Current Opinion in Environmental Science and Health最新文献

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Constructed wetlands for combined sewer overflow treatment: A 30-year review, current trends and future projections 人工湿地联合污水溢流处理：30年回顾，当前趋势和未来预测

IF 6.6 Q1 ENVIRONMENTAL SCIENCES

Current Opinion in Environmental Science and Health

Pub Date : 2025-10-30 DOI: 10.1016/j.coesh.2025.100681

Ismael Vera-Puerto , Darja Istenič , Pascal Molle , Carmen Hernández-Crespo , Carlos A. Arias

Combined sewer overflow (CSO) discharges pose a significant challenge to urban water management. Constructed wetlands (CWs) are a promising blue-green infrastructure solution for CSO management and water quality improvement, with recognized economic, social, and environmental benefits. This review synthesizes the state-of-the-art in CSO treatment using CWs over the past 30 years and explores current trends and future projections. A bibliometric analysis of 68 papers from the Web of Science Core Collection revealed that although CWs have been applied at a full scale for CSO treatment since the 1990s, they remain an emerging research topic. Germany, France, Italy, the United Kingdom and the United States of America lead in literature production and application. However, there is a significant lack of information from the Global South (developing countries) and tropical/subtropical regions. Reports from temperate developed countries indicate good performance, with removal efficiencies above 70 % for conventional pollutants such as solids, organic matter, and nutrients (nitrogen and phosphorus). However, pathogen removal was limited. Contaminants of emerging concern such as pharmaceuticals, polycyclic aromatic hydrocarbons (PAHs), and microplastics, have also been investigated in CW-treated CSOs with divergent results. This review also discusses various aspects, including regulations, design, environmental performance, and trade-offs. While CWs demonstrate substantial potential for preventing surface water pollution, their application and associated knowledge must expand beyond developed temperate regions, mirroring the global adoption of CWs for domestic wastewater and stormwater treatment. This expansion is crucial for CWs to be considered a truly global solution for CSO treatment.

复合式污水溢流（CSO）排放对城市水管理提出了重大挑战。人工湿地（CWs）是一种很有前途的蓝绿色基础设施解决方案，用于公民社会组织的管理和水质改善，具有公认的经济、社会和环境效益。本综述综合了过去30年来使用化学武器治疗CSO的最新进展，并探讨了目前的趋势和未来的预测。对Web of Science核心合集68篇论文的文献计量分析表明，尽管自20世纪90年代以来，CWs已经全面应用于CSO治疗，但它们仍然是一个新兴的研究课题。德国、法国、意大利、英国和美国在文献生产和应用方面处于领先地位。然而，全球南方（发展中国家）和热带/亚热带地区的资料严重缺乏。来自温带发达国家的报告显示了良好的性能，对固体、有机物和营养物质（氮和磷）等常规污染物的去除效率超过70%。然而，病原菌的去除是有限的。新出现的关注污染物，如药物、多环芳烃（PAHs）和微塑料，也在化化水处理的公民社会组织中进行了研究，结果不同。本综述还讨论了各个方面，包括法规、设计、环境性能和权衡。虽然化粪池在防止地表水污染方面显示出巨大的潜力，但它们的应用和相关知识必须扩展到发达温带地区以外，反映出全球在生活废水和雨水处理中采用化粪池的情况。这一扩展对于将CWs视为CSO治疗的真正全球解决方案至关重要。

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A review of the full-scale constructed wetlands for the treatment and management of winery wastewater 大规模人工湿地处理和管理葡萄酒废水的研究进展

IF 6.6 Q1 ENVIRONMENTAL SCIENCES

Current Opinion in Environmental Science and Health

Pub Date : 2025-10-28 DOI: 10.1016/j.coesh.2025.100680

Alessia Marzo , Juliano Rezende Mudadu Silva , Fabio Masi , Anacleto Rizzo , Giuseppe Luigi Cirelli

Constructed wetlands (CWs) have been demonstrated to be effective solution for treating winery wastewater (WWW). In this paper, worldwide experiences over the last 25 years of full-scale CWs for WWW treatment are gathered. In total, three CW types were identified: horizontal subsurface flow, vertical subsurface flow and hybrid CWs. The organic and hydraulic loading rate ranged between 15.74–315 gCODm⁻²d⁻¹ and 13–313 mmd^-1, respectively. The most common plant species were Phragmites australis, Typha spp., and Schoenoplectus tabernaemontani. In this review, treatment efficiency of CWs is presented as well as their operational challenges and opportunities.

