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Basin-scale spatio-temporal development of glacial lakes in the Hindukush-Karakoram-Himalayas 兴都库什-喀喇昆仑-喜马拉雅地区冰川湖泊的流域尺度时空演化
IF 4 1区 地球科学 Q1 GEOGRAPHY, PHYSICAL Pub Date : 2024-11-28 DOI: 10.1016/j.gloplacha.2024.104656
Atul Kumar , Suraj Mal , Udo Schickhoff , A.P. Dimri
Glacial lakes are expanding exponentially in the cryospheric environment of the Hindukush-Karakoram-Himalayas (HKH). Rapid glacier melting due to an above mean global annual temperature increase in HKH is attributed as the main reason for the expansion of the glacial lakes. The rapid expansion of glacial lakes increases the risk of future Glacial Lake Outburst Floods (GLOFs) events in the HKH.
In the present study, glacial lake inventories for the Indus, Ganga and Brahmaputra (IGB) river basins in the HKH were generated for 1990, 2000, 2010 and 2020 using Landsat (TM & OLI) at the sub-basin level to understand the spatio-temporal and regional patterns of glacial lakes dynamics, elevational evolution, and changes in the typology. We mapped 17,641 glacial lakes (area: 1082.57 ± 192.601 km2) in 1990, 18,206 (area: 1120.95 ± 198.49 km2) in 2000, 18,399 (area: 1147.12 ± 201.26 km2) in 2010, and 19,284 (area: 1191.81 ± 209.21 km2) in 2020. Between 1990 and 2020, IGB basins showed an increase of 9.31 % in total number and 10.09 % in total area of glacial lakes. In 2020, the Brahmaputra basin had the maximum total area (area: 763.59 ± 132.14 km2), followed by Indus basin (area: 217.47 ± 43.39 km2) and the Ganga basin (area: 210.74 ± 33.66 km2). However, between 1990 and 2020, glacial lakes in the Ganga basin (n: 22.08 %) had the highest growth rate, followed by the Indus basin (n: 14.73 %) and the Brahmaputra basin (n: 4.41 %). In 2020, 76.11 % of glacial lakes were end-moraine-dammed M(e) lakes, followed by other bedrock-dammed B(o) lakes (16.45 %), supraglacial lakes (2.79 %), lateral moraine-dammed M(l) lakes (2 %), cirque B(c) lakes (1.06 %), other moraine-dammed M(o) lakes (0.38 %), and other glacial (O) lakes (1.18 %). Given the rapid growth of glacial lakes in the region along with their likely flood volumes and damage potential in case of their failures, the present study will be of importance for disaster management authorities, an important input for detection of potentially hazardous glacial lakes and for development of mitigation strategies to minimize the impact of potential future GLOF events.
在兴都库什-喀喇昆仑-喜马拉雅山脉(HKH)的冰冻圈环境中,冰川湖泊呈指数级增长。由于全球年平均气温高于HKH而导致的冰川快速融化被认为是冰湖扩大的主要原因。冰湖的快速扩张增加了未来HKH冰湖溃决洪水(GLOFs)事件的风险。在本研究中,利用Landsat (TM &;OLI)在次流域水平上了解冰湖动态、海拔演变和类型变化的时空和区域格局。1990年绘制了17641个冰湖(面积:1082.57±192.601 km2), 2000年绘制了18206个(面积:1120.95±198.49 km2), 2010年绘制了18399个(面积:1147.12±201.26 km2), 2020年绘制了19284个(面积:1191.81±209.21 km2)。1990 ~ 2020年,IGB流域冰湖总数增加了9.31%,面积增加了10.09%。2020年,雅鲁藏布江流域面积最大(763.59±132.14 km2),其次是印度河流域(217.47±43.39 km2)和恒河流域(210.74±33.66 km2)。1990 - 2020年间,恒河流域的冰川湖泊增长率最高(22.08%),其次是印度河流域(14.73%)和雅鲁藏布江流域(4.41%)。2020年,终碛垄M(e)型冰湖占76.11%,其次为其他基岩坝B(o)型冰湖(16.45%)、冰上湖(2.79%)、侧碛垄M(l)型冰湖(2%)、环碛垄B(c)型冰湖(1.06%)、其他冰碛垄M(o)型冰湖(0.38%)、其他冰碛垄M(o)型冰湖(1.18%)。考虑到该地区冰川湖的迅速增长及其可能的洪水量和一旦冰川湖破裂可能造成的损害,本研究对灾害管理当局具有重要意义,是发现潜在危险冰川湖和制定缓解战略以尽量减少未来潜在冰川湖事件影响的重要投入。
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引用次数: 0
Zooplankton fecal pellet flux and carbon export: The South China Sea record and its global comparison 浮游动物粪便颗粒通量和碳输出:南海记录及其全球比较
IF 4 1区 地球科学 Q1 GEOGRAPHY, PHYSICAL Pub Date : 2024-11-26 DOI: 10.1016/j.gloplacha.2024.104657
Jiaying Li, Zhifei Liu, Baozhi Lin, Yulong Zhao, Xiaodong Zhang, Junyuan Cao, Jingwen Zhang, Hongzhe Song
