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Nitrogen removal in constructed wetlands 人工湿地的氮去除
IF 6.6 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2025-09-12 DOI: 10.1016/j.coesh.2025.100668
Jan Vymazal
The most important processes responsible for nitrogen removal in constructed wetlands (CWs) are nitrification and denitrification. These processes were well-described in the second part of the 19th century and are still valid. During the recent years, other processes responsible for nitrogen removal in CWs have been identified, namely anaerobic ammonia oxidation (Anammox), anaerobic ammonia-oxidation-coupled-to-dissimilatory ferric iron reduction (Feammox) and autotrophic denitrification. Also, bacteria that can perform complete oxidation of ammonia to nitrate (Comammox) have been discovered. This review is mostly aimed at these newly discovered processes in relation to wastewater treatment in CWs.
人工湿地中最重要的脱氮过程是硝化和反硝化。这些过程在19世纪下半叶得到了很好的描述,现在仍然有效。近年来,人们还发现了其他一些处理生化水脱氮的方法,如厌氧氨氧化(Anammox)、厌氧氨氧化-偶联异化铁还原(Feammox)和自养反硝化。此外,还发现了可以将氨完全氧化为硝酸盐的细菌(Comammox)。本文主要针对这些新发现的与化粪池废水处理有关的工艺进行综述。
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引用次数: 0
Tire-wear particles and tire-related emerging contaminants: Characteristics, occurrence, and toxicity in the environment 轮胎磨损颗粒和与轮胎相关的新兴污染物:特征、发生和环境中的毒性
IF 6.6 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2025-09-08 DOI: 10.1016/j.coesh.2025.100666
Mahyar Ghanadi , Lou Caubrière , Melanie Kah , Lokesh P. Padhye
The discovery of 6PPD-quinone as a toxic transformation product and aqueous contaminant from a common tire antioxidant has catalyzed extensive research into its environmental occurrence and other tire-related emerging contaminants (TRECs). However, many other tire-derived chemicals remain understudied, yet may pose significant environmental risks. This review provides a critical overview of the characteristics, occurrence, and fate of TRECs, as well as their toxicological impacts. While advancements in analytical techniques have enhanced the detection of these contaminants, knowledge gaps exist regarding their persistence, transformation, and long-term effects in various environmental compartments. Recent findings suggest that several TRECs, including diphenylguanidine (DPG) and hexamethoxymethylmelamine (HMMM), are frequently detected in road runoff, wastewater, sediments, and even biota. Given their widespread occurrence and potential toxicity, further investigations into their environmental behavior, regulatory implications, and mitigation strategies are urgently needed. This review highlights the pressing need for expanded research beyond 6PPD-quinone to address the broader risks associated with TRECs.
作为一种常见轮胎抗氧化剂的有毒转化产物和含水污染物,6ppd -醌的发现催化了对其环境发生和其他与轮胎相关的新兴污染物(trec)的广泛研究。然而,许多其他轮胎衍生的化学品仍未得到充分研究,但可能会造成重大的环境风险。本文综述了trec的特征、发生和命运,以及它们的毒理学影响。虽然分析技术的进步加强了对这些污染物的检测,但在各种环境隔间中,它们的持久性、转化和长期影响方面存在知识空白。最近的研究结果表明,在道路径流、废水、沉积物甚至生物群中经常检测到几种trec,包括二苯基胍(DPG)和六聚甲氧基甲基三聚氰胺(HMMM)。鉴于它们的广泛存在和潜在毒性,迫切需要进一步调查它们的环境行为、监管影响和缓解策略。本综述强调,迫切需要扩大6ppd -醌以外的研究,以解决与trec相关的更广泛的风险。
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引用次数: 0
New developments in paleo-ecotoxicology: Emerging approaches in applying lake sediment archives to assess impacts from aquatic pollution 古生态毒理学的新进展:应用湖泊沉积物档案评估水生污染影响的新方法
IF 6.6 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2025-09-06 DOI: 10.1016/j.coesh.2025.100667
Joshua R. Thienpont , Jennifer B. Korosi , Jules M. Blais , John P. Smol