人工湿地（CWs）已被证明是处理酒厂废水的有效解决方案。本文收集了近25年来世界范围内大规模化武治疗WWW的经验。总的来说，确定了三种连续流类型：水平地下流、垂直地下流和混合型连续流。有机和水力加载速率分别为15.74-315 gCODm−2d−1和13-313 mmd-1。最常见的植物种类为芦苇、田螺和雪蚤。本文介绍了水化液的处理效率，以及水化液在操作上面临的挑战和机遇。

引用次数: 0

Wildfire-induced shifts in dissolved organic carbon reactivity toward trihalomethane formation 野火引起的溶解有机碳反应性向三卤甲烷形成的转变

IF 6.6 Q1 ENVIRONMENTAL SCIENCES

Current Opinion in Environmental Science and Health

Pub Date : 2025-10-11 DOI: 10.1016/j.coesh.2025.100679

Shiyue Zhang, Penghui Du, Alex Tat-Shing Chow

Wildfires increasingly degrade source-water quality, yet the reactivity of fire-altered dissolved organic carbon (DOC) toward trihalomethane (THM) formation remains unclear. This mini-review synthesizes 14 paired pre/post-fire datasets under a carbon-normalized framework (THM-specific formation potential, THM-SFP). (i) Occurrence: most studies show lower THM-SFP after fire from loss of oxygen-rich moieties. (ii) Severity: moderate burning can produce phenolic/carbonyl fragments, elevating THM-SFP, whereas high severity suppresses it. (iii) Rainfall: first flushes raise DOC and bulk THMs, while THM-SFP responses are mixed. Cross-study interpretation remains constrained by methodological heterogeneity and limited data. Findings support severity-stratified, time-resolved monitoring for post-fire water management.

野火日益降低水源水质，但火灾改变的溶解有机碳（DOC）对三卤甲烷（THM）形成的反应性尚不清楚。这篇小型综述在碳标准化框架（THM-specific formation potential, THM-SFP）下综合了14组配对的火灾前后数据集。(i)发生：大多数研究表明，火灾后由于富氧部分的损失，THM-SFP降低。（ii）严重程度：中度燃烧可以产生酚/羰基碎片，提高THM-SFP，而高严重程度则抑制它。（iii）降雨：第一次冲水会提高DOC和大量THMs，而THM-SFP响应是混合的。交叉研究解释仍然受到方法异质性和有限数据的限制。研究结果支持对火灾后水管理进行严重程度分层、时间分辨的监测。

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Applying effect-based methods to evaluate the mixture effects of disinfection by-products and other chemicals in disinfected water 应用基于效果的方法评价消毒副产物与其他化学物质在消毒液中的混合效果

IF 6.6 Q1 ENVIRONMENTAL SCIENCES

Current Opinion in Environmental Science and Health

Pub Date : 2025-10-11 DOI: 10.1016/j.coesh.2025.100678

Peta A. Neale , Beate I. Escher , Frederic D.L. Leusch

Effect-based methods (EBM) are increasingly used to assess disinfected water quality as they can detect the mixture effects of all bioactive chemicals, including disinfection by-products (DBPs). In this review, we discuss the application of EBM to extracts of disinfected water, with bioassays for cytotoxicity, genotoxicity and oxidative stress response being the most responsive to DBPs. The contribution of known DBPs to the mixture effect can be predicted from single DBPs’ effects using established mixture models. Regulated DBPs typically have a minor contribution to the observed effect. Effect-based trigger values can be used to determine if the treated water quality is acceptable.