Zooplankton fecal pellets constitute a major component of passively sinking particles in the ocean. The sinking of zooplankton fecal pellets provides an efficient vehicle for the transfer and sequestration of particulate organic carbon (POC) in the deep sea, which has been widely reported in different regions. However, most existing studies focus on the sinking flux of fecal pellets within the upper ocean, while lower mesopelagic and bathypelagic zones are rarely investigated. Here, we report the spatiotemporal flux variation of zooplankton fecal pellets collected by two sediment traps deployed in mesopelagic and bathypelagic zones (500 m and 2190 m, respectively) of the South China Sea from June 2020 to May 2022, and compare it with deep-sea (>500 m) fecal pellet flux data reported in the global ocean. In the South China Sea, fecal pellet fluxes display distinct seasonal patterns due to the control of the East Asian monsoon system, with higher fluxes in winter and spring, and lower fluxes in summer and autumn. Small fecal pellets (width < 100 μm) dominate the overall pellet numerical flux (more than 98 %), while rare large pellets (width > 100 μm) account for averaging 20 % of fecal pellet carbon flux. Both large and small pellet fluxes appear to be higher at 2190 m, mainly due to the in-situ reworking and repackaging of deep-dwelling zooplankton communities, as well as the input of lateral advection from high productive continental coasts and shelves. Identifiable zooplankton fecal pellets constitute approximately 10 % to the total POC flux in the deep South China Sea. Comparing the eutrophic polar and upwelling regions with mesotrophic and oligotrophic regions, we find a good correlation between marine primary production and fecal pellet carbon export. On the global scale, carbon fluxes through zooplankton fecal pellets to the deep sea are mainly constrained by the grazing impacts of zooplanktons, influenced by temperature, zooplankton biomass, and zooplankton size spectrum.
浮游动物粪便颗粒是海洋中被动下沉颗粒的主要组成部分。浮游动物粪便颗粒的下沉为深海颗粒有机碳(POC)的转移和封存提供了有效的载体,这在不同地区得到了广泛的报道。然而,现有的研究大多集中在上层海洋中粪便颗粒的下沉通量,而对下层中深海和深海区域的研究很少。本文报道了2020年6月至2022年5月在南海中远洋和深海(分别为500 m和2190 m)部署的两个沉积物捕集器收集的浮游动物粪便颗粒的时空通量变化,并与全球海洋中深海(>500 m)粪便颗粒通量数据进行了比较。在南海,由于东亚季风系统的控制,粪便颗粒通量表现出明显的季节特征,冬春季通量较高,夏秋季通量较低。小粪粒(宽度<;粒径为100 μm)的颗粒在整体数值通量中占主导地位(98%以上),而罕见的大颗粒(宽度>;100 μm)平均占粪便颗粒碳通量的20%。大颗粒通量和小颗粒通量在2190 m似乎都较高,这主要是由于深海浮游动物群落的原位改造和重新包装,以及来自高产大陆海岸和大陆架的侧向平流的输入。可识别的浮游动物粪便颗粒约占南海深海总POC通量的10%。将富营养区和上升流区与中营养区和少营养区进行比较,发现海洋初级生产与粪便颗粒碳输出具有良好的相关性。在全球尺度上,浮游动物粪球向深海的碳通量主要受浮游动物的放牧影响,受温度、浮游动物生物量和浮游动物粒径谱的影响。
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引用次数: 0
Microbe-forced Mn‑carbonate direct precipitation in Ediacaran micro-stromatolites of South China 中国南方埃迪卡拉系微叠层石的微生物强迫碳酸锰直接降水
IF 3.9 1区 地球科学 Q1 GEOGRAPHY, PHYSICAL Pub Date : 2024-11-26 DOI: 10.1016/j.gloplacha.2024.104658
Yi Zhang, Zhiwei Liao, Qin Huang, Gary G. Lash, Jian Cao, Bin Zhang
The direct precipitation model of Mn‑carbonate formation, based on investigation of the modern sedimentary record and simulation experiments, is commonly used to explain the genesis of both modern and ancient Mn‑carbonate deposits. This process is considered to be primarily influenced by physicochemical conditions and lacks microbial mediation. Despite the established role of microbes in global Mn cycling and biomineralization, the specific contribution of microbial processes to Mn‑carbonate formation remains understudied. In this study, Ediacaran Mn‑carbonates from South China with well-preserved micro-stromatolites offer a novel insight into understanding the microbes involved in the formation of