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Optical storage of circular airy beam in atomic vapor 原子蒸气中圆形空气光束的光学存储
Pub Date : 2024-05-15 DOI: 10.1088/1674-1056/ad4bbf
Hong Chang, Xin Yang, Yan Ma, Xin Yang, Mingtao Cao, Xiaofei Zhang, Ruifang Dong, Shougang Zhang
The realization of quantum storage of spatial light field is of great significance to the construction of high-dimensional quantum repeater. In this paper, we experimentally realize the storage and retrieval of circular airy beams (CABs) by using the Λ-type three-level energy system based on the electromagnetically induced transparency in a hot rubidium atomic vapor cell. The weak probe beam field is modulated with phase distribution of CABs by a spatial light modulator. We store the probe circular airy beam (CAB) into the rubidium atomic vapor cell and retrieve after the demanded delay. We quantitatively analyze the storage results and give corresponding theoretical explanations. Moreover, we investigate the autofocusing and self-healing effect of the retrieved CAB, which indicates that the properties and beam shape of CAB maintains well after storage. Our work will have potential applications in the storage of high-dimensional quantum information, and is also useful for improving the channel capacities of quantum internet.
实现空间光场的量子存储对构建高维量子中继器具有重要意义。本文利用基于热铷原子蒸气电池中电磁诱导透明的Λ型三电平能量系统,通过实验实现了环空光束(CAB)的存储和检索。弱探针光束场通过空间光调制器与 CAB 的相位分布进行调制。我们将探针环空光束(CAB)存储到铷原子蒸气电池中,并在要求的延迟后取出。我们对存储结果进行了定量分析,并给出了相应的理论解释。此外,我们还研究了取回的环空光束的自动聚焦和自愈效应,结果表明环空光束的特性和光束形状在存储后保持良好。我们的工作将在高维量子信息的存储中得到潜在应用,同时也有助于提高量子互联网的信道容量。
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引用次数: 0
Multi-objective-Global-Optimization-Approach Predicted Quasi-Layered Ternary TiOS Crystals with Promising Photocatalytic Properties 多目标全局优化方法预测出具有良好光催化性能的准层状三元 TiOS 晶体
Pub Date : 2024-05-15 DOI: 10.1088/1674-1056/ad4bc3
Yi-Jie Xiang, Siyan Gao, Chunlei Wang, Haiping Fang, Xiangmei Duan, Yi-Feng Zheng, Yue-Yu Zhang
Titanium dioxide (TiO2) has attracted considerable research attentions for its promising applications in solar cells and photocatalytic devices. However, the intrinsic challenge lies in the relatively low energy conversion efficiency of TiO2, primarily attributed to the substantial band gaps (exceeding 3.0 eV) associated with its rutile and anatase phases. Leveraging multi-objective global optimization, we have identified two quasi-layered ternary Ti-O-S crystals, composed of titanium, oxygen and sulfur. The calculations of formation energy, phonon dispersions, and thermal stability confirm the chemical, dynamical and thermal stability of these newly discovered phases. Employing the state-of-art hybrid density functional approach and many-body perturbation theory (quasiparticle GW approach and Bethe-Salpeter equation), we calculate the optical properties of both the TiOS phases. Significantly, both phases show favorable photocatalytic characteristics, featuring band gaps suitable for visible optical absorption and appropriate band alignments with water for effective charge carrier separation. Therefore, ternary compound TiOS hold the potential for achieving high-efficiency photochemical conversion, showing our multi-objective global optimization provides a new approach for novel environmental and energy materials design with multicomponent compounds.
