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High-resolution HO2 radical detection by optical feedback linear cavity-enhanced absorption spectroscopy 利用光反馈线性空腔增强吸收光谱法进行高分辨率 HO2 自由基检测
IF 2 3区 物理与天体物理 Q3 OPTICS Pub Date : 2024-07-24 DOI: 10.1007/s00340-024-08283-0
Yang Chen, Nana Yang, Bo Fang, Weixiong Zhao, Weijun Zhang, Shuangshuang Li, Weihua Cui

We report the development of an optical feedback linear cavity-enhanced absorption spectroscopy instrument for HO2 detection using a distributed feedback (DFB) diode laser operating at 1506 nm. A direct and accurate method of reflectivity measurement based on the analysis of cavity mode signals was proposed. A differential circuit was used to judge the zero crossing point of the optical feedback cavity mode in the center of the frequency locking region, and shift the laser operating current to the non-resonant region. In this way, a ring-down signal was obtained with a time of 17.9 μs, corresponding to an effective absorption pathlength of 5.37 km. Combining the standing wave condition, the relationship between cavity length and drive voltage of the PZT mounted on the cavity rear mirror is translated into a correlation between the transmitted light wavenumber and the PZT voltage. The spectral resolution was improved from 290 MHz to 97 MHz by precisely tuning the PZT voltage. The achieved detection sensitivity of the system was 7 × 10− 10 cm− 1 with a data acquisition time of 10.6 s. The absorption spectrum of HO2 at 6638.205 cm− 1 was measured at a cell pressure of 50 mbar with a detection limit of 3.24 × 109 molecule/cm3.

我们报告了利用波长为 1506 nm 的分布式反馈 (DFB) 二极管激光器开发的用于检测 HO2 的光反馈线性空穴增强吸收光谱仪器。我们提出了一种基于空腔模式信号分析的直接而精确的反射率测量方法。利用差分电路来判断位于频率锁定区域中心的光反馈空腔模式的过零点,并将激光工作电流转移到非谐振区域。通过这种方法,获得了时间为 17.9 μs 的环降信号,对应的有效吸收路径长度为 5.37 km。结合驻波条件,空腔长度与安装在空腔后反射镜上的 PZT 驱动电压之间的关系转化为透射光波长与 PZT 电压之间的相关性。通过精确调节 PZT 电压,光谱分辨率从 290 MHz 提高到 97 MHz。该系统的检测灵敏度为 7 × 10- 10 cm- 1,数据采集时间为 10.6 秒。在样品池压力为 50 毫巴时,在 6638.205 cm- 1 处测量了 HO2 的吸收光谱,检测限为 3.24 × 109 个分子/立方厘米。
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引用次数: 0
2.53 W of 261 nm continuous wave generation in a pr: YLF laser pumped by blue laser diode at 444.2 nm 在波长为 444.2 纳米的蓝色激光二极管泵浦的pr: YLF 激光器中产生 2.53 W 的 261 纳米连续波
IF 2 3区 物理与天体物理 Q3 OPTICS Pub Date : 2024-07-24 DOI: 10.1007/s00340-024-08281-2
Yi Yao, Quan Zheng,  XiChen, Jinyan Wang, Huidong Xiao, Yan Wang, Yuning Wang, Huizhen Liu, Donghe Tian
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引用次数: 0
Gas detection using cavity-enhanced Raman spectroscopy with a bidirectional multi-pass cell and polarization beam-splitting optical path 利用带有双向多通室和偏振分束光路的空腔增强拉曼光谱进行气体检测
IF 2 3区 物理与天体物理 Q3 OPTICS Pub Date : 2024-07-24 DOI: 10.1007/s00340-024-08285-y
Yuhao Zheng, Xiaer Zou, Sailing He