Many aquatic ecosystems have experienced a history of impacts from exposure to environmental contaminants, with aquatic biota often exhibiting population and/or community changes following toxicant exposure. However, identifying aquatic effects can be challenging due to a paucity of monitoring data and gaps in monitoring records. The study of lake sediments as natural environmental archives (paleolimnology) provides an opportunity to assess the long-term impacts of pollution on aquatic organisms and ecosystems. Cores collected from polluted systems can preserve both a record of the toxicant(s) in question, and also an archive of biotic changes at multiple scales of organization, from molecular levels to communities to ecosystem processes (paleo-ecotoxicology). Here, we review recent examples of the application of the paleo-ecotoxicological approach based on ‘classical’ paleolimnological indicators of contamination (e.g. metals, organic contaminants) and ecotoxicological response variables (e.g. pigments and subfossil morphological indicators). We also outline emerging environmental contaminants (e.g. microplastics, pharmaceuticals) that are increasingly being detected and documented in sediment records, highlighting evolving sources and intensities of toxicological stressors that are fruitful areas for future paleo-ecotoxicological inquiry. In addition, the ability to characterize aquatic community changes using emerging sedimentary DNA approaches has rapidly expanded, providing a powerful opportunity to build on the ecological information obtained from traditional indicators to better understand ecosystem responses to contamination. Finally, we argue for the importance of methodological approaches that specifically examine the ecotoxicological impacts of contamination in the future application of the paleo-ecotoxicological approach by exploring several recent examples.
许多水生生态系统都经历过暴露于环境污染物的影响,水生生物群在暴露于有毒物质后往往表现出种群和/或群落的变化。然而,由于监测数据的缺乏和监测记录的空白,确定水生影响可能具有挑战性。湖泊沉积物作为自然环境档案(古湖泊学)的研究为评估污染对水生生物和生态系统的长期影响提供了机会。从污染系统中收集的岩心既可以保存有关有毒物质的记录,也可以保存从分子水平到群落到生态系统过程等多个组织尺度上生物变化的档案(古生态毒理学)。在此,我们回顾了基于“经典”古湖泊污染指标(如金属、有机污染物)和生态毒理学响应变量(如色素和亚化石形态指标)的古生态毒理学方法的最新应用实例。我们还概述了越来越多地在沉积物记录中被检测和记录的新出现的环境污染物(例如微塑料,药物),强调了毒理学压力源的演变来源和强度,这是未来古生态毒理学研究的成果领域。此外,利用新兴的沉积DNA方法表征水生群落变化的能力已经迅速扩大,为建立从传统指标获得的生态信息提供了强大的机会,以更好地了解生态系统对污染的响应。最后,我们通过探索最近的几个例子,论证了在古生态毒理学方法的未来应用中,专门研究污染的生态毒理学影响的方法学方法的重要性。
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引用次数: 0
Sustainable nanoadsorbents from lignocellulosic waste: A green approach to wastewater treatment 木质纤维素废弃物的可持续纳米吸附剂:废水处理的绿色途径
IF 6.6 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2025-09-04 DOI: 10.1016/j.coesh.2025.100665
Parushi Nargotra , Mei-Ling Tsai , Cheng-Di Dong , Chia-Hung Kuo , Bijender Kumar Bajaj , Vishal Sharma
In the face of escalating water pollution, the development of innovative and sustainable processes for wastewater treatment has become imperative to safeguard ecosystems. The current review explores the integration of nanotechnology with lignocellulosic materials to develop cost-effective, high-performance nanoadsorbents for wastewater treatment. The nanostructured cellulose and lignin exhibit enhanced porosity, surface area, and functionalization capabilities, enabling efficient removal of environmental pollutants, including heavy metals. The advancements in using nanocellulose/nanolignin for removing water pollutants and understanding the underlying mechanisms, as well as life cycle analysis, are discussed. These bio-based nanomaterials reduce environmental impact, improve resource efficiency, and support sustainable development goals (SDGs).
面对不断升级的水污染,开发创新和可持续的废水处理工艺已成为保护生态系统的必要条件。本文综述了纳米技术与木质纤维素材料的结合,以开发具有成本效益、高性能的废水处理纳米吸附剂。纳米结构的纤维素和木质素表现出增强的孔隙度、表面积和功能化能力,能够有效地去除包括重金属在内的环境污染物。综述了纳米纤维素/纳米木质素在去除水污染物方面的研究进展,探讨了纳米纤维素/纳米木质素去除水污染物的机理,并对其生命周期进行了分析。这些生物基纳米材料减少了环境影响,提高了资源效率,并支持可持续发展目标(sdg)。
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引用次数: 0
Which sources contribute more to nitrosamines and their precursors in water resources: The natural or the anthropogenic? 哪些来源对亚硝胺及其在水资源中的前体的贡献更大:自然的还是人为的?