二氧化钛(TiO2)在太阳能电池和光催化设备中的应用前景广阔,因此吸引了大量研究人员的关注。然而,其固有的挑战在于二氧化钛的能量转换效率相对较低,这主要归因于其金红石相和锐钛相具有较大的带隙(超过 3.0 eV)。利用多目标全局优化,我们确定了两种由钛、氧和硫组成的准层状三元钛-氧-硫晶体。对形成能、声子色散和热稳定性的计算证实了这些新发现相的化学、动力学和热稳定性。利用最先进的混合密度泛函方法和多体扰动理论(准粒子 GW 方法和 Bethe-Salpeter 方程),我们计算了这两种 TiOS 相的光学特性。值得注意的是,这两种相都显示出良好的光催化特性,具有适合可见光吸收的带隙,以及与水适当的带排列,可有效分离电荷载流子。因此,三元化合物 TiOS 具有实现高效光化学转换的潜力,这表明我们的多目标全局优化为使用多组分化合物设计新型环境和能源材料提供了一种新方法。
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引用次数: 0
Steering the energy sharing of electrons in nonsequential double ionization with orthogonally polarized two-color field 用正交偏振双色场引导非连续双电离中电子的能量共享
Pub Date : 2024-05-15 DOI: 10.1088/1674-1056/ad4bc0
Guangqi Fan, Zhijie Yang, Fenghao Sun, Jinmei Zheng, Yuntian Han, Mingqian Huang, Qingcao Liu
Using the semiclassical ensemble model, the dependence of relative amplitude for the recollision dynamics in nonsequential double ionization (NSDI) of neon atom driven by the orthogonally polarized two-color field (OTC) laser field was theoretically studied. And the dynamics in two typical collision pathways, recollision-impact-ionization (RII) and recollision-excitation with subsequent ionization (RESI) is systematically explored. Our results reveal that the V-shaped structure in the correlated momentum distribution is mainly caused by the RII mechanism when relative amplitude of OTC laser field is zero, and the first ionized electrons will quickly skim through the nucleus and share few energy with the second electron. As the relative amplitude increases, the V-shaped structure gradually disappears and electrons are concentrated on the diagonal in the electron correlation spectrum indicating that the energy sharing after electrons collision is symmetric for OTC laser fields with large relative amplitudes. Our studies show that changing the relative amplitude of the OTC laser field can efficiently control the electron-electron collisions and energy exchange efficiency of the NSDI process.
利用半经典集合模型,对正交偏振双色场(OTC)激光场驱动下的氖原子非连续双电离(NSDI)再碰撞动力学的相对振幅依赖性进行了理论研究。系统地探讨了再碰撞-撞击-电离(RII)和再碰撞-激发与后续电离(RESI)两种典型碰撞途径的动力学。我们的结果表明,当 OTC 激光场的相对振幅为零时,相关动量分布中的 V 形结构主要是由 RII 机制引起的,第一个电离电子会迅速掠过原子核,并与第二个电子分享少量能量。随着相对振幅的增大,电子相关谱中的 V 形结构逐渐消失,电子集中在对角线上,这表明在相对振幅较大的 OTC 激光场中,电子碰撞后的能量分享是对称的。我们的研究表明,改变 OTC 激光场的相对振幅可以有效地控制 NSDI 过程的电子-电子碰撞和能量交换效率。
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引用次数: 0
Intrinsic valley-polarized quantum anomalous Hall effect in a two-dimensional germanene/MnI2 van der Waals heterostructure 二维锗/锰离子范德华异质结构中的本征谷极化量子反常霍尔效应
Pub Date : 2024-05-15 DOI: 10.1088/1674-1056/ad4bbd
Xiao-jing Dong, Chang-Wen Zhang
Valley-polarized quantum anomalous Hall effect (VQAHE), combined nontrivial band topology with valleytronics, is of importance for both fundamental sciences and emerging applications. However, the experimental realization of this property is challengeable. Here, by using first-principles calculations and modal analysis, we predict a mechanism of producing VQAHE in two-dimensional ferromagnetic van der Waals germanene/MnI2 heterostructure. This heterostructure exhibits both valley anomalous Hall effect and VQAHE due to the joint effects of magnetic exchange effect and spin-orbital coupling with the aid of anomalous Hall conductance and chiral edge state. Moreover interestingly, through the electrical modulation of ferroelectric polarization state in In2Se3, the germanene/MnI2/In2Se3 heterostructure can undergo reversible switching from a semiconductor to a metallic behavior. This work offers a guiding advancement for searching for VQAHE in ferromagnetic van der Waals heterostructures and exploiting energy-efficient devices based on the VQAHE.