Mn-deposits. Petrological observations reveal that the laminated Mn-ores mainly consist of alternating layers of dark Mn‑carbonate and light-colored dolomite laminae. Mn‑carbonate minerals, dominantly rod-like rhodochrosite crystals, exhibit a close spatial relationship with micro-stromatolites, suggesting a possible link to microbial activity. Geochemical results display that these Mn‑carbonates document high δ13C values (average = −1.65 ‰) compared to typical diagenetic Mn‑carbonate indicating the seawater likely contributed to the carbon source. Combined with alabandite deposition, small-sized pyrite framboids, and positive Eu anomalies, the Ediacaran Mn‑carbonates may have formed by microbially-mediated direct precipitation in Mn-rich anoxic seawater. The Mn‑carbonate and micro-stromatolite laminae accumulated during a period of enhanced bacterial activity, driven by episodic inputs of hydrothermal Mn2+ and bioessential elements. The present study highlights the microbially-mediated significant role in the primary precipitation pathway of Mn‑carbonate. Direct precipitation of Mn‑carbonate deposits, controlled by ocean conditions as well as enhanced by microbial processes, may account for the formation of other ancient economic manganiferous sedimentary deposits.
在现代沉积记录研究和模拟实验的基础上,碳酸锰形成的直接降水模式被广泛用于解释现代和古代碳酸锰矿床的成因。这一过程被认为主要受物理化学条件的影响,缺乏微生物的调解。尽管微生物在全球锰循环和生物矿化中的作用已经确立,但微生物过程对碳酸锰形成的具体贡献仍未得到充分研究。在这项研究中,来自中国南方的埃迪卡拉纪碳酸锰盐岩和保存完好的微叠层石为理解参与锰矿形成的微生物提供了新的见解。岩石学观察表明,层状锰矿主要由深色碳酸锰矿和浅色白云岩相间层状组成。锰碳酸盐矿物,主要是棒状红锰矿晶体,与微叠层石表现出密切的空间关系,表明可能与微生物活动有关。地球化学结果表明,与典型成岩型碳酸锰相比,这些碳酸锰具有较高的δ13C值(平均= - 1.65‰),表明海水可能是碳源的来源。结合藻绿岩沉积、小型黄铁矿树状体和正Eu异常,埃迪卡拉纪碳酸锰盐岩可能是由富锰缺氧海水中微生物介导的直接降水形成的。在热液Mn2+和生物必需元素的间歇性输入的驱动下,在细菌活动增强的时期,碳酸锰和微叠层石层沉积。本研究强调了微生物介导在碳酸锰初级沉淀途径中的重要作用。受海洋条件控制和微生物作用增强的碳酸锰矿床的直接降水可能是其他古代经济含锰矿床形成的原因。
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引用次数: 0
Nanoparticles of iridium and other platinum group elements identified in Chicxulub asteroid impact spherules – Implications for impact winter and profound climate change 在希克苏鲁伯小行星撞击球体中发现的铱纳米粒子和其他铂族元素-对撞击冬季和深刻气候变化的影响
IF 3.9 1区 地球科学 Q1 GEOGRAPHY, PHYSICAL Pub Date : 2024-11-26 DOI: 10.1016/j.gloplacha.2024.104659
Vivi Vajda, Susan Nehzati, Gavin Kenny, Hermann D. Bermúdez, Ashley Krüger, Alexander Björling, Adriana Ocampo, Ying Cui, Kajsa G.V. Sigfridsson Clauss
The Chicxulub asteroid that ended the Cretaceous Era ∼66.05 million years ago caused a prolonged time of global darkness – the impact winter – leading to mass extinctions. Elements from the asteroid, including the platinum group elements (PGEs) osmium, iridium and platinum are known from the globally distributed boundary clay but their carrier elements have so far been unknown. We identify, for the first time in detail, the presence of these PGEs within Chicxulub impact spherules and importantly, we identify their carrier elements. We show through synchrotron Nano-XRF how these PGEs occur in nanostructures as un-ordered cube- and/or needle-like crystals co-localizing with both siderophile and chalcophile elements including Co, Ni, Cu, Zn, and Pb, derived from the asteroid. These crystals are set within a matrix of iron-rich calcium and silica glass revealing the mix of vaporized target rock and the asteroid. The results provide insights into the combination of elements present in the spherules, indicating formation of new minerals. We argue that the nano-shards of unreactive elements such as platinum, iridium and copper acted as nuclei for aerosol formation and potentially contributed to a prolonged impact winter with darkness and cooling leading to a profound and long-term climate change.
