be optimized in a detailed engineering study. This moderator will be complemented by secondary sources to provide intense beams of Very- and Ultra-Cold Neutrons.
正在瑞典隆德建造的欧洲散裂源将为用户社区提供前所未有的亮度中子源。到2025年,一套由15台仪器组成的高亮度慢化剂系统将被放置在散裂目标上方。ESS基础设施由质子直线加速器、目标站和仪器大厅组成,允许在散裂目标下方实施第二个源。我们建议开发一种具有高强度慢化剂的第二中子源,它能够(1)提供更大的总冷中子通量,(2)在冷(4-10 Å)、极冷(10-40 Å)和超冷(100 Å)中子的光谱区域提供波长更长的高强度,而不是由顶部慢化剂提供的热中子和冷中子。在单一设施中提供前所未有的亮度,通量和光谱范围,这次升级将使ESS成为世界上最通用的中子源,并将进一步加强欧洲在中子科学方面的领导地位。新的光源将促进凝聚态物质研究的几个领域,如成像和自旋回波,并将为自然规律的基础物理研究提供杰出的机会,其精度在其他任何地方都无法实现。该系统的核心是体积液态氘慢化剂。基于成熟的技术,将在详细的工程研究中优化其性能。这个慢化剂将由次级源补充,以提供极冷和超冷中子的强束。
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引用次数: 13
Routines for optimizing neutron scattering instruments with McStas 用McStas优化中子散射仪器的例程
IF 1.1 Q3 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2020-01-29 DOI: 10.3233/jnr-190117
V. Laliena, M. V. Alvarez, J. D. Campo
We acknowledge Grant No. PGC-2018-099024-B-I00 from Spanish Ministry of Science Innovation and Universities and funding from the project I-COOP B20319. This work was performed within the world class Science and Innovation with Neutrons in Europe 2020 (“SINE2020”) project, funded by the European Union’s Horizon 2020 research and innovation programme under grant agreement No. 654000.
我们确认第PGC-2018-099024-B-I00由西班牙科学创新和大学部资助,项目资金来自I-COOP B20319。这项工作是在欧洲2020年世界级中子科学与创新(“SINE2020”)项目中进行的,该项目由欧盟地平线2020研究与创新计划资助,资助协议号为654000。
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引用次数: 2
Advances in the use of Paris-Edinburgh presses for high pressure neutron scattering 利用巴黎-爱丁堡压机进行高压中子散射的进展
IF 1.1 Q3 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2020-01-29 DOI: 10.3233/jnr-190120
S. Klotz, T. Hansen, E. Lelièvre-Berna, L. Amand, J. Maurice, C. Payre
Paris-Edinburgh (PE) presses are nowadays the dominant high pressure devices for neutron scattering in the 10 GPa range and above. Here, we present developments of gasket-anvil assemblies with 30% improved pressure performance and considerably increased lifetime compared to the currently used “single-toroidal” anvils, and giving nevertheless a similar signal-to-background ratio. We also present an improved Bridgman seal package which makes the low-temperature operation of the PE press significantly more reliable. A systematic investigation of background sources in the “equatorial” scattering geometry is reported.
巴黎-爱丁堡(PE)压机是目前用于10GPa及以上范围中子散射的主要高压设备。在这里,我们介绍了垫圈砧座组件的发展,与目前使用的“单环面”砧座相比,该组件的压力性能提高了30%,使用寿命显著延长,但仍给出了类似的信号与背景比。我们还提供了一种改进的Bridgman密封包装,使PE压机的低温运行更加可靠。报道了对“赤道”散射几何中背景源的系统研究。
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引用次数: 6
An introduction to SECoP – the sample environment communication protocol 介绍SECoP -示例环境通信协议
IF 1.1 Q3 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2020-01-29 DOI: 10.3233/jnr-190143
K. Kiefer, L. Rossa, Frank Wutzler, Niklas Ektröm, Anders Pettersson, E. Faulhaber, Markus Zolliker
. The Sample Environment Communication Protocol (SECoP) serves as an international standard for the communication between sample environment equipment and the experiment control software at neutron and photon sources. It eases the integration of sample environment equipment supplied by external research groups and by industrial manufacturers. SECoP is designed to be simple, inclusive and self-describing. SECoP facilitates and structures the provision of metadata which is associated with sample environment equipment. Several existing implementations of SECoP support the development of SECoP-compatible sample environment control software. This article intro- duces SECoP Version 1.0, the first official version of SECoP published in September 2019. It was developed during the SINE2020 project in close cooperation with the International Society for Sample Environment. The complete specifications of SECoP Version 1.0 are available on GitHub.