谷极化量子反常霍尔效应(VQAHE)结合了非难带拓扑学和谷电学,对基础科学和新兴应用都具有重要意义。然而,这一特性的实验实现却面临挑战。在此,我们通过第一原理计算和模态分析,预测了在二维铁磁范德华锗/MnI2 异质结构中产生 VQAHE 的机制。在反常霍尔电导和手性边缘状态的帮助下,由于磁交换效应和自旋轨道耦合的共同作用,这种异质结构同时表现出山谷反常霍尔效应和 VQAHE。此外,有趣的是,通过对 In2Se3 中铁电极化态的电调制,锗/锰离子/In2Se3 异质结构可以实现从半导体到金属行为的可逆转换。这项工作为在铁磁范德华异质结构中寻找 VQAHE 以及利用基于 VQAHE 的高能效器件提供了指导性进展。
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引用次数: 0
All-electron basis sets for H to Xe specific for ZORA calculations: Applications in atoms and molecules 用于 ZORA 计算的 H 至 Xe 的全电子基础集:原子和分子中的应用
Pub Date : 2024-05-15 DOI: 10.1088/1674-1056/ad4bbe
C. S. Gomes, F. E. Jorge, A. Canal Neto
A segmented basis set of quadruple zeta valence quality plus polarization functions (QZP) for H through Xe was developed to be used in conjunction with the ZORA Hamiltonian. This set was augmented with diffuse functions to describe electrons farther away from the nuclei adequately. Using the ZORA-CCSD(T)/QZP-ZORA theoretical model, atomic ionization energies and bond lengths, harmonic vibrational frequencies, and atomization energies of some molecules were calculated. The addition of core-valence corrections has been shown to improve the agreement between theoretical and experimental results for molecular properties. For atomization energies, a similar observation emerges when considering spin-orbit couplings. With the augmented QZP-ZORA set, static mean dipole polarizabilities of a set of atoms were calculated and compared with previously published recommended and experimental values. Performance evaluations of the ZORA and Douglas-Kroll-Hess Hamiltonians were made for each property studied.
为 H 至 Xe 开发了一个四重 zeta 价质加极化函数 (QZP) 的分段基础集,以便与 ZORA 哈密顿公式结合使用。为了充分描述离原子核较远的电子,还使用扩散函数对该基集进行了扩充。利用 ZORA-CCSD(T)/QZP-ZORA 理论模型,计算了一些分子的原子电离能和键长、谐振频率和原子化能。结果表明,增加核价修正可以改善分子性质的理论和实验结果之间的一致性。对于原子化能,在考虑自旋轨道耦合时也出现了类似的观察结果。利用增强 QZP-ZORA 集计算了一组原子的静态平均偶极极化率,并将其与之前公布的推荐值和实验值进行了比较。针对所研究的每种性质,对 ZORA 和 Douglas-Kroll-Hess 哈密顿进行了性能评估。
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引用次数: 0
Two-dimensional Sb net generated nontrivial topological states in SmAgSb2 probed by quantum oscillations 通过量子振荡探测 SmAgSb2 中二维 Sb 网产生的非难拓扑态
Pub Date : 2024-05-15 DOI: 10.1088/1674-1056/ad4bc2
Jian Yuan, Xian-Biao Shi, Hong Du, Tian Li, Chuanying Xi, Xia Wang, Wei Xia, Bao-Tian Wang, Ruidan Zhong, Yan-Feng Guo
The REAgSb2 (RE = rare earth and Y) family has drawn considerable research interest because the two-dimensional Sb net in their crystal structure hosts topological fermions and hence rich topological properties. We report herein the magnetization and magnetotransport measurements of SmAgSb2 single crystal, which unveil very large magnetoresistance and high carrier mobility up to 6.2×103% and 5.58×103 cm2V-1s-1, respectively. The analysis of both Shubnikov-de Haas and de Haas-van Alphen quantum oscillations indicates nontrivial Berry phases in the paramagnetic state while trivial Berry curvature in the antiferromagnetic state, indicating a topological phase transition induced by the antiferromagnetic order. It is also supported by the first-principles calculations. The results not only provide a new interesting topological material but also offer valuable insights into the correlation between magnetism and nontrivial topological states.