大约6605万年前结束白垩纪的希克苏鲁伯小行星造成了长时间的全球黑暗-撞击冬季-导致大规模灭绝。小行星的元素,包括铂族元素(PGEs)锇、铱和铂,从全球分布的边界粘土中已知,但其载体元素迄今为止尚不清楚。我们首次在希克苏鲁伯撞击球体中详细确定了这些pge的存在,重要的是,我们确定了它们的载体元素。我们通过同步加速器纳米xrf展示了这些PGEs如何在纳米结构中以无序的立方体和/或针状晶体的形式与来自小行星的亲铁和亲铜元素(包括Co, Ni, Cu, Zn和Pb)共定位。这些晶体位于富含铁的钙和二氧化硅玻璃的基质中,揭示了蒸发的目标岩石和小行星的混合物。这些结果提供了对球粒中存在的元素组合的见解,表明了新矿物的形成。我们认为,铂、铱和铜等非活性元素的纳米碎片是气溶胶形成的核心,并可能导致冬季黑暗和寒冷的长期影响,从而导致深刻而长期的气候变化。
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引用次数: 0
Radium fingerprinting traces hydrology of the global cryosphere under climate warming 镭指纹追踪气候变暖下全球冰冻圈的水文情况
IF 4 1区 地球科学 Q1 GEOGRAPHY, PHYSICAL Pub Date : 2024-11-26 DOI: 10.1016/j.gloplacha.2024.104654
Zhe Zhang, Lixin Yi, Ruotong Li, Tianxue Lyu, Chenyi Liu, Yingchun Dong
Dynamic changes in the cryosphere have profound implications for global warming. This study, through case studies of seasonal ice lakes and glacier-originated rivers, complemented by global data, offers novel insights into radium (Ra) isotopes' characteristic in the cryosphere. It elucidates the quantification of the “Ra quartet” as tracers in frozen hydrological processes across various timescales. (1) Theoretical case studies. Significant differences in water chemistry and Ra activities were observed, highlighting distinct Ra supply and depletion mechanisms. The improved Ra mass model was utilized to estimate the freezing duration of the lakes and the groundwater discharge beneath the ice, while also elucidating the recharge dynamics of groundwater along glacial rivers. (2) Global scale theoretical discoveries. The low 224Ra/228Ra ratio, including the case studies presented, may be a significant characteristic of the non-subterranean cryosphere. This phenomenon can be attributed to various processes, including decay, particulate scavenging, groundwater discharge, upwelling, and glacial meltwater. In contrast, the ratio observed in permafrost is more complex, potentially influenced by diverse hydrogeological conditions and intricate sampling protocols. While Ra isotopes are well-traced in the ocean cryosphere—covering groundwater discharge, water exchange, and composition-particle interactions—their application in terrestrial and atmospheric cryospheric studies remains underexplored. Our study provides novel perspectives on Ra isotopes in the cryosphere, offering crucial theoretical and practical implications for addressing ongoing climate warming.