基于效果的方法（EBM）越来越多地用于评估消毒水质，因为它们可以检测所有生物活性化学物质的混合效应，包括消毒副产物（DBPs）。在这篇综述中，我们讨论了EBM在消毒水提取物中的应用，其中dbp对细胞毒性、遗传毒性和氧化应激反应最敏感。已知dbp对混合效应的贡献可以利用已建立的混合模型从单个dbp的效应中预测出来。受调节的舒张压通常对观察到的效果贡献不大。基于效应的触发值可用于确定处理后的水质是否可接受。

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Mechanisms and potential for disinfection byproduct formation from peracetic acid 过氧乙酸消毒副产物形成的机理和潜力

IF 6.6 Q1 ENVIRONMENTAL SCIENCES

Current Opinion in Environmental Science and Health

Pub Date : 2025-10-08 DOI: 10.1016/j.coesh.2025.100677

Jiaqi Li, Ching-Hua Huang

Peracetic acid (PAA), an organic compound with the formula CH₃CO₃H, and a sterilant and disinfectant, has emerged as a promising alternative to free chlorine for achieving high-level disinfection in combined sewer overflow, wastewater, and stormwater. However, a major concern with any water disinfectant is its potential to react with natural organic matter or other constituents, leading to the unintentional formation of disinfection byproducts (DBPs). This review examines DBP formation during PAA disinfection and PAA-based advanced oxidation processes (AOPs), with an emphasis on studies published within the past five years. It summarizes the influence of halides, nitrite, and various AOP operational conditions on DBP formation. Additionally, it explores the mechanisms of DBP formation in the presence of halides during PAA disinfection, highlighting key intermediates involved in the reactions. The insights provided in this review offer valuable guidance for minimizing DBP formation in further applications of PAA in water treatment.

过氧乙酸（PAA）是一种化学式为CH3CO3H的有机化合物，也是一种灭菌剂和消毒剂，已成为一种有前途的游离氯替代品，可用于在综合下水道溢流、废水和雨水中实现高水平消毒。然而，任何水消毒剂的一个主要问题是它可能与天然有机物或其他成分发生反应，导致无意中形成消毒副产物（DBPs）。本文综述了PAA消毒和PAA基高级氧化过程（AOPs）中DBP的形成，重点介绍了过去五年发表的研究。总结了卤化物、亚硝酸盐和各种AOP操作条件对DBP形成的影响。此外，它还探讨了在PAA消毒过程中卤化物存在下DBP形成的机制，突出了参与反应的关键中间体。本文的研究结果为PAA在水处理中的进一步应用提供了有价值的指导。

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Algae-derived organic matter in drinking water sources and the formation of disinfection byproducts: A critical review 饮用水水源中藻类来源的有机物及其消毒副产物的形成：综述

IF 6.6 Q1 ENVIRONMENTAL SCIENCES

Current Opinion in Environmental Science and Health

Pub Date : 2025-10-03 DOI: 10.1016/j.coesh.2025.100675

Marlena M. Cheshire, William A. Mitch

The proliferation of algal blooms in freshwater is a water quality concern. Algae release algal organic matter (AOM) that is a disinfection byproduct (DBP) precursor. Monitoring blooms remains challenging as cell concentration and diversity vary across seasons and locations. Compared to natural organic matter (NOM), AOM has distinct characteristics. The low aromaticity and high nitrogen content of AOM favor unregulated nitrogen-containing DBPs, such as haloacetonitriles and haloacetamides, over regulated trihalomethanes, and haloacetic acids. Research utilizing ultra-high-resolution mass spectrometry found that AOM is an important precursor of >2-carbon DBPs. With prevalent fatty acids and peptides, studies have identified chlorinated biomolecule formation from AOM.