IF 6.6 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2025-08-27 DOI: 10.1016/j.coesh.2025.100664
Fan Zhou , Yuxuan Xie , Yu Wang , Xiaobin Liao , Chao Chen
This paper summarizes recent progress in identifying sources of nitrosamines (NAs) and their precursors in water resources. Natural sources include humic substances, microbial and algal metabolites, which will be exacerbated by natural disasters and extreme climate events. Anthropogenic sources include domestic wastewater, industrial wastewater and agricultural wastewater. Natural sources generally contribute a few to dozens of ng/L of precursors but provide minimal NAs, while anthropogenic sources provide a few to hundreds of ng/L of NAs and higher levels of precursors. These insights aid differentiation of natural vs. anthropogenic contributions, providing guidance for pollution control and sustainable management of water resources.
本文综述了近年来在水资源中亚硝胺及其前体来源鉴定方面的研究进展。自然来源包括腐殖质物质、微生物和藻类代谢物,自然灾害和极端气候事件会加剧这一问题。人为来源包括生活废水、工业废水和农业废水。天然来源通常提供几到几十ng/L的前体,但提供很少的NAs,而人为来源提供几到数百ng/L的NAs和更高水平的前体。这些见解有助于区分自然和人为的贡献,为污染控制和水资源的可持续管理提供指导。
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引用次数: 0
Microalgae-based treatment for wastewater management and valorization 以微藻为基础的废水处理及增值
IF 6.6 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2025-08-23 DOI: 10.1016/j.coesh.2025.100662
Shailja Pant , Mukesh Goel , Naresh Kumar Sahoo , Qiuyan Yuan , Prangya Ranjan Rout
Wastewater treatment is a critical process for building a water-resilient economy, ensuring pollutant removal before environmental discharge. Conventional treatment methods, though effective, are energy-intensive, reliant on chemical processes, and generate large volumes of sludge, posing economic and environmental challenges. In recent years, microalgae-based wastewater treatment has emerged as a promising alternative due to its potential for efficient nutrient removal, biomass valorization, and carbon sequestration. However, despite its advantages, large-scale implementation remains constrained by operational costs, biomass harvesting inefficiencies, and variable treatment performance. Recent advancements in techno-economic assessments, bioprocess optimization, and multiomics approaches have improved system efficiency, cost-effectiveness, and bioproduct recovery. This study reviews the latest developments, opportunities, and challenges in microalgal wastewater treatment, providing insights into its feasibility and future prospects. A comprehensive understanding of emerging technologies and integrated system approaches will be crucial in advancing microalgal-based solutions for sustainable wastewater management.