冰冻圈的动态变化对全球变暖有着深远的影响。本研究通过对季节性冰湖和冰川河流的案例研究,并辅以全球数据,对镭同位素在冰冻圈中的特性提出了新的见解。该研究阐明了 "镭同位素四重奏 "作为示踪剂在不同时间尺度的冰冻水文过程中的量化问题。(1) 理论案例研究。观察到水化学和 Ra 活性的显著差异,突出了不同的 Ra 供应和耗竭机制。利用改进的镭质量模型估算了湖泊的冻结时间和冰下地下水的排放量,同时还阐明了冰川河流沿岸地下水的补给动态。(2) 全球范围的理论发现。低 224Ra/228Ra 比率,包括所介绍的案例研究,可能是非地下冰冻圈的一个重要特征。这种现象可归因于各种过程,包括衰变、微粒清除、地下水排放、上涌和冰川融水。相比之下,在永久冻土层中观察到的比率更为复杂,可能受到不同水文地质条件和复杂采样方案的影响。虽然镭同位素在海洋冰冻圈中的应用范围很广,包括地下水排放、水交换以及成分与粒子之间的相互作用,但它们在陆地和大气冰冻圈研究中的应用仍未得到充分探索。我们的研究为冰冻圈中的镭同位素提供了新的视角,为解决当前气候变暖问题提供了重要的理论和实践意义。
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引用次数: 0
Late Cretaceous ecosystem dynamics in the southern incipient Arctic Ocean: A micropaleontological and geochemical perspective 初生北冰洋南部的晚白垩世生态系统动力学:微古生物学和地球化学视角
IF 4 1区 地球科学 Q1 GEOGRAPHY, PHYSICAL Pub Date : 2024-11-24 DOI: 10.1016/j.gloplacha.2024.104643
J.F. Diaz , L. Schwark , P.K. Pedersen , J.M. Galloway , M. Bringué , S.E. Grasby
Micropaleontological and geochemical analyses in samples from the Coniacian-Maastrichtian-aged Smoking Hills and Mason River formations in the Anderson Basin of the northern mainland coast of Arctic Canada provide a refined picture of the environmental conditions occurring in the incipient southern Arctic Ocean at the end of the Cretaceous. These units were deposited within a 22 myr time span in an outer shelf setting characterized by relatively stable tectonic conditions and low sedimentation rates. The Coniacian-middle Campanian Smoking Hills Formation was deposited during times of marine transgression and water column stratification. Surface waters were highly productive and dominated by dinoflagellates, red algae, green algae and likely diatoms and silicoflagellates. Bottom waters were predominantly anoxic-euxinic, but the presence of benthic foraminifera and variations of geochemical signatures in some intervals indicate episodic ventilation. The deposition of the Smoking Hills Formation is temporally consistent with the Oceanic Anoxic Event 3 (OAE3), but the duration of these anoxic conditions is much longer in the Anderson Basin. During the middle Campanian, relative sea level reached a highstand, fostering the expansion of planktic siliceous microorganisms, including diatoms, silicoflagellates and radiolarians. During the late Campanian to at least the Maastrichtian, sediments of the Mason River Formation were deposited during a regressive sedimentation phase characterized by high productivity fueled by river run-off and the proliferation of diatoms, red and green algae. Despite high productivity, bottom waters were oxygenated. This study highlights the importance of data integration to reconstruct the environmental conditions of the past as many, if not all, of the proxies utilized to this end are subjected to preservational and diagenetic bias.
对加拿大北冰洋北部大陆海岸安德森盆地科尼阿克纪-马斯特里赫特纪时期的吸烟山地层和梅森河地层样本进行的微古生物学和地球化学分析,提供了白垩纪末期北冰洋南部萌芽时期环境条件的精细图景。这些单元是在 22 百万年的时间跨度内沉积在外陆架环境中的,该环境的特点是构造条件相对稳定,沉积速率较低。康尼阿克纪--坎帕尼亚中期的烟丘地层沉积于海洋横断和水柱分层时期。表层水的生产力很高,主要是甲藻、红藻、绿藻,可能还有硅藻和硅鞭毛藻。底层水主要为缺氧-缺氧状态,但底栖有孔虫的存在和某些区间地球化学特征的变化表明存在偶发性通风。烟山地层的沉积在时间上与大洋缺氧事件 3(OAE3)一致,但在安德森盆地,这些缺氧条件的持续时间要长得多。在中元古代,相对海平面达到高位,促进了硅藻、硅鞭毛虫和放射虫等浮游硅质微生物的繁殖。在钟乳期晚期至至少马斯特里赫特期,梅森河地层的沉积物沉积在一个回归沉积阶段,其特点是河流径流和硅藻、红藻和绿藻的大量繁殖促进了高生产力。尽管生产力很高,但底层水含氧量很低。这项研究强调了数据整合对于重建过去环境条件的重要性,因为许多(如果不是全部)用于重建环境条件的代用指标都会受到保存和成岩偏差的影响。
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引用次数: 0
Molybdenum isotopic evidence for linked changes in North Pacific Intermediate Water and subtropical Northwest Pacific redox conditions over the last 200 k.y 过去 200 千年北太平洋中层水和西北太平洋亚热带氧化还原条件关联变化的钼同位素证据
IF 4 1区 地球科学 Q1 GEOGRAPHY, PHYSICAL Pub Date : 2024-11-23 DOI: 10.1016/j.gloplacha.2024.104637
Yanguang Dou , Chenghui Sun , Shouye Yang , Xuefa Shi , Yonghua Wu , Jingyi Cong , Yong Zhang , Fengmei Wang , Feng Cai , Peter D. Clift
Through biological productivity and ocean-atmosphere CO2 exchange, North Pacific mid-depth ventilation has the potential to regulate regional climate over glacial timescales. Nevertheless, the subtropical Northwest Pacific currently lacks continuous long redox records that would enable us to evaluate this process. In this instance, we present δ98/95Mo and redox-sensitive trace element data derived from Okinawa Trough sediments to reconstruct redox conditions and assess their possible significance in regulating atmospheric CO2 in the subtropical Northwest Pacific over the last 200 k.y. Enhanced oxic conditions induced by a strengthened Kuroshio Current during Marine Isotope Stage (MIS) 1 suggest the presence of enhanced deep water ventilation and upwelling in the Okinawa Trough, which likely contributed to high atmospheric CO2 concentrations during interglacial periods. The Okinawa Trough may have been oxic and served as a regional net carbon sink during MIS2 and MIS6, due to glacial North Pacific Intermediate Water (GNPIW) and a weak Kuroshio Current. During interglacials, high productivity brought on by the stronger East Asian Summer Monsoon (EASM) leads to an increase in organic matter burial and oxygen consumption. This substantial positive excursion in δ98/95Mo values during MIS4 and early MIS3 can be linked to the anaerobic oxidation of methane (AOM) and the release of methane-rich fluids from methane hydrate decomposition. Our findings highlight potential links between higher upwelling, GNPIW expansion, and the underlying processes regulating the atmospheric CO2 budget in the subtropical North Pacific during the late Quaternary.