淡水中藻类大量繁殖是一个水质问题。藻类释放的藻类有机物（AOM）是一种消毒副产物（DBP）前体。由于细胞浓度和多样性随季节和地点的变化而变化，监测花朵仍然具有挑战性。与天然有机质（NOM）相比，AOM具有明显的特性。AOM的低芳构性和高氮含量有利于卤代乙腈和卤代乙酰胺、过度调控的三卤甲烷和卤代乙酸等不受管制的含氮dbp。利用超高分辨率质谱法研究发现，AOM是2-碳DBPs的重要前体。与普遍的脂肪酸和肽，研究已经确定氯代生物分子的形成从AOM。

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Beyond 1–2 carbon compounds: Emerging insights on higher-carbon disinfection byproducts 超越1-2碳化合物：对高碳消毒副产物的新见解

IF 6.6 Q1 ENVIRONMENTAL SCIENCES

Current Opinion in Environmental Science and Health

Pub Date : 2025-10-01 DOI: 10.1016/j.coesh.2025.100676

Zachary T. Kralles , Carsten Prasse

Disinfection byproducts (DBPs) are ubiquitous contaminants in drinking water that are formed through reactions between disinfectants and natural or anthropogenic precursors. While regulatory and research efforts have historically focused on 1–2 carbon DBPs, these compounds account for only a fraction of the total organic halogen and measured toxicity in finished drinking water. Recent research has shifted attention to higher-carbon DBPs with >2-carbon atoms (>C₂ DBPs). We summarize recent advancements in the discovery, occurrence, and formation mechanisms of >C₂ DBPs and highlight the need to integrate >C₂ DBPs into toxicity frameworks to better assess their contribution to the overall toxicity of disinfected waters.

消毒副产物（DBPs）是饮用水中普遍存在的污染物，通过消毒剂与自然或人为前体之间的反应形成。虽然监管和研究工作历来集中在1-2碳dbp上，但这些化合物仅占饮用水中有机卤素总量和测量毒性的一小部分。最近的研究已将注意力转移到具有2碳原子的高碳DBPs （>C2 DBPs）上。我们总结了最近在发现、发生和形成机制方面的进展，并强调需要将>；C2 DBPs整合到毒性框架中，以更好地评估它们对消毒水的整体毒性的贡献。

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Arsenic removal in constructed wetlands 人工湿地除砷研究

IF 6.6 Q1 ENVIRONMENTAL SCIENCES

Current Opinion in Environmental Science and Health

Pub Date : 2025-09-24 DOI: 10.1016/j.coesh.2025.100673

Katherine Lizama-Allende, Diego Bravo-Riquelme

Constructed wetlands are a promising arsenic removal technology. Laboratory-scale experiments have proved their arsenic removal capacity and identified the main factors affecting it. However, very few pilot and full-scale systems are reported. Most of the recent studies report on laboratory-scale systems operated during short periods, therefore lifespan, seasonal effects, and the long-term effects of vegetation cannot be evaluated. Recent work on mechanistic models could guide the development of design guidelines, which are not currently available. Confirming laboratory-scale results in pilot and full-scale systems remains a challenge, as well as the use of their data for future calibration and validation of models.

人工湿地是一种很有前途的除砷技术。实验室规模的实验证明了其除砷能力，并确定了影响其除砷能力的主要因素。然而，很少有试点和全尺寸系统的报道。最近的大多数研究报告的是实验室规模的系统在短时间内运行，因此无法评估植被的寿命、季节效应和长期效应。最近在机械模型上的工作可以指导设计指南的发展，这是目前还没有的。在中试和全尺寸系统中确认实验室规模的结果仍然是一个挑战，以及使用他们的数据进行未来的模型校准和验证。

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Constructed wetlands as a sustainable solution for pesticide pollution mitigation 人工湿地是缓解农药污染的可持续解决方案

IF 6.6 Q1 ENVIRONMENTAL SCIENCES

Current Opinion in Environmental Science and Health

Pub Date : 2025-09-18 DOI: 10.1016/j.coesh.2025.100672

Jyoti Singh , Mahima Choudhary , Rajesh Singh , Sujata Kashyap , Vinay Kumar Tyagi , Kalzang Chhoden , Sandeep Singh