污水处理是建设水韧性经济的关键过程,确保污染物在环境排放之前被去除。传统的处理方法虽然有效,但能源密集,依赖化学过程,产生大量污泥,对经济和环境构成挑战。近年来,基于微藻的废水处理因其高效去除营养物质、生物质增值和碳封存的潜力而成为一种有前途的替代方案。然而,尽管有其优势,大规模实施仍然受到运营成本、生物质收获效率低下和处理性能变化的限制。技术经济评估、生物过程优化和多组学方法的最新进展提高了系统效率、成本效益和生物产品回收率。本文综述了微藻废水处理的最新进展、机遇和挑战,并对其可行性和未来前景进行了展望。全面了解新兴技术和综合系统方法对于推进基于微藻的可持续废水管理解决方案至关重要。
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引用次数: 0
Greenhouse gas emissions in industrial wastewater treatment: technologies, challenges, and strategies 工业废水处理中的温室气体排放:技术、挑战和策略
IF 6.6 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2025-08-21 DOI: 10.1016/j.coesh.2025.100661
Nguyen The Tung Lam , Le Thi Lan Anh , Tran Le Luu
Greenhouse gas (GHG) emissions from industrial wastewater treatment are increasingly acknowledged as a significant contributor to climate change but remain underrepresented in mitigation strategies, especially in developing countries. Methane (CH4), nitrous oxide (N2O), and carbon dioxide (CO2) are emitted through anaerobic digestion, biological nitrogen removal, and energy-intensive operations. In Vietnam, centralized WWTPs have reported emissions as high as 476.1 MtCO2e from CH4 and 13,103.9 MtCO2e from N2O, emphasizing the need for targeted intervention. It is hypothesized that when equipped with low-emission technologies and supported by integrated approaches, such as energy recovery, optimized nutrient removal, and real-time digital monitoring, industrial wastewater systems can be transformed into climate-resilient infrastructure with significantly reduced emission intensities. In this review, mitigation pathways are synthesized through a critical evaluation of peer-reviewed literature, field-based data, and global policy frameworks. Key emission factors, including 0.0011 g CH4/g BOD5 and 0.0017 g N2O–N/g TN-influent, are analyzed alongside operational metrics. Technologies such as anaerobic membrane bioreactors (AnMBRs), partial nitritation–anammox (PN/A) processes, AME-AD systems, and photovoltaic-supported biogas recovery are comprehensively reviewed. A four-phase roadmap to net-zero emissions by 2050 is proposed, integrating life cycle assessment, AI-enhanced monitoring, and carbon finance mechanisms. Emphasis is placed on the co-benefits of GHG mitigation strategies for public health resilience, energy security, and the achievement of Sustainable Development Goals. By repositioning industrial wastewater as a strategic entry point for climate action, this study outlines actionable, cross-sectoral solutions to support decarbonization and circular economy transformation in rapidly industrializing economies. These findings hold particular relevance for journals focusing on environmental engineering, sustainable infrastructure, climate governance, and low-carbon development pathways.
工业废水处理产生的温室气体(GHG)排放日益被认为是造成气候变化的一个重要因素,但在缓解战略中所占比例仍然不足,尤其是在发展中国家。甲烷(CH4)、氧化亚氮(N2O)和二氧化碳(CO2)通过厌氧消化、生物脱氮和能源密集型操作排放。在越南,集中式污水处理厂报告的CH4排放量高达4.761亿吨二氧化碳当量,N2O排放量高达13103.9亿吨二氧化碳当量,这强调了有针对性干预的必要性。我们假设,当配备低排放技术并辅以能源回收、优化营养物去除和实时数字监测等综合方法时,工业废水系统可以转变为具有气候适应型的基础设施,显著降低排放强度。在本综述中,通过对同行评议文献、实地数据和全球政策框架的批判性评估,综合了缓解途径。关键排放因子,包括0.0011 g CH4/g BOD5和0.0017 g N2O-N /g tn,与操作指标一起分析。对厌氧膜生物反应器(anmbr)、部分硝化-厌氧氨氧化(PN/A)工艺、AME-AD系统和光伏支持的沼气回收等技术进行了全面综述。提出了到2050年实现净零排放的四阶段路线图,整合了生命周期评估、人工智能增强监测和碳融资机制。重点是温室气体缓解战略对公共卫生抗灾能力、能源安全和实现可持续发展目标的共同益处。通过将工业废水重新定位为气候行动的战略切入点,本研究概述了可操作的跨部门解决方案,以支持快速工业化经济体的脱碳和循环经济转型。这些发现对关注环境工程、可持续基础设施、气候治理和低碳发展途径的期刊尤其重要。
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引用次数: 0
A review on fate and transport of biodegradable and non-biodegradable microplastics in the aquatic environment 可生物降解和不可生物降解微塑料在水生环境中的归宿和迁移研究进展
IF 6.6 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2025-08-20 DOI: 10.1016/j.coesh.2025.100660
Basanta Kumar Biswal, Rajasekhar Balasubramanian
Biodegradable plastics have received considerable attention as an eco-friendly material to replace non-biodegradable plastics. This paper critically reviews recent studies on the occurrence, fate, transport, and ecotoxicity of biodegradable and non-biodegradable microplastics (MPs) in the aquatic environment. The fate and transport of MPs largely depend on their properties, hydrodynamic conditions, and climatic factors. MPs show various levels of ecotoxicity toward aquatic biota. The overall aim of this review is to improve the current understanding on the fate and transport of MPs and help regulatory agencies to develop effective strategies for mitigation of pollution, caused by MPs in the aquatic environment.