REAgSb2(RE = 稀土和 Y)家族引起了人们相当大的研究兴趣,因为其晶体结构中的二维 Sb 网承载着拓扑费米子,因而具有丰富的拓扑特性。我们在此报告了 SmAgSb2 单晶的磁化和磁迁移测量结果,结果显示其磁电阻和载流子迁移率分别高达 6.2×103% 和 5.58×103 cm2V-1s-1。对舒布尼科夫-德哈斯量子振荡和德哈斯-范阿尔芬量子振荡的分析表明,顺磁态存在非三相贝里相,而反铁磁态存在三相贝里曲率,这表明反铁磁秩序诱导了拓扑相变。这也得到了第一原理计算的支持。这些结果不仅提供了一种新的有趣的拓扑材料,而且为研究磁性与非三重拓扑态之间的相关性提供了宝贵的见解。
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引用次数: 0
Physics Package Based on Intracavity Laser Cooling 87Rb Atoms for Space Cold Atom Microwave Clock 基于腔内激光冷却 87Rb 原子的物理软件包,用于空间冷原子微波钟
Pub Date : 2024-05-15 DOI: 10.1088/1674-1056/ad4bc1
Siminda Deng, W. Ren, Jing-Feng Xiang, Jianbo Zhao, Lin Li, Di Zhang, J. Wan, Y. Meng, Xiaojun Jiang, Tang Li, Liang Liu, De-Sheng Lü
This article proposes a new physics package to enhance the frequency stability of the space cold atom clock with the advantages of a microgravity environment. Clock working processes, including atom cooling, atomic state preparation, microwave interrogation, and transition probability detection, are integrated into the cylindrical microwave cavity to achieve a high-performance and compact physics package for the space cold atom clock. We present the detailed design and ground-test results of the cold atom clock physics package in this article, which demonstrates a frequency stability of 1.2 × 10-12 τ-1/2 with a Ramsey linewidth of 12.5 Hz, and a better performance is predicted with a 1 Hz or a narrower Ramsey linewidth in microgravity environment. The miniaturized cold atom clock based on intracavity cooling has great potential for achieving space high-precision time-frequency reference in the future.
本文提出了一种新的物理包,利用微重力环境的优势增强空间冷原子钟的频率稳定性。将原子冷却、原子态制备、微波讯问、跃迁概率检测等时钟工作过程集成到圆柱形微波腔中,实现了高性能、紧凑型的空间冷原子钟物理包。我们在本文中介绍了冷原子钟物理包的详细设计和地面测试结果,该物理包在拉姆齐线宽为 12.5 Hz 时的频率稳定性为 1.2 × 10-12 τ-1/2,预计在微重力环境下拉姆齐线宽为 1 Hz 或更窄时性能会更好。基于腔内冷却的小型化冷原子钟在未来实现空间高精度时频基准方面具有巨大潜力。
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引用次数: 0
The evolution of anomalous Hall effect in ferromagnetic Weyl semimetal Nb x Zr1-x Co2Sn 铁磁性韦尔半金属 Nb x Zr1-x Co2Sn 中反常霍尔效应的演化
Pub Date : 2024-05-13 DOI: 10.1088/1674-1056/ad4a3b
Bo-wen Chen, Bing Shen
Magnetic topological semimetal can host various topological non-trivial states leading to exotic novel transport properties. Here we report the systematic magneto-transport studies on the Heusler alloy Nb x Zr1-x Co2Sn considered as a ferromagnetic(FM) Weyl semimetal. The cusp anomaly of temperature-dependent resistivity and large isotropic negative MR emerge around the FM transition consistent with the theoretical half-metallic predictions. The prominent anomalous Hall effect(AHE) has the same behavior with the applied field along various crystal directions. The Nb doping introduces more disorder resulting in the enhancement of the upturn for the temperature-dependent resistivity in low temperatures. With Nb doping, the AHE exhibits systemic evolution with the Fermi level lifted. At the doping level of x=0.25, the AHE mainly originates from the intrinsic contribution related to non-trivial topological Weyl states.
磁性拓扑半金属可以容纳各种拓扑非三维态,从而产生奇异的新传输特性。在此,我们报告了对被视为铁磁性(FM)韦尔半金属的 Heusler 合金 Nb x Zr1-x Co2Sn 的系统磁传输研究。在调频转变周围出现了随温度变化的电阻率尖顶异常和各向同性的大负磁迁移率,这与半金属理论预测一致。突出的反常霍尔效应(AHE)与沿不同晶向施加的场具有相同的行为。掺杂铌会引入更多的无序,从而导致随温度变化的电阻率在低温下上行增强。掺入铌后,AHE 随着费米级的升高而呈现系统演化。在 x=0.25 的掺杂水平下,AHE 主要来自与非三维拓扑韦尔态相关的本征贡献。
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引用次数: 0
Surface phonon resonance: A new mechanism for enhancing photonic spin Hall effect and refractive index sensor 表面声子共振:增强光子自旋霍尔效应和折射率传感器的新机制
Pub Date : 2024-05-13 DOI: 10.1088/1674-1056/ad4a3c
Jie Cheng, Chenglong Wang, Yiming Li, Yalin Zhang, Shengli Liu, P. Dong
Metal-based surface plasmon resonance (SPR) plays an important role in enhancing the photonic spin Hall effect (SHE) and developing sensitive optical sensors. However, the very large negative permittivities of metals limit their applications beyond the near-infrared regime. In this work, we theoretically present a new mechanism to enhance the photonic SHE by taking advantage of SiC-supported surface phonon resonance (SPhR) in the mid-infrared regime. The transverse displacement of photonic SHE is very sensitive to the wavelength of incident light and the thickness of SiC layer. Under the optimal parameter setup, the calculated largest transverse displacement of SiC-based SPhR structure reaches up to 163.8 μm, which is much larger than the condition of SPR. Moreover, a NO2 gas sensor based on the SPhR-enhanced photonic SHE is theoretically proposed with the superior sensing performance. Both the intensity and angle sensitivity of this sensor can be effectively manipulated by varying the damping rate of SiC. The results may provide a promising paradigm to enhance the photonic SHE in the mid-infrared region and open up new opportunity of highly sensitive refractive index sensors.