样品环境通信协议(SECoP)用作中子源和光子源处的样品环境设备与实验控制软件之间的通信的国际标准。它简化了外部研究小组和工业制造商提供的样品环境设备的集成。SECoP被设计为简单、包容和自我描述。SECoP促进并构建与样本环境设备相关联的元数据的提供。SECoP的几个现有实现支持SECoP兼容的样本环境控制软件的开发。本文介绍了SECoP 1.0版,这是SECoP于2019年9月发布的第一个官方版本。它是在SINE2020项目期间与国际样品环境学会密切合作开发的。SECoP 1.0版的完整规范可在GitHub上获得。
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引用次数: 2
A fast-cooling mode for blue series furnaces 蓝色系列炉的快速冷却模式
IF 1.1 Q3 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2020-01-29 DOI: 10.3233/jnr-190128
C. Goodway, P. Mcintyre, A. Sears, Nadir Belkhier, G. Burgess, O. Kirichek, E. Lelièvre-Berna, F. Marchal, Sébastien Turc, S. Wakefield
Blue series top-loading furnaces are regularly used at neutron facilities to carry out experiments at up to 1700◦C. The sample temperature is controlled using the indirect resistance heating method which consists in placing the sample inside a radiating cylindrical heater made from vanadium or niobium into which a current of up to 180 A circulates. To prevent the oxydation and deterioration of the heated elements, the sample, the heater and the heat shields are in a secondary vacuum which limits very much the cooling rate. We present an automated fast-cooling technique which reduces the cool-down time by a factor of 4 to 5 without impacting the lifetime of the heated elements. This method is now routinely used at the ILL and ISIS facilities and reduces very much beam time losses.
蓝色系列顶载炉通常用于中子设施,以进行高达1700◦C的实验。使用间接电阻加热方法控制样品温度,该方法包括将样品放入由钒或铌制成的辐射圆柱形加热器中,其中高达180 a的电流循环。为了防止被加热元件的氧化和变质,样品、加热器和隔热罩处于二级真空中,这极大地限制了冷却速度。我们提出了一种自动快速冷却技术,该技术将冷却时间减少了4到5倍,而不会影响被加热元件的寿命。这种方法现在在ILL和ISIS设施中经常使用,并大大减少了波束时间损失。
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引用次数: 0
Next generation equipment for muon chemistry research 下一代介子化学研究设备
IF 1.1 Q3 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2020-01-29 DOI: 10.3233/jnr-190118
M. Aramini, S. Cottrell, J. Peck, K. Yokoyama
Muon spectroscopy offers a uniquely sensitive method for exploring many mechanisms in chemistry and chemical physics through the study of muonium, a probe species formed during muon implantation that is chemically equivalent to hydrogen. Next generation experiments in the field of muonium chemistry will require reliable liquid handling systems, in-situ experimental capabilities and access to advanced methods such as Radio-Frequency (RF) muon spin resonance spectroscopy. This paper discusses the development and commissioning of systems for sample handling, describing details of two liquid panels suitable for deoxygenation and transfer of liquid samples, the development of a centre stick for an existing 4He flow cryostat suitable for RF muon chemistry experiments, a dedicated muon chemistry insert specifically optimized for RF liquid phase chemistry experiments, and a birdcage RF cavity optimized for high frequency measurements and with a geometry wellsuited for beamline experiments that exploit the chemistry insert. Example data is presented, demonstrating the application of these various pieces of equipment.