通过生物生产力和海洋-大气二氧化碳交换,北太平洋中深层通风有可能在冰川时间尺度上调节区域气候。然而,西北太平洋亚热带地区目前缺乏连续的长氧化还原记录,因此我们无法对这一过程进行评估。在本研究中,我们展示了冲绳海槽沉积物中提取的δ98/95Mo和氧化还原敏感痕量元素数据,以重建氧化还原条件,并评估其在过去200 k.y.中调节西北太平洋亚热带大气CO2的可能意义。在海洋同位素阶段(MIS)1,黑潮的增强导致氧化条件增强,这表明冲绳海槽存在增强的深水通风和上涌,这很可能导致间冰期大气二氧化碳浓度升高。在 MIS2 和 MIS6 期间,由于冰川期北太平洋中间水(GNPIW)和黑潮的减弱,冲绳海槽可能一直处于缺氧状态,并成为区域净碳汇。在间冰期,较强的东亚夏季季风(EASM)带来的高生产力导致有机物埋藏量和耗氧量增加。在 MIS4 和 MIS3 早期,δ98/95Mo 值的大幅正向偏移可能与甲烷的厌氧氧化(AOM)以及甲烷水合物分解释放的富甲烷流体有关。我们的研究结果突显了第四纪晚期北太平洋亚热带地区较高的上升流、GNPIW扩张和调节大气二氧化碳预算的基本过程之间的潜在联系。
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引用次数: 0
Possible influence of low latitude wetland area changes on the Holocene global atmospheric methane concentration trend 低纬度湿地面积变化对全新世全球大气甲烷浓度趋势的可能影响
IF 4 1区 地球科学 Q1 GEOGRAPHY, PHYSICAL Pub Date : 2024-11-23 DOI: 10.1016/j.gloplacha.2024.104655
Yunping Song , Hai Xu , Kevin M. Yeager
Understanding the causes of variations in global atmospheric methane concentration (GAMC) is an important issue in the study of global climatic changes. Long-term GAMC varied rhythmically on glacial-interglacial timescales, and broadly followed the orbital/suborbital cycles in northern hemisphere solar insolation. Yet the late Holocene has witnessed an increasing GAMC trend since the mid-Holocene, which decouples with the global atmospheric CO2 concentration trend and the northern hemisphere solar insolation trend. The causes of this decoupling have been extensively studied, but remain highly debated. Here we show that the Holocene GAMC trend closely follows the long-term trend in global low latitude wetland extent as inferred from our lake-level reconstruction and from other existing hydroclimate records. We contend that changes in low latitude wetland extent play an important role in shaping the GAMC trend. We propose that reduced low latitude wetland areas during the mid-Holocene, which were likely due to the submersion of tropical wetlands by rising sea levels, and reduced low latitude wetland areas inferred from lower lake levels, could be responsible for the observed mid-Holocene GAMC drop. Increasing global low latitude wetland areas during the late Holocene are likely responsible for the contemporary increasing GAMC trend.