We demonstrate a substantial enhancement of gas Raman scattering using a bidirectional multi-pass cavity CERS system, which incorporates a polarization beam-splitting optical path. The system design allows the laser light to traverse the multi-pass cavity for four specific trips, satisfying the need for quick detection of various gas components. Our gas detection experiments using multi-pass cavities with different times of reflection indicate that the addition of polarization beam-splitting optical path gives 1.5 to 1.68 times enhancement of Raman signal compared with that of the system without polarization beam-splitting. For the detection of CH4, a limit of detection of 1.66 ppm was achieved with our system using a multi-pass cell with 41 times of reflection and an integration time of 30s. Our proposed design, which integrates a bidirectional multi-pass cavity with polarization beam-splitting optical path, gives an economical multicomponent gas detection system and a valuable tool for guiding the design and precise alignment of these cavities. This system shows significant promise for applications in e.g. human breath and environmental monitoring.

我们利用双向多通腔 CERS 系统演示了气体拉曼散射的大幅增强,该系统采用了偏振分束光路。该系统的设计允许激光在多通腔中进行四次特定的穿越,从而满足了快速检测各种气体成分的需要。我们使用不同反射时间的多通腔进行的气体检测实验表明,与没有偏振分束的系统相比,增加偏振分束光路可使拉曼信号增强 1.5 至 1.68 倍。在检测 CH4 时,我们的系统使用了一个反射次数为 41 次、积分时间为 30 秒的多通单元,检测限达到了 1.66 ppm。我们提出的设计方案将双向多通腔与偏振分光光路集成在一起,提供了一种经济的多组分气体检测系统,同时也是指导这些腔体的设计和精确对准的重要工具。该系统在人体呼吸和环境监测等方面的应用前景广阔。
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引用次数: 0
Wavelength optimization of space-borne electro-optic dual-comb lidar for CO2 detection at 1572 nm 用于 1572 nm 波长二氧化碳探测的星载电光双梳状激光雷达的波长优化
IF 2 3区 物理与天体物理 Q3 OPTICS Pub Date : 2024-07-24 DOI: 10.1007/s00340-024-08286-x
Zheng Liu, Tengteng Xia, Xiaopeng Zhu, Juxin Yang, Jiqiao Liu, Weibiao Chen

The space-borne Integrated Path Differential Absorption (IPDA) lidar can measure the global distribution of CO2. Here, we simulate measurements on the R16 absorption line employing a 1572 nm electro-optic dual-comb interferometer. We introduce a comprehensive modeling and retrieval framework to assess the lidar’s capability in measuring the column-averaged of CO2 in the atmosphere. The assessment combines data simulation with linearization error analysis to solve the nonlinearity in retrieval. Our findings suggest that positioning any sampling wavelength at the absorption peak will significantly increase the random error by about 30%. The lidar can operate with an optimal wavelength strategy where the wavelength bias has virtually no effect, but it must still account for the effects of atmospheric temperature and pressure. We performed a comprehensive global evaluation using geophysical data, comparing results across 3 to 17 wavelengths. Distributing 20 W launched power over 11 wavelengths enables measurement with an error below 0.9 ppm over most of the Earth’s surface.

星载综合路径差分吸收(IPDA)激光雷达可以测量二氧化碳的全球分布。在这里,我们利用 1572 nm 的电光双梳束干涉仪模拟了对 R16 吸收线的测量。我们引入了一个综合建模和检索框架,以评估激光雷达测量大气中二氧化碳柱平均值的能力。评估结合了数据模拟和线性化误差分析,以解决检索中的非线性问题。我们的研究结果表明,将任何采样波长定位在吸收峰值都会使随机误差显著增加约 30%。激光雷达可以采用最佳波长策略,在这种情况下,波长偏差几乎没有影响,但仍必须考虑大气温度和压力的影响。我们利用地球物理数据进行了全面的全球评估,比较了 3 到 17 个波长的结果。将 20 W 发射功率分布在 11 个波长上,可对地球表面大部分区域进行误差低于 0.9 ppm 的测量。
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引用次数: 0
Efficient control of three-dimensional atom localization via probe absorption in a phase-coherent atomic medium 通过相干原子介质中的探针吸收有效控制三维原子定位
IF 2 3区 物理与天体物理 Q3 OPTICS Pub Date : 2024-07-20 DOI: 10.1007/s00340-024-08278-x
Aniket Banerjee, Pradipta Panchadhyayee, Bibhas Kumar Dutta