Pesticides widely used in agriculture and households pose environmental risks due to their persistence, toxicity, and bioaccumulative nature. Constructed wetlands (CWs) have emerged as a sustainable solution for removing pesticides from agricultural runoff and wastewater. Their performance depends on factors like plant species, substrate, wastewater composition, climate, and retention time. Key challenges include seasonal performance variability, substrate clogging, and pesticide accumulation in sediments. Full-scale studies show removal rates from 38% to over 99%, influenced by pH, temperature, vegetation, microbial activity, and retention time. Emerging strategies, such as solar photocatalytic oxidation and real-time monitoring, offer promising enhancements to CW functionality, supporting sustainable and environmentally friendly water treatment solutions.

农业和家庭中广泛使用的农药因其持久性、毒性和生物蓄积性而构成环境风险。人工湿地（CWs）已成为去除农业径流和废水中农药的可持续解决方案。它们的性能取决于植物种类、基质、废水成分、气候和滞留时间等因素。主要挑战包括季节性性能变化、基质堵塞和沉积物中的农药积累。全面研究表明，受pH值、温度、植被、微生物活性和滞留时间的影响，去除率从38%到99%以上。新兴战略，如太阳能光催化氧化和实时监测，为连续水处理功能提供了有希望的增强，支持可持续和环保的水处理解决方案。

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Impacts of unplanned de facto wastewater reuse on disinfection byproduct formation at downstream drinking water treatment plants 无计划污水回用对下游饮用水处理厂消毒副产物形成的影响

IF 6.6 Q1 ENVIRONMENTAL SCIENCES

Current Opinion in Environmental Science and Health

Pub Date : 2025-09-13 DOI: 10.1016/j.coesh.2025.100669

Paul Westerhoff , Minhazul Islam , Tanju Karanfil , Eric Dickenson , Jacelyn Rice-Boayue , Kenan Ozekin , Chad Seidel

De facto reuse (DFR) refers to the unplanned inclusion of treated wastewater in drinking water supplies due to upstream wastewater treatment plant effluents. Nearly half of drinking water treatment plants (DWTPs) in the USA are impacted to some extent by DFR, with maximum estimated DFR percentage streamflow approaching 90% in some cases. DFR is not unique to the U.S. but been reported globally in Asia, Europe, Africa, and others. Treated wastewater discharged to surface waters can contain significant levels of inorganic (e.g. bromide and iodide) and organic compounds (e.g. micropollutants, extracellular products, and nitrogen-containing organic matter) that serve as precursors to both regulated and unregulated disinfection by-products (DBPs) in downstream DWTPs. Although identified as a national concern over a decade ago, the lack of standardized methodologies for quantifying and reporting DFR hinders comparative assessments and regulatory decision-making. We believe DFR is underappreciated or outright ignored as compared to the water community focus on highly managed and regulated indirect and direct potable reuse—although risks from DFR are just as real and important to address. This review explores how DFR contributes to DBP risks at DWTPs and discusses strategies for monitoring, modeling, and managing these risks considering recent research.

事实上的回用（DFR）是指由于上游污水处理厂的废水而意外地将处理过的废水纳入饮用水供应。在美国，近一半的饮用水处理厂（DWTPs）在一定程度上受到DFR的影响，在某些情况下，最大估计DFR百分比流量接近90%。DFR不是美国独有的，在亚洲、欧洲、非洲和其他地区都有报道。排入地表水的经处理废水可能含有大量的无机（如溴化物和碘化物）和有机化合物（如微污染物、细胞外产物和含氮有机物），这些化合物可作为下游污水处理厂中受管制和不受管制的消毒副产物（dbp）的前体。虽然十多年前就确定为国家关注的问题，但缺乏量化和报告DFR的标准化方法阻碍了比较评估和管理决策。我们认为，与水资源社区高度关注管理和监管的间接和直接饮用水再利用相比，DFR被低估或完全忽视了——尽管DFR带来的风险同样真实存在，也同样重要。本文探讨了DFR如何导致dwtp的DBP风险，并结合最近的研究讨论了监测、建模和管理这些风险的策略。

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