μ子光谱学通过对μ子离子的研究,为探索化学和化学物理中的许多机制提供了一种独特的灵敏方法。μ子离子是在μ子注入过程中形成的一种探针物质,化学上相当于氢。子化学领域的下一代实验将需要可靠的液体处理系统、现场实验能力和先进的方法,如射频(RF) μ子自旋共振光谱。本文讨论了样品处理系统的开发和调试,描述了适用于液体样品的除氧和转移的两个液体面板的细节,适用于射频μ子化学实验的现有4He流低温恒温器的中心棒的开发,专门针对射频液相化学实验优化的专用μ子化学插入,以及针对高频测量进行优化的鸟笼式射频腔,其几何形状非常适合利用化学插入的光束线实验。给出了实例数据,说明了这些设备的应用情况。
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引用次数: 1
Neutron activation properties of PE-B4C-concrete assessed by measurements and simulations 通过测量和模拟评价pe - b4c混凝土的中子活化性能
IF 1.1 Q3 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2020-01-29 DOI: 10.3233/jnr-190126
D. Hajdú, E. Dian, E. Klinkby, C. Cooper-Jensen, J. Osán, P. Zagyvai
The neutron activation properties of the PE-B4C-concrete recently developed for the European Spallation Source (ESS) ERIC (European Spallation Source, https://europeanspallationsource.se/about) were investigated. On the one hand the concrete activation was compared to that of the ordinary concrete from which it was developed by means of irradiating concrete samples in the Budapest Research Reactor (BRR) (Budapest Neutron Centre, https://www.bnc.hu/). On the other hand, the measured activities were used to study the impact of input composition on Monte Carlo activation simulations. For this purpose, the complete course of the irradiation experiments were reproduced with MCNPX and Cinder90 simulations with nominal and measured elemental concrete compositions. Simulations suggest that for realistic activation predictions more detailed elemental compositions are required than the nominal ones. Energy-dispersive X-ray fluorescence (EDXRF) analysis technique was applied for this purpose, providing fair results for short-term activation estimations.
研究了新研制的用于欧洲散裂源(ESS) ERIC (European Spallation Source, https://europeanspallationsource.se/about)的pe - b4c混凝土的中子活化性能。一方面,混凝土活化与普通混凝土的活化进行了比较,普通混凝土是通过布达佩斯研究反应堆(BRR)(布达佩斯中子中心,https://www.bnc.hu/)中的辐照混凝土样品开发的。另一方面,测量的活度用于研究输入成分对蒙特卡罗激活模拟的影响。为此,用MCNPX和Cinder90模拟模拟了名义和实测混凝土元素成分,再现了辐照实验的完整过程。模拟表明,对于实际的活化预测,需要比名义上的更详细的元素组成。为此应用了能量色散x射线荧光(EDXRF)分析技术,为短期激活估计提供了公平的结果。
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引用次数: 4
Low-background materials for high pressure cells used in inelastic neutron scattering experiments 用于非弹性中子散射实验的高压电池的低本底材料
IF 1.1 Q3 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2020-01-29 DOI: 10.3233/jnr-190115
M. Kibble, V. Laliena, C. Goodway, E. Lelièvre-Berna, K. Kamenev, S. Klotz, O. Kirichek
This work was performed within the world class Science and Innovation with Neutrons in Europe 2020 (“SINE 2020”) project, funded by the European Commission, Grant Agreement n°654000.
这项工作是在欧洲委员会资助的世界级中子科学与创新2020(“sin2020”)项目中进行的,资助协议n°654000。
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引用次数: 3
Coupling NMR to SANS: Addressing at once structure and dynamics in soft matter 核磁共振与SANS的耦合:同时解决软物质的结构和动力学问题
IF 1.1 Q3 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2020-01-29 DOI: 10.3233/jnr-190114
R. Oliveira-Silva, Agathe Belime, Clémence Le Coeur, Alexis Chennevière, A. Hélary, F. Cousin, P. Judeinstein, D. Sakellariou, J. Zanotti
. In soft condensed matter, Small Angle Neutron Scattering (SANS) is a central tool to probe structures with characteristic sizes ranging from 1 to 100 nm. However, when used as a standalone technique, the dynamic properties of the sample are not accessible. Nuclear Magnetic Resonance (NMR) is a versatile technique which can easily probe dynamical information. Here, we report on the coupling of a low-field NMR system to a SANS instrument. We show that this original set-up makes it possible to obtain structural information and to simultaneously extract in situ on a same sample, long-range translational diffusion coefficient, T 1 and T 2 nuclear spin relaxation times. Such a feature is of major interest when a sample experiences a transient physical state or evolves rapidly. We illustrate the capabilities of alliancing these experimental methods by following the critical temperature-induced phase separation of a concentrated Poly(Methacrylic Acid) solution at its Lower Critical Solution Temperature. The characteristic size related to the domain growth of the polymer-rich phase of the gel is monitored by the evolution of the SANS spectra, while the dynamics of the sol phase (H 2 O and polymer) is simultaneously characterized by NMR by measuring T 1 , T 2 and the diffusion coefficient. Great care has been taken to design a cell able to optimize the thermalization of the sample and in particular its equilibration time. Details are given on the sample cell specifically designed and manufactured for these experiments. The acquisition time needed to reach good signal-to-noise ratios, for both NMR and SANS, match: it is of the order of one hour. Altogether, we show that in situ low-field NMR/SANS coupling the NMR is meaningful and is a promising experimental approach.