了解全球大气甲烷浓度(GAMC)变化的原因是研究全球气候变化的一个重要问题。在冰川-间冰期的时间尺度上,全球大气甲烷浓度的长期变化是有节奏的,并且大致跟随北半球太阳日照的轨道/亚轨道周期。然而,自全新世中期以来,全新世晚期的 GAMC 呈上升趋势,与全球大气二氧化碳浓度趋势和北半球太阳日照趋势脱钩。这种脱钩的原因已被广泛研究,但仍存在很大争议。在这里,我们展示了全新世 GAMC 趋势与全球低纬度湿地范围的长期趋势密切相关,这是从我们的湖泊水位重建和其他现有的水文气候记录中推断出来的。我们认为,低纬度湿地范围的变化在形成 GAMC 趋势方面发挥了重要作用。我们认为,全新世中期低纬度湿地面积的减少(可能是由于海平面上升淹没了热带湿地),以及根据较低的湖泊水位推断出的低纬度湿地面积的减少,可能是观测到的全新世中期全球平均海平面上升率下降的原因。全新世晚期全球低纬度湿地面积的增加可能是当代全球平均海平面上升趋势的原因。
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引用次数: 0
Iron isotope fractionation during granite weathering under different climates 不同气候条件下花岗岩风化过程中的铁同位素分馏
IF 4 1区 地球科学 Q1 GEOGRAPHY, PHYSICAL Pub Date : 2024-11-22 DOI: 10.1016/j.gloplacha.2024.104653
Meng Qi , Chengshuai Liu , Ting Gao , Zhengrong Wang , Yuhui Liu , Yafei Xia
Climate controls chemical weathering of silicate rocks on the transport of iron (Fe) and its isotopes from continent to the ocean, impacting the global Fe geochemical cycle. However, it's elusive if Fe isotope fractionation during silicate weathering reflects variations in climate factors. This study examines two granite-derived regolith profiles; one in Beijing (BJ), representing a temperate climate, and the other in Guangdong (GD), representing a tropical climate, to investigate their mineralogy, Fe-bearing phases, element concentrations, and Fe isotope compositions. Our results show that, despite climate differences, the two granite weathering profiles have average δ56Febulk regolith values within analytical uncertainty (0.09 ± 0.02 ‰ vs. 0.12 ± 0.04 ‰, 2SD). The δ56Febulk regolith values of temperate and tropical regolith are similar to or slightly higher than those of their respective bedrocks and remain steady along the entire weathering profile. The limited variation of Fe isotope composition in weakly weathered temperate regolith likely reflects the dissolution of primary minerals rather than the formation of secondary minerals. The Rayleigh fractionation calculations also show a Δ56Fepore solution-regolith value of ∼0 ‰ between pore solution and regolith. In contrast, in the tropical profile, despite the abundance of secondary minerals and the differences in δ56Fe values among the extracted Fe-pools exceeding 0.68 ‰, only limited Fe isotope fractionation is observed in the bulk regolith (0.01 ‰ to 0.24 ‰). These variations are likely driven by the formation of Fe oxides, relying on the atomic distribution of Fe in hematite and goethite. The linear regression analysis estimates the apparent Fe isotope fractionation factor between hematite and goethite as 0.46 ± 0.07 ‰ (Δ56Fehematite-goethite, 1SE). These findings indicate that the sensitivity of Fe isotope fractionation in bulk regolith to variations in climate factors is relatively limited. However, combined with results from other weathering profiles in different climate zones, two models suggest that changes in δ56Fe values of easily leachable and silicate-bound Fe pools are likely influenced by climate factors such as temperature and precipitation. This work advances our understanding of the Fe isotope fractionation during silicate weathering and its potential climate connection on Earth's surface.