金属基表面等离子体共振(SPR)在增强光子自旋霍尔效应(SHE)和开发灵敏光学传感器方面发挥着重要作用。然而,金属非常大的负介电常数限制了其在近红外领域以外的应用。在这项工作中,我们从理论上提出了一种新的机制,利用 SiC 支持的表面声子共振(SPhR)在中红外波段增强光子自旋霍尔效应。光子 SHE 的横向位移对入射光的波长和 SiC 层的厚度非常敏感。在最佳参数设置下,计算得到的基于 SiC 的 SPhR 结构的最大横向位移可达 163.8 μm,远大于 SPR 的条件。此外,理论上还提出了一种基于 SPhR 增强光子 SHE 的 NO2 气体传感器,其传感性能优越。该传感器的强度和角度灵敏度都可以通过改变 SiC 的阻尼率来有效控制。这些结果为增强中红外区域的光子 SHE 提供了一种有前途的范例,并为高灵敏折射率传感器开辟了新的机遇。
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引用次数: 0
Magnetic domain structures in ultrathin Bi2Te3/CrTe2 heterostructures 超薄 Bi2Te3/CrTe2 异质结构中的磁畴结构
Pub Date : 2024-05-13 DOI: 10.1088/1674-1056/ad4a3a
Tirui Xia, Xiaotian Yang, Yifan Zhang, Xinqi Liu, Xinyu Cai, Chang Liu, Qi Yao, X. Kou, Wenbo Wang
Chromium tellurium compounds are important two-dimensional van der Waals ferromagnetic materials with high Curie temperature and chemical stability in air, which is promising for applications in spintronic devices. Here, high-quality spin-orbital-torque (SOT) device, Bi2Te3/CrTe2 heterostructure was epitaxially grown on Al2O3 (0001) substrates. Anomalous Hall measurements indicate the existence of strong ferromagnetism in this device with the CrTe2 thickness down to 10 nm. In order to investigate its micromagnetic structure, cryogenic magnetic force microscope (MFM) was utilized to measure the magnetic domain evolutions at various temperatures and magnetic fields. The virgin domain state of the device shows a worm-like magnetic domain structure with the size around 0.6 ~ 0.8 µm. Larger irregular-shape magnetic domains (>1µm) can be induced and pinned, after the field is increased to coercive field and ramped back to low fields. The temperature-dependent MFM signals exhibit a nice mean-field-like ferromagnetic transition with Curie temperature around 201.5 K, indicating a robust ferromagnetic ordering. Such device can be potentially implemented in future magnetic memory technology.
铬碲化合物是一种重要的二维范德华铁磁材料,具有较高的居里温度和在空气中的化学稳定性,有望应用于自旋电子器件。本文在 Al2O3 (0001) 基底上外延生长了高质量的自旋轨道转矩(SOT)器件--Bi2Te3/CrTe2 异质结构。反常霍尔测量结果表明,该器件具有很强的铁磁性,CrTe2 厚度低至 10 纳米。为了研究它的微磁结构,我们利用低温磁力显微镜(MFM)测量了不同温度和磁场下的磁畴演变。该器件的原始磁畴状态显示出蠕虫状磁畴结构,大小约为 0.6 ~ 0.8 µm。在磁场升高到胁迫磁场并回升到低磁场后,可以诱导和钉住较大的不规则形状磁畴(>1µm)。随温度变化的 MFM 信号显示出良好的均场类铁磁转变,居里温度约为 201.5 K,表明铁磁有序性很强。这种器件有可能应用于未来的磁存储器技术中。
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引用次数: 0
期刊
Chinese Physics B
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