. 在软凝聚态物质中,小角中子散射(SANS)是探测特征尺寸从1到100 nm的结构的核心工具。然而,当作为一个独立的技术使用时,样本的动态属性是不可访问的。核磁共振(NMR)是一种可以方便地探测动态信息的通用技术。在这里,我们报告了低场核磁共振系统与SANS仪器的耦合。我们表明,这种原始设置使得获得结构信息成为可能,并同时在同一样品上原位提取,远程平移扩散系数,t1和t2核自旋弛豫时间。当样品经历短暂的物理状态或快速演变时,这样的特征是主要的兴趣。我们通过在较低的临界溶液温度下对浓聚(甲基丙烯酸)溶液进行临界温度诱导的相分离,说明了将这些实验方法结合起来的能力。通过SANS光谱的演变监测凝胶富聚合物相的畴生长特征尺寸,同时通过核磁共振测量t1, t2和扩散系数来表征溶胶相(h2o和聚合物)的动力学。设计一个能够优化样品的热化,特别是其平衡时间的电池是非常小心的。详细介绍了为这些实验专门设计和制造的样品池。对于NMR和SANS而言,达到良好信噪比所需的采集时间是匹配的:大约是一小时。总之,我们证明了原位低场核磁共振/SANS耦合核磁共振是有意义的,是一种有前途的实验方法。
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引用次数: 2
Semi-analytical calculations of intrinsic field magnetic field inhomogeneities for a Neutron Spin Echo spectrometer at the ESS ESS中子自旋回波光谱仪本征场磁场不均匀性的半解析计算
IF 1.1 Q3 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2020-01-29 DOI: 10.3233/jnr-190121
A. Kusmin, C. Pappas
Neutron Spin Echo methods (NSE) use Larmor labelling to measure the precession phase of the neutron beam polarization around well-defined magnetic fields. Scattering by a sample can affect the resulting precession phase providing information on the sample's structure and dynamics with high accuracy and resolution. A major limitation for the performance of Neutron Spin Echo instruments is the homogeneity of the precession magnetic fields. Here we investigate the influence of the new 'pancake' moderator, which is being built at the European Spallation Source, on the design of a Neutron Spin Echo spectrometer. The calculations show clear gains when the height to width ratios of the rectangular beam cross-sections mimic those of the ESS 'pancake' moderator beams. In such a case the homogeneity of the magnetic field integrals could improve by at least 30%. However, the calculations show that will not be possible to preserve a high resolution and at the same time reduce the length of the instrument. Consequently, NSE spectrometers will perform better at the ESS but they will not be substantially compacter than at other neutron sources e.g. ILL or FRM2.
中子自旋回波方法(NSE)使用拉莫尔标记来测量在明确定义的磁场周围中子束极化的进动相位。样品的散射可以影响所产生的进动相位,从而以高精度和高分辨率提供关于样品的结构和动力学的信息。中子自旋回波仪器性能的一个主要限制是进动磁场的均匀性。在这里,我们研究了欧洲散裂源正在建造的新型“煎饼”慢化剂对中子自旋回波光谱仪设计的影响。当矩形梁横截面的高宽比模拟ESS“煎饼”减速梁时,计算显示出明显的增益。在这种情况下,磁场积分的均匀性可以提高至少30%。然而,计算表明,这将不可能在保持高分辨率的同时减少仪器的长度。因此,NSE光谱仪将在ESS处表现更好,但它们不会比在其他中子源(如ILL或FRM2)处更紧凑。
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引用次数: 0
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Journal of Neutron Research
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