We propose a new scheme for the study of three-dimensional (3D) atom localization by observing spatially modulated absorption of a weak probe field operating in a multi-wave-mixing induced four-level atomic system. The field-coupled atomic model can be envisaged as a closed-loop double-lambda configuration. By controlling Rabi frequency, detuning, and field-induced collective phase-coherence, different spatial structures of localization patterns are presented with a variety of standing wave field configurations. Our results highlight that 100% detection probability of atom is possible in the present model in many ways with high-precision measurement of spatial absorption. It has been shown that position information of the atom with maximum detection probability can be efficiently controlled by employing a travelling-wave field in association with the standing wave fields in the system. For a specific field configuration, the maximum detection probability of finding the atom can be obtained with a limit of spatial resolution better than (lambda)/40 in our model. The efficacy of the present model is to find its applications in quantum information processing in the near future.

我们提出了一种研究三维(3D)原子定位的新方案,通过观察在多波混合诱导的四级原子系统中运行的弱探针场的空间调制吸收。场耦合原子模型可以设想为闭环双蓝斑配置。通过控制拉比频率、失谐和场诱导的集体相干性,不同空间结构的定位模式在各种驻波场配置下呈现出来。我们的研究结果表明,在目前的模型中,通过高精度测量空间吸收,原子的 100% 检测概率是可能的。研究表明,通过在系统中采用与驻波场相关联的行波场,可以有效地控制原子的位置信息,从而获得最大探测概率。对于特定的场配置,在我们的模型中,可以获得空间分辨率优于 (lambda)/40 的最大原子探测概率。本模型的功效将在不久的将来应用于量子信息处理。
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引用次数: 0
Resonant wavelengths of whispering gallery modes in dispersive materials 色散材料中耳语廊模式的共振波长
IF 2 3区 物理与天体物理 Q3 OPTICS Pub Date : 2024-07-20 DOI: 10.1007/s00340-024-08282-1
Lorena Velazquez-Ibarra, Juan Barranco

In this work we compute the resonant wavelengths of whispering gallery modes for bulk-fused silica microspheres taking into consideration the material chromatic dispersion. This is done by following two approaches: solving the exact characteristic equation and solving the nonlinear equations that result from the asymptotic approximations for a wavelength-dependent refractive index. Similar results with both methods are obtained with differences below 1%. Nevertheless, important differences are found between the resonant wavelengths computed for a non-dispersive and a dispersive material. We compute the free spectral range and the quality factor, and make a comparison between the variable index and the constant index cases. Our results show that the quality factor is unaffected by chromatic dispersion. However, there are differences of significant relevance in the case of the free spectral range. Our work could be useful as a pathway for designing microspheres for different applications.

在这项工作中,我们计算了块状熔融石英微球的耳语画廊模式共振波长,并考虑了材料色散。计算方法有两种:一是求解精确的特征方程,二是求解由波长相关折射率的渐近近似所产生的非线性方程。两种方法得到的结果相似,差异低于 1%。然而,在计算非色散材料和色散材料的共振波长时,发现两者之间存在很大差异。我们计算了自由光谱范围和品质因数,并对可变折射率和恒定折射率情况进行了比较。结果表明,品质因数不受色散的影响。然而,在自由光谱范围的情况下,两者之间存在着显著的相关性差异。我们的研究成果可作为设计不同用途微球的有用途径。
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引用次数: 0
Effects of discharge tube and coolant materials on longitudinally excited CO2 laser with fast pulsed discharge 放电管和冷却剂材料对纵向激励二氧化碳激光器快速脉冲放电的影响
IF 2 3区 物理与天体物理 Q3 OPTICS Pub Date : 2024-07-17 DOI: 10.1007/s00340-024-08277-y
Yasushi Kodama, Shohei Watarai, Kazuyuki Uno

In diffusion-cooled gas lasers, the laser medium gas is cooled through the discharge tube wall. Empirical findings suggest that, in longitudinally excited CO2 lasers with fast pulsed discharges, the materials of the discharge tube and coolant impact the discharge. This study investigates their effects on fast discharges rather than on cooling. Within a discharge tube with a cooling tube, the discharge tube and coolant create a capacitor, influencing the discharge. The laser output energy varies based on the discharge tube and coolant materials. The primary discharge input energy is influenced by these materials, as is the efficiency of converting it into laser output energy.