气候控制着硅酸盐岩的化学风化,影响着铁(Fe)及其同位素从大陆向海洋的迁移,从而影响着全球铁地球化学循环。然而,硅酸盐风化过程中铁同位素的分馏是否反映了气候因素的变化,目前还难以确定。本研究考察了两个花岗岩来源的碎屑岩剖面,一个位于代表温带气候的北京(BJ),另一个位于代表热带气候的广东(GD),研究它们的矿物学、含铁矿相、元素浓度和铁同位素组成。结果表明,尽管气候不同,但两个花岗岩风化剖面的平均δ56Febulk回归岩值在分析不确定性范围内(0.09 ± 0.02 ‰ vs. 0.12 ± 0.04 ‰,2SD)。温带和热带沉积岩的δ56Febulk值与各自基岩的值相近或略高于基岩,并在整个风化剖面上保持稳定。弱风化温带碎屑岩中铁同位素组成的有限变化可能反映了原生矿物质的溶解而非次生矿物质的形成。瑞利分馏计算还显示,孔隙溶液和风化沉积物之间的Δ56F孔隙溶液-风化沉积物值为0‰。与此相反,在热带剖面中,尽管次生矿物丰富,提取的Fe-pools之间的δ56Fe值差异超过0.68 ‰,但在大块团岩中只观察到有限的Fe同位素分馏(0.01 ‰至0.24 ‰)。这些变化可能是由铁氧化物的形成驱动的,依赖于赤铁矿和鹅铁矿中铁的原子分布。线性回归分析估计赤铁矿和鹅铁矿之间的表观铁同位素分馏系数为 0.46 ± 0.07 ‰(Δ56Fehematite-鹅铁矿,1SE)。这些研究结果表明,块状沉积物中铁同位素分馏对气候因子变化的敏感性相对有限。然而,结合不同气候带其他风化剖面的结果,两个模型表明,易浸出和硅酸盐结合铁池中δ56Fe值的变化很可能受到温度和降水等气候因素的影响。这项研究加深了我们对硅酸盐风化过程中铁同位素分馏及其与地球表面潜在气候联系的理解。
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引用次数: 0
Impact of ENSO on extreme precipitation in Southwest Asia 厄尔尼诺/南方涛动对西南亚极端降水的影响
IF 4 1区 地球科学 Q1 GEOGRAPHY, PHYSICAL Pub Date : 2024-11-22 DOI: 10.1016/j.gloplacha.2024.104645
Omid Alizadeh , Morteza Mousavizadeh
The El Niño-Southern Oscillation (ENSO) is a primary driver of interannual variability in extreme precipitation in many regions worldwide. Understanding the relationship between ENSO and extreme precipitation is crucial, as it has implications for understanding the interannual variability of flood risk. We investigated the frequency of extreme daily precipitation in Southwest Asia across different seasons during El Niño and La Niña using the daily GPCP and ERA5 precipitation datasets for the period 1997–2022. Extreme precipitation at each grid point is defined as daily accumulated precipitation exceeding the 95th percentile on wet days, where a wet day is defined as one with at least 0.1 mm rainfall. El Niño is associated with an overall increase in the frequency of extreme precipitation in Southwest Asia during autumn, winter, and spring, whereas La Niña shows the opposite effect. To explore the dynamics of El Niño and La Niña teleconnections to Southwest Asia, we applied a feature tracking method on the ERA5 relative velocity at 850 hPa in different seasons. Overall, the storm track density and the mean intensity of storms increase in Southwest Asia during El Niño and decrease during La Niña in autumn, winter, and spring. In summer, El Niño favors less frequent extreme precipitation in the southern parts of Southwest Asia, where the tropical summer monsoon circulation is dominated, while La Niña is associated with more frequent extreme precipitation in this region. This pattern is expected, as the monsoon circulation is weaker during El Niño and stronger during La Niña. In line with this, we identified a decrease in the mean intensity of storms in the southern parts of Southwest Asia during El Niño, with the opposite occuring during La Niña. Our findings have important implications for understanding interannual variability of extreme precipitation in Southwest Asia and providing a framework for predicting such events.
厄尔尼诺-南方涛动(ENSO)是全球许多地区极端降水量年际变化的主要驱动因素。了解厄尔尼诺/南方涛动与极端降水之间的关系至关重要,因为这对了解洪水风险的年际变化具有重要意义。我们利用 1997-2022 年期间的 GPCP 和 ERA5 日降水数据集,研究了厄尔尼诺和拉尼娜现象期间西南亚不同季节的极端日降水频率。每个网格点的极端降水量定义为湿润日累计降水量超过第 95 百分位数,其中湿润日定义为降水量至少为 0.1 毫米的一天。厄尔尼诺现象与西南亚秋、冬、春季极端降水频率的整体增加有关,而拉尼娜现象则显示出相反的影响。为了探索厄尔尼诺和拉尼娜对西南亚遥联系的动态变化,我们对不同季节ERA5 850 hPa相对速度采用了特征跟踪方法。总体而言,在秋季、冬季和春季,厄尔尼诺期间西南亚的风暴径迹密度和风暴平均强度增加,而拉尼娜期间则减少。在夏季,厄尔尼诺现象有利于西南亚南部地区较少出现极端降水,因为那里主要是热带夏季季风环流,而拉尼娜现象则与该地区较频繁的极端降水有关。这种模式是预料之中的,因为在厄尔尼诺期间季风环流较弱,而在拉尼娜期间季风环流较强。与此相一致,我们发现在厄尔尼诺现象期间,西南亚南部地区风暴的平均强度有所下降,而在拉尼娜现象期间则相反。我们的研究结果对于了解西南亚极端降水的年际变化和提供预测此类事件的框架具有重要意义。
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引用次数: 0
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