生物降解塑料作为一种替代非生物降解塑料的环保材料受到了广泛关注。本文综述了生物可降解和不可降解微塑料(MPs)在水生环境中的发生、命运、运输和生态毒性的最新研究。MPs的命运和运输在很大程度上取决于它们的性质、水动力条件和气候因素。MPs对水生生物表现出不同程度的生态毒性。本综述的总体目标是提高目前对MPs命运和运输的理解,并帮助监管机构制定有效的战略,以减轻由MPs在水生环境中造成的污染。
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引用次数: 0
Erratum to “BiVO4-based photoanodes for the photoelectrocatalytic removal of trace organic pollutants from water: A mini review on recent developments” [Curr Opin Environ Sci Health 45 (June 2025) 1–1 100615] “基于bivo4的光阳极用于光电催化去除水中痕量有机污染物:近期发展综述”[当代观点,环境科学与健康45 (June 2025) 1-1 100615]
IF 6.6 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2025-08-19 DOI: 10.1016/j.coesh.2025.100663
Agha Zeeshan Ali , Sanjeeb Mohapatra , Jan Peter van der Hoek , Henri Spanjers
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引用次数: 0
Greenhouse gas emissions from municipal wastewater treatment: Global insights and Vietnam's approach 城市污水处理的温室气体排放:全球视角和越南的做法
IF 6.6 Q1 ENVIRONMENTAL SCIENCES Pub Date : 2025-08-13 DOI: 10.1016/j.coesh.2025.100655
Le Thi Lan Anh, Tran Le Luu
Greenhouse gas (GHG) emissions from wastewater treatment plants (WWTPs), including carbon dioxide (CO2), methane (CH4), and nitrous oxide (N2O), are significant contributors to global climate change. This study addresses the lack of data in Vietnam's fragmented and under-monitored wastewater systems by integrating field measurements, dynamic modeling, and life cycle assessment (LCA) to quantify GHG emissions from 29 centralized plants and multiple decentralized systems. The results indicate that CH4 and N2O emissions amount to 378 and 79.7 million tons of CO2-equivalent annually, with local emission factors significantly exceeding the IPCC Tier 1 defaults. Methane is primarily produced from anaerobic sludge digestion and septic tanks, while N2O arises from nitrogen removal processes under low dissolved oxygen (DO) conditions. Indirect CO2 emissions from electricity and fuel consumption contribute an additional 17 % to the sector's GHG footprint. Technologies such as Johkasou, Anammox, and biogas recovery demonstrate strong mitigation potential, with Johkasou reducing emissions by approximately 16 % and Anammox lowering N2O outputs. Additional solutions including photovoltaic (PV) systems, machine learning-based process optimization, and microbial fuel cells (MFCs) offer promising pathways for operational efficiency and long-term sustainability. These findings provide critical inputs for Vietnam's carbon market implementation and align with global efforts to improve the accuracy of GHG accounting in wastewater systems.
废水处理厂(WWTPs)排放的温室气体(GHG),包括二氧化碳(CO2)、甲烷(CH4)和氧化亚氮(N2O),是全球气候变化的重要贡献者。本研究通过整合现场测量、动态建模和生命周期评估(LCA)来量化29个集中式工厂和多个分散式系统的温室气体排放,解决了越南零散和监测不足的废水系统数据缺乏的问题。结果表明:年CH4和N2O排放量分别为3.78和7970万吨co2当量,当地排放因子显著超过IPCC一级违约值。甲烷主要由厌氧污泥消化和化粪池产生,而N2O则由低溶解氧(DO)条件下的脱氮过程产生。电力和燃料消耗产生的间接二氧化碳排放量占该行业温室气体足迹的17%。Johkasou、厌氧氨氧化和沼气回收等技术显示出强大的缓解潜力,Johkasou可减少约16%的排放量,而厌氧氨氧化可降低N2O的产量。其他解决方案包括光伏(PV)系统、基于机器学习的流程优化和微生物燃料电池(mfc),为提高运营效率和长期可持续性提供了有希望的途径。这些发现为越南的碳市场实施提供了重要的投入,并与全球提高废水系统温室气体核算准确性的努力保持一致。
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引用次数: 0
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