在扩散冷却气体激光器中,激光介质气体是通过放电管壁冷却的。经验研究结果表明,在纵向激励的二氧化碳激光器中,快速脉冲放电时,放电管和冷却剂的材料会对放电产生影响。本研究调查的是它们对快速放电的影响,而不是对冷却的影响。在带有冷却管的放电管内,放电管和冷却剂会形成一个电容器,对放电产生影响。激光输出能量因放电管和冷却剂材料而异。原放电输入能量受这些材料的影响,而将其转换为激光输出能量的效率也受这些材料的影响。
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引用次数: 0
Z-scan technique: a review from conventional Z-scan to white light Z-scan Z 扫描技术:从传统 Z 扫描到白光 Z 扫描的综述
IF 2 3区 物理与天体物理 Q3 OPTICS Pub Date : 2024-07-14 DOI: 10.1007/s00340-024-08262-5
Aliasghar Ajami, Aleksandr Ovsianikov, Robert Liska, Stefan Baudis

Nonlinear (NL) absorption and refraction are crucial optical phenomena in the development and application of optical materials. The Z-scan technique, first proposed by Bahae, is widely used to accurately measure the coefficients of NL absorption and refraction. This review presents a comprehensive overview of the most established versions of the Z-scan technique, including the transmittance closed aperture (CA) and open aperture (OA) Z-scan, reflecting CA and OA Z-scan, eclipsing Z-scan, and white light Z-scan. In each version, different sources with varying spatial and temporal intensity distributions are usually utilized. Numerical and analytical calculation results are provided for each version considering both continuous wave (CW) and pulsed laser sources. Unlike conventional reviews, which often summarize previously published results, this review primarily focuses on reproducing the findings from the literature. The analytical results, which are typically derived under specific approximations, are compared with numerical calculations to highlight the limitations of analytically derived relations. Furthermore, the necessary criteria and conditions for applying each Z-scan version are discussed.

非线性(NL)吸收和折射是光学材料开发和应用中的关键光学现象。由 Bahae 首次提出的 Z 扫描技术被广泛用于精确测量非线性吸收和折射系数。本综述全面概述了最成熟的 Z 扫描技术版本,包括透射闭孔 (CA) 和开孔 (OA) Z 扫描、反射 CA 和 OA Z 扫描、日蚀 Z 扫描和白光 Z 扫描。在每个版本中,通常会使用具有不同空间和时间强度分布的不同光源。考虑到连续波(CW)和脉冲激光源,每个版本都提供了数值和分析计算结果。传统的综述通常是对以前发表的结果进行总结,与此不同,本综述主要侧重于再现文献中的研究结果。分析结果通常是在特定近似条件下得出的,本综述将分析结果与数值计算结果进行比较,以突出分析得出的关系的局限性。此外,还讨论了应用每种 Z 扫描版本的必要标准和条件。
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引用次数: 0
Birefringence changes induced by thermal cycling in lithium niobate 铌酸锂热循环引起的双折射变化
IF 2 3区 物理与天体物理 Q3 OPTICS Pub Date : 2024-07-12 DOI: 10.1007/s00340-024-08276-z
Dieter H. Jundt, Matthew T. Whittaker

Lithium niobate exhibits slow refractive index drift after temperature excursions typical in device manufacturing. Such drift can degrade performance in certain devices. We analyze the birefringence changes in a range of temperatures to measure the magnitude and rate of change. Experiments were conducted by first annealing congruently grown, magnesium doped, and lithium-enriched crystals at a temperatures between 95 and 215 (^circ)C. Subsequent optical evaluation was performed between 95 and 122 (^circ)C using a table-top apparatus. The sample was illuminated with incandescent polarized light and transmitted light was collected with a compact spectrometer after passing through an analyzer so fringes could be recorded. Careful fringe analysis allows a precise estimate of birefringence changes at a reference wavelength with precision (<10^{-6}). The observed birefringence changes can be explained by assuming that existing lithium vacancies re-arrange around positively charged point defects via lithium vacancy migration. Computer simulations for a simple model reproduce the major observations such as magnitude of change, activation energy for relaxation and the stretched exponential nature of the change. Similar effects are expected in lithium tantalate and the results suggest ways to minimize the influence on device operation.

铌酸锂在设备制造过程中出现典型的温度偏移后,会表现出缓慢的折射率漂移。这种漂移会降低某些器件的性能。我们分析了一系列温度下的双折射变化,以测量变化的幅度和速率。实验是通过在 95 到 215 (^circ)C 之间的温度下首先对一致生长、掺镁和富锂晶体进行退火。随后使用台式仪器在 95 到 122 摄氏度之间进行光学评估。样品用白炽偏振光照明,透射光通过分析仪后用紧凑型光谱仪收集,以便记录条纹。通过仔细的条纹分析,可以精确地估算出参考波长处的双折射变化,精度为(<10^{-6})。假设现有的锂空位通过锂空位迁移在带正电的点缺陷周围重新排列,就可以解释观察到的双折射变化。一个简单模型的计算机模拟再现了主要的观察结果,如变化幅度、弛豫活化能和变化的拉伸指数性质。预计在钽酸锂中也会产生类似的影响,研究结果提出了将对器件运行的影响降至最低的方法。
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引用次数: 0
The nonlinear absorption properties of TaSe2 and its application in ~ 2.0 µm pulsed solid-state lasers TaSe2 的非线性吸收特性及其在 ~ 2.0 µm 脉冲固体激光器中的应用
IF 2 3区 物理与天体物理 Q3 OPTICS Pub Date : 2024-07-12 DOI: 10.1007/s00340-024-08275-0
Lulu Dong, Mengxin Xue, Junting Liu, Kuan Li, Jiawen Lv, Yicheng Jin, Shande Liu

Enhancing the performance of saturable absorbers (SAs) crafted from two-dimensional (2D) narrow-bandgap materials is crucial for their use in ~ 2.0 µm pulse laser applications. In this context, a high-quality TaSe2 SA was successfully fabricated by mechanical exfoliation. The TaSe2 SA exhibited saturable absorption characteristics at around 2.0 μm, with a modulation depth of 7.1% and an unsaturated loss of 3.1%. Utilizing this newly fabricated SA, a passively Q-switched Tm:YAP laser operating near 2.0 μm was achieved. At the highest absorbed pump power of 5.58 W, the laser produced a maximum average output power of 1.34 W, with a pulse width measuring 550 ns at 89 kHz. This performance translates to a peak single pulse energy of 15.0 μJ and a maximum peak power of 27.27 W.

提高二维(2D)窄带隙材料制成的可饱和吸收体(SA)的性能,对于它们在 ~ 2.0 µm 脉冲激光应用中的应用至关重要。在此背景下,通过机械剥离法成功制造出了高质量的 TaSe2 SA。TaSe2 SA 在 2.0 μm 左右表现出可饱和吸收特性,调制深度为 7.1%,不饱和损耗为 3.1%。利用这种新制造的 SA,实现了工作在 2.0 μm 附近的无源 Q 开关 Tm:YAP 激光器。在最高吸收泵浦功率为 5.58 W 时,激光器产生的最大平均输出功率为 1.34 W,脉冲宽度为 550 ns,频率为 89 kHz。这一性能可转化为 15.0 μJ 的峰值单脉冲能量和 27.27 W 的最大峰值功率。
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引用次数: 0
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Applied Physics B
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